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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 271 records · Page 15
All sourcesNASA NTRSDOE OSTI
DOE OSTI2026

One Earth Energy CO 2 Capture Facility FEED Study and Class 4 Cost Estimate

The One Earth Energy (OEE) plant in Gibson City, Illinois produces ethanol through a corn fermentation process. For this project, the maximum possible ethanol production rate for this facility is 160 million gallons per year (MMgal/yr) based on discussions with plant personnel regarding recent annual production rates and any foreseeable plans or possibilities to increase ethanol production at this facility. Yeast ferments the corn mash to produce ethanol and produces carbon dioxide (CO 2 ) as a by-product at the same time. The CO 2 bubbles out of the mash and flows through a packed bed water scrubber to remove volatile organic compounds before the gas vents to atmosphere. CO 2 will be captured after it has passed through the existing scrubber.

09 BIOMASS FUELS↗
DOE OSTI2024

Probabilistic and maximum entropy modeling of chemical reaction systems: Characteristics and comparisons to mass action kinetic models

We demonstrate and characterize a first-principles approach to modeling the mass action dynamics of metabolism. Starting from a basic definition of entropy expressed as a multinomial probability density using Boltzmann probabilities with standard chemical potentials, we derive and compare the free energy dissipation and the entropy production rates. We express the relation between entropy production and the chemical master equation for modeling metabolism, which unifies chemical kinetics and chemical thermodynamics. Because prediction uncertainty with respect to parameter variability is frequently a concern with mass action models utilizing rate constants, we compare and contrast the maximum entropy model, which has its own set of rate parameters, to a population of standard mass action models in which the rate constants are randomly chosen. We show that a maximum entropy model is characterized by a high probability of free energy dissipation rate and likewise entropy production rate, relative to other models. We then characterize the variability of the maximum entropy model predictions with respect to uncertainties in parameters (standard free energies of formation) and with respect to ionic strengths typically found in a cell.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

Measurement of the branching ratio of 16 N , 15 C , 12 B , and 13 B isotopes through the nuclear muon capture reaction in the Super-Kamiokande detector

The Super-Kamiokande detector has measured solar neutrinos for more than 25 years. The sensitivity for solar neutrino measurement is limited by the uncertainties of energy scale and background modeling. Decays of unstable isotopes with relatively long half-lives through nuclear muon capture, such as 16 N, 15 C, 12 B, and 13 B, are detected as background events for solar neutrino observations. Here, in this study, we developed a method to form a pair of stopping muon and decay candidate events and evaluated the production rates of such unstable isotopes. We then measured their branching ratios considering both their production rates and the estimated number of nuclear muon capture processes as Br⁡( 16 N) = (9.0 ± 0.1)%, Br⁡( 15 C) = (0.6 ± 0.1)%, Br⁡( 12 B) = (0.98 ± 0.18)%, Br⁡( 13 B) = (0.14 ± 0.12)%, respectively. The result for 16 N has world-leading precision at present and the results for 15 C, 12 B, and 13 B are the first branching ratio measurements for those isotopes.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRS1980

Silver isotopic anomalies in iron meteorites - Cosmic-ray production and other possible sources

Sources of excess Ag-107 observed in iron meteorites are investigated with emphasis on reactions of cosmic-ray particles with palladium. Cross sections for the production of the silver isotopes from palladium by energetic cosmic-ray particles are estimated to calculate spallogenic production rates relative to that of Mn-53 from iron. The upper limits for the production rates of Ag-107 and Ag-109 by energetic galactic cosmic-ray particles are 690 and 270 atoms/min/kg(Pd), respectively, and the maximum rate for making excess Ag-107 by spallation reactions is 400 atoms/min/kg(Pd). The excess Ag-107 cannot be produced by a long exposure to cosmic-ray particles, and because it is harder to make the amount of Pd-107 observed in the iron meteorites by an early intense proton irradiation than it is to make the Al-26 observed in other meteorites, it is concluded that the excess Ag-107 is due to the decay of nucleosynthetic Pd-107 in the iron meteorites.

