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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 253 records · Page 14
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Probing individual single atom electrocatalyst sites by advanced analytical scanning transmission electron microscopy

Single atom electrocatalysts (SAEs) are promising next-generation materials for promoting a variety of important reactions, such as the oxygen reduction, nitrogen reduction, and CO 2 reduction reactions. While bulk characterization techniques such as X-ray absorption spectroscopy and Mössbauer spectroscopy have significantly enhanced our understanding of these catalysts, direct probing of individual single metal atom sites at the atomic scale is necessary to understand local variations in the properties of these sites and accelerate design and synthesis of improved SAEs. Aberration-corrected scanning transmission electron microscopy (STEM) has become a powerful tool for providing this type of atomic-scale information about SAE metal sites. These sites are typically unstable under the electron beam, however, which, in combination with conventional acquisition methods and detectors, has limited the type and quantity of information obtainable by spectroscopic STEM techniques. Here, we map multiple individual SAE metal sites in a nitrogen-doped carbon containing atomically dispersed Fe and Re (FeReNC) at the atomic scale by direct electron detection electron energy-loss spectroscopy (EELS). Direct electron detection provides an improved signal-to-noise ratio over conventional scintillator-based detectors and enables detection and real space localization of weak signals. In addition, we demonstrate an automated method for identification of metal atom positions, placement of the probe on these sites, and simultaneous EELS and energy dispersive X-ray spectroscopic (EDS) signal acquisition. This simultaneous acquisition of EELS and EDS provides access to the composition and bonding of a wide range of SAE metal sites. In this study, focusing the probe directly on the metal sites also increases the relevant data acquisition rate by more than an order of magnitude over two-dimensional mapping, enabling improved statistical measurements of site properties. The versatility, sensitivity, and speed that these techniques provide enhances our ability to probe the local elemental and chemical environment of a large number of individual SAE metal site structures at the atomic scale, enabling an improved understanding of the variations in the local properties of these electrocatalysts to be gained. As a result, significantly increased information about individual metal sites will be available to future electrochemical studies through these techniques, accelerating the development of advanced SAEs.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Characterization of stilbene-d 12 for neutron spectroscopy without time of flight

In this work, we have experimentally characterized the light-output response of a deuterated trans-stilbene (stilbene-d 12 ) crystal to quasi-monoenergetic neutrons in the 0.8 to 4.4 MeV energy range. These data allowed us to perform neutron spectroscopy measurements of a DT 14.1 MeV source and a 239 PuBe source by unfolding the impinging neutron spectrum from the measured light-output response. The stilbene-d 12 outperforms a 1 H-stilbene of similar size when comparing the shape of the unfolded spectra and the reference ones. These results confirm the viability of non-hygroscopic stilbene-d 12 crystal for direct neutron spectroscopy without need for time-of-flight measurements. This capability makes stilbene-d 12 a well suited detector for fast-neutron spectroscopy in many applications including nuclear reaction studies, radiation protection, nuclear non-proliferation, and space travel.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Time calibration and synchronization of the scintillation light detection system in ICARUS-T600

The ICARUS-T600 Liquid Argon (LAr) Time Projection Chamber (TPC) is presently taking data in the Short Baseline Neutrino (SBN) program at Fermilab (U.S.A.) to search for a possible LSND-like sterile neutrino signal at Δm 2 ≈ 1 eV 2 with the Booster Neutrino Beam (BNB). A light detection system, based on 360 large area Photo-Multiplier Tubes (PMTs), has been realized for ICARUS-T600 to detect VUV photons produced by the passage of ionizing particles in LAr. This system is fundamental for the TPC operation, providing an efficient trigger and contributing to the 3D reconstruction of events. Moreover, since the detector is exposed to a huge flux of cosmic rays due to its shallow depths installation, the light detection system allows for the time reconstruction of events, contributing to the identification and to the selection of genuine neutrino interactions. The correct time reconstruction of events requires the precise knowledge of the delay of each PMT channel and a good synchronization of recording electronics, this last based on fast sampling digitizers. To achieve a time resolution better than 1 ns, we perform three consecutive timing corrections deployed at different stages of the optical data flow. Results demonstrate the capability of the ICARUS-T600 light detection system to allow a precise reconstruction of the temporal evolution of each event occurring in the detector and the association of neutrino events with the bunched structure of BNB.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2021

Simultaneous measurement of organic scintillator response to carbon and proton recoils

