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At least 235 records · Page 13

Energy loss by resonance line photons in an absorbing medium

The mean path length of photons undergoing repeated scatterings in media of large optical thickness is calculated from accurate numerical solutions of the transfer equation including the effect of frequency redistribution characteristic of combined Doppler and natural broadening. Energy loss by continuous absorption processes, such as ionization or dust absorption, is discussed, and asymptotic scaling laws for the energy loss, the mean path length, and the mean number of scatterings are inferred from the numerical data.

Hummer, D. G.↗

Requirements for theoretical models of outflows

Recent observational and theoretical investigations of astrophysical mass outflows are reviewed, with a focus on the basic physical principles. Specific limitations on the observational data and their interpretation are listed and discussed. Modeling problems considered include the role of the critical point in determining the mass-loss rate and terminal velocity, the physical processes controlling density at the critical point, the possible coexistence of multiple mass-loss mechanisms, time scales, instabilities and phase changes, multiphase atmospheres and winds, the definition of geometries, the role of the environment, explosive transient events, stochastic phenomena, mode-mode coupling and damping processes, departures from ionization equilibrium, and nonthermal phenomena.

Linsky, Jeffrey L.↗

A new class of solutions for interstellar magnetohydrodynamic shock waves

An analysis is presented of the equations of motion for steady MHD shock waves proopagating in interstellar clouds, for boundary conditions that preclude C shocks. In addition to J shocks, in which the neutral fluid component becomes subsonic at an adiabatic jump front, the equations admit a new class of solutions, called C-asterisk shocks, in which the transition to subsonic flow occurs continuously at a sonic point. Numerical methods are developed for computing the structure of J and C-asterisk shocks propagating in diffuse interstellar clouds. The effects of chemical, ionization, and recombination processes are included in this treatment. An alternative numerical method, which uses artificial viscosity to facilitate integration through sonic points, is analyzed and shown to be invalid. A set of exemplary solutions, computed for realistic shock parameters, shows that C-asterisk shocks occur for a broad range of conditions relevant to diffuse interstellar clouds.

Roberge, W. G.↗

The computation of thermo-chemical nonequilibrium hypersonic flows

Several conceptual designs for vehicles that would fly in the atmosphere at hypersonic speeds have been developed recently. For the proposed flight conditions the air in the shock layer that envelops the body is at a sufficiently high temperature to cause chemical reaction, vibrational excitation, and ionization. However, these processes occur at finite rates which, when coupled with large convection speeds, cause the gas to be removed from thermo-chemical equilibrium. This non-ideal behavior affects the aerothermal loading on the vehicle and has ramifications in its design. A numerical method to solve the equations that describe these types of flows in 2-D was developed. The state of the gas is represented with seven chemical species, a separate vibrational temperature for each diatomic species, an electron translational temperature, and a mass-average translational-rotational temperature for the heavy particles. The equations for this gas model are solved numerically in a fully coupled fashion using an implicit finite volume time-marching technique. Gauss-Seidel line-relaxation is used to reduce the cost of the solution and flux-dependent differencing is employed to maintain stability. The numerical method was tested against several experiments. The calculated bow shock wave detachment on a sphere and two cones was compared to those measured in ground testing facilities. The computed peak electron number density on a sphere-cone was compared to that measured in a flight test. In each case the results from the numerical method were in excellent agreement with experiment. The technique was used to predict the aerothermal loads on an Aeroassisted Orbital Transfer Vehicle including radiative heating. These results indicate that the current physical model of high temperature air is appropriate and that the numerical algorithm is capable of treating this class of flows.

Candler, Graham↗

A hydrodynamic approach to cosmology - Methodology

The present study describes an accurate and efficient hydrodynamic code for evolving self-gravitating cosmological systems. The hydrodynamic code is a flux-based mesh code originally designed for engineering hydrodynamical applications. A variety of checks were performed which indicate that the resolution of the code is a few cells, providing accuracy for integral energy quantities in the present simulations of 1-3 percent over the whole runs. Six species (H I, H II, He I, He II, He III) are tracked separately, and relevant ionization and recombination processes, as well as line and continuum heating and cooling, are computed. The background radiation field is simultaneously determined in the range 1 eV to 100 keV, allowing for absorption, emission, and cosmological effects. It is shown how the inevitable numerical inaccuracies can be estimated and to some extent overcome.

