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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 271 records · Page 15
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Precision measurements on oxygen formation in stellar helium burning with gamma-ray beams and a Time Projection Chamber

The carbon/oxygen (C/O) ratio at the end of stellar helium burning is the single most important nuclear input to stellar evolution theory. However, it is not known with sufficient accuracy, due to large uncertainties in the cross-section for the fusion of helium with 12 C to form 16 O, denoted as 12 C( α , γ ) 16 O. Here we present results based on a method that is significantly different from the experimental efforts of the past four decades. With data measured inside one detector and with vanishingly small background, angular distributions of the 12 C( α , γ ) 16 O reaction were obtained by measuring the inverse 16 O( γ , α ) 12 C reaction with gamma-beams and a Time Projection Chamber (TPC) detector. We agree with current world data for the total reaction cross-section and further evidence the strength of our method with accurate angular distributions measured over the 1 - resonance at E cm ~2.4 MeV. Our technique promises to yield results that will surpass the quality of the currently available data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Augmenting machine learning of energy landscapes with local structural information

We present a machine learning approach for accurately predicting formation energies of binary compounds in the context of crystal structure predictions. The success of any machine learning model depends significantly on the choice of representation used to encode the relevant physical information into machine-learnable data. We test different representation schemes based on partial radial and angular distribution functions (RDF+ADF) on Al–Ni and Cd–Te structures generated using our genetic algorithm for structure prediction. We observe a remarkable improvement in predictive accuracy upon transitioning from global to atom-centered representations, resulting in a threefold decrease in prediction errors. We show that a support vector regression model using a combination of atomic radial and angular distribution functions performs best at the formation energy prediction task, providing small root mean squared errors of 3.9 meV/atom and 10.9 meV/atom for Al–Ni and Cd–Te, respectively. We test the performance of our models against common traditional descriptors and find that RDF- and ADF-based representations significantly outperform many of those in the prediction of formation energies. The high accuracy of predictions makes our machine learning models great candidates for the exploration of energy landscapes.

Honrao, Shreyas J. (ORCID:0000000166155257)↗
DOE OSTI2023

Resolved Resonance Region Analysis of 206 Pb, 207 Pb, and 208 Pb for Next Generation Lead-Cooled Fast Systems

Recently, great interest has been generated in using lead as a coolant for fast neutron systems and as a result it is important to investigate the ENDF/B-VIII.0 isotopic evaluations that comprise stable le ad. To this end, resonance parameters for 206 Pb, 207 Pb, and 208 Pb were re-evaluated because their resolved reso­nance regions extend beyond 0.5 MeV meaning resonance parameters used in reconstructing cross sections and elastic scattering angular distributions impact fast systems. The impact of resonance parameters is demon­strated by the differences between the evaluations in predicting experimental results from the fully modeled RPI Quasi-Differential Scattering Experiment via MCNPv6.2. In addition, MCNP KCODE calculations of lead-sensitive fast spectra critical benchmarks showed variations of keff on average of 400 pcm, caused solely from differences in elastic scattering angular distributions in 208 Pb. Re-evaluation entailed fitting data with the program SAMMY.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
NASA NTRS1973

Energy transfer from a pulsed thermal source to He II below 0.3 K.

Results of measurements of the angular distribution of the energy flux radiated from a pulsed heater immersed in He II at low temperatures (around 230 mK). It is shown that the energy transfer from a pulsed carbon heater at a relatively high temperature to ambient liquid helium maintained at low temperature cannot be adequately described by the phonon-coupling models. The experimental data on the velocity and angular distribution of the energy flux radiated from the plane of the heater indicate that the energy from the heater is transferred to a layer of hot helium adjacent to the surface of the heater and that this layer acts as the effective source of excitations radiated into the ambient liquid helium. The extent and shape of this source depend on the total energy flux produced by the heater.

Pfeifer, C. D.↗
NASA NTRS1973

Low-energy electron experiment for Atmosphere Explorer-C and -D.

