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At least 235 records · Page 13

Enhancement and Saturation of Near-Field Radiative Heat Transfer in Nanogaps between Metallic Surfaces

Near-field radiative heat transfer (NFRHT) between planar metallic surfaces was computationally explored over five decades ago by Polder and van Hove [Phys. Rev. B 4, 3303 (1971)]. These studies predicted that, as the gap size (d) between the surfaces decreased, the radiative heat flux first increases by several orders of magnitude until d is ~100 nm after which the heat flux saturates. However, despite both the fundamental and practical importance of these predictions, the combined enhancement and saturation of NFRHT at small gaps in metallic surfaces remains experimentally unverified. Here, we probe NFRHT between planar metallic (Pt, Au) surfaces and show that RHT rates can exceed the far-field rate by over a thousand times when d is reduced to ~25 nm. More importantly, we show that for small values of d RHT saturates due to the dominant contributions from transverse electric evanescent modes. Finally, our results are in excellent agreement with the predictions of fluctuational electrodynamics and are expected to inform the development of technologies such as near-field thermophotovoltaics, radiative heat-assisted magnetic recording, and nanolithography.

36 MATERIALS SCIENCE↗

Chemo–mechanical properties of carbon fiber reinforced geopolymer interphase

Geopolymers, as a potentially environmentally friendly alternative to Portland cement, are increasingly attracting attention in the construction industry. Various methods have been applied for customizing the properties of geopolymers and improving their commercial viability. One of the promising methods for refining the properties of geopolymers such as their toughness is the use of short fibers. The effectiveness of a high-strength short fiber in the geopolymer matrix is largely dependent on the interfacial bonding between the fiber and its surrounding matrix. While the importance of this interfacial chemistry is highlighted in the literature, the characteristics of this bonding structure have not been fully understood. In this paper, we aim to investigate the bonding mechanism between the carbon fiber and metakaolin-based geopolymer matrix. For the first time, the existence and nature of the chemical bonding at the interfacial region (interphase) between carbon fiber and geopolymer matrix has been revealed. X-ray pair distribution function computed tomography (PDF-CT), field emission-scanning electron microscopy imaging, and nanoindentation techniques are employed to discern the chemo-mechanical properties of the interphase. PDF-CT results show the emergence of a new atom-atom correlation at the interfacial region (around 1.82 angstrom). This correlation is a characteristic of interfacial bonding between the fiber and its surrounding matrix, where the existence of chemical linkages (potentially Al-V-O-C) between fibers and the matrix contributes to the adhesion between the two constituents making up the composite. Due to such chemical bonding, the nanomechanical properties of the interfacial region fall between that of the carbon fiber and geopolymer. The combination of advanced techniques is proved useful for enhancing our understanding of the interfacial chemistry between fibers and the binding matrix. This level of knowledge facilitates the engineering of composite systems through the manipulation of their nanostructure.

36 MATERIALS SCIENCE↗

High-current electron sources for Superconducting Radiofrequency injectors

Accelerators are finding increasing use in numerous fields such as medicine, industry accelerator-based nuclear energy programs and others. A recent survey reveals only 20 high-energy accelerators worldwide serve elementary-particle physics while thousands of accelerators are routinely used in hospitals and industry (packaging, food sterilization, etc.).

43 PARTICLE ACCELERATORS↗

2024 OES-Environmental 2024 State of the Science Report, Chapter 9: Beyond Single Marine Renewable Energy Devices: A System-wide Effects Approach

Global expansion of renewable energy, including marine renewable energy (MRE) technology development is necessary to mitigate the effects of climate change, facilitate a sustainable transition from carbon-based energy sources, and satisfy national energy security needs using locally produced electricity (European Commission 2022; IPCC 2023; IRENA 2020). As MRE engineering and research continue to focus on designing devices for deployment in nearshore and offshore waters around the world, researchers are also examining potential environmental effects on marine animals, habitats, and ecosystem processes. To date, the focus has been on interactions between small numbers of MRE devices (1-6) and the environment, such as collisions between animals and turbine blades, the effects of underwater noise and electromagnetic field (EMF) emissions, changes in habitats and oceanographic processes, risk of entanglement of animals, and displacement of animals (Boehlert & Gill 2010; Copping & Hemery 2020) (see Chapter 3).

