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At least 235 records · Page 13

Quantum Choreography of the Nucleus: Rotations, Vibrations, and Emergent Structure

Abstract Nuclei are complex many-body quantum systems where interactions of the neutrons and protons via the strong, the weak, and the electromagnetic forces lead to the emergence of simple patterns of energy states that have been described by various theoretical approaches. One of the goals of all the theoretical models is the development of a universal theory that can be applied across the entire chart of nuclides. Significant progress has been made by experiments as well as the increasing sophistication of models, but a universal theory has yet to be established. A recent review of nuclei in the Z = 50–82 region of the chart of nuclides has analyzed all the available compiled data from several decades of studies towards a clarification of the low-lying structure of nuclei. Other reviews have reported and explained the emergence of multiple different shapes in nuclei at somewhat higher excitation energies than the ground state. Some have challenged the interpretation of the first excited K π = 0 + band as a vibration of ground state. This work attempts to provide a guide to determining the nature of the first excited K π = 0 + band in nuclei by the combined use of nuclear lifetimes, energy level evolutions, dynamic moments of inertia, and intrinsic quadrupole moments extracted from transition probabilities. The result is that for a subset of the nuclei in this region, the K π = 0 + band is consistent with the traditional 𝛽-vibration description of an oscillation built on the ground state.

CHFB+5DCH↗

Collective Neutrino Oscillations and Heavy-element Nucleosynthesis in Supernovae: Exploring Potential Effects of Many-body Neutrino Correlations

In high-energy astrophysical processes involving compact objects, such as core-collapse supernovae or binary neutron star mergers, neutrinos play an important role in the synthesis of nuclides. Neutrinos in these environments can experience collective flavor oscillations driven by neutrino–neutrino interactions, including coherent forward scattering and incoherent (collisional) effects. Recently, there has been interest in exploring potential novel behaviors in collective oscillations of neutrinos by going beyond the one-particle effective or "mean-field" treatments. Here, we seek to explore implications of collective neutrino oscillations, in the mean-field treatment and beyond, for the nucleosynthesis yields in supernova environments with different astrophysical conditions and neutrino inputs. We find that collective oscillations can impact the operation of the νp-process and r-process nucleosynthesis in supernovae. The potential impact is particularly strong in high-entropy, proton-rich conditions, where we find that neutrino interactions can nudge an initial νp-process neutron-rich, resulting in a unique combination of proton-rich low-mass nuclei as well as neutron-rich high-mass nuclei. We describe this neutrino-induced neutron-capture process as the "νi-process." In addition, nontrivial quantum correlations among neutrinos, if present significantly, could lead to different nuclide yields compared to the corresponding mean-field oscillation treatments, by virtue of modifying the evolution of the relevant one-body neutrino observables.

79 ASTRONOMY AND ASTROPHYSICS↗

Short communication: Mechanism and prevention of irreversible trapping of atmospheric He during mineral crushing

A pervasive challenge in noble gas geochemistry is to ensure that analytical techniques do not modify the composition of the noble gases in the samples. Noble gases are present in the atmosphere and are used in a number of manufacturing procedures and by laboratory equipment. Of particular concern is the introduction of atmospheric or laboratory noble gases to samples during preparation before samples are placed in a vacuum chamber for analysis. Recent work has shown the potential for contamination of crushed samples with air-derived He that is not released by placing the samples under vacuum at room temperature. Using pure He gas as a tracer, we show that the act of crushing samples to a fine powder itself can introduce He contamination but that this is easily avoided by crushing under liquid or in an inert atmosphere. Because the He is trapped during crushing, the same concern does not extend to samples that are naturally fine-grained when collected. We also show model results that demonstrate when this effect might significantly impact samples for (U–Th) / He geochronology or 3 He cosmogenic nuclide dating. The degree of He contamination from crushing samples to sizes smaller than the > 63 µm range typically used for geochronology is insignificant for samples with a date of at least 1 Ma and 1 ppm U, and the degree of He contamination from crushing samples to sizes smaller than the 100–500 µm range typically used for cosmogenic nuclide dating is also insignificant for samples with a date of at least 10 ka with typical 3 He production rates.

