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At least 271 records · Page 15

Engineered unique elastic modes at a BaTiO 3 /2x1-Ge(001) interface

Here, the strong interaction at an interface between a substrate and thin film leads to epitaxy and provides a means of inducing structural changes in the epitaxial film. These induced material phases often exhibit technologically relevant electronic, magnetic, and functional properties. The 2×1 surface of a Ge(001) substrate applies a unique type of epitaxial constraint on thin films of the perovskite oxide BaTiO 3 where a change in bonding and symmetry at the interface leads to a non-bulk-like crystal structure of the BaTiO 3 . While the complex crystal structure is predicted using first-principles theory, it is further shown that the details of the structure are a consequence of hidden phases found in the bulk elastic response of the BaTiO 3 induced by the symmetry of forces exerted by the germanium substrate.

29 ENERGY PLANNING, POLICY, AND ECONOMY↗

Large exciton binding energy in a bulk van der Waals magnet from quasi-1D electronic localization

Excitons, bound electron-hole pairs, influence the optical properties in strongly interacting solid-state systems and are typically most stable and pronounced in monolayer materials. Bulk systems with large exciton binding energies, on the other hand, are rare and the mechanisms driving their stability are still relatively unexplored. Here, we report an exceptionally large exciton binding energy in single crystals of the bulk van der Waals antiferromagnet CrSBr. Utilizing state-of-the-art angle-resolved photoemission spectroscopy and self-consistent ab-initio GW calculations, we present direct spectroscopic evidence supporting electronic localization and weak dielectric screening as mechanisms contributing to the amplified exciton binding energy. Furthermore, we report that surface doping enables broad tunability of the band gap offering promise for engineering of the optical and electronic properties. Our results indicate that CrSBr is a promising material for the study of the role of anisotropy in strongly interacting bulk systems and for the development of exciton-based optoelectronics.

36 MATERIALS SCIENCE↗

Locating the QCD critical point through contours of constant entropy density

We propose a new method to investigate the existence and location of the conjectured high-temperature critical point of strongly interacting matter via contours of constant entropy density. By approximating these lines as a power series in the baryon chemical potential 𝜇 𝐵 , one can extrapolate them from first-principle results at zero net-baryon density, and use them to locate the quantum chromodynamics (QCD) critical point, including the associated first-order and spinodal lines. As a proof of principle, we employ currently available continuum-extrapolated lattice data from the Wuppertal-Budapest collaboration to find a critical point at a temperature and a baryon chemical potential of 𝑇 𝑐 = 114.3 ± 6.9 MeV and 𝜇 𝐵,𝑐 = 602.1 ± 62.1 MeV, respectively, at expansion order 𝒪⁡(𝜇$^{2}_{𝐵}$). We advocate for a more precise determination of the required expansion coefficients via lattice QCD simulations as a means of pinpointing the location of the critical endpoint in the phase diagram of strongly interacting matter.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

[C II] and {sup 12}CO(1-0) emission maps in HLSJ091828.6+514223: A strongly lensed interacting system at z = 5.24

We present Submillimeter Array [C II] 158 μm and Karl G. Jansky Very Large Array {sup 12}CO(1-0) line emission maps for the bright, lensed, submillimeter source at z = 5.2430 behind A 773: HLSJ091828.6+514223 (HLS0918). We combine these measurements with previously reported line profiles, including multiple {sup 12}CO rotational transitions, [C I], water, and [N II], providing some of the best constraints on the properties of the interstellar medium in a galaxy at z > 5. HLS0918 has a total far-infrared (FIR) luminosity L {sub FIR(8–1000} {sub μm)} = (1.6 ± 0.1) × 10{sup 14} L {sub ☉} μ{sup –1}, where the total magnification μ{sub total} = 8.9 ± 1.9, via a new lens model from the [C II] and continuum maps. Despite a HyLIRG luminosity, the FIR continuum shape resembles that of a local LIRG. We simultaneously fit all of the observed spectral line profiles, finding four components that correspond cleanly to discrete spatial structures identified in the maps. The two most redshifted spectral components occupy the nucleus of a massive galaxy, with a source-plane separation <1 kpc. The reddest dominates the continuum map (demagnified L {sub FIR,} {sub component} = (1.1 ± 0.2) × 10{sup 13} L {sub ☉}) and excites strong water emission in both nuclear components via a powerful FIR radiation field from the intense star formation. A third star-forming component is most likely a region of a merging companion (ΔV ∼ 500 km s{sup –1}) exhibiting generally similar gas properties. The bluest component originates from a spatially distinct region and photodissociation region analysis suggests that it is lower density, cooler, and forming stars less vigorously than the other components. Strikingly, it has very strong [N II] emission, which may suggest an ionized, molecular outflow. This comprehensive view of gas properties and morphology in HLS0918 previews the science possible for a large sample of high-redshift galaxies once ALMA attains full sensitivity.