Organic scintillators are widely used for neutron detection in both basic nuclear physics and applications. While the proton light yield of organic scintillators has been extensively studied, measurements of the light yield from neutron interactions with carbon nuclei are scarce. Demonstrate a new approach for the simultaneous measurement of the proton and carbon light yield of organic scintillators. Provide new carbon light yield data for the EJ-309 liquid and EJ-204 plastic organic scintillators. A 33-MeV 2 H + beam from the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory was impinged upon a 3-mm-thick Be target to produce a high-flux, broad-spectrum neutron beam. The double time-of-flight technique was extended to simultaneously measure the proton and carbon light yields of the organic scintillators, wherein the light output associated with the recoil particle was determined using np and nC elastic scattering kinematics. The proton and carbon light yield relations of the EJ-309 liquid and EJ-204 plastic organic scintillators were measured over a recoil energy range of approximately 0.3 to 1 MeV and 2 to 5 MeV, respectively, for EJ-309, and 0.2 to 0.5 MeV and 1 to 4 MeV, respectively, for EJ-204. Furthermore, these data provide new insight into the ionization quenching effect in organic scintillators and key input for simulation of the response of organic scintillators for both basic science and a broad range of applications.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Novel Sensors for Particle Tracking: a Contribution to the Snowmass Community Planning Exercise of 2021

Five contemporary technologies are discussed in the context of their potential roles in particle tracking for future high energy physics applications. These include sensors of the 3D configuration, in both diamond and silicon, submicron-dimension pixels, thin film detectors, and scintillating quantum dots in gallium arsenide. Drivers of the technologies include radiation hardness, excellent position, vertex, and timing resolution, simplified integration, and optimized power, cost, and material.

Detectors↗
DOE OSTI2020

Mixed-Material Scintillators (MMSS Quarterly Report FY20Q2)

This project aims to invent, model, and prototype mixed-material scintillator systems (MMSSs), a new class of radiation detectors that use heterogenous internal structures of different scintillating materials to detect additional properties of radiation. These internal structures can be produced using additive manufacture (3D printing) of scintillator, a currently emerging application of additive manufacture technology. MMSSs combine the low cost and complexity of conventional scintillation detectors with capabilities currently only available in more expensive and complex detectors. By identifying promising MMSS designs, this project will enable a new class of detectors to meet DNN’s mission needs for SNM detection. This quarter, we delivered one the MMSS Particle-ID Modeling report, a major deliverable of this project. This report describes our results on simulations of the particle-ID (PID) class of detectors. We found that these detectors outperform competing approaches for neutron-gamma discrimination, neutron source pointing, and neutron spectroscopy. Further highlights of the report are described below. During this quarter, We alerted HQ to a change in schedule for the remaining simulations planned for this project: we plan to put off further simulation and reporting of the position-resolving (PR) detector class until July. This change in schedule has allowed us to go into additional detail in the PID work that is both very promising and motivates our upcoming proposal. The other active task in this project is prototyping 3D-printed scintillators with the aim of realizing the designs we’ve simulated. On that front, we had three focuses: measuring the light output, increasing the size of printed parts, and combining blue and green scintillators. We succeeded in measuring the light output, showing an output of 30% of commercial standard. This result leaves room for improvement but is within striking distance of where we need to be. We were on track to demonstrate a key requirement for increasing the size of parts and also to show combined green/blue prints before the laboratory moved to a Minimum Safe (MinSafe) Operations posture as a result of local Shelter In Place orders due to Covid-19.

42 ENGINEERING↗
DOE OSTI2023

Determination of energy-dependent neutron backgrounds using shadow bars

Understanding the neutron background is essential for determining the neutron yield from nuclear reactions. Here, the neutron backgrounds were determined for heavy-ion collision experiment using the shadow-bar method, where beams of 40,48 Ca at 56, 140 MeV/u impinged on targets of 58,64 Ni and 112,124 Sn. In the analysis presented here, brass shadow bars are placed in front of organic liquid scintillator neutron detectors to determine the energy-dependent neutron background fractions. The measurement of neutron spectra with and without shadow bars is important to determine the neutron background more accurately. The neutron background, along with its sources and systematic uncertainties, are explored with a focus on the impact of background models and their dependence on neutron energy.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

