Ultra low background time projection alpha particle detector
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McNally, Brendan D.↗
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Nuclear Spectroscopy in the alpha-Particle
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Prediction of Alpha-Particle-Immune Gate-All-Around Field-Effect Transistors (GAA-FET) Based SRAM Design
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Lu, Albert [San Jose State University]↗
Alpha-decay induced shortening of fission tracks simulated by in situ ion irradiation
The diffusion of defects (e.g., vacancies and interstitials) and elements used for dating (e.g., He and Pb) in a mineral structure is a thermal process: This is the primary assumption used to determine the age and thermal history of minerals. For instance, thermal history reconstruction, through the number and length distribution of tracks produced by spontaneous fission of 238 U, is obtained by assuming a thermal event to be the only energy source for shortening of fission tracks. Here, we report a new, non-thermal energy source that induces additional shortening of fission tracks by the irradiation of alpha-recoils from the alpha-decay of 238 U and 232 Th. We simulate alpha-decay induced track-shortening by combining ion accelerator irradiations with transmission electron microscopy. This allows for the first observation of track-shrinkage during in situ ion irradiation. We show that rather than alpha-particles, alpha-recoils induce a significant shortening of fission tracks by nuclear-collisions. The shortening of track-length can be quantified as a function of alpha-decay event dose. However, apatite is less sensitive than zircon to this non-thermal process. Furthermore, the findings exemplify the interactions among different types of self-irradiation from alpha-particles, alpha-recoils and fission-fragment nuclei in single mineral grains and have important implications for the use of zircon and apatite for radiometric dating and thermochronology.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
In situ chemical analyses of extraterrestrial bodies
One of the most important tasks on any sample return mission will have to be a quick sample characterization in order to guarantee a variety of collected samples. An alpha particle instrument with alpha, proton and X-ray modes can provide a quick and almost complete chemical analysis of Mars samples. This instrument is based on three interactions of the alpha particles from a radioactive source with matter: elastic scattering of the alpha particles by nuclei (alpha mode), (alpha,p) nuclear reaction with some light elements (proton mode), and excitation of the atomic structure of atoms by alpha particles, leading to emission of characteristic X-rays of the lunar surface at three sites during the Surveyor mission of 1967 to 1968. Since then the instrument has been improved and miniaturized substantially. As shown in the past, the alpha particle instrument can operate under Martian conditions without any degradation in the performance. The alpha and proton modes can provide vital information about the light elements, while the X-ray mode with its ambient temperature X-ray detector will be useful for the heavier elements. The excitation of the atomic structure is provided by the same alpha radioactive source that is used by alpha and proton modes or by an auxiliary X-ray source that is selected to enhance the sensitivity to some important geochemical elements.
Economou, Thanasis E.↗
Analysis of Alfven eigenmode destabilization in ITER using a Landau closure model
Alfvén eigenmodes (AE) can be destabilized during ITER discharges driven by neutral beam injection (NBI) energetic particles (EP) and alpha particles. The aim of the present study is to analyze the AE stability of different ITER operation scenarios considering multiple energetic particle species. We use the reduced magneto-hydrodynamic (MHD) equations to describe the linear evolution of the poloidal flux and the toroidal component of the vorticity in a full 3D system, coupled with equations of density and parallel velocity moments for the EP species including the effect of the acoustic modes. Furthermore, the AEs driven by the NBI EP and alpha particles are stable in the configurations analyzed, only MHD-like modes with large toroidal couplings are unstable, although both can be destabilized if the EP increases above a threshold. The threshold is two times the model value for the NBI EP and alpha particles in the reverse shear (RS) case, leading to the destabilization of Beta induced AE (BAE) near the magnetic axis with a frequency of kHz and toroidal or elliptical AE (TAE/EAE) in the RS region with a frequency of kHz, respectively. On the other hand, the hybrid and steady state configurations show a threshold 3 times larger with respect to the model for the alpha particle and 40 times for the NBI EP, also destabilizing BAE and TAE between the inner and middle plasma region. In addition, a extended analysis of the RS scenario where the of both alpha particles and NBI EP are above the AE threshold, multiple EP damping effects are also identified as well as optimization trends regarding the resonance properties of the alpha particle and NBI EP with the bulk plasma.