The low-energy electron experiment will provide differential measurements of the energy influx and angular distributions of electrons and protons on the Atmosphere Explorer-C and -D missions. The detectors consist of cylindrical electrostatic analyzers for species and energy selection and Spiraltron electron multipliers as particle sensors. The C version will contain three detectors, two measuring electrons and protons from 0.2 to 25 keV in 16 logarithmically spaced steps and one measuring 5 keV electrons continuously. Angular distributions will be acquired utilizing the spin of the spacecraft. The D version will contain 19 detectors, one proton-stepped energy analyzer, and two electron-stepped energy analyzers at two different angles, again over the energy range 0.2 to 25 keV.

Hoffman, R. A.↗
NASA NTRS1977

The angular dependence of partially redistributed resonance radiation

Explicit expressions for the angular distribution and frequency dependence of radiation scattered by a spatially degenerate atom undergoing collisions are derived using a previously developed formalism of the quantum theory of line broadening for an atom in its rest frame. Results valid in the impact regime for resonant scattering are presented for the cases of linear incident and scattered polarization circular incident and linear scattered polarization, and unpolarized incident radiation with no monitoring of the scattered polarization. These results relate to scattering involving a j - j + or - 1 - j atomic transition, with lower-state interactions neglected; the expressions obtained take a relatively simple form involving atomic multipolar relaxation rates of the order of k = 0 and k = 2. The angular distributions for each case are combined with the frequency dependences to yield a three-component frequency redistribution function for an s-p-s transition, the components being a coherent term, a frequency-redistributed term with the same angular dependence as the coherent term, and an isotropic frequency-redistributed term.

Ballagh, R. J.↗
DOE OSTI2023

Polarized fusion and potential in situ tests of fuel polarization survival in a tokamak plasma

Abstract The use of spin-polarized fusion fuels would provide a significant boost towards the ignition of a burning plasma. The cross section for D + T → α + n, would be increased by 1.5 if the fuels were injected with parallel polarization. Furthermore, our simulations demonstrate additional non-linear power gains in large-scale machines such as ITER, due to increased alpha heating. Such benefits require the survival of spin polarizations for periods comparable to the particle confinement time. During the 1980s, calculations predicted that polarizations could survive a plasma environment, although concerns persisted regarding the cumulative impacts of wall recycling. In that era, technical challenges prevented direct tests and left the large scale fueling of a power reactor beyond reach. Over the last decades, this situation has changed dramatically. Detailed simulations of ITER have predicted negligible wall recycling in a high-power reactor, and recent advances in laser-driven sources project the capability of producing large quantities of ∼100% polarized D and T. The remaining crucial step is an in-situ demonstration of polarization survival in a plasma. For this, we outline a measurement strategy using the isospin-mirror reaction, D + 3 He → α + p. Polarized 3 He avoids the complexities of handling tritium, while encompassing the same spin-physics. We evaluate two methods of delivering deuterium, using dynamically polarized Lithium-Deuteride (with vector polarization P V D of 70%) or frozen-spin Hydrogen-Deuteride (with P V D of 40%), together with a method of injecting optically-pumped 3 He (with 65% polarization). Pellets of these materials all have long polarization decay times (∼6 min for LiD at 2 K, ∼2 months for HD at 2 K, and ∼3 d for 3 He at 77 K), all far greater than a plasma shot in a research tokamak such as DIII-D (∼20 s). Both species can be propelled from a single cryogenic injection gun. We review plasma requirements and strategies for detecting polarization survival. Polarization alters both fusion yields and the angular distribution of fusion products, and each of these provides a potential signal. In this paper we simulate a selection of shots with similar characteristics in a future high-T ion H plasma, and find ratios of yields from shots with fuel spins parallel and antiparallel reaching 1.3 (HD + 3 He) to 1.6 (LiD + 3 He) over a wide range of poloidal angles. (A companion paper finds sensitivity to fusion product angular distributions as reflected in the pitch angles of protons and alphas reaching the plasma facing wall.)

