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NASA NTRS1977

International Conference on Problems Related to the Stratosphere

The conference focused on four main areas of investigation: laboratory studies and stratospheric chemistry and constituents, sources for and chemical budget of stratospheric halogen compounds, sources for and chemical budget of stratospheric nitrous oxide, and the dynamics of decision making on regulation of potential pollutants of the stratosphere. Abstracts of the scientific sessions of the conference as well as complete transcriptions of the panel discussions on sources for an atmospheric budget of holocarbons and nitrous oxide are included. The political, social and economic issues involving regulation of potential stratospheric pollutants were examined extensively.

Huntress, W., Jr.↗

NASA NTRS1977

Direct measurements of stratospheric fluoride

Stratospheric fluoride mass mixing ratios were measured by passing stratospheric air through filters half of which is impregnated in a base. Measurements of stratospheric fluoride were obtained at altitudes from 15 to 40 km at latitude 30-33 N and longitude 95-105 W at different months of the year. The significant amount of fluoride collected on the base-impregnated portion of the filters suggests that fluoride is present in the stratosphere as an acid gas. The mixing ratios decrease markedly at altitudes less than 20-25 km, suggesting the troposphere as the major sink for stratospheric fluoride.

Mroz, E. J.↗

NASA NTRS1977

Microphysical processes affecting stratospheric aerosol particles

Physical processes which affect stratospheric aerosol particles include nucleation, condensation, evaporation, coagulation and sedimentation. Quantitative studies of these mechanisms to determine if they can account for some of the observed properties of the aerosol are carried out. It is shown that the altitude range in which nucleation of sulfuric acid-water solution droplets can take place corresponds to that region of the stratosphere where the aerosol is generally found. Since heterogeneous nucleation is the dominant nucleation mechanism, the stratospheric solution droplets are mainly formed on particles which have been mixed up from the troposphere or injected into the stratosphere by volcanoes or meteorites. Particle growth by heteromolecular condensation can account for the observed increase in mixing ratio of large particles in the stratosphere. Coagulation is important in reducing the number of particles smaller than 0.05 micron radius. Growth by condensation, applied to the mixed nature of the particles, shows that available information is consistent with ammonium sulfate being formed by liquid phase chemical reactions in the aerosol particles. The upper altitude limit of the aerosol layer is probably due to the evaporation of sulfuric acid aerosol particles, while the lower limit is due to mixing across the tropopause.

Hamill, P.↗

NASA NTRS1977

Systems theoretic model of stratospheric pollution on ozone

Discrete state space analysis is applied to the development of a model for predicting the reduction in the amount of stratospheric ozone due to stratospheric pollution. The modeling approach is to segment the stratosphere into a number of altitudinal bands and to associate state variables with the state of ozone reduction in each band due to NO(x) injections. The ozone reductions in each band are then combined into an estimate of total global ozone reduction. The model proposed predicts changes in stratospheric ozone based on altitude of pollutant injection and volume of pollutant injected at that altitude. The present approach is not a detailed analysis of stratospheric constituents and their interactions, but rather an analysis procedure for modeling the results of other researchers in the field.

Wilkins, R. D.↗

NASA NTRS1979

A Saturnian stratospheric seasonal climate model

Motivated by recent observational evidence that seasonal processes occur within Saturn's stratosphere, a seasonal stratospheric climate model has been constructed. This model predicts stratospheric temperatures above the P = 0.1-atm level as a function of time throughout the Saturnian year. Specific results are presented for south-polar and equatorial temperatures. The model predicts that substantial seasonal phase lags exist; maximum stratospheric temperatures at the south pole occur at the southern hemisphere's autumnal equinox. Brightness temperature observations at 17.8 microns, taken during 1977/1978, indicate that stratospheric temperatures are greater at the south pole than at the equator. The model is consistent with these observations, predicting enhanced south polar temperatures, relative to the equator, from 1975 to 1983.

Cess, R. D.↗

NASA NTRS1980

Stratospheric free chlorine measured by balloon-borne in situ resonance fluorescence

Eight balloon-borne in situ measurements of ClO in the stratosphere are analyzed and are compared with recent model calculations. While the use of in situ stratospheric studies of free radicals to test models by comparing observed and predicted concentration profiles is essential for a prognosis of changes in stratospheric ozone, resulting from future changes in stratospheric ozone, such studies provide only limited insight into the nature of stratospheric photochemistry, because natural variability and the large number of fast reactions which compete in the coupling among the key radicals frustrate a detailed comparison between a mean distribution provided by the models and an instantaneous distribution provided by a single observation.

