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At least 253 records · Page 14

Effect of sintering treatment on structural and magnetic properties of Ni{sub 0.5}Co{sub 0.5}Fe{sub 2}O{sub 4} ferrites

Two sets of Ni{sub 0.5}Co{sub 0.5}Fe{sub 2}O{sub 4} ferrites were synthesized using sol-gel method. Both the samples were heat treated at different temperatures. The effect of sintering treatment analyzed on structural and magnetic properties. X-ray diffraction (XRD) and scanning electron microscope (SEM) were used for structural analysis. Alternating gradient magnetometer (AGM) is used for magnetic measurements. In structural analysis, grains size is calculated using Debye - Scherrer’s formula and Williamson-Hall (W-H) plot. From both the techniques, grain size is found nearly same and increased in size with increase sintering temperature. Increased particle size is confirmed from SEM micrographs. Strain value is calculated from intercept of W-H plot. In both the samples, compressive strain in nature is found. Magnetic properties were also varying under different heat treatment. The change in magnetic properties with change in structural change at different sintering treatment is discussed in this report.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Electron and Proton Heating in Transrelativistic Magnetic Reconnection

Hot collisionless accretion flows, such as the one in Sgr A* at our Galactic center, provide a unique setting for the investigation of magnetic reconnection. Here protons are nonrelativistic, while electrons can be ultrarelativistic. By means of 2D particle-in-cell simulations, we investigate electron and proton heating in the outflows of transrelativistic reconnection (i.e., ${\sigma }_{w}\sim 0.1\mbox{--}1$, where the magnetization ${\sigma }_{w}$ is the ratio of magnetic energy density to enthalpy density). For both electrons and protons, we find that heating at high ${\beta }_{{\rm{i}}}$ (here ${\beta }_{{\rm{i}}}$ is the ratio of proton thermal pressure to magnetic pressure) is dominated by adiabatic compression ("adiabatic heating"), while at low ${\beta }_{{\rm{i}}}$ it is accompanied by a genuine increase in entropy ("irreversible heating"). For our fiducial ${\sigma }_{w}=0.1$, the irreversible heating efficiency at ${\beta }_{{\rm{i}}}\lesssim 1$ is nearly independent of the electron-to-proton temperature ratio ${T}_{{\rm{e}}}/{T}_{{\rm{i}}}$ (which we vary from 0.1 up to 1), and it asymptotes to $\sim 2 \% $ of the inflowing magnetic energy in the low-${\beta }_{{\rm{i}}}$ limit. Protons are heated more efficiently than electrons at low and moderate ${\beta }_{{\rm{i}}}$ (by a factor of ~7), whereas the electron and proton heating efficiencies become comparable at ${\beta }_{{\rm{i}}}\sim 2$ if ${T}_{{\rm{e}}}/{T}_{{\rm{i}}}=1$, when both species start already relativistically hot. We find comparable heating efficiencies between the two species also in the limit of relativistic reconnection (${\sigma }_{w}\gtrsim 1$). Finally, our results have important implications for the two-temperature nature of collisionless accretion flows and may provide the subgrid physics needed in general relativistic MHD simulations.

79 ASTRONOMY AND ASTROPHYSICS↗

The Operating Principle of a Fully Solid State Active Magnetic Regenerator

As an alternative refrigeration technology, magnetocaloric refrigeration has the potential to be safer, quieter, more efficient, and more environmentally friendly than the conventional vapor compression refrigeration technology. Most of the reported active magnetic regenerator (AMR) systems that operate based on the magnetocaloric effect use heat transfer fluid to exchange heat, which results in complicated mechanical subsystems and components such as rotating valves and hydraulic pumps. This paper presents an operating principle of a fully solid state AMR, in which an alternative mechanism for heat transfer between the AMR and the heat source/sink is proposed. The operating principle of the fully solid state AMR is based on moving rods/sheets (e.g. copper, brass, iron or aluminum), which are employed to replace the heat transfer fluid. Such fully solid state AMR would provide a significantly higher heat transfer rate than a conventional AMR because the conductivity of moving solid rods/plates is high and it enables the increase in the machine operating frequency hence the cooling capacity. The details of operating principle are presented and discussed here. One of the key enabling features for this technology is the contact between the moving rods/sheets and magnetocaloric material, and heat exchange mechanism at the heat source/sink. This paper provides an overview of the design for a fully solid state magnetocaloric refrigeration system along with guidelines for their optimal design.

