Solid-State High Harmonic Generation in Common Large Bandgap Substrate Materials
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Molecular systems capable of directing the flow of excitons are key to the development and optimization of optoelectronic materials. The transport of excitons across multiple molecules is governed by an intermolecular electronic coupling network. In this article, we consider the effects of complex-valued intermolecular electronic coupling on exciton transport. Here, we present a molecular motif capable of generating complex-valued coupling under excitation with circularly polarized light. We use theoretical modeling and simulation to illustrate how complex coupling can be leveraged to drive the rotational flux of excitons in cyclic molecular networks and direct the exciton population in branched molecular networks.
Here, a modification to the di-homodyne transient grating spectroscopy optical arrangement is presented that removes the need to individually align two spatially separated probe laser beams. This work details the novel application of a single probe beam that utilizes birefringent materials to produce two optically homodyned signals with a relative phase shift of π radians. This arrangement effectively simplifies the alignment to one probe beam and removes the relative phase shift ambiguity between each homodyned signal. Several example measurements for tungsten, titanium, molybdenum, and silicon are shown to illustrate the utility of the new optical system.
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Here, we demonstrate that the suppression in the lensing power spectrum of the cosmic microwave background (CMB) caused by massive neutrinos can be mimicked by dark matter-baryon interactions at the precision of next-generation CMB experiments. Thus, a determination of neutrino masses from the CMB lensing power spectrum may be compromised. We illustrate the degeneracy for a dark matter-proton cross section ∝ $v$ –4 , which arises in the t-channel exchange of an ultralight mediator in the nonrelativistic limit.
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