Reedy, R. C.↗
NASA NTRS1984

Thermal modeling of Halley's Comet

The comet thermal model of Weissman and Kieffer is used to calculate gas production rates and other parameters for the 1986 perihelion passages of Halley's Comet. Gas production estimates are very close to revised pre-perihelion estimates by Newburn based on 1910 observations of Halley; the increase in observed gas production post-perihelion may be explained by a variety of factors. The energy contribution from multiply scattered sunlight and thermal emission by coma dust increases the total energy reaching the Halley nucleus at perihelion by a factor of 2.4. The high obliquity of the Halley nucleus found by Sekanina and Larson may help to explain the asymmetry in Halley's gas production rates around perihelion.

Weissman, P. R.↗
DOE OSTI2021

Microwave-enhanced catalytic ammonia synthesis under moderate pressure and temperature

In this study, an alternative approach based on microwave-enhanced ammonia synthesis for Haber-Bosch process was carried out under moderate pressure of 0.1–0.65 MPa and temperature range of 280–400 °C over a stable CsRu/CeO 2 catalyst. The ammonia production rate is significantly improved under microwave conditions. At 0.65 MPa and 320 °C, maximum ammonia production rate was achieved at H 2 /N 2 ratio of 1/1. Stable performance was obtained in a 6-cycles of startup-shutdown operation for cumulative on-line time of 80 h. The work demonstrates the potential of microwave catalytic technology for the distributed ammonia synthesis using renewable power having intermittent nature of energy supply.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1986

Spectrophotometric observations of Comet Halley

Comet Halley was observed using an intensified dissector scanner spectrograph on the 2.7 m telescope at McDonald Observatory from Dec. 1984 through June 1986. Molecular emissions were first detected in February 1985 when CN was observed. Spatial maps probing different regions of the coma were made starting in November 1985. Haser model production rates were computed for each night's data. The brightness of Halley, and therefore the production rates, are variable on timescales of a day, with variations of a magnitude or more in this time period. Nonequilibrium chemical models were calculated using Giotto and Vega data as constraints and inputs. The variability of Halley cannot be explained solely by water sublimation, nor do the variations show the 52 to 53 hr period of rotation.

Cochran, A. L.↗
NASA NTRS1979

Reaction rate and products for the reaction O/3P/ + H2CO

A study of reaction kinetics of O + H2CO in a discharge-flow system using mass spectrometric detection of reactants and products is presented. It was performed under both oxygen-atom-rich and formaldehyde-rich conditions over the 296 to 437 K range, showing that the global bimolecular rate constant is in agreement with other studies. This study differs from others in that the reaction products can be observed, and a substantial yield of a primary reaction product was measured with a mass spectral peak at m/e=44. This suggests that the global reaction rate probably consists of combination, as well as of simple abstraction. For the combination, one hypothesis is that triplet dioxymethylene is formed which polymerizes to triplet formic acid; the vibrationally excited triplet formic acid may decompose to form several sets of products, including HCO + OH and HCO2 + H.

Chang, J. S.↗
NASA NTRS1980

Determination of the thermal rate coefficient, products, and branching ratios for the reaction of O/+/ /D-2/ with N2

Atmosphere Explorer-C satellite measurements are used to determine rate coefficients (RCs) for the following reactions: O(+)(D-2) + N2 yields N2(+) + O (reaction 1), O(+)(D-2) + N2 yields O(+)(S-4) + N2 (reaction 2), and O(+)(D-2) + N2 yields NO(+) + N (reaction 3). Results show the RC for reaction 1 to be 1 (plus 1 or minus 0.5) x 10 to the -10th cu cm per sec, for reaction 2 to be 3 (plus 1 or minus 2) x 10 to the -11th cu cm per sec, and 3 to be less than 5.5 x 10 to the -11th cu cm per sec. It is also found that the reaction of O(+)(D-2) with N2 does not constitute a detectable source of NO(+) ions in the thermosphere.

