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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 235 records · Page 13
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

All-electron, density-functional-based method for angle-resolved tunneling ionization in the adiabatic regime

Here we develop and test a method that integrates many-electron weak-field asymptotic theory (ME-WFAT) [O. I. Tolstikhin, L. B. Madsen, and T. Morishita, Phys. Rev. A 89, 013421 (2014)] in the integral representation (IR) into the density-functional-theory (DFT) framework. In particular, we present modifications of the integral formula in the IR ME-WFAT to incorporate the potential terms unique to DFT. By solving an adiabatic rate equation for the angle-resolved ionization yield in our DFT-based ME-WFAT method, we show that the results are in excellent agreement with those of real-time time-dependent density-functional-theory (TDDFT) simulations for NO, OCS, C⁢H 3 ⁢Br, and C⁢H 3 ⁢Cl interacting with one- and two-color laser fields with a fundamental wavelength of 800 nm. This agreement is significant because the WFAT calculations take only a small fraction of the time of full TDDFT calculations. These results suggest that in the wavelength region commonly used in strong-field experiments (800 nm and longer), our DFT-based WFAT treatment can be used to rapidly screen for the ionization properties of a large number of molecules as a function of alignment or orientation between the molecule and the strong field.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Microtructure and Low-Cycle Fatigue Behavior of Additively Manufactured 316L Stainless Steel at 300°C

Metal additive manufacturing (AM) or 3D printing has the potential to transform the nuclear industry by producing high quality components faster and cheaper, thus enhancing the operating performance of current plants and advanced reactors. Two AM 316L tubes - intended to act as surrogates for complex components where nuclear equipment vendors are more likely to consider AM technologies - were printed using a Renishaw AM400 Laser Powder Bed Fusion (L-PBF) system. The porosity of the as-built material was found to be small, 0.06%. In prior research, the fatigue and corrosion fatigue crack growth rate (CGR) response of the AM specimens in the as-built condition was found to be similar to that expected for conventional alloys, and extremely resistant to stress corrosion cracking (SCC). The present research demonstrates that the low-cycle fatigue behavior of the AM material in air is similar to that of wrought stainless steel at LWR temperature. The data suggest that low porosity levels do not have a significant effect on the fatigue performance of AM materials. Taken together, all data generated to date demonstrate that the use of AM alloys in a nuclear environment is plausible. Additional research on environmental fatigue, crack initiation, and SCC needs to be conducted to provide the performance information needed to qualify AM materials for LWR applications.

36 MATERIALS SCIENCE↗
DOE OSTI2022

The Kinetics of Aragonite Formation from Solution via Amorphous Calcium Carbonate

Magnesium doped Amorphous Calcium Carbonate was synthesised from precursor solutions containing varying amounts of calcium, magnesium, H2O and D2O. The Mg/Ca ratio in the resultant Amorphous Calcium Carbonate was found to vary linearly with the Mg/Ca ratio in the precursor solution. All samples crystallised as aragonite. No Mg was found in the final aragonite crystals. Changes in the Mg to Ca ratio were found to only marginally effect nucleation rates but strongly effect crystal growth rates. These results are consistent with a dissolution-reprecipitation model for aragonite formation via an Amorphous Calcium Carbonate intermediate.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Simulations of Laser Experiments to Study the Origin of Cosmic Magnetic Fields

