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DOE OSTI2023

Effect of He seeding on hydrogen isotope permeation in tungsten by H-D mixed plasma exposure

Hydrogen (H) and deuterium (D) permeation fluxes for tungsten (W) by H-D mixed plasma were studied to clarify the hydrogen isotope effect on permeation by a newly designed plasma driven permeation (PDP) device at Shizuoka University. A mixed H-D plasma was produced by introducing H and D gasses with various ratios. The atomic ratio and permeation flux in the plasma were measured during the experiments. It was found that the H:D atomic ratio in the plasma was almost proportional to the introduced H:D gas ratio. When single species of H or D was irradiated, the H permeation rate showed approximately 1.6 times as high as that of D. Under H-D mixed plasma irradiation, the highest HD permeation rate was observed when the atomic ratio of H:D in the plasma was 50:50. In addition, the effect of He seeding on H-D mixed plasma driven permeation behavior was also evaluated. The recycling of hydrogen isotopes on the upstream side was enhanced due to the formation of He bubbles near the surface, which would prevent the dissolution of hydrogen isotopes into bulk W and enhance the reflection process during plasma exposure. H and D permeation fluxes were clearly reduced by seeding He in H-D mixed plasma. At lower temperature (~723 K), the ratio of steady permeation fluxes of H and D was about 75 : 25, confirming the high permeation flux of H . These results have demonstrated a significant hydrogen isotope effect, even if He was seeded or not. As the temperature increased, H and D permeation fluxes approached unity at 923 K. Therefore,this indicates that the hydrogen isotope effect was determined by the combination of recycling / reflection at or beneath the surface, which will be controlled by the temperature during plasma exposure.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2020

D retention and depth profile behavior for single crystal tungsten with high temperature neutron irradiation

Single crystalline W (tungsten) samples irradiated at 633, 963 and 1073 K by neutrons to a damage level of 0.1 dpa were exposed to a high-flux D (deuterium) plasma at 673, 873 and 973 K, respectively, in TPE (Tritium Plasma Experiment) at INL (Idaho National Laboratory). Deuterium desorption was analyzed by TDS (Thermal Desorption Spectroscopy), and D depth profiles were determined by NRA (Nuclear Reaction Analysis) at SNL (Sandia National Laboratories). HIDT (Hydrogen Isotope Diffusion and Trapping) simulation code was applied to evaluate D behavior for neutron-damaged W at higher temperature. The D retention at depths up to 3 f.tm for the neutron-damaged sample at 673 K was two orders of magnitude larger than that for undamaged tungsten, and its D desorption spectrum had a single broad stage at around 900 K. As the neutron irradiation/plasma exposure temperature increased, D retention was largely reduced, and the desorption temperature was increased to higher temperatures above 1100 K. The D depth profiles by NRA also showed D migration toward bulk by higher temperature irradiation, compared to undamaged W. The HIDT simulation indicated that the major binding energy of D was changed from 1.43 eV to 2.07 eV at higher neutron irradiation and plasma exposure temperatures, suggesting that some vacancies and small vacancy clusters would aggregate to form larger voids, or depopulation of weak traps at high D plasma exposure temperatures. It can be said that more stable trapping sites played dominant roles in the D retention at higher neutron irradiation and plasma exposure temperature. The binding energy by HIDT simulation was almost consistent with the reported value by TMAP, but the consideration of not only total D retention measured by TDS but also D depth profile by NRA led to the more accurate D behavior in neutron-damaged W.

36 MATERIALS SCIENCE↗

DOE OSTI2023

Measurement of beauty-strange meson production in Pb–Pb collisions at s NN = 5.02 TeV via non-prompt D s + mesons

