Design Optimization of the Transformational Challenge Reactor Outlet Plenum
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22 GENERAL STUDIES OF NUCLEAR REACTORS↗
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Quantum decoherence by Coulomb interaction
The performance of modern quantum devices in communication, metrology or microscopy relies on the quantum-classical interaction which is generally described by the theory of decoherence. Despite the high relevance for long coherence times in quantum electronics, decoherence mechanisms mediated by the Coulomb force are not well understood yet and several competing theoretical models exist. Here, we present an experimental study of the Coulomb-induced decoherence of free electrons in a superposition state in a biprism electron interferometer close to a semiconducting and metallic surface. The decoherence was determined through a contrast loss at different beam path separations, surface distances and conductibilities. To clarify the current literature discussion, four theoretical models were compared to our data. We could rule out three of them and got good agreement with a theory based on macroscopic quantum electrodynamics. The results will enable the determination and minimization of specific decoherence channels in the design of novel quantum instruments.
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
Photoelectron spectroscopy of CsK2Sb photocathode at Synchrotron Radiation Facility using vacuum transport system
As accelerators and electron microscopes become more advanced, high-performance photocathodes are required. In particular, Cesium potassium antimonide (CsK 2 Sb) photocathode is of interest because of its low emittance, excitability in visible light, and high quantum efficiency (QE). The challenge is its high susceptibility to environment that lead to low operating vacuum pressure and short lifetime/low extraction charge. To resolve these issues, it is necessary to understand the molecular structure of the cathode and its degradation mechanism. In this study, we transported CsK 2 Sb photocathode to a beamline of synchrotron radiation facility using a vacuum transport system for molecular structure analysis. Specifically, the cathode was deposited in an evaporation system at Nagoya University. We transported it to Aichi Synchrotron Radiation Center (Aichi SR) located 15 km away, and analyzed it in the depth direction by X-ray photoelectron spectroscopy (XPS) at BL7U. Based on the results, we quantitatively evaluated the composition ratios and stoichiometry of the cathode elements (Sb, K, Cs). A Cs ex-cess state of surface was observed at the surface, and it is consistent with previous studies. The intended atomic structure of CsK 2 Sb was formed only at a few nanometres of the surface on the Mo substrate. On the other hand, the CsK 2 Sb cathode structure on the graphene substrate was preserved further in the depth direction.
47 OTHER INSTRUMENTATION↗
Production and testing of the powerboard for ATLAS ITk Strip barrel modules
The upgrade of the ATLAS ITk strips detector for HL-LHC will employ a custom PCB (powerboard) for on-module DC-DC conversion, HV switching, and monitoring. Production of about 14100 of such PCBs with high reliability is a big challenge. In this paper we will present the production procedure and quality control (QC) testing system for the powerboards to be installed on ITk Strip barrel modules. During production, about 150 powerboards will be produced every week. Each powerboard will need to pass QC tests before they are assembled to module. The QC tests include thermal cycling between -35 °C and 40 °C, soak test (continuous running of DC-DC converter at high load at 20 °C), and basic functionality and characterization electrical tests of the low voltage (LV), high voltage (HV), and monitoring functions of the powerboard. A custom QC test system is described, which is based on a reusable PCB (active board) with all testing circuits, a one-time powerboard carrier card, and a Z-turn SoC board which hosts and runs the testing program. The production procedure and QC test system has been tested with 400 powerboards during pre-production, and the system has been proven ready for production with the desired testing program, speed, safety, and cost. Performance and typical failures of powerboards observed during the QC test of pre-production powerboards is also presented.
