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At least 271 records · Page 15

Impacts of secondary ice production on Arctic mixed-phase clouds based on ARM observations and CAM6 single-column model simulations

For decades, measured ice crystal number concentrations have been found to be orders of magnitude higher than measured ice-nucleating particle number concentrations in moderately cold clouds. This observed discrepancy reveals the existence of secondary ice production (SIP) in addition to the primary ice nucleation. However, the importance of SIP relative to primary ice nucleation remains highly unclear. Furthermore, most weather and climate models do not represent SIP processes well, leading to large biases in simulated cloud properties. This study demonstrates a first attempt to represent different SIP mechanisms (frozen raindrop shattering, ice–ice collisional breakup, and rime splintering) in a global climate model (GCM). The model is run in the single column mode to facilitate comparisons with the Department of Energy (DOE)'s Atmospheric Radiation Measurement (ARM) Mixed-Phase Arctic Cloud Experiment (M-PACE) observations. We show the important role of SIP in four types of clouds during M-PACE (i.e., multilayer, single-layer stratus, transition, and frontal clouds), with the maximum enhancement in ice crystal number concentrations up to 4 orders of magnitude in moderately supercooled clouds. We reveal that SIP is the dominant source of ice crystals near the cloud base for the long-lived Arctic single-layer mixed-phase clouds. The model with SIP improves the occurrence and phase partitioning of the mixed-phase clouds, reverses the vertical distribution pattern of ice number concentrations, and provides a better agreement with observations. The findings of this study highlight the importance of considering SIP in GCMs.

54 ENVIRONMENTAL SCIENCES↗

Influence of open ocean biogeochemistry on aerosol and clouds: Recent findings and perspectives

Aerosols and clouds are key components of the marine atmosphere, impacting the Earth’s radiative budget with a net cooling effect over the industrial era that counterbalances greenhouse gas warming, yet with an uncertain amplitude. Here we report recent advances in our understanding of how open ocean aerosol sources are modulated by ocean biogeochemistry and how they, in turn, shape cloud coverage and properties. We organize these findings in successive steps from ocean biogeochemical processes to particle formation by nucleation and sea spray emissions, further particle growth by condensation of gases, the potential to act as cloud condensation nuclei or ice nucleating particles, and finally, their effects on cloud formation, optical properties, and life cycle. We discuss how these processes may be impacted in a warming climate and the potential for ocean biogeochemistry—climate feedbacks through aerosols and clouds.

54 ENVIRONMENTAL SCIENCES↗

A Solar Radiation Parameterization for Atmospheric Studies

The solar radiation parameterization (CLIRAD-SW) developed at the Goddard Climate and Radiation Branch for application to atmospheric models are described. It includes the absorption by water vapor, O3, O2, CO2, clouds, and aerosols and the scattering by clouds, aerosols, and gases. Depending upon the nature of absorption, different approaches are applied to different absorbers. In the ultraviolet and visible regions, the spectrum is divided into 8 bands, and single O3 absorption coefficient and Rayleigh scattering coefficient are used for each band. In the infrared, the spectrum is divided into 3 bands, and the k-distribution method is applied for water vapor absorption. The flux reduction due to O2 is derived from a simple function, while the flux reduction due to CO2 is derived from precomputed tables. Cloud single-scattering properties are parameterized, separately for liquid drops and ice, as functions of water amount and effective particle size. A maximum-random approximation is adopted for the overlapping of clouds at different heights. Fluxes are computed using the Delta-Eddington approximation.

