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At least 253 records · Page 14

Identification of lunar rock types and search for polar ice by gamma ray spectroscopy

This paper examines the possibility of mapping the surface composition of the moon from an orbiting spin-stabilized spacecraft, using gamma ray spectroscopy and a cooled germanium solid-state device as a detector. A design for accommodating the germanium detector gamma ray spectrometer was devised, and the detection sensitivity was applied to typical lunar-rock compositions. For sets comprising nine highland and 16 mare types, the most useful elements were found to be Mg, Al, K, Ti, Fe, U, and Th. An analysis of the expected instrument response to the gamma ray and neutron fluxes of water ice indicated that a neutron mode added to the spectrometer will be more sensitive than the gamma ray mode to the possible presence of polar ice. It was calculated that, with a pair of selected neutron absorbers and a model which provides that 2.5 percent of the area above 75-deg latitude is occupied by trapping sites, the instrument will provide a 1-yr mission detection limit of 0.056 percent H2O by weight for each polar region.

Metzger, Albert E.↗

Spectator Proton Detection and Reconstruction in Deep Inelastic D(E,EPS) Scattering

A Radial Time Projection Chamber (RTPC) was designed and installed in Jefferson Lab's Hall B as part of the BONuS12 (Barely Off-shell Nucleon Structure) experiment. The goal of BONuS12 is to accurately measure the structure function of the neutron by scattering 11 GeV electrons and detecting them with the CLAS12 spectrometer. Deuterium gas was used as an effective neutron target, and the new RTPC was used to detect low momentum spectator protons. Protons follow a curved path in the 5 Tesla solenoid that is part of CLAS12, ionizing the He-CO2 gas in an annular drift region surrounding the target. These ionization electrons are radially drifted outwards, amplified using cylindrical GEM (Gaseous Electron Multiplication) foils and recorded using readout pads located along the entire outer face of the cylindrical detector. The particle track reconstruction software discussed in detail in this thesis uses the signals from these pads to build tracks, which are reconstructed into the drift region using the arrival times of the signals and the positions of the pads. The proton momentum is measured from the track?s curvature and thus used to extract information about the struck neutron. This thesis introduces the theory of spectator tagging as an effective strategy for measuring neutron structure, by minimizing nuclear effects in the absence of a free neutron target. Along with discussing the many detectors that make up the CLAS12 spectrometer, the RTPC will be covered in detail, along with the tracking software designed to interpret the electronic signals to rebuild the low-momentum particle tracks, and fit them to extract the relevant kinematics. The results of the software, and preliminary analysis will be shown in the final chapter, as well as the discussion of possible improvements which could be made to the tracking software.

Payette, David↗

Measuring Surface Bulk Elemental Composition on Venus

The extreme surface environment (462 C, 93 bars pressure) of Venus makes subsurface measurements of its bulk elemental composition extremely challenging. Instruments landed on the surface of Venus must be enclosed in a pressure vessel. The high surface temperatures also require a thermal control system to keep the instrumentation temperatures within their operational range for as long as possible. Since Venus surface probes can currently operate for only a few hours, it is crucial that the lander instrumentation be able to make statistically significant measurements in a short time. An instrument is described that can achieve such a measurement over a volume of thousands of cubic centimeters of material by using high energy penetrating neutron and gamma radiation. The instrument consists of a Pulsed Neutron Generator (PNG) and a Gamma-Ray Spectrometer (GRS). The PNG emits isotropic pulses of 14.1 MeV neutrons that penetrate the pressure vessel walls, the dense atmosphere and the surface rock. The neutrons induce nuclear reactions in the rock to produce gamma rays with energies specific to the element and nuclear process involved. Thus the energies of the detected gamma rays identify the elements present and their intensities provide the abundance of each element. The GRS spectra are analyzed to determine the Venus elemental composition from the spectral signature of individual major, minor, and trace radioactive elements. As a test of such an instrument, a Schlumberger Litho Scanner oil well logging tool was used in a series of experiments at NASA's Goddard Space Flight Center. The Litho Scanner tool was mounted above large (1.8 m x 1.8 m x.9 m) granite and basalt monuments and made a series of one-hour elemental composition measurements in a planar geometry more similar to a planetary lander measurement. Initial analysis of the results shows good agreement with target elemental assays

