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At least 253 records · Page 14

Marangoni effect induced convection in material processing under microgravity (M-18)

On the ground the upper layer of the liquid in a vessel heated from below becomes hotter than the lower layer. This well-known phenomenon results from buoyancy-induced convection. Though this means that the buoyancy-induced convection is not dominant under microgravity conditions in space, another convection called Marangoni convection may possibly occur. This convection results from an intermolecular force which acts on a free surface, that is surface tension. Since it is stronger at lower temperatures, the liquid surface near the heated wall is pulled to the cooled side as shown. This surface movement causes the inner convection. Marangoni convection, however, may be negligible on the Earth, for the molecular force is generally smaller than buoyancy. Various tests on material processing were recently conducted in space and some high quality crystals free from buoyancy convection were obtained. But, at the same time, others proved to be less uniform than expected in the components' distribution. This nonuniformity seems to be mainly caused by Marangoni convection. It is, therefore, very important to know how to control the convection by studying its characteristics, but the problem is that on the ground it is impossible to carry out the experiment without gravity. That is what a space experiment aboard the space shuttle is planned as the First Material Processing Tests (FMPT) of Japan. The experiment on Marangoni flow visualization is being performed in order to investigate the characteristics of convection in uni-dimensional melt growth under microgravity conditions.

Enya, S.↗

Cumulus cloud venting of mixed layer ozone

Observations are presented which substantiate the hypothesis that significant vertical exchange of ozone and aerosols occurs between the mixed layer and the free troposphere during cumulus cloud convective activity. The experiments utilized the airborne Ultra-Violet Differential Absorption Lidar (UV-DIAL) system. This system provides simultaneous range resolved ozone concentration and aerosol backscatter profiles with high spatial resolution. Evening transects were obtained in the downwind area where the air mass had been advected. Space-height analyses for the evening flight show the cloud debris as patterns of ozone typically in excess of the ambient free tropospheric background. This ozone excess was approximately the value of the concentration difference between the mixed layer and free troposphere determined from independent vertical soundings made by another aircraft in the afternoon.

Ching, J. K. S.↗

Cumulus cloud venting of mixed layer ozone

Observations are presented which substantiate the hypothesis that significant vertical exchange of ozone and aerosols occurs between the mixed layer and the free troposphere during cumulus cloud convective activity. The experiments utilized the airborne Ultra-Violet Differential Absorption Lidar (UV-DIAL) system. This system provides simultaneous range resolved ozone concentration and aerosol backscatter profiles with high spatial resolution. Evening transects were obtained in the downwind area where the air mass had been advected. Space-height analyses for the evening flight show the cloud debris as patterns of ozone typically in excess of the ambient free tropospheric background. This ozone excess was approximately the value of the concentration difference between the mixed layer and free troposphere determined from independent vertical soundings made by another aircraft in the afternoon.

Ching, J. K. S.↗

Growth of Si spherical crystals and the surface oxidation (M-9)

Nearly 90 percent of semiconductor devices are produced with Si single crystals as the starting materials. For instance, the integrated circuits (IC), which are used in almost all electronic equipments such as TV, tape recorders, audio amplifiers, etc., are made after various processings of Si single crystal wafers. In these wafers, the same controlled amounts of impurities are added and the uniformities in their distributions are extremely important. Growth under microgravity makes it possible to eliminate the buoyancy-driven convection in the melt, which is one of the main origins of convections which results in non-uniformity of the impurity. Another source of convection is known as Marangoni convection which is driven on the free surface when a temperature gradient occurs. One of the merits of microgravity experimentation is that the detailed study of this convection becomes possible. Another important advantage of microgravity is that growth of crystals without a crucible is possible. This makes it possible to study melt growth without the strain which is usually introduced on the ground. Nevertheless, we should repeat and analyze many growth experiments in space to get reliable results. However, since in the FMPT, the time for the experiment is limited, we plan to carry out two kinds of very simple and basic experiments as the first step for the semiconductor growth experiment. In the first experiment, we use single crystal Si sphere as the starting material and as shown, this sphere is heated in the furnace at a slightly higher temperature than the melting point. After the melting front moves nearly half way to its center, the temperature is decreased to stop the melting and to start the growth from the seed for which we use the unmelted solid party of the sphere. The sphere is centered by quartz protuberances inside of the quartz crucible. There exists the possibility of temperature fluctuations being introduced when the molten sphere occasionally touches the protuberances. The total time needed for the melting and the growth processes is estimated to be 30 minutes. Infrared emission from the sphere is monitored in order to prevent the accidental loss of the central solid core. The schematical illustration of the second experient is shown. A single crystal, Si rod is used as the starting material. In the first stage, the rod is melted from one end to obtain a liquid sphere. In the second stage, the single crystal is grown by decreasing the temperature from the unmelted part of the rod which is used as the seed. The second experient somewhat resembles the Czochralski method used on the ground; however, in the space experiment, no crucible is employed and the temperature uniformity is much superior. In both experiments, phosphorous is doped to allow observation of the change in the shape of the liquid solid interface during crystal growth and the impurity striations, if any.

