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DOE OSTI2024

Subsurface cosmogenic and radiogenic production of 42 Ar

Radioactive decays from 42 Ar and its progeny 42 K are potential background sources in large-scale liquid-argon-based neutrino and dark matter experiments. In the atmosphere, 42 Ar is produced primarily by cosmogenic activation on 40 Ar. The use of low radioactivity argon from cosmogenically shielded underground sources can expand the reach and sensitivity of liquid-argon-based rare event searches. We estimate 42 Ar production underground by nuclear reactions induced by natural radioactivity and cosmic-ray muon-induced interactions. At 3,000 mwe, 42 Ar production rate is 1.8×10 -3 atoms per ton of crust per year, 7 orders of magnitude smaller than the 39 Ar production rate at a similar depth in the crust. In conclusion, by comparing the calculated production rate of 42 Ar to that of 39 Ar for which the concentration has been measured in an underground gas sample, we estimate the activity of 42 Ar in gas extracted from 3,000 mwe depth to be less than two decays per ton of argon per year.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2024

First detailed calculation of atmospheric neutrino foregrounds to the diffuse supernova neutrino background in Super-Kamiokande

The diffuse supernova neutrino background (DSNB)—a probe of the core-collapse mechanism and the cosmic star-formation history—has not been detected, but its discovery may be imminent. A significant obstacle for DSNB detection in Super-Kamiokande (Super-K) is detector backgrounds, especially due to atmospheric neutrinos (more precisely, these are foregrounds), which are not sufficiently understood. We perform the first detailed theoretical calculations of these foregrounds in the range 16–90 MeV in detected electron energy, taking into account several physical and detector effects, quantifying uncertainties, and comparing our predictions to the 15.9 live time years of pre-gadolinium data from Super-K stages I–IV. We show that our modeling reasonably reproduces this low-energy data as well as the usual high-energy atmospheric-neutrino data. To accelerate progress on detecting the DSNB, we outline key actions to be taken in future theoretical and experimental work. In a forthcoming paper, we use our modeling to detail how low-energy atmospheric-neutrino events register in Super-K and suggest new cuts to reduce their impact. Published by the American Physical Society 2024

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2020

Testing H 0 in Acoustic Dark Energy with Planck and ACT Polarization

The canonical acoustic dark energy model (cADE), which is based on a scalar field with a canonical kinetic term that rapidly converts potential to kinetic energy around matter radiation equality, alleviates the Hubble tension found in ΛCDM. Here, we show that it successfully passes new consistency tests in the CMB damping tail provided by the ACT data, while being increasingly constrained and distinguished from alternate mechanisms by the improved CMB acoustic polarization data from Planck. The best fit cADE model to a suite of cosmological observations, including the SH0ES H 0 measurement, has H 0 = 70.25 compared with 68.23 (km s –1 Mpc –1 ) in ΛCDM and a finite cADE component is preferred at the 2.8σ level. The ability to raise H0 is now mainly constrained by the improved Planck acoustic polarization data, which also plays a crucial role in distinguishing cADE from the wider class of early dark energy models. ACT and Planck TE polarization data are currently mildly discrepant in normalization and drive correspondingly different preferences in parameters. Improved constraints on intermediate scale polarization approaching the cosmic variance limit will be an incisive test of the acoustic dynamics of these models and their alternatives.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2024

Ratio-preserving approach to cosmological concordance

Cosmological observables are particularly sensitive to key ratios of energy densities and rates, both today and at earlier epochs of the Universe. Well-known examples include the photon-to-baryon and the matter-to-radiation ratios. Equally important, though less publicized, are the ratios of pressure-supported to pressureless matter and the Thomson scattering rate to the Hubble rate around recombination, both of which observations tightly constrain. Preserving these key ratios in theories beyond the Λ Cold-Dark-Matter ( Λ CDM ) model ensures broad concordance with a large swath of datasets when addressing cosmological tensions. We demonstrate that a mirror dark sector, reflecting a partial Z 2 symmetry with the Standard Model, in conjunction with percentage level changes to the visible fine-structure constant and electron mass which represent a phenomenological change to the Thomson scattering rate, maintains essential cosmological ratios. Incorporating this ratio-preserving approach into a cosmological framework significantly improves agreement to observational data ( Δ χ 2 = - 35.72 ) and completely eliminates the Hubble tension with a cosmologically inferred H 0 = 73.80 ± 1.02 km / s / Mpc when including the S H 0 ES calibration in our analysis. While our approach is certainly nonminimal, it emphasizes the importance of keeping key ratios constant when exploring models beyond Λ CDM .

