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At least 253 records · Page 14

CACTI: Fast Liquid Water Content

These data were collected during the Cloud, Aerosol, and Complex Terrain Interactions (CACTI; https://www.arm.gov/research/campaigns/amf2018cacti ) field campaign in the Sierras de Córdoba mountain range of north-central Argentina as part of the ARM Aerial Facility (AAF) deployment. The ARM Aerial Facility Gulfstream-1 was operated from Las Higueras Airport (IATA: RCU, ICAO: SAOC), Río Cuarto, Córdoba, Argentina, for the Intensive Observation Period (IOP) from Nov. 1 through Dec. 15, 2018. The G-1 aircraft performed 22 research flights over the first ARM Mobile Facility (AMF1) location in the Sierras de Córdoba mountain range to measure atmospheric state and turbulence, cloud water content and droplet size distributions, aerosol precursor gases, and aerosol chemical composition and size distributions. The current data set presents re-processed Particle Volume Monitor PVM-100A (aka Gerber probe) data: Liquid Water Content (LWC), Particle Surface Area (PSA), and the effective droplet radius (re) averaged to 50Hz, 10Hz, and 1Hz.

54 ENVIRONMENTAL SCIENCES↗

Gas release and conductivity modification studies

The behavior of gas clouds produced by releases from orbital velocity in either a point release or venting mode is described by the modification of snowplow equations valid in an intermediate altitude regime. Quantitative estimates are produced for the time dependence of the radius of the cloud, the average internal energy, the translational velocity, and the distance traveled. The dependence of these quantities on the assumed density profile, the internal energy of the gas, and the ratio of specific heats is examined. The new feature is the inclusion of the effect of the large orbital velocity. The resulting gas cloud models are used to calculate the characteristics of the field line integrated Pedersen conductivity enhancements that would be produced by the release of barium thermite at orbital velocity in either the point release or venting modes as a function of release altitude and chemical payload weight.

Linson, L. M.↗

Composition of interstellar clouds in the disk and halo. 2: Gamma(sup 2) Velorum

High-resolution observations of gamma(sup 2) Vel with the Goddard High-Resolution Spectrograph (GHRS) echelle on the Hubble Space Telescope reveal the presence of seven narrow absorption components, with LSR velocities between -23 and +9 km s(exp -1). Three of these show column density ratios N(S(++))/N(S(+)) and N(P(++))/N(P+)) of about 1 or more, and can be identified as H II regions, while the other four are H I regions, consistent with the O I profile and with the overall H(sup 0) column density of 5.9 x 10(exp 19) cm(exp -2), given the usual assumptions that S is undepleted while O has a depletion D(O) = -0.3 dex. The depletions of Fe, Si, and Mn, which could be measure accurately for two of the four H I regions (components 6 and 7), differ somewhat from the values of D(sub ws) found for slowly moving warm clouds in HD 93521; in particular, for the component at 4.0 km s(exp -1) (No. 6), abosolute of D exceeds absolute of D(sub ws) by 0.1-0.4 dex, while for that at 9.3 km s(exp -1) (No. 7), absolute of D equals absolute of D(sub ws) on the average. The observed ratio of Fe + Mg atoms to Si atoms in the grains of component 6 is 2.04 +/-0.10, consistent with an olivine grain composition; the Fe/Mg ratio is 1.5 +/- 0.2. The electron density in component 6, determined from the C II(sup *) feature, is 0.075 +/- 0.013 cm (exp -3), about two-thirds of that found for clouds of this velocity in HD 93521. In the two conspicuous H II regions, components 3 and 4, n(sub e), determined from the Si II(sup *) feature, is about 1 cm(exp -3). From the column density of S(+) + S(++) in these two components, the total H II path length is about 40 pc. With the radius of a wind-blown bubble around gamma(sup 2) Vel set equal to 60 pc, the effective Stromgren radius is about 100 pc, requiring that T approx. equal to 50,000 K for the Wolf-Rayet component of the gamma(sup 2) Vel binary. Since zeta Pup is a comparable source of ionizing radiation, this temperature is an upper limit. The profiles of the strongest H2 absorption features, from Copernicus archives, indicate that the absorbing molecules have a mean velocity identical with that of the strongest H II component (No. 4). We have no explanation for the possible presence of these H2 molecules in a region of ionized H. Alternatively, the H2 profiles can be explained by molecules in the two adjacent (in velocity) H I regions, components 2 and 5, provided their H I gas has densities and temperatures typical of normal cold clouds. The GHRS data show absorption by highly ionized atoms Si(3+) and C(3+), N(4+) in broad features, in addition to the narrow-line absorption by Si(3+) and C(3+) observed in the dominant H II components, Nos. 3 and 4. The broad C(3+) and N(4+) features have widths corresponding to T in the range (4-8) x 10(exp 5) K, consistent with the broad O(5+) line shown in Copernicus data. Despite some observational uncertainties, the ratios of column densities in the broad C(3+), N(4+), and O(5+) features agree to +/- 0.1 dex with theoretical values for warm gas, heating and evaporating by thermal conduction from an adjacent hot region. Outward evaporation from an isolated cloud in a hot ambient gas cannot be distinguished, on the basis of these data, from inward evaporation of a warm shell, compressed by an expanding, hot stellar-wind bubble. For several halo stars, the C IV/O VI ratio has a quite different average value, perhaps consistent with cooling of infalling hot gas instead of conductive heating and evaporation.