70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
Four α correlations in nuclear fragmentation: a game of resonances *
Abstract Heavy ion collisions near the Fermi energy produce a ‘freezout’ region where fragments appear and later decay, emitting mainly neutrons, protons, alpha particles, and gamma rays. These decay products carry information about the decaying nuclei. Fragmentation events may result in high yields of boson particles, especially alpha particles, and may carry important information about the nuclear Bose Einstein condensate (BEC). We study ‘in medium’ four α correlations and link them to the ‘fission’ of 16 O in two 8 Be in the ground state or 12 C * (Hoyle state)+ α . Using novel techniques for the correlation functions, we confirm the resonance of 16 O at 15.2 MeV excitation energy, and the possibility of a lower resonance, close to 14.72 MeV. The latter resonance is the result of all α particles having 92 keV relative kinetic energies.
Physics↗
Effects of He Ion Irradiation in Simple Borosilicate Glasses for HLW Immobilisation - 20324
High-level radioactive waste (HLW) consists of fission products and minor actinides. Borosilicate glass is the host material of choice in most countries to safely immobilize HLW, followed by eventual geological disposal. HLW glasses will experience both self-heating and self-irradiation effects due to the decay of fission products and minor actinides present therein. During the first 500 years of geological disposal, beta-gamma decay will be the main source of radiation due to short half-lives of fission products, as compared to very long-lived actinides which will be responsible for irradiation over much longer timescales. High-energy alpha particles and alpha recoil nuclei can potentially have significant impact (stored energy, volume change, accumulated dose, chemical durability) on the performance of the wasteform over longer timescales. Thus, to ensure safe and economic disposal over geological periods (10{sup 4} - 10{sup 6} years), the assessment of performance and properties in terms of radiation effects becomes indispensable. This work aims to simulate the effects of alpha decay in radioactive waste glasses. Two international glasses, namely UK 'MW' lithium-sodium borosilicate and Indian sodium-barium borosilicate, which are being used as HLW immobilization matrices by the UK and India respectively, were prepared by a melt-quench method and annealed below their glass transition temperatures. Both glasses were irradiated with 650 KeV He{sup 2+} ions with doses ranging from 10{sup 15} to 10{sup 17} ions/cm{sup 2}. Structural analysis was carried out using electron paramagnetic resonance (EPR) and Raman spectroscopies. First derivative continuous wave EPR spectra were recorded for all pristine and irradiated glass monoliths at room temperature using an X-band (frequency 9.6 GHz) EPR Bruker spectrometer. Results from EPR analyses showed the formation of irradiation induced paramagnetic centers at g ∼ 2.00 in all irradiated glasses. Raman spectra of pristine and irradiated samples were acquired, and showed notable changes in glass structure post-irradiation, with the emergence of a broad Raman band at 1560 cm{sup -1} upon irradiation with high fluences. (authors)
12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
Study of aging of nuclear detector based on n-silicon/copper phthalocyanine heterojunction
Nuclear detectors based on n-silicon/copper-phthalocyanine (CuPc) heterojunction were fabricated using thermally evaporated CuPc thin film. These detectors exhibited stable electrical and {alpha}-particle characteristics for prolonged periods of time under ordinary laboratory conditions and also exposing to {alpha}- particles (during {alpha}- spectroscopic measurements). The electrical and alpha particle characteristics of these detectors were studied after a long gap of 3 - 5 years and the best result obtained from one detector (five year old) is reported here. Degradation in electrical and alpha particle characteristics were not found to be very significant over the period.
36 MATERIALS SCIENCE↗
Molecular water adsorption and reactions on (alpha)-Al2O3(0001) and (alpha)-Alumina Particles
The adsorption and reaction of water on single crystal, -Al2O3(0001) in ultrahigh vacuum, and -alumina particles in ambient conditions, was investigated using temperature programmed desorption (TPD), infrared reflection absorption spectroscopy (IRAS), diffuse reflectance infrared Fourier transform spectra (DRIFTS) and other surface science techniques. For a water coverage of 1 H2O/(surface Al3+) on -Al¬2O3(0001), no evidence for the surface hydroxyls expected from dissociative adsorption was observed in the infrared spectra, while the 2 vibration of molecular water was observed. Electron-stimulated desorption of molecular water at low coverages also indicated molecular or mixed (molecular plus dissociative) adsorption. Analysis of Kr TPD spectra showed that the water films wet the alumina substrate and suggested that the films were initially growing layer-by-layer. In contrast with the single crystal results, DRIFTS of water adsorption on alumina particles indicated the presence of surface hydroxyls that persist even after annealing to high temperatures in oxygen. For water on -Al2O3(0001) at coverages less than 0.3 H2O/(surface Al3+), water desorbed over a broad temperature range extending from ~250 K to 700 K. For larger coverages, water desorption occurred at temperatures between ~160 K and 250 K, consistent with desorption of molecular water. The results, which are consistent with at most a small amount of water dissociation on the Al-terminated (0001) surface, are difficult to reconcile with calculations suggesting that the barrier to dissociation is small. However, the results are consistent with recent vibrational sum frequency experiments showing that the hydroxylation of the Al-terminated (0001) surface takes many days even at ambient pressures and temperatures.