Torr, D. G.↗
NASA NTRS1973

Neutral-pion-decay gamma rays from the galaxy and the interstellar gas content

Knowledge of the total gamma ray production rate per H atom from the decay of pion(0) produced in interstellar cosmic ray interactions is essential for determining the possible amount of interstellar H2. This production rate is recalculated using the latest accelerator data on pion(0) production in pp interactions up to approximately 300 GeV. A simple but accurate approximation resolves the past disagreement over the magnitude of this rate. An upper limit is obtained of (1.51 + or - 0.23) x 10 to the minus 25th power/sec. consistent with the observed upper limit of 1.6 x 10 to the minus 25th power/sec.

Stecker, F. W.↗
NASA NTRS2011

Possible Increase in Nitric Oxide Production by Lightning Discharges Due to Catalytic Effects of Ice Particles

We address the question of whether ice crystals with habits typically encountered by lightning discharges may serve as catalysts for the production of NOx by lightning. If so, and if the effect is sufficiently large, it would need to be taken into account in estimates of global NOx production by lightning. In this study, we make a series of plausible assumptions about the temperatures and concentrations of reactant species in the environment of discharges and we postulate a mechanism by which ice crystals could adsorb nitrogen atoms. We then compare production rates between uncatalyzed and catalyzed reactions at 2000 K, 3000 K, and 4000 K, temperatures observed in lightning channels during the cool-down period after a return stroke. Catalyzed NO production rates are greater at 2000 K, whereas uncatalyzed production occurs most rapidly at 4000 K. The channel temperature stays around 2000 K for a longer period of time than at 4000 K. The longer residence time at 2000 K is sufficient to allow fresh reactants to participate in the mix in. Therefore, our results suggest that nearly three times as much NO per flash is produced by ice-catalyzed reactions as compared with uncatalyzed reactions.

Peterson, Harold↗
DOE OSTI2021

Numerical simulation of gas production from natural gas hydrate deposits with multi-branch wells: Influence of reservoir properties

Vast amounts of natural gas hydrate are buried in subseafloor sediments without impermeable boundaries, which is recognized as an essential energy source for the future. Previously, the multi-branch well was proposed to enhance the recovery efficiency of natural gas hydrate, and the gas production rate has been dramatically improved comparing with the vertical well. However, the multi-branch well shows a terrible performance in gas production duration. Here, as a continuation of the previous study, numerical simulations were conducted to investigate the influence of hydrate reservoir properties on the gas production potential. Results indicate that it is hard to extract hydrate commercially for hydrate accumulations without impermeable boundaries. A high initial hydrate saturation leads to a long gas production duration but a low gas production rate. An increase in the intrinsic permeability of isotropic reservoirs would shorten the gas production duration and result in a low gas recovery ratio. Permeability anisotropy shows a noticeable effect on enhancing the gas recovery ratio and the gas production duration due to the improved pressure propagation pattern. Therefore, in the upcoming field tests, reservoir reconstructions that enhance permeability anisotropy are strongly suggested to obtain better outcomes.

03 NATURAL GAS↗
NASA NTRS1987

Radio OH observations of P/Halley with the NRAO 43-m telescope

Results of the radio OH emission from Comet Halley obtained with the 43-m NRAO telescope over the period from July 1985 to May 1986 show the global properties to be close to those predicted by Schloerb and Gerard (1985). The OH production rates are found to be well correlated with heliocentric magnitude estimates and to roughly follow the production rates determined from UV OH observations. After correction for the Greenstein effect, the mean velocities suggest that there is anisotropic outgassing of the parent molecule. An increase in the linewidths of the OH emission near and after perihelion is also noted.

