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NASA NTRS1985

Laser radar observation of the polar stratospheric aerosol layer

The polar stratosphere has been speculated to be an active sink region of various stratospheric materials; ozone, water vapor, NOX, aerosol particles and so on, but this process is not theoretically and/or observationally made clear. The observation of the polar stratospheric aerosol layer using laser radar certainly contributes to the study of the global transport of these stratospheric minor constituents. In addition to this, from the viewpoint of aerosol science, there may be many interesting phenomena which cannot be found in the stratosphere at mid and low latitudes; the effect of precipitation of high energy molecules and atoms, of very cold winter stratosphere, of very cold mesopause in summer. Laser radar observation is one of the main activities of the Antarctic Middle Atmosphere (AMA) project at Syowa Station (69.00 deg S, 39.35 deg E), Antarctica since May 1983. Laser radar measurement at Syowa Station is discussed in detail.

Iwasaka, Y.↗

DOE OSTI2022

Invisible ship tracks show large cloud sensitivity to aerosol

Cloud reflectivity is sensitive to atmospheric aerosol concentrations because aerosols provide the condensation nuclei on which water condenses. Increased aerosol concentrations due to human activity affect droplet number concentration, liquid water and cloud fraction, but these changes are subject to large uncertainties. Ship tracks, long lines of polluted clouds that are visible in satellite images, are one of the main tools for quantifying aerosol–cloud interactions. However, only a small fraction of the clouds polluted by shipping show ship tracks. Here we show that even when no ship tracks are visible in satellite images, aerosol emissions change cloud properties substantially. We develop a new method to quantify the effect of shipping on all clouds, showing a cloud droplet number increase and a more positive liquid water response when there are no visible tracks. We directly detect shipping-induced cloud property changes in the trade cumulus regions of the Atlantic, which are known to display almost no visible tracks. Our results indicate that previous studies of ship tracks were suffering from selection biases by focusing only on visible tracks from satellite imagery. The strong liquid water path response we find translates to a larger aerosol cooling effect on the climate, potentially masking a higher climate sensitivity than observed temperature trends would otherwise suggest.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1980

Atmospheric aerosols and climate

The impact of terrestrial aerosols on the earth's climate and solar and infrared radiation budget are considered. Attention is given to the optical properties of aerosols, that is, optical depth, the single scattering albedo, and the asymmetry parameter, and to the relation between the optical depth and surface temperature for tropospheric and stratospheric aerosols. Also considered are experimental projects to determine the single scattering albedo, as well as the optical properties of natural aerosols such as sea salt, soil, and sulfates, and their variability. In addition, the impact of volcanic activity and the question of whether aerosols cause climatic warming or cooling are discussed, and the available observational evidence linking aerosols and climate is reviewed.

Toon, O. B.↗

NASA NTRS2006

The Glory Program: Global Science from a Unique Spacecraft Integration

The Glory program is an Earth and Solar science mission designed to broaden science community knowledge of the environment. The causes and effects of global warming have become a concern in recent years and Glory aims to contribute to the knowledge base of the science community. Glory is designed for two functions: one is solar viewing to monitor the total solar irradiance and the other is observing the Earth s atmosphere for aerosol composition. The former is done with an active cavity radiometer, while the latter is accomplished with an aerosol polarimeter sensor to discern atmospheric particles. The Glory program is managed by NASA Goddard Space Flight Center (GSFC) with Orbital Sciences in Dulles, VA as the prime contractor for the spacecraft bus, mission operations, and ground system. This paper will describe some of the more unique features of the Glory program including the integration and testing of the satellite and instruments as well as the science data processing. The spacecraft integration and test approach requires extensive analysis and additional planning to ensure existing components are successfully functioning with the new Glory components. The science mission data analysis requires development of mission unique processing systems and algorithms. Science data analysis and distribution will utilize our national assets at the Goddard Institute for Space Studies (GISS) and the University of Colorado's Laboratory for Atmospheric and Space Physics (LASP). The Satellite was originally designed and built for the Vegetation Canopy Lidar (VCL) mission, which was terminated in the middle of integration and testing due to payload development issues. The bus was then placed in secure storage in 2001 and removed from an environmentally controlled container in late 2003 to be refurbished to meet the Glory program requirements. Functional testing of all the components was done as a system at the start of the program, very different from a traditional program. The plan for Glory is to minimize any changes to the spacecraft in order to meet the Glory requirements. This means that the instrument designs must adhere to the existing interfaces and capabilities as much as possible. Given Glory's unique history and the potential science return, the program is one of significant value to both the science community and the world. The findings Glory promises will improve our understanding of the drivers for global climate change for a minimal investment. The program hopes to show that reuse of existing government assets can result in a lower cost, and fully successful mission.

