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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 235 records · Page 13
All sourcesNASA NTRSDOE OSTI
NASA NTRS1987

Time dependent boundary conditions for hyperbolic systems

Nonreflecting boundary conditions are defined for multidimensional fluid dynamics problems where waves enter and leave the interior of a domain modeled by hyperbolic equations. Separate equations are defined for each type of incoming and outgoing wave. Temporally varying problems are considered in terms of a nonreflecting boundary condition which permit the amplitude of incoming waves to remain constant over time. Conservative expressions are presented that include dissipative terms. Applications of the computational techniques are illustrated with sample results for a traveling shock wave, a shock tube, a spherical explosion and expansion problems on one- and two-dimensions.

Thompson, Kevin W.↗
NASA NTRS1989

HF sideband generation in the ionosphere

The temporal development of sidebands excited near sunrise by two strong HF waves separated by a few hertz is presented. Sidebands are not observed before sunrise when the ionospheric critical frequency is less than the heater frequency. As the ionospheric density increases following sunrise and overdense conditions are established, strong sidebands emerge. Even though these results favor a mechanism which phase modulates the reflected HF wave over one which first downconverts the HF power to ULF before exciting sidebands, it is possible that either mechanism could at times contribute to sideband production.

Noble, S. T.↗
NASA NTRSDate not supplied

Probing the Sun with Imaging Spectrographs

EUV and X-ray images of the Sun have revolutionized our understanding of our closest star. With them, we can probe the morphology and temperature structure of the solar atmosphere and see how they evolve as a function of space and time. However, image data cannot be used to determine line-of-sight velocities, abundances, or densities. This information is required to calculate the energy budget of eruptive events, provide boundary conditions for global solar models, and explore fundamental processes occurring in the solar atmosphere. For those diagnostics, we require spectroscopy. Because the structures on the Sun are extended sources, most modern-day spectrographs observe the Sun through long narrow slits. Two-dimensional, spectrally pure solar images with velocity, abundance, and density information are built up by stepping the slit over regions of interest. This mode of operation implies that two-dimensional information is highly limited by cadence and the temporal evolution and spatial structure of these parameters can never be truly separated. Both spatial and spectral information can be obtained in a single snapshot with slitless spectrographs, which were often used in the 1950-1970s, but were abandoned due to the difficulty of unfolding the overlapping spatial and spectral information. Thanks to advances in computer processing speeds and machine learning algorithms, there have been several techniques developed to complete the spatial/spectral unfolding, unlocking the full capability of slitless spectrographs for solar observations. The goal of this talk is to give a broad overview of the capability of such instruments and demonstrate their usefulness in the next decade of solar observatories and beyond.

Amy Winebarger↗
NASA NTRSDate not supplied

Probing the Sun with Imaging Spectrographs

EUV and X-ray images of the Sun have revolutionized our understanding of our closest star. With them, we can probe the morphology and temperature structure of the solar atmosphere and see how they evolve as a function of space and time. However, image data cannot be used to determine line-of-sight velocities, abundances, or densities. This information is required to calculate the energy budget of eruptive events, provide boundary conditions for global solar models, and explore fundamental processes occurring in the solar atmosphere. For those diagnostics, we require spectroscopy. Because the structures on the Sun are extended sources, most modern-day spectrometers observe the Sun through long narrow slits. Two-dimensional, spectrally pure solar images with velocity, abundance, and density information are built up by stepping the slit over regions of interest. This method implies that two-dimensional information is highly limited by cadence and the temporal evolution and spatial structure of these parameters can never be truly separated. Both spatial and spectral information can be obtained in a single snapshot with slitless spectrometers, which were often used in the 1950-1970s, but were abandoned due to the difficulty of unfolding the overlapping spatial and spectral information. Thanks to advances in computer processing speeds and machine learning algorithms, there have been several techniques developed to complete the spatial/spectral unfolding, unlocking the full capability of slitless spectrometers for solar observations. The goal of this talk is to give an overview of the capability of such instruments, including recent results from a sounding rocket flight, and demonstrate their usefulness in the next decade of solar observatories and beyond.