Magnetic fields are ubiquitous in the universe; however, their origin is not fully understood. Cosmologists and astrophysicists have proposed a variety of ways in which small seed magnetic fields could be created. It is widely thought that the much larger values of the cosmic magnetic fields that we observe are a result of the amplification of these seed fields by the nonlinear turbulent dynamo mechanism. Such a mechanism had not yet been demonstrated in a controlled laboratory environment. We conceived experiments designed to demonstrate and study the nonlinear turbulent dynamo mechanism in the laboratory. These experiments characterize the distribution of turbulent energy among the velocity, magnetic field, and density fluctuations, providing a comprehensive picture of the energy cascade in a magnetized, turbulent plasma. The experiments build on the pathfinder experiments we have conducted on the Vulcan laser at the Rutherford-Appleton Laboratory in the UK and the OMEGA laser at Laboratory for Laser Energetics at Rochester. They utilize the high-intensity lasers at the Omega Laser Facility, the National Ignition Facility (NIF) at LLNL and the Laser Megajoule (LMJ) Facility in France – the largest laser facilities in the world. The goal of this project was to design and model the highly demanding experiments through simulation campaigns using FLASH, a highly capable radiation-MHD code we have developed, and large-scale 3D simulations on the Mira supercomputer at ANL. The simulations were vital to ensuring the experiments achieve the strong turbulence and large magnetic Reynolds numbers required for the nonlinear turbulent dynamo mechanism to operate. The simulations were also critical to determining when to fire the diagnostics, since the experiments last tens of nanoseconds but the signals of the strongly amplified magnetic fields last only a few nanoseconds. Finally, high-fidelity, validated FLASH simulations were crucial to interpreting the results of the experiments. By combining theory, experiments, and simulations, we were able to succeed in demonstrating and characterizing the nonlinear turbulent dynamo mechanism. The effort leveraged (1) the emergence of the Flash Center for Computational Science as a leader in numerical modeling of academic High Energy Density Physics (HEDP) experiments; (2) the FLASH code, which has been developed by the Flash Center and is a leadership-class, multi- physics, publicly available community code that has been applied successfully in many laser-driven experiments; (3) the expertise acquired through pathfinder experiments we performed on the Vulcan laser at the Rutherford-Appleton Laboratory in the UK and on the Omega laser facility; (4) the experience we have gained in designing and interpreting these experiments using validated simulations done with FLASH; and (5) the close collaborations we have established with outstanding experimental groups in the US and abroad. The broader impacts of the project are two-fold: (1) the work furthered the transformation of the academic community’s ability to design and analyze HEDP experiments at large laser facilities that is happening through the availability of FLASH and its widespread adoption by the academic community – a community that previously had had limited access to open and validated hydro/MHD simulation tools for HEDP experiments; and (2) the work trained young scientists to design and interpret HEDP experiments using validated simulations – a critical national need.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

Versatile & Intelligent Biodetection via Environmental Sensing (VIBES)

Reactive health monitoring strategies during events like the COVID-19 pandemic highlighted the need for predictive, threat-agnostic diagnostics that can detect both known diseases and novel chemical or biological threats. To address this, we investigated an optical biosensor as a breath volatile organic compound (VOC) analyzer, aiming to emulate biological olfaction. We assembled and validated the device with thin film metal coated substrate-based sensors. We immobilized small biological recognition elements on the substrates and delivered controlled concentrations of target VOCs. The sensor was irradiated with a visible laser and the sensor signal was recorded. We characterized the laser performance and tested 3 recognition elements for 2 VOCs with varying concentrations (1-100 ppm). We also evaluated enhancement of the signal using nanostructures on the metal film in comparison with planar film substrate. We demonstrated detecting ethanol reliably at concentrations as low as ~2 ppm along with preliminary detection of acetone (<100 ppm). We also found several unexpected factors that influence the sensor behavior that should be addressed to further refine the device’s performance. The nanostructures were, as expected, found to amplify the sensor signals. These findings demonstrate the feasibility of the optical bio-sensing modality for breath VOC monitoring at physiologically relevant levels. This positions LLNL to develop a low-cost, scalable, broad-spectrum health monitoring capability aligned with the Early Detection thrust of the Bioresilience Mission Focus Area and attract external funding.

47 OTHER INSTRUMENTATION↗
DOE OSTI2025

The advent of third-harmonic-generation laser systems: personal recollections

In the mid to late 1970s there was considerable debate as to which laser technology should be pursued—glass lasers (1-μm wavelength) or CO 2 lasers (10 μm). Based on target-physics considerations, theorists were advocating for shorter wavelengths. The physics understanding was confirmed by exciting results from the group at the École Polytechnique, who observed close to 100% target absorption with just a few joules of fourth-harmonic energy. These results motivated the leadership at LLE to plan similar experiments at the third harmonic, with a few more joules. This presentation covers a small time period from 1979 to 1980 during which highly efficient Third-Harmonic Generation (THG) became understood theoretically and demonstrated experimentally, leading to the worldwide adoption of THG with glass lasers for fusion research.

