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At least 235 records · Page 13
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Effect of Surface Ionic Screening on Polarization Reversal and Phase Diagrams in Thin Antiferroelectric Films for Information and Energy Storage

Emergent behaviors in antiferroelectric thin films due to a coupling between surface electrochemistry and intrinsic polar instabilities are explored within the framework of the modified 2-4-6 Landau-Ginzburg-Devonshire (LGD) thermodynamic approach. By using phenomenological parameters of the LGD potential for a bulk antiferroelectric and a Stephenson-Highland (SH) approach, we study the role of surface ions with a charge density proportional to the relative partial oxygen pressure on the dipole states and their reversal mechanisms in antiferroelectric thin films. The combined LGDSH approach allows the boundaries of antiferroelectric, ferroelectriclike antiferroionic, and electretlike paraelectric states as a function of temperature, oxygen pressure, surface-ion formation energy and concentration, and film thickness to be delineated. This approach also allows the characterization of the polar and antipolar orderings dependence on the voltage applied to the antiferroelectric film, as well as the analysis of their static and dynamic hysteresis loops. Furthermore, the applications of the antiferroelectric films covered with a surface-ion layer for energy and information storage are explored and discussed.

25 ENERGY STORAGE↗
NASA NTRS2021

Boundary Layer Instabilities Over a Cone-Cylinder-Flare Model at Mach 6

Computations are performed to investigate the boundary-layer instabilities over a sharp cone-cylinder-flare model at zero degrees angle of attack. The model geometry and the flow conditions are selected to match the experiments conducted in the Boeing/AFOSR Mach 6 Quiet Tunnel (BAM6QT) at Purdue University. The geometry consists of a nominally sharp 5-degree half-angle cone, followed by a cylindrical segment and then a 10-degree flare. An axisymmetric separation bubble is generated as a result of the laminar shock/boundary-layer interaction in the cylinder-flare region. The comparison of the laminar flow solution and the schlieren images shows a remarkable agreement between the respective locations of both the boundarylayer edge and the reattachment shock. The predicted heat flux distribution is also in agreement with the measured values downstream of the reattachment location. The analysis of convective and global instabilities is performed for flare half angles equal to 8, 10, and 12 degrees and nosetip radii equal to 0.1, 1, and 5 mm. The linear amplification of first and second Mack mode instabilities that begin to amplify in the cone region are computed with a combination of the parabolized stability equations (PSE) and the harmonic linearized Navier-Stokes equations (HLNSE). The predicted frequency spectra of the surface pressure fluctuations associated with both planar and oblique instability waves are compared with the measured spectra at the various locations of the PCB and Kulite sensors. The comparison shows that the computational analysis captures the distinct lobes within the disturbance amplification spectra measured in the experiments, but some differences in amplification characteristics are noted at low frequencies. Overall, the oblique disturbances are found to be more amplified than the planar disturbances. To our knowledge, this represents the first successful comparison between convective instability analysis and measured surface pressure fluctuations for a hypersonic configuration with a separation bubble. Finally, the global instability analysis shows that the laminar flow becomes supercritical for flare half angles larger than 8 degrees. The unstable global mode for the experimental configuration of a 10 degrees flare and a sharp nosetip cone corresponds to a stationary three-dimensional disturbance that is concentrated in the recirculation region and achieves its maximum growth rate for an azimuthal wavenumber of 5.