Abdelaziz, Omar↗

STRONG SOLAR WIND DYNAMIC PRESSURE PULSES: INTERPLANETARY SOURCES AND THEIR IMPACTS ON GEOSYNCHRONOUS MAGNETIC FIELDS

In this investigation, we first present a statistical result of the interplanetary sources of very strong solar wind dynamic pressure pulses (DPPs) detected by WIND during solar cycle 23. It is found that the vast majority of strong DPPs reside within solar wind disturbances. Although the variabilities of geosynchronous magnetic fields (GMFs) due to the impact of positive DPPs have been well established, there appears to be no systematic investigations on the response of GMFs to negative DPPs. Here, we study both the decompression effects of very strong negative DPPs and the compression from strong positive DPPs on GMFs at different magnetic local time sectors. In response to the decompression of strong negative DPPs, GMFs on the dayside near dawn and near dusk on the nightside, are generally depressed. But near the midnight region, the responses of GMF are very diverse, being either positive or negative. For part of the events when GOES is located at the midnight sector, the GMF is found to abnormally increase as the result of magnetospheric decompression caused by negative DPPs. It is known that under certain conditions magnetic depression of nightside GMFs can be caused by the impact of positive DPPs. Here, we find that a stronger pressure enhancement may have a higher probability of producing the exceptional depression of GMF at the midnight region. Statistically, both the decompression effect of strong negative DPPs and the compression effect of strong positive DPPs depend on the magnetic local time, which are stronger at the noon sector.

79 ASTRONOMY AND ASTROPHYSICS↗

Study of Implosion of Combined Nested Arrays

New experimental data on the implosion of plasma of nested kapron−tungsten arrays are obtained at the Angara-5-1 facility. The mode of plasma implosion is implemented in which a shock wave region forms in the space between the inner and outer arrays where a transition from the super-Alfvénic (V{sub r} > V{sub A}) to sub-Alfvénic (V{sub r} < V{sub A}) plasma flow takes place. Specific features of the formation and decay of the shock region are studied using laser shadow imaging and X-ray frame photography. The plasma density in the transition region is estimated. By comparing the experimental data with the results of simulations of quasi-steady implosion of a nested array with allowance for extended plasma production, the physical conditions are determined at which the implosion mode with the formation the shock region takes place. Stable compression of the plasma of the inner array was observed during the implosion of combined nested arrays with a fiber outer array and tungsten inner array. Suppression of magnetic Rayleigh-Taylor instability during the compression of the inner array plasma results in the formation of a compact radiating Z-pinch and generation of a soft X-ray pulse with a peak power of 4 TW and duration of about 5 ns.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Controlling Magnetism of F-Adsorbed BN Nanosheets by Applying Isotropic Strain

Magnetic properties of the h-BN monolayer with nonmetal atoms adsorbed are studied by the first-principle methods. Different dopants (C, Cl, F, and O) and adsorption sites are considered. On one hand, magnetic behavior is observed in two-dimensional (2D) BN system with C, Cl, and O atoms and nonmagnetic state is shown in the F-adsorbed system. On the other hand, the F-adsorbed system shows a more stable formed structure among all the systems. Thus, we study the magnetic properties in F-adsorbed 2D-BN system under the applied tensile and compressive strain. Interestingly, as the strain increases, a maximum magnetic moment of 1.12 μ{sub B} is observed, which originates from the p-p hybridization among F, B, and N atoms. Our results suggest some potential applications of the F-adsorbed BN nanosheet.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Tuning magnetic coercivity with external pressure in iron-rhenium based ferrimagnetic double perovskites