Amy Winebarger↗
NASA NTRSDate not supplied

Probing the Sun with Imaging Spectrographs

EUV and X-ray images of the Sun have revolutionized our understanding of our closest star. With them, we can probe the morphology and temperature structure of the solar atmosphere and see how they evolve as a function of space and time. However, image data cannot be used to determine line-of-sight velocities, abundances, or densities. This information is required to calculate the energy budget of eruptive events, provide boundary conditions for global solar models, and explore fundamental processes occurring in the solar atmosphere. For those diagnostics, we require spectroscopy. Because the structures on the Sun are extended sources, most modern-day spectrometers observe the Sun through long narrow slits. Two-dimensional, spectrally pure solar images with velocity, abundance, and density information are built up by stepping the slit over regions of interest. This method implies that two-dimensional information is highly limited by cadence and the temporal evolution and spatial structure of these parameters can never be truly separated. Both spatial and spectral information can be obtained in a single snapshot with slitless spectrometers, which were often used in the 1950-1970s, but were abandoned due to the difficulty of unfolding the overlapping spatial and spectral information. Thanks to advances in computer processing speeds and machine learning algorithms, there have been several techniques developed to complete the spatial/spectral unfolding, unlocking the full capability of slitless spectrometers for solar observations. The goal of this talk is to give an overview of the capability of such instruments, including recent results from a sounding rocket flight, and demonstrate their usefulness in the next decade of solar observatories and beyond.

Amy Winebarger↗
NASA NTRSDate not supplied

Probing the Sun with Imaging Spectrographs

EUV and X-ray images of the Sun have revolutionized our understanding of our closest star. With them, we can probe the structure of the solar atmosphere and see how they evolve as a function of space and time. However, image data cannot be used to determine line-of-sight velocities, abundances, or densities. This information is required to calculate the energy budget of eruptive events, provide boundary conditions for global solar models, and explore fundamental processes occurring in the solar atmosphere. For those diagnostics, we require spectroscopy. Because the structures on the Sun are extended sources, most modern-day spectrometers observe the Sun through long narrow slits. Two-dimensional, spectrally pure solar images with velocity, abundance, and density information are built up by stepping the slit over regions of interest. This method implies that two-dimensional information is highly limited by cadence and the temporal evolution and spatial structure of these parameters can never be truly separated. Both spatial and spectral information can be obtained in a single snapshot with slitless spectrometers, which were often used in the 1950-1970s, but were abandoned due to the difficulty of unfolding the overlapping spatial and spectral information. Thanks to advances in computer processing speeds and machine learning algorithms, there have been several techniques developed to complete the spatial/spectral unfolding, unlocking the full capability of slitless spectrometers for solar observations. The goal of this talk is to give an overview of the capability of such instruments and demonstrate their usefulness in the next decade of solar observatories and beyond.

Amy Winebarger↗
DOE OSTI2020

Multiresolution GPC-Structured Control of a Single-Loop Cold-Flow Chemical Looping Testbed

Chemical looping is a near-zero emission process for generating power from coal. It is based on a multi-phase gas-solid flow and has extremely challenging nonlinear, multi-scale dynamics with jumps, producing large dynamic model uncertainty, which renders traditional robust control techniques, such as linear parameter varying H ∞ design, largely inapplicable. This process complexity is addressed in the present work through the temporal and the spatiotemporal multiresolution modeling along with the corresponding model-based control laws. Namely, the nonlinear autoregressive with exogenous input model structure, nonlinear in the wavelet basis, but linear in parameters, is used to identify the dominant temporal chemical looping process dynamics. The control inputs and the wavelet model parameters are calculated by optimizing a quadratic cost function using a gradient descent method. The respective identification and tracking error convergence of the proposed self-tuning identification and control schemes, the latter using the unconstrained generalized predictive control structure, is separately ascertained through the Lyapunov stability theorem. The rate constraint on the control signal in the temporal control law is then imposed and the control topology is augmented by an additional control loop with self-tuning deadbeat controller which uses the spatiotemporal wavelet riser dynamics representation. The novelty of this work is three-fold: (1) developing the self-tuning controller design methodology that consists in embedding the real-time tunable temporal highly nonlinear, but linearly parametrizable, multiresolution system representations into the classical rate-constrained generalized predictive quadratic optimal control structure, (2) augmenting the temporal multiresolution loop by a more complex spatiotemporal multiresolution self-tuning deadbeat control loop, and (3) demonstrating the effectiveness of the proposed methodology in producing fast recursive real-time algorithms for controlling highly uncertain nonlinear multiscale processes. The latter is shown through the data from the implemented temporal and augmented spatiotemporal solutions of a difficult chemical looping cold flow tracking control problem.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

Imaging Carrier Dynamics and Transport in Hybrid Perovskites with Transient Absorption Microscopy

