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At least 235 records · Page 13

Final report: Mapping Interactions in Hybrid Systems with Active Scanning Probes

This project aimed to study and map interactions between components of hybrid nanodevices using a novel scanning probe approach. To enable this work, we initially constructed a flexible experimental apparatus allowing for simultaneous scanning probe and confocal optical microscopy measurements. This setup was first used for all-optical measurements of nanostructures, with the focus then shifting to hybrid devices in which single coherent electron spins are coupled to micron-scale ferromagnetic elements, which may prove useful for addressing single spins, enhanced sensing, or spin-wave-mediated coupling of spins for quantum information applications. A significant breakthrough was the realization that it is not necessary to fabricate a magnetic structure on a scanning probe – instead a ferromagnetic vortex core can act as an integrated, solid state, scanning probe. The core of the vortex produces a very strong, localized fringe field which can be used analogously to an MFM tip. Unlike a traditional MFM tip, however, the vortex core is scanned within an integrated device (eliminating drift), and can be moved on vastly faster timescales. This approach allows the detailed investigation of interactions between single spins and complex driven ferromagnetic dynamics.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

On the Diversity of Asymmetries in Gapped Protoplanetary Disks

Protoplanetary disks with large inner dust cavities are thought to host massive planetary or substellar companions. These disks show asymmetries and rings in the millimeter continuum caused by dust trapping in pressure bumps and potentially vortices or horseshoes. The origin of the asymmetries and their diversity remains unclear. We present a comprehensive study of 16 disks for which the gas surface density profile has been constrained by CO isotopologue data. First, we compare the azimuthal extents of the dust continuum profiles with the local gas surface density in each disk and find that the asymmetries correspond to higher Stokes numbers or low gas surface density. We discuss which asymmetric structures can be explained by a horseshoe, a vortex, or spiral density waves. Second, we reassess the gas gap radii from the {sup 13}CO maps, which are about a factor of 2 smaller than the dust ring radii, suggesting that the companions in these disks are in the brown dwarf (∼15–50 M {sub Jup}) or super-Jovian (∼3–15 M {sub Jup}) mass regime on eccentric orbits. This is consistent with the estimates from contrast curves on companion mass limits. These curves rule out (sub)stellar companions (q > 0.05) for the majority of the sample at the gap location, but it remains possible at even smaller radii. Third, we find that spiral arms in scattered-light images are primarily detected around high-luminosity stars with disks with wide gaps, which can be understood by the dependence of the spiral arm pitch angle on disk temperature and companion mass.

47 OTHER INSTRUMENTATION↗

Controllable vortex shedding from dissipative exchange flows in ferromagnetic channels

Ferromagnetic channels subject to spin injection at one extremum sustain long-range coherent textures that carry spin currents known as dissipative exchange flows (DEFs). In the weak injection regime, spin currents carried by DEFs decay algebraically and extend through the length of the channel, a regime known as spin superfluidity. Similar to fluids, these structures are prone to phase slips that manifest as vortex-antivortex pairs. In this work, we numerically study vortex shedding from DEFs excited in a magnetic nanowire with a physical obstacle. Using micromagnetic simulations, we find regimes of laminar flow and vortex shedding as a function of obstacle position tunable by the spin injection sign and magnitude. Vortex-antivortex pairs translate forward (VF regime) or backward (VB regime) with respect to the detector's extremum, resulting in well-defined spectral features. Qualitatively similar results are obtained when temperature, anisotropy, and weak nonlocal dipole fields are included in the simulations. These results provide clear features associated with DEFs that may be detected experimentally in devices with nominally identical boundary conditions. Furthermore, our results suggest that obstacles can be considered as DEF control gates, opening an avenue to manipulate DEFs via physical defects.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Strain effects on stability of topological ferroelectric polar configurations in (PbTiO3) n /(SrTiO3) n superlattices