Fitzpatrick, Edward L.↗

Non-planar MHD model for solar flare-generated disturbances in the heliospheric equatorial plane

An analysis, with a representative (canonical) example of solar-flare-generated equatorial disturbances, is made for the temporal and spatial changes in the solar wind plasma and magnetic field environment between the sun and 1 AU. The goal is to search for first-order global consequences rather than to make a parametric study. The analysis treats all three plasma velocity and magnetic field components in any convenient heliospheric plane of symmetry. The representative disturbance is examined for the canonical case in which the temporal and spatial changes in a homogeneous solar wind caused by a solar-flare-generated shock wave are described. All plasma and field parameters at three radial locations are examined. These are the central meridian and 33 deg W and 90 deg W of the flare's central meridian. It is found that the incorporation of a small meridional magnetic field in the ambient magnetic spiral field has negligible effect on the results. The magnetic field exhibits strong kinking within the interplanetary shocked flow, even reversed polarity that, coupled with low temperature and low density, suggests a plausible explanation for magnetic clouds' with accompanying double-streaming of electrons observed at directions approximately 90 deg to the heliocentric radius.

Wu, S. T.↗

Remote Sensing of Aerosol and their Radiative Properties from the MODIS Instrument on EOS-Terra Satellite: First Results and Evaluation

The MODIS instrument was launched on the NASA Terra satellite in Dec. 1999. Since last Oct., the sensor and the aerosol algorithm reached maturity and provide global daily retrievals of aerosol optical thickness and properties. MODIS has 36 spectral channels in the visible to IR with resolution down to 250 m. This allows accurate cloud screening and multi-spectral aerosol retrievals. We derive the aerosol optical thickness over the ocean and most of the land areas, distinguishing between fine (mainly man-made aerosol) and coarse aerosol particles. The information is more precise over the ocean where we derive also the effective radius and scattering asymmetry parameter of the aerosol. New methods to derive the aerosol single scattering albedo are also being developed. These measurements are use to track different aerosol sources, transport and the radiative forcing at the top and bottom of the atmosphere. The AErosol RObotic NETwork of ground based radiometers is used for global validation of the satellite derived optical thickness, size parameters and single scattering albedo and measure additional aerosol parameters that cannot be derived from space.

Kaufman, Yoram↗

Vertical structure of biomass burning aerosol transported over the southeast Atlantic Ocean

Biomass burning in southwestern Africa produces smoke plumes that are transported over the Atlantic Ocean and overlie vast regions of stratocumulus clouds. This aerosol layer contributes to direct and indirect radiative forcing of the atmosphere in this region particularly during the months of August, September, and October. There was a multi-year international campaign to study this aerosol and its interactions with clouds. Here, we report on the evolution of aerosol distributions and properties as measured by the airborne high spectral resolution lidar (HSRL-2) during the ORACLES (Observations of Aerosols above Clouds and their intEractionS) campaign in September 2016. The NASA Langley HSRL-2 instrument was flown on the NASA ER-2 aircraft for several days in September 2016. Data were aggregated at two pairs of 2° × 2° grid boxes to examine the evolution of the vertical profile of aerosol properties during transport over the ocean. Results showed that the structure of the profile of aerosol extinction and microphysical properties is maintained over a 1 to 2 d timescale. In the 3–5 km altitude range, 95 % of the aerosol extinction was contributed by particles in the 0.05–0.50 µm radius size range with the aerosol in this size range having an average effective radius of 0.16 µm. This indicates that there is essentially no scavenging or dry deposition at these altitudes. Moreover, there is very little day-to-day variation in these properties, such that time sampling as happens in such campaigns may be representative of longer periods such as monthly means. Below 3 km, there is considerable mixing with larger aerosol, most likely continental source near land. Furthermore, these measurements indicated that there was often a distinct gap between the bottom of the aerosol layer and cloud tops at the selected locations as evidenced by a layer of several hundred meters that contained relatively low aerosol extinction values above the clouds.