Chou, Ming-Dah↗

Role of small ice crystals in radiative properties of cirrus: A case study, FIRE II, November 22, 1991

Aircraft observations of cirrus cloud were made near Coffeyville, Kansas, during November 1991 as part of the First ISCCP Regional Experiment II (FIRE II) project. Cloud ice particle spectra measurements were made using both a particle measuring system (PMS) 2DC probe and an ice particle replicator. Particles larger than 200 micrometers were column rosettes. The replicator shows the presence of large numbers of ice crystals smaller than 66 micrometers (two PMS size bins) that are not recorded by the PMS 2DC probe. Calculations based on the replicator data of the geometrical blocked area and absorption cross section of the cloud per unit volume show that small particles can contribute significantly to and sometimes dominate both the solar extinction and the infrared emission. Intercomparison is made of the ice particle size, area, and mass distributions determined by these different instruments. Power law relationships for area occluded by a crystal as a function of crystal maximum dimension were computed from the PMS 2DC data. The wavelength-dependent infrared absorption cross section per volume was computed using a simple model based on anomalous diffraction and area and mass dimensional relationships for the ice crystals.

Arnott, W. Patrick↗

Cirrus microphysics and radiative transfer: Cloud field study on October 28, 1986

The radiative properties of cirrus clouds present one of the unresolved problems in weather and climate research. Uncertainties in ice particle amount and size and, also, the general inability to model the single scattering properties of their usually complex particle shapes, prevent accurate model predictions. For an improved understanding of cirrus radiative effects, field experiments, as those of the Cirrus IFO of FIRE, are necessary. Simultaneous measurements of radiative fluxes and cirrus microphysics at multiple cirrus cloud altitudes allows the pitting of calculated versus measured vertical flux profiles; with the potential to judge current cirrus cloud modeling. Most of the problems in this study are linked to the inhomogeneity of the cloud field. Thus, only studies on more homogeneous cirrus cloud cases promises a possibility to improve current cirrus parameterizations. Still, the current inability to detect small ice particles will remain as a considerable handicap.

Kinne, Stefan↗

KAZR Hydrometeor and Insect Masks

The Ka-band ARM zenith pointing radar (aka, KAZR) is so sensitive that it detects cloud particles and individual insects. While detecting insects with Ka-band radar is beneficial and desirable to advance radar entomology, this sensitivity can be detrimental to radar meteorology because insects could be interpreted as clouds or precipitation. For example, misclassifying insects as clouds has been a problem for the ARM Active Remote Sensing of Clouds (ARSCL) Value Added Product since its inception (Clothiaux et al. 2000). Based on cloud particle and insect radar scattering properties, an algorithm was developed that identifies clouds, raindrops, ice particles, and insects in KAZR co- and cross-polarimeteric Doppler velocity spectra. The algorithm produces affirmative masks in the KAZR native time and height resolution indicating time-height locations of hydrometeors and insects. The hydrometeor mask contains binary information (e.g., yes/no hydrometeor presence), and the insect mask includes a proxy for insect activity that increases when more insects are detected in the Doppler velocity spectra. The algorithm was developed using KAZR medium sensitivity mode (MD) observations and was applied to two summer seasons of KAZR observations at the Southern Great Plains (SGP) Central Facility: May-October 2018 and 2019. In the future, this data set will be expanded to include other KAZR operating modes and observations from other ARM field sites. Details of the algorithm and data set can be found in: Williams, C.R., K.L. Johnson, S.E. Giangrande, J. C. Hardin, R. Oktem, and D. M. Romps, 2021: Identifying Insects, Clouds, and Precipitation using Vertically Pointing Polarimetric Radar Doppler Velocity Spectra. Atmospheric Measurement Techniques, submitted 6-Feb-2021. https://amt.copernicus.org/preprints/amt-2021-27/#discussion.For more information on the ARSCL VAP, see Clothiaux, E. E., T. P. Ackerman, G. G. Mace, K. P. Moran, R. T. Marchand, M. A. Miller, and B. E. Martner, 2000; J. Appl. Meteor., 39, 645-665.