Boundary layer transition↗
NASA NTRS2022

Boundary Layer Instabilities Over a Cone-Cylinder-Flare Model at Mach 6

Computations are performed to investigate the boundary-layer instabilities over a sharp cone-cylinder-flare model at zero degrees angle of attack. The model geometry and the flow conditions are selected to match the experiments conducted in the Boeing/AFOSR Mach 6 Quiet Tunnel (BAM6QT) at Purdue University. The geometry consists of a nominally sharp 5-degree half-angle cone, followed by a cylindrical segment and then a 10-degree flare. An axisymmetric separation bubble is generated as a result of the laminar shock/boundary-layer interaction in the cylinder-flare region. The comparison of the laminar flow solution and the schlieren images shows a remarkable agreement between the respective locations of both the boundarylayer edge and the reattachment shock. The predicted heat flux distribution is also in agreement with the measured values downstream of the reattachment location. The analysis of convective and global instabilities is performed for flare half angles equal to 8, 10, and 12 degrees and nosetip radii equal to 0.1, 1, and 5 mm. The linear amplification of first and second Mack mode instabilities that begin to amplify in the cone region are computed with a combination of the parabolized stability equations (PSE) and the harmonic linearized Navier-Stokes equations (HLNSE). The predicted frequency spectra of the surface pressure fluctuations associated with both planar and oblique instability waves are compared with the measured spectra at the various locations of the PCB and Kulite sensors. The comparison shows that the computational analysis captures the distinct lobes within the disturbance amplification spectra measured in the experiments, but some differences in amplification characteristics are noted at low frequencies. Overall, the oblique disturbances are found to be more amplified than the planar disturbances. To our knowledge, this represents the first successful comparison between convective instability analysis and measured surface pressure fluctuations for a hypersonic configuration with a separation bubble. Finally, the global instability analysis shows that the laminar flow becomes supercritical for flare half angles larger than 8 degrees. The unstable global mode for the experimental configuration of a 10 degrees flare and a sharp nosetip cone corresponds to a stationary three-dimensional disturbance that is concentrated in the recirculation region and achieves its maximum growth rate for an azimuthal wavenumber of 5.

Hydrodynamic instability↗
NASA NTRS2019

Effect of 3D Roughness Patch on Instability Amplification in a Supersonic Boundary Layer

Surface roughness is known to have a substantial impact on the aerothermodynamic loading of high-speed vehicles, particularly via its influence on the laminar-turbulent transition process within the boundary layer. Numerical simulations are performed to investigate the effects of a distributed region of densely packed, sinusoidal shape roughness elements on a Mach 3.5 flat plate boundary layer for flow conditions corresponding to the planned conditions of an upcoming experiment in the Mach 3.5 Supersonic Low Disturbance Tunnel at the NASA Langley Research Center. Analysis of convective instabilities in the wake of the roughness patch was reported in a previous paper and the current work extends that analysis to instability amplification across the length of the roughness patch. Quasi-parallel stability analysis of the modified boundary layer flow over the patch indicates two dominant families of unstable disturbances, namely, a group of high frequency modes that amplify in localized regions along the roughness patch and another group of low frequency modes that have smaller peak amplification rates but amplify steadily both above the roughness patch and in the wake region behind it. The results suggest that the amplification factors associated with the high-frequency modes are sufficiently low, at least for the roughness patches considered in this paper, so that these modes are unlikely to have a major influence on the transition process. The amplification of the low-frequency modes within the region of the roughness patch is further quantified via direct numerical simulations. Results confirm the strongly destabilizing influence of the roughness patch on the first mode instabilities, yielding an N-factor increment of ΔN ≈ 3.6 for a roughness patch length of eight wavelengths.

Laminar turbulent transition↗
NASA NTRS1998

Hydrodynamic Instability in an Extended Landau/Levich Model of Liquid-Propellant Combustion

The classical Landau/Levich models of liquid propellant combustion, which serve as seminal examples of hydrodynamic instability in reactive systems, have been combined and extended to account for a dynamic dependence, absent in the original formulations, of the local burning rate on the local pressure and/or temperature fields. The resulting model admits an extremely rich variety of both hydrodynamic and reactive/diffusive instabilities that can be analyzed in various limiting parameter regimes. In the present work, a formal asymptotic analysis, based on the realistic smallness of the gas-to-liquid density ratio, is developed to investigate the combined effects of gravity, surface tension and viscosity on the hydrodynamic instability of the propagating liquid/gas interface. In particular, a composite asymptotic expression, spanning three distinguished wavenumber regimes, is derived for both cellular and pulsating hydrodynamic neutral stability boundaries A(sub p)(k), where A(sub p) is the pressure sensitivity of the burning rate and k is the disturbance wavenumber. For the case of cellular (Landau) instability, the results demonstrate explicitly the stabilizing effect of gravity on long-wave disturbances, the stabilizing effect of viscosity and surface tension on short-wave perturbations, and the instability associated with intermediate wavenumbers for critical negative values of A(sub p). In the limiting case of weak gravity, it is shown that cellular hydrodynamic instability in this context is a long-wave instability phenomenon, whereas at normal gravity, this instability is first manifested through O(l) wavenumber disturbances. It is also demonstrated that, in the large wavenumber regime, surface tension and both liquid and gas viscosity all produce comparable stabilizing effects in the large-wavenumber regime, thereby providing significant modifications to previous analyses of Landau instability in which one or more of these effects were neglected. In contrast, the pulsating hydrodynamic stability boundary is found to be insensitive to gravitational and surface-tension effects, but is more sensitive to the effects of liquid viscosity, which is a significant stabilizing effect for O(l) and higher wavenumbers. Liquid-propellant combustion is predicted to be stable (i.e., steady and planar) only for a range of negative pressure sensitivities that lie between the two types of hydrodynamic stability boundaries.