lidar↗

Contact ice nucleation by submicron atmospheric aerosols

An apparatus designed to measure the concentrations of submicron contact ice nuclei is described. Here, natural forces transfer nuclei to supercooled sample drops suspended in an aerosol stream. Experimental measurements of the scavenging rate of the sample drops for several humidities and aerosol sizes are found to be in agreement with theory to within a factor of two. This fact, together with the statistical tests showing a difference between the data and control samples, is seen as indicating that a reliable measurement of the concentrations of submicron contact ice nuclei has been effected. A figure is included showing the ice nucleus concentrations as a function of temperature and assumed aerosol radius. For a 0.01 micron radius, the average is 1/liter at -15 C and 3/liter at -18 C. It is noted that the measurements are in fair agreement with ice crystal concentrations in stable winter clouds measured over Elk Mountain, WY (Vali et al., 1982).

Deshler, T.↗

Entrainment and detrainment in a simple cumulus cloud model

A cumulus cloud model, analogous to the mixed-layer models of the planetary boundary layer and the upper ocean, is developed using a single, unitary entrainment process in which the motion of the cloud boundary relative to the mean flow is permitted, produced, and controlled by turbulent processes. An alternate theory to the mixing-length theory of Asai and Kasahara (1967) is proposed which completely removes the strong scale-dependence of the Asai-Kasahara model. The model reintroduces scale-dependence by introducing including the pe5turbation pressure term of the equation of vertical motion. It is shown that the model predicts deeper clouds than the Asai-Kasahara model for a given sounding, due to the entrainment assumption and the effects of the perturbation pressure. Lateral entrainment dominates cloud-top entrainment, although finite-difference errors increase the cloud-top entrainment rate from zero to a positive value in actual situations. The fractional entrainment rate for updrafts is determined to vary only slightly with height and to decrease only slowly as the cloud radius increases, while the fractional detrainment rate for updrafts increases with height.

Randall, D. A.↗

Determination of stack plume properties from satellite imagery

LANDSAT imagery data were analyzed to determine the quantitative properties of a stack plume emitted from a moderate-sized pulp mill. Overlapping, consecutive-day MSS data provided plume/no plume radiances upwelling from the area of interest. These values from both the plume and its shadow were used to evaluate plume radius, height, particle concentration and scattering function, and total particle loading. Imagery data from a 10 by 10 km region in the vicinity of the mill were normalized to correct for minor atmospheric, solar and viewing angle changes for the two observation days, and cloud shadow data were used to evaluate sky radiance. The effects of the Sun angle, surface reflectance, SNR and spatial resolution are treated in the paper.

Staylor, W. F.↗

Numberical simulation of the effects of radially injected barium plasma in the ionosphere

The morphology of the ion cloud in the radial shaped charge barium injection was studied. The shape of the ion cloud that remains after the explosive products and neutral barium clears away was examined. The ion cloud which has the configuration of a rimless wagon wheel is shown. The major features are the 2.5 km radius black hole in the center of the cloud, the surrounding ring of barium ion and the spokes of barium ionization radiating away from the center. The cloud shows no evolution after it emerges from the neutral debris and it is concluded that it is formed within 5 seconds of the event. A numerical model is used to calculate the motion of ions and electrons subject to the electrostatic and lorenz forces.