Drones for Decommissioning

The U.S. Nuclear Regulatory Commission has responsibility for regulating the safe decommissioning of facilities and sites to meet the License Termination Rule in 10 Code of Federal Regulations (CFR) Part 20, Standards for Protection Against Radiation, Subpart E “Radiological Criteria for License Termination.” Decommissioning is performed in accordance with 10 CFR Part 50, Domestic Licensing of Production and Utilization Facilities, as part of license termination (§50.82) and release of the facility or site for unrestricted use (§50.83). The guidance currently demonstrates the minimum requirements and necessary conditions for conducting radiological surveys by a person carrying a radiation detector(s). The Pacific Northwest National Laboratory (PNNL) evaluated the use of an unoccupied aerial vehicle (UAV) to conduct radiological surveys that could be used in decommissioning to potentially reduce time, cost, and worker safety compared to current survey methods. The objective of this project was to evaluate the performance and limitations of a UAV to support a decommissioning radiological survey and compare it to a radiological survey conducted by a human. The primary research questions of interest evaluated were: 1. Did observed UAV paths differ from human paths and, if so, how much? 2. Did survey path deviation affect survey results and, if so, how? 3. Were radiological measurements from human and UAV surveys significantly different? To answer these research questions, an experimental field was set up at PNNL’s 3440 test track, and it included radiological sources commonly surveyed during decommissioning: cobalt-60 (Co-60), cesium-137 (Cs-137), and americium-241 (Am-241). Nine check sources (three each of Am-241, Cs-137, and Co-60) with activities ranging from 3.54 µCi to 39.34 µCi were set over a path that also included an area for measuring background radiation. An Aurelia X6 UAV coupled with a GPS and lidar unit was used to conduct the radiological surveys. UAV and human surveys were conducted using two different NaI(Tl) scintillation radiation detectors (2 in. × 2 in. Ludlum, Inc. and 2 in. × 0.04 in. Alpha Spectra, Inc.) at a travel velocity of approximately 0.2 m/s at a low (15–40 cm median altitude) or high (87–105 cm median altitude) survey altitude. Since the survey velocity and altitude parameters were atypical for normal UAV operations, testing was done prior to conducting the radiological surveys to establish airworthiness, evaluate the navigation system, and establish flight control. Human and UAV surveys were paired according to the detector type and altitude regime to compare the survey data. The results of this proof-of-concept research determined that the UAV and human surveys followed similar survey paths and detected the radiological sources with no significant statistical difference (in 33 out of 36 surveys). However, further research is needed prior to deploying UAVs for decommissioning surveys.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗
DOE OSTI2022

Erratum: Production and validation of scintillating structural components from low-background Poly(ethylene naphthalate)

Regretfully, the author list of the original paper did not contain the members of the groups being responsible for the HPGe screening, Radon emanation measurement and ICPMS surface characterization works. As the work performed is to be considered more than “just service work”, the authors together with the members of these groups have decided to amend the authors list. At publication the following authors were not included in the author list: • From Pacific Northwest National Laboratory, Richland, WA, U.S.A.: E.W. Hoppe, I.J. Arnquist, K.P. Hobbs, A.D. French, M.L. diVacri • From INFN, Laboratori Nazionali del Gran Sasso, 67100 Assergi, Italy: M. Laubenstein • From M. Smoluchowski Institute of Physics, Jagiellonian University, 30-348 Krakow, Poland: G. Zuzel The metadata of the present erratum are already correct.

99 GENERAL AND MISCELLANEOUS↗
DOE OSTI2021

Fabrication of Low-Cost Large-Volume Ceramic A 2 HfX 6 (A= Cs or Tl, X = Cl, Br, or I) Scintillators for Gamma Ray Detection (SBIR Phase I Final Technical Report)

Scintillator crystals play an important role in the radiation detection field. Widespread use of scintillators as gamma-ray detectors is largely generated by their extensive availability and tunable properties, such high light output, high stopping power (Z eff ), fast decay time, and good proportionality. Additionally, the cost for manufacturing a scintillation detector like NaI:Tl is usually considerably lower than the cost for manufacturing a semiconductor detector like CdZnTe. Because there is no such thing as an ideal scintillation material, an application requiring certain detection characteristics may incorporate a scintillator tailored to its specific properties. The vast variety of applications and requirements necessitates more research into new scintillation materials and/or better methods of producing existing materials.The goal of this project was to grow low cost and environmentally stable inorganic transparent ceramic scintillators with excellent gamma ray resolution, excellent energy proportionality, excellent detection efficiency due to high density (>5 g/cm 3 ) and very high Z eff (55-80), and good light yields (>40,000 ph/MeV). In Phase I Xtallized Intelligence, Inc. (XI, Inc) developed a novel ceramic fabrication technique to produce low cost and environmentally stable highly efficient inorganic transparent ceramic scintillators of various dimensions. XI, Inc., collaborating with Fisk University (Fisk), investigated the scintillation properties of these new ceramic scintillators and compared them to in their single crystal counterparts. The results of this Phase I project show that successful production of high-quality inorganic halide ceramic scintillators Cs 2 HfCl 6 (CHC) and Tl 2 HfCl 6 (THC). Both ceramic CHC and THC scintillators have achieved good performance close to the performance of their single crystal counterparts. Fabricating these inorganic ceramic scintillators mitigate many issues encountered during conventional bulk crystal growth by melt methods. Additional benefits of the ceramic fabrication technique include high production yield, low production cost, fast production time, and no material waste Inorganic transparent ceramic scintillators produced in this project will enhance cost effectiveness at the instrument level based on low projected cost of the proposed compounds, as much smaller crystal sizes would be required to achieve similar efficiency as current radioisotope identification devices (RIID’s) used in homeland security applications as well as spectrometers in high energy physics applications.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Discrimination of electronic recoils from nuclear recoils in two-phase xenon time projection chambers