The (PbTiO3)n/(SrTiO3)n (PTO/STO) superlattice system has been shown to exhibit interesting topological phases (e.g., vortices and skyrmions) in addition to normal ferroelectric domain states. Existing studies are mostly focused on the dependence of topological polar distributions and properties of PTO/STO superlattice on its periodicity. Here, we study the strain effect on the topological phase transitions and ferroelectric domain structures employing phase-field simulations. We summarized in an isotropic strain (in-plane misfit strain along the x direction is equal to that along the y direction) periodicity phase diagram displaying the stability regions of different polar topological states, including normal ferroelectric twins, vortices, skyrmions, and mixtures of vortices and twins. We also analyzed the polarization configurations under anisotropic in-plane strains (in-plane misfit strain along the x direction is not equal to that along the y direction) and demonstrated that the strain anisotropy can be used to tune the directions of vortex arrays along either the [100] pc or [010] pc directions or labyrinth vortex arrays. This work offers guidance to manipulating polar structures in the PTO/STO superlattices via strain engineering.

Physics↗

Giving rise to a set of fractional dipoles using spiral hyperbolic zone plate

We demonstrate a structured spiral hyperbolic zone plate which is able to generate a set of fractional vortex dipoles. The element is created by superimposition of two perpendicular hyperbolic zone plates in horizontal and vertical directions and its phase structure is then modified by adding an azimuthal characteristics factor. By setting different parameters when designing the element, characteristics of the generated FVDs will be changed. We then observed FVDs with different orders and topological charges rotate around the propagation axes upon propagation. This technique provides the possibility to generate multiple FVDs, and can be used in domains where sorting and guiding of small particles are of high interest such as optical tweezers and particle trapping configurations. Numerical and experimental results verify the superior features of SHFZP.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Vortex motion induced losses in tantalum resonators

Tantalum (Ta)-based superconducting circuits have been demonstrated to enable ultrahigh qubit quality factors (𝑄), motivating a careful study of the microscopic origin of the remaining losses that limit their performance. We have recently shown that the losses in Ta-based resonators are dominated by two-level systems at low microwave powers and millikelvin temperatures. We also observe that some devices exhibit loss that is exponentially activated at a lower temperature inconsistent with the superconducting critical temperature (T 𝑐 ) of the constituent film. Specifically, dc resistivity measurements show a T 𝑐 of over 4 K, while microwave measurements of resonators fabricated from these films show losses that increase exponentially with temperature with an activation energy as low as 0.3 K. Here, in this study, we present a comparative study of the structural and thermodynamic properties of Ta-based resonators and identify vortex motion-induced loss as the source of thermally activated microwave loss. Through careful magnetoresistance and x-ray diffraction measurements, we observe that the increased loss occurs for films that are in the clean limit, where the superconducting coherence length (𝜉) is shorter than the mean free path (𝑙). Vortex motion-induced losses are suppressed for films in the dirty limit, which show evidence of structural defects that can pin vortices. We verify this hypothesis by explicitly pinning vortices via patterning, and we find that we can suppress the loss by microfabrication.

36 MATERIALS SCIENCE↗

Stability of Polar Vortex Lattice in Ferroelectric Superlattices

A novel mesoscale state comprising of an ordered polar vortex lattice has been demonstrated in ferroelectric superlattices of PbTiO 3 /SrTiO 3 . In this study, we employ phase-field simulations, analytical theory, and experimental observations to evaluate thermodynamic conditions and geometric length scales that are critical for the formation of such exotic vortex states. We show that the stability of these vortex lattices involves an intimate competition between long-range electrostatic, long-range elastic, and short-range polarization gradient-related interactions leading to both an upper and a lower bound to the length scale at which these states can be observed. Finally, we found that the critical length is related to the intrinsic domain wall width, which could serve as a simple intuitive design rule for the discovery of novel ultrafine topological structures in ferroic systems.

