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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 253 records · Page 14

Modeling and design of compact, permanent-magnet transport systems for highly divergent, broad energy spread laser-driven proton beams

Laser-driven (LD) ion acceleration has been explored in a newly constructed short focal length laser beamline at the BELLA petawatt facility (interaction point 2, iP2). For applications utilizing such LD ion beams, a beam transport system is required, which for reasons of compactness be ideally contained within 3 m. While they are generated from a micron-scale source, large divergence and energy spread of LD ion beams present a unique challenge to transporting them compared to beams from conventional accelerators. This study gives an overview of proposed compact transport designs using permanent magnets satisfying different requirements depending on the application for the iP2 laser beamline such as radiation biology, material science, and high-energy density science. These designs are optimized for different parameters such as energy spread and peak proton density according to the application’s need. The various designs consist solely of permanent magnet elements, which can provide high magnetic field gradients on a small footprint. While the field strengths are fixed, we have shown that the beam size is able to be tuned effectively by varying the placement of the magnets. The performance of each design was evaluated based on high-order particle tracking simulations of typical LD proton beams. We also examine the ability of certain configurations to tune and select beam energies, critical for specific applications. A more detailed investigation was carried out for a design to deliver 10 MeV LD accelerated ions for radiation biology applications. With these transport system designs, the iP2 laser beamline is ready to house various application experiments.

43 PARTICLE ACCELERATORS↗

Accelerators for the Future: R&D at the Fermilab FAST Facility

High energy physics in the U.S. has ambitious plans requiring new and improved accelerator technologies, including an upgraded complex at Fermilab for DUNE, next-generation light sources, and the potential of a future collider to be built on U.S. soil. To address these requirements, Fermilab operates the Fermilab Accelerator Science and Technology (FAST) facility, dedicated to accelerator R&D. FAST includes an electron gun and superconducting RF linac (up to 300 MeV), a storage ring, and an upcoming proton source and injector line (up to 2.5 MeV). In addition to the future of Fermilab accelerators, the broad physics program includes general R&D with potential impact across the DOE science program. This colloquium will provide a basic introduction to accelerator technologies and describe the principles of proton and electron accelerators, including the challenges associated with next-generation operations. We will discuss the exciting R&D ongoing at FAST to address the required technological advancements, focusing on Non-Linear Integrable Optics (NIO) for improved beam intensity and Optical Stochastic Cooling (OSC) for improved beam quality, and touching on a wide range of additional ongoing research. I intend to make the content interesting and accessible to those who have never taken any formal courses in accelerator physics.

43 PARTICLE ACCELERATORS↗

Design and Prototyping of the 162.5 MHz PIP-II RF Reference-Line Station

The Proton Improvement Plan II (PIP-II) Reference Line distributes phase-stable radio-frequency signals so accelerating cavities transfer energy to the proton beam at the correct point in each RF cycle. The full system contains 162.5, 325, and 650 MHz sections; this project focuses on the 162.5 MHz station. Commercial filters, amplifiers, splitters, mixers, and hardware were assembled into a compact, serviceable heat-plate layout and tested to verify performance metrics at 162.5 MHz.

Subedi, Harsheet [Unlisted, US]↗

Amine Structure Governs Corrosion Rates of Copper Catalysts in Electrochemical Reactive Capture of CO 2

Reactive capture of CO 2 (RCC) offers an integrated approach that combines CO 2 capture with its direct electrochemical conversion, eliminating the need for CO 2 release from the capture agent. By avoiding the pH, pressure, and temperature swings required for the release step, RCC has the potential to reduce both energy consumption and capital costs compared to the conventional sequential process of CO 2 capture, release, concentration, and conversion. Amines, widely used in industrial CO 2 capture, face challenges in RCC systems due to their incompatibility with transition metal catalysts as well as their tendency to promote electrode corrosion and parasitic hydrogen evolution. Identifying suitable combinations of amines and catalysts is therefore critical to enabling integrated CO 2 capture and conversion. Here, this work systematically investigates the performance of four primary and four secondary amines for RCC on polycrystalline Cu catalysts. Among the eight tested amines, only dimethylamine showed no measurable Cu corrosion near the open circuit potential. In contrast, ammonia, methylamine, ethylamine, monoethanolamine, diethylamine, diethanolamine, and piperazine all induced Cu corrosion. Corrosion rates correlate with the pK a and steric hindrance of the amines, highlighting key parameters for catalyst–amine codesign. Grand canonical DFT calculations indicate a correlation between the adsorption strength of protonated amines, their pK a , and the extent of Cu corrosion, suggesting that both the surface binding of protonated amines and the lability of their protons play critical roles in corrosion acceleration near open circuit potentials. These finding suggest that amines with high pK a values and weak binding of their protonated forms to Cu surfaces are preferred, as they offer better corrosion resistance.