Venus↗

Decay studies of the 𝛽-delayed neutron emitters 87 Br and 88 Br measured by means of the Modular Total Absorption Spectrometer at ORNL HRIBF

The β decays of 87 Br, 88 Br, and 87 Kr were measured with the Modular Total Absorption Spectrometer (MTAS) at Oak Ridge National Laboratory’s Holifield Radioactive Ion Beam Facility (HRIBF). Both bromine isotopes are β-delayed neutron emitters that have large cumulative fission yields and were identified as top-priority cases for total absorption study by the Nuclear Energy Agency in 2007. Our investigations corroborate that the decay schemes of 87 Br and 88 Br suffer from the so-called pandemonium effect. Unique MTAS properties enable direct neutron measurements. Here, we present MTAS-derived β-delayed neutron spectra, β-delayed neutron emission probabilities of P n ( 87 Br) = 2.36(24)%, and P n ( 88 Br) = 6.4(6)%, and the β-delayed neutron transitions intensity of 4(2)% to the first excited 87 Kr state, populated in the β-neutron decay of 88Br. Incorporating new data into calculations of the electromagnetic decay heat component emitted during thermal neutron fission of 235 U and 239 Pu improves agreement with experimental data up to approximately 80 s after fission. The estimation of the nuclear reactor $\bar{ν}_e$ flux results in changes of up to 1% in the expected $\bar{ν}_e$ interactions with the detector material for 235 U, 238 U, 239Pu, and 241 Pu.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Second gadolinium loading to Super-Kamiokande

The first loading of gadolinium (Gd) into Super-Kamiokande in 2020 was successful, and the neutron capture efficiency on Gd reached 50%. To further increase the Gd neutron capture efficiency to 75%, 26.1 tons of Gd 2 (SO 4 ) 3 ∙ 8H 2 O was additionally loaded into Super-Kamiokande (SK) from May 31 to July 4, 2022. As the amount of loaded Gd 2 (SO 4 ) 3 ∙ 8H 2 O was doubled compared to the first loading, the capacity of the powder dissolving system was doubled. We also developed new batches of gadolinium sulfate with even further reduced radioactive impurities. In addition, a more efficient screening method was devised and implemented to evaluate these new batches of Gd 2 (SO 4 ) 3 ∙ 8H 2 O. Following the second loading, the Gd concentration in SK was measured to be 333.5 ± 2.5 ppm via an Atomic Absorption Spectrometer (AAS). From the mean neutron capture time constant of neutrons from an Am/Be calibration source, the Gd concentration was independently measured to be 332.7 ± 6.8(sys.) ± 1.1(stat.) ppm, consistent with the AAS result. Furthermore, during the loading the Gd concentration was monitored continually using the capture time constant of each spallation neutron produced by cosmic-ray muons, and the final neutron capture efficiency was shown to become 1.5 times higher than that of the first loaded phase, as expected.

Gadolinium↗

A direct observation of solar neutrons following the 0118 UT flare on 1980 June 21

The Gamma Ray Spectrometer on the Solar Maximum Mission satellite has observed energetic solar neutrons (greater than 50 MeV) at the earth following a solar flare that occurred on the west limb on June 21, 1980 at 01:18:20 UT. Impulsive photon emission from 10 keV to greater than 65 MeV lasting over a period of about 66 s was followed by a transient flux of 50-600 MeV neutrons incident over a 17 minute period. The peak counting rate corresponds to an average flux at the earth of (3.8 + or - 0.6) x 10 to the -2nd neutrons/sq cm s at 130 MeV. These observations indicate the emission of 3 x 10 to the 28th neutrons/sr with energies greater than 50 MeV, requiring the rapid acceleration (much less than 60 s) of protons to GeV energies during the impulsive phase of the flare.