The production yields of non-prompt ${D}^{+}_{s}$ mesons, namely ${D}^{+}_{s}$ mesons from beauty-hadron decays, were measured for the first time as a function of the transverse momentum ($p_T$) at midrapidity (|$y$| < 0.5) in central and semi-central Pb–Pb collisions at a centre-of-mass energy per nucleon pair $\sqrt{s{NN}}$ = 5.02 TeV with the ALICE experiment at the LHC. The ${D}^{+}_{s}$ mesons and their charge conjugates were reconstructed from the hadronic decay channel ${D}^{+}_{s}$ → $φπ^+$, with $φ$ → K - K + , in the 4 < $p_T$ < 36 GeV/c and 2 < $p_T$ < 24 GeV/ $c$ intervals for the 0–10% and 30–50% centrality classes, respectively. The measured yields of non-prompt ${D}^{+}_{s}$ mesons are compared to those of prompt ${D}^{+}_{s}$ and non-prompt $D^0$ mesons by calculating the ratios of the production yields in Pb–Pb collisions and the nuclear modification factor $R_{AA}$. The ratio between the $R_{AA}$ of non-prompt ${D}^{+}_{s}$ prompt ${D}^{+}_{s}$ mesons, and that between the $R_{AA}$ of non-prompt ${D}^{+}_{s}$ and non-prompt $D^0$ mesons in central Pb–Pb collisions are found to be on average higher than unity in the 4 < $p_T$ < 12 GeV/ $c$ interval with a statistical significance of about 1.6σ and 1.7σ, respectively. The measured $R_{AA}$ ratios are compared with the predictions of theoretical models of heavy-quark transport in a hydrodynamically expanding QGP that incorporate hadronisation via quark recombination.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2023

First measurement of prompt and non-prompt D* + vector meson spin alignment in pp collisions at $\sqrt{s}$ = 13 TeV

This letter reports the first measurement of spin alignment, with respect to the helicity axis, for D* + vector mesons and their charge conjugates from charm-quark hadronisation (prompt) and from beauty meson decays (non-prompt) in hadron collisions. The measurements were performed at midrapidity (|y| < 0.8) as a function of transverse momentum (p T ) in proton–proton (pp) collisions collected by ALICE at the centre-of-mass energy $\sqrt{s}$ = 13 TeV. The diagonal spin density matrix element $ρ$00 of D* + mesons was measured from the angular distribution of the D* + → D 0 (→ K - π + )π + decay products, in the D* + rest frame, with respect to the D* + momentum direction in the pp centre of mass frame. The $ρ$00 value for prompt D* + mesons is consistent with 1/3, which implies no spin alignment. However, for non prompt D* + mesons an evidence of $ρ$00 larger than 1/3 is found. The measured value of the spin density element is $ρ$00 = 0.455±0.022(stat.)±0.035(syst.) in the 5 < p T < 20 GeV/c interval, which is consistent with a Pythia 8 Monte Carlo simulation coupled with the EvtGen package, which implements the helicity conservation in the decay of D* + meson from beauty mesons. In non-central heavy-ion collisions, the spin of the D* + mesons may be globally aligned with the direction of the initial angular momentum and magnetic field. Based on the results for pp collisions reported in this letter it is shown that alignment of non-prompt D* + mesons due to the helicity conservation coupled to the collective anisotropic expansion may mimic the signal of global spin alignment in heavy-ion collisions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2024

Randomized control trial of moderate dose vitamin D alters microbiota stability and metabolite networks in healthy adults

ABSTRACT Evidence indicates that both vitamin D and the gut microbiome are involved in the process of colon carcinogenesis. However, it is unclear what effects supplemental vitamin D 3 has on the gut microbiome and its metabolites in healthy adults. We conducted a double-blind, randomized, placebo-controlled trial to identify the acute and long-term microbiota structural and metabolite changes that occur in response to a moderate dose (4,000 IU) of vitamin D 3 for 12 weeks in healthy adults. Our results demonstrated a significant increase in serum 25-hydroxy-vitamin D (25(OH)D) in the treatment group compared to placebo ( P < 0.0001). Vitamin D 3 significantly increased compositional similarity ( P < 0.0001) in the treatment group, and enriched members of the Bifidobacteriaceae family. We also identified a significant inverse relationship between the percent change in serum 25(OH)D and microbial stability in the treatment group ( R = −0.52, P < 0.019). Furthermore, vitamin D 3 supplementation resulted in notable metabolic shifts, in addition to resulting in a drastic rewiring of key gut microbial-metabolic associations. In conclusion, we show that a moderate dose of vitamin D 3 among healthy adults has unique acute and persistent effects on the fecal microbiota, and suggest novel mechanisms by which vitamin D may affect the host-microbiota relationship. IMPORTANCE Preventative measures to reduce the rise in early-onset colorectal cancer are of critical need. Both vitamin D, dietary and serum levels, and the gut microbiome are implicated in the etiology of colorectal cancer. By understanding the intimate relationship between vitamin D, the gut microbiome, and its metabolites, we may be able to identify key mechanisms that can be targeted for intervention, including inflammation and metabolic dysfunction. Furthermore, the similarity of vitamin D to cholesterol, which is metabolized by the gut microbiome, gives precedence to its ability to produce metabolites that can be further studied and leveraged for controlling colorectal cancer incidence and mortality.