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS1980

Observations of energetic ions and electrons in Saturn's magnetosphere

Observations of the magnetosphere of Saturn made by the cosmic-ray experiment on board Pioneer 11 are summarized. Detailed energy spectra and angular distributions of protons from 0.2 to 22 MeV and electrons from 0.1 to 2 MeV were obtained, together with measurements of helium nuclei between 0.65 and 22 MeV/n. The time histories of proton and electron data suggest a division of the Saturn magnetosphere into three regions: (1) an outer magnetosphere between 17 and 7.5 Saturn radii, which is characterized by monotonically increasing fluxes and spectral hardening inward from the magnetosphere, with large changes in low-energy electron angular distributions; (2) a slot region between 7.5 and 4 Saturn radii where marked decreases in proton and low-energy electron fluxes are observed, apparently due to the presence of Dione, Tethys and Enceladus; and (3) an inner region between 4 Saturn radii and the ring edge, which exhibits sharp increases in proton fluxes with energies up to 20 MeV, which are broken near the orbits of Mimas, Janus and possibly S 11. A sharp cutoff of proton and electron fluxes is observed just beyond the nominal edge of the A ring.

Trainor, J. H.↗
DOE OSTI2025

Systematic study of the validity of the eikonal model including uncertainties

Nuclear reactions at intermediate beam energies are often interpreted using the eikonal model. In the analysis of complex reaction probes, where few-body reaction methods are needed, the eikonal method may be used as an efficient way for describing the fragment-target reaction process. In this work, we perform a systematic study to test the validity of the eikonal approximation for nucleon-nucleus reactions. We also quantify uncertainties due to the nucleon optical potential on reaction observables. We inspect the validity of the eikonal model and its semiclassical correction by comparing it to exact solutions (obtained from solving the optical-model equation with a finite-differences method) for a wide range of reactions. We also study the effect of relativistic corrections, both kinematic and dynamic, by effectively incorporating the relativistic effects at intermediate energies. The uncertainties from a Bayesian global optical potential (KDUQ) are propagated to the observables of interest. Our study includes neutron and proton reactions on 27 Al , 40 Ca , 90 Zr , and 208 Pb , for a wide range of energies 𝐸 lab = 0–400 MeV. We calculate neutron-total cross sections (elastic and reactions) as well as proton-absorption cross sections as a function of beam energy, using the eikonal model, the eikonal model with a semiclassical correction, and the exact solution. Here, we also compute angular distributions for the methods above. Our results show that for the proton-absorption cross section, the eikonal model can be used down to around 60 MeV and the semiclassical correction extends its use to 30 MeV. However, the validity of the eikonal model for the neutron-total cross section only goes down to ≈120 MeV, a range extended to ≈ 50 MeV when using the semiclassical correction. We find the semiclassical correction to the eikonal model to be less effective in describing the angular distributions. The 1⁢𝜎 uncertainty intervals on the observables we studied is less than 5% for most of the energies considered, but increases rapidly for higher energies, namely energies outside the range of KDUQ (𝐸 lab > 200MeV).

Cluster models↗
NASA NTRS1991

Ion burst event in the earth's dayside magnetosheath

The Medium Energy Particle Analizer instrument on the AMPTE/CCE Spacecraft provided ion angular distributions as rapidly as every 6 sec for H, He, and O at energies of 10 keV to 2 MeV in the dayside magnetosheath whenever the solar wind pressure compressed the magnetopause within 8.75 R(E), the CCE apogee. This paper discusses a burst of energetic particles in the subsolar magnetosheath and its association with rapid changes in the local magnetic field direction in such a way the magnetic field connected the spacecraft to the magnetopause during the enhancement. It is found that magnetosheath angular distributions outside the burst peaked at 90 deg pitch angles, whereas during the burst they exhibited field-aligned streaming either parallel or antiparallel to the magnetic-field combined with a clear earthward gradient. The clear earthward gradients at E not smaller than 10 KeV, the streaming, and the slope change in the burst-time magnetosheath spectrum at about 10 KeV suggest magnetospheric source for the burst-time not smaller than 10 KeV ions and heated solar wind for E less than 10 KeV.