Margolis, Stephen B.↗
NASA NTRS1999

Electric Field Induced Interfacial Instabilities

The study of the interface in a charge-free, critical and near-critical binary fluid in the presence of an externally applied electric field is presented. At sufficiently large fields, the interface between the two phases of the binary fluid should become unstable and exhibit an undulation with a predefined wavelength on the order of the capillary length. As the critical point is approached, this wavelength is reduced, potentially approaching length-scales such as the correlation length or critical nucleation radius. At this point the critical properties of the system may be affected. In this paper, the flat interface of a marginally polar binary fluid mixture is stressed by a perpendicular alternating electric field and the resulting instability is characterized by the critical electric field E(sub c) and the pattern observed. The character of the surface dynamics at the onset of instability is found to be strongly dependent on the frequency f of the field applied. The plot of E(sub c) vs. f for a fixed temperature shows a sigmoidal shape, whose low and high frequency limits are well described by a power-law relationship, E(sub c) = epsilon(exp zeta) with zeta = 0.35 and zeta = 0.08, respectively. The low-limit exponent compares well with the value zeta = 4 for a system of conducting and non-conducting fluids. On the other hand, the high-limit exponent coincides with what was first predicted by Onuki. The instability manifests itself as the conducting phase penetrates the non-conducting phase. As the frequency increases, the shape of the pattern changes from an array of bifurcating strings to an array of column-like (or rod-like) protrusions, each of which spans the space between the plane interface and one of the electrodes. For an extremely high frequency, the disturbance quickly grows into a parabolic cone pointing toward the upper plate. As a result, the interface itself changes its shape from that of a plane to that of a high sloping pyramid.

Kusner, Robert E.↗
NASA NTRS1992

Surface heat transfer and flow properties of vortex arrays induced artificially and from centrifugal instabilities

The paper presents and compares fluid-flow and heat transfer properties from artificially induced vortices in a flat-plate turbulent boundary layer and naturally occurring vortices due to centrifugal instabilities in a curved-channel laminar flow. Pairs and arrays of vortices are artificially induced by placing half-delta wings on the plate surface. With both arrays and pairs of vortices, streamwise velocities and total pressures are high, and surface heat transfer is locally augmented in vortex downwash regions. In contrast to vortices in the arrays vortices in the pairs tend to move in the streamwise direction with significant divergence (when the common flow between pair is toward the wall) or convergence (when the common flow between pair is away from the wall). The vortices in the arrays cause maximum peak-to-peak heat transfer variations of up to 12 percent of local spanwise-averaged values for initial vortex spacings between 1 to 2.5 generator heights.

Subramanian, C. S.↗
NASA NTRS1999

Ground-Based Experiments on Vibrational Thermal Convection

Ground-based experiments on g-jitter effects in fluid flow provide insight that complements both theoretical studies and space-based experiments on this problem. We report preliminary results for experiments on Rayleigh-Benard convection subjected to time-dependent accelerations on a shaker table. For sinusoidal modulation, two qualitatively different pattern forming mechanisms come into play: geometry induced wavenumber selection (as in the standard "no-shake" Rayleigh-Benard problem) and dispersion induced wavenumber selection due to parametric instability (as in the Faraday surface-wave problem). We discuss preliminary results on the competition and co-existence of patterns due to these different instability mechanisms. We also discuss the implications of this work on the general question of pattern formation in the presence of noise.