Bajpayee Jaya↗

NASA NTRS2012

Variability and Trends of Aerosol Properties over Kanpur, Northern India using AERONET Data (2001-10)

Natural and anthropogenic aerosols over northern India play an important role in influencing the regional radiation budget, causing climate implications to the overall hydrological cycle of South Asia. In the context of regional climate change and air quality, we discuss aerosol loading variability and trends at Kanpur AERONET station located in the central part of the Indo-Gangetic plains (IGP), during the last decade (2001-10). Ground-based radiometric measurements show an overall increase in column-integrated aerosol optical depth (AOD) on a yearly basis. This upward trend is mainly due to a sustained increase in the seasonal/monthly averaged AOD during the winter (Dec-Feb) and post-monsoon (Oct-Nov) seasons (dominated by anthropogenic emissions). In contrast, a neutral to weak declining trend is observed during late pre-monsoon (Mar-May) and monsoon (Jun-Sep) months, mainly influenced by inter-annual variations of dust outbreaks. A general decrease in coarse-mode aerosols associated with variable dust activity is observed, whereas the statistically significant increasing post-monsoon/winter AOD is reflected in a shift of the columnar size distribution towards relatively larger particles in the accumulation mode. Overall, the present study provides an insight into the pronounced seasonal behavior in aerosol loading trends and, in general, is in agreement with that associating the findings with those recently reported by satellite observations (MODIS and MISR) over northern India. Our results further suggest that anthropogenic emissions (due mainly to fossil-fuel and biomass combustion) over the IGP have continued to increase in the last decade.

AERONET↗

NASA NTRS1994

Quantifying and minimizing uncertainty of climate forcing by anthropogenic aerosols

In this article, a research strategy for improving the estimates of the clear sky forcing is defined. The strategy encompasses five major, and necessarily coordinated, activities: surface-based observations of aerosol chemical and physical properties and their influence on the radiation field; aircraft-based observations of the same properties; process studies to refine model treatments; satellite observations of aerosol abundance and size distribution; and modeling studies to demonstrate consistency between the observations, to provide guidance for determination of the most important parameters, and to allow extension of the limited set of observations to the global scale. Such a strategy, if aggressively implemented, should allow these effects to be incorporated into climate models in the next several years. A similar strategy for defining the magnitude of the cloudy sky forcing should also be possible, but the less firm understanding of this forcing suggests that research of a more exploratory nature be carried out before undertaking a research strategy of the magnitude recommended for the clear sky forcing.

Penner, J. E.↗

NASA NTRS2002

The Radiative Impact of Smoke Aerosols on Clouds in Southeast Asia

The impact of smoke aerosols generated from biomass burning activities in Southeast Asia on the total (direct and indirect) reflected solar radiation from clouds was investigated using satellite data. Narrowband measurements from UV to near-infrared wavelengths (from SeaWiFS and TOMS) were combined with broadband radiation measurements (from CERES). Using this information, we quantified how smoke aerosols change the cloud forcing spectrally and as a whole in the Southeast Asia region. In this region our results show that smoke is present over large areas of cloud-covered regions, and that the frequency of such occurrences is high in the boreal spring. Depending on the thickness of the smoke aerosol, the reflected solar radiation from clouds could he reduced by as much as 100 Watt/sq m, on average over the March 2000 data. We also found that the reduction in the reflectance of the clouds at 670 nm is large enough to lead to significant errors in cloud optical thickness retrievals from satellites such as AVHRR and MODIS.