58 GEOSCIENCES↗

Technical note: 21 Ne in the CoQtz-N quartz standard material

Intercomparison standards produced from mineral samples exposed to the natural cosmic ray flux are routinely used for interlaboratory comparison and normalization of measurements of the cosmogenic noble gases 3 He and 21 Ne. This effort is facilitated by the availability of multiple standard materials with a wide range of cosmogenic nuclide concentrations. The “CoQtz-N” quartz standard, which was originally produced and distributed as an intercomparison standard for cosmogenic 10 Be and 26 Al, has a significantly lower cosmogenic nuclide concentration than other mineral standards used for cosmogenic noble gas analysis and is therefore potentially useful for assessing the linearity of interlaboratory offsets across a wide range of concentrations. This paper reports 21 Ne analysis of 13 aliquots of CoQtz-N, interspersed with 14 aliquots of the commonly used CRONUS-A quartz standard, in three analytical sessions on two noble gas mass spectrometer systems. The excess 21 Ne concentration in CoQtz-N, normalized to the accepted value of 320 × 10 6 atoms g −1 for CRONUS-A, is 13.87 ± 0.24 × 10 6 atoms g −1 . Alternatively, the ratio of excess 21 Ne concentrations in CoQtz-N and CRONUS-A is 0.04330 ± 0.00077.

Balco, Greg [Lawrence Livermore National Laborator↗

Nuclear Data Impact on Key Metrics for a Representative Molten Chloride Fast Reactor Model

Nuclear data are an essential component of the foundation on which all modeling and simulation methods and tools are relying upon, from the front end to the back end of the nuclear fuel cycle. In this study, the impact of uncertainties in nuclear data is investigated for a representative molten chloride fast reactor, for several important metrics, including eigenvalue, reactivity differences, and nuclide inventories in fuel at 5-yr irradiation. Uncertainty of keff for a full core model was found to be similar between the fresh fuel and the irradiated fuel states (1.7-1.8%), with its primary driver being the uncertainty in the 235U (n,γ) cross section. The results obtained for the reactivity differences show large uncertainties, of over 100%, in elastic scattering sensitivities of several nuclides, which led to large uncertainties of temperature reactivity differences for cladding and reflector. These results provide evidence that the currently applied methods may not be sufficiently adequate for ensuring the reliable determination of such metrics.

Procop, Germina [ORNL] (ORCID:0000000342226393)↗

Measurement of cosmic ray produced Mn-53 in deep sea metallic spherules

Cosmic ray originated Mn-53 nuclides were measured in deep sea metallic spherules by neutron activation analysis. The spherules may be fused micrometeoroids or ablation droplets from larger objects; the low activities of Mn-53 may indicate its evaporation loss resulting from the heating in the earth's atmosphere or short exposure age. The Mn-53 nuclide is now being measured in chondritic spherules, and Be-10 and Cl-36 concentrations are determined in individual spherules using ion counting methods.

Nishiizumi, K.↗

Solar-system abundances of the elements

Elemental analyses of the Ogueil Cl meteorite and all previous Cl chondrite analyses were employed to develop a new solar system abundance table, including the standard deviation and number of analyses for each element. The table also comprises the abundances of radioactive and radiogenic nuclides at the present and 4.55 AE ago, as well as abundances by weight in a typical Cl chondrite. The new abundances were within 20% of those determined by Cameron (1982), except for 14 cases in the range 20-50%, and 5 over 50%. The solar abundances were compared with the Cl abundances, showing a total of only 7 disagreements. No significant discrepancies were detected in the major cosmochemical groups, and a smooth trend was found in the abundances of odd-A nuclides. The new set is interpreted as accurate to 10%, with the Cl chondrites matching the primordial solar system abundances to at most 10% deviation.

Anders, E.↗

Terrestrial and exposure histories of Antarctic meteorites

Records of cosmogenic effects were studied in a large suite of Antarctic meteorites. The cosmogenic nuclide measurements together with cosmic ray track measurements on Antartic meteorites provide information such as exposure age, terrestrial age, size and depth in meteoroid or parent body, influx rate in the past, and pairing. The terrestrail age is the time period between the fall of the meteorite on the Earth and the present. To define terrestrial age, two or more nuclides with different half-lives and possibly noble gases are required. The cosmogenic radionuclides used are C-14, Kr-81, Cl-36, Al-26, Be-10, Mn-53, and K-40.