79 ASTRONOMY AND ASTROPHYSICS↗

Abundance and properties of dark radiation from the cosmic microwave background

We study the cosmological signatures of new light relics that are collisionless like standard neutrinos or are strongly interacting. We provide a simple and succinct rephrasing of their physical effects in the cosmic microwave background, as well as the resulting parameter degeneracies with other cosmological parameters, in terms of the total radiation abundance and the fraction thereof that freely streams. In these more general terms, interacting and noninteracting light relics are differentiated by their respective decrease and increase of the free-streaming fraction, and, moreover, the scale-dependent interplay thereof with a common, correlated reduction of the fraction of matter in baryons. We then derive updated constraints on various dark-radiation scenarios with the latest cosmological observations, employing this language to identify the physical origin of the impact of each dataset. The “PR4” reanalyses of Planck CMB data prefer a larger primordial helium yield and therefore also slightly more radiation than the 2018 analysis; we investigate the differences between the two releases that drives these shifts. Smaller free-streaming fractions are disfavored by the excess lensing of the CMB measured in lensing reconstruction data from Planck and the Atacama Cosmology Telescope. On the other hand, baryon acoustic oscillation measurements from the Dark Energy Spectroscopic Instrument drive marginal detections of new, strongly interacting light relics due to that data's preference for lower matter fractions. Finally, we forecast measurements from the CMB-S4 experiment.

cosmological parameters from CMBR↗

Chiral Effective Field Theory and the High-Density Nuclear Equation of State

Born in the aftermath of core-collapse supernovae, neutron stars contain matter under extraordinary conditions of density and temperature that are difficult to reproduce in the laboratory. In recent years, neutron star observations have begun to yield novel insights into the nature of strongly interacting matter in the high-density regime where current theoretical models are challenged. At the same time, chiral effective field theory has developed into a powerful framework to study nuclear matter properties with quantified uncertainties in the moderate-density regime for modeling neutron stars. In this article, we review recent developments in chiral effective field theory and focus on many-body perturbation theory as a computationally efficient tool for calculating the properties of hot and dense nuclear matter. We also demonstrate how effective field theory enables statistically meaningful comparisons among nuclear theory predictions, nuclear experiments, and observational constraints on the nuclear equation of state.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Gel phase formation in dilute triblock copolyelectrolyte complexes

Assembly of oppositely charged triblock copolyelectrolytes into phase-separated gels at low polymer concentrations (<1% by mass) has been observed in scattering experiments and molecular dynamics simulations. Here we show that in contrast to uncharged, amphiphilic block copolymers that form discrete micelles at low concentrations and enter a phase of strongly interacting micelles in a gradual manner with increasing concentration, the formation of a dilute phase of individual micelles is prevented in polyelectrolyte complexation-driven assembly of triblock copolyelectrolytes. Gel phases form and phase separate almost instantaneously on solvation of the copolymers. Furthermore, molecular models of self-assembly demonstrate the presence of oligo-chain aggregates in early stages of copolyelectrolyte assembly, at experimentally unobservable polymer concentrations. Our discoveries contribute to the fundamental understanding of the structure and pathways of complexation-driven assemblies, and raise intriguing prospects for gel formation at extraordinarily low concentrations, with applications in tissue engineering, agriculture, water purification and theranostics.