Wyatt, Madhur↗

DOE OSTI2023

D-Egg: a dual PMT optical module for IceCube

The D-Egg, an acronym for "Dual optical sensors in an Ellipsoid Glass for Gen2," is one of the optical modules designed for future extensions of the IceCube experiment at the South Pole. The D-Egg has an elongated-sphere shape to maximize the photon-sensitive effective area while maintaining a narrow diameter to reduce the cost and the time needed for drilling of the deployment holes in the glacial ice for the optical modules at depths up to 2700 m. The D-Egg design is utilized for the IceCube Upgrade, the next stage of the IceCube project also known as IceCube-Gen2 Phase 1, where nearly half of the optical sensors to be deployed are D-Eggs. With two 8-inch high-quantum efficiency photomultiplier tubes (PMTs) per module, D-Eggs offer an increased effective area while retaining the successful design of the IceCube digital optical module (DOM). The convolution of the wavelength-dependent effective area and the Cherenkov emission spectrum provides an effective photodetection sensitivity that is 2.8 times larger than that of IceCube DOMs. The signal of each of the two PMTs is digitized using ultra-low-power 14-bit analog-to-digital converters with a sampling frequency of 240 MSPS, enabling a flexible event triggering, as well as seamless and lossless event recording of single-photon signals to multi-photons exceeding 200 photoelectrons within 10 ns. Mass production of D-Eggs has been completed, with 277 out of the 310 D-Eggs produced to be used in the IceCube Upgrade. In this paper, we report the design of the D-Eggs, as well as the sensitivity and the single to multi-photon detection performance of mass-produced D-Eggs measured in a laboratory using the built-in data acquisition system in each D-Egg optical sensor module.

47 OTHER INSTRUMENTATION↗

DOE OSTI2023

Studies of the decay $$ {\textrm{D}}_{\textrm{s}}^{+}\to {\textrm{K}}^{+}{\textrm{K}}^{-}{\mu}^{+}{\nu}_{\mu } $$

Abstract The$$ {D}_s^{+}\to {K}^{+}{K}^{-}{\mu}^{+}{\nu}_{\mu } $$ D s + → K + K − μ + ν μ decay is studied based on 7.33 fb −1 ofe + e − collision data collected with the BESIII detector at center-of-mass energies in the range from 4.128 to 4.226 GeV. The absolute branching fraction is measured as$$ \mathcal{B}\left({D}_s^{+}\to \phi {\mu}^{+}{\nu}_{\mu}\right)=\left(2.25\pm 0.09\pm 0.07\right)\times {10}^{-2} $$ B D s + → ϕ μ + ν μ = 2.25 ± 0.09 ± 0.07 × 10 − 2 , the most precise measurement to date. Combining with the world average of$$ \mathcal{B}\left({D}_s^{+}\to \phi {e}^{+}{\nu}_e\right) $$ B D s + → ϕ e + ν e , the ratio of the branching fractions obtained is$$ \frac{\mathcal{B}\left({D}_s^{+}\to \phi {\mu}^{+}{\nu}_{\mu}\right)}{\mathcal{B}\left({D}_s^{+}\to \phi {e}^{+}{\nu}_e\right)}=0.94\pm 0.08 $$ B D s + → ϕ μ + ν μ B D s + → ϕ e + ν e = 0.94 ± 0.08 , in agreement with lepton universality. By performing a partial wave analysis, the hadronic form factor ratios atq 2 = 0 are extracted, finding$$ {r}_V=\frac{V(0)}{A_1(0)}=1.58\pm 0.17\pm 0.02 $$ r V = V 0 A 1 0 = 1.58 ± 0.17 ± 0.02 and$$ {r}_2=\frac{A_2(0)}{A_1(0)}=0.71\pm 0.14\pm 0.02 $$ r 2 = A 2 0 A 1 0 = 0.71 ± 0.14 ± 0.02 , where the first uncertainties are statistical and the second are systematic. No significantS-wave contribution fromf 0 (980)→ K + K − is found. The upper limit$$ \mathcal{B}\left({D}_s^{+}\to {f}_0(980){\mu}^{+}{\nu}_{\mu}\right)\cdot \mathcal{B}\left({f}_0(980)\to {K}^{+}{K}^{-}\right)<5.45\times {10}^{-4} $$ B D s + → f 0 980 μ + ν μ ⋅ B f 0 980 → K + K − < 5.45 × 10 − 4 is set at 90% credibility level.