47 OTHER INSTRUMENTATION↗
DRiFT - Release 1.0.0 Organic Scintillators
DRiFT (a Detector Response Function Toolkit) is LANL-developed software that postprocesses output from the extensively validated radiation transport code, MCNP [1], and generates realistic nuclear instrumentation response. DRiFT is designed to be flexible, enabling users to specify detector type and many experimental settings, as well as accommodating the addition of their own desired features. Although DRiFT development has included scintillator [2], gas [3], and semiconductor features [4], the focus of this release is on organic scintillator and associated capabilities. Organic scintillators are widely used in the areas of nuclear safeguards and nuclear non-proliferation efforts [5, 6]. DRiFT has several diagnostic and detector physics features relevant to detailed scintillator simulations including: tracking source particle information, scintillation light production, the effects of PMT quantum efficiency and gain, and digitizer settings. Users can select responses from many scintillator and PMT types supported natively by DRiFT, or add their own by following the instructions in this document. We acknowledge that DRiFT is under active development, bug reports and general questions and comments should be directed to Madison Andrews, madison@lanl.gov. This manual is divided into four parts: I) An overview of DRiFT, including how to obtain and install the executable, II) A description of the detector physics related to scintillators available, III) a description of more general DRiFT features the user may find useful, and IV) a description of the test suite and examples made available with the code release.
61 RADIATION PROTECTION AND DOSIMETRY↗
Contactless Position Measurement System for Remote Alignment of Highly Reflective Objects
The Contactless Position Measurement System (CPMS) permits automatic alignment of highly-reflecting components that cannot or should not be touched by human hands, such as those used in SRF cavities. CPMS also has application during maintenance of fusion reactors, when the components in the reactor are radioactive. The length of time for which humans can handle the components in order to carry out maintenance or repairs is limited. We would like to measure the relative positions of such objects so we can bring them into alignment with motorized stages, thus eliminating the need for human contact. The CPMS is a computer vision system that measures the location of highly reflective components to within a fraction of a millimeter by finding the edges of silhouette images. This is done by placing a uniform, infrared backlight behind the components, and viewing each component with two low-aberration, infrared cameras. Each of these stereoscopic cameras are located within a coordinate system we set up with reference platforms, light sources, and survey cameras distributed around the perimeter of the string assembly room, or fusion reactor. We obtain stereoscopic silhouette images of each component, and we use these to determine the position of the component within our string assembly coordinate system. The CPMS combines the silhouette images with knowledge of the dimensions of the objects to obtain the relative positions of components in its field of view. These position measurements then allow us to mechanically maneuver the components into contact. Once we know where they are, we can move the components to where they are supposed to be with motorized stages or other mechanical means, check they are in the right place, and bolt them together. In Phase I, we built a prototype infrared backlights and cameras, tested it, wrote an analysis program to fit the images. At a range of 50 cm, we are able to measure the relative positions of two stainless steel flanges with an accuracy of 150 μm rms. The next steps are to test the analysis program with motorized stages, build a full-size prototype, and implement it in an cleanroom with SRF cavity assembly. This can be done in a cost effective way given the materials with which the system is designed. As Open Source Instruments achieved more in Phase I than anticipated, despite not receiving a Phase II SBIR grant, we hope to move forward with product development and sales with a testing partner.
43 PARTICLE ACCELERATORS↗
Open-Source Tidal Energy Converter (OSTEC) Testbed: Design Basis Report
This report describes the design basis and design details for an instrumented marine turbine system intended to serve as the DOE’s marine tidal turbine test bed for foundational open-source R&D and data generation to advance our understanding and to identify knowledge gaps on the techno-economic performance of tidal energy converters (TEC) under real tidal flow conditions and at sufficiently large scale to enable upscaling of fluid-structure-interactions and component and material load responses
16 TIDAL AND WAVE POWER↗
Fluorescence-Based Aqueous Phosphate Sensing Using Eu(cpboda)(DMF) 2
Fluorescence-based phosphate sensing using phosphate-sensitive phosphors is a promising approach for in situ monitoring of phosphate pollution in waterways and reservoirs. To date, the most sensitive phosphor developed for this purpose is Tb(cpboda)(DMF) 2 , where cpboda = (3,3'-((5-Carboxy-1,3-phenylene)bis(oxy))dibenzoic acid). In this study, we further improve this sensitivity by replacing the Tb 3+ ions with Eu 3+ ions to make Eu(cpboda)(DMF) 2 and find concentration-independent phosphate-sensitivity of 1570 ± 120, which is ≈8× more sensitive than the Tb-version. This improvement is attributed to Eu 3+ having a hypersensitive transition, while Tb 3+ does not. Additionally, we characterize the phosphor’s optical properties, photodegradation, and water solubility. We find that the phosphor presents challenges with regards to both photodegradation and solubility, as it is found to be poorly soluble in water and is quickly photodegraded under UV radiation <360 nm. However, these obstacles can, in theory, be overcome with the use of direct excitation of the Eu 3+ ions at 394 nm and careful design of an analysis instrument to reduce concentration variations.