36 MATERIALS SCIENCE↗

γvNN^* Transition Amplitudes and Excited Baryon Structure from CLAS

Studying excited nucleon structure through exclusive-meson electroproduction reactions is key for understanding the nature of the strong interaction in the non-perturbative regime. With its nearly complete coverage of the final-state phase space, the CLAS detector at JLab has provided the lion's share of the world's meson-electroproduction data for differential cross sections and the asymmetries arising from single- and double-polarization observables. Electrocouplings for most of the excited nucleon states (N*) in mass range of up to 1.8~GeV have been determined from several analyses of the CLAS data for photon virtualities (Q2) up to 5.0 GeV2 for the pi+n, pi0p, and eta p channels [1,3] as well as for the pi+pi-p reaction for Q2<1.5~GeV2 [2,3]. Physics analyses of these N* electrocouplings [2,3] have revealed that the structure of excited nucleon is formed of an internal core of dressed quarks with an external meson-baryon cloud. Our N*-electrocoupling results afford access to the non-perturbative strong interaction responsible for generating the different N* states and will also provide testing ground for the inspired by QCD quark model predictions. A dedicated experiment will run after the 12 GeV upgrade to JLab on the extraction of the N* electrocouplings in the yet unexplored region of high photon virtualities ranging from 5.0 to 12 GeV2. The anticipated results are of particular importance in providing a understanding of the nature of confinement and dynamical chiral symmetry breaking in baryons based upon the QCD [3].\\[4pt] [1] I.G. Aznauryan and V.D. Burkert, Prog. Part. Nucl. Phys. \textbf{67}, 1 (2012).\\[0pt] [2] V.I. Mokeev \textit{et~al.} (CLAS Collaboration), Phys. Rev. \textbf{C86}, 035203 (2012).\\[0pt] [3] I.G. Aznauryan \textit{et~al.}, ``Studies of Nucleon Resonance Structure in Exclusive Meson Electroproduction,'' arXiv:1212.4891[nucl-th].

Mokeev, Victor↗

Analyzing Single Giant Unilamellar Vesicles With a Slotline-Based RF Nanometer Sensor

Novel techniques that enable reagent free detection and analysis of single cells are of great interest for the development of biological and medical sciences as well as point-of-care health service technologies. Highly sensitive and broadband radio-frequency (RF) sensors are promising candidates for such a technique. In this work, we present a highly sensitive and tunable RF sensor, which is based on interference processes and built with a 100 nm slotline structure. The highly concentrated RF fields, up to ~1.76×107 V/m, enable strong interactions between Giant unilamellar vesicles (GUVs) and fields for high sensitivity operations. We also provide two modeling approaches to extract cell dielectric properties from measured scattering parameters. GUVs of different molecular compositions are synthesized and analyzed with the RF sensor at ~2 GHz, ~2.5 GHz, and ~2.8 GHz with an initial |S21|min of ~-100 dB. Corresponding GUV dielectric properties are obtained. A one-dimensional scanning of single GUV is also demonstrated.

Cui, Yan↗

A glimpse of gluons through deeply virtual compton scattering on the proton

The proton is composed of quarks and gluons, bound by the most elusive mechanism of strong interaction called confinement. In this work, the dynamics of quarks and gluons are investigated using deeply virtual Compton scattering (DVCS): produced by a multi-GeV electron, a highly virtual photon scatters off the proton which subsequently radiates a high energy photon. Similarly to holography, measuring not only the magnitude but also the phase of the DVCS amplitude allows to perform 3D images of the internal structure of the proton. The phase is made accessible through the quantum-mechanical interference of DVCS with the Bethe-Heitler (BH) process, in which the final photon is emitted by the electron rather than the proton. Here, we report herein the first full determination of the BH-DVCS interference by exploiting the distinct energy dependences of the DVCS and BH amplitudes. In the high energy regime where the scattering process is expected to occur off a single quark in the proton, these accurate measurements show an intriguing sensitivity to gluons, the carriers of the strong interaction.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Two-component exciton condensates in an electron–hole bilayer