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

Fast neutron background characterization of the future Ricochet experiment at the ILL research nuclear reactor

Abstract The future Ricochet experiment aims at searching for new physics in the electroweak sector by providing a high precision measurement of the Coherent Elastic Neutrino-Nucleus Scattering (CENNS) process down to the sub-100 eV nuclear recoil energy range. The experiment will deploy a kg-scale low-energy-threshold detector array combining Ge and Zn target crystals 8.8 m away from the 58 MW research nuclear reactor core of the Institut Laue Langevin (ILL) in Grenoble, France. Currently, the Ricochet Collaboration is characterizing the backgrounds at its future experimental site in order to optimize the experiment’s shielding design. The most threatening background component, which cannot be actively rejected by particle identification, consists of keV-scale neutron-induced nuclear recoils. These initial fast neutrons are generated by the reactor core and surrounding experiments (reactogenics), and by the cosmic rays producing primary neutrons and muon-induced neutrons in the surrounding materials. In this paper, we present the Ricochet neutron background characterization using $$^3$$ 3 He proportional counters which exhibit a high sensitivity to thermal, epithermal and fast neutrons. We compare these measurements to the Ricochet Geant4 simulations to validate our reactogenic and cosmogenic neutron background estimations. Eventually, we present our estimated neutron background for the future Ricochet experiment and the resulting CENNS detection significance. Our results show that depending on the effectiveness of the muon veto, we expect a total nuclear recoil background rate between 44 ± 3 and 9 ± 2 events/day/kg in the CENNS region of interest, i.e. between 50 eV and 1 keV. We therefore found that the Ricochet experiment should reach a statistical significance of 4.6 to 13.6 $$\sigma $$ σ for the detection of CENNS after one reactor cycle, when only the limiting neutron background is considered.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Confirmation of the spectral excess in DAMIC at SNOLAB with skipper CCDs

Here, we present results from a 3.25 kg–day target exposure of two silicon charge-coupled devices (CCDs), each with 24 megapixels and skipper readout, deployed in the DAMIC setup at SNOLAB. With a reduction in pixel readout noise of a factor of 10 relative to the previous detector, we investigate the excess population of low-energy events in the CCD bulk previously observed above expected backgrounds. We address the dominant systematic uncertainty of the previous analysis through a depth fiducialization designed to reject surface backgrounds on the CCDs. The measured bulk ionization spectrum confirms the presence of an excess population of low-energy events in the CCD target with characteristic rate of ~7 events per kg-day and electron-equivalent energies of ~80 eV, whose origin remains unknown.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2020

