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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 235 records · Page 13
All sourcesNASA NTRSDOE OSTI
NASA NTRS2007

Large-Area Permanent-Magnet ECR Plasma Source

A 40-cm-diameter plasma device has been developed as a source of ions for material-processing and ion-thruster applications. Like the device described in the immediately preceding article, this device utilizes electron cyclotron resonance (ECR) excited by microwave power in a magnetic field to generate a plasma in an electrodeless (noncontact) manner and without need for an electrically insulating, microwave-transmissive window at the source. Hence, this device offers the same advantages of electrodeless, windowless design - low contamination and long operational life. The device generates a uniform, high-density plasma capable of sustaining uniform ion-current densities at its exit plane while operating at low pressure [<10(exp -4) torr (less than about 1.3 10(exp -2) Pa)] and input power <200 W at a frequency of 2.45 GHz. Though the prototype model operates at 2.45 GHz, operation at higher frequencies can be achieved by straightforward modification to the input microwave waveguide. Higher frequency operation may be desirable in those applications that require even higher background plasma densities. In the design of this ECR plasma source, there are no cumbersome, power-hungry electromagnets. The magnetic field in this device is generated by a permanent-magnet circuit that is optimized to generate resonance surfaces. The microwave power is injected on the centerline of the device. The resulting discharge plasma jumps into a "high mode" when the input power rises above 150 W. This mode is associated with elevated plasma density and high uniformity. The large area and uniformity of the plasma and the low operating pressure are well suited for such material-processing applications as etching and deposition on large silicon wafers. The high exit-plane ion-current density makes it possible to attain a high rate of etching or deposition. The plasma potential is <3 V low enough that there is little likelihood of sputtering, which, in plasma processing, is undesired because it is associated with erosion and contamination. The electron temperature is low and does not vary appreciably with power.

Foster, John E.↗
DOE OSTI2026

A Dendrite-Resistant Sodium/Porous-Carbon Anode for Solid-State Batteries – Strategies and Challenges for Low-Pressure Operation

Sodium solid-state batteries (Na-SSB) have gained interest recently due to the abundance of Na over Li, but they still tend to fail due to dendrites under practical current densities and cycling capacities. To overcome this, Na-SSBs are frequently tested with impractically high applied pressure. In this work, a porous carbon interfacial layer is utilized in conjunction with Na-ß”-Al2O3 solid electrolytes to enable Na-cycling at milder cell pressures. This sodium/porous carbon layer enables improved solid-state Na cycling in symmetric cells, up to a current density of 10 mA cm-2 at 25 °C. Cycling up to 1 mAh cm-2 is challenging with low pressure, but 1 mAh cm-2 capacity can be reliably cycled at 1 mA cm-2 at an elevated temperature of 60 °C in symmetric cells. Finally, the evolution of the interface and sodium/carbon anode is evaluated with cryogenic ion-milling and cross-sectional imaging revealing that, depending on testing temperature, pressure, current density, and capacity, void formation, Na-extraction from porous carbon, delamination of the porous carbon matrix, or a combination of these occurs at the interface between Na-metal and BASE. Despite this, excellent dendrite resistance is achieved, and a full-cell design utilizing a Na-transition metal oxide cathode is still able to achieve an areal capacity of ~ 2.7 mAh cm-2 at 0.125 mA cm-2. This work demonstrates an alternative pathway toward a Na-metal anode for Na-SSBs without the requirement of excessive stack pressure.

low-cost↗
DOE OSTI2024

Electrolyte Design for NMC811||SiO x -Gr Lithium-Ion Batteries with Excellent Low-Temperature and High-Rate Performance

The use of high-nickel NMC811 cathode and SiO x -Gr anode can greatly improve the overall energy densities of lithium-ion batteries. However, the unfavorable solid electrolyte interphase (SEI) layer generated from the decomposition of EC-based electrolytes lead to the poor cycling stability of NMC811||SiO x -Gr cells. Here we report an electrolyte design of 1.5 M LiPF 6 dissolved in FEC/MA/BN 2:2:6 by volume, which can form thin, robust, and homogeneous SEI layer to greatly improve the charge transfer at the electrode-electrolyte interface. Importantly, the designed electrolyte shows an outstanding low temperature performance that it can deliver a capacity of 123.3 mAh g –1 after 50 cycles at −20 °C with a current density of 0.5 C, overwhelming the standard EC-based electrolyte (1.2 M LiPF 6 EC/EMC 3:7 by volume) with a capacity of 35.7 mAh g –1 . The electrolyte also has a superior rate performance that it achieves a capacity of 122.5 mAh g −1 at a high current density of 10 C. Moreover, the LTE electrolyte holds the great potential of extreme fast-charging ability because of the large part of CC contribution in the CCCV charging model at high charging current densities.