Chupp, E. L.↗

The ultrafast pixel array camera system and its applications in high energy density physics

Diagnostics in high energy density physics, shock physics, and related fields are primarily driven by a need to record rapidly time-evolving signals in single-shot events. These measurements are often limited by channel count and signal degradation issues on cable links between the detector and digitizer. Here we present the Ultrafast Pixel Array Camera (UPAC), a compact and flexible detector readout system with 32 waveform-recording channels at up to 10 Gsample/s and 1.8 GHz analog bandwidth. The compact footprint allows the UPAC to be directly embedded in the detector environment. A key enabling technology is the PSEC4A chip, an eight-channel switch-capacitor array sampling device with up to 1056 samples/channel. The UPAC system includes a high-density input connector that can plug directly into an application-specific detector board, programmable control, and serial readout, with less than 5 W of power consumption in full operation. We present the UPAC design and characterization, including a measured timing resolution of ~20 ps or better on acquisitions of sub-nanosecond pulses with minimal system calibrations. Example applications of the UPAC are also shown to demonstrate operation of a solid-state streak camera, an ultrafast imaging array, and a neutron time-of-flight spectrometer.

47 OTHER INSTRUMENTATION↗

Using real-time nuclear activation detectors for measuring neutron yields from D(D, T)n reactions on the national ignition facility (NIF)

The National Ignition Facility (NIF) has 48 Real-Time Nuclear Activation Detectors distributed around the target chamber capable of measuring deuterium-triton reaction neutron yields with high precision. Here, in this work, we extend this functionality to deuterium–deuterium (DD) reaction neutrons using a nuclear reaction that occurs in the detector’s scintillator material. The corresponding decay of the activated material has a very short half-life of 5 s, which necessitates rapid data collection immediately following an experiment. In this regime, dead time can be very high (>50%) adding significant uncertainty to the measurement. To combat this, we have developed a dead time model that can self-consistently describe the measured data. Initial results show reasonable agreement (within 20%) with DD neutron yields from neutron time-of-flight spectrometers.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Searching for the origin of the rare-earth peak with precision mass measurements across Ce–Eu isotopic chains

A nuclear mass survey of rare-earth isotopes has been conducted with the Canadian Penning Trap mass spectrometer using the most neutron-rich nuclei thus far extracted from the CARIBU facility. Here, we present a collection of 12 nuclear masses determined with a precision of ≤ 10 keV/c 2 for Z = 58-63 nuclei near N = 100. Independently, a detailed study exploring the role of nuclear masses in the formation of the r-process rare-earth abundance peak has been performed. Employing a Markov chain Monte Carlo (MCMC) technique, mass predictions of lanthanide isotopes have been made which uniquely reproduce the observed solar abundances near A = 164 under three distinct astrophysical outflow conditions. We demonstrate that the mass surface trends thus far mapped out by our measurements are most consistent with MCMC mass predictions given an r process that forms the rare-earth peak during an extended (n, γ) ⇌ (γ, n) equilibrium.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Investigation of Proton Beam-Driven Fusion Reactions Generated by an Ultra-Short Petawatt-Scale Laser Pulse

We present results from a pitcher-catcher experiment utilizing a proton beam generated with nanostructured targets at a petawatt-class, short-pulse laser facility to induce proton-boron fusion reactions in a secondary target. A 45-fs laser pulse with either 400 nm wavelength and 7 J energy, or 800 nm and 14 J, and an intensity of up to 5 × 10 21 W/cm 2 was used to irradiate either thin foil targets or near-solid density, nanostructured targets made of boron nitride (BN) nanotubes. In particular, for 800 nm wavelength irradiation, a BN nanotube target created a proton beam with about five times higher maximum energy and about ten times more protons than a foil target. This proton beam was used to irradiate a thick plate made of boron nitride placed in close proximity to trigger 11 B (p, α) 2α fusion reactions. A suite of diagnostics consisting of Thomson parabola ion spectrometers, postshot nuclear activation measurements, neutron time-of-flight detectors, and differentially filtered solid-state nuclear track detectors were used to measure both the primary proton spectrum and the fusion products. From the primary proton spectrum, we calculated (p, n) and (α,n) reactions in the catcher and compare with our measurements. The nuclear activation results agree quantitatively and neutron signals agree qualitatively with the calculations, giving confidence that primary particle distributions can be obtained from such measurements. These results provide new insights for measuring the ion distributions inside of proton-boron fusion targets.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Spin-phonon coupling in AFM transition-metal mono-oxide