47 OTHER INSTRUMENTATION↗
DOE OSTI2020

Control of the optical properties of gum and dentin tissue of a human tooth at laser spectral lines in the range of 200 – 800 nm

A change in the optical properties of the tissue of the gums and dentin of a human tooth is experimentally investigated in vitro with the application of a 99.5 % glycerol solution. The kinetics of the total transmittance in the spectral range of 200 – 800 nm on characteristic laser lines is studied. It is shown that the effectiveness of optical clearing, expressed as a relative increase in the total transmittance, for gum tissue in the laser radiation range of 200 – 800 nm can vary significantly (by an order of magnitude). In this case, the absolute values of optical transmittance in the UV region are relatively small due to the strong absorption by the endogenous chromophores of the studied tissues, and in the visible and NIR regions, on the contrary, they are significant, which is due to the absence of strongly absorbing chromophores. The effectiveness of dentin clearing in the entire visible and NIR spectral regions is on average 25 % for 300 minutes of immersion of the sample in a 99.5 % glycerol solution. The presented results are necessary for increasing the efficiency of laser therapy and methods for optical monitoring of morphological changes in biological tissues for the purpose of early diagnosis of diseases. (paper)

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2020

Laser-free trapped-ion entangling gates with simultaneous insensitivity to qubit and motional decoherence

The dominant error sources for state-of-the-art laser-free trapped-ion entangling gates are decoherence of the qubit state and the ion motion. The effect of these decoherence mechanisms can be suppressed with additional control fields or with techniques that have the disadvantage of reducing gate speed. In this study, we propose using a near-motional-frequency magnetic field gradient to implement a laser-free gate that is simultaneously resilient to both types of decoherence, does not require additional control fields, and has a relatively small cost in gate speed.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2024

Towards a Next Generation Search for Time-Reversal Violation Using Optically Addressable Nuclei in Cryogenic Solids (Final Technical Report, September 2018 - August 2023)

Certain rare pear-shaped nuclei have unmatched sensitivity to new kinds of forces between subatomic particles that are not the same when the arrow of time is reversed. Such forces are believed to be responsible for the near absence of antimatter in the observable Universe. These rare isotopes, some for the first time, will be produced in large numbers at the Facility for Rare Isotope Beams currently under operating at Michigan State University providing an unprecedented opportunity to probe for new physics. In anticipation, we are using abundant isotopes to develop new techniques to manipulate nuclei embedded inside an optically transparent solid at cryogenic temperatures. Implantation into a solid, such as neon and argon, is potentially an effective way to both efficiently capture and repeatedly probe the small number of rare nuclei, such as radium and protactinium. An optically transparent host medium at cryogenic temperatures would allow for the laser manipulation of the nuclei in a thermally quiet and stable environment for a wide variety of guest species such as polar molecules. In such systems, the nuclei are exposed to extraordinarily large electric fields and magnetic field gradients, which significantly amplifies the measurability of certain time-reversal violating effects. The potential sensitivity of this new approach could be at least a few hundred times greater than the current leading experiment which uses stable mercury atoms. We report on the design considerations and preliminary performance of an instrument used to produce and implant molecules into a frozen argon solid.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Performance Assessment of Portable Optical Particle Spectrometer (POPS)

Accurate representation of atmospheric aerosol properties is a long-standing problem in atmospheric research. Modern pilotless aerial systems provide a new platform for atmospheric in situ measurement. However, small airborne platforms require miniaturized instrumentation due to apparent size, power, and weight limitations. A Portable Optical Particle Spectrometer (POPS) is an emerged instrument to measure ambient aerosol size distribution with high time and size resolution, designed for deployment on a small unmanned aerial system (UAS) or tethered balloon system (TBS) platforms. This study evaluates the performance of a POPS with an upgraded laser heater and additional temperature sensors in the aerosol pathway. POPS maintains its performance under different environmental conditions as long as the laser temperature remains above 25 °C and the aerosol flow temperature inside the optical chamber is 15 °C higher than the ambient temperature. The comparison between POPS and an Ultra-High Sensitivity Aerosol Spectrometer (UHSAS) suggests that the coincidence error is less than 25% when the number concentration is less than 4000 cm –3 . The size distributions measured by both of them remained unaffected up to 15,000 cm –3 . While both instruments’ sizing accuracy is affected by the aerosol chemical composition and morphology, the influence is more profound on the POPS.