Hsu, N. Christina↗

NASA NTRS2024

Opinion: Aerosol Remote Sensing Over the Next Twenty Years

More than two decades ago, aerosol remote sensing underwent a revolution with the launch of the Terra and Aqua satellites. Advancement continued via additional launches carrying new passive and active sensors. Capable of retrieving parameters characterizing aerosol loading, rudimentary particle properties and in some cases aerosol layer height, the satellite view of Earth’s aerosol system came into focus.The modeling communities have made similar advances. Now the efforts have continued long enough that we can see developing trends in both remote sensing and modeling communities, allowing us to speculate about the future and how the community will approach aerosol remote sensing twenty years from now. We anticipate technology that will replace today’s standard multi-wavelength radiometers with hyperspectral and/or polarimetry all viewing in multiple angles.These will be supported by advanced active sensors with the ability to measure profiles of aerosol extinction in addition to backscatter. The result will be greater insight into aerosol particle properties. Algorithms will move from being primarily physically-based to include an increasing degree of Machine Learning methods, but physically-based techniques will not go extinct. However, the practice of applying algorithms to a single sensor will be in decline. Retrieval algorithms will encompass multiple sensors and all available ground measurements into a unifying framework, and these inverted products will be ingested directly into assimilation systems, becoming “cyborgs”: half observations, half model. In twenty years we will see a true democratization in space with nations large and small, private organizations and commercial entities of all sizes launching space sensors. With this increasing amount of data and aerosol products available, there will be a lot of bad data. User communities will organize to set standards and the large national space agencies will lead the effort to maintain quality by deploying and maintaining validation ground networks and focused field experiments. Through it all, interest will remain high in the global aerosol system and how that system affects climate, clouds, precipitation and dynamics, air quality, the environment and public health, transport of pathogens and fertilization of ecosystems, and how these processes are adapting to a changing climate.

aerosol remote sensing↗

NASA NTRS1986

Measuring Sodium Chloride Contents of Aerosols

Amount of sodium chloride in individual aerosol particles measured in real time by analyzer that includes mass spectrometer. Analyzer used to determine mass distributions of active agents in therapeutic or diagnostic aerosols derived from saline solutions and in analyzing ocean spray. Aerosol particles composed of sodium chloride introduced into oven, where individually vaporized on hot wall. Vapor molecules thermally dissociated, and some of resulting sodium atoms ionized on wall. Ions leave oven in burst and analyzed by spectrometer, which is set to monitor sodium-ion intensity.

Sinha, M. P.↗

NASA NTRS1993

The impact of the eruptions of Mount Pinatubo and Cerro Hudson on antarctic aerosol levels during the 1991 austral spring

At the beginning of the 1991 Austral spring, volcanic aerosols from Mt. Pinatubo and Cerro Hudson were present in the polar stratosphere of the Southern Hemisphere. Satellite observations of aerosol extinction were used to identify and track the movement of these aerosols in the vicinity of the Antarctic vortex during August through November 1991. A layer of mature Mt. Pinatubo aerosols was identified near 21 km and a layer of fresh Cerro Hudson aerosols was identified near 12 km. This altitude separation of the Mt. Pinatubo and Cerro Hudson aerosols was observed throughout the period. Below 15 km, the polar stratosphere was subject to episodes of strong wave activity which transported the Cerro Hudson aerosols poleward and, after the middle of September, they became a persistent feature beneath the vortex. Above 15 km, signatures of Mt. Pinatubo aerosols were observed near the vortex boundary, but significant portions of the vortex interior remained free of any detectable intrusions of Mt. Pinatubo aerosols until the final warming in mid-November.