Anderson, J. G.↗

NASA NTRS1980

Analysis and interpretation of lidar observations of the stratospheric aerosol

Data obtained with a 48 in. telescope lidar system are compared with results obtained using a one-dimensional stratospheric aerosol model to analyze various microphysical processes influencing the formation of this aerosol. Special attention is given to the following problems: (1) how lidar data can help determine the composition of the aerosol particles and (2) how the layer corresponds to temperature profile variations. The lidar record during the period 1974 to 1979 shows a considerable decrease of the peak value of the backscatter ratio. Seasonal variations in the aerosol layer and a gradual decrease in stratospheric loading are observed. The aerosol model simulates a background stratospheric aerosol layer, and it predicts stratospheric aerosol concentrations and compositions. Numerical experiments are carried out by using the model and by comparing the theoretical results with the experimentally obtained lidar record. Comparisons show that the backscatter profile is consistent with the composition when the particles are sulfuric acid and water; it is not consistent with an ammonium sulfate composition. It is shown that the backscatter ratio is not sensitive to the composition or stratospheric loading of condensation nuclei such as meteoritic debris.

Hamill, P.↗

NASA NTRS1981

SAGE measurements of the stratospheric aerosol dispersion and loading from the Soufriere Volcano

Explosions of the Soufriere volcano on the Caribbean Island of St. Vincent reduced two major stratospheric plumes which the stratospheric aerosol and gas experiment (SAGE) satellite tracked to West Africa and the North Atlantic Ocean. The total mass of the stratospheric ejecta measured is less than 0.5% of the global stratospheric aerosol burden. No significant temperature or climate perturbation is expected. It is found that the movement and dispersion of the plumes agree with those deduced from high altitude meteorological data and dispersion theory. The stratospheric aerosol dispersion and loading from the Soufrier volcano was measured.

Mccormick, M. P.↗

NASA NTRS1982

SAM 2 Measurements of the Polar Stratospheric Aerosol, volume 2. April 1979 to October 1979

The Stratospheric Aerosol Measurement (SAM) II sensor is abroad the Earth orbiting Nimbus 7 spacecraft proving extinction measurements of the Antarctic and Arctic stratospheric aerosol with a vertical resolution of 1 km. Representative examples and weekly averages of aerosol data and corresponding temperature profiles for the time and place of each SAM II measurement (April 29, 1979, to October 27, 1979) is presented. Contours of aerosol extinction as a function of altitude and longitude or time were plotted and weekly aerosol optical depths were calculated. Seasonal variations and variations in space (altitude and longitude) for both polar regions are easily seen. Typical values of aerosol extinction at the SAM II wavelength of 1.0 micron for the time priod were 1 to 3 x 10 to the -4th power km -1 in the main stratospheric aerosol layer. Optical depths for the stratosphere were about 0.002. Polar stratospheric clouds at altitudes between the tropopause and 20 km were observed during the Antarctic winter at various times and locations. A ready-to-use format containing a representative sample of the second 6 months of data to be used in atmospheric and climatic studies is presented.

Mccormick, M. P.↗

NASA NTRS1982

A dehydration mechanism for the stratosphere

Although mean circulations are generally credited with dehydration of the earth's stratosphere, convective instability in the tropics converts mean circulations to small residuals of local convective circulations. The effects of large cumulonimbus which penetrate the stratosphere and form huge anvils in the lower stratosphere are discussed with respect to hydration and dehydration of the stratosphere. Radiative heating at anvil base combined with cooling at anvil top drives a dehydration engine considered essential to explain the dry stratosphere. Seasonal and longitudinal variations in dehydration potentials are examined with maximum potential attributed to Micronesian area during winter and early spring.

Danielsen, E. F.↗

NASA NTRS1982

Measurements of stratospheric aerosols over Mauna Loa, Hawaii and Boulder, Colorado

The direct solar radiation transmission record at Mauna Loa, dating from 1958 to the present, revealed with remarkable precision the presence of stratospheric aerosol from volcanic activity. This record can be used to quantify the intensity of the stratospheric volcanic aerosol perturbation following a significant eruption in reference to the Agung event in 1963. The Mount St. Helens' stratospheric cloud was first detected by lidar at 18 km over Mauna Loa on 17 July. The atmospheric transmission was seen to decrease slightly after that time, but only a few tenths of 1 percent. Although it is still fairly early to draw a definite conclusion on the ultimate magnitude of the Mount St. Helens stratospheric aerosol from the Mauna Loa results, it can be stated that the stratospheric aerosol optical depth presently observed is comparable with that observed from Fuego which erupted in 1974. At Boulder, Colorado, the atmospheric debris from Mount St. Helens was observed by lidar on a number of occasions. Also, observations of the diffuse, total and direct transmission of solar radiation were made on June 3 and 4. The latter set of observations is useful for deriving information on the scattering properties of the volcanic cloud. The lidar and solar radiation data are presented and some of their special features are discussed.