Nishinaga, Tatau↗

Surface tension driven convection

In a normal gravitational environment, the free surface of a liquid in a container plays a passive role in the transport processes. However, at microgravity, the free surface can become the dominant factor. A simple but meaningful spaceflight experiment is proposed to investigate the nature and extent of flows induced by surface-tension gradients along the free surface. The influences of container geometry, wetability, contamination, and imposed heating modes will be investigated.

Ostrach, S.↗

Low-gravity experiments on Liquid Phase Miscibility Gap (LPMG) alloys: Materials Experiments Assembly (MEA)

Space shuttle experiments which study the massive separation which occurred during sounding rocket Al-In alloy tests are described. The gradient cool experiment studies surface tension driven droplet migration and particle pushing in an LPMG alloy. Isothermal experiments on the Te-Tl alloys test the hypothesis that LPMG systems with low surface energies produce relatively fine, and uniform emulsions and dispersions. It also examines the effect of droplet concentration on phase separation kinetics. Isothermal plunger experiments on Al-In alloys determine whether surface tension driven convection currents originating at a free surface contribute to massive separation. They ascertain whether In-rich droplets migrate under the action of a temperature gradient when they are not influenced by the crucible walls.

Gelles, S. H.↗

Space shuttle experiments on Al-In liquid phase miscibility gap (LPMG) alloys

Massive phase separation observed at low-g was studied during the phase separation process while cooling through the miscibility gap under a controlled thermal gradient was investigated. The molten drops which form during the phase separation process appear to move in a direction opposite to that predicted by the theory of thermocapillary droplet motion. A second experiment utilized a plunger arrangement designed to eliminate the surface tension driven convection currents originating at a free surface. This experiment suggests that the free surface does contribute to the coalescence process but that there are other mechanisms which are more important.

Gelles, S. H.↗

Space Station Freedom research capabilities

NASA's plan for enhancing space-based research capabilities begins with extended-duration Space Shuttle missions that will double the research capability currently provided by Spacelab and culminate in Space Station Freedom. The 14-day USML 1 mission flown on the Space Shuttle in June 1992 was a space station precursor mission, dedicated to microgravity and life science research. Freedom will be a permanent space-based research facility, providing a working environment nearly free of buoyancy-driven convection, sedimentation, and hydrostatic pressure and featuring access to the ultra-high vacuum of space (for external payloads). In its crew-tended phase, Space Station Freedom will provide 40 times Spacelab's capability, and in its permanently occupied phase, Freedom will provide 110 times Spacelab's capability. (The Russian space station, Mir, offers 26 times Spacelab's capabilities.) According to NASA's current schedule, the first launch of a space station element will take place in November 1995, with permanently occupied capability planned for September 1999. This year, NASA will conduct space station critical design reviews (CDR's). Work package design reviews will take place from February to April 1993, followed by a systems CDR.

Moorehead, Robert↗

Development of an infrared imaging system for the surface tension driven convection experiment

An infrared imaging system is used to quantify the imposed surface temperature distribution along a liquid/gas free surface in support of the Surface Tension Driven Convection Experiment, a planned Space Transportation System flight experiment. For ground-based work a commercially available instrument was used to determine the feasibility of using the type of imaging system for this experiment. The ground-based work was used as a baseline for compiling specifications for a flight qualified imager to be designed, fabricated, tested and qualified for flight. The requirements and specifications for the flight model are given along with the reasons for departures from the ground-based equipment. The flight qualification requirements discussed are a representative sample of the necessary procedures which must be followed to flight qualify diagnostic equipment for use aboard the STS. The potential problems and concerns associated with operating an imaging system in orbit are also discussed.

Pline, Alexander D.↗

Development of an infrared imaging system for the surface tension driven convection experiment

An infrared imaging system is used to quantify the imposed surface temperature distribution along a liquid/gas free surface in support of the Surface Tension Driven Convection Experiment, a planned Space Transportation System flight experiment. For ground-based work a commercially available instrument was used to determine the feasibility of using this type of imaging system for this experiment. The ground-based work was used as a baseline for compiling specifications for a flight qualified imager to be designed, fabricated, tested and qualified for flight. The requirements and the specifications for the flight model are given along with the reasons for departures from the ground-based equipment. The flight qualification requirements discussed are a representative sample of the necessary procedures which must be followed to flight qualify diagnostic equipment for use aboard the STS. The potential problems and concerns associated with operating an imaging system on orbit are also discussed.

Pline, Alexander D.↗

Combined buoyancy-thermocapillary convection

Combined buoyancy-thermocapillary convection was studied in 2D and 3D. Fluid motion caused by thermally induced tension gradients on the free surface of a fluid is termed thermocapillary convection. It is well-known that in containerless processing of materials in space, thermocapillary convection is a dominant mechanism of fluid flow. Welding and crystal growth processes are terrestrial applications where thermocapillary convection has direct relevance.

