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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 253 records · Page 14
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NASA NTRS1989

Chemical stratification in white dwarf atmospheres and envelopes

Theoretical arguments supporting a new mechanism maintaining a homogeneously mixed composition in white dwarf atmospheres with traces of helium are presented. Diffusion time scales, meridional circulation, mass loss, accretion of interstellar matter, convection, and radiative levitation are discussed. Theoretically, layered envelopes, with hydrogen on top of helium and an abundance profile in the transition layer determined by diffusion equilibrium, are expected. In cases with observed helium and hydrogen in the atmosphere this means that the total hydrogen mass must be very small. The empirical evidence for such atmospheres are assessed, using a new grid of model atmospheres with stratified element abundances and applying it to typical mixed abundance cases at the hot end of the white dwarf temperature sequence.

Koester, D.↗
NASA NTRS1989

Laboratory investigation of electric charging of dust particles by electrons, ions, and UV radiation

In many cosmic environments electric charging of dust particles occurs by electrons, ions, and UV radiation. In case of interstellar dust particles the value of their electric charge can have, for instance, very important consequences for their destruction rate in supernova remnant's shock waves and can globally influence the overall life cycle of dust particles in galaxies. For experimental simulation of charging processes a vacuum chamber was used in which the particles fall through an electron or ion beam of energies up to 10 KeV. The aim of the experiments was to attain maximum charge of dust particles. Furthermore the influence of the rest gas was also determined because electrons and ions produced by collisional ionization of the rest gas can result in significant effects. For measurement particles from 1 to 100 microns from glass, carbon, Al, Fe, MgO, and very loosely bound conglomerates of Al2O3 were used.

Svestka, Jiri↗
NASA NTRS1992

The ultraviolet and visible spectrum of the polycyclic aromatic hydrocarbon C10H8(+) - Possible contributions to the diffuse interstellar bands and to the ultraviolet-visible extinction

The properties of the cation of the PAH naphthalene (C10H8(+)) isolated in inert gas matrices under conditions relevant to astrophysical environments are described. The band at 6741 A is the strongest and falls close to the weak 6742 A diffuse interstellar bands (DIBs). Five other weaker bands also fall remarkably close to the positions of known DIBs. A very intense and broad continuum extended from the UV to the visible, which seems to be associated with the ion, is reported. The molar absorption coefficient at the peak of the continuum is 2.0 x 10 exp 6 cu dm/mol cm. If a continuum is a general property of PAH cations, this characteristic will have a strong impact on the understanding of how PAHs convert interstellar UV and visible radiation into IR radiation.

Salama, F.↗
NASA NTRS1993

Neutral and ionized polycyclic aromatic hydrocarbons, diffuse interstellar bands and the ultraviolet extinction curve

Neutral naphthalene C10H8, phenanthrene C14H10 and pyrene C16H10 absorb strongly in the ultraviolet region and may contribute to the extinction curve. High abundances are required to produce detectable structures. The cations of these polycyclic aromatic hydrocarbons (PAHs) absorb in the visible C10H8(+) has 13 discrete absorption bands which fall between 6800 and 4500 A. The strongest band at 6741 A falls close to the weak 6742 A diffuse interstellar band (DIB). Five other weaker bands also match DIBs. The possibility that C10H8(+) is responsible for some of the DIBs can be tested by searching for new DIBs at 6520 and 6151 A, other strong naphthalene cation band positions. If C10H8(+) is indeed responsible for the 6742 A feature, it accounts for 0.3% of the cosmic carbon. The spectrum of C16H10(+) is dominated by a strong band at 4435 A in an Ar matrix and 4395 A in Ne, wavelengths which fall very close to the strongest DIB at 4430 A. If C16H10(+) or a closely related pyrene-like ion, is indeed responsible for the 4430 A feature, it accounts for 0.2% of the cosmic carbon. An intense, very broad UV-to-visible continuum is reported which is associated with both ions and could explain how PAHs convert interstellar UV and visible radiation into IR radiation.

Salama, Farid↗
NASA NTRS1995

Polycyclic aromatic hydrocarbon ions and the diffuse interstellar bands

Neutral naphthalene (C10H8), phenanthrene (C14H10), and pyrene (C16H10) absorb strongly in the ultraviolet and may contribute to the extinction curve. High abundances are required to produce detectable structures. The cations of these Polycyclic Aromatic Hydrocarbons (PAHs) absorb in the visible. C10H8(+) has 12 discrete absorption bands which fall between 6800 and 5000 A. The strongest band at 6741 A falls close to the weak 6742 A diffuse interstellar band (DIB). Five other weaker bands also match DIBs. The possibility that C10H8(+) is responsible for some of the DIBs can be tested by searching for new DIBS at 6520, 6151, and 5965 A, other moderately strong naphthalene cation band positions. If C10H8(+) is indeed responsible for the 6742 A feature, it accounts for 0.3% of the cosmic carbon. The spectrum of C16H10(+) is dominated by a strong band at 4435 A in an Ar matrix and 4395 A in a Ne matrix, a position which falls very close to the strongest DIB, that at 4430 A. If C16H10(+), or a closely related pyrene-like ion is indeed responsible for the 4430 A feature, it accounts for 0.2% of the cosmic carbon. We also report an intense, very broad UV-to-visible continuum which is associated with both ions and could explain how PAHs convert interstellar UV and visible radiation into IR.