16 TIDAL AND WAVE POWER↗

Advanced Diagnostics of Broad Spectrum Multipactor

Multipactor is a resonance event between electron emission and RF fields causing exponential secondary electron re-emission growth when the secondary electron yield of the primary electron impact energy exceeds unity. Multipactor is a serious problem in vacuum electron devices (VEDs) such as particle accelerators, radars, electronic warfare systems, directed energy devices, and even Hall effect thrusters. It also poses an even greater threat to space communication systems where high power, multi-channel links are required. The UC Davis and SLAC team will conduct basic research to advance the fundamental understanding of multipactor physics by developing and carrying out full spectrum, radio frequency (RF) laboratory tests aimed at understanding both single and two-surface multipactor phenomena and at evaluating novel multipactor mitigation approaches for accelerator, space-based RF systems, as well as high power microwave (HPM) applications.

36 MATERIALS SCIENCE↗

A complete catalogue of broad-line AGNs and double-peaked emission lines from MaNGA integral-field spectroscopy of 10K galaxies: stellar population of AGNs, supermassive black holes, and dual AGNs

We analyse the integral field spectroscopy data for the ≈10 000 galaxies in final data release of the MaNGA survey. We identify 188 galaxies for which the emission lines cannot be described by single Gaussian components. These galaxies can be classified into (1) 38 galaxies with broad $\rm H\alpha$ and [O III] $\rm \lambda$5007 lines, (2) 101 galaxies with broad $\rm H\alpha$ lines but no broad [O III] $\rm \lambda$5007 lines, and (3) 49 galaxies with double-peaked narrow emission lines. Most of the broad-line galaxies are classified as active galactic nuclei (AGNs) from their line ratios. The catalogue helps us further understand the AGN-galaxy coevolution through the stellar population of broad-line region host galaxies and the relation between broad lines’ properties and the host galaxies’ dynamical properties. The stellar population properties (including mass, age, and metallicity) of broad-line host galaxies suggest there is no significant difference between narrow-line Seyfert-2 galaxies and Type-1 AGNs with broad $\rm H\alpha$ lines. We use the broad-$\rm H\alpha$ line width and luminosity to estimate masses of black hole in these galaxies, and test the MBH–σe relation in Type-1 AGN host galaxies. Furthermore, we find three dual AGN candidates supported by radio images from the VLA FIRST survey. This sample may be useful for further studies on AGN activities and feedback processes.

79 ASTRONOMY AND ASTROPHYSICS↗

Neutrino Emissivities as a Probe of the Internal Magnetic Fields of White Dwarfs

Abstract The evolution of white dwarfs (WDs) depends crucially on thermal processes. The plasma in their core can produce neutrinos that escape from the star, thus contributing to the energy loss. While in the absence of a magnetic field the main cooling mechanism is plasmon decay at high temperature and photon surface emission at low temperature, a large magnetic field in the core hiding beneath the surface even of ordinary WDs, and undetectable to spectropolarimetric measurements, could potentially leave an imprint in the cooling. In this paper, we revisit the contribution to WD cooling stemming from neutrino pair synchrotron radiation and the effects of the magnetic field on plasmon decay. Our key finding is that even if observations limit the magnetic field strength at the stellar surface, magnetic fields in the interior of WDs—with or without a surface magnetic field—can be strong enough to modify the cooling rate, with neutrino pair synchrotron emission being the most important contribution. This effect may not only be relevant for the quantification and interpretation of cooling anomalies, but suggests that the internal magnetic fields of WDs should be smaller than ∼ 6 × 10 11 G, slightly improving bounds coming from a stability requirement. While our simplified treatment of the WD structure implies that further studies are needed to reduce the systematic uncertainties, the estimates based on comparing the emissivities illustrate the potential of neutrino emission as a diagnostic tool to study the interior of WDs.