Nishiizumi, K.↗

Cosmogenic rare gases and 10-Be in a cross section of Knyahinya

The concentrations of cosmogenic nuclides were studied as a function of shielding on samples from a cross section of the 293 kg main fragment of the L5 chondrite Knyahinya. The stone broke into two nearly symmetrical parts upon its fall in 1866. The planar cross section has diameters between 40 and 55 cm. He, Ne, and Ar were measured on about 20 samples by mass spectrometry and the 10-Be activities on aliquots of 10 selected samples were determined by AMS. The 10-Be data are presented and the abundances of spallogenic nuclides are compared with the model calculations reported by Reedy for spherical L chondrites. The 10-Be production rates in Knyahinya are shown versus the shielding parameter 22-Ne/21-Ne.

Wieler, R.↗

Nucleogenic noble gas components in the Cape York iron meteorite

The paper reports data on neutron capture products of the secondary cosmic ray component, the inferred proton and neutron fluences, and the identification of double beta decay of Se-82 in heavily shielded samples of the Cape York iron meteorite. One purpose of this study is to develop a new chronometer for cosmic ray exposure, based on the nuclides I-129 (16 My half-life) and Xe-129 from low energy cosmic ray reactions on Te. The abundance ratio of these two nuclides permits the determination of an (effective) exposure age of 93 + or - 16 My, which represents the first exposure age datum of Cape York. The very small concentrations of spallogenic Ar-38 = 6.5 x 10 to the -10th cu cm STP/g in the metal and troilite (per g Fe) document the heavily shielded locations of the sample. An excess of Xe-129 in the troilite is shown to be entirely due to the decay of cosmic-ray-produced I-129. On the other hand, an inclusion in the troilite reveals the presence of Xe-129 from extinct I-129 and documents its about 4.5 Gy formation age. Mono-isotopic excess of Kr-82 is identified as due to beta-beta-decay of Se-82 with an inferred half-life of 1.0 x 10 to the 20th y. This represents the first beta-beta-decay product observed in a meteorite.

Murty, S. V. S.↗

Al-26 and Be-10 production in iron meteorites

To compare the Al-26/Ne-21 ages with K-40/K-41 ages, the contents of Al-26 were determined in seven iron meteorites using accelerator mass spectrometry and the light noble gas contents were determined using conventional mass spectrometry, for samples for which these values were not available. In addition, contents of Be-10 were measured. Due to the presence of boron in the samples, the values of Al-26 were found to be at least 30 percent lower than the literature values obtained by low-level counting techniques, while the Be-10 values were 10-15 percent lower. The production rates of these nuclides at different He-4/Ne-21 ratios were estimated, showing that the increase in He-4/Ne-21 ratios corresponded with decreases in Al-26 and Be-10. It was shown that the exposure ages calculated from the Ne-21/Al-26 ratio cannot be calibrated so as to agree with both the K-40/K-41 ages and ages based on the shorter-lived nuclides Ar-39 and Cl-36.

Aylmer, D.↗

Solar-system abundances and processes of nucleosynthesis

The origin of the elements is studied. The average elemental composition of the solar system is examined and used to infer the primordial solar system abundances of the individual nuclides. Patterns in these nuclide abundances are used as clues to their origin. The possible cosmic significance of the patterns are considered. The astrophysical settings for nucleosynthesis and the chemical evolution of the Galaxy and information based on observed isotopic anomalies in meteorites are taken into account.

Woolum, Dorothy S.↗

Surface activation of Concorde by Be-7

Activation analysis of two airframe parts from Concorde aircraft has identified the presence of Be-7, a nuclide which was found by other investigators to have been collected on the forward edge of the Long Duration Exposure Facility (LDEF) structure. The results of the Concorde analysis indicate that this phenomenon is very much a surface effect, and that the areal densities of the Be-7 are comparable to those found for LDEF. The collection of Be-7 by the aircraft must be greater than in the case of LDEF (since the duration for which Concorde is accumulating the nuclide is shorter) and is of the order of 1.9 to 40 nuclei sq cm/s, depending upon assumptions made regarding the efficiency of the process which removes the radionuclide.