36 MATERIALS SCIENCE↗

Gyrokinetic simulations of the effects of magnetic islands on microturbulence in KSTAR

Gyrokinetic simulations are utilized to study effects of magnetic islands (MIs) on the ion temperature gradient (ITG) turbulence in the KSTAR tokamak with resonant magnetic perturbations. Simulations show that the transport is controlled by the nonlinear interactions between the ITG turbulence and self-generated vortex flows and zonal flows, leading to an anisotropic structure of fluctuation and transport on the poloidal plane and in the toroidal direction. MIs greatly enhance turbulent transport of both particle and heat. The turbulent transport exhibits variations in the toroidal direction, with transport through the resonant layer near the island X-point being enhanced when the X-point is located at the outer mid-plane. A quantitative agreement is shown between simulations and KSTAR experiments in terms of time frequency and perpendicular wavevector spectrum.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Magnetism and its coexistence with superconductivity in CaK(Fe 0.949 Ni 0.051 ) 4 As 4 : Muon spin rotation/relaxation studies

Here, the magnetic response of Ca K ( Fe 0.949 Ni 0.051 ) 4 As 4 was investigated by means of the muon spin rotation/relaxation. The long-range commensurate magnetic order sets in below the Néel temperature T N = 50.0 ( 5 ) K. The density-functional theory calculations have identified three possible muon stopping sites. The experimental data were found to be consistent with only one type of magnetic structure, namely, the long-range magnetic spin-vortex-crystal order with the hedgehog motif within the a b plane and the antiferromagnetic stacking along the c direction. The value of the ordered magnetic moment at T ≈ 3 K was estimated to be m Fe = 0.38 ( 11 ) μ B ( μ B is the Bohr magneton). A microscopic coexistence of magnetic and superconducting phases accompanied by a reduction of the magnetic order parameter below the superconducting transition temperature T c ≃ 9 K is observed. Comparison with 11, 122, and 1144 families of Fe-based pnictides points to existence of correlation between the reduction of the magnetic order parameter at T → 0 and the ratio of the transition temperatures T c / T N . Such correlations were found to be described by Machida's model for coexistence of itinerant spin-density-wave magnetism and superconductivity [K. Machida, J. Phys. Soc. Jpn. 50 , 2195 (1981) ; S. L. Bud'ko et al. , Phys. Rev. B 98 , 144520 (2018) ].

36 MATERIALS SCIENCE↗

GPU-based simulation of the two-dimensional unstable structure of gaseous oblique detonations

In this paper, the two-dimensional structure of unstable oblique detonations induced by the wedge from a supersonic combustible gas flow is simulated using the reactive Euler equations with a one-step Arrhenius chemistry model. A wide range of activation energy of the combustible mixture is considered. Computations are performed on the Graphical Processing Unit (GPU) to reduce the simulation runtimes. A large computational domain covered by a uniform mesh with high grid resolution is used to properly capture the development of instabilities and the formation of different transverse wave structures. After the initiation point, where the oblique shock transits into a detonation, an instability begins to manifest and in all cases, the left-running transverse waves first appear, followed by the subsequent emergence of right-running transverse waves forming the dual-head triple point structure. This study shows that for low activation energies, a long computational length must be carefully considered to reveal the unstable surface due to the slow growth rate of the instability. For high activation energies, the flow behind the unstable oblique detonation features the formation of unburnt gas pockets and strong vortex-pressure wave interaction resulting in a chaotic-like vortical structure.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Equilibrium vortex lattices of a binary rotating atomic Bose–Einstein condensate with unequal atomic masses

We perform a detailed numerical study of the equilibrium ground-state structures of a binary rotating Bose–Einstein condensate with unequal atomic masses. Our results show that the ground-state distribution and its related vortex configurations are complex events that differ markedly depending strongly on the strength of rotation frequency, as well as on the ratio of atomic masses. We also discuss the structures and radii of the clouds, the number and the size of the core region of the vortices, as a function of the rotation frequency, and of the ratio of atomic masses, and the analytical results agree well with our numerical simulations. This work may open an alternate way in the quantum control of the binary rotating quantum gases with unequal atomic masses. - Highlights: • A binary quantum gases with unequal atomic masses is considered. • Effects of the ratio of atomic masses and rotation frequency are discussed in full parameter space. • The detailed information about both the cloud and vortices are also discussed.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Identifying Topological Defects in Lamellar Phases through Contour Analysis of Complex Wave Fields