Choi, Jounghwan [Univ. of California, Los Angeles,↗

Real-Time Edge AI for Distributed Systems (READS): Progress on Beam Loss De-Blending for the Fermilab Main Injector and Recycler

The Fermilab Main Injector enclosure houses two accelerators, the Main Injector and Recycler. During normal operation, high intensity proton beams exist simultaneously in both. The two accelerators share the same beam loss monitors (BLM) and monitoring system. Beam losses in the Main Injector enclosure are monitored for tuning the accelerators and machine protection. Losses are currently attributed to a specific machine based on timing. However, this method alone is insufficient and often inaccurate, resulting in more difficult machine tuning and unnecessary machine downtime. Machine experts can often distinguish the correct source of beam loss. This suggests a machine learning (ML) model may be producible to help de-blend losses between machines. Work is underway as part of the Fermilab Real-time Edge AI for Distributed Systems Project (READS) to develop a ML empowered system that collects streamed BLM data and additional machine readings to infer in real-time, which machine generated beam loss.

43 PARTICLE ACCELERATORS↗

Novel design and diagnostics improvements for increased production capacity and improved reliability at the Los Alamos Isotope Production Facility

The Isotope Production Facility (IPF) at Los Alamos National Laboratory (LANL) is used to produce an array of isotopes for medical, global security, and research applications with an intense beam of protons supplied by the linear accelerator at the Los Alamos Neutron Science Center (LANSCE). An Accelerator Improvement Project (AIP) was recently conducted at IPF to improve facility reliability and reduce programmatic risk while increasing general isotope production capacity and flexibility. This was accomplished through the installation of an improved beam window assembly, more robust beam diagnostics, an active and adjustable collimator, and a new beam rastering system. This paper will highlight the four exciting innovations and how they were designed, validated, and installed in parallel as well as the significant operational advantages they provide to IPF. Key experiments and the increased currents achieved in routine production runs demonstrating the enhanced capability from the AIP will be presented. As a result, the most notable capability enhancements include irradiations with beam currents ranging from 100 nA experimental runs up to 300 μA on routine production targets and utilization of a range of cylindrical target diameters.

100 MeV protons↗

Laser-assisted high-energy proton pulse extraction for feasibility study of co-located muon source at the SNS

Here, we have experimentally demonstrated the first non-intrusive 1-GeV proton beam extraction for the generation of muons with a temporal structure optimized for Muon Spin Relaxation/Rotation/Resonance (μSR) applications. The proton pulses are extracted based on the laser neutralization of 1 GeV hydrogen ion (H - ) beam in the high energy beam transport of the Spallation Neutron Source (SNS) accelerator. The maximum flux of the extracted proton beam based on laser neutralization causes only 0.2% reduction of the total proton beam used for neutron production, a marked difference from the 20% reduction at other co-located muon and neutron facilities, and thus the proposed method will result in negligible impact on the SNS operation. This paper describes the development of a fiber/solid-state hybrid laser system that has high flexibility of pulse structure and output power, initial experiments on laser neutralization of beam and separation of H 0 beam from the existing SNS accelerator beam line, conversion of H 0 to proton at the SNS linac dump, and measurement results of 30 ns/50 kHz proton pulses. This system conclusively demonstrates the feasibility of laser-based proton beam extraction to power a world-leading μSR facility at the SNS.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Discerning the effect of various irradiation modes on the corrosion of Zircaloy-4

