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At least 235 records · Page 13

Generalized eikonal identities for charged currents

Abstract We discuss QED radiative corrections to contact operators coupling two heavy fields and one light field. These operators appear ubiquitously in weak interactions with nuclei such as beta decay and neutrino nucleus scattering. New eikonal identities are derived in the static limit (i.e., neglecting nuclear recoil) that allow for manifest power counting of enhancements proportional to the charge of the nucleus. We apply these new identities to nuclear beta decays and find that the “independent particle model” used by Jaus, Rasche, Sirlin & Zucchini is closely related, though not identical, to a model independent effective field theorcalculation.

Physics↗

Machine-Learning Analysis of Radiative Decays to Dark Matter at the LHC

The search for weakly interacting matter particles (WIMPs) is one of the main objectives of the High Luminosity Large Hadron Collider (HL-LHC). In this work we use Machine-Learning (ML) techniques to explore WIMP radiative decays into a Dark Matter (DM) candidate in a supersymmetric framework. The minimal supersymmetric WIMP sector includes the lightest neutralino that can provide the observed DM relic density through its co-annihilation with the second lightest neutralino and lightest chargino. Moreover, the direct DM detection cross section rates fulfill current experimental bounds and provide discovery targets for the same region of model parameters in which the radiative decay of the second lightest neutralino into a photon and the lightest neutralino is enhanced. This strongly motivates the search for radiatively decaying neutralinos which, however, suffers from strong backgrounds. We investigate the LHC reach in the search for these radiatively decaying particles by means of cut-based and ML methods and estimate its discovery potential in this well-motivated, new physics scenario. We demonstrate that using ML techniques would enable access to most of the parameter space unexplored by other searches.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Search for invisible Higgs-boson decays in events with vector-boson fusion signatures using 139 fb -1 of proton-proton data recorded by the ATLAS experiment

A direct search for Higgs bosons produced via vector-boson fusion and subsequently decaying into invisible particles is reported. The analysis uses 139 fb -1 of pp collision data at a centre-of-mass energy of $\sqrt{s}$ = 13 TeV recorded by the ATLAS detector at the LHC. The observed numbers of events are found to be in agreement with the background expectation from Standard Model processes. For a scalar Higgs boson with a mass of 125 GeV and a Standard Model production cross section, an observed upper limit of 0.145 is placed on the branching fraction of its decay into invisible particles at 95% confidence level, with an expected limit of 0.103. These results are interpreted in the context of models where the Higgs boson acts as a portal to dark matter, and limits are set on the scattering cross section of weakly interacting massive particles and nucleons. Invisible decays of additional scalar bosons with masses from 50 GeV to 2 TeV are also studied, and the derived upper limits on the cross section times branching fraction decrease with increasing mass from 1.0 pb for a scalar boson mass of 50 GeV to 0.1 pb at a mass of 2 TeV.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Upper bound on Parity breaking scale for doublet WIMP dark matter

A bstract We consider weakly interacting massive particle (WIMP) dark matter in a Parity solution to the strong CP problem. The WIMP phenomenology can be drastically affected by the presence of Parity partners of the WIMP and electroweak gauge bosons. We focus on a Parity extension of SU(2) L -doublet fermion dark matter, identify the viable parameter space, and derive the predictions of the theory. We find that the Parity symmetry breaking scale is bounded from above, with the bound given by 25–60 TeV, depending on whether or not dark matter and its Parity partner coannihilate with each other. The High-Luminosity Large Hadron Collider, future colliders, and direct and indirect detection experiments can probe the parameter space further, with correlated signal rates.

