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At least 235 records · Page 13

An airborne lidar system for ozone and aerosol profiling in the troposphere and lower stratosphere

A description is presented of an airborne UV optical radar (lidar) system, taking into account also the first range-resolved ozone measurements from an aircraft using the differential absorption lidar (Dial) technique. The discussed system is the first to use an aircraft platform for ozone profile measurements. The Dial technique determines the average gas concentration over some selected range interval. The airborne Dial system uses two high conversion efficiency dye lasers which are optically pumped by two frequency-doubled Nd:YAG lasers. The first remote measurements of ozone profiles with an airborne Dial system were made during flight tests between May 22 and June 6, 1980. The UV Dial system was operated at a nominal altitude of 3.2 km. Initial measurements of ozone and aerosol profiles with the Dial system were performed on 4 flights in the vicinity of the Chesapeake Bay.

Browell, E. V.↗

Backscattered UV radiation - Effects of multiple scattering and the lower boundary of the atmosphere

A method is proposed for the calculation of a multiple-scattering correction to the single-scattering calculation of the radiance of the terrestrial atmosphere resulting from backscattered ultraviolet solar radiation in the spectral region used in the ozone profile inversion. This method uses jointly the usual analytical and Monte Carlo methods. Effects of the lower boundary of the atmosphere, cloud tops, and ground surface are investigated both qualitatively and quantitatively. The ratio of multiple to single scattering is determined, and its importance in ozone profile inversion of backscattered UV solar radiation from the terrestrial atmosphere is evaluated. The polarization of the atmospheric radiance is treated briefly.

Aruga, T.↗

Airborne Lidar measurements of aerosols, mixed layer heights, and ozone during the 1980 PEPE/NEROS summer field experiment

A detailed summary of the NASA Ultraviolet Differential Absorption Lidar (UV DIAL) data archive obtained during the EPA Persistent Elevated Pollution Episode/Northeast Regional Oxidant Study (PEPE/NEROS) Summer Field Experiment Program (July through August 1980) is presented. The UV dial data set consists of remote measurements of mixed layer heights, aerosol backscatter cross sections, and sequential ozone profiles taken during 14 long-range flights onboard the NASA Wallops Flight Center Electra aircraft. These data are presented in graphic and tabular form, and they have been submitted to the PEPE/NEROS data archive on digital magnetic tape. The derivation of mixing heights and ozone profiles from UV Dial signals is discussed, and detailed intercomparisons with measurements obtained by in situ sensors are presented.

Browell, E. V.↗

A study of satellite remote measurements of stratospheric aerosol and gas parameters using the solar occultation technique

Satellite remote measurements of stratospheric aerosol and ozone profiles using the solar occultation approach were analyzed based on the known properties of the atmospheric parameters. Atmospheric refraction effects which are important in this experiment were determined analytically. Different inversion techniques were developed based on inverting simulated irradiance data. It was shown that aerosol and ozone profiles in the stratosphere can be inverted from the irradiance measurements to an accuracy of better than 10 percent.

Chu, W. P.↗

Determination of vertical ozone distributions by spacecraft measurements using a limb-scan technique

The principle of a new inversion technique which uses multiple wavelength-solar UV radiation satellite measurements for determining vertical ozone profiles is described, and examples of computer simulations for 280, 300, 320, and 340 nm are discussed. Weighting functions corresponding to the sensitivity of the limb radiance to the relative ozone density at each altitude are the basis for the inversion equation, which is then solved by an iteration technique. The use of multiple wavelengths can provide more information of higher accuracy over a wider height range than those profiles recovered at a single wavelength. It is indicated that an effective range of altitude of approximately 20-70 km with a vertical resolution of 1-2 km is feasible for determining ozone profiles with an inferred profile error about three to four times larger than the measurement error within that altitude region. Ozone profile accuracy of the highest altitude region may be improved using wavelengths down to 260 nm, and inferred ozone profiles above 70 km are possible, but with a larger error.