Study of the Mu2e sensitivity to the $\mu^-\rightarrow e^+$ conversion process

The Mu2e experiment at Fermilab (Batavia, IL) will search for the coherent neutrinoless conversion of a muon into an electron in the electric field of an aluminum atom. The conversion process results in a monochromatic electron with energy slightly below the muon rest mass ($E_e= 104.97$ MeV). The experiment goal is to improve the previous measurement by four orders of magnitude and reach a single event sensitivity of $3 \times 10^{-17} $ on the conversion rate with respect to the muon capture rate. \\ The experiment will deliver a very intense pulsed negative muon beam to an aluminum target to achieve a total number of $10^{18}$ stopped muons in three years of running. Production and transport of the muons are accomplished with a sophisticated magnetic system comprised of a Production, a Transport and a Detector solenoid, with the last one hosting a Straw-tube Tracker and a Crystal Calorimeter. The entire detector region is surrounded by a Cosmic Ray Veto system. Mu2e is und er construction at the Muon Campus of Fermilab. \\ The INFN italian group is responsible for the design and construction of the crystal calorimeter, which plays a crucial role in the Mu2e measurement, providing particle identification capabilities fundamental for the rejection of the different background sources that can mimic a conversion electron. The calorimeter information allows also to improve the tracking performances it provides a fast standalone trigger for the experiment.\\ After a long R\&D phase, the final drawings see a calorimeter comprised of 1348 pure CsI crystals arranged in two annular disks. Each crystal is readout by two custom UV-extended Silicon Photomultipliers (SiPMs). Performances of the selected components were verified with an electron beam test, carried out in 2017 at the Beam Test Facility (BTF) at the National Laboratories of Frascati, on a large size prototype of 51 crystals and 102 SiPMs, confirming excellent energy ($\sigma_{E}/E = \mathcal{O }(10\%)$) and timing ($\sigma_{T} <500$ ps) resolutions in a! greement with the Mu2e specifications.\\ In the first chapters of this thesis, I describe my involvement in the calorimeter activities, with particular emphasis on the data analysis of the prototype energy response and resolution, that I was personally leading. Moreover, a description of the tuning of the simulation and the careful data-MC comparison is also reported.\\ An auxiliary measurement that can be performed with Mu2e is the search for a Lepton Number Violation (LNV) process where the negatively charged muon converts, without neutrinos, into a positron, $\mu ^{-} +N(A,Z) \rightarrow $ e$^+ +N(A,Z-2)$. At the moment of writing, Neutrinoless Double Beta Decay (0$\nu \beta \beta$) has set the most stringent limit on the LNV processes (T$^{0\nu \beta \beta}_{1/2} > 1.1 \times 10^{26} $ yr at 90$\%$ CL) with the GERDA experiment. In 0$\nu \beta \beta$ a pair of free electrons is created in the transformation from a nucleus $(A, Z)$ into its daughter $(A, Z + 2)$, namely: $(A,Z)\rightarrow (A, Z+2) =2 e^-$. Similar transitions could proceed through the emission of a pair of positrons, double electron capture (EC), or EC and single emission of a positron, with the nucleus changing from $(A, Z)$ to $(A, Z - 2)$. All these variations are equally interesting when discussing of new Physics, since they all manifest a non-conservation of the number of leptons.\\ Moreover, recent studies show that, because of flavor effect, off-diagonal processes, such as the $\mu^- -e^+$ conversion, can have their rate enhanced with respect to processes occurring in the $e-e$ sector.\\ Mu2e will search for $\mu^- + Al(27,13) \rightarrow e^+ +Na(27,11)$, only considering ground state transition, producing a conversion positron with energy $E_{e^+}= 92.32 $ MeV.\\ This thesis is focused on this search. In particular, I developed an algorithm to account for the radiative corrections to be applied to the conversion positrons that resulted in a few percent reduction in s ignal acceptance.\\ One of the most prominent background to ! this sear! ch is the Radiative Muon Capture (RMC) $ \mu+ N(Z,A)\rightarrow \gamma + \nu_{\mu} + N(Z-1,A)$. The produced photon can convert, virtually or in the detector materials (in the following referred as internal or external conversion respectively) in an electron-positron pair, producing positrons with energies approaching the expected conversion energy. Experimental results from previous experiments indicate the RMC endpoint ($\kmax$) to be of $\sim$ 90 MeV. A precise modeling of this background is relevant due to the proximity of the photon spectrum endpoint to the positron conversion energy. The calorimeter group is obviously interested to reconstruct the RMC distribution having also the opportunity to improve the current knowledge of the process. \\ A toy MC has been developed to evaluate the number of $e^+$ from external RMC background in the signal window. Knowing this value and ev...

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

First measurement of the yield of 8 He isotopes produced in liquid scintillator by cosmic-ray muons at Daya Bay

Here, Daya Bay presents the first measurement of cosmogenic 8 He isotope production in liquid scintillator, using an innovative method for identifying cascade decays of 8 He and its child isotope, 8 Li. We also measure the production yield of 9 Li isotopes using well-established methodology. The results, in units of 10 –8 μ –1 ⁢g –1 cm 2 , are 0.307 ± 0.042, 0.341 ± 0.040, and 0.546 ± 0.076 for 8 He, and 6.73 ± 0.73, 6.75 ± 0.70, and 13.74 ± 0.82 for 9 Li at average muon energies of 63.9 GeV, 64.7 GeV, and 143.0 GeV, respectively. The measured production rate of 8 He isotopes is more than an order of magnitude lower than any other measurement of cosmogenic isotope production. It replaces the results of previous attempts to determine the ratio of 8 He to 9 Li production that yielded a wide range of limits from 0% to 30%. The results provide future liquid-scintillator-based experiments with improved ability to predict cosmogenic backgrounds.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Mitigation of backgrounds from cosmogenic 137 Xe in xenon gas experiments using 3 He neutron capture

136 Xe is used as the target medium for many experiments searching for 0νββ. Despite underground operation, cosmic muons that reach the laboratory can produce spallation neutrons causing activation of detector materials. A potential background that is difficult to veto using muon tagging comes in the form of 137 Xe created by the capture of neutrons on 136 Xe. This isotope decays via beta decay with a half-life of 3.8 minutes and a Q β of ~4.16 MeV. This work proposes and explores the concept of adding a small percentage of 3 He to xenon as a means to capture thermal neutrons and reduce the number of activations in the detector volume. When using this technique we find the contamination from 137 Xe activation can be reduced to negligible levels in tonne and multi-tonne scale high pressure gas xenon neutrinoless double beta decay experiments running at any depth in an underground laboratory.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2020

Discrimination of electronic recoils from nuclear recoils in two-phase xenon time projection chambers