Cen, Renyue↗

Laser-induced fluorescence detection strategies for sodium atoms and compounds in high-pressure combustors

A variety of laser-induced fluorescence schemes were examined experimentally in atmospheric pressure flames to determine their use for sodium atom and salt detection in high-pressure, optically thick environments. Collisional energy transfer plays a large role in fluorescence detection. Optimum sensitivity, at the parts in 10 exp 9 level for a single laser pulse, was obtained with the excitation of the 4p-3s transition at 330 nm and the detection of the 3d-3p fluorescence at 818 nm. Fluorescence loss processes, such as ionization and amplified spontaneous emission, were examined. A new laser-induced atomization/laser-induced fluorescence detection technique was demonstrated for NaOH and NaCl. A 248-nm excimer laser photodissociates the salt molecules present in the seeded flames prior to atom detection by laser-induced fluorescence.

Weiland, Karen J. R.↗

Momentum deposition on Wolf-Rayet winds: Nonisotropic diffusion with effective gray opacity

We derive the velocity and mass-loss rate of a steady state Wolf-Rayet (WR) wind, using a nonisotropic diffusion approximation applied to the transfer between strongly overlapping spectral lines. Following the approach of Friend & Castor (1983), the line list is assumed to approximate a statistically parameterized Poisson distribution in frequency, so that photon transport is controlled by an angle-dependent, effectively gray opacity. We show the nonisotropic diffusion approximation yields good agreement with more accurate numerical treatments of the radiative transfer, while providing analytic insight into wind driving by multiple scattering. We illustrate, in particular, that multiple radiative momentum deposition does not require that potons be repeatedly reflected across substantial distances within the spherical envelope, but indeed is greatest when photons undergo a nearly local diffusion, e.g., through scattering by many lines closely spaced in frequency. Our results reiterate the view that the so-called 'momentum problem' of Wolf-Rayet winds is better characterized as an 'opacity problem' of simply identfying enough lines. One way of increasing the number of thick lines in Wolf-Rayet winds is to transfer opacity from saturated to unsaturated lines, yielding a steeper opacity distribution than that found in OB winds. We discuss the implications of this perspective for extending our approach to W-R wind models that incorporate a more fundamental treatment of the ionization and excitation processes that determine the line opacity. In particular, we argue that developing statistical descriptions of the lines to allow an improved effective opacity for the line ensemble would offer several advantages for deriving such more fundamental W-R wind models.

Gayley, Kenneth G.↗

Pick-up ion pressure gradients modulating the solar wind dynamics

Neutral interstellar atoms penetrate deeply into the inner heliosphere before they become ionized by various processes. As ions they are picked-up by the frozen-in magnetic fields and are convected outwards with the solar wind plasma. Thereby the primary plasma flow is mass, momentum, and energy-loaded. The dynamics of the distant multi-constituent solar wind is, however, not solely determined by these loading processes, but is also affected by the wave-mediated pick-up ion pressure gradients derivable from the pick-up ion distribution function. The action of the radial components of these pressures essentially counter balances the decelerating effect of the solar wind momentum loading, diminishing strongly the deceleration of the distant solar wind. Furthermore the latitudinal components of the pick-up ion pressures induce latitudinal forces acting on the multiconstituent solar plasma outflow and inducing nonradial bulk flow components. The enforced nonradial outflow geometry on the upwind hemisphere may partly be responsible for the magnetic flux deficit which was claimed since several years in the PIONEER-10 magnetic flux data.

Fahr, Hans J.↗

Competition Effect in Atomic-Molecular System

The competition effects among the processes of atomic ionization, optical pumped stimulated radiation (OPSR), four-wave frequency mixing (FWFM) and molecular stimulated diffuse band radiation at the atomic two-photon resonance of 3S approaches 4D in Na2 - Na mixture were observed. The dip at the two-photon resonance in the excitation spectrum for the diffuse-band radiation was interpreted as suppression of population in 4D state.

Jia, Suotang↗

Laser Lightcraft Performance

The purpose of this study is to establish the technical ground for modeling the physics of laser powered pulse detonation phenomenon. The principle of the laser power propulsion is that when high-powered laser is focused at a small area near the surface of a thruster, the intense energy causes the electrical breakdown of the working fluid (e.g. air) and forming high speed plasma (known as the inverse Bremsstrahlung, IB, effect). The intense heat and high pressure created in the plasma consequently causes the surrounding to heat up and expand until the thrust producing shock waves are formed. This complex process of gas ionization, increase in radiation absorption and the forming of plasma and shock waves will be investigated in the development of the present numerical model. In the first phase of this study, laser light focusing, radiation absorption and shock wave propagation over the entire pulsed cycle are modeled. The model geometry and test conditions of known benchmark experiments such as those in Myrabo's experiment will be employed in the numerical model validation simulations. The calculated performance data will be compared to the test data.