Baldwin, Matthew J. [University of Chicago; Univer↗

Grey Galaxies’ as an endpoint of the Kerr-AdS superradiant instability

Kerr-AdS d+1 black holes for d ≥ 3 suffer from classical superradiant instabilities over a range of masses above extremality. We conjecture that these instabilities settle down into Grey Galaxies (GGs) — a new class of coarse-grained solutions to Einstein’s equations which we construct in d = 3. Grey Galaxies are made up of a black hole with critical angular velocity ω = 1 in the ‘centre’ of AdS, surrounded by a large flat disk of thermal bulk gas that revolves around the centre of AdS at the speed of light. The gas carries a finite fraction of the total energy, as its parametrically low energy density and large radius are inversely related. GGs exist at masses that extend all the way down to the unitarity bound. Their thermodynamics is that of a weakly interacting mix of Kerr-AdS black holes and the bulk gas. Their boundary stress tensor is the sum of a smooth ‘black hole’ contribution and a peaked gas contribution that is delta function localized around the equator of the boundary sphere in the large N limit. We also construct another class of solutions with the same charges; ‘Revolving Black Holes (RBHs)’. RBHs are macroscopically charged SO(d, 2) descendants of AdS-Kerr solutions, and consist of ω = 1 black holes revolving around the centre of AdS at a fixed radial location but in a quantum wave function in the angular directions. RBH solutions are marginally entropically subdominant to GG solutions and do not constitute the endpoint of the superradiant instability. Nonetheless, we argue that supersymmetric versions of these solutions have interesting implications for the spectrum of supersymmetric states in, e.g. N = 4 Yang-Mills theory.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Search for new particles in events with a hadronically decaying W or Z boson and large missing transverse momentum at $\sqrt{s}$ = 13 TeV using the ATLAS detector

A search is presented for new particles produced in proton-proton collisions at a centre-of-mass energy of 13 TeV that result in final states comprising a massive vector ( W or Z ) boson that decays hadronically and large missing transverse momentum. The data sample was collected with the ATLAS experiment at the Large Hadron Collider from 2015 to 2018 and corresponds to an integrated luminosity of 140 fb - 1 . No significant excess over the Standard Model expectation is observed. Model-independent 95% confidence-level limits on the visible cross-section that range from 0.3 fb to 79.5 fb are obtained for non-Standard-Model processes. Exclusion limits are also presented for models with axion-like particles, for two-Higgs-doublet models with a pseudo-scalar mediator between the Standard Model and the dark sector, for the invisible decay of the Higgs boson and for pair-produced weakly interacting dark matter candidates.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

WIMP cogenesis for asymmetric dark matter and the baryon asymmetry

We propose a new mechanism where asymmetric dark matter (ADM) and the baryon asymmetry are both generated in the same decay chain of a metastable weakly interacting massive particle (WIMP) after its thermal freezeout. Dark matter and baryons are connected by a generalized baryon number that is conserved, while the DM asymmetry and baryon asymmetry compensate each other. This unified framework addresses the DM-baryon coincidence while inheriting the merit of the conventional WIMP miracle in predicting relic abundances of matter. Examples of renormalizable models realizing this scenario are presented. These models generically predict ADM with sub-GeV to GeV-scale mass that interacts with Standard Model quarks or leptons, thus rendering potential signatures at direct detection experiments sensitive to low mass DM. Other interesting phenomenological predictions are also discussed, including: LHC signatures of new intermediate particles with color or electroweak charge and DM induced nucleon decay; the long-lived WIMP may be within reach of future high energy collider experiments.

79 ASTRONOMY AND ASTROPHYSICS↗

The scale of superpartner masses and electroweakino searches at the high-luminosity LHC

Searches for weakly interacting particles is one of the main goals of the high luminosity LHC run. In this work we study the well motivated cases of electroweakinos with mostly Wino and Bino components. We show the relevance of squark induced t-channel production in defining the production cross section and hence the LHC reach. Moreover, a realistic evaluation of the decay branching ratios show a strong dependence on the sign of μ and, for negative values of μ, on the relative size of the ratio of μ to the gaugino masses compared with tan β. Overall, unless it is kinematically suppressed, or specific conditions are fulfilled, the Higgs decay channel is the most significant one, and the trilepton channel becomes subdominant with respect to final states including bottom quarks. Although the properties are different than in the Higgsino-Bino case, also in this case the discovery reach extends to mass values that are significantly larger than the ones probed at current luminosities, leading to a strong motivation for the search for electroweakinos in the high luminosity LHC run.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Light Dark Matter Detection with Hydrogen-Rich Targets and Low-$T_c$ TES Detectors