Deluisi, J. J.↗

NASA NTRS1983

SAM 2 measurements of the polar stratospheric aerosol. Volume 3: October 1979 to April 1980

The Stratospheric Aerosol Measurement (SAM) II sensor is aboard the Earth-orbiting Nimbus 7 spacecraft providing extinction measurements of the Antarctic and Arctic stratospheric aerosol with a vertical resolution of 1 km. Representative examples and weekly averages of aerosol data and corresponding temperature profiles for the time and place of each SAM II measurement (Oct. 1979 through Apr. 1980) are presented. Contours of aerosol extinction as a function of altitude and longitude or time are plotted and weekly aerosol optical depths are calculated. Seasonal variations and variations in space (altitude and longitude) for both polar regions are easily seen. Typical values of aerosol extinction at the SAM II wavelength of 1.0 microns for this time period are 2 to 4 times .0001/km in the main stratospheric aerosol layer. Optical depths for the stratosphere are about 0.002 to 0.003, up slightly over normal background levels (due to the eruption of Sierra Negra, Nov. 1979). Polar stratospheric clouds at altitudes of about 22 km were observed during the Arctic winter. A ready-to-use format containing a representative sample of the third 6 months of data to be used in atmospheric and climatic studies is presented.

Mccormick, M. P.↗

NASA NTRS1982

Photochemistry of the stratosphere of Venus - Implications for atmospheric evolution

The photochemistry of the Venus stratosphere is modeled using an updated and expanded chemical scheme along with the results of recent observations and laboratory studies. Three models, with H2 mixing ratio equal to 2 x 10 to the -5th, 5 x 10 to the -7th, and 1 x 10 to the -13th, respectively, are examined. All three models are found to satisfactorily account for the observations of CO, O2, O2(1Delta), and SO2 in the stratosphere, but only the last one may be able to account for the diurnal behavior of mesospheric CO and the UV albedo. Oxygen, derived from CO2 photolysis, is mainly consumed by CO2 recombination and oxidation of SO2 to H2SO4. The photolysis of HCl in the upper stratosphere provides a major source of odd hydrogen and free chlorine radicals, essential for the catalytic oxidation of CO. Oxidation of SO2 by O occurs in the lower stratosphere. The modeling reveals a number of interesting similarities, previously unsuspected between the chemistry of the stratosphere of Venus and that of the earth; photochemistry may have played a major role in the evolution of the atmosphere.

Yung, Y. L.↗

NASA NTRS1985

Development of algorithms for using satellite meteorological data sets to study global transport of stratospheric aerosols and ozone

The utilization of stratospheric aerosol and ozone measurements obtained from the NASA developed SAM II and SAGE satellite instruments were investigated for their global scale transports. The stratospheric aerosols showed that during the stratospheric warming of the winter 1978 to 1979, the distribution of the zonal mean aerosol extinction ratio in the northern high latitude exhibited distinct changes. Dynamic processes might have played an important role in maintenance role in maintenance of this zonal mean distribution. As to the stratospheric ozone, large poleward ozone transports are shown to occur in the altitude region from 24 km to 38 km near 55N during this warming. This altitude region is shown to be a transition region of the phase relationship between ozone and temperature waves from an in-phase one above 38 km. It is shown that the ozone solar heating in the upper stratosphere might lead to enhancement of the damping rate of the planetary waves due to infrared radiation alone in agreement with theoretical analyses and an earlier observational study.

Want, P. H.↗

NASA NTRS1985

Aspects of the stratospheric circulation as derived from SSU data

Five years of global data are available for the stratosphere up to 1 mb from Stratospheric Sounding Units (SSUs) on board NOAA satellites. These data form the basis for a climatological study which concentrates on the seasonal and inter-annual variability of the stratosphere and the connection between the stratospheric circulation and that of the troposphere. Particular emphasis is on the structure of the Southern Hemisphere and how it compares with that of the Northern Hemisphere. The characteristic difference in the vertical structure and propagation of disturbances in the two hemispheres is related to differences in the tropospheric flow and the long-term variation of the basic state of the stratosphere. Disturbances in both hemispheres occur in preferred geographical locations. The final warming, marking the transition from westerly to easterly winds, is an example. These occur asymmetrically with respect to the pole as warm air moves over the pole, usually from the same region.