Swift, D. W.↗

AGN Black Hole Masses from Reverberation Mapping

Emission-line variability data on bright AGNs indicates that the central objects in these sources have masses in the million to few-hundred million solar mass range. The time-delayed response of the emission lines to continuum variations can be used to infer the size of the line-emitting region via light travel-time arguments. By combining these sizes with the Doppler widths of the variable part of the emission lines, a virial mass estimate can be obtained. For three especially well-studied sources, NGC 5548, NGC 7469, and 3C 390.3, data on multiple emission lines can be used to test the virial hypothesis. In each of these cases, the response time of the various emission lines is anticorrelated with the line width, with the dependence as expected for gravitationally bound motion of the line-emitting clouds, i.e., that the square of the Doppler line width is inversely proportional to the emission-line time delay. Virial masses based on the Balmer lines have now been measured for about three dozen AGNs. Systematic effects currently limit the accuracy of these masses to a factor of several, but characteristics of the radius-luminosity and mass-luminosity relationships for AGNs are beginning to emerge.

Peterson, B. M.↗

TPSAS-NF1676L-29931-DND

The ACE science working group satellite concept calls for a combination of high spectral resolution aerosol lidar and a polarimeter able to determine vertical profiles of aerosol extinction and clouds. Here we discuss why an HSRL lidar is required to achieve these requirements. The primary advantage of an HSRL over an elastic backscatter lidar is that the HSRL channel allows for the independent retrieval of vertically resolved aerosol extinction without constraint. Not requiring a constraint means greater availability of retrievals in polar regions, on the night side, and in broken cloud situations, plus greater accuracy particularly in the lowest part of the atmosphere and in scenes with aerosol heterogeneity. Advantages go beyond the extinction products. Unlike attenuated backscatter, which is an integrated quantity, the aerosol backscatter coefficient depends only on the aerosol at a specific level in the atmosphere, making it preferable for use in quantitative applications. The aerosol backscatter coefficient is more accurate from an HSRL system compared to the retrieval from a single-channel system. This is because errors in both extinction and backscatter from a single-channel system increase with decreasing altitude, due to the need to accurately characterize the overlying attenuation. This means that an HSRL will also have more valid data in and near the boundary layer where aerosol is of primary interest for air quality and weather applications and for many climate objectives including aerosol-cloud interaction studies. Even cloud properties that do not directly use the HSRL capability (cloud phase and thin cirrus retrievals) benefit from the more accurate calibration of an HSRL system. The improved accuracy of backscatter and extinction also lead to better capabilities for aerosol typing, improved retrievals of aerosol radiative effect, and increased information content for combined lidar + polarimeter retrievals of profiles of microphysical properties such as vertically resolved effective radius.

S P Burton↗

A Simple Model of Global Aerosol Indirect Effects

Most estimates of the global mean indirect effect of anthropogenic aerosol on the Earth's energy balance are from simulations by global models of the aerosol lifecycle coupled with global models of clouds and the hydrologic cycle. Extremely simple models have been developed for integrated assessment models, but lack the flexibility to distinguish between primary and secondary sources of aerosol. Here a simple but more physically based model expresses the aerosol indirect effect (AIE) using analytic representations of cloud and aerosol distributions and processes. Although the simple model is able to produce estimates of AIEs that are comparable to those from some global aerosol models using the same global mean aerosol properties, the estimates by the simple model are sensitive to preindustrial cloud condensation nuclei concentration, preindustrial accumulation mode radius, width of the accumulation mode, size of primary particles, cloud thickness, primary and secondary anthropogenic emissions, the fraction of the secondary anthropogenic emissions that accumulates on the coarse mode, the fraction of the secondary mass that forms new particles, and the sensitivity of liquid water path to droplet number concentration. Estimates of present-day AIEs as low as 5 W/sq m and as high as 0.3 W/sq m are obtained for plausible sets of parameter values. Estimates are surprisingly linear in emissions. The estimates depend on parameter values in ways that are consistent with results from detailed global aerosol-climate simulation models, which adds to understanding of the dependence on AIE uncertainty on uncertainty in parameter values.

Clouds↗

Measurements and Simulations of Nadir-Viewing Radar Returns from the Melting Layer at X- and W-Bands

Simulated radar signatures within the melting layer in stratiform rain, namely the radar bright band, are checked by means of comparisons with simultaneous measurements of the bright band made by the EDOP (X-band) and CRS (W-band) airborne Doppler radars during the CRYSTAL-FACE campaign in 2002. A stratified-sphere model, allowing the fractional water content to vary along the radius of the particle, is used to compute the scattering properties of individual melting snowflakes. Using the effective dielectric constants computed by the conjugate gradient-fast Fourier transform (CGFFT) numerical method for X and W bands, and expressing the fractional water content of melting particle as an exponential function in particle radius, it is found that at X band the simulated radar bright-band profiles are in an excellent agreement with the measured profiles. It is also found that the simulated W-band profiles usually resemble the shapes of the measured bright-band profiles even though persistent offsets between them are present. These offsets, however, can be explained by the attenuation caused by cloud water and water vapor at W band. This is confirmed by the comparisons of the radar profiles made in the rain regions where the un-attenuated W-band reflectivity profiles can be estimated through the X- and W band Doppler velocity measurements. The bright-band model described in this paper has the potential to be used effectively for both radar and radiometer algorithms relevant to the TRMM and GPM satellite missions.