Direct detection of nuclear scatterings of sub-GeV dark matter (DM) particles favors low-Z nuclei. Hydrogen nucleus, which has a single proton, provides the best kinematic match. The characteristic nuclear recoil energy is boosted by a factor of a few tens from those for larger nuclei used in traditional Weakly Interacting Massive Particles searches. Furthermore, hydrogen is optimal for detecting spin-dependent nuclear scatterings of sub-GeV DM, where large parameter space still remains unconstrained yet. In this paper, we first introduce several hydrogen-rich targets, which emit two classes of signals under kinetic excitations. One class of the signals is infrared photons, which are from fundamental vibrational and rotational modes of molecules and at several characteristic wavelengths. Another is acoustic phonons and optical phonons that decay into acoustic phonons. Then we discuss the technical status and future researches of low-T c transition-edge sensor (TES) detectors, which measure the infrared photons and acoustic phonons with desirable sensitivities. Utilization of hydrogen-rich targets and ultra-sensitive low-T c TES detectors for light DM detection requires both theoretical modeling and experimental prototyping.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Physical, numerical, and computational challenges of modeling neutrino transport in core-collapse supernovae

The proposal that core collapse supernovae are neutrino driven is still the subject of active investigation more than 50 years after the seminal paper by Colgate and White. The modern version of this paradigm, which we owe to Wilson, proposes that the supernova shock wave is powered by neutrino heating, mediated by the absorption of electron-flavor neutrinos and antineutrinos emanating from the proto-neutron star surface, or neutrinosphere. Neutrino weak interactions with the stellar core fluid, the theory of which is still evolving, are flavor and energy dependent. The associated neutrino mean free paths extend over many orders of magnitude and are never always small relative to the stellar core radius. Thus, neutrinos are never always fluid like. Instead, a kinetic description of them in terms of distribution functions that determine the number density of neutrinos in the six-dimensional phase space of position, direction, and energy, for both neutrinos and antineutrinos of each flavor, or in terms of angular moments of these neutrino distributions that instead provide neutrino number densities in the four-dimensional phase-space subspace of position and energy, is needed. In turn, the computational challenge is twofold: (i) to map the kinetic equations governing the evolution of these distributions or moments onto discrete representations that are stable, accurate, and, perhaps most important, respect physical laws such as conservation of lepton number and energy and the Fermi–Dirac nature of neutrinos and (ii) to develop efficient, supercomputer-architecture-aware solution methods for the resultant nonlinear algebraic equations. In this review, we present the current state of the art in attempts to meet this challenge.

79 ASTRONOMY AND ASTROPHYSICS↗

Synergistic effect of dual Brønsted acidic deep eutectic solvents for oxidative desulfurization of diesel fuel

Deep eutectic solvents (DESs) are generally used as attractive solvents or extractants rather than catalysts in the field of synthesis and separation. Herein, dual Brønsted acidic DESs were prepared by mixing sulfonated quaternary ammonium and oxalic acid as extractants and catalysts for deep oxidative desulfurization. Compared to the DESs with single acidic group, the dual acidic DESs exhibited much higher catalytic activity likely due to the synergistic effect. The 1 H NMR study indicated that the weak interaction between DES and sulfur compounds led to a low extraction capacity. However, the sulfur removal could reach 97.7% under optimized reaction conditions. Density functional theory (DFT) calculations demonstrated that sulfonic group and carboxylic group are of equal importance to desulfurization performance. Further, the desulfurization efficiency was also strongly affected by the viscosity of DESs. Here, we put forward a new strategy that the reaction time could be sharply shortened to 40 min and 100 min by adding low viscous acetonitrile and polyethylene glycol into DES to form mixing reaction system, respectively.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

The first experimental evidence for improved nanomechanical properties of calcium silicate hydrate by polycarboxylate ether and graphene oxide

Graphene oxide (GO) efficiently enhances macroscale mechanical properties of cement-based materials. Yet the nanoscale reinforcing mechanism of GO for calcium silicate hydrate (C-S-H), the key binding phase of concrete, remains poorly understood. Moreover, how polycarboxylate ether (PCE)-based superplasticizers affect the nanomechanical properties of C-S-H remains unclear. The intrinsic mechanical properties of the nanocomposites are measured using high-pressure X-ray diffraction. The influences of GO and PCE on the local Ca and Si environments are probed using X-ray absorption spectroscopy. For the first time, we evidence that PCE-induced well-dispersed GO nanoplatelets strengthen the C-S-H basal planes, whereas poorly water-dispersed GO weakly interacts with basal planes and does not strengthen in plane Casingle bondO bonds. Both PCE and GO only slightly strengthen C-S-H's c-axis. Here, the bulk modulus of C-S-H/PCE/GO nanocomposite is 190% than pure C-S-H. Functional groups of PCE and GO prefer interacting with the Casingle bondO sheets of C-S-Hs instead of silicate tetrahedra.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

