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DOE OSTI2021

Bias-dependent displacement damage effects in a silicon avalanche photodiode

Radiation effects studies on a commercial beveled-edge avalanche photodiode (APD) showed that applying reverse bias to the device during irradiation enhanced the severity of apparent damage. Proton microbeam irradiations were made using a proton beam energy of 2 MeV and fluence ranging from 2.0 × 10 10 to 5.1 × 10 12 cm -2 . Charge collection measurements using the ion beam induced charge (IBIC) technique showed that relative losses increased by up to an order of magnitude when the reverse bias applied during irradiation increased from 50 to 1500 V. The presence of reverse bias also led to equivalent losses in charge collection that would only be seen in irradiations with an order of magnitude higher fluence in unbiased APDs. The results demonstrate that bias-enhanced irradiation damage is insufficiently understood and must be accounted for in characterizations of radiation effects.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2022

Cesium intercalation of graphene: A 2D protective layer on alkali antimonide photocathode

Alkali antimonide photocathodes have wide applications in free-electron lasers and electron cooling. The short lifetime of alkali antimonide photocathodes necessitates frequent replacement of the photocathodes during a beam operation. Furthermore, exposure to mediocre vacuum causes loss of photocathode quantum efficiency due to the chemical reaction with residual gas molecules. Theoretical analyses have shown that covering an alkali antimonide photocathode with a monolayer graphene or hexagonal boron nitride protects it in a coarse vacuum environment due to the inhibition of chemical reactions with residual gas molecules. Alkali antimonide photocathodes require an ultra-high vacuum environment, and depositing a monolayer 2D material on it poses a serious challenge. In the present work, we have incorporated a novel method known as intercalation, in which alkali atoms pass through the defects of a graphene thin film to create a photocathode material underneath. Initially, Sb was deposited on a Si substrate, and a monolayer graphene was transferred on top of the Sb film. Heat cleaning around 550–600 °C effectively removed the Sb oxides, leaving metallic Sb underneath the graphene layer. Depositing Cs on top of a monolayer graphene enabled the intercalation process. Atomic force microscopy, Raman spectroscopy, x-ray photoelectron spectroscopy, low energy electron microscopy, and x-ray diffraction measurements were performed to evaluate photocathode formation underneath the monolayer graphene. Our analysis shows that Cs penetrated the graphene and reacted with Sb and formed Cs 3 Sb.

2D materials↗

DOE OSTI2024

The self-annealing of irradiation induced defects in magnetite Fe 3 O 4 : Revealing reversible irradiation-induced disorder transformation through in situ TEM

This work reports heavy ion-irradiation effects in polycrystalline Fe 3 O 4 . For this matter, Fe/Fe 3 O 4 heterostructures were irradiated in situ in a transmission electron microscopy with 1 MeV Kr ions at 50 K. Evidence of cubic to monoclinic transformation (a.k.a Verwey transition) was recorded in some magnetite grains upon cooling the sample (around 90 K); however, most of the oxide grains retain their cubic spinel structure. Irradiation effects were analyzed in the cubic phase up to a maximum dose of 38 dpa without the sign of amorphization. The extinction of first-order reflections was recorded at doses below 1 dpa, indicating the formation of a new (metastable) phase with half of the lattice parameters compared to the unirradiated Fe 3 O 4 crystal. The formation of the new crystalline phase, which also presents a high resistance to amorphization, is related to the disordering of the cation lattice and the high mobility of the cation interstitials. The metastable phase readily recovers around 225 K during the natural warming of the sample from 50 K to room temperature.