Macroscopic quantum coherence emerges when bosons condense into a Bose–Einstein condensate (BEC). Excitons are a long-sought solid-state route to high-temperature BECs with strong interactions, electrical tunability and potentially multicomponent spinor order, but conclusive evidence for equilibrium condensation has remained elusive. Here we report evidence for two-component exciton BECs in MoSe 2 /hBN/WSe 2 electron–hole bilayers by probing the spin–valley susceptibility of constituent electrons and holes. This heterostructure hosts equilibrium exciton fluids with four spin–valley flavours. Magneto-optical spectroscopy in a dilution refrigerator reveals three exciton condensate phases with distinct flavour polarizations. At zero magnetic field, the many-body ground state is a coherent superposition of two condensed intravalley exciton flavours. Under a magnetic field, the intravalley exciton condensate first switches to a two-component intervalley condensate through a first-order quantum phase transition at a weak critical field and then turns into a fully polarized single-component condensate at high fields. The condensate signatures form a dome in density–temperature space, persisting up to approximately 1.8 K. Our results establish van der Waals electron–hole bilayers as a versatile platform for strongly interacting, multicomponent exciton BECs.

Qi, Ruishi [University of California, Berkeley, CA↗

Deep learning: Extrapolation tool for ab initio nuclear theory

Ab initio approaches in nuclear theory, such as the no-core shell model (NCSM), have been developed for approximately solving finite nuclei with realistic strong interactions. The NCSM and other approaches require an extrapolation of the results obtained in a finite basis space to the infinite basis space limit and assessment of the uncertainty of those extrapolations. Each observable requires a separate extrapolation and many observables have no proven extrapolation method. Herein, we propose a feed-forward artificial neural network (ANN) method as an extrapolation tool to obtain the ground-state energy and the ground-state point-proton root-mean-square (rms) radius along with their extrapolation uncertainties. The designed ANNs are sufficient to produce results for these two very different observables in 6 Li from the ab initio NCSM results in small basis spaces that satisfy the following theoretical physics condition: independence of basis space parameters in the limit of extremely large matrices. Comparisons of the ANN findings with other extrapolation methods are also provided.

6Li↗

Production of Jet Fuel-Range Hydrocarbons from Hydrodeoxygenation of Lignin over Super Lewis Acid Combined with Metal Catalysts

Super Lewis acids containing the triflate anion (e.g. Hf(OTf)4, Ln(OTf)3, Al(OTf)3) and noble metal catalysts (e.g. Ru/C, Ru/Al2O3) formed efficient catalytic systems to generate saturated hydrocarbons from lignin in high yields. In such catalytic systems, the metal triflates mediated rapid ether bond cleavage via selective bonding to etheric oxygens while the noble metal catalysed subsequent hydrodeoxygenation (HDO) reactions. Near theoretical yields of hydrocarbons were produced from lignin model compounds by the combined catalysis of Hf(OTf)4 and ruthenium-based catalysts. When a technical lignin derived from a pilot-scale biorefinery was used, more than 30 wt% of the hydrocarbons produced with this catalytic system were cyclohexane and alkylcyclohexanes in the jet fuel range. Super Lewis acids are postulated to strongly interact with lignin substrates via protonating hydroxyls and ether linkages, forming intermediate species that enhance hydrogenation catalysis by supported noble metal catalysts. Meanwhile, the hydrogenation of aromatic rings by the noble metal catalysts can promote oxygenation reactions catalysed by super Lewis acids.

Wang, Hongliang↗

Effective matrix model for nuclear physics on a quantum computer

In this project we studied a simplified potential from [1] describing nuclear physics from quark and gluon fields, where spatial degrees of freedom have been integrated over. This potential deals with the phase structure of the strong interaction. We created a matrix representation of the Hamiltonian for this theory using discrete quantum mechanics [2]. We then feed this Hamiltonian to IBM's Qiskit package [3]. We run on IBM's 32-qubit quantum simulator, which approximates the ground state energy using the variational quantum eigensolver (VQE) algorithm [4]. This result is then compared with the exact ground state energy, which we can calculate classically since the matrices we use are still small enough. The bosonic Hamiltonian for a 6-qubit representation took over 1000 Pauli factors to represent fully. To improve our performance, we can look for a more efficient representation of this model's Hamiltonian. We will develop a better variational trial wave function and initial state, as well as include the effect of fermions and heavy quarks on the potential.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Dynamic localization and shear-induced hopping of particles: A way to understand the rheology of dense colloidal dispersions