37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
AGR-5/6/7 Irradiation As Run Predictions Using PARFUME
The PARticle FUel ModEl (PARFUME), a fuel performance modeling code used for high-temperature gas-cooled reactors, was used to model the Advanced Gas Reactor (AGR)-5/6/7 irradiation test using as-run physics and thermal data. The AGR-5/6/7 irradiation test consists of the combined fifth, sixth, and seventh planned irradiations of the AGR Fuel Development and Qualification Program. The AGR-5/6/7 test train is a multi-capsule, instrumented experiment that is designed for irradiation in the 133.4-mm diameter northeast flux trap position of the Advanced Test Reactor (ATR) at Idaho National Laboratory. Each capsule contains compacts filled with uranium oxycarbide unaltered fuel particles. This report documents the calculations performed to predict the failure probability of tristructural isotropic (TRISO)-coated fuel particles during the AGR-5/6/7 experiment. In addition, this report documents the calculated fission product release fraction from the fuel. The calculations include modeling of the AGR 5/6/7 irradiation that occurred from February 2018 to July 2020 over nine ATR cycles, including six normal cycles and three power axial locator mechanism cycles, for a total of approximately 376 effective full power days (EFPD). The irradiation conditions and material properties of the AGR-5/6/7 test predicted zero fuel particle failures in Capsules 1, 3, and 4. Fuel particle failures were predicted in two of the compacts in Capsule 2 and one particle failure is predicted in each one of the compacts in Capsule 5. All compacts that exhibited fuel particle failures predicted by PARFUME were caused by localized stress concentrations in the silicon carbide (SiC) layer caused by cracking in the inner pyrolytic (IPyC) layer. In addition, shrinkage of the buffer and IPyC layer during irradiation resulted in formation of a buffer-IPyC gap. Compacts with a lower irradiation temperature and fluence experienced the smallest buffer-IPyC gap formation. Conversely, higher irradiated temperature compacts with a high fluence experienced the largest buffer-IPyC gap formation. Compact 3-6-3 experienced the largest buffer IPyC gap formation of just under 21.7 µm. The release fraction of fission products silver (Ag), cesium (Cs), and strontium (Sr) vary depending on capsule location and irradiation temperature. The maximum release fraction of Ag occurs in Capsule 3, reaching up to 59.5% for the TRISO fuel particles (compact 3-6-3). The release fraction of the other two fission products, Cs and Sr, are much smaller. A maximum Cs release fraction of 1.1% occurred in compact 3-4-3 and 4.4% for Sr in compact 3-6-3.