Lamellar phases frequently contain structural imperfections that significantly affect their behaviors and properties. Our previous research successfully reconstructed real-space configurations of defective lamellar phases from diffuse scattering patterns, indicating the presence of phase vortices as a potential method for identifying topological defects disrupting the smectic ordering. Here, this report presents a mathematical framework using regularized wave fields to represent defective lamellar structures in real space. Phase singularities, resulting from the interference of random waves and indicating lamellar order disruption, are identified through a contour integral. These wave fields, derived from coherent scattering in reciprocal space, were validated via computational benchmarks analyzing small-angle neutron scattering data from AOT surfactant solutions, facilitating further statistical analysis of the defects. Our study highlights the potential to extract meaningful information about topological defects in lyotropic phases by inversely analyzing experimentally measured two-point static correlations. Our method allows for detailed structural analysis of various lyotropic phases, both particulate and nonparticulate, in their quiescent states and facilitates quantitative investigation of defects’ role in phase transitions. By integrating small-angle scattering, deep learning, and vortex tangle analysis, our comprehensive approach shows promise in addressing complex challenges in the structural analysis of soft matter systems.

36 MATERIALS SCIENCE↗

Dynamic realization of emergent high-dimensional optical vortices

The dimensionality of vortical structures has recently been extended beyond two dimensions, providing additional topological complexity and robustness for high-capacity information processing and turbulence control. The generation of high-dimensional vortical structures has mostly been demonstrated in classical systems through the complex interference of fluidic, acoustic, or electromagnetic waves. However, natural materials rarely support three- or higher-dimensional vortical structures and their physical interactions. Here, we experimentally demonstrate a high-dimensional gradient thickness optical cavity (GTOC) in which the optical coupling of planar metal-dielectric multilayers implements topological interactions across multiple dimensions. At non-trivial topological phases, high-dimensional GTOC induces high-dimensional vortical structures in generalized parameter space in three, four dimensions, and beyond. These emergent high-dimensional vortical structures are observed under electro-optic tomography as optical vortex dynamics in two-dimensional real-space, employing the optical thicknesses of dielectric layers as synthetic dimensions. Our findings hold significant promise for emulating high-dimensional physics and developing active topological photonic devices.

36 MATERIALS SCIENCE↗

Geometrical frustration and competing orders in the dipolar trimerized triangular lattice

Here, we introduce and explore low-energy configurations in two-dimensional arrays consisting of Ising-type dipolar coupled nanomagnets lithographically defined onto three-nanomagnet vertices arranged in a triangular coordination. Thus, the system is dubbed the trimerized triangular lattice. Employing synchrotron-based photoemission electron microscopy, we perform temperature-dependent magnetic imaging of moment configurations. These states are then characterized in terms of spin correlations and magnetic structure factors. The results reveal a competition between ferromagnetic and vortex dominated orders, which can be controlled by varying the relevant lattice parameter and the corresponding competing interactions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Transferring orbital angular momentum to an electron beam reveals toroidal and chiral order

Orbital angular momentum (OAM) and torque transfer play central roles in a wide range of magnetic textures and devices including skyrmions and spin-torque electronics. Analogous topological structures are now also being explored in ferroelectrics, including polarization vortex arrays in ferroelectric/dielectric superlattices. Unlike magnetic toroidal order, electric toroidal order does not couple directly to linear external fields. Instead, we find that the presence of an electric toroidal moment in a ferrorotational phase transfers measurable torque and OAM to a localized electron beam in the ballistic limit. We record these torque transfers from a high-energy electron beam using a momentum-resolved detector. This approach provides a high-sensitivity method to detect polarization fields and their more complex order parameters and topologies. In addition to toroidal order, we also demonstrate high-precision measurements of vorticity and chirality for polar vortexlike phases.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Staircase resiliency in a fluctuating cellular array