In this review, the recent progress in using transient absorption microscopy to image charge transport and dynamics in semiconducting hybrid organic–inorganic perovskites is discussed. The basic principles, instrumentation, and resolution of transient absorption microscopy are outlined. With temporal resolution as high as 10 fs, sub-diffraction-limit spatial resolution, and excited-state structural resolution, these experiments have provided crucial details on charge transport mechanisms that have been previously obscured in conventional ultrafast spectroscopy measurements. Morphology-dependent mapping unveils spatial heterogeneity in carrier recombination and cooling dynamics. By spatially separating the pump and probe beams, carrier transport across grain boundaries has been directly visualized. Further, femtosecond temporal resolution allows for the examination of nonequilibrium transport directly, revealing extraordinarily long-range hot carrier migration. The application of transient absorption microscopy is not limited to hybrid perovskites but can also be useful for other polycrystalline materials in which morphology plays an important role in carrier transport.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Simultaneous Decomposition and Dewetting of Nanoscale Alloys: A Comparison of Experiment and Theory

In this work, we consider the coupled process of phase separation and dewetting of metal alloys of nanoscale thickness deposited on solid substrates. The experiments involve applying nanosecond laser pulses that melt the Ag40Ni60 alloy films in two setups: either on thin supporting membranes or on bulk substrates. These two setups allow for extracting both temporal and spatial scales on which the considered processes occur. The theoretical model involves a longwave version of the Cahn–Hilliard formulation used to describe spinodal decomposition, coupled with an asymptotically consistent longwave-based description of dewetting that occurs due to destabilizing interactions between the alloy and the substrate, modeled using the disjoining pressure approach. Careful modeling, combined with linear stability analysis and fully nonlinear simulations, leads to results consistent with the experiments. In particular, we find that the two instability mechanisms occur concurrently, with the phase separation occurring faster and on shorter temporal scales. The modeling results show a strong influence of the temperature dependence of relevant material properties, implying that such a dependence is crucial for the understanding of the experimental findings. The agreement between theory and experiment suggests the utility of the proposed theoretical approach in helping to develop further experiments directed toward formation of metallic alloy nanoparticles of desired properties.

36 MATERIALS SCIENCE↗
NASA NTRS1996

Climate Change and Neotectonic History of Northwestern China

The progress, results and future plans for the following objectives are presented: (1) To compare the types, rates, and magnitudes of surficial modification processes that have operated in Northwest China and the Southwestern U.S.; (2) To quantify and understand the basis of the remote sensing signatures of these processes to allow extrapolation from field sites to regional maps and to allow comparisons between widely separated arid regions; (3) To use the resulting chronologies to help define the temporal and spatial distribution of continental climate changes; and (4) Determine the ages of movements on some of the active faults in Northwestern China.

Farr, Tom G.↗
NASA NTRS1995

Profiles of Gamma-Ray Bursts and Their Component Pulses

One physically informative regularity of their otherwise heterogeneous ensemble, is that many Gamma-Ray Bursts consist of well defined pulses. To objectively quantify the temporal structure of BATSE bursts, we have developed an automatic modeling procedure that separates overlapping pulses and determines the energy-dependence of the pulse-shape parameters. No binning of photon arrival times is needed, so when applied to time-tagged events (TTE) the procedure captures variability information down to the shortest time scales present in the raw data. Maximizing the Bayesian likelihood function Pr(data/model) yields estimates of the model parameters, including the number of pulses present, and allows intercomparison of models of different forms. As with any nonlinear optimization, good initial guesses are crucial to avoid convergence to undesirable local minima. We find excellent initial pulse decompositions by wavelet-denoising a cumulative distribution of the raw photon arrival data; differentiation then gives a time profile mostly free of the systematic effects of degraded resolution (as in ordinary Fourier smoothing) and binning. We present statistical information on pulse rise-time, decay-time, peakedness, and amplitudes, plus their energy dependences - both within a single burst and for a large ensemble of bursts.