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
Equivalent Breakeven Installed Cost: A Tradeoff-Informed Measure for Technoeconomic Analysis of Candidate Heliostat Improvements: Preprint
Technoeconomic analysis (TEA) is commonly used to determine economic viability of power-generating technologies, including concentrating solar power (CSP) and thermal (CST) production plants. Levelized cost of electricity (LCOE) and analogous measures provide an estimate of long-term costs for operating power plants over their designed lifetimes by accounting for revenues and costs in a time-discounted manner. While these measures are effective when assessing a technology's total lifecycle costs and productivity under various designs, TEA of candidate incremental technology improvements from the lens of LCOE can be limited when required investment and LCOE impacts are small. In this work, we propose a novel metric for TEA of a plant component technology that recasts relative changes in levelized system costs into component-specific capital cost budgets. This measure, which we refer to as the equivalent breakeven installed cost, is the maximum budget for the technology component that leads to improved levelized costs. We illustrate the usefulness of this metric using the example of candidate heliostat improvements for a CSP tower plant. Here, the results suggest that a reduction in mirror washing costs yield a total plant O&M cost of $37/kWe-yr, which is a breakeven proposition if the average reflectance is reduced from 0.90 to 0.85 as a result of the cost savings.
concentrating solar power↗
Bicep/Keck XV: The Bicep3 Cosmic Microwave Background Polarimeter and the First Three-year Data Set
Abstract We report on the design and performance of the B icep3 instrument and its first three-year data set collected from 2016 to 2018. B icep3 is a 52 cm aperture refracting telescope designed to observe the polarization of the cosmic microwave background (CMB) on degree angular scales at 95 GHz. It started science observation at the South Pole in 2016 with 2400 antenna-coupled transition-edge sensor bolometers. The receiver first demonstrated new technologies such as large-diameter alumina optics, Zotefoam infrared filters, and flux-activated SQUIDs, allowing ∼10× higher optical throughput compared to the Keck design. B icep3 achieved instrument noise equivalent temperatures of 9.2, 6.8, and 7.1 μ K CMB s and reached Stokes Q and U map depths of 5.9, 4.4, and 4.4 μ K arcmin in 2016, 2017, and 2018, respectively. The combined three-year data set achieved a polarization map depth of 2.8 μ K arcmin over an effective area of 585 square degrees, which is the deepest CMB polarization map made to date at 95 GHz.
79 ASTRONOMY AND ASTROPHYSICS↗
Sensitivity and Importance Measure Analyses for Various Design Architectures for High Safety-Significant Safety-Related Digital Instrumentation and Control Systems of Nuclear Power Plants
A transition from analog instrumentation and control (I&C) technologies to digital I&C technologies is taking place for license renewals of existing nuclear power plants and for operating licenses of new advanced reactors. This transition necessitates research on risk and economic assessments of digital I&C technologies to ensure the long-term safety and reliability of vital systems, reduce uncertainty in licensing costs in addition to timeline, support integration of digital I&C systems in the plant, and find the most efficient technology upgrades. Adding redundancy within systems or components is a common means of improving design safety; however, it can also make designs more prone to common-cause failures (CCFs). Introducing diversity into redundant systems or components is a way to mitigate and possibly eliminate CCFs, but it also increases plant complexity and may be costly. The balance between redundancy and diversity remains a challenge for digital I&C systems. This study performs sensitivity and importance analyses for four design architectures of two digital I&C systems—the reactor-trip system and the engineered safety features actuation system. For each system, two architectures are examined, including a redundant, non-diverse configuration and a redundant, diverse configuration. The sensitivity analysis will provide insights on the impact of introducing diversity to system reliability. The importance results will help identify risk-significant and risk-sensitive components and failure modes, which may be good candidates for future design improvement.
99 GENERAL AND MISCELLANEOUS↗
mystic : software for autonomous discovery and design under uncertainty
Throughout the diverse range of science and engineering applications, there is a growing desire to develop computational methods that can reliably predict the behavior of complex systems. Specifically, there is a strategic need for tools that can robustly forecast the behavior of complex physical systems, where data may be high-dimensional, noisy, or sparse, and models of the system may be time-dependent or include uncertainty. We use mystic to build tools that leverage statistical learning, physics-informed learning, and active learning in the efficient generation of reliably predictive surrogates for complex physical systems. mystic is a robust, proven, open-source optimization and uncertainty quantification toolkit with over a decade of use in the design and optimization of neutron instrumentation, solar-powered drones, and gasguns, and in iterative tuning of models for Raman spectroscopy and elastoplastic materials strength. Recent developments have focused on automated learning of statistically robust surrogates under uncertainty, with applications in materials in extreme environments, nanostructures, materials simulations and strength models, and the failure of shielding under particle radiation. In 2020, McKerns demonstrated active learning of optimally robust surrogates with respect to new simulated data for molecular dynamics simulations of materials mixing in warm dense matter, and is currently applying active learning to the automated steering of particle accelerator beams and the optimal design and control of quantum optical sensor instrumentation.