We present a comprehensive analysis of electronic recoil vs. nuclear recoil discrimination in liquid/gas xenon time projection chambers, using calibration data from the 2013 and 2014-16 runs of the Large Underground Xenon (LUX) experiment. We observe strong charge-to-light discrimination enhancement with increased event energy. For events with S1 = 120 detected photons, i.e. equivalent to a nuclear recoil energy of ~100 keV, we observe an electronic recoil background acceptance of <10 –5 at a nuclear recoil signal acceptance of 50%. We also observe modest electric field dependence of the discrimination power, which peaks at a field of around 300 V/cm over the range of fields explored in this study (50-500 V/cm). In the WIMP search region of S1 = 1-80 phd, the minimum electronic recoil leakage we observe is (7.3 ± 0.6) 10 –4 , which is obtained for a drift field of 240-290 V/cm. Pulse shape discrimination is utilized to improve our results, and we find that, at low energies and low fields, there is an additional reduction in background leakage by a factor of up to 3. We develop an empirical model for recombination fluctuations which, when used alongside the Noble Element Scintillation Technique (NEST) simulation package, correctly reproduces the skewness of the electronic recoil data. We use this updated simulation to study the width of the electronic recoil band, finding that its dominant contribution comes from electron-ion recombination fluctuations, followed in magnitude of contribution by fluctuations in the S1 signal, fluctuations in the S2 signal, and fluctuations in the total number of quanta produced for a given energy deposition.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2020

Measurement of the gamma ray background in the Davis cavern at the Sanford Underground Research Facility

Deep underground environments are ideal for low background searches due to the attenuation of cosmic rays by passage through the earth. However, they are affected by backgrounds from γ -rays emitted by 40 K and the 238 U and 232 Th decay chains in the surrounding rock. The LUX-ZEPLIN (LZ) experiment will search for dark matter particle interactions with a liquid xenon TPC located within the Davis campus at the Sanford Underground Research Facility, Lead, South Dakota, at the 4850-foot level. In order to characterise the cavern background, in-situ γ -ray measurements were taken with a sodium iodide detector in various locations and with lead shielding. The integral count rates (0–3300 keV) varied from 596 Hz to 1355 Hz for unshielded measurements, corresponding to a total flux from the cavern walls of 1.9 ± 0.4 γ cm −2 s −1 . The resulting activity in the walls of the cavern can be characterised as 220 ± 60 Bq/kg of 40 K, 29 ± 15 Bq/kg of 238 U, and 13 ± 3 Bq/kg of 232 Th.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2026

Dark Energy Survey Year 3: Blue shear

Modeling the intrinsic alignment (IA) of galaxies poses a challenge to weak lensing analyses. Here, using the Dark Energy Survey Year 3 shape catalog, we expect less impact from IA when we limit the sample to blue, star-forming galaxies. The cosmological parameter constraints from this BLUE cosmic shear sample are stable to IA model choice, unlike passive galaxies in the full DES Y3 sample, the goodness-of-fit is improved and the Ω m and 𝑆 8 better agree with the observations from Planck on the cosmic microwave background. Mitigating IA with sample selection in DES, rather than flexible model choices, can reduce uncertainty in 𝑆 8 by a factor of 1.5.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

First Constraint on Atmospheric Millicharged Particles with the LUX-ZEPLIN Experiment

We report on a search for millicharged particles (mCPs) produced in cosmic ray atmospheric interactions using data collected during the first science run of the LUX-ZEPLIN experiment. The mCPs produced by two processes—meson decay and proton bremsstrahlung—are considered in this study. This search utilized a novel signature unique to liquid xenon (LXe) time projection chambers, allowing sensitivity to mCPs with masses ranging from 10 to 1000 MeV/c 2 and fractional charges between 0.001 and 0.02 of the electron charge (𝑒). With an exposure of 60 live days and a 5.5 metric ton fiducial mass, we observed no significant excess over background. This represents the first experimental search for atmospheric mCPs and the first search for mCPs using an underground LXe experiment.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Measurement of the branching ratio of 16 N , 15 C , 12 B , and 13 B isotopes through the nuclear muon capture reaction in the Super-Kamiokande detector

The Super-Kamiokande detector has measured solar neutrinos for more than 25 years. The sensitivity for solar neutrino measurement is limited by the uncertainties of energy scale and background modeling. Decays of unstable isotopes with relatively long half-lives through nuclear muon capture, such as 16 N, 15 C, 12 B, and 13 B, are detected as background events for solar neutrino observations. Here, in this study, we developed a method to form a pair of stopping muon and decay candidate events and evaluated the production rates of such unstable isotopes. We then measured their branching ratios considering both their production rates and the estimated number of nuclear muon capture processes as Br⁡( 16 N) = (9.0 ± 0.1)%, Br⁡( 15 C) = (0.6 ± 0.1)%, Br⁡( 12 B) = (0.98 ± 0.18)%, Br⁡( 13 B) = (0.14 ± 0.12)%, respectively. The result for 16 N has world-leading precision at present and the results for 15 C, 12 B, and 13 B are the first branching ratio measurements for those isotopes.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