Pitts, M. C.↗

DOE OSTI2024

Applying a Phase-Separation Parameterization in Modeling Secondary Organic Aerosol Formation from Acid-Driven Reactive Uptake of Isoprene Epoxydiols under Humid Conditions

Secondary organic aerosol (SOA) from acid-driven reactive uptake of isoprene epoxydiols (IEPOX) contributes up to 40% of organic aerosol (OA) mass in fine particulate matter. Our previous work showed substantial conversions of particulate inorganic sulfates to surface-active organosulfates (OSs) by IEPOX decreases aerosol acidity and creates a viscous organic-rich shell that poses as a diffusion barrier, inhibiting additional reactive uptake of IEPOX. In this study, to account for this “self-limiting” effect, a phase-separation box model was developed to evaluate parameterizations of IEPOX reactive uptake against time-resolved chamber measurements of IEPOX-SOA tracers, including 2-methyltetrols (2-MT) and methyltetrol sulfates (MTS), at ~ 50% relative humidity. The phase-separation model was most sensitive to mass accommodation coefficient, IEPOX diffusivity in the organic shell, and ratio of the third-order reaction rate constants forming 2-MT and MTS (k MT /k MTS ). In particular, k MT /k MTS had to be lower than 0.1 to bring model predictions of 2-MT and MTS in closer agreement with chamber measurements, while prior studies reported values larger than 0.71. The model-derived rate constants favor more particulate MTS formation due to 2-MT likely off-gassing at ambient-relevant OA loadings. Incorporating this parametrization into chemical transport models is expected to predict lower IEPOX-SOA mass and volatility due to the predominance of OSs.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

NASA NTRS2016

Aerosol Meteorology of Maritime Continent for the 2012 7SEAS Southwest Monsoon Intensive Study - Part 2: Philippine Receptor Observations of Fine-Scale Aerosol Behavior

The largest 7 Southeast Asian Studies (7SEAS) operations period within the Maritime Continent (MC) occurred in the August-September 2012 biomass burning season. Data included were observations aboard the MY Vasco, dispatched to the Palawan Archipelago and Sulu Sea of the Philippines for September 2012. At these locations, the Vasco observed MC smoke and pollution entering the southwest monsoon (SWM) monsoonal trough. Here we describe the research cruise findings and the finer-scale aerosol meteorology of this convectively active region. This 2012 cruise complemented a 2-week cruise in 2011 and was generally consistent with previous findings in terms of how smoke emission and transport related to monsoonal flows, tropical cyclones (TC), and the covariance between smoke transport events and the atmosphere's thermodynamic structure. Biomass burning plumes were usually mixed with significant amounts of anthropogenic pollution. Also key to aerosol behavior were squall lines and cold pools propagating across the South China Sea (SCS) and scavenging aerosol particles in their path. However, the 2012 cruise showed much higher modulation in aerosol frequency than its 2011 counterpart. Whereas in 2011 large synoptic-scale aerosol events transported high concentrations of smoke into the Philippines over days, in 2012 measured aerosol events exhibited a much shorter-term variation, sometimes only 312h. Strong monsoonal flow reversals were also experienced in 2012. Nucleation events in cleaner and polluted conditions, as well as in urban plumes, were observed. Perhaps most interestingly, several cases of squall lines preceding major aerosol events were observed, as opposed to 2011 observations where these lines largely scavenged aerosol particles from the marine boundary layer. Combined, these observations indicate pockets of high and low particle counts that are not uncommon in the region. These perturbations are difficult to observe by satellite and very difficult to model. Indeed, the Navy Aerosol Analysis and Prediction System (NAAPS) simulations captured longer period aerosol events quite well but largely failed to capture the timing of high-frequency phenomena. Ultimately, the research findings of these cruises demonstrate the real world challenges of satellite-based missions, significant aerosol life cycle questions such as those the future Aerosol/Clouds/Ecosystems (ACE) will investigate, and the importance of small-scale phenomena such as sea breezes, squall lines, and nucleation events embedded within SWM patterns in dominating aerosol life cycle and potential relationships to clouds.