Salama, F.↗
NASA NTRS2004

Photoionization in Ultraviolet Processing of Astrophysical Ice Analogs at Cryogenic Temperatures

Two recent experimental studies have demonstrated that amino acids or amino acid precursors are generated when astrophysical ice analogs are subjected to ultraviolet (UV) irradiation at cryogenic temperatures. Understanding the complete phenomenology of photoprocessing is critical to elucidating chemical reaction mechanisms that can function within an ice matrix under very cold conditions. Pushing beyond the much better characterized study of photolytic dissociation of chemical bonds through electronic excitation, this work explored the ability of UV radiation present in the interstellar medium to ionize small molecules embedded in ices. Quantum chemical calculations, including bulk solvation effects, were used to study the ionization of hydrogen (H2), water, and methanol (CH3OH) bound in small clusters of water. Ionization potentials were found to be much smaller in the condensed phase than in the gas phase; even a small cluster can account for large changes in the ionization potentials in ice, as well as the known formation of an OH--H3O+ pair in the case of H2O photoionization. To gauge the impact of photoionization on subsequent grain chemistry, the reaction between OH and CO in the presence of H3O+ was studied and compared with the potential energy surface without hydronium present, which is relevant to chemistry following photolysis. The differences indicate that the reaction is somewhat more likely to proceed to products (H + CO2) in the case of photoionization.

Woon, David E.↗
NASA NTRS2003

The Chemical Composition and Gas-to-Dust Mass Ratio of Nearby Interstellar Matter

We use recent results on interstellar gas toward nearby stars and interstellar by-products within the solar system to select among the equilibrium radiative transfer models of the nearest interstellar material presented in Slavin & Frisch. For the assumption that O/H - 400 parts per million, models 2 and 8 are found to yield good fits to available data on interstellar material inside and outside of the heliosphere, with the exception of the Ne abundance in the pickup ion and anomalous cosmic-ray populations. For these models, the interstellar medium (ISM) at the entry point to the heliosphere has n(H(sup 0)) = 0.202-0.208/cu cm, n(He(sup 0) = 0.0137-0.0152/cu cm, and ionizations X(H) = 0.29-0.30, X(He) = 0.47-0.51. These best models suggest that the chemical composition of the nearby ISM is approx.60%-70% subsolar if S is undepleted. Both H(0) and H(+) need to be included when evaluating abundances of ions found in warm diffuse clouds. Models 2 and 8 yield an H filtration factor of approx.0.46. Gas-to-dust mass ratios for the ISM toward epsilon CMa are R(sub gd) = 178-183 for solar abundances of Holweger or R(sub gd) = 611-657 for an interstellar abundance standard 70% solar. Direct observations of dust grains in the solar system by Ulysses and Galileo yield R(sub gd) appr0x. 115 for models 2 and 8, supporting earlier results (Frisch and coworkers). If the local ISM abundances are subsolar, then gas and dust are decoupled over small spatial scales. The inferred variation in R(sub gd) over parsec length scales is consistent with the fact that the ISM near the Sun is part of a dynamically active cluster of cloudlets flowing away from the Sco-Cen association. Observations toward stars within approx.500 pc show that R(sub gd) correlates with the percentage of the dust mass that is carried by iron, suggesting that an Fe-rich grain core (by mass) remains after grain destruction. Evidently large dust grains (>10(exp -13) g) and small dust grains (<10(exp -13) g) are not well mixed over parsec length spatial scales in the ISM. It also appears that very small C-dominated dust grains have been destroyed in the ISM within several parsecs of the Sun, since C appears to be essentially undepleted. However, if gas-dust coupling breaks down over the cloud lifetime, the missing mass arguments applied here to determine R(sub gd) and dust grain mineralogy are not appropriate.