54 ENVIRONMENTAL SCIENCES↗

A new look at dust and clouds in the Mars atmosphere - Analysis of emission-phase-function sequences from global Viking IRTM observations

The present analysis of emission-phase function (EPF) observations from the IR thermal mapper aboard the Viking Orbiter encompasses polar latitudes, and Viking Lander sites, and spans a wide range of solar longitudes. A multiple scattering radiative transfer model which incorporates a bidirectional phase function for the surface and atmospheric scattering by dust and clouds yields surface albedos and dust and ice optical properties and optical depths for the variety of Mars conditions. It is possible to fit all analyzed EPF sequences corresponding to dust scattering with an albedo of 0.92, rather than the 0.86 given by Pollack et al. on the bases of Viking Lander observations.

Clancy, R. T.↗

Tropical and Arctic Cloud Observations From CALIPSO Between 2008-2014 and its Implications

There has been studies (e.g., Schweiger, 2004) suggest significant increase of Arctic clouds during the last three decades, especially in the western Arctic region. Such studies are based on passive remote sensing that are not highly reliable due to the lack of contrasts in temperature and reflectance between clouds and snow/ice surfaces. Changes in the Arctic clouds can be evaluated more accurately using the space-based lidar measurements from CALIPSO during the last nine years since CALIPSO can provide much more accurate detection and classification of both water and ice clouds in the Arctic. Time series of Arctic cloud properties (e.g., cloud fraction, cloud thermodynamic phase, water cloud depolarization ratio and droplet number concentration) from CALIPSO data are analyzed in this study. This study reveals the changes in both cloud fraction and cloud microphysical properties during the last nine years when CALIPSO data are available. We will evaluate the changes in Arctic cloud fraction and cloud microphysical properties, their seasonal and spatial characteristics and the potential impact on the energy budget and the climate of the Arctic.

Hu, Yongxiang↗

Water-ice Clouds on Mars: Location and Seasonal Variation

Water-ice clouds were located on Mars using Viking infrared thermal mapper (IRTM) broadband spectral observations. The IRTM instrument had 5 thermal bands centered at 7, 9, 11, 15, and 20 microns. Clouds and hazes were consistently observed in four northern hemisphere regions centered over Tharsis, Arabia, Elysium, and along the boundary between the crater uplands and the northern plains. During the northern spring and summer when the atmosphere is relatively free of dust, there is a distinct difference between the cloud abundance in the Northern and Southern Hemispheres, with clouds and hazes being rare in the south. A second important class of water-ice clouds are those observed along the boundary of the retreating north polar cap. These clouds occur at all longitudes around the cap and are generally confined to within +/- 5 deg of the cap boundary. The cloud opacities can be estimated using a delta-Eddington radiative transfer model which incorporates Mie scattering and the electrical properties of water-ice. Assuming realistic, but non-unique, values for the ice particle size and cloud temperature, the derived opacities range from near-zero to 1.

Christensen, P. R.↗

Effective Radius of Ice Cloud Particle Populations Derived from Aircraft Probes

The effective radius(r(sub e)) is a crucial variable in representing the radiative properties of cloud layers in general circulation models. This parameter is proportional to the condensed water content (CWC) divided by the extinction (sigma). For ice cloud layers, parameterizations for r(sub e), have been developed from aircraft in-situ measurements 1) indirectly, using data obtained from particle spectrometer probes and assumptions or observations about particle shape and mass to get the ice water content (IWC) and area to get sigma, and recently 2) from probes that measure IWC and sigma directly. This study compares [IWC/sigma] derived from the two methods using data sets acquired from comparable instruments on two aircraft, one sampling clouds at mid-levels and the other at upper-levels during the CRYSTAL-FACE field program in Florida in 2002. The sigma and IWC derived by each method are compared and evaluated in different ways for each aircraft data set. Direct measurements of sigma exceed those derived indirectly by a factor of two to two and a half. The IWC probes, relying on ice sublimation, appear to measure accurately except when the IWC is high or the particles too large to sublimate completely during the short transit time through the probe. The IWC estimated from the particle probes are accurate when direct measurements are available to provide constraints and useful information in high IWC/large particle situations. Because of the discrepancy in sigma estimates between the direct and indirect approaches, there is a factor of 2 to 3 difference in [IWC/sigma] between them. Although there are significant uncertainties involved in its use, comparisons with several independent data sources suggest that the indirect method is the more accurate of the two approaches. However, experiments are needed to resolve the source of the discrepancy in sigma.