We present a comprehensive analysis of electronic recoil vs. nuclear recoil discrimination in liquid/gas xenon time projection chambers, using calibration data from the 2013 and 2014-16 runs of the Large Underground Xenon (LUX) experiment. We observe strong charge-to-light discrimination enhancement with increased event energy. For events with S1 = 120 detected photons, i.e. equivalent to a nuclear recoil energy of ~100 keV, we observe an electronic recoil background acceptance of <10 –5 at a nuclear recoil signal acceptance of 50%. We also observe modest electric field dependence of the discrimination power, which peaks at a field of around 300 V/cm over the range of fields explored in this study (50-500 V/cm). In the WIMP search region of S1 = 1-80 phd, the minimum electronic recoil leakage we observe is (7.3 ± 0.6) 10 –4 , which is obtained for a drift field of 240-290 V/cm. Pulse shape discrimination is utilized to improve our results, and we find that, at low energies and low fields, there is an additional reduction in background leakage by a factor of up to 3. We develop an empirical model for recombination fluctuations which, when used alongside the Noble Element Scintillation Technique (NEST) simulation package, correctly reproduces the skewness of the electronic recoil data. We use this updated simulation to study the width of the electronic recoil band, finding that its dominant contribution comes from electron-ion recombination fluctuations, followed in magnitude of contribution by fluctuations in the S1 signal, fluctuations in the S2 signal, and fluctuations in the total number of quanta produced for a given energy deposition.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2026

Neutrino oscillation prospects with a dual-baseline beam from BNL to SNOLAB and SURF

The Electron-Ion Collider (EIC) is a next-generation accelerator primarily designed to study the internal structure of nucleons through high-precision electron-hadron collisions. In this work, we explore the feasibility of employing a 1 MW fraction of the EIC proton beam to generate a high-intensity GeV-scale neutrino beam for long-baseline oscillation studies. We have simulated proton-target interactions and optimize the resulting neutrino fluxes for water-based liquid scintillator (WbLS) detectors located at distinct baselines of 900 km and at 2900 km. Oscillation analyses performed with GLoBES show that extended baselines allow access to multiple oscillation maxima, significantly enhancing sensitivity to leptonic CP violation. The study also examines the interplay between matter effects and the intrinsic CP violating phase in shaping observable asymmetries. We note that simplified systematics and no backgrounds are used in this analysis to establish the baseline physics potential. These results suggest that the EIC proton beam could provide a novel and complementary source for precision neutrino physics, extending the scientific reach of the EIC program.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Improvement in the spatial resolution for imaging with fast neutrons

In this paper, we report on the realization of an improved concept for the detection of fast neutrons using a specific setup of scintillators with the aim to overcome limitations in spatial resolution. While fast neutron imaging (FNI) is a technique to investigate very thick material layers in transmission mode, currently there is a limit in the spatial resolution at ~1 mm, which hinders the performance for the detection of features like cracks, material damage or pores in large objects ($\gg$1 cm 3 ). The improved concept presented here is based on the separation of the converter material from the scintillation layer in a suitable way, which was successfully tested and referenced to the standard devices at the NECTAR facility (FRM-2, MLZ, Garching) under realistic beamline conditions. The results imply a break-through in enabling detection of structures on the order of 0.2 to 0.5 mm (a more precise estimation is not possible due to other resolution determing factors in a realistic setup). Potential additional improvements are discussed.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Spherical time-encoded radiation imaging simulations