Electrochemistry↗
NASA NTRS1975

Charge-exchange plasma generated by an ion thruster

The use of high voltage solar arrays greatly reduces or eliminates power processing requirements in space electric propulsion systems. This use also requires substantial areas of solar array to be at high positive potential relative to space and most of the spacecraft. The charge exchange plasma conducts electrons from the ion beam to such positive surfaces, and thereby electrically load the high voltage solar array. To evaluate this problem, the charge-exchange plasma generated by an ion beam was investigated experimentally. Based upon the experimental data, a simple model was derived for the charge-exchange plasma. This model is conservative in the sense that both the electron/ion density and the electron current density should be equal to, or less than, the preducted value for all directions in the hemisphere upstream of the ion beam direction. Increasing the distance between a positive potential surface (such as a high voltage solar array) and the thruster is the simplest way to control interactions. Both densities and currents vary as the inverse square of this distance.

Kaufman, H. R.↗
NASA NTRS1984

Effect of reabsorbed recombination radiation on the saturation current of direct gap p-n junctions

The application of the radiative transfer theory for semiconductors to p-n homojunctions subject to low level injection conditions is discussed. By virtue of the interaction of the radiation field with free carriers across the depletion layer, the saturation current density in Shockley's expression for the diode current is reduced at high doping levels. The reduction, due to self-induced photon generation, is noticeable for n-type material owing to the small electron effective mass in direct band-gap III-V compounds. The effect is insignificant in p-type material. At an equilibrium electron concentration of 2 x 10 to the 18th/cu cm in GaAs, a reduction of the saturation current density by 15 percent is predicted. It is concluded that realistic GaAs p-n junctions possess a finite thickness.

Von Roos, O.↗
NASA NTRS1994

Regional-scale flows in mountainous terrain. Part 1: A numerical and observational comparison

This study uses observed data and a numerical simulation to examine the generation of thermally driven flows across the Colorado mountain barrier on meso-beta to meso-alpha scales. The observations were collected from remote surface observing systems at exposed mountaintop locations throughout the state of Colorado, over the summers of 1984-88, as part of the Rocky Mountain Peaks Experiment (ROMPEX). The data show the development of a recurrent circulation system across the Colorado mountain barrier, operating on a diurnal timescale. From the observations, the basic structure of the flow system appears as a daytime inflow toward the highest terrain, and a nocturnal outflow away from it. However, when examined in detail, the flow system exhibits more unusual behavior, especially west of the barrier crest. Here, winds in the early evening are occasionally observed to onset abruptly from an easterly direction, generally counter to the upper-level winds. Observations from ROMPEX for 26 August 1985 are used to provide comparison data for a numerical simulation with the Regional Atmospheric Modeling System (RAMS). This three-dimensional case study experiment is initialized with data from the National Meteorological Center and incorporates two-way interactive grid nesting. From the observed data and case study simulation, four distinct phases of the regional-scale circulation system have been identified. In the development phase, a deep mountain-plains solenoid is generated through terrain heating along the Front Range. This circulation system transforms in the late afternoon transition phase into a westward-propagating density current (WPDC). The third phase, called the 'density-current propagation phase,' occurs as the WPDC moves westward across the mountains, leaving in its wake strong southeasterly flow at the mountaintop level. This current appears to be the cause of the peculiar easterly component winds found in the ROMPEX mountaintop observations along the western slope. In the final late-night adjustment phase, the WPDC dissipates near the western edge of the Colorado mountains and steady southerly flow evolves over the high mountain terrain. This southerly flow is the steady response to the differential heating that develops between the low-lying plains and the intermountain region.

