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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 253 records · Page 14
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Transient quantum beatings of trions in hybrid organic tri-iodine perovskite single crystal

Utilizing the spin degree of freedom of photoexcitations in hybrid organic inorganic perovskites for quantum information science applications has been recently proposed and explored. However, it is still unclear whether the stable photoexcitations in these compounds correspond to excitons, free/trapped electron-hole pairs, or charged exciton complexes such as trions. Here we investigate quantum beating oscillations in the picosecond time-resolved circularly polarized photoinduced reflection of single crystal methyl-ammonium tri-iodine perovskite (MAPbI 3 ) measured at cryogenic temperatures. We observe two quantum beating oscillations (fast and slow) whose frequencies increase linearly with B with slopes that depend on the crystal orientation with respect to the applied magnetic field. We assign the quantum beatings to positive and negative trions whose Landé g-factors are determined by those of the electron and hole, respectively, or by the carriers left behind after trion recombination. These are $g^{e}_{[001]}$ = 2.52 and $g^{e}_{[1\bar10]}$ = 2.63 for electrons, whereas |$g^{h}_{[001]}$| = 0.28 and |$g^{h}_{[1\bar10]}$| = 0.57 for holes. The obtained g-values are in excellent agreement with an 8-band K.P calculation for orthorhombic MAPbI3. Using the technique of resonant spin amplification of the quantum beatings we measure a relatively long spin coherence time of ~ 11 (6) nanoseconds for electrons (holes) at 4 K.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS1984

First measurements of supersonic polar wind in the polar magnetosphere

Measurements from the Retarding Ion Mass Spectrometer on the Dynamics Explorer have, for the first time, revealed a supersonic polar wind along polar cap field lines. The observations reported were obtained on the nightside (22:30 to 23:30 MLT) from 65 to 81 deg invariant latitude and at altitudes near 2 earth radii. Fitting the data using a thin-sheath model gives a range of temperatures of 0.1 to 0.2 eV with corresponding flow velocities of 25 to 16 km/s over the estimated range of spacecraft potential of +3 to +5 V. For these values the Mach number ranged from 5.1 to 2.6 (with a most likely value of 3). Characteristics of the H(+) flow are in general agreement with those predicted by 'classical' polar wind theory, but high variabilty of the He(+)/H(+) ratio was observed.

Nagai, T.↗
DOE OSTI2023

Formulation and testing of a high-tin borosilicate nuclear waste glass for in-can melting

Here, borosilicate waste glasses were successfully developed to immobilize two high-level waste raffinate streams via an in-can melter process with an Inconel 601 canister at 1050 °C. Measured viscosity and crystallinity thermal profiles were within the targeted processing constraints for the in-can melter process. Measured chemical durability of the glass by ASTM C1285–21 (Method A), ranged from normalized loss of boron, NL(B) = 1.44 – 2.65 g•m -2 , and NL(B) decreased with increased waste loading, accompanied by increased SnO 2 crystallinity. Measured corrosion of the in-can melter canister by a glass melt showed that Inconel 601 performed well at 1100 °C for up to 500 hr. Resistance polarization measurements versus time revealed that Inconel 601 corrosion rates in (and by) glass melts decreased from an initial rate of 63 mm•y -1 down to 10.2 mm•y -1 after 137 h with increased duration, which was attributed to formation of an oxide passivation layer (mainly Cr 2 O 3 ) at the alloy-glass interface.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2022

High-temperature fractional quantum Hall state in the Floquet kagome flat band

A fractional quantum Hall effect (FQHE) has been predicted in a topological flat band (FB) by a single-particle band structure combined with phenomenological theory or solution of a many-body lattice Hamiltonian with fuzzy parameters. A long-standing roadblock toward the realization of a FB-FQHE is lacking the many-body solution of specific materials under realistic conditions. Here, we demonstrate a combined study of single-particle Floquet band theory with exact diagonalization (ED) of a many-body Hamiltonian. We show that a time-periodic circularly polarized laser inverts the sign of second-nearest-neighbor hopping in a kagome lattice and enhances spin-orbit coupling in one spin channel to produce a Floquet FB with a high flatness ratio of bandwidth over band gap, as exemplified in monolayer Pt 3 C 36 S 12 H 12 . The ED of the resultant Floquet-kagome lattice Hamiltonian gives a one-third-filling ground state with a laser-dependent excitation gap of a FQH state, up to an estimated temperature above 70 K. Our findings pave the way for exploring the alluding high-temperature FB-FQHE.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Giant spin-selective bandgap renormalization in CsPbBr 3 colloidal nanocrystals