Atom irradiation effects↗

DOE OSTI2024

Discovery of Dielectric Response and Forces in Sub-Nanoscale Objects (Final Technical Report)

This is the final technical report for DOE Award DE-SC0005132 entitled “Discovery of Dielectric Response and Forces in Sub-Nanoscale Objects.” This award originated on August 15, 2010 with Principle Investigator Prof. Phil Batson of Rutgers, The State University of New Jersey. Prof. Batson transitioned to Professor Emeritus status on January 31, 2023. At that time PI status was transferred to Prof. Robert Bartynski of the Department of Physics and Astronomy at Rutgers, The State University of New Jersey, and Director of the Rutgers Laboratory for Surface Modification. The central theme of the research performed under this award is develop and refine a NION aberration-corrected Scanning Transmission Electron Microscope to attain atomic spatial resolution and sub 10meV energy resolution in electron energy loss spectroscopy (EELS) performed on the transmitted electron beam. These capabilities allow examination of the excitation properties (primarily plasmonic and vibrational [ie., phonons] of nanoscale objects when excited with a highly-localized (~ Angstrom-scale) high energy (~ 60 keV) electron beam. Direct excitations (i.e., the response to electrons impinging directly on the sample) as well as excitations in response to the dynamic electric (and magnetic!) fields of an aloof electron beam (i.e., a beam that is close to but displaced from the target) have been studied. Our experimental work has benefited greatly from close collaborations with theoretical colleagues, but at Rutgers and from around the world, providing a much more complete understanding of the observed phenomena and suggesting avenues for further study and practical applications. This report summarizes the technical and scientific achievements accomplished during the entire award period. More extensive details are available in the Progress Reports that have already been filed with the Department of Energy. The report is divided into six sections. The first four sections focus on exploring, developing and understanding several unique capabilities and phenomena discovered and accessible owing to the high spatial- and energy-resolution we have been able to achieve. The latter two sections focus on applications of the STEM’s novel capabilities to study atomic- and nanometer-scale properties of solids, as well as broader applications to advanced and bio-materials.

47 OTHER INSTRUMENTATION↗

DOE OSTI2026

Thermal Compton Scattering of Electron Beams on Blackbody Photons: A Monte Carlo Event Generator for Multi-Turn Tracking at the Electron-Ion Collider

Compton scattering of ultra-relativistic electrons on thermal (blackbody) photons is typically a subdominant process in electron storage rings, but at sufficiently high electron energy and low residual gas pressure it can become competitive with beam-gas scattering and contribute to dis tributed losses and backgrounds. We present a self-contained Monte Carlo event generator for thermal Compton scattering designed for integration into multi-turn tracking workflows. The im plementation follows H. Burkhardt’s proposal method: trial scattering angles are sampled from the Thomson differential cross section and accepted/rejected using the Klein-Nishina to Thomson ratio, yielding the correct Compton spectrum while retaining simple absolute-rate normalization. Ther mal photon energies are sampled from the blackbody photon-number spectrum via an exact mixture representation.

43 PARTICLE ACCELERATORS↗

DOE OSTI2020

Nanostructure Accelerators: Novel concept and path to its realization

TeV/m acceleration gradients using crystals as originally envisioned by R. Hofstadter, an early pioneer of HEP, have remained unrealizable. Fundamental obstacles that have hampered efforts on particle acceleration using bulk-crystals arise from collisional energy loss and emittance degradation in addition to severe beam disruption despite the favorable effect of particle channeling along interatomic planes in bulk. We aspire for the union of nanoscience with accelerator science to not only overcome these problems using nanostructured tubes to avoid direct impact of the beam on bulk ion-lattice but also to utilize the highly tunable characteristics of nanomaterials. We pioneer a novel surface wave mechanism in nanostructured materials with a strong electrostatic component which not only attains tens of TeV/m gradients but also has focusing fields. Under our initiative, the proof-of-principle demonstration of tens of TeV/m gradients and beam nanomodulation is underway. Realizable nanostructure accelerators naturally promise new horizons in HEP as well as in a wide range of areas of research that utilize beams of high-energy particles or photons.

