Gamma Ray Spectrometry Assay Results of 242 Pu Samples at the Chemistry and Metallurgy Research Facility
Thirty individual items at the Chemistry and Metallurgy Research (CMR) facility with accountable amounts of 242 Pu required assay by gamma ray spectrometry in order to establish their masses with reasonable precision. There were two phases to this measurement campaign: 1) a preliminary screening phase in which each item was measured for a short 600 second count time to establish the relative masses between similar or like items, and 2) a second phase in which groups of items were counted for a considerably longer time in order to establish the group mass of 242 Pu in a reasonable time frame. The data from the two phases were assessed in a manner that allowed the project team to assign a 242 Pu mass to each individual item in the inventory, with the exception of three column tubes that could not be measured individually because of radiological contamination issues. The project team performed technical analyses with the SNAP™ analysis routine, PC-FRAM plutonium isotopic routine, and the NEN-2 PeakEasy routine. When total measurement uncertainties are factored in, the individual mass quantities calculated for all samples are statistically equivalent to the expected mass of 0.88 grams of total plutonium per sample.