Reid, Jeffrey S.↗

NASA NTRS2022

Simultaneous Retrievals of Biomass Burning Aerosols and Trace Gases From the Ultraviolet to Near-Infrared Over Northern Thailand During the 2019 Pre-Monsoon Season

With the advent of spaceborne spectroradiometers in a geostationary constellation, measuring high spectral resolution ultraviolet–visible (UV-VIS) and selected near-/shortwave-infrared (NIR/SWIR) radiances can enable the probing of the life cycle of key atmospheric trace gases and aerosols at higher temporal resolutions over the globe. The UV-VIS measurements are important for retrieving several key trace gases (e.g., O 3 , SO 2 , NO 2 , and HCHO) and particularly for deriving aerosol characteristics (e.g., aerosol absorption and vertical profile). This study examines the merit of simultaneous retrievals of trace gases and aerosols using a ground-based spectroradiometer covering the UV-NIR to monitor their physicochemical processes and to obtain reliable aerosol information for various applications. During the 2019 pre-monsoon season over northern Thailand, we deployed a ground-based SMART–s (Spectral Measurements for Atmospheric Radiative Transfer–spectroradiometer) instrument, which is an extended-range Pandora with reliable radiometric calibration in the 330–820 nm range, to retrieve remotely sensed chemical and aerosol properties for the first time near biomass burning sources. The high spectral resolution (∼ 1.0 nm full width half maximum with ∼ 3.7 × oversampling) of sun and sky measurements from SMART–s provides several key trace gases (e.g., O 3 , NO 2 , and H 2 O) and aerosol properties covering the UV where significant light absorption occurs by the carbonaceous particles. During the measurement period, highly correlated total column amounts of NO 2 and aerosol optical thickness (т aer ) retrieved from SMART–s (correlation coefficient, R=0.74) indicated their common emissions from biomass burning events. The SMART–s retrievals of the spectral single scattering albedo (ω 0 ) of smoke aerosols showed an abrupt decrease in the UV, which is an important parameter dictating photochemical processes in the atmosphere. The values of ω 0 and column precipitable water vapor (H 2 O) gradually increase with the mixing of biomass burning smoke particles and higher water vapor concentrations when approaching the monsoon season. The retrieved ω 0 and weighted mean radius of fine-mode aerosols from SMART–s showed positive correlations with the H 2 O (R=0.81 for ω 0 at 330 nm and 0.56 for the volume-weighted mean radius), whereas the real part of the refractive index of fine-mode aerosol (n f ) showed negative correlations (R = -0.61 at 330 nm), which suggest that aerosol aging processes including hygroscopic growth (e.g., humidification and cloud processing) can be a major factor affecting the temporal trends of aerosol optical properties. Retrieved n f and ω 0 were closer to those of the water droplet (i.e., n f of about 1.33 and ω 0 of about 1.0) under lower amounts of NO 2 during the measurement period; considering that the NO 2 amounts in the smoke may indicate the aging of the plume after emission due to its short lifetime, the tendency is also consistent with active hygroscopic processes of the aerosols over this area. Retrieved UV aerosol properties from SMART–s generally support the assumed smoke aerosol models (i.e., the spectral shape of aerosol absorption) used in NASA's current satellite algorithms, and their spectral ω 0 retrievals from ground and satellites showed good agreements (R = 0.73–0.79). However, temporal and spectral variabilities in the aerosol absorption properties in the UV emphasize the importance of a realistic optical model of aerosols for further improvements in satellite retrievals.

biomass burning↗

NASA NTRS2014

Quantification of Aerosol Type, and Sources of Aerosols Over the Indo- Gangetic Plain

Differences and similarities in aerosol characteristics, for the first time, over two environmentally distinct locations in Indo-Gangetic plain (IGP) e Kanpur (KPR) (urban location) and Gandhi College (GC) (rural site) are examined. Aerosol optical depths (AODs) exhibit pronounced seasonal variability with higher values during winter and premonsoon. Aerosol fine mode fraction (FMF) and Ångstrom exponent (a) are higher over GC than KPR indicating relatively higher fine mode aerosol concentration over GC. Higher FMF over GC is attributed to local biomass burning activities. Analysis of AOD spectra revealed that aerosol size distribution is dominated by wide range of fine mode fractions or mixture of modes during winter and postmonsoon, while during premonsoon and monsoon coarse mode aerosols are more abundant. Single scattering albedo (SSA) is lower over GC than KPR. SSA spectra reveals the abundance of fine mode (coarse mode) absorbing (scattering) aerosols during winter and postmonsoon (premonsoon and monsoon). Spectral SSA features reveal that OC contribution to enhanced absorption is negligible. Analysis shows that absorbing aerosols can be classified as Mostly Black Carbon (BC), and Mixed BC and Dust over IGP. Mixed BC and dust is always higher over KPR, while Mostly BC is higher over GC throughout the year. The amount of long range transported dust exhibits a gradient between KPR (higher) and GC (lower). Results on seasonally varying aerosol types, and absorbing aerosol types and their gradients over an aerosol hotspot are important to tune models and to reduce the uncertainty in radiative and climate impact of aerosols.