We studied the effect of physical pressure on the electronic and magnetic properties of ferrimagnetic double perovskites A 2 FeReO 6 (A = Ca, Ba) using Re L 2,3 edge x-ray absorption spectroscopy and powder diffraction measurements. Volume compression is shown to dramatically increase the magnetic coercivity (H c ) in polycrystalline samples of both compounds with ΔH c /ΔV similar to 150-200 Oe/Å 3 . A nearly eight-fold increase in H c , from 0.2 to 1.55 T, is obtained in Ba 2 FeReO 6 at P = 29 GPa. While no signs of structural phase transitions are seen in either sample to similar to 30 GPa, the structural data points to a pressure-driven increase in tetragonal distortion of ReO 6 octahedra. A sizable but pressure-independent Re orbital-to-spin magnetic moment ratio is observed, pointing to the critical role of spin-orbit interactions at Re sites. We present a J(eff) description of the electronic structure that combines effects of crystal field and spin-orbit coupling on the Re 5d 2 orbitals and use this description to provide insight into the pressure-induced enhancement of magnetic anisotropy.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Effect of MWCNT Content on the Structure and Properties of Spark Plasma-Sintered Iron-MWCNT Composites Synthesized by High-Energy Ball Milling

The effect of multiwall carbon nanotube (MWCNT) content on the physical and mechanical properties of Fe-MWCNT composites has been studied. High-energy ball milling (HEBM) is employed to produce the composite powder; following this, spark plasma sintering (SPS) process has been adopted for powder consolidation. The composite powder and the sintered products were subjected to structural characterization by XRD. Microstructural studies were carried out by optical, field-emission scanning and high-resolution transmission electron microscopy. While Fourier transform infrared spectroscopic study of composites was done to understand the bonding characteristics, Raman spectroscopy was employed to assess the structural damage of MWCNT after HEBM. The effects of processing on the behavior of C-C, C-O and Fe-O bonds are studied by x-ray photoelectron spectroscopy. Microhardness and compressive strength of composites are also determined. Finally, magnetic and electrical properties of the composites were characterized. It was observed that optimized ball milling conditions help to preserve the structural identity of MWCNT. Consolidation by SPS insured good interfacial bonding. The microhardness and compression strength are significantly improved in MWCNT-reinforced iron matrix composite. MWCNT has appreciably improved the electrical conductivity of the composites. Tethering of MWCNT by iron oxide has led to appreciable improvement in saturation magnetization till 3 wt.% MWCNT.

36 MATERIALS SCIENCE↗

Measurements of the Strain Dependence of Critical Current of Commercial REBCO Tapes at 15 T Between 4.2 and 40 K for High Field Magnets

Interest for high magnetic fields (>16 T) for applications in high energy physics (HEP) and fusion machines, requires the development of high current cables capable to withstand the large forces, mechanical and electromagnetic, experienced during manufacturing and operations. The critical current (I c ) of REBCO tapes depends on strain, magnetic fields, and operational temperatures. Understanding how these parameters affect the I c of the conductor will be critical to develop robust high-current REBCO cables. However, there are limited reports on the strain dependence of I c , in particular at high fields and elevated temperatures relevant for future high-field compact fusion reactor magnets. We present here I c of commercial REBCO tapes measured as a function of compressive and tensile strain (between -0.6% and +0.65%) at high magnetic fields (12 and 15 T) and different temperatures (within 4.2-40 K). Results at 4.2 and 20 K showed less than 5% reduction in the normalized I c at high strain, while a stronger strain dependence was observed at 40 K. Samples tested at 12 T and 4.2 K showed similar strain dependence as 15 T and 4.2 K. In all tested conditions, the tape experienced reversible I c reduction in both tension and compression. Finite element analysis was used to predict the residual thermal strain accumulated in the REBCO layer prior of testing to account for the effect of the cooldown. A method was also developed to account for the current sharing observed between the sample and the sample holder during the ramp of the current. Our results provide useful input for the development of high-field fusion and HEP magnets using REBCO conductors.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Modeling the one-dimensional imager of neutrons (ODIN) for neutron response functions at the Sandia Z facility