The spin-dependence of the strongly correlated phenomena and many-body interactions play an important role in quantum information science. In particular, it is quite interesting but unclear how the spin degree of freedom ramifies the bandgap renormalization, one of the fundamental many-body phenomena. We report the first room-temperature observation of giant spin-selective bandgap renormalization (SS-BGR) in CsPbBr 3 colloidal nanocrystals using time-resolved circularly polarized femtosecond pump-probe spectroscopy. The SS-BGR results from many-body interactions among carriers with the same spin that renormalize their joint density of states by 57+/- 1 meV, visualized here as photoinduced absorption (PIA) below band-edge transition energy when the pump and probe are co-polarized. The hallmark result of spectrally resolved SS-BGR is in stark contrast to the usually submerged signal in II-VI and III-V semiconductors and is 3 orders of magnitude larger than that observed in Ge/SiGe quantum wells, highlighting the unique and beneficial band structure of the metal-halide semiconductors. We propose that the PIA, due to SS-BGR, can be used to describe the spin-polarization and spin-relaxation dynamics. The experimental and theoretical findings open up new possibilities for optical manipulation of spin degrees of freedom and their many-body interactions in metal-halide perovskite nanocrystals for potential room-temperature applications.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

Floquet-driven indirect exchange interaction mediated by topological insulator surface states

Light drives offer a potential tool for the dynamical control of magnetic interactions in matter. We theoretically investigate the indirect exchange coupling between two parallel chains of magnetic impurities on the surface of a topological insulator, driven by a time-periodic circularly polarized light field in the high-frequency, off-resonant regime. We derive a closed-form analytic expression for the spin susceptibility of the photon-dressed topological insulator surface states and obtain the irradiation dependence of the Ising, Heisenberg, and Dzyaloshinskii-Moriya exchange couplings between the impurity chains. Our results show a two-pronged modification of these exchange couplings by periodic drives. First, the Ruderman-Kittel-Kasuya-Yosida (RKKY) oscillation period of the exchange couplings can be extended by enhancing the driving strength. Second, increasing driving strength enhances the envelope of RKKY oscillations of the Ising type while suppressing those of the Heisenberg type and Dzyaloshinskii-Moriya type. Furthermore, our work provides useful insights for realizing Floquet engineering of collinear and noncollinear indirect exchange interactions in topological insulating systems.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2020

Gravitational-wave signal of a core-collapse supernova explosion of a 15M ⊙ star

In this paper we report on the gravitational-wave signal computed in the context of a three-dimensional simulation of a core-collapse supernova explosion of a 15 M ⊙ star. The simulation was performed with our neutrino hydrodynamics code chimera . We detail the gravitational wave strains as a function of time, for both polarizations, and discuss their physical origins. We also present the corresponding spectral signatures. Gravitational wave emission in our model has two key features: low-frequency emission (less than 200 Hz) emanates from the gain layer as a result of neutrino-driven convection and the standing accretion shock instability (SASI), and high-frequency emission (greater than 600 Hz) emanates from the proto–neutron star due to Ledoux convection within it. The high-frequency emission dominates the gravitational wave emission in our model and emanates largely from the convective layer itself, not from the convectively stable layer above it, due to convective overshoot. Moreover, the low-frequency emission emanates from the gain layer itself, not from the proto–neutron star, due to accretion onto it. We provide evidence of the SASI in our model and demonstrate that the peak of our low-frequency gravitational wave emission spectrum corresponds to it. Given its origin in the gain layer, we classify the SASI emission in our model as p-mode emission and assign a purely acoustic origin, not a vortical–acoustic origin, to it. We compare the results of our three-dimensional model analysis with those obtained from the model’s two-dimensional counterpart and find a significant reduction in the strain amplitudes in the former case, as well as significant reductions in all related quantities. Our dominant proto–neutron star gravitational wave emission is not well characterized by emission from surface g modes, complicating the relationship between peak frequencies observed and the mass and radius of the proto–neutron star expressed by analytic estimates under the assumption of surface g-mode emission. We present our frequency normalized characteristic strain along with the sensitivity curves of current- and next-generation gravitational wave detectors. This simple analysis indicates that the spectrum of gravitational wave emission between approximately 20 Hz and approximately 1 kHz, stemming from neutrino-driven convection, the SASI, accretion onto the proto–neutron star, and proto–neutron star convection, will be accessible for a Galactic event.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1972

Pulsar rotation and dispersion measures and the galactic magnetic field.