Schatz, Michael F.↗
DOE OSTI2023

The Linkage Between Electro-Chemical Mechanical Instabilities in Battery Materials

Battery chemistry must be diversified to achieve a sustainable energy landscape by effectively utilizing renewable energy sources. Alkali metal-ion, all-solid-state, metal–air batteries, and multivalent batteries offer unique cost, safety, raw material abundance, energy, and power density solutions. However, realizing these “beyond Li-ion batteries” must uncover their working principles and performance & property relationships. In this aspect, mitigating chemo-mechanical instabilities in the structure and surface of the electrodes plays a crucial role in their performance. Unfortunately, the coupling between electrochemical and mechanical interactions is often poorly understood due to a lack of operando characterization. Here, this review article explains the working principles of curvature measurement and digital image correlation for measuring stress and strain generations in battery materials. We provided specific examples of how these operando mechanical measurements shed light on instabilities in alkali metal ion electrodes, solid electrolytes, Li-O 2 batteries, and aqueous Zn-ion batteries. Operando mechanical measurements offer an effective way to map changes in the physical fingerprint of the battery materials, therefore providing crucial information to elucidate instabilities in battery materials.

25 ENERGY STORAGE↗
NASA NTRS2022

Winds at the Mars 2020 Landing Site: 1. Near-Surface Wind Patterns at Jezero Crater

This is the first part of a two-part paper. NASA's Mars 2020 Perseverance rover measured winds on the Jezero crater floor close to the delta of an ancient river. A mostly repeatable diurnal cycle was observed and presented two regimes: (a) a convective regime, from dawn to sunset, with average easterly to southeasterly winds, during which maximum wind speeds were measured, and (b) a nighttime regime with westerly-northwesterly winds followed by a relatively calm period with highly variable wind directions as a function of sol and time of night. The timing and magnitude of the observed regimes are consistent with primary control by regional and local slope flows. Data suggest that the surface circulation at Jezero region in northern spring and summer is highly unaffected by large-scale circulation except during particular periods in the diurnal cycle or generally during dust storms, which is supported by MarsWRF model simulations. Consequently, the observed seasonal variability was weak. However, sol-to-sol and seasonal variability were measured, most of it during certain nighttime periods. Traveling waves consistent with baroclinic instability were clearly observed in surface winds at L_s ∼ 75°. The early MY36/2022A regional dust storm at L_s ∼ 153° disturbed the wind patterns with changes suggesting enhanced tidal flows. After sunset, the dust storm also produced detectable gravity wave activity, increasing the mixing in the nighttime planetary boundary layer during storm conditions. Inferred wind directions from dust devil movies strongly suggest that prevailing winds continued to be slope-driven during the late summer, fall and early winter seasons.

D. Viúdez-Moreiras↗
DOE OSTI2026

A point-particle-based hydride shell-shedding model for ejecta particle transport in reactive environments

A shock wave passing over a rough or perturbed metal surface will induce a limiting case of Richtmyer–Meshkov instability and will cause small particles to eject from the surface and transport into the surrounding medium. These particles are known as ejecta and can be either solid or liquid in nature. Recent experiments have shown that liquid cerium ejecta clouds exhibit unexpected non-monotonic acceleration behaviors as well as temperature plateaus after a brief temperature rise if they are transporting in a chemically reactive, hydrogen-based medium while they act as expected in an inert medium. This work details a point-particle model developed for reactive cerium ejecta transport, which attempts to account for these new physics through the behavior of a developing solid hydride shell, which is believed to form as a product of the reaction. The overall model incorporates the effects of the reaction on the particle properties as well as the effects of potential shedding of the shell into sub-micrometer scale flakes and potential phase change of the hydride if the ejecta particles reach the melt point of the hydride layer. The model is tested by performing simulations of the original motivating experiments and comparing quantities, such as ejected mass, velocimetry, and temperature profiles, against the experimental data. While the model is able to capture many general features of the observed anomalies, some inaccuracies still exist. These point to both missing physics in the model (such as a deuterium adsorption mechanism on the hydride layer) as well as a lack of knowledge of certain material properties (such as the strength of cerium hydride to determine dynamic fracture thicknesses) needed to fully reduce the uncertainties in the model by up to an order of magnitude and perform a true attempt at model validation.