Heymsfield, Andrew J.↗

Dynamical States of Low Temperature Cirrus

Low ice crystal concentration and sustained in-cloud supersaturation, commonly found in cloud observations at low temperature, challenge our understanding of cirrus formation. Heterogeneous freezing from effloresced ammonium sulfate, glassy aerosol, dust and black carbon are proposed to cause these phenomena; this requires low updrafts for cirrus characteristics to agree with observations and is at odds with the gravity wave spectrum in the upper troposphere. Background temperature fluctuations however can establish a dynamical equilibrium between ice production and sedimentation loss (as opposed to ice crystal formation during the first stages of cloud evolution and subsequent slow cloud decay) that explains low temperature cirrus properties. This newly-discovered state is favored at low temperatures and does not require heterogeneous nucleation to occur (the presence of ice nuclei can however facilitate its onset). Our understanding of cirrus clouds and their role in anthropogenic climate change is reshaped, as the type of dynamical forcing will set these clouds in one of two preferred microphysical regimes with very different susceptibility to aerosol.

Barahona, D.↗

A Network of Surface Pressure Observations to Constrain Aerosol Forcing in Mars Climate Models

The evolving distribution of radiatively active dust and water ice clouds plays a major role in modulating the seasonal and interannual variation in the thermal forcing of the Martian atmosphere. Thermal tides are the global-scale atmospheric response to the diurnally varying thermal forcing due to aerosol heating within the atmosphere and radiative and convective heat transfer from the surface. The tide includes westward propagating (sun-synchronous) waves driven in response to solar heating, as well as nonmigrating waves that result from zonal variations in the thermotidal forcing caused by variations in topography and surface thermal properties and in the distribution of aerosols (dust and water ice clouds).

R. J. Wilson↗

Characterizing Ice Nucleating Particles Over the Southern Ocean Using Simultaneous Aircraft and Ship Observations

Abstract Supercooled liquid clouds are ubiquitous over the Southern Ocean (SO), even to temperatures below −20°C, and comprise a large fraction of the marine boundary layer (MBL) clouds. Earth system models and reanalysis products have struggled to reproduce the observed cloud phase distribution and occurrence of cloud ice in the region. Recent simulations found the microphysical representation of ice nucleation and growth has a large impact on these properties, however, measurements of SO ice nucleating particles (INPs) to validate simulations are sparse. This study presents measurements of INPs from simultaneous aircraft and ship campaigns conducted over the SO in austral summer 2018, which include the first in situ observations in and above cloud in the region. Our results confirm recent observations that INP concentrations are uniformly lower than measurements made in the late 1960s. While INP concentrations below and above cloud are similar, higher ice nucleation efficiency above cloud supports model simulations that the dominant INP composition varies with height. Model parameterizations based solely on aerosol properties capture the mean relationship between INP concentration and temperature but not the observed variability, which is likely related to the only modest correlations observed between INPs and environmental or aerosol metrics. Including wind speed in addition to activation temperature in a marine INP parameterization reduces bias but does not explain the large range of observed INP concentrations. Direct and indirect inference of marine INP size suggests MBL INPs, at least during Austral summer, are dominated by particles with diameters smaller than 500 nm.

Meteorology & Atmospheric Sciences↗

Atmospheric System Research Workshop Report: New Directions in Atmospheric Ice Processes Research

Atmospheric ice processes are critical for precipitation production, cloud dynamics, and radiative properties and contribute to uncertainties in Earth’s energy budget and hydrological cycle, yet they remain poorly understood. To address this, ASR convened a 2.5-day workshop with 28 experts in laboratory measurements, field observations, and cloud modeling. The primary goal was to identify key knowledge gaps and prioritize future directions in atmospheric ice processes research. The outcomes of this workshop are expected to inform ASR and prompt improvements in cloud and Earth system models (ESMs) by advancing the fundamental understanding of ice processes.