43 PARTICLE ACCELERATORS↗

DOE OSTI2024

Effects of electron beam irradiation on CrMnV and CrMnTiV high entropy alloys: Nano-mechanical, structural, and thermodynamic perspectives

Beam exit windows are crucial components of any particle accelerator as they provide an interface between the beamline vacuum and target material at atmospheric media. For high beam power machines, special materials and designs are required to withstand high radiation and mechanical loads, while minimizing energy loss during transition and maximizing window lifetime. This research investigates the impact of electron beam exposure to bulk CrMnV and CrMnTiV high entropy alloys (HEAs) with the primary goal of identifying suitable candidate materials for the design of robust and durable exit window settings. The selection criteria include intrinsic characteristics, power dissipation, and mechanical responses. According to the thermodynamic calculations, both equiatomic CrMnV and the addition of 7% of Ti with equiatomic CrMnV yield solid-solutions phases. The structural and mechanical properties of CrMnV and CrMnTiV samples were tested using field emission scanning electron microscopy, atomic force microscopy, scanning electron microcopy with energy dispersive x-ray spectroscopy, x-ray diffraction, and nanoindentation before and after exposure to a dose of ~66 kGy from a 10 MeV e-beam accelerator. Despite exhibiting beam transmission characteristics comparable to Cr and V, the indentation hardness of HEAs exceeded that of the Cr and V samples by five to six times. The examination of the CrMnTiV irradiated samples revealed organized deformation patterns depicting new features, which we suspect twinning and twin boundaries due to the addition of Ti to CrMnV. Ti, a hexagonal-close-packed crystal structure, is commonly known for deformation twinning behavior.

36 MATERIALS SCIENCE↗

DOE OSTI2025

Quasilinear Analysis in the Source Region of Jovian Hectometric Emission Associated With Upward Electron Beams

Abstract Intense upward electron beams were measured by the Juno JADE instrument in the northern hemisphere, low‐latitude auroral zone source region. In this study we report on how these electron beams interact with plasma near and within the Jovian hectometric (HOM) emission (1 MHz 5 MHz) source region. Within the source region large upward loss cones are observed in the northern polar region at radial distances of 2Rj, magnetic latitude of . Intense, narrow electron beams ( 3 keV) are then observed, but within one second wave‐particle scattering is observed, filling the loss cone to energies 50 keV. These energies persist for several seconds before fading, leaving an empty loss cone again. The loss cone provides a free‐energy source for HOM emission resulting from the cyclotron maser instability. We use quasilinear analysis to examine the generation of HOM and the dynamics of wave‐particle interaction of the electron beams with HOM, and the generation via Landau interaction of whistler mode emission. The dynamic spectrum of the HOM emission generated by the loss‐cone electrons as well as that of the low‐frequency whistler‐mode waves generated by the up‐going electron beam can be constructed by quasilinear theory, which compare well with observation. The saturated state of the energetic electron velocity distribution function constructed via quasilinear theory also compare reasonably with observation.

Yoon, P. H. [Institute for Physical Science and Te↗

DOE OSTI2025

Electronic effects in radiation-induced collision cascades in nickel

The accurate treatment of electronic effects in multi-million-atom simulations of radiation-induced collision cascades is crucial for reliable predictions of primary radiation damage. In this work, we explore the fidelity of a recently developed two-temperature molecular dynamics model implementing an electron density-dependent coupling of electronic and atomic subsystems for cascade simulations in nickel. We show that the parameter-free model realistically captures the instantaneous energy losses during all stages of the highly nonequilibrium cascade process. Our simulations predict two distinct coupling regimes, corresponding to the rapid energy losses through electronic stopping in the early stages of the cascade and to the slow equilibration through the electron-phonon coupling mechanism in the later stages, without the use of separate models or coupling terms. The intermediate stage of the cascade dynamics displays a complex energy transfer between the subsystems, which cannot be interpreted by comparison to either electronic stopping or electron-phonon coupling theories. We therefore compare the predicted atomic mixing, which is sensitive to the energy losses during the intermediate cascade stage, with experimental ion beam mixing measurements. We find good agreement with the experiments, validating the coupling model for the intermediate stage of the cascade. Predictions of final defect numbers and cluster sizes are found in line with the results from conventional electronic stopping-based methods, while significantly reducing the theoretical uncertainty in the outcomes of conventional models stemming from arbitrary choices of thresholds for different coupling terms. Our results represent a notable improvement in cascade damage predictions in nickel, providing validation of the electron density-dependent coupling model for radiation damage simulations in general. The results lead us to propose an interpretation of the electronic energy losses in the intermediate regime of velocities, where we find an effectively nonlinear dissipation.