The one-dimensional imager of neutrons (ODIN) at the Sandia Z facility consists of a 10-cm block of tungsten with rolled edges, creating a slit imager with slit widths of either 250, 500, or 750 μm. Designed with a 1-m neutron imaging line of sight, we achieve about 4:1 magnification and 500-μm axial spatial resolution. The baseline inertial confinement fusion concept at Sandia is magnetized liner inertial fusion, which nominally creates a 1-cm line source of neutrons. ODIN was designed to determine the size, shape, and location of the neutron producing region, furthering the understanding of compression quality along the cylindrical axis of magnetized liner implosions. Challenges include discriminating neutrons from hard x-rays and gammas with adequate signal-to-noise in the 2 × 10 12 deuterium-deuterium (DD) neutron yield range, as well as understanding the point spread function of the imager to various imaging detectors (namely, CR-39). Modeling efforts were conducted with MCNP6.1 to determine neutron response functions for varying configurations in a clean DD neutron environment (without x-rays or gammas). Configuration alterations that will be shown include rolled-edge slit orientation and slit width, affecting the resolution and response function. The experiment to determine CR-39 neutron sensitivity, with and without a high density polyethylene (n, p) converter, an edge spread function, and resolution will be discussed.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Development of a cryogenically cooled platform for the Magnetized Liner Inertial Fusion (MagLIF) Program [Development of a cryogenically-cooled platform for the Magnetized Liner Inertial Fusion (MagLIF) Concept]

A cryogenically cooled hardware platform has been developed and commissioned on the Z Facility at Sandia National Laboratories in support of the Magnetized Liner Inertial Fusion (MagLIF) Program. MagLIF is a magneto-inertial fusion concept that employs a magnetically imploded metallic tube (liner) to compress and inertially confine premagnetized and preheated fusion fuel. The fuel is preheated using a ~2 kJ laser that must pass through a ~1.5-3.5-μm-thick polyimide “window” at the target’s laser entrance hole (LEH). As the terawatt-class laser interacts with the dense window, laser plasma instabilities (LPIs) can develop, which reduce the preheat energy delivered to the fuel, initiate fuel contamination, and degrade target performance. Cryogenically cooled targets increase the parameter space accessible to MagLIF target designs by allowing nearly 10 times thinner windows to be used for any accessible gas density. Thinner LEH windows reduce the deleterious effects of difficult to model LPIs. The Z Facility’s cryogenic infrastructure has been significantly altered to enable compatibility with the premagnetization and fuel preheat stages of MagLIF. The MagLIF cryostat brings the liquid helium coolant directly to the target via an electrically resistive conduit. This design maximizes cooling power while allowing rapid diffusion of the axial magnetic field supplied by external Helmholtz-like coils. A variety of techniques have been developed to mitigate the accumulation of ice from vacuum chamber contaminants on the cooled LEH window, as even a few hundred nanometers of ice would impact laser energy coupling to the fuel region. Here, the MagLIF cryostat has demonstrated compatibility with the premagnetization and preheat stages of MagLIF and the ability to cool targets to liquid deuterium temperatures in approximately 5 min.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