97 MATHEMATICS AND COMPUTING↗
NASA NTRS1992

Cooling of the magma ocean due to accretional disruption of the surface insulating layer

Planetary accretion has been considered as a process to heat planets. Some fraction of the kinetic energy of incoming planetesimals is trapped to heat the planetary interior (Kaula, 1979; Davies, 1984). Moreover, blanketing effect of a primary atmosphere (Hayashi et al., 1979; Sasaki, 1990) or a degassed atmosphere (Abe and Matsui, 1986; Zahnle et al., 1988) would raise the surface temperature of the Earth-size planets to be higher than the melting temperature. The primordial magma ocean was likely to be formed during accretion of terrestrial planets. In the magma ocean, if crystallized fractions were heavier than melt, they would sink. But if solidified materials were lighter than the melt (like anorthosite of the lunar early crust) they would float to form a solid shell surrounding the planet. (In an icy satellite, solidified water ice should easily float on liquid water because of its small density.) The surface solid lid would prevent efficient convective heat transfer and slow the interior cooling. Consider that the accretion of planetesimals still continues in this cooling stage. Shock disruption at planetesimal impact events may destroy the solid insulating layer. Even if the layer survives impacts, the surface layer is finally overturned by Rayleigh-Taylor instability, since accreting materials containing metals are heavier than the surface solidified lid of silicates.

Sasaki, Sho↗
DOE OSTI2023

Ballistic Ejection of Microdroplets from Overpacked Interfacial Assemblies

Spontaneous emulsification, resulting from the assembly and accumulation of surfactants at liquid–liquid interfaces, is an interfacial instability where microdroplets are generated and diffusively spread from the interface until complete emulsification. Here, it is shown that an external magnetic field can modulate the assembly of paramagnetic nanoparticle surfactants (NPSs) at liquid–liquid interfaces to trigger an oversaturation in the areal density of the NPSs at the interface, as evidenced by a marked reduction in the interfacial tension, γ, and corroborated with a magnetostatic continuum theory. Despite the significant reduction in γ, the presence of the magnetic field does not cause stable interfaces to become unstable. Upon rapid removal of the field, however, an explosive ejection of a plume of microdroplets from the surface occurs, a dynamical interfacial instability which is termed explosive emulsification. Further, this explosive event rapidly reduces the areal density of the NPSs to its pre-field level, stabilizing the interface. The ability to externally suppress or trigger the explosive emulsification and controlled generation of tens of thousands of microdroplets, uncovers an efficient energy storage and release process, that has potential applications for controlled and directed delivery of chemicals and remotely controlled soft microrobots, taking advantage of the ferromagnetic nature of the microdroplets.

36 MATERIALS SCIENCE↗
NASA NTRS2011

System and method for determining stability of a neural system

Disclosed are methods, systems, and computer-readable media for determining stability of a neural system. The method includes tracking a function world line of an N element neural system within at least one behavioral space, determining whether the tracking function world line is approaching a psychological stability surface, and implementing a quantitative solution that corrects instability if the tracked function world line is approaching the psychological stability surface.

Curtis, Steven A.↗
DOE OSTI2020

Exploration of Sn 70 Li 30 alloy as possible material for flowing liquid metal plasma facing components