79 ASTRONOMY AND ASTROPHYSICS↗

Impact of strong magnetization in cylindrical plasma implosions with applied B-field measured via x-ray emission spectroscopy

Magnetization is a key strategy for enhancing inertial fusion performance, though accurate characterization of magnetized dense plasmas is needed for a better comprehension of the underlying physics. Measured spectra from imploding Ar-doped D 2 -filled cylinders at the OMEGA laser show distinctive features with and without an imposed magnetic field. A multizone spectroscopic diagnosis leads to quantitative estimates of the plasma conditions, namely revealing a 50% core temperature rise at half mass density when a 30-T seed field is applied. Concurrently, experimental spectra align well with predictions from extended-magnetohydrodynamics simulations, providing strong evidence that the attained core conditions at peak compression are consistent with the impact of a 10-kT compressed field. These results pave the way for the validation of magnetized transport models in dense plasmas and for future magnetized laser implosion experiments at a larger scale. Published by the American Physical Society 2024

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Changes in soil pore structure generated by the root systems of maize , sorghum and switchgrass affect in situ N 2 O emissions and bacterial denitrification

Due to the heterogeneous nature of soil pore structure, processes such as nitrification and denitrification can occur simultaneously at microscopic levels, making prediction of small-scale nitrous oxide (N 2 O) emissions in the field notoriously difficult. We assessed N 2 O+N 2 emissions from soils under maize (Zea mays L.), switchgrass (Panicum virgatum L.), and energy sorghum (Sorghum bicolor L.), three potential bioenergy crops in order to identify the importance of different N 2 O sources to microsite production, and relate N 2 O source differences to crop-associated differences in pore structure formation. The combination of isotopic surveys of N 2 O in the field during one growing season and X-ray computed tomography (CT) enabled us to link results from isotopic mappings to soil structural properties. Further, our methodology allowed us to evaluate the potential for in situ N 2 O suppression by biological nitrification inhibition (BNI) in energy sorghum. Our results demonstrated that the fraction of N 2 O originating from bacterial denitrification and reduction of N 2 O to N 2 is largely determined by the volume of particulate organic matter occluded within the soil matrix and the anaerobic soil volume. Bacterial denitrification was greater in switchgrass than in the annual crops, related to changes in pore structure caused by the coarse root system. This led to high N-loses through N 2 emissions in the switchgrass system throughout the season a novel finding given the lack of data in the literature for total denitrification. Isotopic mapping indicated no differences in N 2 O-fluxes or their source processes between maize and energy sorghum that could be associated with the release of BNI by the investigated sorghum variety. The results of this research show how differences in soil pore structures among cropping systems can determine both N 2 O production via denitrification and total denitrification N losses in situ.

59 BASIC BIOLOGICAL SCIENCES↗

Integrating collapsible plasmonic gaps on near-field probes for polarization-resolved mapping of plasmon-enhanced emission in 2D material

Scanning near-field optical microscopy (SNOM) is an important technique used to study the optical properties of material systems at the nanoscale. In previous work, we reported on the use of nanoimprinting to improve the reproducibility and throughput of near-field probes including complicated optical antenna structures such as the ‘campanile’ probe. However, precise control over the plasmonic gap size, which determines the near-field enhancement and spatial resolution, remains a challenge. Here, we present a novel approach to fabricating a sub-20 nm plasmonic gap in a near-field plasmonic probe through the controlled collapse of imprinted nanostructures using atomic layer deposition (ALD) coatings to define the gap width. The resulting ultranarrow gap at the apex of the probe provides a strong polarization-sensitive near-field optical response, which results in an enhancement of the optical transmission in a broad wavelength range from 620 to 820 nm, enabling tip-enhanced photoluminescence (TEPL) mapping of 2-dimensional (2D) materials. We demonstrate the potential of this near-field probe by mapping a 2D exciton coupled to a linearly polarized plasmonic resonance with below 30 nm spatial resolution. This work proposes a novel approach for integrating a plasmonic antenna at the apex of the near-field probe, paving the way for the fundamental study of light-matter interactions at the nanoscale.