Claussen, M. J.↗
NASA NTRS1991

Infrared spectroscopy of cometary parent molecules

The wealth of information on cometary physics provided by high-resolution spectroscopy of the IR water transitions is discussed. Specifically, the absolute line intensities and spatial brightness profiles are used to determine water production rates and lifetimes; the relative line intensities and spatial brightness profiles are used to determine water production rates and lifetimes; the relative line intensities probe the kinetic temperature profile in the coma; the line widths and line positions shed light on the coma outflow dynamics; and the temporal variability in the lines provides information on the structure of the nucleus. These observations also make it possible to determine the water ortho-to-para ratio, which may elucidate the origin and/or evolution of cometary nuclei. Recent advances in IR instrumentation promise to extend sensitivities for parent molecule searches to relative abundances well below 1 percent, especially if cooled, earth-orbiting facilities are available.

Weaver, H. A.↗
NASA NTRS1995

Analysis of hydrogen Lyman-alpha observations of the coma of Comet P/Halley near the perihelion

The pioneer Venus Orbiter Ultraviolet Spectrometer measurements of the Lyman-alpha intensity of atomic hydrogen excited by solar resonance scattering in the coma of Comet P/Halley acquired from December 28, 1985, to January 6, 1986, and from January 31, 1986, to March 6, 1986, are simulated with the Monte Carlo Particle Trajectory Model corrected for optical depth effects. Spatially detailed comparisons between data and model show excellent agreement and are used to infer that the highest cometary activity may not be at perihelion, but about 2 1/2 weeks before. An improved set of H2O production rates is presented for the period of time that the spectrometer was observing and is found to be consistent with the rates from other types of measurements. The apparent discrepancy between Stewart (1987) in early March and International Ultraviolet Explorer OH derived rates is resolved. The problem with the conversion of 18-cm OH radio brightness to H2O production rates is also discussed.

Smyth, William H.↗
NASA NTRS1985

Phase change water processing for Space Station

The use of a vapor compression distillation subsystem (VCDS) for water recovery on the Space Station is analyzed. The self-contained automated system can process waste water at a rate of 32.6 kg/day and requires only 115 W of electric power. The improvements in the mechanical components of VCDS are studied. The operation of VCDS in the normal mode is examined. The VCDS preprototype is evaluated based on water quality, water production rate, and specific energy. The relation between water production rate and fluids pump speed is investigated; it is concluded that a variable speed fluids pump will optimize water production. Components development and testing currently being conducted are described. The properties and operation of the proposed phase change water processing system for the Space Station, based on vapor compression distillation, are examined.

Zdankiewicz, E. M.↗
NASA NTRS1973

Neutral-pion-decay gamma rays from the Galaxy and the interstellar gas content

Knowledge of the total gamma-ray production rate per H atom from the decay of neutral pions produced in interstellar cosmic-ray interactions is essential for determining the possible amount of interstellar H2. This production rate is recalculated here using the latest accelerator data on neutral pion production in p-p interactions up to about 1500 GeV. A simple but accurate approximation used here resolves the past disagreement over the magnitude of this rate. An upper limit is obtained of (1.51 plus or minus 0.23) times 10 to the -25th power/sec, consistent with the observed upper limit of 1.6 times 10 to the -25th power/sec.

Stecker, F. W.↗
NASA NTRS1982

Narrowband photometry of Comet P/Stephan-Oterma and the backscattering properties of cometary grains

The results of narrowband filter photometry of Comet P/Stephan-Oterma are presented. For heliocentric distances between 1.95 and 1.58 AU prior to perihelion, OH, CN, and C2 production rates varied approximately as r to the -5th power. Following perihelion, an even steeper dependence of production rate on heliocentric distance was observed for these species. A pronounced brightening of the comet's continuum near opposition is interpreted in terms of preferential backscattering by the cometary dust. While Comet P/Stephan-Oterma is one of the dustier comets observed, it shows no indication of compositional anomalies in either the gas or the dust.

Millis, R. L.↗