Crystal defects↗

DOE OSTI2020

Beam impedance and heating analysis of the diagnostic stripline

In this work the heat transfer analysis has been performed for the stripline kicker, design of which is used at many accelerator facilities as a part of the transverse bunch-by-bunch feed-back system, including NSLS-II. The experimental data of the electrode temperature have been collected from a special diagnostic stripline designed with six infrared view ports. The temperature analysis is based on the power loss calculations and the loss factor computed by the 3-D electromagnetic simulation code GdfidL. To estimate the power loss, we analyze the real part of the longitudinal impedance and the loss factor for two different regimes. We use the ANSYS finite element code to correlate the temperature with the power loss. Lambertson and Shafer formalisms of the longitudinal and transverse beam impedances are discussed for the simplified stripline geometries. The required characteristic impedances and the geometric factors are determined analytically for the simplified geometries and compared with the results for the designed stripline geometry using the 2-D POISSON code by solving the Laplace’s equation in two dimensions. Lambertson’s equations are compared with numerical results. We introduce the frequency range, within which we can apply the analytical approach.

43 PARTICLE ACCELERATORS↗

DOE OSTI2024

Determination of the mean energy of fast electron losses and anisotropies through thick-target emission on WEST

Abstract A new method to obtain the mean energy of fast electron losses in fusion plasmas using a versatile multi-energy hard x-ray (HXR) detector is presented. The method is based on measuring the thick-target emission of tungsten in the divertor region produced by fast electron losses interacting with the target and modeling the tungsten spectra by a Monte Carlo code which simulates the interaction between a beam of electrons and a solid target. The mean energy of the fast electron losses is determined through the comparison between the experimental and synthetic emission. The results show that fast electron losses during lower hybrid current drive discharges at WEST have a mean energy of 90–140 keV and represent only 2% of the total heat flux at the target. Additionally, anisotropic HXR emission has been detected for the first time at the WEST core and edge plasma, with opposite directions. It is due to the forward-peak emission of two distinctive populations of fast electrons: co-current fast electrons in the core and counter-current fast electron losses at the inner strike point. In view of future experiments like ITER where electron cyclotron current drive will generate a fast electron population, this technique could serve as a real-time monitor of fast electron losses and eventually feed an actuator on the current drive generation.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2024

Full-Cycle Simulations of the Fermilab Booster

The Proton Improvement Plan phase II (PIP-II) project currently under construction at FNAL will replace the existing 400 MeV normal conducting linac with a new 800 MeV superconducting linac. The beam power in the downstream rapid-cycling Booster synchrotron will be doubled by raising the machine cycle frequency from 15 to 20 Hz and by increasing the injected beam intensity by a factor 1.5. This has to be accomplished without raising uncontrolled losses beyond the administrative limit of 500 W. In addition, slip-stacking efficiency in the Recycler, the next machine in the accelerator chain, sets an upper limit on the longitudinal emittance of the beam delivered by the Booster. As part of an effort to better understand potential losses and emittance blow-up in the Booster, we have been conducting full cycle 6D simulations using the code PyORBIT. The simulations include space charge, wall impedance effects and transition crossing. In this paper, we discuss our experience with the code and present representative results for possible operational scenarios.

43 PARTICLE ACCELERATORS↗

DOE OSTI2024

Full Cycle Simulations of The Fermilab Booster

43 PARTICLE ACCELERATORS↗

DOE OSTI2022

Specular reflections (“glint”) of the inner beams in a gas-filled cylindrical hohlraum