Zhou, Junze (ORCID:000000020682767X)↗

Excessive charge, beam loading, and impedance collapse thresholds for a velvet emitter

Excess emission has been observed from velvet cathodes with total emission times >150 ns. In this diode experiment, we produce a sub-relativistic electron beam with the ability to consistently change γ from 1.2 to 1.5 and β = 0.5–0.75. Electron emission in this particular diode geometry requires electric fields >40 kV/cm. The current increases at steady rates >0.05 A/ns after the head of the pulse, indicating an expansion of the emission surface and reduction in the effective AK gap. Small transients of excess emission (or arcs) are consistently observed for current pulses exceeding 150 ns. The excess emission results in beam loaded levels ≥10 kV on the diode voltage. The effects described here are compounded as diode voltage is increased. The principal objective of these experiments is to quantify electric field emission thresholds, current ramps, excess emission delays, effective beam loading, and impedance collapse.

43 PARTICLE ACCELERATORS↗

Intergalactic magnetic field studies by means of γ -ray emission from GRB 190114C

The presence of delayed GeV emission after a strong transient, such as a gamma-ray burst (GRB), in the very-high energy (VHE) E > 100 GeV band can be the signature of a nonzero magnetic field in the intergalactic medium. Here we used a synchrotron self-Compton multiwavelength model to infer an analytical description of the intrinsic VHE spectrum (corrected for absorption by the extragalactic background light) of GRB 190114C to predict the light curves and spectral energy distributions of the delayed emission with Monte Carlo simulations for different intergalactic magnetic field (IGMF) configurations (strengths B = 8 × 10 -21 G, 10 -20 G, 3 × 10 -20 G and correlation length $\lambda$ > 1 Mpc), and compared them with the Fermi Large Area Telescope (Fermi LAT) limits computed for several exposure times. We found that the Fermi LAT is not sensitive enough to constrain any IGMF strengths using GRB 190114C.

79 ASTRONOMY AND ASTROPHYSICS↗

Tailoring composition and deformation modes at the microstructural level for next generation low-cost high-strength austenitic stainless steels

The objective of this project is to enable deliberate development of cost-effective, hydrogen resistant alloys by establishing detailed relationships specific to the effects of alloy composition, short-range order (SRO), and microsegregation in the presence of hydrogen on the transition between homogeneous deformation and localized plasticity in shear bands. In collaboration with the International Institute for Carbon-Neutral Energy Research, I2CNER, at Kyushu University in Japan, we conceptualized, designed, and manufactured four austenitic alloys that maintain corrosion resistance and ensure lower cost relative to baseline commercial alloys. The mechanical properties and deformation modes of the novel alloys (KU alloys) were assessed in the presence of hydrogen (H). Correlations between composition and performance revealed that two of the KU alloys are suitable replacements for 316 steel, while another is a viable replacement for 304 steel at room temperature. We found that, in the presence of other austenite stabilizing elements namely Mn and N, replacing Ni with Cu does not lead to martensite formation as has been previously reported.1–3 Furthermore, we found that the addition of Cu leads to an earlier onset of multiple slip resulting in an relative earlier onset of a higher work hardening rate (WHR). Greater understanding of the relationships between alloy composition and SRO required the development of a novel advanced electron diffraction methodology to characterize SRO in complex FCC alloys. This innovative approach, which combines fluctuation and correlation analyses of diffuse-scattering signals, successfully differentiated between SRO and long-range ordering (LRO). Further investigations into annealed austenitic stainless steels could provide insights into manipulating SRO and its effects on material properties. Atomistic simulations provided understanding of SRO behavior that was difficult to capture experimentally. This project created the first spin cluster expansion model that is able to capture and describe SRO effects in Fe-Ni-Cr FCC alloys, accounting for the non-negligible effects of magnetism. An automated computational workflow was established to provide reliable predictions of SRO in Fe-Ni-Cr austenitic alloys, both with and without the presence of H atoms. Analysis of the propensity for SRO in Fe-Ni-Cr alloys revealed that H tends to cluster with specific, well-defined SRO domains. The computational framework is general purpose and can be extended to realistic stainless steels across diverse composition ranges. With confidence that SRO is possible in austenitic stainless steels, we developed a discrete dislocation finite element code to understand the interaction of dislocations with SRO in the presence of H. By incorporating H effects on the dislocation emission and SRO stress field we show that the critical stress for the dislocation pileup to breakthrough the SRO domain decreases in the presence of H, which directly contributes localized deformation at the macroscale. Through the simulation of a uniaxial tension test, we demonstrated that H-induced weakening of SRO stress field and H-enhanced dislocation emission can lead to the onset of shear localization at lower macroscopic strains. As a whole, this project identified three novel alloys that show improvements in performance and cost efficiency for H-facing applications by studying correlations between alloy chemistry and deformation behavior. We also made significant advancements to experimental and computational methodologies necessary to study the chemistry and distribution of SRO across a range of alloys, which in turn allowed us to demonstrate how deformation mechanisms change due to the contributions of SRO in austenitic alloys in the presence of H. The combined advancements in fundamental understanding with novel alloy development in this project has increased the viability of next generation H-technologies for the broader public through accessible low-cost alloys and accelerated development towards future H-infrastructure.

