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At least 253 records · Page 14

Arctic Ozone Depletion from UARS MLS Measurements

Microwave Limb Sounder (MLS) measurements of ozone during four Arctic winters are compared. The evolution of ozone in the lower stratosphere is related to temperature, chlorine monoxide (also measured by MLS), and the evolution of the polar vortex. Lagrangian transport calculations using winds from the United Kingdom Meteorological Office's Stratosphere-Troposphere Data Assimilation system are used to estimate to what extent the evolution of lower stratospheric ozone is controlled by dynamics. Observations, along with calculations of the expected dynamical behavior, show evidence for chemical ozone depletion throughout most of the Arctic lower stratospheric vortex during the 1992-93 middle and late winter, and during all of the 1994-95 winter that was observed by MLS. Both of these winters were unusually cold and had unusually cold and had unusually strong Arctic polar vortices compared to meteorological data over the past 17 years.

UARS MLS↗

Abstract of Lectures

Three lectures will be given. The first one will draw from the general literature on microwave sounding from space. The next two will focus on a description of the Microwave Limb Sounder (MLS) and results obtained from its measurements relating to atmospheric chemistry and dynamics; this will draw from material recently published (or soon-to-be published) by the MLS team.

Froidevaux, Lucien↗

Mid-latitude Ozone and CIO Trends Based on Two Years of UARS MLS Data

Variations in ozone and chlorine monoxide observed by the Microwave Limb Sounder (MLS) abroad the Upper Atmosphere Research Satellite (UARS) during the first two years of operation are presented. We focus on mid-latitudes, where significant ozone decreases are observed in the lower stratosphere, and we offer some comparisons with other data sets. We will attempt to place the mid-latitude changes in context with changes observed at other latitudes. Possible correlations between the MLS ozone and CIO observations will be discussed.

Froidevaux, L.↗

Extratropical Influence of Upper Tropospheric Water Vapor on Greenhouse Warming

The purpose of this paper is to re-examine the impact of upper tropospheric water vapor on greenhouse warming in midlatitudes by analyzing the recent observations of the upper tropospheric water vapor from the Microwave Limb Sounder (MLS) on the Upper Atmosphere Research Satellite (UARS), in conjuction with other space-based measurement and model simulation products.

upper troposphere water vapor greenhouse warming↗

Evolution of MLS Ozone and the Polar Vortex During Winter

The evolution of polar ozone observed by the Upper Atmosphere Research Satellite Microwave Limb Sounder is described for the northern hemisphere (NH) winters of 1991/1992, 1992/1993, and 1993/1994, and the southern hemisphere (SH) winters of 1992 and 1993. Ozone in the mid-stratospheric vortex increases over the winter, with largest increases associated with stratospheric warmings, and a much larger increase in the NH than in the SH.

ozone↗

Discoveries from EOS Aura

Aura, the third and final of three large observatories that are part of NASA s Earth Observing System, was launched July 15,2004. Aura carries four instruments - the Microwave Limb Sounder (MLS), the Tropospheric Emission Spectrometer (TES), the Ozone Monitoring Instrument (OMI) and the High Resolution Dynamics Limb Sounder (HIRDLS), all of which measure atmospheric constituents. Aura measurements provide information to address broad questions about the Earth atmosphere, particularly concerning the recovery of the stratospheric ozone layer, tropospheric air quality, and climate change. TES has made the simultaneous measurements of carbon monoxide and ozone in the lower and upper troposphere. OM1 continues to observe the total ozone column and measures columns of important pollutants like NO2 at unprecedented horizontal resolution and coverage. MLS measures profiles of stratospheric ozone and constituents that affect ozone from the mesosphere into the upper troposphere. This talk will highlight results from Aura s first years in orbit, and will emphasize the way information from Aura and other satellites has contributed to the development, evaluation, and application of global chemistry climate models.

Douglass, Anne↗

The Evolution of the Stratopause During the 2006 Major Warming: Satellite Data and Assimilated Meteorological Analyses

Microwave Limb Sounder and Sounding of the Atmosphere with Broadband Emission Radiometry data show the polar stratopause, usually higher than and separated from that at midlatitudes, dropping from <55-60 to near 30 km, and cooling dramatically in January 2006 during a major stratospheric sudden warming (SSW). After a nearly isothermal period, a cool stratopause reforms near 75 km in early February, then drops to <55 km and warms. The stratopause is separated in longitude as well as latitude, with lowest temperatures in the transition regions between higher and lower stratopauses. Operational assimilated meteorological analyses, which are not constrained by data at stratopause altitude, do not capture a secondary temperature maximum that overlies the stratopause or the very high stratopause that reforms after the SSW; they underestimate the stratopause altitude variation during the SSW. High-quality daily satellite temperature measurements are invaluable in improving our understanding of stratopause evolution and its representation in models and assimilation systems.