Paschalidis, N. P.↗
NASA NTRS1986

Differential electron scattering cross sections for the first optically forbidden and resonance transitions in Mg II, Zn II and Cd II

Differential electron scattering cross sections have been measured for dipole-forbidden and resonance transitions in Mg II, Zn II and Cd II in the angular range theta = 4-17 deg at 50 eV. These provide the first recorded angular distributions for an optically forbidden transition. It is found that while the cross section for excitation of the 4s (2)S-3d(9)4s(2) (2)D transition in Zn II is small, those for the 3s (2)S-3d (2)D, 4s (2)S (unresolved lines) in Mg II, and the 5s (2)S-4d(9)5s(2) D in Cd II are comparable in magnitude with the cross sections for resonance excitation. In addition, for Cd II it is found that the allowed and forbidden transitions have very similar angular distributions, and it is proposed that excitation to the 2D state may be dominated by a virtual 'double-dipole' transition via the 2P state. Also, the total excitation cross section of the resonance 2P state in Cd II is a factor of four higher than that predicted by the Gaunt factor approximation, suggesting that the accepted value for the oscillator strength may be too low.

Williams, I. D.↗
NASA NTRS2021

Results from the MISSE 6 Scattered Space Atomic Oxygen Experiment (SSAOE)

Polymers and other oxidizable materials used on the exterior of spacecraft in the low Earth orbit (LEO) space environment can be eroded away by reaction with atomic oxygen (AO). NASA Glenn Research Center developed an active flight experiment, called the Scattered Space Atomic Oxygen Experiment (SSAOE), to characterize AO scattering erosion in space. The SSAOE is comprised of three independent sub-experiments: A two part active experiment to measure both in-situ direct ram AO erosion and in-situ scattered AO erosion within an AO scatterometer; a passive AO scatterometer to measure the angular distribution of LEO AO scattered off an inclined angle; and passive samples for AO erosion yield (Ey) characterization. The SSAOE was originally flown on the Wake Shield Facility (WSF) during the STS-60 shuttle mission, and was later flown as part of the MISSE 6 mission on the exterior of the ISS. During the MISSE-6 mission the SSAOE was exposed to the space environment for 1.45 years. This paper provides an overview of the SSAOE, information on the flight missions, post-flight photographs of the passive flight samples and results on the angular distribution of scattered LEO AO obtained from the passive AO scatterometer sub-experiment. The LEO scattered AO erosion data can be used to improve AO undercutting models and durability predictions of spacecraft components receiving scattered AO.

Atomic oxygen, erosion, undercutting, spaceflight ↗
NASA NTRS1978

Single and multiple scattering contributions to circumsolar radiation

The contributions to the angular distribution of the almucantar radiance in the forward direction due to multiple scattering are compared to those due to single scattering. The contributions have been calculated by a computer code employing the Gauss-Seidel iterative approach to the solution of the radiative transfer equation for a plane parallel atmosphere composed of air molecules, aerosol particles, and ozone. The code is similar to that of Dave (1972) except in the construction of the source matrix. In the near-forward direction the multiple scattering contributions are significant for optical depths of the order of 0.4. The shape of the angular distribution of almucantar radiance to 10 degrees is less sensitive to multiple scattering.

Box, M. A.↗
NASA NTRSDate not supplied

Radiative Flux Measurements from ARISE: A Comparison with CERES Top-of-Atmosphere Radiative Fluxes