The influence of LiH and TiH 2 on hydrogen storage in MgB 2 I: Promotion of bulk hydrogenation at reduced temperature

Mg(BH 4 ) 2 is an attractive hydrogen storage material, owing to its high gravimetric capacity of 14.9 wt %. However, the dehydrogenated material MgB 2 is very difficult to rehydrogenate, requiring excessive pressures and temperatures. Here we report the influence of LiH and TiH 2 on hydrogen storage reactions involving Bulk MgB 2 using XRD, XAS, FTIR and NMR. In ball-milled mixtures of LiH/MgB 2 , the LiH loses crystallinity but remains undissociated, forming a weakly bound complex with MgB 2 . The weak interactions produce minor variations in the local electronic structure at B and Mg, but do not markedly affect the underlying MgB 2 hexagonal crystal structure. No evidence is found for a mixed-metal boride Mg 1-x Li x B 2 in the as-prepared LiH/MgB 2 materials. The presence of LiH dramatically improves the hydrogenation of MgB 2 at 700 bar, forming borohydride 100 °C below the minimum hydrogenation temperature of pure MgB 2 and without the formation of undesirable intermediates such as [B 3 H 8 ] - , [B 10 H 10 ] 2- or [B 12 H 12 ] 2- . Evidence is reported for a mixed-metal borohydride of the type Mg (3-x)/2 Li x (BH 4 ) 3 produced by the hydrogenation. Subsequent desorption is also improved compared to pure Mg(BH 4 ) 2 and LiBH 4 , showing single-step hydrogen release up to ~8 wt% by 380 °C, whereas Mg(BH 4 ) 2 and LiBH 4 still retain significant amounts of hydrogen at this temperature. The material produced by desorption contains both MgB 2 and Mg metal, revealing the original LiH/MgB 2 system is not fully reversible. In contrast to LiH, TiH 2 is essentially inert when ball-milled with MgB 2 , and high-pressure hydrogenation leaves only unreacted TiH 2 and MgB 2 . Thus, added TiH 2 provides no benefit to MgB 2 hydrogenation.

08 HYDROGEN↗

Experimental and computational kinetics study of the liquid-phase hydrogenation of C=C and C=O bonds

Solvent effects on adsorption equilibrium and reaction kinetics are evaluated for hydrogenation reactions catalyzed by Pd/alumina in a series of different solvents. Three reactants – cyclohexene, benzene and benzaldehyde – and three solvents – n-heptane (HEP), methylcyclohexane (MCHA), decalin (DL) – have been investigated. Kinetic analysis of hydrogenation of cyclohexene reveals that hydrogen adsorbs on different sites from those where cyclohexene and the solvents adsorb; however, the presence of hydrogen on these separate sites affects the heats of adsorption of the hydrocarbons. When the solvent is a weakly interacting linear alkane (HEP), the rate determining step of the reaction is the first hydrogenation of adsorbed cyclohexene. Furthermore, this conclusion is supported by DFT calculations that show a higher enthalpy barrier for the first hydrogenation than for the second, while statistical thermodynamics analysis validates the physical significance of the entropy of adsorption parameters derived from the kinetic fitting of experimental data. By contrast, with solvents such as MCHA and DL, which interact more strongly with the metal surface and compete for active sites with the reactant and the surface intermediate, the rate limiting step seems to shift to the second hydrogenation step.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Enhanced ionic conductivity and lack of paddle-wheel effect in pseudohalogen-substituted Li argyrodites

Superionic conductors are key to the development of safe and high-energy-density, all-solid-state batteries. Using a combined theoretical and experimental approach, we explore the feasibility of increasing the ionic conductivity through pseudohalogen substitution in the Li argyrodite structure. Under the guidance of calculated thermodynamic stability, BH 4 -substituted Li argyrodite, Li 5.91 PS 4.91 (BH 4 ) 1.09 , was successfully synthesized via a mechanochemical method. As-synthesized BH 4- substituted Li argyrodite displays an ionic conductivity of 4.8 mS/cm at 25°C. Ab initio molecular dynamics simulation trajectory analysis was used to investigate how BH 4 facilitates Li-ion diffusion and indicates only a weak correlation with the B–H bond motion. Here, we find that the enhanced conductivity mainly originates from the weak interaction between Li and BH 4 and find no evidence of a paddle-wheel effect from the polyanion. This work provides insight into how cluster ions enhance Li diffusion and systematically describes how to explore superionic conductors with pseudohalogen substitution.