Organic Carbon↗

NASA NTRS2024

High Spectral Resolution Lidar – Generation 2 (HSRL-2) Retrievals of Ocean Surface Wind Speed: Methodology and Evaluation

Ocean surface wind speed (i.e., wind speed 10 m above sea level) is a critical parameter used by atmospheric models to estimate the state of the marine atmospheric boundary layer (MABL). Accurate surface wind speed measurements in diverse locations are required to improve characterization of MABL dynamics and assess how models simulate large-scale phenomena related to climate change and global weather patterns. To provide these measurements, this study introduces and evaluates a new surface wind speed data product from the NASA Langley Research Center nadir-viewing High Spectral Resolution Lidar – generation 2 (HSRL-2) using data collected as part of the NASA Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) mission. The HSRL-2 can directly measure vertically resolved aerosol backscatter and extinction profiles without additional constraints or assumptions, enabling the instrument to accurately derive atmospheric attenuation and directly determine surface reflectance (i.e., surface backscatter). Also, the high horizontal spatial resolution of the HSRL-2 retrievals (0.5 s or ∼ 75 m along track) allows the instrument to probe the fine-scale spatial variability in surface wind speeds over time along the flight track and over breaks in broken cloud fields. A rigorous evaluation of these retrievals is performed by comparing coincident HSRL-2 and National Center for Atmospheric Research (NCAR) Airborne Vertical Atmosphere Profiling System (AVAPS) dropsonde data, owing to the joint deployment of these two instruments on the ACTIVATE King Air aircraft. These comparisons show correlations of 0.89, slopes of 1.04 and 1.17, and y intercepts of −0.13 and −1.05 m s−1 for linear and bisector regressions, respectively, and the overall accuracy is calculated to be 0.15 ± 1.80 m s−1. It is also shown that the dropsonde surface wind speed data most closely follow the HSRL-2 distribution of wave slope variance using the distribution proposed by Hu et al. (2008) rather than the ones proposed by Cox and Munk (1954) and Wu (1990) for surface wind speeds below 7 m s−1, with this category comprising most of the ACTIVATE data set. The retrievals are then evaluated separately for surface wind speeds below 7 m s−1 and between 7 and 13.3 m s−1 and show that the HSRL-2 retrieves surface wind speeds with a bias of ∼ 0.5 m s−1 and an error of ∼ 1.5 m s−1, a finding not apparent in the cumulative comparisons. Also, it is shown that the HSRL-2 retrievals are more accurate in the summer (−0.18 ± 1.52 m s−1) than in the winter (0.63 ± 2.07 m s−1), but the HSRL-2 is still able to make numerous (N=236) accurate retrievals in the winter. Overall, this study highlights the abilities and assesses the performance of the HSRL-2 surface wind speed retrievals, and it is hoped that further evaluation of these retrievals will be performed using other airborne and satellite data sets.

Sanja Dmitrovic↗

DOE OSTI2024

Understanding aerosol–cloud interactions using a single-column model for a cold-air outbreak case during the ACTIVATE campaign