Chen, Yen-Sen↗

Atomic Data Needs for X-Ray Astronomy

This publication contains written versions of most of the invited talks presented at the workshop on Atomic Data Needs for X-ray Astronomy which was held at NASA's Goddard Space Flight Center on December 16-1 7 1999. The idea of hosting such a workshop emerged from an imminent need to update and complete current atomic datasets in anticipation of a new era of high quality X-ray spectra starting with the launching of Chandra and XMM-Newton observatories. At first, our vision of the workshop was of a short and limited attendance event, given the specialization of the topic. But it, was soon realized, from the response to the first workshop announcement, that the topic was of much interest, to researchers working in X-ray spectra (physicists and astronomers). As a result, the workshop grew to approximately 120 participants from several countries. The kind of atomic data that interests us are those parameters needed for analysis and modeling of spectra shortward of about about 100 A and relevant to ionic species of astronomical interest. The physical mechanisms of interest in the formation of spectra include photoionization. collisional ionization, recombination (radiative and dielectronic). collisional excitation (by electrons and protons). and radiative deexcitation. Unique to X-ray spectroscopy are the ionization and excitation processes from inner-closed shells. in addition to the challenges in interpret,ing the medium resolution (epsilon/delta epsilon is about 0.05 - 0.1) data obtained by current X-ray astronomy experiments. Line wavelengths are of interest too, particularly owing to the high resolution spectra from the new experiments. The workshop was divided into five major areas: Observational Spectroscopy, Theoretical Calculations of Atomic Data, Laboratory Measurements of Atomic Parameters. Spectra Modeling, and Atomic Databases. One comforting finding from the work shop is that the enthusiasm felt by X-ray astronomers about the new observational missions seems to be shared by theoretical and experimental physicists. Talks were presented about several exciting new projects and experimental and theoretical techniques devoted to X-ray spectroscopy. Simultaneously, several new tools for spectral analysis and modeling have recently been developed, together with improved atomic databases. These proceeding are expected to be of interests to producers and users of atomic data. Moreover. the contributions presented here have been written in a way that can be used by a general audience of scientists and graduate students in X-ray astronomy, modelling, and in computational and experimental atomic physics.

Kallman, Timothy↗

An Overview of the Impact of Energetic Particle Precipitation on the Mesosphere and Stratosphere

Energetic precipitating particles (EPPs) can cause significant constituent changes in the polar mesosphere and stratosphere (middle atmosphere) during certain periods. Both protons and electrons can influence the polar middle atmosphere through ionization and dissociation processes. EPPs can enhance HOx (H, OH, HO2) through the formation of positive ions followed by complex ion chemistry and NOx (N, NO, NO2) through the dissociation of molecular nitrogen. The HO, increases can lead to ozone destruction in the mesosphere and upper stratosphere via several catalytic loss cycles. Such middle atmospheric HOx,-caused ozone loss is rather short-lived due to the relatively short lifetime (hours) of the HOx constituents. The HOx,-caused ozone depletion has been observed during several solar proton events (SPEs) in the past 40 years. HOx enhancements due to SPEs were confirmed by observations in the past solar cycle. A number of modeling studies have been undertaken over this time period that show predictions of enhanced HO, accompanied by decreased ozone due to energetic particles. The NO, family has a longer lifetime than the HOx family and can also lead to catalytic ozone destruction. EPP-caused enhancements of the NOx family can affect ozone promptly, if produced in the stratosphere, or subsequently, if produced in the 1ow.er thermosphere or mesosphere and transported to the stratosphere. NOx enhancements due to auroral electrons, medium and high energy electrons, relativistic electron precipitation (REP) events, and SPEs have been measured and/or modeled for decades Only a small number of SPEs (less than 10) in each solar cycle have sufficient flux of high energy protons (greater than 30 MeV) to produce a significant amount of NOx directly in the stratosphere to cause a measurable ozone destruction. Very high energy electrons (greater than 1500 keV) during REP events can also produce NOx directly in the stratosphere, however, the frequency and intensity of these electrons is uncertain. Indirect stratospheric EPP effects result when NO, is produced in the mesosphere and lower thermosphere and transported to the stratosphere during the late fall or winter. Such EPP-produced NOx may last up to months beyond its initial production. This EPP-produced mesospheric and lower thermospheric NOx primarily results from auroral electrons (approx. 1- 30 keV), medium- and high-energy electrons (approx. 30-1500 keV), and medium energy protons (approx. 1-30 MeV). The EPP-caused direct and indirect effects on the stratosphere are important in the polar regions during particular years, especially near solar maximum. This talk will attempt to provide an overview of several of the EPP-related important processes and their impact on the mesosphere and stratosphere. Much progress has been made in this field in the past several years and it is anticipated that other workshop participants will address aspects of this topic in their presentations.