For decades, attempts have been made to understand the formation of colloidal glasses and gels by linking suspension mechanics to particle properties where details of size, shape, and spatial dependencies of pair potentials present a bewildering array of variables that can be manipulated to achieve observed properties. Despite the range of variables that control suspension properties, one consistent observation is the remarkably similarity of flow properties observed as particle properties are varied. Understanding the underlying origins of the commonality in those behaviors (e.g., shear-thinning with increasing stress, diverging zero shear rate viscosity with increasing volume fraction, development of a dynamic yield stress plateau with increases in volume faction or strength of attraction, development of two characteristic relaxation times probed in linear viscoelasticity, the creation of a rubbery plateau modulus at high strain frequencies, and shear-thickening) remains a challenge. Recently, naïve mode coupling and dynamic localization theories have been developed to capture collective behavior giving rise to formation of colloidal glasses and gels. This approach characterizes suspension mechanics of strongly interacting particles in terms of sluggish long-range particle diffusion modulated by varying particle interactions and volume fraction. These theories capture the scaling of the modulus with the volume fraction and strength of interparticle attraction, the frequency dependence of the moduli at the onset of the gel/glass transition, together with the divergence of the zero shear rate viscosity and cessation of diffusivity for hard sphere systems as close packing is approached. In this study, we explore the generality of the predictions of dynamic localization theory for systems of particles composed of bimodal particle size distributions experiencing weak interactions. We find that the mechanical properties of these suspensions are well captured within the framework of dynamic localization theory and that suspension mechanics can be understood in terms of a dynamical potential barrier, the magnitude of which governs the zero shear rate viscosity, and onset of a dynamic yield stress plateau as volume fraction or strength of interaction is raised.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Measurement of the proton spin structure at long distances

Measuring the spin structure of protons and neutrons tests our understanding of how they arise from quarks and gluons, the fundamental building blocks of nuclear matter. At long distances, the coupling constant of the strong interaction becomes large, requiring non-perturbative methods to calculate quantum chromodynamics processes, such as lattice gauge theory or effective field theories. In this work, we report proton spin structure measurements from scattering a polarized electron beam off polarized protons. The spin-dependent cross-sections were measured at large distances, corresponding to the region of low momentum transfer squared between 0.012 and 1.0GeV 2 . This kinematic range provides unique tests of chiral effective field theory predictions. Our results show that a complete description of the nucleon spin remains elusive, and call for further theoretical works, for example, in lattice quantum chromodynamics. Finally, our data extrapolated to the photon point agree with the Gerasimov–Drell–Hearn sum rule, a fundamental prediction of quantum field theory that relates the anomalous magnetic moment of the proton to its integrated spin-dependent cross-sections.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Proceedings of RIKEN BNL Research Center Workshop: The Physics of p ↑ +A Collisions at RHIC