Petrik, Nikolay G.↗
Quiet time mass composition at near-geosynchronous altitudes
Mass composition data acquired from the near-geosynchronous SCATHA spacecraft during magnetically quiet times are analyzed. The time intervals over which data were included in the study span some four months in the spring and summer of 1979. This allows a reasonable coverage in both L shell and magnetic local time. At the higher L shells, L greater than 6.5, the mass composition data are consistent with sunward convection of plasma sheet particles. Protons and alpha particle fluxes peak near the 90 deg pitch angle. There is evidence that the alpha particle spatial distribution has a sharp inner edge near L = 6.5. At lower L values, the proton characteristics change. The density of protons above 1 keV decreases, while the lower-energy protons show an increase in density. The oxygen ions show a similar change, in that there is a large increase in the lower-energy oxygen ions from high L to low L, especially, in the dusk and midnight local time sectors. This suggests that the ionosphere may be continuously supplying plasma to the inner magnetosphere even during magnetically quiet times.
Strangeway, R. J.↗
Microphysics of Waves and Instabilities in the Solar Wind and Their Macro Manifestations in the Corona and Interplanetary Space
A breakthrough resulted from the investigation of plasma heating by ion-cyclotron waves in rapidly expanding flow tubes, often referred to as coronal funnels and expected to originate in the low transition region where the temperature gradient in the solar atmosphere rises very sharply. The investigation was made using a three-fluid plasma consisting of protons, electrons and alpha particles. It was found that these waves heat the solar wind plasma by directly heating the heavier species, namely the alphas. Although only alpha particles dissipate the waves, the strong Coulomb coupling between alpha particles and protons, and between protons and electrons, makes it possible for protons and electrons to be heated also to more than one million degrees, i.e. to coronal temperatures. Interestingly, the extreme heating of the alpha particles, however, is such that they end up being hotter and faster, and are no longer in thermal equilibrium with the protons and electrons. once the rapid expansion of the flow tube is complete, the particles return to thermal equilibrium. The observational signatures of these results are such that if spectral lines formed below a million degrees are observed at different heights in the corona, the inferred outflow velocities may vary by a factor of 5 to 6. In addition, if minor ions are indeed much faster than protons and electrons at temperatures below a million degrees, then one cannot reliably determine the bulk outflow velocity of the solar wind in that region from inferences of minor ion outflow velocities. A detailed parameter study on the resonant interaction between ion cyclotron waves and alpha particles and other minor ions is also under way. It is found that the highest frequency of the waves, or the location of the heating determines whether a thermal equilibrium can be established between minor ions and protons. As the maximum frequency is increased, alpha particles and protons become farther away from thermal equilibrium. As the maximum frequency becomes smaller, alpha particles and protons are more likely to be in thermal equilibrium. However, if the maximum frequency is below a critical value, ion cyclotron resonance occurs at a greater height and a hot corona cannot be produced.
Habbal, Shadia Rifai↗
Alpha voltaic batteries and methods thereof
An alpha voltaic battery includes at least one layer of a semiconductor material comprising at least one p/n junction, at least one absorption and conversion layer on the at least one layer of semiconductor layer, and at least one alpha particle emitter. The absorption and conversion layer prevents at least a portion of alpha particles from the alpha particle emitter from damaging the p/n junction in the layer of semiconductor material. The absorption and conversion layer also converts at least a portion of energy from the alpha particles into electron-hole pairs for collection by the one p/n junction in the layer of semiconductor material.