Time-of-flight INS measurements were performed on single crystal NiO with the Wide Angular Range Chopper Spectrometer (ARCS) at the Spallation Neutron Source. Experiments were performed on NiO single crystal mounted in an aluminum can and cooled using a closed-cycle helium refrigerator. Measurements were conducted at T = 100 K and 650 K, with the [HHL] scattering plane aligned horizontally. A Fermi chopper with slit spacing of 1.52mm, spinning at 300 Hz, was used to select an incident neutron energy of 100 meV. All datasets were normalized to a vanadium standard to correct for detector efficiency and solid angle coverage. The data sets include the .nxs files, the generated .hdf5 files (for use with Phonon Explorer), and Python scripts used to create them.

36 MATERIALS SCIENCE↗

History and current understanding of the Suess abundance curve

By means of a gamma ray sum spectrometer currently under development, many neutron capture cross sections will be determined with high accuracy, thereby facilitating the inferrence of the abundance ratios of neighboring elements with the same accuracy. Attention is presently given to this and other prospects emerging in the study of nuclide abundances and the data base for theories of element synthesis. Poorly understood structures in the abundance curve are discussed in view of recent models on nuclear structure and stability.

Marti, K.↗

Measurements of the Neutron Magnetic Form Factor and the Two-Photon Exchange Contribution to the Electron-Neutron Elastic Scattering Cross Section

The Super BigBite Spectrometer (SBS) program in Experimental Hall A of Jefferson Lab is a series of high-precision, large ?2 , electromagnetic form factor experiments. GMn and nTPE were the first two experiments of the SBS program and ran from Oc?tober 2021 through February 2022. Both experiments detect neutron-tagged ?(?, ???) and proton-tagged ?(?, ???) quasi-elastic electrons scattering from a deuterium tar?get. The GMn experiment is a measurement of the magnetic form factor of the neutron, ?? ?, via the ratio method over a ?2 range of 3.5 to 13.5 (GeV/c)2 . The nTPE experiment ran in-parallel with the GMn experiment and shared an overlap?ping kinematic point with GMn. nTPE extends the GMn experiment to assess the differences between Rosenbluth Slop and the single-photon exchange approximation. The nTPE experiment had two kinematic settings corresponding to different electron scatting angles at a fixed ?2 of 4.5 (GeV/c)? . Comparisons of nucleon form factor ratio measurements acquired through polarization transfer and LT separation reveal discrepancies as ?2 increases. Two-photon exchange is strongly favored as the reason for this discrepancy. ?? ? has been extracted at two kinematic settings corresponding to ?2 values of 3.0 and 4.5 (GeV/c)2 . Additionally, I will present an assessment of the differences between Rosenbluth Separation and single-photon exchange measure?ments.

Boyd III, John Alan↗

The pNab experiment and the quest for ever better neutron beam polarization

The Nab and pNAB collaborations are conducting a program of studies of free neutron beta decay, with the primary goal of testing the unitarity of the Cabbibo-Kobayashi-Maskawa matrix that describes quark mixing due to the weak interaction. For this purpose, a large, novel electromagnetic spectrometer, the Nab spectrometer, has been designed, built, and placed in use to determine the correlation coefficients in unpolarized neutron beta decay: "a", the neutrino-electron correlation coefficient; and "b", the Fierz term. The subject of this paper is pNAB, the second phase of the program, that will deploy the same spectrometer with a polarized neutron beam to determine "A", the beta asymmetry; and "B", the neutrino asymmetry coefficients. A focus of this paper will be on the strategies to provide a high and precisely known neutron beam polarization.