47 OTHER INSTRUMENTATION↗
DOE OSTI2022

Scaling high-energy pulsed solid-state lasers to high average power

Techniques are provided for scaling the average power of high-energy solid-state lasers to high values of average output power while maintaining high efficiency. An exemplary technique combines a gas-cooled-slab amplifier architecture with a pattern of amplifier pumping and extraction in which pumping is continuous and in which only a small fraction of the energy stored in the amplifier is extracted on any one pulse. Efficient operation is achieved by propagating many pulses through the amplifier during each period equal to the fluorescence decay time of the gain medium, so that the preponderance of the energy cycled through the upper laser level decays through extraction by the amplified pulses rather than through fluorescence decay.

Erlandson, Alvin C.↗
DOE OSTI2023

Intense laser interaction with micro-bars

Intense laser fields interact very differently with micrometric rough surfaces than with flat objects. The interaction features high laser energy absorption and increased emission of MeV electrons, ions, and of hard x-rays. In this work, we irradiated isolated, translationally-symmetric objects in the form of micrometric Au bars. The interaction resulted in the emission of two forward-directed electron jets having a small opening angle, a narrow energy spread in the MeV range, and a positive angle to energy correlation. Our numerical simulations show that following ionization, those electrons that are pulled into vacuum near the object’s edge, remain in-phase with the laser pulse for long enough so that the Lorentz force they experience drive them around the object’s edge. After these electrons pass the object, they form attosecond duration bunches and interact with the laser field over large distances in vacuum in confined volumes that trap and accelerate them within a narrow range of momentum. The selectivity in energy of the interaction, its directionality, and the preservation of the attosecond duration of the electron bunches over large distances, offer new means for designing future laser-based light sources.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

Non-radiative luminescence decay with self-trapped hole migration in strontium titanate: Interplay between optical and transport properties

A novel model for the non-radiative decay of self-trapped excitons (STEs) in the advanced functional oxide SrTiO3 is proposed and supported by experimental observations. The study is based on the initial ionoluminescence stage for STE emission at 2.5 eV, and its dependence on temperature and electronic excitation rate under energetic heavy-ion irradiation. For all temperatures, this initial stage reaches rapidly a quasi-steady level, and then decreases as induced-structural damage increases. The quasi-steady luminescence exhibits a linear dependence on the excitation rate, suggesting a constant efficiency for STEs formation. An activation energy of 55 meV, essentially independent of the incident ion mass and energy of projectile-ion, is deduced from an Arrhenius-type relationship with irradiation temperature. This energy is in good agreement with experimental values, measured for non-radiative STE decay under ns-laser pulse excitation, and reasonably consistent with density functional theory calculations for migration of self-trapped holes (STHs) described by a small-polaron adiabatic hopping model. A new mechanism dealing with a non-radiative contribution to the STE transition is discussed, consisting of STH migration through thermally-activated hopping and annihilation with the STE-electron. Luminescence kinetics from the chromium intrinsic impurity strongly supports this model, being consistent with the annihilation of Cr 3+ centers through recombination with migrating STHs.

luminescence↗
DOE OSTI2020

Experiments to explore the influence of pulse shaping at the National Ignition Facility

The shaping of the drive pulse in time is a key tool in the design of fusion experiments that use inertia to confine burning plasmas. Here, it is directly related to the adiabat and compressibility of the DT fuel, and the characteristics of the laser and target that are needed to ignite. With this in mind, we have performed experiments at the National Ignition Facility that test small changes in the shape of the pulse. In contrast to theory, we find implosions at lower adiabats can have reduced yield and areal density. We discuss implications to performance and the mechanism(s) that could be responsible.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Laser-induced patterning for a diffraction grating using the phase change material of Ge 2 Sb 2 Te 5 (GST) as a spatial light modulator in X-ray optics: a proof of concept