Aruga, T.↗

A New Raman DIAL Technique for Measuring Stratospheric Ozone in the Presence of Volcanic Aerosols

This paper describes a new lidar scheme to measure stratospheric ozone in the presence of heavy volcanic aerosol loading. The eruptions of the Philippine volcano Pinatubo during June 1991 ejected large amounts of sulfur dioxide into the atmosphere to altitudes of at least 30 km. The resulting aerosols have severely affected the measurements of stratospheric ozone when using traditional Rayleigh differential absorption lidar (DIAL) technique, in which the scattering mechanism is almost entirely Rayleigh and which assumes a small amount or no aerosols. In order to extract an ozone profile in the regions below about 30 km where the Rayleigh lidar returns are contaminated by aerosol scattering from Mt. Pinatubo cloud, we have used a Raman lidar technique, where the scattering mechanism depends solely on molecular nitrogen. In this scheme there is no aerosol scattering component to the backscattered lidar return. Using this technique in conjunction with the Rayleigh DIAL measurement, the GSFC stratospheric ozone lidar has measured ozone profiles between 15 and 50 km during the recently held UARS correlative measurement campaign (February-March 1992) at JPL's Table Mountain Facility in California.

Upendra N. Singh↗

Tropospheric Ozone Climatology over Irene, South Africa, From 1990-1994 and 1998-2002

This paper describes ozone profiles from sonde data during the period of NASA s TRACE-A and the more recent SHADOZ (Southern Hemisphere Additional Ozonesondes) period. The data were taken by the South African Weather Service at the Irene (25 deg.54 min S; 28 deg. 13 min. E) station near Pretoria, South Africa, an area that is a unique mixture of local industry, heavy biofuels use and importation of biomass burning ozone from neighboring countries to the north. The main findings are: (1) With its geographical position at the edge of the subtropical transition zone, mid- latitude dynamical influences are evident at Irene, predominantly in winter when upper tropospheric ozone is enhanced as a result of stratospheric-tropospheric exchange. (2) There has been an increase in the near-surface ozone amount between the early 1990s and a decade later, presumably due to an influx of rural population toward the Johannesburg-Pretoria area, as well as with industrial growth and development. (3) Most significant for developing approaches for satellite ozone profile climatologies, cluster analysis has enabled the delineation of a background and "most polluted" profile. Enhancements of at least 30% occur throughout the troposphere in spring and in certain layers increases of 100 % are observed.

Diab, R. D.↗

Estimation of Smoothing Error in SBUV Profile and Total Ozone Retrieval

Data from the Nimbus-4, Nimbus-7 Solar Backscatter Ultra Violet (SBUV) and seven of the NOAA series of SBUV/2 instruments spanning 41 years are being reprocessed using V8.6 algorithm. The data are scheduled to be released by the end of August 2011. An important focus of the new algorithm is to estimate various sources of errors in the SBUV profiles and total ozone retrievals. We discuss here the smoothing errors that describe the components of the profile variability that the SBUV observing system can not measure. The SBUV(/2) instruments have a vertical resolution of 5 km in the middle stratosphere, decreasing to 8 to 10 km below the ozone peak and above 0.5 hPa. To estimate the smoothing effect of the SBUV algorithm, the actual statistics of the fine vertical structure of ozone profiles must be known. The covariance matrix of the ensemble of measured ozone profiles with the high vertical resolution would be a formal representation of the actual ozone variability. We merged the MLS (version 3) and sonde ozone profiles to calculate the covariance matrix, which in general case, for single profile retrieval, might be a function of the latitude and month. Using the averaging kernels of the SBUV(/2) measurements and calculated total covariance matrix one can estimate the smoothing errors for the SBUV ozone profiles. A method to estimate the smoothing effect of the SBUV algorithm is described and the covariance matrixes and averaging kernels are provided along with the SBUV(/2) ozone profiles. The magnitude of the smoothing error varies with altitude, latitude, season and solar zenith angle. The analysis of the smoothing errors, based on the SBUV(/2) monthly zonal mean time series, shows that the largest smoothing errors were detected in the troposphere and might be as large as 15-20% and rapidly decrease with the altitude. In the stratosphere above 40 hPa the smoothing errors are less than 5% and between 10 and 1 hPa the smoothing errors are on the order of 1%. We validate our estimated smoothing errors by comparing the SBUV ozone profiles with other ozone profiling sensors.

Kramarova, N. A.↗

Assessment and Applications of NASA Ozone Data Products Derived from Aura OMI-MLS Satellite Measurements in Context of the GMI Chemical Transport Model