Inhomogeneous mixing by stationary convective cells set in a fixed array is a particularly simple route to layering. Layered profile structures, or staircases, have been observed in many systems, including drift-wave turbulence in magnetic confinement devices. The simplest type of staircase occurs in passive-scalar advection, due to the existence and interplay of two disparate timescales, the cell turn-over (τ H ), and the cell diffusion (τ D ) time. In this simple system, we study the resiliency of the staircase structure in the presence of global transverse shear and weak vortex scattering. The fixed cellular array is then generalized to a fluctuating vortex array in a series of numerical experiments. The focus is on regimes of low-modest effective Reynolds numbers, as found in magnetic fusion devices. By systematically perturbing the elements of the vortex array, we learn that staircases form and are resilient (although steps become less regular, due to cell mergers) over a broad range of Reynolds numbers. The criteria for resiliency are (a) τ D >>τ H and (b) a sufficiently high profile curvature (κ ≥ 1.5). We learn that scalar concentration travels along regions of shear, thus staircase barriers form first, and scalar concentration "homogenizes" in vortices later. The scattering of vortices induces a lower effective speed of scalar concentration front propagation. The paths are those of the least time. We observe that if background diffusion is kept fixed, the cell geometric properties can be used to derive an approximation for the effective diffusivity of the scalar. Furthermore, the effective diffusivity of the fluctuating vortex array does not deviate significantly from that of the fixed cellular array.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Magnetic small-angle neutron scattering

Small-angle neutron scattering (SANS) is one of the most important techniques for microstructure determination, being utilized in a wide range of scientific disciplines, such as materials science, physics, chemistry, and biology. The reason for its great significance is that conventional SANS is probably the only method capable of probing structural inhomogeneities in the bulk of materials on a mesoscopic real-space length scale from roughly 1 to 300 nm. Moreover, the exploitation of the spin degree of freedom of the neutron provides SANS with a unique sensitivity to study magnetism and magnetic materials at the nanoscale. As such, magnetic SANS ideally complements more real-space and surface-sensitive magnetic imaging techniques, e.g., Lorentz transmission electron microscopy, electron holography, magnetic force microscopy, Kerr microscopy, or spin-polarized scanning tunneling microscopy. This review summarizes the recent applications of the SANS method to study magnetism and magnetic materials. Here, this includes a wide range of materials classes from nanomagnetic systems such as soft magnetic Fe-based nanocomposites, hard magnetic Nd-Fe-B-based permanent magnets, magnetic steels, ferrofluids, nanoparticles, and magnetic oxides to more fundamental open issues in contemporary condensed matter physics such as skyrmion crystals, noncollinear magnetic structures in noncentrosymmetric compounds, magnetic or electronic phase separation, and vortex lattices in type-II superconductors. Special attention is paid not only to the vast variety of magnetic materials and problems where SANS has provided direct insight, but also to the enormous progress made regarding the micromagnetic simulation of magnetic neutron scattering.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Magnetic vortex in epitaxially-grown Co{sub 2}(Fe,Mn)Si alloy

We report magnetic vortex formation in epitaxially grown Co{sub 2}Fe{sub 0.4}Mn{sub 0.6}Si (CFMS) Heusler alloy discs that was confirmed using photoemission electron microscopy and the magneto-optical Kerr effect. The phase diagram of magnetic domain structures as functions of the disc thickness (t) and diameter (D) indicates that the magnetic vortex is stable in wide ranges of t and D even for the epitaxial CFMS. The annihilation field of vortex core depended not only on the disc aspect ratio but also on t. Numerical simulation suggests that this t dependence results from extrinsic pinning of a vortex core due to the epitaxial growth.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