The proposed X-ray spatial light modulator (SLM) concept is based on the difference of X-ray scattering from amorphous and crystalline regions of phase change materials (PCMs) such as Ge 2 Sb 2 Te 5 (GST). In our X-ray SLM design, the “ on” and “ off” states correspond to a patterned and homogeneous state of a GST thin film, respectively. The patterned state is obtained by exposing the homogeneous film to laser pulses. In this paper, we present patterning results in GST thin films characterized by microwave impedance microscopy and X-ray small-angle scattering at the Stanford Synchrotron Radiation Lightsource.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Comparing Pr 3+ and Nd 3+ for deactivating the Er 3+ : 4 I 13/2 level in lanthanum titanate glass

Erbium lanthanum titanate glasses were prepared by levitation melting for the spectroscopic study of ways to promote the mid-infrared fluorescence. Two series of heavily erbium doped glasses (15 wt%) were prepared with the addition of either Pr 3+ or Nd 3+ in amounts relative to Er 3+ of 0.05, 0.1, and 0.2. Both ions quench the lower Er 3+ laser level with the Pr 3+ doing so more rapidly. Although high co-dopant concentrations result in higher energy transfer, as clearly evidenced in upconversion and downconversion fluorescence measurements, the mid-infrared lifetime also suffers a reduction and, therefore, a balance must be struck in the co-dopant concentration. Lifetime and spectral measurements indicate that, at a fixed relative co-dopant amount, Pr 3+ is more effective than Nd 3+ at removing the bottleneck of the Er 3+ 4 I 13/2 level. Moreover, consideration of the lifetimes alongside the absorption data of the individual ions indicates that despite the large absorption cross-section of Nd 3+ at 808 nm, the concentration needed to yield more absorbed power than utilizing direct 976 nm excitation of Er 3+ results in unfavorable lifetimes of the mid-infrared transition. In the end, Pr 3+ prevails as the superior co-dopant in terms of the effects on fluorescence lifetimes as well as potential laser system design considerations. In a unique self-doping approach, a reducing melt atmosphere of Ar instead of O 2 creates a small fraction of Ti 3+ . In 5Er 2 O 3 -12La 2 O 3 -83TiO 2 glass, the presence of Ti 3+ quenches the 4 I 13/2 emission about 2.6 times more than the 4 I 11/2 when lifetimes are compared to an O 2 melt environment. As an additional means of increasing the mid-infrared emission, the effect of temperature on the mid- and near- infrared lifetimes of a lightly doped lanthanum titanate composition is investigated between 77-300 K. The mid-infrared lifetime increases by ∼30% while the near-infrared lifetime increases by ∼10%, which suggests in addition to co-doping, active cooling of the gain media will further enhance performance.

Materials Science↗
DOE OSTI2021

Experiments to explore the influence of pulse shaping at the National Ignition Facility

The shaping of the drive pulse in time is a key tool in the design of fusion experiments that use inertia to confine burning plasmas. It is directly related to the adiabat and compressibility of the DT fuel, and the characteristics of the laser and target that are needed to ignite. With this in mind, we have performed experiments at the National Ignition Facility that test small changes in the shape of the pulse. In contrast to theory, we find implosions at lower adiabats can have reduced yield and areal density. We discuss implications to performance and the mechanism(s) that could be responsible.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

Millisecond Phase Transition Kinetics of Lyotropic Liquid Crystalline Nanoparticles Observed by Time‐Resolved Small Angle X‐ray Solution Scattering

This study investigates the dynamic behavior of lyotropic liquid crystal nanoparticles (LCNPs), which are widely recognized for their applications in drug delivery. By employing nanosecond near‐infrared laser pulse‐induced temperature jump (T‐jump) and time‐resolved X‐ray solution scattering, the structural dynamics of phase transitions in phytantriol‐based cubosomes and hexosomes are revealed. Both cubosome and hexosome LCNPs undergo phase transitions into noncrystalline phases at high temperatures. Their phase transition kinetics, occurring within milliseconds (ms) and involving one intermediate structure, are captured. Additionally, the reverse self‐assembly processes of LCNPs were observed, occurring on the timescale of a few hundred ms. To our knowledge, this is the first observation of LCNP T‐jump induced phase transitions on the ms timescale and their reverse self‐assembly. These findings provide valuable insights into the LCNP phase transition processes, with potential implications for drug delivery applications.

Chemistry↗