08 HYDROGEN↗

Radius-to-frequency Mapping and FRB Frequency Drifts

We build a model of radius-to-frequency mapping in magnetospheres of neutron stars and apply it to frequency drifts observed in fast radio bursts (FRBs). We assume that an emission patch propagates along the dipolar magnetic field lines, producing coherent emission with frequency, direction, and polarization defined by the local magnetic field. The observed temporal evolution of the frequency depends on the relativistic effects of time contraction and the curvature of the magnetic field lines. The model generically produces linear scaling of the drift rate, $\dot{\omega}$ ∝-${\omega}$, matching both numerically and parametrically the rates observed in FBRs; a more complicated behavior of $\dot{\omega}$ is also possible. Fast rotating magnetospheres produce higher drifts rates for similar viewing parameters than the slowly rotating ones. In the case of repeaters, the same source may show variable drift patterns depending on the observing phase. We expect rotational of polarization position angle through a burst, though by smaller amount than in radio pulsars. All of these findings compare favorably with properties of FBRs, strengthening their possible loci in the magnetospheres of neutron stars.

Magnetars↗

Lightwave-driven electron emission for polarity-sensitive terahertz beam profiling

The full exploitation of advanced light sources in the terahertz (THz) frequency range requires versatile experimental tools to fully characterize the spatial, temporal, and spectral shapes of the THz electric field. Several techniques for passive THz beam profiling exist that offer information about the temporally integrated intensity. Thus, any information about the electric field itself is lost. Here, we show that a UV–visible light emission produced via a lightwave-driven field emission from single-layer metasurfaces can be used to visualize the peak electric field distribution of THz beams in real time. Our technique is scalable up to frequencies approaching the plasma frequency of the metal used for the metasurface. Uniquely, our device is sensitive to the absolute polarity of the THz lightwave. These findings demonstrate a general pathway to designing metamaterial-based field-sensitive optical detectors suitable for the entire THz and IR spectral region.

42 ENGINEERING↗

Precipitation and nitrogen application stimulate soil nitrous oxide emission

Precipitation and nitrogen (N) fertilization are the two most important drivers for soil nitrous oxide (N 2 O) emission. However, the effects of changes in N fertilization and precipitation patterns (i.e., precipitation intensity and frequency) on N 2 O emissions in agricultural fields are still unclear. In this study, we simulated soil N 2 O emission under different precipitation patterns (6 precipitation intensities, and 12 precipitation frequencies by either merging or splitting precipitation events) and N fertilization rates (low, typical, and high N fertilization) in a cornfield using the DeNitrification-DeComposition model. The model was parameterized and validated using meteorological data and N experimental measurements in Nashville, Tennessee, USA. Results showed that soil water filled pore space (WFPS) and simulated soil N 2 O emission increased as precipitation intensity increased. Less frequent but high intensity precipitation treatments reduced the soil WFPS by 25.2% and stimulated soil N 2 O emission by 45.3%, while more frequent but low intensity precipitation treatments increased soil WFPS by 9.0% and reduced soil N 2 O emission by 23.9%. Compared to typical N fertilization, the sensitivity of soil N 2 O emission to precipitation was higher under high N than low N fertilization treatments, and the response ratios were 50.0% and 40.1%, respectively. There was significant interactive effect of precipitation intensity and N fertilization on soil N 2 O emission. Furthermore, these findings improved our understanding of precipitation and N impacts on soil N 2 O emissions and provided useful knowledge for irrigation and N fertilizer management in agriculture to mitigate greenhouse gas emissions.

54 ENVIRONMENTAL SCIENCES↗