Physics↗

DOE OSTI2021

Measurement of beauty and charm production in pp collisions at $\sqrt{s}$ = 5.02 TeV via non-prompt and prompt D mesons

The pT-differential production cross sections of prompt and non-prompt (produced in beauty-hadron decays) D mesons were measured by the ALICE experiment at midrapidity (|y| < 0.5) in proton-proton collisions at s√ = 5.02 TeV. The data sample used in the analysis corresponds to an integrated luminosity of (19.3 ± 0.4) nb -1 . D mesons were reconstructed from their decays D 0 → K - π + , D + → K - π + π + , and D$^+_s$→ φπ + → K - K + π + and their charge conjugates. Compared to previous measurements in the same rapidity region, the cross sections of prompt D + and D$^+_s$ mesons have an extended pT coverage and total uncertainties reduced by a factor ranging from 1.05 to 1.6, depending on pT, allowing for a more precise determination of their pT-integrated cross sections. The results are well described by perturbative QCD calculations. The fragmentation fraction of heavy quarks to strange mesons divided by the one to non-strange mesons, f s /(f u + f d ), is compatible for charm and beauty quarks and with previous measurements at different centre-of-mass energies and collision systems. The $b\bar{b}$ production cross section per rapidity unit at midrapidity, estimated from non-prompt D-meson measurements, is d$σ_{b\bar{b}}$/d$y$| |y|<0.5 = $34.5 ± 2.4(stat)^{+4.7}_{-2.9}$(tot.syst) μb. It is compatible with previous measurements at the same centre-of-mass energy and with the cross section pre- dicted by perturbative QCD calculations.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2024

Measurement of beauty-quark production in pp collisions at $\sqrt{s}$ = 13 TeV via non-prompt D mesons

The p T -diferential production cross sections of non-prompt D 0 , D + , and D$^+_s$ at a centre-of-mass energy $\sqrt{s}$ = 13 TeV. The measurements are performed at midrapidity, |y| < 0.5, with the data sample collected by ALICE from 2016 to 2018. The results are in agreement with predictions from several perturbative QCD calculations. The fragmentation fraction of beauty quarks to strange mesons divided by the one to non-strange mesons, $f_s$/($f_u$ +$f_d$), is found to be 0.114 ± 0.016 (stat.) ± 0.006 (syst.) ± 0.003 (BR) ± 0.003 (extrap.). This value is compatible with previous measurements at lower centre-of-mass energies and in diferent collision systems in agreement with the assumption of universality of fragmentation functions. In addition, the dependence of the non-prompt D meson production on the centre of-mass energy is investigated by comparing the results obtained at $\sqrt{s}$ = 5.02 and 13 TeV, showing a hardening of the non-prompt D-meson p T -diferential production cross section at higher $\sqrt{s}$. Finally, the $b\overline{b}$ production cross section per unit of rapidity at midrapidity is calculated from the non-prompt D 0 , D + , D$^+_s$, and $Λ^+_c$ hadron measurements, obtaining dσ/dy = 75.2 ± 3.2 (stat.) ± 5.2 (syst.)$^{+12.3}_{-3.2}$ (extrap.) µb.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2020