Using proton irradiation, this study investigates the individual influence of several factors on the corrosion kinetics of Zircaloy-4 in a hydrogenated water environment simulating a Pressurized Water Reactor (PWR). Using both simultaneous irradiation-corrosion and autoclave corrosion, we separately examine: (i) the effect of pre-irradiation on modifying the structure of the material, (ii) the impact of irradiation on creating defects in the growing oxide layer during corrosion, and (iii) the influence of irradiation on increasing the corrosion potential through radiolysis during corrosion. To replicate neutron-irradiated microstructure, two proton pre-irradiation schedules were employed: Schedule 1 (isothermal irradiation at 350 °C to 5 dpa) to simulate high-temperature PWR conditions, and Schedule 2 (two-step process: irradiation to 2.5 dpa at -10 °C followed by 2.5 dpa at 350 °C) to simulate lower temperature PWR and Boiling Water Reactor (BWR) conditions. Long-term autoclave corrosion testing over 360 days at 320 °C revealed no significant difference between unirradiated samples and those pre-irradiated according to either schedule, with all samples exhibiting sub-cubic kinetics within the pre-transition regime. Irradiated samples underwent Simultaneous Irradiation Corrosion (SIC) tests, corroding in 320 °C water while being irradiated with protons. Corrosion was found to accelerate in all SIC-tested samples relative to autoclave conditions, with the greatest increase observed in non-pre-irradiated samples. Pre-irradiation with either schedule resulted in a slower corrosion rate compared to non-pre-irradiated regions under SIC conditions. The degree of radiolysis observed in the SIC tests surpassed typical PWR conditions, approaching levels found in BWRs. Radiolysis products were identified as the primary contributors to accelerated corrosion, corroborated by radiolysis bar tests. Furthermore, these findings underscore the intricate interactions between irradiation, corrosion, and water chemistry in determining Zircaloy-4 corrosion kinetics within nuclear reactor environments.

Pressurized Water Reactor↗

Development and Commercialization of a Nanosegrated Oxygen Evolution Reaction Electrocatalyst (CRADA)

This collaborative project leverages advanced characterization tools, catalyst treatment and electrochemical testing capabilities at LBNL to help commercialize a bimetallic nanosegrated catalysts for oxygen evolution reaction in proton-exchange membrane water electrolyzers. This project also has three industrial partners who are involved in catalyst scale-up synthesis, large electrode fabrication and large electrode electrochemical testing. This project investigates a broad range of topics including electrocatalysis, ink rheology and electrode fabrication and testing. This knowledge could help bridge the performance and durability gap from laboratory-developed materials (such as electrocatalysts) to applications in commercial devices. The research results also bring fundamental understanding of possible degradation mechanisms that occur under extremely oxidative potentials including material and morphological changes. The project will help accelerate the deployment of proton-exchange membrane water electrolyzers. The public benefits could include creating jobs and increasing public awareness of potential clean technologies for green hydrogen production. Ultimately, the project will help national wide effort of flighting climate change and achieving carbon neutrality by 2050.

30 DIRECT ENERGY CONVERSION↗

Disentangling Beam Losses in The Fermilab Main Injector Enclosure Using Real-Time Edge AI

The Fermilab Main Injector enclosure houses two accelerators, the Main Injector and Recycler Ring. During normal operation, high intensity proton beams exist simultaneously in both. The two accelerators share the same beam loss monitors (BLM) and monitoring system. Deciphering the origin of any of the 260 BLM readings is often difficult. The (Accelerator) Real-time Edge AI for Distributed Systems project, or READS, has developed an AI/ML model, and implemented it on fast FPGA hardware, that disentangles mixed beam losses and attributes probabilities to each BLM as to which machine(s) the loss originated from in real-time. The model inferences are then streamed to the Fermilab accelerator controls network (ACNET) where they are available for operators and experts alike to aid in tuning the machines.

43 PARTICLE ACCELERATORS↗

IOTA Proton Injector Beamline Installation

The IOTA Proton Injector (IPI), currently under installation at the Fermilab Accelerator Science and Technology facility, is a beamline capable of delivering 20-mA pulses of protons at 2.5 MeV to the Integrable Optics Test Accelerator (IOTA) ring. First beam in the IPI beamline is anticipated in 2023, when it will operate alongside the existing electron injector beamline to facilitate further fundamental physics research and continued development of novel accelerator technologies in the IOTA ring. This report details the expected operational profile, known challenges, and the current state of installation.