Uncertainty in top-of-atmosphere (TOA) radiation fluxes observations are larger in the Arctic than in other regions. These uncertainties are due to the low sun angles and the highly reflective, anisotropic, and heterogeneous surface conditions. Quantifying, attributing, and reducing Arctic TOA radiative flux uncertainty enables a better understanding of the rapidly changing Arctic. To advance this goal, we compare the Cloud and Earth’s Radiant Energy System (CERES) TOA radiative fluxes with Arctic Radiation-IceBridge Sea and Ice Experiment (ARISE) campaign measurements collected in September 2014. We compare CERES TOA and aircraft radiative flux measurements using two complementary approaches: grid box average fluxes and instantaneously matched footprints. The grid box mean flux comparison indicates an agreement between CERES and aircraft measurements within 2 uncertainty (calibration and inversion) in the longwave for all five grid boxes and for four-of-five grid boxes in the shortwave; shortwave and longwave mean differences are -7.9 and +2.3 Wm‑2, respectively. The comparison of 36 instantaneously matched footprints with aircraft measurements reveals mean differences of -10.5 and 0.4 Wm‑2 in the shortwave and longwave, respectively. To further explore the persistent negative difference in the shortwave, we further quantify the effects of temporal and spatial sampling differences, angular distribution models, and scene identification to CERES-aircraft differences. Our analysis indicates that sampling differences (including scene evolution) account for an additional 1.8 and 1.7% uncertainty in the shortwave and longwave, respectively and indicates no bias. After accounting for this sampling uncertainty, all CERES-aircraft grid box mean fluxes agree within 2 uncertainty. Scene identification errors due to sea ice concentration data set differences exhibit no bias in the shortwave flux difference and indicate the possibility of substantial differences in the CERES fluxes in specific cases with large spatial heterogeneity. Considering the instantaneously matched footprints, we find that the angular distribution models account may account for up to ‑7.3 Wm-2 of the persistent CERES-aircraft shortwave flux difference due to systematic differences in the anisotropy for sea ice partly cloudy scenes. Additional analysis using a special scan model with the CERES FM2 instrument suggests a significant view zenith angle dependence of the CERES fluxes for sea ice partly cloudy scenes where shortwave fluxes systematically decrease with increasing view zenith angle; no dependence is found for other scene types. We conclude that (1) spatial heterogeneity and scene temporal evolution substantially limit our ability to use aircraft measurements to place strong constraints on CERES TOA fluxes and (2) that the representation of anisotropy in sea ice partly cloudy scenes is a significant factor contributing to the persistent negative CERES-aircraft shortwave flux difference in this comparison and require additional data to analysis fully quantify the potential bias.

Patrick C Taylor↗
NASA NTRSDate not supplied

A comparison between CERES TOA Radiative Fluxes and Airborne Radiative Flux Measurements from ARISE

Uncertainty in top-of-atmosphere (TOA) radiation fluxes observations are larger in the Arctic than in other regions. These uncertainties are due to the low sun angles and the highly reflective, anisotropic, and heterogeneous surface conditions. Quantifying, attributing, and reducing Arctic TOA radiative flux uncertainty enables a better understanding of the rapidly changing Arctic. To advance this goal, we compare the Cloud and Earth’s Radiant Energy System (CERES) TOA radiative fluxes with Arctic Radiation-IceBridge Sea and Ice Experiment (ARISE) campaign measurements collected in September 2014. We compare CERES TOA and aircraft radiative flux measurements using two complementary approaches: grid box average fluxes and instantaneously matched footprints. The grid box mean flux comparison indicates an agreement between CERES and aircraft measurements within 2σ uncertainty (calibration and inversion) in the longwave for all five grid boxes and for four-of-five grid boxes in the shortwave; shortwave and longwave mean differences are -7.9 and +2.3 Wm 2, respectively. The comparison of 36 40 instantaneously matched footprints with aircraft measurements reveals mean differences of -120.25 and -1.00.4 Wm 2 in the shortwave and longwave, respectively. To further explore the persistent negative difference in the shortwave, Wwe further quantify the effects of temporal and spatial sampling differences, angular distribution models, and scene identification to CERES-aircraft differences. Our analysis indicates that sampling differences (including scene evolution) account for an additional 1.8 and 1.7% uncertainty in the shortwave and longwave, respectively and , but indicates no bias. After accounting for this sampling uncertainty, all CERES-aircraft grid box mean fluxes agree within 2σ uncertainty. Scene identification errors due to sea ice concentration data set differences exhibit no bias in the shortwave flux difference and indicate the possibility of substantial differences in the CERES fluxes in specific cases with large spatial heterogeneity. Considering the instantaneously matched footprints, we find that the angular distribution models account may account for up to 7.3 Wm-2 of the persistent CERES-aircraft shortwave flux difference due to systematic differences in the anisotropy for sea ice partly cloudy scenes. Additional analysis using a special programmable scan model with the CERES FM2 instrument suggests a significant view zenith angle dependence of the CERES fluxes for sea ice partly cloudy scenes where shortwave fluxes systematically decrease with increasing view zenith angle; no dependence is found for other scene types. We conclude that (1) spatial heterogeneity and scene temporal evolution substantially limit our ability to use aircraft measurements to place strong constraints on CERES TOA fluxes and (2) that the representation of anisotropy in sea ice partly cloudy scenes is likely a significant factor contributing to the persistent negative CERES-aircraft shortwave flux difference in this comparison and require additional data to analysis fully quantify the potential bias.