Jackman, Charles H.↗

Direct EPP Affects on the Middle Atmosphere

Energetic precipitating particles (EPPs) can cause significant direct constituent changes in the mesosphere and stratosphere (middle atmosphere) during certain periods. Both protons and electrons can influence the polar middle atmosphere through ionization and dissociation processes. EPPs can enhance HOx (H, OH, HO2) through the formation of positive ions followed by complex ion chemistry and NOx (N, NO, NO2) through the dissociation of molecular nitrogen. The HOx increases result in direct ozone destruction in the mesosphere and upper stratosphere via several catalytic loss cycles. Such middle atmospheric HOx-caused ozone loss is rather short-lived due to the relatively short lifetime (hours) of the HOx constituents. The NOx family has a considerably longer lifetime than the HOx family and can also lead to catalytic ozone destruction. EPP-caused enhancements of the NOx family can affect ozone directly, if produced in the stratosphere. Ozone decreases from the EPPs lead to a reduction in atmospheric heating and, subsequent atmospheric cooling. Conversely, EPPs can cause direct atmospheric heating through Joule heating. Measured HOx constituents OH and HO2 showed increases due to solar protons. Observed NOx constituents NO and NO2 were enhanced due to both solar protons and precipitating electrons. Other hydrogen- and nitrogen-ocntaining constituents were also measured to be directly influenced by EPPs, including N2O, HNO3, HO2NO2, N2OS, H2O2, ClONO2, HCl, and HOCl. Observed constituents ClO and CO were directly affected by EPPs as well. Many measurements indicated significant direct ozone decreases. A significant number of satellites housed instruments, which observed direct EPP-caused atmospheric effects, including Nimbus 4 (BUV), Nimbus 7 (SBUV), several NOAA platforms (SBUV/2), SME, UARS (HALOE, CLAES), SCISAT-1 (ACE-FTS), Odin (OSIRIS), Envisat-l (GOMOS, MIPAS, SCIAMACHY), and Aura (MLS). Measurements by rockets and ground-based radar also indicated EPP direct impacts. Atmospheric models have been used with some success in predicting the direct EPP impacts on the mesosphere and stratosphere. A review of the observed direct effects of EPP on the middle atmosphere will be given in this presentation.

Jackman, Charles H.↗

An Overview of Energetic Particle Precipitation Effects on the Earth's Atmosphere and (Potentially) Climate

Energetic precipitating particles (EPPs) can cause significant constituent changes in the polar mesosphere and stratosphere (middle atmosphere) during certain periods. Both protons and electrons can influence the polar middle atmosphere through ionization and dissociation processes. EPPs can enhance HOx (H, OH, HO2) through the formation of positive ions followed by complex ion chemistry and NOx (N, NO, NO2) through the dissociation of molecular nitrogen. The solar EPP-created HOx increases can lead to ozone destruction in the mesosphere and upper stratosphere via several catalytic loss cycles. Such middle atmospheric HOx-caused ozone loss is rather short-lived due to the relatively short lifetime (hours) of the HOx constituents. The HOx-caused ozone depletion of greater than 30% has been observed during several large solar proton events (SPEs) in the past 50 years. HOx enhancements due to SPEs were confirmed by observations in solar cycle 23. A number of modeling studies have been undertaken over this time period that show predictions of enhanced HOx accompanied by decreased ozone due to energetic particles. The solar EPP-created NOx family has a longer lifetime than the HOx family and can also lead to catalytic ozone destruction. EPP-caused enhancements of the NOx family can affect ozone promptly, if produced in the stratosphere, or subsequently, if produced in the lower thermosphere or mesosphere and transported to the stratosphere. NOx enhancements due to auroral electrons, medium and high energy electrons, relativistic electron precipitation (REP) events, and SPEs have been measured and/or modeled for decades. Model predictions and measurements show that certain years have significant winter-time meteorological events, which result in the transport of EPP-caused NOx enhancements in the upper mesosphere and lower thermosphere to lower altitudes. The NOx-caused ozone depletion has also been observed during several solar proton events (SPEs) in the past 50 years. Model predictions indicate that the longer-lived SPE-caused polar stratospheric and mesospheric ozone decrease can be >10% for up to five months past the largest events and is statistically significant; however, total ozone measurements do not indicate any long-term SPE impact.