Herein we report on the experimental measurement of specular reflection (“glint”) of laser beams off the hohlraum wall in inertial confinement fusion experiments at the National Ignition Facility. In a hohlraum, glinted light can escape the opposite laser entrance hole of the hohlraum and is a potential laser energy loss mechanism. The total measured glint on the inner cones of beams is measured to be less than 8 TW (when using the full National Ignition Facility laser), which is <2% of incident peak power. The simulated x-ray flux exceeds the measurement by 10%–20%, and glinted laser light is unable to account for this discrepancy. Similar inner beam glint was measured for ρ = 0.3 and 0.6 mg/cc gas fill hohlraums, but no glint was detected for 1.2 mg/cc densities. Inner beam glint is dominated by the lowest angle 21.5 beams within a 23.5 quad, and it is at most 30% sensitive to different quad polarization arrangements.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2025

Multi-Gigawatt Electric Highway

Ultra-Compact Electrical Transmission Lines are a new transmission line technology that uses large, hollow, aluminum beams to carry current instead of thin wires. Capacity is 4.5 times higher, power losses are 3 times lower, and cost per mile is a little lower than conventional lines. Resilience and reliability are higher. The beams are enclosed within concrete walls and out of the weather, protected from high winds, ice storms, fires, and lightning. The 230 kV version is 9 feet high x 11 feet wide and can use existing rights of way next to existing transmission lines or highways. With a little landscaping, these transmission lines are not an eyesore and will be much easier to permit on existing rights of way.

24 POWER TRANSMISSION AND DISTRIBUTION↗

DOE OSTI2024

Space charge dominated momentum spread and compensation strategies in the post-linac section of Proton Improvement Plan-II at Fermilab

The upcoming Proton Improvement Plan-II (PIP-II), designated for enhancements to the Fermilab accelerator complex, features a new 800 MeV superconducting linac and a Beam Transfer Line (BTL) to transport the beam to the existing Booster synchrotron. To mitigate the space charge tune shift associated with a high intensity accumulated beam, the low emittance linac beam is used to paint the ring phase space both transversely and longitudinally. To prevent losses caused by particles injected outside the rf separatrix while painting longitudinal phase space, the momentum spread of the incoming beam should not exceed 2.1 x 10^-4. Detailed simulations showed that due to space charge, the rms momentum spread increases to 4 x 10^-4 while it is transported in the BTL --about twice the allowable limit. In this paper, we outline a mitigation strategy involving a debuncher cavity. We discuss location, operating frequency, and gap voltage under both nominal and perturbed beam conditions, specifically accounting for momentum jitter. The impact of cavity misalignments is also assessed. The paper concludes by recommending an optimized configuration.

43 PARTICLE ACCELERATORS↗

DOE OSTI2020

Effect of mass flow rate on gas propagation after vacuum break in a liquid helium cooled tube

Vacuum break in particle accelerators is a major concern due to risks associated with personnel and extensive equipment damage. Continuing research in our lab focuses on the sudden loss of vacuum in the liquid helium cooled beam-line tubes of superconducting particle accelerators. In our previous research, we studied nitrogen gas propagation in a uniform tube system immersed in both normal helium (He I) and superfluid helium (He II). It was observed that He II has a stronger effect in slowing down the gas propagation compared to He I, but this effect was largely due to the variation of the point where condensation and deposition of the nitrogen gas on the tube inner wall. Here, we discuss our modifications to the tube system that now allow us to accurately control the starting location of gas condensation in both the He I and He II experiments. Systematic studies of gas propagation were conducted using this new tube system by varying the nitrogen mass flow rate at the tube inlet.

43 PARTICLE ACCELERATORS↗

DOE OSTI2022

Model/Measurement Comparison of the Transverse Phase Space Distribution of an RFQ-Generated Bunch at the SNS BTF

The research program at the SNS Beam Test Facility is focused on resolving observed model/measurement discrepancies that preclude accurate loss prediction in high-power linacs. The current program of study is focused on deploying direct 6D measurements to reconstruct a realistic model of the initial beam distribution at the RFQ output. This detailed characterization also provides an opportunity for benchmark of RFQ simulations. Here we compare PARMTEQ predictions against 5D-resolved (x, x’, y, y’, dE) phase space measurements of the BTF H⁻ bunch, focusing on the transverse distribution. This work is an extension of [1], which focused on the longitudinal phase space.

Ruisard, Kiersten↗