The RIKEN BNL Research Center (RBRC) was established in April 1997 at Brookhaven National Laboratory. It is funded by the "Rikagaku Kenkyusho" (RIKEN, The Institute of Physical and Chemical Research) of Japan. The Memorandum of Understanding between RIKEN and BNL, initiated in 1997, has been renewed in 2002, 2007 and again in 2012. The Center is dedicated to the study of strong interactions, including spin physics, lattice QCD, and RHIC physics through the nurturing of a new generation of young physicists. The RBRC has both a theory and experimental component. The RBRC Theory Group and the RBRC Experimental Group consists of a total of 25-30 researchers. Positions include the following: full time RBRC Fellow, half-time RHIC Physics Fellow, and full-time postdoctoral Research Associate. The RHIC Physics Fellows hold joint appointments with RBRC and other institutions and have tenure track positions at their respective universities or BNL. To date, RBRC has over 95 graduates (Fellows and Post- docs) of which approximately 40 theorists and 20 experimenters have already attained tenure positions at major institutions worldwide. Beginning in 2001 a new RIKEN Spin Program (RSP) category was implemented at RBRC. These appointments are joint positions of RBRC and RIKEN and include the following positions in theory and experiment: RSP Researchers, RSP Research Associates, and Young Researchers, who are mentored by senior RBRC Scientists. A number of RIKEN Jr. Research Associates and Visiting Scientists also contribute to the physics program at the Center. RBRC has an active workshop program on strong interaction physics with each workshop focused on a specific physics problem. In most cases all the talks are made available on the RBRC website. In addition, highlights to each speaker’s presentation are collected to form proceedings which can therefore be made available within a short time after the workshop. To date there are over one hundred proceeding volumes available. A 10 teraflops RBRC QCDOC computer funded by RIKEN, Japan, was unveiled at a dedication ceremony at BNL on May 26, 2005. This supercomputer was designed and built by individuals from Columbia University, IBM, BNL, RBRC, and the University of Edinburgh, with the U.S. D.O.E. Office of Science providing infrastructure support at BNL. Physics results were reported at the RBRC QCDOC Symposium following the dedication. QCDSP, a 0.6 teraflops parallel processor, dedicated to lattice QCD, was begun at the Center on February 19, 1998, was completed on August 28, 1998, and was decommissioned in 2006. It was awarded the Gordon Bell Prize for price performance in 1998. QCDOC was decommissioned in May 2012. The next generation computer in this sequence, QCDCQ (600 Teraflops), is currently operational and is expected to produce many more interesting discoveries in the future.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Proceedings of RIKEN BNL Research Center Workshop, Volume 113: Thermal Radiation Workshop

The RIKEN BNL Research Center (RBRC) was established in April 1997 at Brookhaven National Laboratory. It is funded by the "Rikagaku Kenkyusho" (RIKEN, The Institute of Physical and Chemical Research) of Japan. The Memorandum of Understanding between RIKEN and BNL, initiated in 1997, has been renewed in 2002, 2007 and again in 2012. The Center is dedicated to the study of strong interactions, including spin physics, lattice QCD, and RHIC physics through the nurturing of a new generation of young physicists. The RBRC has both a theory and experimental component. The RBRC Theory Group and the RBRC Experimental Group consists of a total of 25-30 researchers. Positions include the following: full time RBRC Fellow, half-time RHIC Physics Fellow, and full-time post doctoral Research Associate. The RHIC Physics Fellows hold joint appointments with RBRC and other institutions and have tenure track positions at their respective universities or BNL. To date, RBRC has over 95 graduates (Fellows and Post- docs) of which approximately 40 theorists and 20 experimenters have already attained tenure positions at major institutions worldwide. Beginning in 2001 a new RIKEN Spin Program (RSP) category was implemented at RBRC. These appointments are joint positions of RBRC and RIKEN and include the following positions in theory and experiment: RSP Researchers, RSP Research Associates, and Young Researchers, who are mentored by senior RBRC Scientists. A number of RIKEN Jr. Research Associates and Visiting Scientists also contribute to the physics program at the Center. RBRC has an active workshop program on strong interaction physics with each workshop focused on a specific physics problem. In most cases all the talks are made available on the RBRC website. In addition, highlights to each speaker’s presentation are collected to form proceedings which can therefore be made available within a short time after the workshop. To date there are over one hundred proceeding volumes available. A 10 teraflops RBRC QCDOC computer funded by RIKEN, Japan, was unveiled at a dedication ceremony at BNL on May 26, 2005. This supercomputer was designed and built by individuals from Columbia University, IBM, BNL, RBRC, and the University of Edinburgh, with the U.S. D.O.E. Office of Science providing infrastructure support at BNL. Physics results were reported at the RBRC QCDOC Symposium following the dedication. QCDSP, a 0.6 teraflops parallel processor, dedicated to lattice QCD, was begun at the Center on February 19, 1998, was completed on August 28, 1998, and was decommissioned in 2006. It was awarded the Gordon Bell Prize for price performance in 1998. QCDOC was decommissioned in May 2012. The next generation computer in this sequence, QCDCQ (600 Teraflops), is currently operational and is expected to produce many more interesting discoveries in the future.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