Bossert, James E.↗
NASA NTRS2023

Analytical model of foreshock ion interaction with a discontinuity: A statistical study

When a solar wind discontinuity interacts with foreshock ions, foreshock transients such as hot flow anomalies and foreshock bubbles can form. These create significant dynamic pressure perturbations disturbing the bow shock, magnetopause, and magnetosphere-ionosphere system. However, presently these phenomena are not predictable. In the accompanying paper, we derived analytical equations of foreshock ion partial gyration around a discontinuity and the resultant current density. In this study, we utilize the derived current density strength to model the energy conversion from the foreshock ions, which drives the outward motion or expansion of the solar wind plasma away from the discontinuity. We show that the model expansion speeds match those from local hybrid simulations for varying foreshock ion parameters. Using MMS, we conduct a statistical study showing that the model expansion speeds are moderately correlated with the magnetic field strength variations and the dynamic pressure decreases around discontinuities with correlation coefficients larger than 0.5. We use conjunctions between ARTEMIS and MMS to show that the model expansion speeds are typically large for those already-formed foreshock transients. Our results show that our model can be reasonably successful in predicting significant dynamic pressure disturbances caused by foreshock ion-discontinuity interactions. We discuss ways to improve the model in the future.

Terry Z. Liu↗
DOE OSTI2025

Ampere-level co-electrosynthesis of formate from CO 2 reduction paired with formaldehyde dehydrogenation reactions

Current catalysts face challenges with low formate selectivity at high current densities during the CO 2 electroreduction. Here, we showcase a versatile strategy to enhance the formate production on p-block metal-based catalysts by incorporating noble metal atoms on their surface, refining oxygen affinity, and tuning adsorption of the critical oxygen-bound *OCHO intermediate. The formate yield is observed to afford a volcano-like dependence on the *OCHO binding strength across a series of modified catalysts. The rhodium-dispersed indium oxide (Rh/In 2 O 3 ) catalyst exhibits impressive performances, achieving Faradaic efficiencies (FEs) of formate exceeding 90% across a broad current density range of 0.20 to 1.21 A cm −2 . In situ Raman spectroscopy and theoretical calculations reveal that the oxophilic Rh site facilitates *OCHO formation by optimizing its adsorption energy, placing Rh/In 2 O 3 near the volcano-shaped apex. A bipolar electrosynthesis system, coupling the CO 2 reduction at the cathode with the formaldehyde oxidative dehydrogenation at the anode, further boosts the FE of formate to nearly 190% with pure hydrogen generation under an ampere-level current density and a low cell voltage of 2.5 V in a membrane electrode assembly cell.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1976

Measurements of field-aligned currents in a multiple auroral arc system

A rocket-borne experiment to study the currents associated with a system of multiple auroral arcs was conducted at Poker Flat, Alaska, at 1122 UT on Feb. 2, 1972. The magnetic field in the vicinity of the auroral system was measured with a cesium vector magnetometer. Possible configurations were inferred by constructing model current systems that reproduced the magnetic field variations measured along the flight path. The data are interpreted in terms of a model current system consisting of two eastward electrojets and one westward electrojet and three pairs of oppositely directed Birkeland sheet currents, all lying in a plane approximately parallel to the auroral arcs. Sheet thicknesses ranged from 20 to 60 km and current densities from 10 to 45 microampere/sq m; the electrojet currents ranged from 1000 to 2000 A. A possible alternate model consisted of four pairs of sheets whose thicknesses range from 10 to 40 km with current densities from 10 to 90 microampere/sq m. There was quite good agreement between the locations of the visual arcs and the upward current sheets. The overall current configuration is discussed in view of the theoretical models constructed by Atkinson and Sato and Holzer and of other observations.

Sesiano, J.↗
DOE OSTI2024

In Situ Characterization of Interface Evolution in Argyrodite‐Based All‐Solid‐State Li Batteries

Interfacial stability is one of the critical challenges in all-solid-state Li metal batteries. Multiple processes such as solid electrolyte (SE) decomposition and lithium dendrite growth take place at the solid interfaces during cycling, leading to the overall cell failure. To deconvolute these complex processes, in situ characterization is of paramount importance to elucidate the interfacial evolution on the SE upon Li plating/stripping. Herein, an all-solid-state asymmetric in situ cell is developed that allows the direct visualization of the highly localized Li plating/stripping processes under the optical microscope. Moreover, this cell configuration enables reliable post-mortem chemical and morphological analysis of the intact SE/Li interface. Using combined scanning electron microscopy and energy-dispersive X-ray spectroscopy, the study reveals that the evolution of the Li argyrodite interface is strongly influenced by the current density, particularly in terms of chemical distribution and Li plating morphology. More specifically, the solid interface is LiCl-rich with the formation of Li cubes at low current densities, while high currents result in more uniform elemental distribution and filament morphology. These findings elucidate the dynamic evolution mechanism at solid interfaces and offer valuable guidance for developing stable solid interfaces in all-solid-state Li metal batteries.