Patrick C. Taylor↗
DOE OSTI2023

Angularly resolved photoionization dynamics in atoms and molecules combining temporally and spectrally resolved experiments at ATTOLab and Synchrotron SOLEIL

We report results for XUV-IR two-photon ionization of Ar, Ne, NO, and O2, where an XUV attosecond pulse train is superimposed with a synchronized IR pulse, obtained at the ATTOLab laser facility using electron–ion coincidence 3D momentum spectroscopy. Temporally resolved photoelectron angular distributions providing angle-resolved time-delays for np ionization of Ar and Ne, achieved by reconstruction of attosecond beating by interference of two-photon transitions through a unified formalism (Joseph et al. in J Phys B At Mol Opt Phys 53:184007, 2020), are summarized. For inner valence XUV-IR dissociative photoionization of NO and O2 molecules, we report electron–ion kinetic energy correlation diagrams and disentangle the dissociative photoionization processes relying on parallel XUV experiments at Synchrotron SOLEIL. For ionization into the NO+(c3Π) ionic state, extending the formalism developed for single-photon ionization, we focus on photoelectron angular distributions averaged on the delay between the XUV and the IR field in the field frame, molecular frame, and electron frame of reference.

Joseph, J↗
DOE OSTI2024

State-Selective Double Photoionization of Atomic Carbon and Neon

Double photoionization (DPI) allows for a sensitive and direct probe of electron correlation, which governs the structure of all matter. For atoms, much of the work in theory and experiment that informs our fullest understanding of this process has been conducted on helium, and efforts continue to explore many-electron targets with the same level of detail to understand the angular distributions of the ejected electrons in full dimensionality. Expanding on previous results, we consider here the double photoionization of two 2p valence electrons of atomic carbon and neon and explore the possible continuum states that are connected by dipole selection rules to the coupling of the outgoing electrons in 3P, 1D, and 1S initial states of the target atoms. Carbon and neon share these possible symmetries for the coupling of their valence electrons. Results are presented for the energy-sharing single differential cross section (SDCS) and triple differential cross section (TDCS), further elucidating the impact of the initial state symmetry in determining the angular distributions that are impacted by the correlation that drives the DPI process.

Yip, Frank L. (ORCID:000000025409495X)↗
DOE OSTI2026

Probing early parton emissions in heavy ion collisions using the Lund jet plane

In scattering experiments, high-virtuality partons, i.e., quarks and gluons, initiate a series of additional parton emissions to create collimated sprays of particles known as jets. This paper presents a measurement of the Lund jet plane (LJP) of high-energy jets produced in lead-lead (PbPb) collisions and compares the results to data for proton-proton (pp) collisions. The LJP is formed by iteratively declustering the constituents of a jet into consecutive emissions and recording the relative transverse momentum ($k_\mathrm{T}$) and angle of the resulting emission with respect to its emitter. The angular distributions of two different $k_\mathrm{T}$ slices of the LJP are investigated for jets with radius parameter of 0.4 and transverse momentum in the range 200$-$1000 GeV. The PbPb (pp) data were recorded by the CMS experiment in 2018 (2017) and correspond to an integrated luminosity of 1.7 nb$^{-1}$ (301 pb$^{-1}$) at a nucleon-nucleon center-of-mass energy of 5.02 TeV. The measurement was designed to test whether the earliest jet emissions are produced before the formation of the quark-gluon plasma (QGP) in PbPb collisions. Within the experimental uncertainties, no significant difference is observed between the angular distribution of high-$k_\mathrm{T}$ emissions in \pp and PbPb collisions, which is consistent with these emissions occurring early in the jet evolution, before substantial interaction with the QGP.

Belyaev, Andrey [Yerevan Phys. Inst.] (ORCID:00000↗