High-resolution hybrid simulations of kinetic plasma turbulence at proton scales

We investigate properties of plasma turbulence from magnetohydrodynamic (MHD) to sub-ion scales by means of two-dimensional, high-resolution hybrid particle-in-cell simulations. We impose an initial ambient magnetic field perpendicular to the simulation box, and we add a spectrum of large-scale magnetic and kinetic fluctuations with energy equipartition and vanishing correlation. Once the turbulence is fully developed, we observe an MHD inertial range, where the spectra of the perpendicular magnetic field and the perpendicular proton bulk velocity fluctuations exhibit power-law scaling with spectral indices of −5/3 and −3/2, respectively. This behavior is extended over a full decade in wavevectors and is very stable in time. A transition is observed around proton scales. At sub-ion scales, both spectra steepen, with the former still following a power law with a spectral index of ∼−3. A −2.8 slope is observed in the density and parallel magnetic fluctuations, highlighting the presence of compressive effects at kinetic scales. The spectrum of the perpendicular electric fluctuations follows that of the proton bulk velocity at MHD scales, and flattens at small scales. All these features, which we carefully tested against variations of many parameters, are in good agreement with solar wind observations. The turbulent cascade leads to on overall proton energization with similar heating rates in the parallel and perpendicular directions. While the parallel proton heating is found to be independent on the resistivity, the number of particles per cell, and the resolution employed, the perpendicular proton temperature strongly depends on these parameters.

79 ASTRONOMY AND ASTROPHYSICS↗

Bursty magnetic reconnection at the Earth's magnetopause triggered by high-speed jets

The impact of high-speed jets—dynamic pressure enhancements in the magnetosheath—on the Earth's magnetopause has been observed to trigger local magnetic reconnection. We perform a three-dimensional hybrid simulation to study the magnetosheath and magnetopause under turbulent conditions using a quasi-radial southward interplanetary magnetic field (IMF). In contrast to quasi-steady reconnection with a strong southward IMF, we show that after the impact of a jet on the magnetopause, the magnetopause moves inward, the current sheet is compressed and intensified and signatures of local magnetic reconnection are observed, showing similarities to spacecraft measurements.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

WEIBEL INSTABILITY DRIVEN BY SPATIALLY ANISOTROPIC DENSITY STRUCTURES

Observations of afterglows of gamma-ray bursts (GRBs) suggest that post-shock magnetic fields are strongly amplified to about 100 times the shock-compressed value. The Weibel instability appears to play an important role in generating the magnetic field. However, recent simulations of collisionless shocks in homogeneous plasmas show that the magnetic field generated by the Weibel instability rapidly decays. There must be some density fluctuations in interstellar and circumstellar media. The density fluctuations are anisotropically compressed in the downstream region of relativistic shocks. In this paper, we study the Weibel instability in electron–positron plasmas with spatially anisotropic density distributions by means of two-dimensional particle-in-cell simulations. We find that large magnetic fields are maintained for a longer time by the Weibel instability driven by spatially anisotropic density structure. Particles anisotropically escape from the high density region, so that a temperature anisotropy is generated and the Weibel instability becomes unstable. Our simulation results suggest that the Weibel instability driven by an anisotropic density structure can generate sufficiently large magnetic fields and they can cover sufficiently large regions to explain the afterglow emission of GRBs.

79 ASTRONOMY AND ASTROPHYSICS↗

CHROMOSPHERIC AND CORONAL WAVE GENERATION IN A MAGNETIC FLUX SHEATH

Using radiation magnetohydrodynamic simulations of the solar atmospheric layers from the upper convection zone to the lower corona, we investigate the self-consistent excitation of slow magneto-acoustic body waves (slow modes) in a magnetic flux concentration. We find that the convective downdrafts in the close surroundings of a two-dimensional flux slab “pump” the plasma inside it in the downward direction. This action produces a downflow inside the flux slab, which encompasses ever higher layers, causing an upwardly propagating rarefaction wave. The slow mode, excited by the adiabatic compression of the downflow near the optical surface, travels along the magnetic field in the upward direction at the tube speed. It develops into a shock wave at chromospheric heights, where it dissipates, lifts the transition region, and produces an offspring in the form of a compressive wave that propagates further into the corona. In the wake of downflows and propagating shock waves, the atmosphere inside the flux slab in the chromosphere and higher tends to oscillate with a period of ν ≈ 4 mHz. We conclude that this process of “magnetic pumping” is a most plausible mechanism for the direct generation of longitudinal chromospheric and coronal compressive waves within magnetic flux concentrations, and it may provide an important heat source in the chromosphere. It may also be responsible for certain types of dynamic fibrils.