Huang, Di↗
DOE OSTI2026

Pulsed Electrolysis Promotes Catalyst Activity in Dilute CO 2 Streams

Industrial CO 2 streams vary widely in composition, from pure to as low as 3%, posing challenges for purification or direct conversion. Electrochemical reduction offers a route for converting dilute CO 2 streams but faces severe mass transport limitations. This study demonstrates that pulsed electrolysis effectively overcomes these limitations, enhancing CO 2 electroreduction across variable feed compositions and current densities, particularly at low CO 2 concentrations and high current densities. At 25% CO 2 and 400 mA cm −2 , pulsing improved selectivity from 25.6 to 78.6%, production rate from 13.7 to 21.0 mol m −2 h −1 , and energy productivity from 0.77 to 2.59 mol kWh −1 . A dynamic, multiphysics continuum model confirms a 64% increase in CO 2 concentration within the catalyst layer during pulsing, resolving the transient chemical microenvironment. These findings establish pulsed electrolysis as a viable strategy for converting dilute industrial CO 2 streams into valuable feedstocks, bypassing costly pre-separation.

Orfali, Dania Muhieddine [New York University (NYU↗
NASA NTRS1978

Boundary-value problem for a counterrotating electrical discharge in an axial magnetic field

An electrical discharge between two ring electrodes embedded in the mantle of a cylindrical chamber is considered, in which the plasma in the anode and cathode regions rotates in opposite directions under the influence of an external axial magnetic field. The associated boundary-value problem for the coupled partial differential equations describing the azimuthal velocity and radial current-density fields is solved in closed form. The velocity, current density, induced magnetic induction, and electric fields are presented for typical Hartmann numbers, magnetic Reynolds numbers, and geometry parameters. The discharge is shown to produce anodic and cathodic plasma sections rotating at speeds of the order 1,000,000 cm/sec for conventional magnetic field intensities. Possible application of the magnetoactive discharge as a plasma centrifuge for isotope separation is discussed.

Hong, S. H.↗
NASA NTRS1986

ISEE 1 and 2 observations of Birkeland currents in the earth's inner magnetosphere

Signatures of Birkeland currents in the earth's inner magnetosphere observed from the ISEE 1 and 2 spacecraft during November 1977-December 1978 at distances ranging from 2.4-7.0 earth radii are examined. The data reveal that most of the currents were detected during outbound rather than inbound passes. Large-scale current structures were identified as parts of the region 1 and 2 current systems in 27 percent of the spacecraft outbound passes; no distinguishable region 1 or 2 currents were detected in 19 percent of the outbound passes; and in 54 percent of the passes multiple current structures and ambiguous magnetic signatures were observed. The properties of Birkeland current structures observed on January 31, 1978, February 28, 1978, March 15, 1978, June 21, 1978, and June 25, 1978 are described. It is observed that the current sheet thicknesses range from 519-18,279 km; sheet current density ranges from 13-150 mA/m; and the volume current density ranges from 1.7-128 nA/sq m.

Kelly, T. J.↗
NASA NTRS2003

Thermo-Electron Ballistic Coolers or Heaters

Electronic heat-transfer devices of a proposed type would exploit some of the quantum-wire-like, pseudo-superconducting properties of single-wall carbon nanotubes or, optionally, room-temperature-superconducting polymers (RTSPs). The devices are denoted thermo-electron ballistic (TEB) coolers or heaters because one of the properties that they exploit is the totally or nearly ballistic (dissipation or scattering free) transport of electrons. This property is observed in RTSPs and carbon nanotubes that are free of material and geometric defects, except under conditions in which oscillatory electron motions become coupled with vibrations of the nanotubes. Another relevant property is the high number density of electrons passing through carbon nanotubes -- sufficient to sustain electron current densities as large as 100 MA/square cm. The combination of ballistic motion and large current density should make it possible for TEB devices to operate at low applied potentials while pumping heat at rates several orders of magnitude greater than those of thermoelectric devices. It may also enable them to operate with efficiency close to the Carnot limit. In addition, the proposed TEB devices are expected to operate over a wider temperature range