43 PARTICLE ACCELERATORS↗

Residual Dose and Environmental Monitoring for the Fermilab Main Injector Tunnel Using the Data Acquisition Logging Engine (Dale)

The Recycler and the Main Injector are part of the Fermilab Accelerator complex used to deliver proton beam to the different experiments. It is very important to control and minimize losses in both machines during operation, to reduce personnel dose from residual activation and to preserve component lifetime. To minimize losses, we need to identify the loss points and adjust the components accordingly. The Data Acquisition Loss Engine (DALE) platform has been developed within the Main Injector department and upgraded throughout the years. DALE is used to survey the entire enclosure for residual dose rates and environmental readings when unrestricted access to the enclosure is possible. Currently DALE has two radiation meters, which are aligned along each machine, so loss points can be identified for both at the same time. DALE attaches to the enclosure carts and is continuously in motion monitoring dose rates and other environmental readings. In this paper we will describe how DALE is used to provide radiation maps of the residual dose rates in the enclosure. We will also compare the loss points with the Beam Loss monitor data.

43 PARTICLE ACCELERATORS↗

Investigating high-energy proton-induced reactions on spherical nuclei: Implications for the preequilibrium exciton model

A number of accelerator-based isotope production facilities utilize $100-200$ MeV proton beams due to the high production rates enabled by high-intensity beam capabilities and the greater diversity of isotope production brought on by the long range of high-energy protons. However, nuclear reaction modeling at these energies can be challenging because of the interplay between different reaction modes and a lack of existing guiding cross section data. A Tri-lab collaboration has been formed between the Lawrence Berkeley, Los Alamos, and Brookhaven National Laboratories to address these complexities by characterizing charged-particle nuclear reactions relevant to the production of established and novel radioisotopes. In the inaugural collaboration experiments, stacked-targets of niobium foils were irradiated at the Brookhaven Linac Isotope Producer ($E_p=200$ MeV) and the Los Alamos Isotope Production Facility ($E_p=100$ MeV) to measure $^{93}$Nb(p,x) cross sections between $50-200$ MeV. The results were compared with literature data as well as the default calculations of the nuclear model codes TALYS, CoH, EMPIRE, and ALICE. The default code predictions largely failed to reproduce the measurements. Therefore, we developed a standardized procedure, which determines the reaction model parameters that best reproduce the most prominent reaction channels in a physically justifiable manner. Overall, the primary focus of the procedure was to determine the best parameterization for the pre-equilibrium two-component exciton model. This modeling study revealed a trend towards a relative decrease for internal transition rates at intermediate proton energies ($E_p=20-60$ MeV) in the current exciton model as compared to the default values. The results of this work are instrumental for the planning, execution, and analysis essential to isotope production.

43 PARTICLE ACCELERATORS↗

Status of the IOTA proton injector

The IOTA Proton Injector (IPI), currently under installation at the Fermilab Accelerator Science and Technology facility (FAST), is a machine capable of delivering 20\,mA pulses of protons at 2.5\,MeV to the Integrable Optics Test Accelerator (IOTA) ring. First beam in the IPI beamline is anticipated in the first half of~2024, when it will operate alongside the existing electron injector beamline to facilitate further beam physics research and continued development of novel accelerator technologies at the IOTA ring. This report details the expected operational profile, known challenges, and the current state of installation.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Status of the IOTA Proton Injector

The IOTA Proton Injector (IPI), currently under installation at the Fermilab Accelerator Science and Technology facility (FAST), is a machine capable of delivering 20 mA pulses of protons at 2.5 MeV to the Integrable Optics Test Accelerator (IOTA) ring. First beam in the IPI beamline is anticipated in the first half of 2024, when it will operate alongside the existing electron injector beamline to facilitate further beam physics research and continued development of novel accelerator technologies at the IOTA ring. This report details the expected operational profile, known challenges, and the current state of installation.

43 PARTICLE ACCELERATORS↗

Operation of the trigger system for the ICARUS detector at Fermilab

The ICARUS liquid argon TPC detector is taking data on the Booster (BNB) and Main Injector (NuMI) Neutrino beam lines at Fermilab with a trigger system based on the scintillation light produced by charged particles in coincidence with the proton beam extraction from the accelerators. The architecture and the deployment of the trigger system in the first two runs for physics are presented, as well as the triggered event rates. The event recognition efficiency has been evaluated as a function of the deposited energy and the position of cosmic muons stopping inside the detector.

Neutrino detectors↗