Homsy, G. M.↗

Surface temperature distribution along a thin liquid layer due to thermocapillary convection

The surface temperature distributions due to thermocapillary convections in a thin liquid layer with heat fluxes imposed on the free surface were investigated. The nondimensional analysis predicts that, when convection is important, the characteristics length scale in the flow direction L, and the characteristic temperature difference delta T sub o can be represented by L and delta T sub o approx. (A2Ma)/1/4 delta T sub R, respectively, where L sub R and delta sub R are the reference scales used in the conduction dominant situations with A denoting the aspect ratio and Ma the Marangoni number. Having L and delta sub o defined, the global surface temperature gradient delta sub o/L, the global thermocapillary driving force, and other interesting features can be determined. Numerical calculations involving a Gaussian heat flux distribution are presented to justify these two relations.

Lai, C. L.↗

Surface temperature distribution along a thin liquid layer due to thermocapillary convection

The surface temperature distributions due to thermocapillary convections in a thin liquid layer with heat fluxes imposed on the free surface were investigated. The nondimensional analysis predicts that, when convection is important, the characteristics length scale in the flow direction L, and the characteristic temperature difference delta T sub o can be represented by L and delta T sub o approx. (A2Ma)/1/4 delta T sub R, respectively, where L sub R and delta sub R are the reference scales used in the conduction dominant situations with A denoting the aspect ratio and Ma the Marangoni number. Having L and delta sub o defined, the global surface temperature gradient delta sub o/L, the global thermocapillary driving force, and other interesting features can be determined. Numerical calculations involving a Gaussian heat flux distribution are presented to justify these two relations.

Lai, C.-L.↗

Marangoni instability in a liquid layer with two free surfaces

The onset of the Marangoni instability in a liquid layer with two free nearly insulating surfaces heated from below is studied. Linear stability analysis yields a condition for the emergence of a longwave or a finite wavelength instability from the quiescent equilibrium state. Using the method of asymptotic expansions, a weakly nonlinear evolution equation describing the spatiotemporal behavior of the velocity and temperature fields at the onset of the longwave instability is derived. The latter is given by delta(M) = 24, delta(M) being the difference between the upper and the lower Marangoni numbers. It is shown that in some parametric range one convective cell forms across the layer, while in other parametric domains two convective cells emerge between the two free surfaces.

Deissler, Robert J.↗

Oscillatory thermocapillary flows

Experimental and theoretical research conducted to understand the physical mechanism of oscillatory thermocapillary convection is discussed. A physical model that plausibly describes the cause of thermocapillary flow oscillations and to yield the proper parameters for identifying their onset is considered. Strong convection indicated by a large Marangoni number, as well as free surface deformation, appear to be important factors for the onset of the convection.

Ostrach, S.↗

Effect of convective Mach number on mixing of coaxial circular and rectangular jets

Rectangular supersonic free and coaxial jets were used to enhance mixing relative to a circular jet in a convective Mach number range of 0.5 to 2.2. The different convective Mach numbers were obtained by changing the central jet gas composition, the temperatures of the inner and outer flows, and the velocity of the coaxial flow. The experimental techniques used were schlieren photography, total pressure, and gas-sampling measurements. For all test conditions the rectangular jets showed substantial improved mixing relative to a circular jet. The free jets showed high mixing in the circumferential region of the jet while the coaxial jet had a high mixing rate inside the central jet.

Gutmark, E.↗

Curvature, Variable Density and Compressibility Effects in Turbulent Shear Layers

The combined effects of variable density, curvature, and convective Mach number on turbulence in time-developing free shear layers are studied using turbulence-resolving simulations. The range of parameters considered include the convective Mach number at 0.2 and 0.8, the density ratio at 1/7, 1 and 7, and the level of streamwise curvature, measured by the shear layer thickness ratio to the radius of curvature at 0.001 and 0.01. Simulations at the limit of zero curvature exhibit mean profiles and turbulent stresses comparable with previously simulated planar (non-curved) shear layers. Growth rate changes depending on compressibility, curvature and density ratio are compared with expected behavior and unexpected trends due to combined effects are investigated. Standard turbulent shear layer statistics are presented, including spreading rates, turbulent stresses, and stress budgets to characterize individual and combined effects of the selected physical parameters.

shear layer↗

Asian Influence Over the Western North Pacific during the Fall Season: Inferences from Lead 210, Soluble Ionic Species and Ozone

Aerosol samples collected over the western Pacific during the NASA/Global Tropospheric Experiment Pacific Exploratory Mission (PEM-West A) expedition (September - October 1991) revealed mean Pb-210 concentrations in the free troposphere in the 5-10 fCi m(exp -3) STP range. Most soluble ionic aerosol-associated species were near detection limits [much less than 40 parts per trillion by volume (pptv)] in these same samples. The altitude distribution of O3 near Asia closely resembled that of Pb-210, while no relationship was found between the concentrations of O3 and Be-7. Free tropospheric air over the western Pacific was depleted in soluble aerosol-associated species but enriched in Pb-210 and O3, indicative of deep wet convection over the Asian continent. The influence of Asian air on the composition of the free troposphere over the western Pacific was evident on most of the PEM-West A flights. However, evidence of continental influence was largely restricted to those species that are relatively insoluble (or have insoluble precursors), hence escape scavenging during vertical transport from the boundary layer into the free troposphere by wet convective activity.

Dibb, J. E.↗