Manney, Gloria L.↗

Temporal Decrease in Upper Atmospheric Chlorine

We report a steady decrease in the upper stratospheric and lower mesospheric abundances of hydrogen chloride (HCl) from August 2004 through January 2006, as measured by the Microwave Limb Sounder (MLS) aboard the Aura satellite. For 60(deg)S to 60(deg)N zonal means, the average yearly change in the 0.7 to 0.1 hPa (approx.50 to 65 km) region is -27 +/- 3 pptv/year, or -0.78 +/- 0.08 percent/year. This is consistent with surface abundance decrease rates (about 6 to 7 years earlier) in chlorine source gases. The MLS data confirm that international agreements to reduce global emissions of ozone-depleting industrial gases are leading to global decreases in the total gaseous chlorine burden. Tracking stratospheric HCl variations on a seasonal basis is now possible with MLS data. Inferred stratospheric total chlorine (CITOT) has a value of 3.60 ppbv at the beginning of 2006, with a (2-sigma) accuracy estimate of 7%; the stratospheric chlorine loading has decreased by about 43 pptv in the 18-month period studied here. We discuss the MLS HCl measurements in the context of other satellite-based HCl data, as well as expectations from surface chlorine data. A mean age of air of approx. 5.5 years and an age spectrum width of 2 years or less provide a fairly good fit to the ensemble of measurements.

chlorine↗

Solar Occultation Satellite Data and Derived Meteorological Products: Sampling Issues and Comparisons with Aura MLS

Derived Meteorological Products (DMPs, including potential temperature (theta), potential vorticity, equivalent latitude (EqL), horizontal winds and tropopause locations) have been produced for the locations and times of measurements by several solar occultation (SO) instruments and the Aura Microwave Limb Sounder (MLS). DMPs are calculated from several meteorological analyses for the Atmospheric Chemistry Experiment-Fourier Transform Spectrometer, Stratospheric Aerosol and Gas Experiment II and III, Halogen Occultation Experiment, and Polar Ozone and Aerosol Measurement II and III SO instruments and MLS. Time-series comparisons of MLS version 1.5 and SO data using DMPs show good qualitative agreement in time evolution of O3, N2O, H20, CO, HNO3, HCl and temperature; quantitative agreement is good in most cases. EqL-coordinate comparisons of MLS version 2.2 and SO data show good quantitative agreement throughout the stratosphere for most of these species, with significant biases for a few species in localized regions. Comparisons in EqL coordinates of MLS and SO data, and of SO data with geographically coincident MLS data provide insight into where and how sampling effects are important in interpretation of the sparse SO data, thus assisting in fully utilizing the SO data in scientific studies and comparisons with other sparse datasets. The DMPs are valuable for scientific studies and to facilitate validation of non-coincident measurements.

Manney, Gloria↗

Climatology and Impact of Convection on the Tropical Tropopause Layer

Water vapor plays an important role in controlling the radiative balance and the chemical composition of the Tropical Tropopause Layer (TTL). Mechanisms ranging from slow transport and dehydration under thermodynamic equilibrium conditions to fast transport in convection have been proposed as regulators of the amount of water vapor in this layer. However,.details of these mechanisms and their relative importance remain poorly understood, The recently completed Tropical Composition, Cloud, and Climate Coupling (TC4) campaign had the opportunity to sample the.TTL over the Eastern Tropical Pacific using ground-based, airborne, and spaceborne instruments. The main goal of this study is to provide the climatological context for this campaign of deep and overshooting convective activity using various satellite observations collected during the summertime. We use the Microwave Humidity Sensor (MRS) aboard the NOAA-18 satellite to investigate the horizontal extent.and the frequency of convection reaching and penetrating into the TTL. We use the Moderate Resolution I1l1aging Spectroradiometer (MODIS) aboard the Aqua satellite to investigate the frequency distribution of daytime cirrus clouds. We use the Tropical Rainfall Measuring Mission(TRMM) and CloudSat to investigate the vertical structure and distribution of hydrometeors in the convective cells, In addition to cloud measurements; we investigate the impact that convection has on the concentration of radiatively important gases such as water vapor and ozone in the TTL by examining satellite measurement obtained from the Microwave Limb Sounder(MLS) aboard the Aura satellite.