79 ASTRONOMY AND ASTROPHYSICS↗

Modulating the Extent of Anisotropic Cuprophilicity via High Pressure with Piezochromic Luminescence Sensitization

We report metallophilicity has been widely studied as a fundamental supramolecular interaction. However, the extent and directionality thereof remain controversial. A major obstacle lies in the difficulty to separately control the geometry and chemical composition. Herein, we address this challenge by modulating metallophilicity with mechanical pressure. Using a multinuclear Cu(I) complex as model system, we report anomalous anisotropies of (supra)molecular structures, vibrations, and interaction energies upon isotropic compression as well as concomitant (essentially turn-on) piezochromic luminescence enhancement with ~10 3 modulation. The in situ characterizations indicate opposite behaviors of contact distances and cuprophilic interactions for intermolecular vs intramolecular Cu-Cu pairs under pressure. Theoretical calculations break down the attractive and repulsive forces associated with cuprophilicity, its spontaneous 4p-3d hybridization origin, and direction-dependent interaction strength. The use of isotropic mechanical force reveals the intrinsic anisotropy of metallophilicity in multinuclear systems.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Electron Heating in Low Mach Number Perpendicular Shocks. II. Dependence on the Pre-shock Conditions

Recent X-ray observations of merger shocks in galaxy clusters have shown that the post-shock plasma is two-temperature, with the protons being hotter than the electrons. Here, the second of a series, we investigate the efficiency of irreversible electron heating in perpendicular low Mach number shocks, by means of two-dimensional particle-in-cell simulations. We consider values of plasma beta (the ratio of thermal and magnetic pressures) in the range 4 ≲ β p0 ≲ 32, and sonic Mach number (the ratio of shock speed to pre-shock sound speed) in the range 2 ≲ M s ≲ 5, as appropriate for galaxy cluster shocks. As reflected in Paper I, magnetic field amplification—induced by shock compression of the pre-shock field, or by strong proton cyclotron and mirror modes accompanying the relaxation of proton temperature anisotropy—can drive the electron temperature anisotropy beyond the threshold of the electron whistler instability. The growth of whistler waves breaks the electron adiabatic invariance, and allows for efficient entropy production. We determine that the post-shock electron temperature T e2 exceeds the adiabatic expectation ${T}_{e2,\mathrm{ad}}$ by an amount $({T}_{e2}-{T}_{e2,\mathrm{ad}})/{T}_{e0}\simeq 0.044\,{M}_{s}({M}_{s}-1)$ (here, T e0 is the pre-shock temperature), which depends only weakly on the plasma beta over the range 4 lesssim β p0 lesssim 32 that we have explored, as well as on the proton-to-electron mass ratio (the coefficient of sime0.044 is measured for our fiducial ${m}_{i}/{m}_{e}=49$, and we estimate that it will decrease to sime0.03 for the realistic mass ratio). Our results have important implications for current and future observations of galaxy cluster shocks in the radio band (synchrotron emission and Sunyaev–Zel'dovich effect) and at X-ray frequencies.

79 ASTRONOMY AND ASTROPHYSICS↗

Magneto-induced tunability of thermo-spin current in deformed zigzag graphene nanoribbons

The aim of this report is to unfold how the thermo-electric spin-polarized current in a transverse-biased zigzag graphene nanoribbon changes in the presence of uniaxial deformations and uniform perpendicular magnetic field. Employing the two-parameter Hubbard model along with the non-equilibrium Green's function formalism, we found that both uniaxial strain and magnetic field can significantly modulate the bandgap, local distribution of edge states, and the critical transverse electric field needed to achieve the half-metallic phase in the ribbon. Our analysis shows a significant enhancement of the maximum attainable spin-polarized current as functions of both source temperature and contacts temperature difference, with increasing the magnetic field or applying any magnitude of compressive strain. Furthermore, it is shown that the magneto-resistance ratio of the device, can be drastically tuned via strain engineering, reaching values as high as 2 × 10{sup 4}% for compressive strains of 5% magnitude.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