Scargle, Jeff D.↗
NASA NTRS2005

Assimilation of MLS and OMI Ozone Data

Ozone data from Aura Microwave Limb Sounder (MLS) and Ozone Monitoring Instrument (OMI) were assimilated into the ozone model at NASA's Global Modeling and Assimilation Office (GMAO). This assimilation produces ozone fields that are superior to those from the operational GMAO assimilation of Solar Backscatter Ultraviolet (SBUV/2) instrument data. Assimilation of Aura data improves the representation of the "ozone hole" and the agreement with independent Stratospheric Aerosol and Gas Experiment (SAGE) III and ozone sonde data. Ozone in the lower stratosphere is captured better: mean state, vertical gradients, spatial and temporal variability are all improved. Inclusion of OMI and MLS data together, or separately, in the assimilation system provides a way of checking how consistent OMI and MLS data are with each other, and with the ozone model. We found that differences between OMI total ozone column data and model forecasts decrease after MLS data are assimilated. This indicates that MLS stratospheric ozone profiles are consistent with OMI total ozone columns. The evaluation of error characteristics of OMI and MLS ozone will continue as data from newer versions of retrievals becomes available. We report on the initial step in obtaining global assimilated ozone fields that combine measurements from different Aura instruments, the ozone model at the GMAO, and their respective error characteristics. We plan to use assimilated ozone fields in estimation of tropospheric ozone. We also plan to investigate impacts of assimilated ozone fields on numerical weather prediction through their use in radiative models and in the assimilation of infrared nadir radiance data from NASA's Advanced Infrared Sounder (AIRS).

Stajner, I.↗
NASA NTRS2004

Three dimensional empirical mode decomposition analysis apparatus, method and article manufacture

An apparatus and method of analysis for three-dimensional (3D) physical phenomena. The physical phenomena may include any varying 3D phenomena such as time varying polar ice flows. A repesentation of the 3D phenomena is passed through a Hilbert transform to convert the data into complex form. A spatial variable is separated from the complex representation by producing a time based covariance matrix. The temporal parts of the principal components are produced by applying Singular Value Decomposition (SVD). Based on the rapidity with which the eigenvalues decay, the first 3-10 complex principal components (CPC) are selected for Empirical Mode Decomposition into intrinsic modes. The intrinsic modes produced are filtered in order to reconstruct the spatial part of the CPC. Finally, a filtered time series may be reconstructed from the first 3-10 filtered complex principal components.

Gloersen, Per↗
NASA NTRS2013

Correlations Between Variations in Solar EUV and Soft X-Ray Irradiance and Photoelectron Energy Spectra Observed on Mars and Earth

Solar extreme ultraviolet (EUV; 10-120 nm) and soft X-ray (XUV; 0-10 nm) radiation are major heat sources for the Mars thermosphere as well as the primary source of ionization that creates the ionosphere. In investigations of Mars thermospheric chemistry and dynamics, solar irradiance models are used to account for variations in this radiation. Because of limited proxies, irradiance models do a poor job of tracking the significant variations in irradiance intensity in the EUV and XUV ranges over solar rotation time scales when the Mars-Sun-Earth angle is large. Recent results from Earth observations show that variations in photoelectron energy spectra are useful monitors of EUV and XUV irradiance variability. Here we investigate photoelectron energy spectra observed by the Mars Global Surveyor (MGS) Electron Reflectometer (ER) and the FAST satellite during the interval in 2005 when Earth, Mars, and the Sun were aligned. The Earth photoelectron data in selected bands correlate well with calculations based on 1 nm resolution observations above 27 nm supplemented by broadband observations and a solar model in the 0-27 nm range. At Mars, we find that instrumental and orbital limitations to the identifications of photoelectron energy spectra in MGS/ER data preclude their use as a monitor of solar EUV and XUV variability. However, observations with higher temporal and energy resolution obtained at lower altitudes on Mars might allow the separation of the solar wind and ionospheric components of electron energy spectra so that they could be used as reliable monitors of variations in solar EUV and XUV irradiance than the time shifted, Earth-based, F(10.7) index currently used.

EUV↗
NASA NTRS1993

Rough surface scattering from moving ocean surfaces as an indicator of scattering mechanisms