Radiation source localization is important for nuclear nonproliferation and can be obtained using time-encoded imaging systems with unsegmented detectors. A scintillation crystal can be used with a moving coded-aperture mask to vary the detected count rate produced from radiation sources in the far field. The modulation of observed counts over time can be used to reconstruct an image with the known coded-aperture mask pattern. Current time-encoded imaging systems incorporate cylindrical coded-aperture masks and have limits to their fully coded imaging field-of-view. This work focuses on expanding the field-of-view to 4π by using a novel spherical coded-aperture mask. A regular icosahedron is used to approximate a spherical mask. This icosahedron consists of 20 equilateral triangles; the faces of which are each subdivided into four equilateral triangle-shaped voxels which are then projected onto a spherical surface, creating an 80-voxel coded-aperture mask. Furthermore, these polygonal voxels can be made from high-Z materials for gamma-ray modulation and/or low-Z materials for neutron modulation. In this work, we present Monte Carlo N-Particle (MCNP) simulations and simple models programmed in Mathematica to explore image reconstruction capabilities of this 80-voxel coded-aperture mask.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

Abundances of Uranium and Thorium Elements in Earth Estimated by Geoneutrino Spectroscopy

Abstract The decay of the primordial isotopes 238 U, 235 U, 232 Th, and 40 K has contributed to the terrestrial heat budget throughout the Earth's history. Hence, the individual abundance of those isotopes are key parameters in reconstructing contemporary Earth models. The geoneutrinos produced by the radioactive decays of uranium and thorium have been observed with the Kamioka Liquid‐Scintillator Antineutrino Detector (KamLAND). Those measurements have been improved with more than 18‐year observation time, and improvement in detector background levels mainly with an 8‐year nearly reactor‐free period, which now permit spectroscopy with geoneutrinos. Our results yield the first constraint on both uranium and thorium heat contributions. The KamLAND result is consistent with geochemical estimations based on elemental abundances of chondritic meteorites and mantle peridotites. The High‐Q model is disfavored at 99.76% C.L. and a fully radiogenic model is excluded at 5.2 σ assuming a homogeneous heat producing element distribution in the mantle.

58 GEOSCIENCES↗
DOE OSTI2025

Search for light sterile neutrinos with two neutrino beams at MicroBooNE

The existence of three distinct neutrino flavours, ν e , ν μ and ν τ , is a central tenet of the Standard Model of particle physics. Quantum-mechanical interference can allow a neutrino of one initial flavour to be detected sometime later as a different flavour, a process called neutrino oscillation. Several anomalous observations inconsistent with this three-flavour picture have motivated the hypothesis that an additional neutrino state exists, which does not interact directly with matter, termed as ‘sterile’ neutrino, ν s . This includes anomalous observations from the Liquid Scintillator Neutrino Detector (LSND)3 experiment and Mini-Booster Neutrino Experiment (MiniBooNE), consistent with ν μ → ν e transitions at a distance inconsistent with the three-neutrino picture. Here we use data obtained from the MicroBooNE liquid-argon time projection chamber in two accelerator neutrino beams to exclude the single light sterile neutrino interpretation of the LSND and MiniBooNE anomalies at the 95% confidence level (CL). Moreover, we rule out a notable portion of the parameter space that could explain the gallium anomaly. This is one of the first measurements to use two accelerator neutrino beams to break a degeneracy between ν e appearance and disappearance, which would otherwise weaken the sensitivity to the sterile neutrino hypothesis. We find no evidence for either ν μ → ν e flavour transitions or ν e disappearance that would indicate non-standard flavour oscillations. Our results indicate that previous anomalous observations consistent with ν μ → ν e transitions cannot be explained by introducing a single sterile neutrino state.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Plasma pressure profiles in a sheared-flow-stabilized Z-pinch

We report the plasma pressure reached inside the central plasma column of a sheared-flow-stabilized Z-pinch using Thomson scattering measurements. Building on previously reported experimental results and the analysis methods established for the high temperature and moderate density plasmas generated on the FuZE device, we show evidence of a central plasma region with higher electron temperature and density, which is consistent with a pinch behavior. Elevated electron temperatures up to 2.25 ± 0.8 keV and densities up to (4.9±0.2)×1017 cm−3 are observed to temporally coincide with the fusion neutron production from the plasma. Reconstructed plasma pressure profiles highlight the presence of a several millimeter-wide column with elevated pressure whose location varies shot-to-shot. The plasma pressure rises as neutron production from the deuterium plasma increases, reaching a peak value of 2.6 kBar. This peak value is consistent with a radially force-balanced pinch equilibrium model based on the measured ∼320 kA pinch current. Complete datasets were obtained at two axial locations, 10 and 20 cm axial position from the tip of the central electrode, which corroborate the estimated neutron source axial lengths.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