Raffaelle, Ryne P.↗
Alpha voltaic batteries and methods thereof
An alpha voltaic battery includes at least one layer of a semiconductor material comprising at least one p/n junction, at least one absorption and conversion layer on the at least one layer of semiconductor layer, and at least one alpha particle emitter. The absorption and conversion layer prevents at least a portion of alpha particles from the alpha particle emitter from damaging the p/n junction in the layer of semiconductor material. The absorption and conversion layer also converts at least a portion of energy from the alpha particles into electron-hole pairs for collection by the one p/n junction in the layer of semiconductor material.
Raffaelle, Ryne P.↗
Modulational and decay instabilities of Alfven waves - Effects of streaming He(2+)
The parametric instability of a circularly polarized Alfven wave propagating along the background magnetic field are considered, with emphasis on the effects of a second ion species, He(2+), which drifts relative to the protons. Even though its abundance is small, the He(2+) modifies the dispersion relation of the 'pump' Alfven wave and introduces a new sound wave (alpha sound) in addition to the usual sound wave carried primarily by the electrons and protons. Instabilities which are close to the He(2+) gyroresonance are found. This may provide a means of directly transferring Alfven wave energy to the alpha particles, if the alphas are able to resonantly extract energy from the unstable waves without quenching the instability altogether. Instabilities which are close to the alpha particle sound speed are also found.
Hollweg, Joseph V.↗
The alpha channeling effect
Alpha particles born through fusion reactions in a tokamak reactor tend to slow down on electrons, but that could take up to hundreds of milliseconds. Before that happens, the energy in these alpha particles can destabilize on collisionless timescales toroidal Alfven modes and other waves, in a way deleterious to energy confinement. However, it has been speculated that this energy might be instead be channeled into useful energy, so as to heat fuel ions or to drive current. Such a channeling needs to be catalyzed by waves Waves can produce diffusion in energy of the alpha particles in a way that is strictly coupled to diffusion in space. If these diffusion paths in energy-position space point from high energy in the center to low energy on the periphery, then alpha particles will be cooled while forced to the periphery. The energy from the alpha particles is absorbed by the wave. The amplified wave can then heat ions or drive current. This process or paradigm for extracting alpha particle energy collisionlessly has been called alpha channeling. While the effect is speculative, the upside potential for economical fusion is immense. The paradigm also operates more generally in other contexts of magnetically confined plasma.
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
HEOS 1 helium observations in the solar wind
Results of alpha-particle observations performed by the European satellite HEOS 1, in the period from December 9, 1968, to April 13, 1969, and from September 6, 1969, to April 15, 1970, are presented. The average bulk velocities of protons V sub p and alpha-particles V sub alpha appear to be equal; however, due to an instrumental bias, the possibility of V sub alpha being lower than V sub p cannot be ruled out. Comparison with observations of Vela 3 and Explorer 34 satellites gives evidence of a dependence of helium abundance on the solar cycle. The problem of the stability of differences between the bulk velocities of protons and alpha-particles is investigated. The behavior of alpha-particles through interplanetary shock waves is illustrated in connection with magnetic field measurements.
Bollea, D.↗
Detection of special nuclear materials with the associate particle technique
In the frame of the French trans-governmental R and D program against chemical, biological, radiological, nuclear and explosives (CBRN-E) threats, CEA is studying the detection of Special Nuclear Materials (SNM) by neutron interrogation with fast neutrons produced by an associated particle sealed tube neutron generator. The deuterium-tritium fusion reaction produces an alpha particle and a 14 MeV neutron almost back to back, allowing tagging neutron emission both in time and direction with an alpha particle position-sensitive sensor embedded in the generator. Fission prompt neutrons and gamma rays induced by tagged neutrons which are tagged by an alpha particle are detected in coincidence with plastic scintillators. This paper presents numerical simulations performed with the MCNP-PoliMi Monte Carlo computer code and with post processing software developed with the ROOT data analysis package. False coincidences due to neutron and photon scattering between adjacent detectors (cross talk) are filtered out to increase the selectivity between nuclear and benign materials. Accidental coincidences, which are not correlated to an alpha particle, are also taken into account in the numerical model, as well as counting statistics, and the time-energy resolution of the data acquisition system. Such realistic calculations show that relevant quantities of SNM (few kg) can be distinguished from cargo and shielding materials in 10 min acquisitions. First laboratory tests of the system under development in CEA laboratories are also presented.
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