As an advanced alternative to solid materials, Liquid Metals (LM) may offer more resilient and feasible Plasma Facing Components (PFCs). Particularly, regarding the unavoidable material erosion/degradation produced by particle/heat fluxes in future fusion devices where much longer duty cycles are expected. Furthermore, configurations that propose a flowing LM surface can add the advantage of a continuously fresh and clean layer facing the plasma. Although lithium is the most widely tested option, tin-lithium (SnLi) alloys have been proposed to attempt to combine the positive characteristics of both pure elements and ameliorate the specific issues of lithium. In this work, the potential use of Sn70Li30 alloy in such flowing concepts has been explored by addressing several preliminary and mandatory aspects for its utilization. Key issues such as wettability and compatibility of the alloy with relevant substrates have been studied in a multidisciplinary approach. The data obtained from deposited liquid tin-lithium droplets indicates approximate wetting temperatures of 360 °C, 390 °C and 405 °C for the fresh alloy on 316 stainless steel, molybdenum, and tungsten, respectively. However, the alloy contamination appeared to strongly affect the wetting characteristics of materials, increasing their wetting temperature by ~130 °C in the worst observed cases. Interestingly, in some instances, the instability of the liquid alloy surface was observed in the form of sudden gaseous ejection. The deposited droplets were posteriorly characterized in terms of absolute composition and depth profile by Inductively Coupled PlasmaOptical Emission Spectroscopy (ICP-OES) and Secondary Ion Mass Spectrometry (SIMS-ToF). Additionally, the nature and composition of the boundaries between the substrates and alloy microparticles was investigated by Scanning Electron Microscopy (SEM), Energy Dispersive X-Ray Spectroscopy (EDS), and 3D Laser microscopy. The overall results of this post-mortem characterization revealed that first signs of corrosion induced by both alloy elements (lithium-chromium association and iron-tin intermetallic mixing) were present on 316 stainless steel after short exposures (≤3 h) at temperatures lower than 550 °C. Conversely, molybdenum and tungsten showed good compatibility with the alloy in equivalent conditions. The global implications of these results are finally addressed, focusing on the future perspectives and the more viable scenarios for the eventual utilization of these alloys in flowing liquid metal configurations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Hydrodynamic instability at impact interfaces and planetary implications

Abstract Impact-induced mixing between bolide and target is fundamental to the geochemical evolution of a growing planet, yet aside from local mixing due to jetting – associated with large angles of incidence between impacting surfaces – mixing during planetary impacts is poorly understood. Here we describe a dynamic instability of the surface between impacting materials, showing that a region of mixing grows between two media having even minimal initial topography. This additional cause of impact-induced mixing is related to Richtmyer-Meshkov instability (RMI), and results from pressure perturbations amplified by shock-wave refraction through the corrugated interface between impactor and target. However, unlike RMI, this new impact-induced instability appears even if the bodies are made of the same material. Hydrocode simulations illustrate the growth of this mixing zone for planetary impacts, and predict results suitable for experimental validation in the laboratory. This form of impact mixing may be relevant to the formation of stony-iron and other meteorites.

58 GEOSCIENCES↗
NASA NTRS1993

Measuring Tollmien-Schlichting Instabilities In Laminar Flow

NASA flight experiment conducted to evaluate surface-mounted hot-film sensors designed to detect Tollmien-Schlichting (T-S) instability in boundary layer in flight. New technique has considerable value in applied research aimed at extending regions of natural laminar flow on aircraft. Aids research into mechanisms leading to transition from laminar to turbulent boundary layers. Makes it practical to take measurements in many locations on wing surface for tests in flight. Useful in studying transitions in such flow as those in pipes, ducts, channels, compressors, and diffusers.

Lee, Cynthia C.↗
NASA NTRS1982

Stable and unstable near-resonant states in multilevel, severely truncated, quasi-geostrophic models

Multilevel, severely truncated, quasi-geostrophic models with damping that extend from the surface to 100 km, are used to study the stationary-wave response to orography and the concomitant feedbacks on the zonal flow. For a typical winter zonal-wind profile, it is shown that large amplitude or resonant planetary waves of intermediate zonal wavenumbers of about 4 or 5 occur with an equivalent barotropic structure. It is also shown that wave-zonal flow interaction with a mountain torque and temperature transport is stable to small perturbations on the low side of resonance and unstable on the high side of resonance. Resonant zonal wavenumbers of lower wave wavenumber also occur for the same zonal profile and have a node in the vertical with a small amplitude maximum near the surface and a larger amplitude maximum in the stratosphere. Instability depends on the presence of the orography and the basic asymmetric state as Newtonian damping and surface friction are sufficient to damp the baroclinic instability associated with a linear inviscid model.

Roads, J. O.↗