Truscott, P. R.↗

Determination of the half-life of Ca-41 from measurements of Antarctic meteorites

Accelerator mass spectrometry is utilized to determine the half-life of Ca-41 from the decrease of its concentration with terrestrial age in five Antarctic meteorites and a recent fall. The meteorites were selected on the basis of their Cl-36 concentrations, which showed a span of terrestrial ages of about 600 ka, and on the basis of other cosmogenic nuclide concentrations which indicated that the meteorites had small preatmospheric sizes, and sufficiently long irradiation times in space that the concentrations of Ca-41 and Cl-36 were in secular equilibrium prior to the meteorites' fall to earth. The half-life of Ca-41 is determined at 103 + or - 7 ka. Topics discussed include the effects of undersaturation (short exposure time in space), shielding (the samples are from the interior of a large meteorite), and weathering on the cosmogenic nuclide concentrations in meteorites.

Klein, Jeffrey↗

Surface activation of Concorde by Be-7

Activation analysis of two airframe components from the Concorde aircraft has identified the presence of Be-7, a nuclide found by other investigators that was deposited on the forward edge of the Long Duration Exposure Facility (LDEF) structure. The results of the Concorde analysis indicate that this phenomenon is very much a surface effect, and that the areal densities of the Be-7 are comparable to those found for LDEF. The collection of Be-7 by the aircraft must be greater than in the case of LDEF (since duration for which Concorde is accumulating the nuclide is shorter) and is of the order of 1.2 to 41 nuclei/sq cm(-)s(exp -1) depending upon assumptions made regarding the altitude at which collection becomes appreciable, and the efficiency of the process which removes the radionuclide.

Truscott, P. R.↗

Cosmogenic-radionuclide profiles in Knyahinya: New measurements and models

Cosmic-ray-produced nuclides measured in samples taken from known locations on a big slab of the large (R approximately equals to 45 cm) L5-chondrite Knyahinya provide good depth-vs-concentration profiles to develop and test models for the production of cosmogenic nuclides in meteorites. We report new profiles for Be-10, Al-26, Cl-36 in metallic and non-magnetic phases of 8 documented samples from Knyahinya and for C-14 in bulk samples from 7 Knyahinya samples. These new measured profiles are very similar to profiles calculated with particle fluxes from the LAHET Monte Carlo production and transport code system and with cross sections for major reactions.

Reedy, R. C.↗

The isotopic composition of iron-group galactic cosmic rays

Results from studies of the isotopic composition of iron group elements in the galactic cosmic radiation are reviewed, emphasizing recently reported measurements from the ISEE-3 spacecraft. The observed isotope distributions for the elements Ti through Mn are in good agreement with those expected for a propagated solar-like source composition, with the possible exception of an enhanced abundance of Ti-50. It is found that a significant fraction of the radioactive secondary nuclide Mn-54 has decayed, indicating a confinement time of iron group cosmic rays in the galaxy of at least 2 Myr. The source ratio Fe-54/Fe-56 is found to be consistent with the solar value, but the ratio Ni-60/Ni-58 is greater than solar by a factor of 2.8+/-1.0. The measured abundance of Co-59 is significantly greater than the calculated secondary contribution, suggesting that this nuclide has been produced in the source regions by the electron capture decay of Ni-59 and implying a time delay between nucleosynthesis and acceleration approximately greater than 10(exp 5) yr.

Wiedenbeck, M. E.↗

Earth and Planetary Science Letters

Systematic measurements of the concentrations of cosmogen Ca-41 (half-life = 1.04 x 10(exp 5) yr) in the Apollo 15 long core 15001-15006 were performed by accelerator mass spectroscopy. Earlier measurements of cosmogenic Be-10, C-14, Al-26, Cl-36, and Mn-53 in the same core have provided confirmation and improvement of theoretical models for predicting production profiles of nuclides by cosmic ray induced spallation in the Moon and large meteorites. Unlike these nuclides, Ca-40 in the lunar surface is produced mainly by thermal neutron capture reactions on Ca-40. The maximum production of Ca-41, about 1 dpm/g Ca, was observed at a depth in the Moon of about 150 g/sq cm. For depths below about 300 g/sq cm, Ca-41 production falls off exponentially with an e-folding length of 175 g/sq cm. Neutron production in the Moon was modeled with the Los Alamos High Energy Transport Code System, and yields of nuclei produced by low-energy thermal and epithermal neutrons were calculated with the Monte Carlo N-Particle code. The new theoretical calculations using these codes are in good agreement with our measured Ca-41 concentrations as well as with Co-60 and direct neutron fluence measurements in the Moon.

K. Nishiizumi↗