Measurements from the Ozone Monitoring Instrument (OMI) and Microwave Limb Sounder (MLS), both onboard the Aura spacecraft, have been used to produce daily global maps of column and profile ozone since August 2004. Here we compare and evaluate three strategies to obtain daily maps of tropospheric and stratospheric ozone from OMI and MLS measurements: trajectory mapping, direct profile retrieval, and data assimilation. Evaluation is based upon an assessment that includes validation using ozonesondes and comparisons with the Global Modeling Initiative (GMI) chemical transport model (CTM). We investigate applications of the three ozone data products from near-decadal and inter-annual timescales to day-to-day case studies. Zonally averaged inter-annual changes in tropospheric ozone from all of the products in any latitude range are of the order 1-2 Dobson Units while changes (increases) over the 8-year Aura record investigated http://eospso.gsfc.nasa.gov/atbd-category/49 vary approximately 2-4 Dobson Units. It is demonstrated that all of the ozone products can measure and monitor exceptional tropospheric ozone events including major forest fire and pollution transport events. Stratospheric ozone during the Aura record has several anomalous inter-annual events including stratospheric warming split events in the Northern Hemisphere extra-tropics that are well captured using the data assimilation ozone profile product. Data assimilation with continuous daily global coverage and vertical ozone profile information is the best of the three strategies at generating a global tropospheric and stratospheric ozone product for science applications.

GMI↗

Systematic stratospheric observations on the Antarctic continent at Dumont d'Urville

Results of different routine measurements performed in Dumont d'Urville (66 deg S, 140 deg E) since 1988 are presented. They include the seasonal variation of total ozone and NO2 as measured by a SAOZ UV-Visible spectrometer, Polar Stratospheric Cloud observations by a backscatter lidar and more recently, vertical ozone profiles by ECC sondes and ozone and aerosols stratospheric profiles by a DIAL lidar. The particular results of 1991 in relation with the volcanic events of Mount Pinatubo and Mount Hudson, and the position of the polar vortex over Dumont d'Urville are discussed.

Godin, S.↗

Impact of Surface Emissions to the Zonal Variability of Tropical Tropospheric Ozone and Carbon Monoxide for November 2004

The chemical and dynamical processes governing the zonal variability of tropical tropospheric ozone and carbon monoxide are investigated for November 2004 using satellite observations, in-situ measurements, and chemical transport models in conjunction with inverse-estimated surface emissions. Vertical ozone profile estimates from the Tropospheric Emission Spectrometer (TES) and ozone sonde measurements from the Southern Hemisphere Additional Ozonesondes (SHADOZ) network show the so called zonal 'wave-one' pattern, which is characterized by peak ozone concentrations (70-80 ppb) centered over the Atlantic, as well as elevated concentrations of ozone over Indonesia and Australia (60-70 ppb) in the lower troposphere. Observational evidence from TES CO vertical profiles and Ozone Monitoring Instrument (OMI) NO2 columns point to regional surface emissions as an important contributor to the elevated ozone over Indonesia. This contribution is investigated with the GEOS-Chem chemistry and transport model using surface emission estimates derived from an optimal inverse model, which was constrained by TES and Measurements Of Pollution In The Troposphere (MOPITT) CO profiles (Jones et al., 2007). These a posteriori estimates, which were over a factor of 2 greater than climatological emissions, reduced differences between GEOS-Chem and TES ozone observations by 30-40% and led to changes in GEOS-Chem upper tropospheric ozone of up to 40% over Indonesia. The remaining residual differences can be explained in part by upper tropospheric ozone produced from lightning NOx in the South Atlantic. Furthermore, model simulations from GEOS-Chem indicate that ozone over Indonesian/Australian is more sensitive to changes in surface emissions of NOx than ozone over the tropical Atlantic.

tropical tropospheric ozone↗

An analysis of the 7-year record of SBUV satellite ozone data - Global profile features and trends in total ozone

Results are presented from an analysis of Nimbus 7 SBUV monthly-average total ozone data for the November 1978 - September 1985 period. Linear drifts are estimated for the differences between SBUV and Dobson ground station total ozone data. The results show an average negative linear drift in SBUV data relative to Dobson data of about -0.4 percent per year. The global estimate of the relation between total ozone and solar flux variations is 0.97 + or - 0.61/100 solar flux units, representing a change of total ozone over the 7-year period associated with solar flux variations of about -0.20 + or - 0.13 percent per year.

Reinsel, Gregory C.↗

Cloud, dust, and ozone vertical profiles from solar occultation measurements: Implications for dynamics