Impact of divertor material on neutral recycling and discharge fueling in DIII-D

We report that experiments with the lower divertor of DIII-D during the Metal Rings Campaign (MRC) show that the fraction F of atomic D in the total recycling flux is material-dependent and varies through the ELM cycle, which may affect divertor fueling. Between ELMs, F C ~ 10% and FW ~ 40%, consistent with expectations if all atomic recycling is due to reflections. During ELMs, F C increases to 50% and F W to 60%. In contrast, the total D recycling coefficient including atoms and molecules R stays close to unity near the strike point where the surface is saturated with D. During ELMs, R can deviate from unity, increasing during high energy ELM-ion deposition (net D release) and decreasing at the end of the ELM which leads to ability of the target to trap the ELM-deposited D. The increase of R > 1 in response to an increase in ion impact energy Ei has been studied with small divertor target samples using Divertor Materials Evaluation System (DiMES). An electrostatic bias was applied to DiMES to change E i by 90 eV. On all studied materials including C, Mo, uncoated and W-coated TZM (>99% Mo, Ti, and Zr alloy), W, and W fuzz, an increase of E i transiently increased the D yield (and R) by ~10%. On C there was also an increase in the molecular D 2 yield, probably due to ion-induced D 2 desorption. Despite the measured increase in F on W compared to C, attached H-mode shots with OSP on W during MRC did not demonstrate a higher pedestal density. About 8% increase in the edge density could be seen only in attached L-mode scenarios. The difference can be explained by higher D trapping in the divertor and lower divertor fueling efficiency in H- versus L-mode.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2024

Search for J / ψ weak decays containing a D meson

Using a sample of about 10 billion J / ψ events with the BESIII detector, we search for the weak decays of J / ψ → D ¯ 0 π 0 + c . c . , J / ψ → D ¯ 0 η + c . c . , J / ψ → D ¯ 0 ρ 0 + c . c . , J / ψ → D − π + + c . c . , and J / ψ → D − ρ + + c . c . . Since no significant signal is observed, we set the upper limits of the branching fractions of these decays to be B ( J / ψ → D ¯ 0 π 0 + c . c . ) < 4.7 × 10 − 7 , B ( J / ψ → D ¯ 0 η + c . c . ) < 6.8 × 10 − 7 , B ( J / ψ → D ¯ 0 ρ 0 + c . c . ) < 5.2 × 10 − 7 , B ( J / ψ → D − π + + c . c . ) < 7.0 × 10 − 8 , and B ( J / ψ → D − ρ + + c . c . ) < 6.0 × 10 − 7 at the 90% confidence level. Published by the American Physical Society 2024

Astronomy & Astrophysics↗

DOE OSTI2024

First observation of Λ b 0 → Σ c ( * ) + + D ( * ) − K − decays

The four decays, Λ b 0 → Σ c ( * ) + + D ( * ) − K − , are observed for the first time using proton-proton collision data collected with the LHCb detector at a center-of-mass energy of 13 TeV, corresponding to an integrated luminosity of 6 fb − 1 . By considering the Λ b 0 → Λ c + D ¯ 0 K − decay as reference channel, the following branching fraction ratios are measured to be B ( Λ b 0 → Σ c + + D − K − ) B ( Λ b 0 → Λ c + D ¯ 0 K − ) = 0.282 ± 0.016 ± 0.016 ± 0.005 , B ( Λ b 0 → Σ c * + + D − K − ) B ( Λ b 0 → Σ c + + D − K − ) = 0.460 ± 0.052 ± 0.028 , B ( Λ b 0 → Σ c + + D * − K − ) B ( Λ b 0 → Σ c + + D − K − ) = 2.261 ± 0.202 ± 0.129 ± 0.046 , B ( Λ b 0 → Σ c * + + D * − K − ) B ( Λ b 0 → Σ c + + D − K − ) = 0.896 ± 0.137 ± 0.066 ± 0.018 , where the first uncertainties are statistical, the second are systematic, and the third are due to uncertainties in the branching fractions of intermediate particle decays. These initial observations mark the beginning of pentaquark searches in these modes, with more datasets to become available following the LHCb upgrade. © 2024 CERN, for the LHCb Collaboration 2024 CERN

Aaij, R. (ORCID:0000000305331952)↗

DOE OSTI2020

Transverse-momentum and event-shape dependence of D-meson flow harmonics in Pb–Pb collisions at s NN = 5.02 TeV

The elliptic and triangular flow coefficients v 2 and v 3 of prompt D 0 , D + , and D * + mesons were measured at midrapidity ( | y | < 0.8 ) in Pb–Pb collisions at the centre-of-mass energy per nucleon pair of s NN = 5.02 TeV with the ALICE detector at the LHC. The D mesons were reconstructed via their hadronic decays in the transverse momentum interval 1 < p T < 36 GeV / c in central (0–10%) and semi-central (30–50%) collisions. Compared to pions, protons, and J / ψ mesons, the average D-meson v n harmonics are compatible within uncertainties with a mass hierarchy for p T ≲ 3 GeV / c , and are similar to those of charged pions for higher p T . The coupling of the charm quark to the light quarks in the underlying medium is further investigated with the application of the event-shape engineering (ESE) technique to the D-meson v 2 and p T -differential yields. The D-meson v 2 is correlated with average bulk elliptic flow in both central and semi-central collisions. Within the current precision, the ratios of per-event D-meson yields in the ESE-selected and unbiased samples are found to be compatible with unity. All the measurements are found to be reasonably well described by theoretical calculations including the effects of charm-quark transport and the recombination of charm quarks with light quarks in a hydrodynamically expanding medium.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2020