Marine boundary layer clouds play a critical role in Earth's energy balance. Their microphysical and radiative properties are highly impacted by ambient aerosols and dynamic forcings. In this study, we evaluate the representation of these clouds and related aerosol–cloud interaction processes in the single-column version of the E3SM climate model (SCM) against field measurements collected during the NASA ACTIVATE campaign over the western North Atlantic, as well as intercompare results with high-resolution process level models. We show that E3SM SCM reproduces the macrophysical properties of post-frontal boundary layer clouds in a cold-air outbreak (CAO) case well. However, it generates fewer but larger cloud droplets compared to aircraft measurements. Further sensitivity tests show that the underestimation of both aerosol number concentration and vertical velocity variance contributes to this bias. Aerosol–cloud interactions are examined by perturbing prescribed aerosol properties in E3SM SCM with fixed dynamics. Higher aerosol number concentration or hygroscopicity leads to more numerous but smaller cloud droplets, resulting in a stronger cooling via shortwave cloud forcing. This apparent Twomey effect is consistent with prior climate model studies. The cloud liquid water path shows a weakly positive relation with cloud droplet number concentration due to precipitation suppression. This weak aerosol effect on cloud macrophysics may be attributed to the dominant impact of strong dynamical forcing associated with the CAO. Our findings indicate that the SCM framework is a key tool to bridge the gap between climate models, process level models, and field observations to facilitate process level understanding.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2018

A13H-2537: Above Cloud Aerosol Optical Properties in the South East Atlantic from airborne observations during ORACLES

Aerosol overlying marine stratocumulus clouds is a persistent feature in the southeast Atlantic during the biomass burning season, July through November. We sampled aerosol and cloud from an airborne research platform, the NASA P3, during the deployments of ObseRvations of CLouds above Aerosols and their intEractionS (ORACLES) encompassing the peak biomass burning season. We used the Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR) to quantify the aerosol’s optical properties, notably the aerosol optical depth (AOD) by directly measuring the amount of light attenuation. We present an overview of very recent AOD measurements and contrast those to previous deployments. We observed an average AOD at 500 nm of 0.33 (0.30) in September 2016 (August 2017), with similar spatial dependence as observed by the MODIS instrument on board the TERRA and AQUA satellites. We also show full spectral vertical dependence of AOD from flight profiles, which compares favorably to the integrated aerosol extinction profile obtained by the active remote sensing High Spectral Resolution Lidar-2 (HSRL-2). We also present a quantification of the gap extent separating cloud top and aerosol layer bottom. Using hyperspectral transmitted light measurements from 4STAR, in conjunction with hyperspectral hemispheric irradiance measurements from the Solar Spectral Flux Radiometers (SSFR), we retrieved aerosol intensive properties (asymmetry parameter, single scattering albedo), aerosol size distributions, cloud optical depth (COD), cloud particle effective radius, and cloud thermodynamic phase. Cloud properties, also presented here, are obtained from 4STAR measurements of scattered light below clouds.

Samuel E LeBlanc↗

NASA NTRS2002

Biomass-burning Aerosols in South East-Asia: Smoke Impact Assessment(BASE-ASIA)

Biomass burning has been a regular practice for land clearing and land conversion in many countries, especially in Africa, South America, and South East Asia. Significant global sources of greenhouse gases (e.g., CO2, CH4), chemically active gases (e.g., NO, CO, HC, CH3Br), and atmospheric aerosols are produced by biomass-burning processes, which influence the Earth-atmosphere energetics and hence impact both global climate and tropospheric chemistry. Some gases and aerosols can serve as active cloud condensation nuclei, which play important role in determining the net radiation budget, precipitation rate, and cloud lifetime. Biomass burning also affects the biogeochemical cycling of nitrogen and carbon compounds from the soil to the atmosphere; the hydrological cycle (i.e., run off and evaporation); the reflectivity and emissivity of the land; and the stability of ecosystems and ecosystem biodiversity. Compared to Africa and South America, the climatology in South East Asia reveals quite different characteristics, showing distinct large-scale smoke and cloud sources and interaction regimes. The fresh water distribution in this region is highly dependent on monsoon rainfall; in fact, the predictability of the tropical climate system is much reduced during the boreal spring, which is associated with the peak season of biomass burning activities. Estimating the burning fuel (e.g., bark, branches, and wood), an important part of studying regional carbon cycle, may rely on utilizing a wide range of distinctive spectral features in the shortwave and longwave regions. Therefore, to accurately assess the impact of smoke aerosols in this region requires continuous observations from satellites, aircraft, networks of ground-based instruments and dedicated field experiments. A new initiative will be proposed and discussed.

Tsay, Si-Chee↗