54 ENVIRONMENTAL SCIENCES↗

SWIRP: Compact Submm-Wave and LWIR Polarimeters for Cirrus Ice Properties

Providing critical information on the make-up and distribution of aerosols and clouds, which in turn improve predictions of future climate conditions and help us assess the impacts of aerosols on human health;Addressing key questions about how changing cloud cover and precipitation will affect climate, weather, and Earth's energy balance in the future, advancing understanding of the movement of air and energy in the atmosphere and its impact on weather, precipitation, and severe storms;

Wu, Dong L.↗

A Model for Ice Accretion Roughness Evolution and Spatial Variations

Over the past decade, multiple investigations of ice accretion roughness and spatial variations have been performed in the Icing Research Tunnel (IRT) at the NASA Glenn Research Center. The early investigations used models of NACA 0012 airfoils with different chord sizes and focused on temporal scaling and primary cloud scaling parameters such as stagnation point collection efficiency. Subsequent investigations included the effects of model sweep, airfoil shape, airfoil lifting condition, and freestream static temperature. To develop a predictive model for roughness evolution in generalized icing situations, the maximum roughness values for the airfoils and conditions used in the angle of attack and freestream temperature investigations were scaled to eliminate the temporal variations. LEWICE simulations were employed to identify the local collection efficiency at the locations of maximum roughness, and a two-dimensional panel-method code was used to identify the local static pressure at the location of the maximum roughness. Because of the stochastic nature of ice accretion roughness, a physics-directed approach was employed to develop a multi-dimensional correlation based on the local pressure coefficient, the local total temperature, the cloud properties, and the cloud exposure time. The resulting correlation predictions are compared to ice shapes measured in the IRT for both a 21-in. NACA 0012 airfoil model and a 60-in. HAARP-II model. The resulting predictions indicate that the local freezing fraction must be included in the roughness predictive model. Implications regarding icing heat transfer predictions using the resulting roughness model are also discussed.

Icing↗

Physicochemical characterization and source apportionment of Arctic ice-nucleating particles observed in Ny-Ålesund in autumn 2019

Abstract. Ice-nucleating particles (INPs) initiate primary ice formation in Arctic mixed-phase clouds (MPCs), altering cloud radiative properties and modulating precipitation. For atmospheric INPs, the complexity of their spatiotemporal variations, heterogeneous sources, and evolution via intricate atmospheric interactions challenge the understanding of their impact on microphysical processes in Arctic MPCs and induce an uncertain representation in climate models. In this work, we performed a comprehensive analysis of atmospheric aerosols at the Arctic coastal site in Ny-Ålesund (Svalbard, Norway) from October to November 2019, including their ice nucleation ability, physicochemical properties, and potential sources. Overall, INP concentrations (NINP) during the observation season were approximately up to 3 orders of magnitude lower compared to the global average, with several samples showing degradation of NINP after heat treatment, implying the presence of proteinaceous INPs. Particle fluorescence was substantially associated with INP concentrations at warmer ice nucleation temperatures, indicating that in the far-reaching Arctic, aerosols of biogenic origin throughout the snow- and ice-free season may serve as important INP sources. In addition, case studies revealed the links between elevated NINP and heat lability, fluorescence, high wind speeds originating from the ocean, augmented concentration of coarse-mode particles, and abundant organics. Backward trajectory analysis demonstrated a potential connection between high-latitude dust sources and high INP concentrations, while prolonged air mass history over the ice pack was identified for most scant INP cases. The combination of the above analyses demonstrates that the abundance, physicochemical properties, and potential sources of INPs in the Arctic are highly variable despite its remote location.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