Efficient 3-D velocity model building using joint inline and crossline plane-wave wave-equation migration velocity analyses

SUMMARY Wave-equation migration velocity analysis (WEMVA) is an image-domain inversion method for velocity model building. Automatic plane-wave WEMVA (PWEMVA) calculates the moveouts of plane-wave common-image gathers (CIGs) by searching a best-fitting parabola with semblance analysis and backprojects residual CIG moveouts into wavefield wave paths with a reflection tomographic kernel. However, 3-D PWEMVA is very computationally expensive because 3-D reflection tomographic inversion requires at least five 3-D reverse-time migrations per iteration and stores two types of source wavefields at model boundaries. We develop a joint inline and crossline PWEMVA method for efficient 3-D velocity model building. We alternatively implement the inline and crossline PWEMVAs with a constraint for each other, in which we iteratively construct the 3-D velocity model update through 1-D spline interpolation of 2-D gradients. The inline and crossline joint inversion is practical since PWEMVA only inverts for low-wavenumber velocity perturbations along wave paths, and the method can take less than 1 per cent of the computational cost of full 3-D PWEMVA. To construct unaliased plane waves for our joint inline and crossline PWEMVA, we develop a 3-D data interpolation method in the frequency–wavenumber (FK) domain to recover regularly and randomly missing traces. The method minimizes the misfit on sufficiently localized data subsets with iterative optimal step lengths and a gradient preconditioner that iteratively selects dominant dips along different azimuths. In numerical experiments, we use a 3-D synthetic seismic data set and a land 3-D field seismic data set acquired at the Farnsworth CO2-EOR (enhanced oil recovery) field to demonstrate the efficacy of our velocity model building and data interpolation methods.

Liu, Xuejian↗

DOE OSTI2025

Radioisotope Science and Technology Division FY 2025 Core R&D Summary Report: Competitive Projects, Postdoctoral Researchers, and Student Interns

R&D efforts in support of the Oak Ridge National Laboratory (ORNL) Isotope Program Radioisotope Portfolio are led by the Radioisotope Science and Technology Division (RSTD). In addition to supporting the ORNL Isotope Program Radioisotope Portfolio, RSTD supports a portfolio of research related to fundamental properties of radioisotopes and radioisotope applications, including diagnostic and therapeutic uses of medical radioisotopes, radioisotopes for national security, and the production of 238 Pu for the National Aeronautics and Space Administration (NASA) and US Department of Energy (DOE) Office of Nuclear Energy. RSTD is organized into functional science and engineering groups, with most staff members supporting multiple programs. The goal of this organization is to enable synergy between programs such that R&D advances coming from other programs may provide benefit to the ORNL Isotope Program. R&D within RSTD is focused around addressing five grand challenges, as documented in the strategic plan for the DOE Office of Isotope R&D and Production, or DOE Isotope Program (IP), Radioisotope Production R&D activities at ORNL: 1. Maximizing the scientific output of radioisotope transmutation resources, 2. Maximizing the scientific output of radioisotope processing resources, 3. Minimizing waste and having optimal waste disposition, 4. Focusing on product quality and reliability, and 5. Expanding the use of beneficial isotopes. The ORNL Core R&D program, one of the primary R&D components within the ORNL Isotope Program Radioisotope Portfolio, ranges from benchtop to demonstration activities, with a focus on researching enhanced production techniques, developing emerging isotopes, and developing the talent pipeline for radioisotope science and technology. Projects within the Core R&D Program are led primarily by RSTD staff members. In supporting enhanced production techniques, the Core R&D program presents an opportunity to fund novel R&D that might not be tied to a specific radioisotope product but still presents a high potential for broad applicability in the longer term. In supporting the development of emerging isotopes, the Core R&D program develops high-priority isotopes that are not able to be fully supported through production funds.