42 ENGINEERING↗
Kilonova Detectability with Wide-Field Instruments [Slides]
A diverse set of instruments increase the chances of detecting and identifying a kilonova. Early observations increase the probability of detection. More sensitive wide-field ultraviolet instruments are needed as GW detectors reach design sensitivity. There is a dearth of wide-field infrared instruments. These results are useful for guiding kilonova searches following a GW detection and sGRD observation, proposals for time on current and upcoming instruments, and planning future wide-field instruments.
79 ASTRONOMY AND ASTROPHYSICS↗
Kilonova Detectability with Wide-Field Instruments
A diverse set of instruments increase the chances of detecting and identifying a kilonova. Early observations increase the probability of detection. More sensitive wide-field ultraviolet instruments are needed as GW detectors reach design sensitivity. There is a dearth of wide-field infrared instruments.
79 ASTRONOMY AND ASTROPHYSICS↗
Conceptual Design of Passive Neutron Albedo Reactivity and Active Neutron Albedo Reactivity Instruments for Various Arrangements of Pebble Bed Reactor Pebbles
MCNP6 simulations were performed to assess the anticipated capability of the Passive Neutron Albedo Reactivity technique for nuclear safeguards measurements of irradiated pebble/pebbles. Two physical setups were examined. One with a single pebble of three different burnups and one with 27 pebbles in a cube. For all cases the sensitivity to removing all the fissile material was examined. For both of the physical setups, 4 assay cases were examined: (a) singles count rates for which the only source neutrons were the inherent neutrons in the fuel, (b) singles count rates again except this time two relatively weak AmLi sources were placed above and below the top central pebble and the combined effect of both neutron source terms were examined, (c) doubles count rates for which the only source neutrons were the inherent neutrons in the fuel, and (d) doubles count rates again except this time two relatively weak AmLi sources were placed above and below the top central pebble and the combined effect of both neutron source terms were examined. Finally, a few parameters such as Cd near the 3 He tubes were perturbed to see if the results could be improved.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Evolution of LIBS technology to mobile instrumentation for expediting firearm-related investigations at the laboratory and the crime scene
Gunshot residue (GSR) is one of the few forensic disciplines that lack accurate screening techniques. This study proposes using a mobile LIBS instrument to detect inorganic GSR and compares performance to a previously validated laboratory instrument. The mobile LIBS is designed with advanced configurations specifically for on-site GSR analysis, including a CMOS detector and a sampling chamber that holds up to six typical GSR collection devices with separate gas flow ports to prevent cross-contamination. A significant novelty of the portable instrument is its image magnification, which allows quick searching and visualization of GSR particle morphology. The single-particle imaging and elemental composition capability is one of a kind and offers superior confirmatory features for GSR. The mobile LIBS performance was evaluated for residues collected from the hands of shooters (100 samples) and non-shooters (200 background samples), analyzed sequentially by the mobile instrument and then the laboratory instrument. Accuracies better than 98.8% were obtained by both instruments, demonstrating their suitability for trace IGSR detection from skin specimens. Implementation of this methodology is anticipated to drastically speed up response times (i.e., from several hours per sample by standard SEM-EDS practice to a few minutes by LIBS). The screening methods can be easily incorporated into workflows to improve decision-making processes at the crime scene and laboratory settings, reduce backlogs, and improve case management.
47 OTHER INSTRUMENTATION↗