25 ENERGY STORAGE↗

Anion-dependent phase behavior of methylimidazolium-based ionic liquids mixed with water: Correlation between local molecular structure and mesoscale behaviors

The mesoscopic phase behavior of decylmethylimidazolium (C 10 mim) ionic liquids (ILs) bearing three monovalent anions—thiocyanate (SCN − ), nitrate (NO 3 − ), and chloride (Cl − )—mixed with water at relatively high IL contents (50–95 wt%) was investigated. Small-angle and wide-angle X-ray scattering (SAXS/WAXS) were employed to follow the evolution of both local and mesoscale structures across this composition range. In the absence of water, C 10 mimSCN and C 10 mimCl behaved as disordered liquids, whereas C 10 mimNO 3 spontaneously formed a hexagonally ordered cylindrical mesophase and displayed a sticky-solid macroscopic appearance. Upon addition of water, C 10 mimSCN remained a viscous liquid and only weakly ordered lamellar domains were observed. This limited ordering is attributed to the lack of hydrogen bonding and weak interaction energy between SCN − anions and C 10 mim + cations. In contrast, the trigonal-planar NO 3 − and point-like Cl − anions promoted the formation of well-defined hexagonal mesophases up to 35–45 wt% water. The formation of hydrogen bonding of the two anions with imidazolium ring protons likely enabled the creation of compact ion clusters that effectively exclude water molecules from the immediate vicinity of the IL aggregates. These findings demonstrate that the interaction energy between ion pairs dictate IL-water interactions and therefore control the transition from disordered liquids to ordered mesophases in IL/water mixtures with high IL contents. In conclusion, the combined SAXS/WAXS analysis reveals a correlation between local intermolecular structure and the emergence of mesoscopic order, providing a systematic framework for tailoring mesoscale structures in alkylimidazolium-based IL/water systems.

36 MATERIALS SCIENCE↗

A modular apparatus for use in high-precision measurements of parity violation in polarized eV neutron transmission

We describe a modular apparatus for use in parity-violation measurements in epithermal neutron–nucleus resonances with high instantaneous neutron fluxes at the Manuel Lujan Jr. Neutron Scattering Center at Los Alamos National Laboratory. This apparatus is designed to conduct high-precision measurements of the parity-odd transmission asymmetry of longitudinally polarized neutrons through targets containing nuclei with p-wave neutron–nucleus resonances in the 0.1–10 eV energy regime and to accommodate a future search for time reversal violation in polarized neutron transmission through polarized nuclear targets. The apparatus consists of an adjustable neutron and gamma collimation system, a 3 He- 4 He ion chamber neutron flux monitor, two identical cryostats for target cooling, an adiabatic eV-neutron spin flipper, a near-unit efficiency 6 Li- 7 Li scintillation detector operated in current mode, a flexible CAEN data acquisition system, and a neutron spin filter based on spin-exchange optical pumping of 3 He gas. We describe the features of the apparatus design devoted to the suppression of systematic errors in parity-odd asymmetry measurements. We describe the configuration of the apparatus used to conduct a precision measurement of parity violation at the 0.7 eV p-wave resonance in 139 La which employs two identical 139 La targets, one to polarize the beam on the p-wave resonance using the weak interaction and one to analyze the polarization.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Performance of $\text{BDX-MINI}$ veto systems

Here this paper describes the veto system of the BDX-MINI detector installed at Jefferson Lab (US). The BDX-MINI experiment is the first electron beam-dump experiment specifically designed to search for Light Dark Matter (LDM) particles in the MeV-GeV mass range. The core of the BDX-MINI detector is a lead-tungstate electromagnetic calorimeter, for a total volume of 4 dm 3 . The calorimeter is surrounded by a multi-layer veto aimed at rejecting cosmic background: the innermost layer of the veto is made by a passive tungsten shielding for low energy radiation, while plastic scintillators make the middle and outer layers for charged cosmic particles rejection. Being located about 20 m downstream, the dirt between the beam dump and the detector provides sufficient shielding from the beam-related background. In 2019–2020, BDX-MINI was exposed for about six months to weakly interacting particles (neutrinos and, if existing, DM) produced by a 2.176 GeV electron beam incident on the beam dump of experimental Hall-A at Jefferson Lab.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