Liao, Liang↗

The absence of circumstellar dust debris around G giants

The IRAS data base has been searched for evidence for circumstellar dust around luminosity class III G giants, stars whose progenitors are mostly main-sequence A stars. While 20 percent of all main-sequence A dwarfs have dust which absorbs at least 5 x 10 to the -6th of the light from the star, less than 3 percent of all G giants have such clouds. One possible explanation for the absence of detectable dust debris around the G giants is that the Poynting-Robertson effect leads to the decay of the dust around the main-sequence A stars, and that the supply of these grains is not renewed indefinitely. In this case, the derived upper limit to the grain radius of about 0.2 cm for the bulk of the grains emitting the far-infrared emission is consistent with data derived from ground-based submillimeter observations. Another possible explanation for the lack of grains around at least some G giants is that the dust around the original A dwarf is mainly composed of relatively volatile material like water ice which thermally evaporates in a relatively short time during the giant phase of higher luminosity.

Jura, M.↗

X-ray photoelectron spectroscopy of surfactants on sub-micron aqueous aerosols

Organic molecules at the aqueous interfaces of droplets and aerosols can influence multiphase chemistry and cloud condensation nuclei activity. While surface tension measurements on flat surfaces are commonly used to quantify organic partitioning and structure, extending these measurements to more realistic aerosols that might exist in metastable, supercooled and supersaturated states remains a challenge. Here, we use aerosol velocity map imaging X-ray photoelectron spectroscopy (A-VMI-XPS), a surface-sensitive and in situ technique, to study the partitioning and structure of a model surfactant (n-octyl β-D-thioglucopyranoside, OTG) in submicron aqueous aerosols with a mean radius of 116 nm. After accounting for finite size effects and evaporative cooling, we find the bulk concentrations of OTG in the aerosol are depleted 600-fold relative to macroscopic solutions. At the low temperatures of the experiment (ca. ∼188 K), we obtain a Langmuir equilibrium constant of 700 m3 mol-1, which corresponds to 4.9 m3 mol-1 at room temperature; a value that is consistent with prior literature reports. Analysis of photoelectron angular distributions, peak areas, and secondary electron escape barriers indicates a transition from a disordered surfactant layer at low [OTG] to a more structured layer at high [OTG]. These results link macroscopic surface tension measurements to nanoparticle surfactant behavior and demonstrate the utility of A-VMI-XPS in probing surfactant coating structure on free aerosols, with implications for understanding the impact of organic coatings on cloud formation and atmospheric chemistry.

Deal, Alexandra M↗

Formation of a rotational accretion column

We consider the problem of the flow produced by the accretion of gas from a rotating cloud onto a point gravitational source. It is shown that, for a cloud initially in uniform rotation, the effect of accretion is to produce a Taylor column in the cloud parallel to the rotation axis. Only gas within the column is accreted; the gas outside the column undergoes oscillatory flow, which is probably subject to shear instability. The column forms in approximately one-half rotation period from the time at which accretion begins. Its initial radius is determined by the accretion rate and the angular velocity of the cloud. Application of the results to the formation of Jupiter by accretion is discussed.

Cassen, P.↗

The diffusion approximation. An application to radiative transfer in clouds

It is shown how the radiative transfer equation reduces to the diffusion equation. To keep the mathematics as simple as possible, the approximation is applied to a cylindrical cloud of radius R and height h. The diffusion equation separates in cylindrical coordinates and, in a sample calculation, the solution is evaluated for a range of cloud radii with cloud heights of 0.5 km and 1.0 km. The simplicity of the method and the speed with which solutions are obtained give it potential as a tool with which to study the effects of finite-sized clouds on the albedo of the earth-atmosphere system.

Arduini, R. F.↗