Michaelis, V.↗

NASA NTRS1985

A new model of resonance in the winter stratosphere

It is generally accepted that the planetary waves observed in the winter stratosphere are primarily a response to dynamical forcing from the troposphere. Nevertheless, the mechanism by which wave amplitudes sometimes become larger remains uncertain. It is possible that anomalously large waves in the stratosphere might simply be the result of anomalously large tropospheric forcing. However, it has also been suggested that they are a response to a stratospheric-tropospheric cavity being in a near-resonant configuration. It has been suggested that nonlinear self-tuning effects could play an important role in the behavior of such a cavity. Self-tuning may occur when a system starts to one side of resonance, such that the mean-state change induced by growing waves brings the system closer to resonance. A new model of the stratospheric cavity is introduced and is then used to re-examine the possibility of wave growth in the real atmosphere and in atmospheric models due to self-tuning effects. The new model is based on the picture of the winter-time stratosphere which has been revealed by the observations of Ertel's potential vorticity, Q. Isentropic maps of Q show two rather distinct regions, the first containing the circumpolar vortex, where gradients of Q are large and Rossby waves may propagate easily. Surrounding this is a second, low-latitude region where the gradients are generally weak and where, because the Eulerian-mean flow is comparable with their phase speed, Rossby waves must be continually breaking. As the waves are observed to grow the relative sizes of these two regions change in time. This leads to the interesting possibility that self-tuning, mainly due to irreversible changes in the size of the polar vortex, is taking place.

Haynes, P. H.↗

NASA NTRS1985

Rossby wavetrains in the stratosphere forced by localised disturbances in the troposphere

Studies have linked elements of the stratospheric circulation with particular localized features in the tropospheric circulation. This suggests a study of the response of the stratosphere to forcing by localized disturbances in the troposphere. A multilevel, primitive equation model is used of the stratosphere and mesosphere the height of whose lower boundary at 300 mb can be prescribed. Localized height disturbances which grow to steady amplitude are applied at this lower boundary, and the response of the initially axially symmetric stratosphere is studied. The perturbation, centered at 45 deg N, has a Gaussian distribution with a half width of 15 deg., corresponding roughly to the size of persistent troughs and blocking ridges in the troposphere. The forcing is nearly at fully amplitude 10 days after being switched on, and thereafter remains steady. Two types of experiments are conducted: in one the forcing is of small amplitude (100 gpm) and in the other it is of large amplitude (600 gpm). These pairs of experiments are compared to determine how nonlinear processes affect the perturbation fields. This is done locally by defining the perturbation response to the forcing as an anomaly, i.e., as a departure from the response in a controlled experiment in which no asymmetric forcing was applied at the lower boundary of the model. Experiments have been conducted for a number of atmospheric states obtained as zonal means of observations made by a stratospheric sounding unit (SSU). In this summary, results for the zonal mean flow on January 19, 1982 are outlined.

Marks, C. J.↗

NASA NTRS1986

SAM 2 measurements of the polar stratospheric aerosol, volume 2

The Stratospheric Aerosol Measurement (SAM) 2 sensor aboard Nimbus 7 is providing extinction measurements of Antarctic and Arctic stratospheric aerosols with a vertical resolution of 1 km. Representative examples and weekly averages including corresponding temperature profiles provided by NOAA for the time and place of each SAM 2 measurement (Oct. 1981 - Apr. 1982) are presented. Contours of aerosol extinction as a function of altitude and longitude or time are plotted, and aerosol optical depths are calculated for each week. Typical values of aerosol extinction at 1.0 micron in the main lower stratospheric aerosol layer for this time period are 2 to 4 times 10 to the -4 power/km. for the Antarctic region and 0.5 to 1 times 10 to the -3 power/km. for the Arctic region. Stratospheric optical depths are about 0.001 to 0.004 for the Antarctic region and 0.003 to 0.004 at the beginning to about 0.006 at the end of the time period for the Arctic region. Polar stratospheric clouds (PSC's) were observed during the Arctic winter, as expected. This report provides, in a ready-to-use format, a representative sample of the seventh semester of data to be used in atmospheric and climatic studies.

Mccormick, M. P.↗