Frisch, Priscilla C.↗
NASA NTRS2010

Environmental Impact Specification for Direct Space Weathering of Kuiper Belt and Oort Cloud Objects

The Direct Space Weathering Project of NASA's Outer Planets Research Program addresses specification of the plasma and energetic particle environments for irradiation and surface chemical processing of icy bodies in the outer solar system and the local interstellar medium. Knowledge of the radiation environments is being expanded by ongoing penetration of the twin Voyager spacecraft into the heliosheath boundary region of the outer heliosphere and expected emergence within the next decade into the very local interstellar medium. The Voyager measurements are being supplemented by remote sensing from Earth orbit of energetic neutral atom emission from this boundary region by NASA's Interstellar Boundary Explorer (IBEX). Although the Voyagers long ago passed the region of the Classical Kuiper Belt, the New Horizons spacecraft will encounter Pluto in 2015 and thereafter explore one or more KBOs, meanwhile providing updated measurements of the heliospheric radiation environment in this region. Modeling of ion transport within the heliosphere allows specification of time-integrated irradiation effects while the combination of Voyager and IBEX data supports projection of the in-situ measurements into interstellar space beyond the heliosheath. Transformation of model ion flux distributions into surface sputtering and volume ionization profiles provides a multi-layer perspective for space weathering impact on the affected icy bodies and may account for some aspects of color and compositional diversity. Other important related factors may include surface erosion and gardening by meteoritic impacts and surface renewal by cryovolcanism. Chemical products of space weathering may contribute to energy resources for the latter.

Cooper, John F.↗
NASA NTRS1990

A new observational approach to investigate the heliospheric interstellar wind interface - The study of extreme and far ultraviolet resonantly scattered solar radiation from neon, oxygen, carbon and nitrogen

One of the outstanding uncertainties in the understanding of the heliosphere concerns the character of the interaction between the outflowing solar wind and the interstellar medium. A new possibility for obtaining information on this topic is suggested. The cosmically abundant elements neon, oxygen, carbon, and nitrogen will be affected differently at their interface passage depending upon the character of this region. Consequently, the distribution of these atoms and their ions will vary within the inner heliosphere. The study of resonantly scattered solar radiation from these species will then provide information on the nature of the interface. A preliminary evaluation of this approach has been carried out, and the results are encouraging. The relevant lines to be studied are in the extreme and far ulraviolet. The existing data in these bands are reviewed; unfortunately, past instrumentation has had insufficient resolution and sensitivity to provide useful information. The capabilities of future approved missions with capabilities in this area are evaluated.

Bowyer, Stuart↗
NASA NTRS1994

Weakly ionized cosmic gas: Ionization and characterization

Since collective plasma behavior may determine important transport processes (e.g., plasma diffusion across a magnetic field) in certain cosmic environments, it is important to delineate the parameter space in which weakly ionized cosmic gases may be characterized as plasmas. In this short note, we do so. First, we use values for the ionization fraction given in the literature, wherein the ionization is generally assumed to be due primarily to ionization by cosmic rays. We also discuss an additional mechanism for ionization in such environments, namely, the photoelectric emission of electrons from cosmic dust grains in an interstellar Far Ultra Violet (FUV) radiation field. Simple estimates suggest that under certain conditions this mechanism may dominate cosmic ray ionization, and possibly also the photoionization of metal atoms by the interstellar FUV field, and thereby lead to an enhanced ionization level.

Rosenberg, M.↗
NASA NTRS1987

Interstellar processes; Proceedings of the Symposium, Grand Teton National Park, WY, July 1-7, 1986

The conference presents papers on the Milky Way as a galaxy; observations of components of the interstellar medium; interstellar magnetic properties; interstellar processes on a galactic scale; dynamical processes in interstellar clouds; interstellar dust grains; interstellar chemical processes; and heating, cooling, and radiative processes. Attention is given to H2 in the Galaxy, hot interstellar gas in the Galactic disk and halo, interstellar magnetic fields, cloud formation and destruction, theoretical approaches to interstellar turbulence, and infrared absorption and emission characteristics of interstellar PAHs. Other topics include gas phase chemical processes in molecular clouds, the chemical evolution of galaxies, and the atomic and molecular physics of interstellar heating and cooling.

Hollenbach, David J.↗
NASA NTRS1989

Red fluorescence and 3-12 micron emission in NGC 2023, HD 44179, M 82, and Lynds 1780

A red excess observed in the Red Rectangle (HD 44179), was attributed to a possible molecular fluorescence mechanism was discovered in NGC 2023 and analyzed in subsequent work in this and other nebulae. An unexpected red light excess was also noticed in a high latitude dark cloud L 1780. The fluorescence was attributed to hydrogenated amorphous carbon by Duley (1985), on the basis of laboratory work. Alternatively, transitions between electronic states of free polycyclic aromatic hydrocarbon molecules, by-passing the cascade along the vibrational states was considered. In L 1780, the red excess was related to the 12 micron emission detected by IRAS. A quantitative comparison of the intensity of the red fluorescence and that of the 3 to 12 micron features is thus warranted in helping assess the physical properties of large interstellar molecules. The red fluorescence radiation, F(R), appears as a bump on the spectra between 0.6 and 0.9 micron. Values were deduced from the spectra for HD 44179, and for the high latitude cloud L 1780. Corrections for the extinction, both interstellar and internal to the nebulae, were included. The 3 to 12 micron brightness, F(IR), was obtained through integration of the spectra for NGC 2023, and for HD 44179 after removal of a smooth continuum due to hot large grains. The values of the ratio of fluorescence flux to the infrared flux, F(R)/F(IR), are summarized. Red fluorescence and infrared radiation are two separate ways to access to the size of the molecules through observation, and it is rewarding that both approaches give similar results. These findings bring a striking coherence into the physical description of the particles, and add further support to the initial attribution of the infrared features to polycyclic aromatic hydrocarbons (PAHs).