Jackman, Charles H.↗

Adhesion in a Vacuum Environment and its Implications for Dust Mitigation Techniques on Airless Bodies

During the Apollo missions, the adhesion of dust to critical spacecraft systems was a greater problem than anticipated and resulted in functional degradation of thermal control surfaces, spacesuit seals, and other spacecraft components. Notably, Earth-based simulation efforts did not predict the magnitude and effects of dust adhesion in the lunar environment. Forty years later, we understand that the ultrahigh vacuum (UHV) environment, coupled with micrometeorite impacts and constant ion and photon bombardment from the sun result in atomically clean and high surface energy dust particles and spacecraft surfaces. However, both the dominant mechanism of adhesion in airless environments and the conditions for high fidelity simulation tests have still to be determined. The experiments presented in here aim to aid in the development of dust mitigation techniques for airless bodies (e.g., lunar surface, asteroids, moons of outer planets). The approach taken consists of (a) quantifying the adhesion between common polymer and metallic spacecraft materials and a synthetic noritic volcanic glass, as a function of surface cleanliness and of triboelectric charge transfer in a UHV environment, and (b) determining parameters for high fidelity tests through investigation of adhesion dependence on vacuum environment and sample treatment. Adhesion force has been measured between pins of spacecraft materials and a plate of synthetic volcanic glass by determining the pull-off force with a torsion balance. Although no significant adhesion is generally observed directly as a result of high surface energies, the adhesion due to induced electrostatic charge is observed to increase with spacecraft material cleanliness, in some cases by over a factor of 10. Furthermore, electrostatically-induced adhesion is found to decrease rapidly above pressures of 10-6 torr. It is concluded that high-fidelity tests should be conducted in high to ultrahigh vacuum and include an ionized surface cleaning process.

Berkebile, Stephen↗

Understanding Ionizing Radiation-Induced Speciation, Chemistry, and Transport in Nuclear Materials

The research to be presented will cover an overview of three projects supported by the United States Department of Energy Office of Science Solar Photochemistry Program: (i) Radiation-Induced Late Actinide Redox Chemistry (2019–2022); (ii) Understanding Radiation-Induced Iodine Speciation, Chemistry, and Transport in High Temperature Molten Salts (2022–2025); and (iii) Radiation-Induced Chemistry of Nuclear Materials (2023–2026). The overarching aim of these distinct projects is to develop a deep fundamental mechanistic understanding of ionizing-radiation-induced processes occurring in solutions over multiple time and length scales. Investigated solutions range from aqueous to organic to molten salt liquids in the presence and absence of ligands and various redox-active ions and molecules, including the actinides. The ultimate goal of these projects is to utilize the new foundational knowledge gained to construct quantitative multiscale computer models with the capacity to predict radiation-induced behavior in complex systems of relevance to nuclear energy technologies and beyond.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Towards the ionizing radiation induced bond dissociation mechanism in oxygen, water, guanine and DNA fragmentation: a density functional theory simulation

The radiation-induced damages in bio-molecules are ubiquitous processes in radiotherapy and radio-biology, and critical to space projects. In this study, we present a precise quantification of the fragmentation mechanisms of deoxyribonucleic acid (DNA) and the molecules surrounding DNA such as oxygen and water under non-equilibrium conditions using the first-principle calculations based on density functional theory (DFT). Our results reveal the structural stability of DNA bases and backbone that withstand up to a combined threshold of charge and hydrogen abstraction owing to simultaneously direct and indirect ionization processes. We show the hydrogen contents of the molecules significantly control the stability in the presence of radiation. This study provides comprehensive information on the impact of the direct and indirect induced bond dissociations and DNA damage and introduces a systematic methodology for fine-tuning the input parameters necessary for the large-scale Monte Carlo simulations of radio-biological responses and mitigation of detrimental effects of ionizing radiation.

59 BASIC BIOLOGICAL SCIENCES↗