07 ISOTOPE AND RADIATION SOURCES↗

DOE OSTI2024

Search for Rare Decays of D s + to Final States π + e + e − , ρ + e + e − , π + π 0 e + e − , K + π 0 e + e − , and K S 0 π + e + e −

Using 7.33 fb − 1 of e + e − collision data collected by the BESIII detector at center-of-mass energies in the range of s = 4.128 – 4.226 GeV , we search for the rare decays D s + → h + ( h 0 ) e + e − , where h represents a kaon or pion. By requiring the e + e − invariant mass to be consistent with a ϕ ( 1020 ) , 0.98 < M ( e + e − ) < 1.04 GeV / c 2 , the decay D s + → π + ϕ , ϕ → e + e − is observed with a statistical significance of 7.8 σ , and evidence for the decay D s + → ρ + ϕ , ϕ → e + e − is found for the first time with a statistical significance of 4.4 σ . The decay branching fractions are measured to be B ( D s + → π + ϕ , ϕ → e + e − ) = ( 1.1 7 − 0.21 + 0.23 ± 0.03 ) × 10 − 5 , and B ( D s + → ρ + ϕ , ϕ → e + e − ) = ( 2.4 4 − 0.62 + 0.67 ± 0.16 ) × 10 − 5 , where the first uncertainties are statistical and the second systematic. No significant signals for the three four-body decays of D s + → π + π 0 e + e − , D s + → K + π 0 e + e − , and D s + → K S 0 π + e + e − are observed. For D s + → π + π 0 e + e − , the ϕ mass region is vetoed to minimize the long-distance effects. The 90% confidence level upper limits set on the branching fractions of these decays are in the range of ( 7.0 – 8.1 ) × 10 − 5 . Published by the American Physical Society 2024

Physics↗

DOE OSTI2025

Poisson Equation for a (General) Homogeneous d-Dimensional Ellipsoid with Applications to Beam Envelope Tracking

This note describes the solution of the free-space Poisson equation in the interior of a $d$-dimensional homogeneous ellipsoid, and the associated space charge fields. An explicit formula (\ref{Sformula}) is provided that relates the $d\times d$ matrix describing the space charge (quadratic) potential to the $d\times d$ covariance matrix of the ellipsoid. For the cases $d=2$ and $d=3$, this result is used to determine the linear map corresponding to a space charge kick, that may be used to push the beam $6\times 6$ covariance matrix during envelope tracking. The treatment of upright ellipsoids for $d=2$ and $d=3$ is well-represented in the literature. However, the approach taken here emphasizes a general ellipsoid with arbitrary correlations in any dimension. The Appendix provides a general solution of the free-space Poisson equation in dimension $d$ for a source distribution with ellipsoidal symmetry.

97 MATHEMATICS AND COMPUTING↗

DOE OSTI2024

Overview of T and D–T results in JET with ITER-like wall

In 2021 JET exploited its unique capabilities to operate with T and D–T fuel with an ITER-like Be/W wall (JET-ILW). This second major JET D–T campaign (DTE2), after DTE1 in 1997, represented the culmination of a series of JET enhancements—new fusion diagnostics, new T injection capabilities, refurbishment of the T plant, increased auxiliary heating, in-vessel calibration of 14 MeV neutron yield monitors—as well as significant advances in plasma theory and modelling in the fusion community. DTE2 was complemented by a sequence of isotope physics campaigns encompassing operation in pure tritium at high T-NBI power. Carefully conducted for safe operation with tritium, the new T and D–T experiments used 1 kg of T (vs 100 g in DTE1), yielding the most fusion reactor relevant D–T plasmas to date and expanding our understanding of isotopes and D–T mixture physics. Furthermore, since the JET T and DTE2 campaigns occurred almost 25 years after the last major D–T tokamak experiment, it was also a strategic goal of the European fusion programme to refresh operational experience of a nuclear tokamak to prepare staff for ITER operation. The key physics results of the JET T and DTE2 experiments, carried out within the EUROfusion JET1 work package, are reported in this paper. Progress in the technological exploitation of JET D–T operations, development and validation of nuclear codes, neutronic tools and techniques for ITER operations carried out by EUROfusion (started within the Horizon 2020 Framework Programme and continuing under the Horizon Europe FP) are reported in (Litaudon et al Nucl. Fusion accepted), while JET experience on T and D–T operations is presented in (King et al Nucl. Fusion submitted).

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