Choi, Sang H.↗
DOE OSTI2025

Novel Electrowinning Reactor for the Energy-Efficient, Low- Cost Production of Rare Earth Metals

This project developed a novel neodymium (Nd) electrowinning reactor for energy-efficient electrowinning of Nd metal. Throughout this project we have developed an alternative chloride based molten salt electrolysis process. Our process lowers the specific electrical energy consumption compared to the state of the art, while producing reusable chlorine gas and eliminating direct CO2 and PFC emissions. Facilities required for implementing the project were setup and designs were finalized, and a standard operating procedure for safe operation of high temperature electrolysis cells was written. The electrowinning reactor was designed and constructed. Electrolysis experiments confirmed the ability to reproducibly electrowin Nd metal on a Mo cathode. The current efficiency for Nd electrowinning was measured as a function of applied current density in the presence of the separator. Successful electrowinning of Nd sponge at high current densities (200 mA/cm2 and above) at a current efficiency >80% was demonstrated using multiple techniques. Stable Nd electrowinning up to 10h at 250 mA/cm2 was demonstrated. All of these design advancements were used to develop a techno-economic and life cycle assessment model that demonstrated that our process could be operated at cost of less than $0.20/kg-Nd (~30% lower compared to state of the art when comparing electrolysis energy cost) with a >20% total reduction in global warming potential compared to the state of the art while generating no direct CO2 or perfluorocarbon emissions.

42 ENGINEERING↗
NASA NTRS1994

Segmented Ion Engine Plume Characteristics

Preliminary evaluation of the segmented ion thruster (SIT) ion beam characteristics was performed by measuring the two dimensional ion current density distribution at four axial locations downstream from the thruster. Current density profiles were measured with the concurrent operation of multiple ion sources. Preliminary assessments regarding symmetry of the plume, characterization of plume development as a function of axial position, and the interactions of multiple simultaneously operating ion sources were conducted. A numerical integration scheme was applied to the acquired data to determine the total beam current. A qualitative analysis of the downstream development of the ion beam was conducted. Most of the data acquired so far has been on somewhat of a trial basis and extensive testing is scheduled to resume in August 1994.

ion↗
NASA NTRS1999

Three-Dimensional Simulations of Electron Beams Focused by Periodic Permanent Magnets

A fully three-dimensional (3D) model of an electron beam focused by a periodic permanent magnet (PPM) stack has been developed. First, the simulation code MAFIA was used to model a PPM stack using the magnetostatic solver. The exact geometry of the magnetic focusing structure was modeled; thus, no approximations were made regarding the off-axis fields. The fields from the static solver were loaded into the 3D particle-in-cell (PIC) solver of MAFIA where fully 3D behavior of the beam was simulated in the magnetic focusing field. The PIC solver computes the time-integration of electromagnetic fields simultaneously with the time integration of the equations of motion of charged particles that move under the influence of those fields. Fields caused by those moving charges are also taken into account; thus, effects like space charge and magnetic forces between particles are fully simulated. The electron beam is simulated by a number of macro-particles. These macro-particles represent a given charge Q amounting to that of several million electrons in order to conserve computational time and memory. Particle motion is unrestricted, so particle trajectories can cross paths and move in three dimensions under the influence of 3D electric and magnetic fields. Correspondingly, there is no limit on the initial current density distribution of the electron beam, nor its density distribution at any time during the simulation. Simulation results including beam current density, percent ripple and percent transmission will be presented, and the effects current, magnetic focusing strength and thermal velocities have on beam behavior will be demonstrated using 3D movies showing the evolution of beam characteristics in time and space. Unlike typical beam optics models, this 3D model allows simulation of asymmetric designs such as non- circularly symmetric electrostatic or magnetic focusing as well as the inclusion of input/output couplers.

Kory, Carol L.↗