Ryter, Charles↗
NASA NTRS1988

The stellar radiation field and the ionization of H and He in the local interstellar medium

Detailed photoionization calculations for the local interstellar medium (LISM) are presented based on constraints imposed by H I column density estimates derived from IUE and Copernicus data toward nearby B stars and hot white dwarfs. It is found that the nearby hot white dwarfs dominate the stellar contributions to the EUV radiation field. Considering stellar contribution to the EUV background alone, the resulting lower limits to the hydrogen and helium fractional ionization in the local diffuse cloud, at the sun, are 0.091 and 0.089, respectively. This result is insensitive to the absorbing geometry of the local cloud. The comparable ionizations of H and He near the sun are due to the lack of absorption from photospheric helium in the hot DA white dwarfs, to the difference in optical depths at wavelengths shortward of the H I and He I ionization edges, and to the fact that the hydrogen ionization controls the electron number density. The derived H and He ionization limits have important implications for the interpretation of the He I and H I backscattering results, for which uncertainties in charge-exchange interactions occurring in or near the heliopause reflect additional significant uncertainties in determining the ionization in the LISM.

Bruhweiler, Frederick C.↗
NASA NTRS2002

Synthesis of HCN and HNC in Ion-Irradiated N2-Rich Ices

Near-IR observations reveal that N2-rich ice containing small amounts of CH4, and CO, is abundant on the surfaces of Triton, a moon of Neptune, and Pluto. N2-rich ices may also exist, in interstellar environments. To investigate the radiation chemistry of such ices we performed a systematic IR study of ion-irradiated Nz-rich mixtures containing CH4 and CO. Irradiation of N2 + CH4 mixtures at 12 K, showed that HCN, HNC, diazomethane, and NH3 were produced. We also found that UV photolysis of these ices produced detectable HCN and HNC. Intrinsic band strengths, A(HCN) and A(HNC), were measured and used to calculate yields of HCN and HNC. Similar results were obtained on irradiation of N2 + CH4 + CO ices at 12 K, with the main difference being the formation of HNCO. In all cases we observed changes on warming. For example, when the temperature of irradiated Nz + CH4 + CO was raised from 12 to 30 K, HCN, HNC, and HNCO reacted with NH3, and OCN-, CN-, N3-, and NH4+ were produced. These ions, appearing at 30 K, are expected to form and survive on the surfaces of Triton, Pluto, and interstellar grains. Our results have astrobiological implications since some of these radiation products are involved in the syntheses of biomolecules such as amino acids and peptides.

Moore, M. H.↗
NASA NTRS1990

An infrared jet in Centaurus A (NGC 5128): Evidence for interaction between the active nucleus and the interstellar medium

In the present study, higher resolution near infrared images of the visually-obscured central region of Centaurus A were obtained in order to investigate the effects of the active nucleus on the surrounding galaxy. Researchers present J(1.25 microns), H(1.65 microns), and K(2.2 microns) images of the central 40 seconds of the galaxy, taken with the Univ. of Texas InSb array camera on the Anglo Australian 3.9 meter telescope. These images reveal a jet extending approx. 10 arcseconds to the northeast of the nucleus at the same position angle as the x ray and radio jets. The infrared jet is most prominent at the shortest wavelength (1.25 microns), where its brightness surpasses that of the nucleus. The blue appearance of the infrared jet is remarkable considering the heavy obscuration that is evident at visual wavelengths. The amount of reddening in the vicinity of the jet is determined from the measured colors of the stellar core of the galaxy, and this value is used to generate an extinction-corrected energy distribution. In contrast to previously studied optical and infrared jets in active nuclei, the short-wavelength prominence of the Cen A jet indicates that it cannot be attributed to synchrotron emission from a beam of relativistic electrons. The remaining viable mechanisms involve an interaction between the interstellar medium and the active nucleus: the infrared radiation from the jet may be due to emission from interstellar gas that has been entrained and heated by the flow of relativistic particles from the nucleus; alternatively, luminous blue stars may have been created by compression of interstellar material by the relativistic plasma. To investigate these proposed mechanisms, near-infrared spectroscopic studies of Cen A are in progress to look for collisionally excited molecular hydrogen emission lines and recombination lines from ionized gas.

Joy, Marshall↗