Use of observations of pulsar polarization and pulse time of arrival at frequencies between 250 and 500 MHz to determine rotation and dispersion measures for 19 and 21 pulsars, respectively. These measurements have been used to calculate mean line-of-sight components of the magnetic field in the path to the pulsars. These and other observations show that there is probably no contribution to the observed rotation measure from the pulsar itself. Low-latitude, low-dispersion pulsars are observed to have strong field components, and a strong dependence of rotation-measure sign on galactic longitude has been found. The observations are consistent with a relatively uniform field of about 3.5 microgauss directed toward about l = 90 deg in the local region, but appear to be inconsistent with the helical model for the local field.

Manchester, R. N.↗
NASA NTRS1972

Analysis of a dual-reflector antenna system using physical optics and digital computers

The application of physical-optics diffraction theory to a deployable dual-reflector geometry is discussed. The methods employed are not restricted to the Conical-Gregorian antenna, but apply in a general way to dual and even multiple reflector systems. Complex vector wave methods are used in the Fresnel and Fraunhofer regions of the reflectors. Field amplitude, phase, polarization data, and time average Poynting vectors are obtained via an IBM 360/91 digital computer. Focal region characteristics are plotted with the aid of a CalComp plotter. Comparison between the GSFC Huygens wavelet approach, JPL measurements, and JPL computer results based on the near field spherical wave expansion method are made wherever possible.

Schmidt, R. F.↗
NASA NTRS1973

Synchrotron sources. II - Pulsars and compact extragalactic objects.

Discussion of some limitations on synchrotron models for optical pulsars and compact extragalactic objects. Using the results of a previous paper, it is shown that several existing models for the pulsar NP 0532 are inconsistent with the measured time variations and polarization of the optical emission. The possibility that the low-frequency falloffs in some extragalactic objects (PKS 2134 + 004, OQ 208, and NGC 1068) could be due to emission from particles with small pitch angles, absorption by a thermal plasma, or synchrotron self-absorption is also considered. It is found that radiation by particles with small pitch angles could explain the radio emission from PKS 2134 + 004 and OQ 208, but this process is inconsistent with the observations of NGC 1068. The absorption interpretations cannot account for the turnover in the spectrum of PKS 2134 + 004.

Epstein, R. I.↗
NASA NTRS1974

Transcontinental baselines and the rotation of the earth measured by radio interferometry

Nine separate very-long-baseline interferometry experiments, carried out in 1972 and 1973 with radio telescopes 3900 kilometers apart, yielded values for the baseline length with an rms deviation about the mean of less than 20 centimeters. The corresponding fractional spread is about five parts in 100,000,000. Changes in universal time and in polar motion were also determined accurately from these data. The rms scatter of these results with respect to those based on optical methods was 2.9 msec and 1.3 m, respectively. Solid-earth tides were apparently detected, but no useful estimate of their amplitude was extracted.

Shapiro, I. I.↗
NASA NTRS1977

Planetary radio astronomy receiver

The planetary radio astronomy (PRA) experiment on the Voyager spacecraft will measure the amplitude, spectrum, time variations, and polarization of radio emissions over a frequency range of 1.2 kHz to 40.5 MHz with the aid of the PRA receiver (PRAR) and two 10-m orthogonal monopoles. Sensitivity and dynamic range will allow observation of a wide range of Jovian emissions from near earth to encounter. This paper describes the system elements, including the preamp/attenuator/calibrator, the LF polarization discriminator, the four LF-IF amplifier stages, the HF polarization discriminator, the translation LO, the log-IF and detector, the frequency synthesizer, the data processor, control system, power supply, and antennas.

Lang, G. J.↗
NASA NTRS1978

Venus - Further evidence of vortex circulation

A space-time composite of polar stereographic ultraviolet images of Venus from Mariner 10 shows a remarkable circumpolar vortex. The vortex is characterized by a cloud which appears similar to dense terrestrial stratus having an albedo that is 50 percent higher. Spiral streaks converge into it from low latitudes, akin to the spiral bands of a hurricane. The bright visible polar cloud is not axisymmetric but has roughly an elliptical shape. The high brightness of the polar cloud suggests that it has a different origin from the rest of the Venus cloud cover.

Suomi, V. E.↗
NASA NTRS1979

CTS 11.7 GHz isolation data for the calendar year 1978

Monthly and annual percent-of-time data on polarization isolation measured for the CTS spacecraft 11.7 GHz downlink are presented. The relationship between isolation and attenuation and the degree to which isolation can be predicted from attenuation data are discussed.

Bostian, C. W.↗