Ever since Crombie used the Doppler spectrum of RF signals scattered from the ocean surface to provide conclusive evidence for Bragg resonant scattering, scattering from the ocean surface has served as a testing ground for the identification of governing scattering mechanisms in rough surface scattering. The moving ocean surface has the advantage for rough surface scattering that, being a dispersive medium, features with different spatial scales the tendency to travel at different speeds. Thus, by looking at the temporal signature of the scattered field, one can try to isolate the scattering mechanism. This feature has been exploited by various authors. To give a recent example, we cite the work of Plant, who examined the Doppler spectrum of the return signal to infer the presence of two-scale scattering in scattering at medium incidence angles. The problem with restricting oneself to the examination of the Doppler spectrum, as has been done traditionally, is that one restricts the phenomena under investigation to temporally homogeneous phenomena: transient phenomena, which are localized in time, are not localized in frequency space. There is increasing evidence that this type of phenomena, due to specular scattering or breaking waves, may also play an important role in determining the scattering mechanism in ocean-like surfaces. To overcome this problem, we introduce the use of the Wavelet Transform to study the frequency-temporal signatures of the scattered field from moving ocean waves. We calculate this signature using various analytic scattering theories and show that the Wavelet Transform provides a useful tool for separating the different scattering mechanisms operating in scattering in ocean-like surfaces. Next we simulate realistic nonlinear moving ocean waves and calculate the temporal scattered field signature by using the method of moments and the stop-start approximation: the surface is assumed stationary during a scattering event, but moves between incident EM pulses. We compute and compare the Doppler frequency spectrum and the Wavelet Transform of the resulting signal for various types of surfaces and show how different scattering mechanisms may be isolated by this technique. Finally, we compare these numerical results against the analytical predictions in order to obtain the domain of applicability of various scattering theories for moving ocean surfaces which may include wave breaking and specular glints.

Rodriguez, Ernesto↗
DOE OSTI2022

Thermoacoustic Soret separation

In a fluid mixture in a channel with an axial time-averaged temperature gradient, high-amplitude oscillating flow can greatly increase the axial flux of thermal diffusion (Soret) separation of the components of the mixture. The enhancement occurs when the oscillating lateral temperature gradient greatly exceeds the axial gradient, causing a large oscillating concentration that can be favorably time-phased with the oscillating flow. This process can occur even with a negligible pressure oscillation or with a negligible temperature response to pressure, as is the case in most liquid solutions. The thermal boundary condition imposed by realistic solids on thermoacoustic liquids is imperfect, adding mathematical complications that are absent for typical gases, for which the solid surface is temporally isothermal. Compared with gas mixtures, the high Lewis number in typical liquid solutions reduces the separation flux associated with the time-averaged temperature gradient, but it also reduces the remixing associated with the time-averaged mole-fraction gradient. For large enough channels, the second-law separation efficiency is only slightly reduced from that of steady liquid Soret separation.

36 MATERIALS SCIENCE↗
DOE OSTI2025

A simple three-component mixing problem for the evaluation of a new reaction rate model

A simple computational mixing problem is presented which can be utilized to assess the behavior of Reynolds-averaged reaction rate models in a problem with temporally varying mixedness. In this problem, three mixing components are homogeneously distributed but initially separated in a triply periodic domain. Further, these components are initialized within a Taylor–Green-like velocity field, which creates a mixing history evolving from the so-called “no-mix limit” to a well-mixed state. Large-eddy simulation results from this problem in configurations involving both premixed and nonpremixed reactants are then compared with zero-dimensional Reynolds-averaged Navier–Stokes results utilizing a new model for multicomponent reacting mixtures. The new model is shown to appropriately respect the no-mix limit and outperforms an earlier model (Morgan, 2022), particularly at early times when components are near the no-mix limit.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2022

Vertical Architecture Solution-Processed Quantum Dot Photodetectors with Amorphous Selenium Hole Transport Layer

Colloidal quantum dots (CQDs) provide wide spectral tunability and high absorption coefficients owing to quantum confinement and large oscillator strengths, which along with solution processability, allow a facile, low-cost, and room-temperature deposition technique for the fabrication of photonic devices. However, many solution-processed CQD photodetector devices demonstrate low specific-detectivity and slow temporal response. To achieve improved photodetector characteristics, limiting carrier recombination and enhancing photogenerated carrier separation are crucial. In this study, we develop and present an alternate vertical-stack photodetector wherein we use a solution-processed quantum dot photoconversion layer coupled to an amorphous selenium (a-Se) wide-bandgap charge transport layer that is capable of exhibiting single-carrier hole impact ionization and is compatible with active-matrix readout circuitry. This a-Se chalcogenide transport layer enables the fabrication of high-performance and reliable solution-processed quantum dot photodetectors, with enhanced charge extraction capabilities, high specific detectivity (D* ~ 0.5–5 × 10 12 Jones), fast 3 dB electrical bandwidth (3 dB BW ~ 22 MHz), low dark current density (J D ~ 5–10 pA/cm 2 ), low noise current (i n ~ 20–25 fW/Hz 1/2 ), and high linear dynamic range (LDR ~130–150 dB) across the measured visible electromagnetic spectrum (~405–656 nm).

77 NANOSCIENCE AND NANOTECHNOLOGY↗