Baessler, Stefan↗

Interpreting scattered neutron spectra on omega cryogenic implosions with measured backgrounds and higher-order scattering

Measurements of the areal density (⁠ρR⁠) of inertially confined implosions are critical to evaluate their performance. On OMEGA, ρR is inferred from measurements of the scattered neutron spectrum via neutron-time-of-flight (nTOF) and magnetic recoil spectrometer detectors. The nTOF measurements, in particular, have the ability to measure a wide range of neutron energies and thus scattering angles, with high precision. However, the neutrons that are backscattered into the detector must transit through the entire dense fuel assembly, and as a result are subject to rescattering effects, which have been heretofore neglected in the interpretation of OMEGA neutron spectra. At the backscatter edge, neglecting rescattering on OMEGA can lead to a ~10 to 20% reduction of the apparent areal density and therefore must be included in the analysis. The low ρR s on OMEGA also mean that backgrounds from non-target physics effects, such as scattering in the target chamber or slow scintillator decays, can significantly alter the measured signal. Here, we discuss how the Monte Carlo neutron spectrum postprocessor IRIS is used to include second-order scattering effects in the interpretation of the scattered neutron spectrum in OMEGA implosion experiments, and how dedicated implosion experiments are used to measure nTOF backgrounds in order to infer backscattered areal densities on OMEGA.

Deuterium↗

Measuring planetary hydrogen by remote gamma-ray sensing

The detection and measurement of hydrogen concentration and neutron leakage flux in planetary bodies by means of a proximate gamma-ray spectrometer (GRS) are discussed. The H concentration and the neutron flux are intimately linked in the planetary surface, and the measurement of hydrogen is dependent on knowledge of the neutron flux. The capture of thermal neutrons is responsible for the production of the 2.223 MeV line which characterizes hydrogen. The 2.223 MeV H signal is observed in the gamma-ray spectrum against an interference spectrum consisting of cosmic gamma rays, planetary background emission, and gamma rays arising from the interaction of cosmic rays with the GRS and the spacecraft (SC). An interfering line background results from the interaction of slow neutrons with H in the GRS and SC. The sources and magnitudes of the signal and background components in the H band are identified in terms of two missions, a lunar orbiter and a comet nucleus rendezvous. For the lunar mission, a 100 h observation at a 100 km altitude permits the detection of H at a level of 0.06 percent with an uncertainty of about 0.02 percent, while at an altitude equal to the radius of the comet's nucleus, in 100 h a GRS detects H at a level of 0.07 percent with an uncertainty of 0.06 percent.

Haines, E. L.↗

Simulation experiments for gamma-ray mapping of planetary surfaces: Scattering of high-energy neutrons

The concentration and distribution of certain elements in surface layers of planetary objects specify constraints on models of their origin and evolution. This information can be obtained by means of remote sensing gamma-ray spectroscopy, as planned for a number of future space missions, i.e., Mars, Moon, asteroids, and comets. To investigate the gamma-rays made by interactions of neutrons with matter, thin targets of different composition were placed between a neutron-source and a high-resolution germanium spectrometer. Gamma-rays in the range of 0.1 to 8 MeV were accumulated. In one set of experiments a 14-MeV neutron generator using the T(d,n) reaction as neutron-source was placed in a small room. Scattering in surrounding walls produced a spectrum of neutron energies from 14 MeV down to thermal. This complex neutron-source induced mainly neutron-capture lines and only a few scattering lines. As a result of the set-up, there was a considerable background of discrete lines from surrounding materials. A similar situation exists under planetary exploration conditions: gamma-rays are induced in the planetary surface as well as in the spacecraft. To investigate the contribution of neutrons with higher energies, an experiment for the measurement of prompt gamma radiation was set up at the end of a beam-line of an isochronous cyclotron.

Brueckner, J.↗