An instrument was designed for solar occultation measurements of the martian atmosphere from the Phobos spacecraft. It was composed of three different dispersive systems working in the ultraviolet (UV: 0.22-0.32 microns) for the measurement of O3 and aerosols, in the near infrared (NIR: 0.76 microns, 0.94 microns) for the detection of O2 and H2O, and in the infrared (IR: 1.9 microns, 3.7 microns) where CO2 and H2O were measured. A detailed description of the instrument may be found in the special issue of Nature. Its principle objective is to measure from the Phobos orbit the spectrum of the Sun, modified by atmospheric extinction, during sunset. The UV-NIR spot has an angular diameter of 1 arcmin, or approximately 3 km vertical resolution, and is located near the center of the solar disk. The IR field is about twice as large and its line of sight is shifted by 8.5 arcmin, or approximately 20 km, relative to the previous one. It is therefore located near the edge of the solar disk. Sampling times are generally 0.5, 1, and 2 s for IR, UV, and NIR channels respectively, corresponding to vertical excursions of the line of sight of 1, 2, and 4 km respectively under nominal conditions. The instrument operated from February 8 to March 26 (the martian equinox occurred on February 17). The latitude of the intersection of the Sun-spacecraft axis with the surface of Mars varied from -11 to +20, the seasonal date L(sub s) being in the range 0 - 20. All measurements were therefore made near northern spring equinox in equatorial regions. Due to an error in the pointing system, only partial results were obtained, the region below approximately equals 30 km altitude being never sounded by the UV-NIR spectrometer. On the contrary, nine complete occultations were obtained in the IR channels, whose line of sight was fortunately approximately equals 20 km below the UV-NIR axis.

Chassefiere, E.↗

Total Ozone from the Ozone Monitoring System (OMI) using TOMS and DOAS Methods

The Ozone Monitoring Instrument (OMI) is the Dutch-Finnish contribution to NASA's EOS-Aura satellite scheduled for launch in January 2004. OMI is an imaging spectrometer that will measure the back-scattered Solar radiance in the wavelength range of 270 to 500 nm. The instrument provides near global coverage in one day with a spatial resolution of 13x24 square kilometers. OMI is a new instrument, with a heritage from TOMS, SBW, GOME, GOMOS and SCIAMACHY. OMI'S unique capabilities for measuring important trace gases and aerosols with a small footprint and daily global coverage, in conjunction with the other Aura instruments, will make a major contribution to our understanding of stratospheric and tropospheric chemistry and climate change. OMI will provide data continuity with the 23-year ozone record of TOMS. There are three ozone products planned for OMI: total column ozone, ozone profile and tropospheric column ozone. We are developing two different algorithms for total column ozone: one similar to the algorithm currently being used to process the TOMS data, and the other an improved version of the differential optical absorption spectroscopy (DOAS) method, which has been applied to GOME and SCIAMACHY data. The main reasons for starting with two algorithms for total ozone have to do with heritage and past experience; our long-term goal is to combine the two to develop a more accurate and reliable total ozone product for OMI. We will compare the performance of these two algorithms by applying both of them to the GOME data. We will examine where and how the results differ, and use the extensive TOMS-Dobson comparison studies to assess the performance of the DOAS algorithm.

Veefkind, J. P.↗

Discoveries about Tropospheric Ozone Pollution from Satellite and Soundings

We have been producing near-red time tropospheric ozone satellite maps from the TOMS (Total Ozone Mapping Spectrometer) sensor since 1997. Maps for 1996-2000 for the operational Earth-Probe instrument are at: . Pollution in the tropics is influenced by biomass burning and by transport patterns that favor recirculation and in other cases reflect climate variability like the El-Nino-Southern Oscillation [Thompson et al., 2001]. The satellite view of chemical-dynamical interactions in tropospheric ozone is not adequate to capture vertical gradients in pollution. Thus, in 1998, NASA's Goddard Space Flight Center and a team of international sponsors established the SHADOZ (Southern Hemisphere ADditional OZonesondes) project to address the gap in tropical ozone soundings. SHADOZ augments launches and provides a public archive of ozonesonde data from twelve tropical stations at http://croc.gsfc.nasa.gov/shadoz. Further insights into the role of chemical and dynamical influences have emerged from the first 4-5 years of SHADOZ data (more than 2000 ozone profiles). Highly variable tropospheric ozone and a zonal wave-one pattern in tropospheric ozone suggest that dynamics is as important as pollution in determining tropical ozone distributions.

Thompson, Anne M.↗

Major Upgrades to the AIRS Version-6 Water Vapor Profile Methodology

This research is a continuation of part of what was shown at the last AIRS Science Team Meeting and the AIRS 2015 NetMeeting. AIRS Version 6 was finalized in late 2012 and is now operational. Version 6 contained many significant improvements in retrieval methodology compared to Version 5. Version 6 retrieval methodology used for the water vapor profile q(p) and ozone profile O3(p) retrievals is basically unchanged from Version 5, or even from Version 4. Subsequent research has made significant improvements in both water vapor and O3 profiles compared to Version 6.

Version-6↗