Robertson, Franklin↗

Convective Formation of Pileus Cloud Near the Tropopause

Pileus clouds form where humid, stably stratified air is mechanically displaced vertically ahead of rising convection. This paper describes convective formation of pileus cloud in the tropopause transition layer (TTL), and explores a possible link to the formation of long-lasting cirrus at cold temperatures. In-situ measurements from off the coast of Honduras during the July 2002 CRYSTALFACE experiment show an example of TTL cirrus associated with, and penetrated by, deep convection. The cirrus was enriched with total water compared to its surroundings, but composed of extremely small ice crystals with effective radii between 2 and 4 m. Through gravity wave analysis, and intercomparison of measured and simulated cloud microphysics, it is argued that the TTL cirrus in this case originated neither from convectively-forced gravity wave motions nor environmental mixing alone. Rather, it is hypothesized that some combination was involved in which, first, convection forced pileus cloud to form from TTL air; second, it punctured the pileus layer, contributing larger ice crystals through interfacial mixing; third, the addition of condensate inhibited evaporation of the original pileus ice crystals in the warm phase of the ensuing gravity wave; fourth, through successive pulses, deep convection formed the observed layer of TTL cirrus. While the general incidence and longevity of pileus cloud remains unknown, in-situ measurements, and satellite-based Microwave Limb Sounder retrievals, suggest that much of the tropical TTL is sufficiently humid to be susceptible to its formation. Where these clouds form and persist, there is potential for an irreversible repartition from water vapor to ice at cold temperatures.

Garrett, Timothy J.↗

The Evolution of the Stratopause during the 2006 Major Warming: Satellite Data and Assimilated Meteorological Analyses

Microwave Limb Sounder and Sounding of the Atmosphere with Broadband Emission Radiometry data provide the first opportunity to characterize the four-dimensional stratopause evolution throughout the life-cycle of a major stratospheric sudden warming (SSW). The polar stratopause, usually higher than that at midlatitudes, dropped by 30 km and warmed during development of a major "wave 1" SSW in January 2006, with accompanying mesospheric cooling. When the polar vortex broke down, the stratopause cooled and became ill-defined, with a nearly isothermal stratosphere. After the polar vortex started to recover in the upper stratosphere/lower mesosphere (USLM), a cool stratopause reformed above 75 km, then dropped and warmed; both the mesosphere above and the stratosphere below cooled at this time. The polar stratopause remained separated from that at midlatitudes across the core of the polar night jet. In the early stages of the SSW, the strongly tilted (westward with increasing altitude) polar vortex extended into the mesosphere, and enclosed a secondary temperature maximum extending westward and slightly equatorward from the highest altitude part of the polar stratopause over the cool stratopause near the vortex edge. The temperature evolution in the USLM resulted in strongly enhanced radiative cooling in the mesosphere during the recovery from the SSW, but significantly reduced radiative cooling in the upper stratosphere. Assimilated meteorological analyses from the European Centre for Medium-Range weather Forecasts (ECMWF) and Goddard Earth Observing System Version 5.0.1 (GEOS-5), which are not constrained by data at polar stratopause altitudes and have model tops near 80 km, could not capture the secondary temperature maximum or the high stratopause after the SSW; they also misrepresent polar temperature structure during and after the stratopause breakdown, leading to large biases in their radiative heating rates. ECMWF analyses represent the stratospheric temperature structure more accurately, suggesting a better representation of vertical motion; GEOS-5 analyses more faithfully describe stratopause level wind and wave amplitudes. The high-quality satellite temperature data used here provide the first daily, global, multiannual data sets suitable for assessing and, eventually, improving representation of the USLM in models and assimilation systems.

Manney, Gloria L.↗

Assimilation of Aura Ozone Data and Comparisons with In Situ Observations

Ozone data from the Ozone Monitoring Instrument (OMI) and the Microwave Limb Sounder (MLS) onboard EOS Aura satellite were assimilated into the Goddard Earth Observing System Version 4 (GEOS-4) ozone assimilation system. Comparison of assimilated ozone with ozone sonde and MOZAIC data indicate an agreement within 10% in the lower stratosphere, where dynamical processes dominate. Assimilation of OMI and MLS data improves tropospheric column estimates in the Atlantic region, but leads to an overestimation in the tropical Pacific in comparison with SHADOZ sondes. Transport and data biases are considered in order to understand these discrepancies. Comparisons of assimilated tropospheric ozone columns with ozone sonde data reveal root-mean-square (RMS) differences of 2.9 to 7.2 DU, which are typically smaller than the model-sonde RMS differences. Four different definitions of the tropopause using temperature lapse rate, potential vorticity (PV) and isentropic surfaces or ozone isosurfaces are compared with respect to their global impact on the estimated tropospheric ozone column. The largest sensitivity in the tropospheric ozone column is found near the subtropical jet, where the ozone or PV determined tropopause typically lies below the lapse rate tropopause.

Stajner, Ivanka↗