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At least 271 records · Page 15

Impact of Three-Dimensional Radiative Effects on Satellite Retrievals of Cloud Droplet Sizes

There are several dozen papers that study the effects of cloud horizontal inhomogeneity on the retrievals of cloud optical thickness, but only a few of them deal with cloud droplet sizes. This paper is one of the first comprehensive attempts to fill this gap: It takes a close theoretical look at the radiative effects of cloud 3-D structure in retrievals of droplet effective radii. Under some general assumptions, it was found that ignoring subpixel (unresolved) variability produces a negative bias in the retrieved effective radius, while ignoring cloud inhomogeneity at scales larger than a pixel scale (resolved variability), on the contrary, leads to overestimation of the domain average droplet size. The theoretical results are illustrated with examples from Large Eddy Simulations (LES) of cumulus (Cu) and stratocumulus (Sc) cloud fields. The analysis of cloud drop size distributions retrieved from both LES fields confirms that ignoring shadowing in 1-D retrievals results in substantial overestimation of effective radii which is more pronounced for broken Cu than for Sc clouds. Collocated measurements of broken Cu clouds by Moderate Resolution Imaging Spectrometer (MODIS) and Advanced Spaceborne Thermal Emission and Reflection Radiometer (ASTER) are used to check simulations and theory with observations. The analysis of ASTER and MODIS data and associated derived products recommends against blindly using retrieved effective radii for broken cloud fields, especially if one wants to relate aerosol amounts to cloud droplet sizes.

Marshak, Alexander↗

An on-demand, drop-on-drop method for studying enzyme catalysis by serial crystallography

Serial femtosecond crystallography has opened up many new opportunities in structural biology. In recent years, several approaches employing light-inducible systems have emerged to enable time-resolved experiments that reveal protein dynamics at high atomic and temporal resolutions. However, very few enzymes are light-dependent, whereas macromolecules requiring ligand diffusion into an active site are ubiquitous. In this work we present a drop-on-drop sample delivery system that enables the study of enzyme-catalyzed reactions in microcrystal slurries. The system delivers ligand solutions in bursts of multiple picoliter-sized drops on top of a larger crystal-containing drop inducing turbulent mixing and transports the mixture to the X-ray interaction region with temporal resolution. We demonstrate mixing using fluorescent dyes, numerical simulations and time-resolved serial femtosecond crystallography, which show rapid ligand diffusion through microdroplets. The drop-on-drop method has the potential to be widely applicable to serial crystallography studies, particularly of enzyme reactions with small molecule substrates.

59 BASIC BIOLOGICAL SCIENCES↗

Rocket drops: The self-propulsion of supercooled freezing drops

Isolated supercooled water drops have been observed to move spontaneously while freezing in vacuum. This motion is caused by an increase of the evaporation rate during the early stages of freezing, which transfers momentum to the drops, similar to rocket propulsion. As in other cases of self-propulsion, symmetry-breaking is necessary, and occurs when ice nucleation occurs away from the center of the drop. The self-propulsion velocity was modeled analytically for a simplified case, and numerically for two experiments. Here, the model predicts peak velocities on the order of 1 m/s in vacuum, and a drop kinematics similar to that observed experimentally. In air, the self-propulsion velocity is expected to be much smaller but may be detectable for micron-sized drops.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Science Support for Space-Based Droplet Combustion: Drop Tower Experiments and Detailed Numerical Modeling

This program supports the engineering design, data analysis, and data interpretation requirements for the study of initially single component, spherically symmetric, isolated droplet combustion studies. Experimental emphasis is on the study of simple alcohols (methanol, ethanol) and alkanes (n-heptane, n-decane) as fuels with time dependent measurements of drop size, flame-stand-off, liquid-phase composition, and finally, extinction. Experiments have included bench-scale studies at Princeton, studies in the 2.2 and 5.18 drop towers at NASA-LeRC, and both the Fiber Supported Droplet Combustion (FSDC-1, FSDC-2) and the free Droplet Combustion Experiment (DCE) studies aboard the shuttle. Test matrix and data interpretation are performed through spherically-symmetric, time-dependent numerical computations which embody detailed sub-models for physical and chemical processes. The computed burning rate, flame stand-off, and extinction diameter are compared with the respective measurements for each individual experiment. In particular, the data from FSDC-1 and subsequent space-based experiments provide the opportunity to compare all three types of data simultaneously with the computed parameters. Recent numerical efforts are extending the computational tools to consider time dependent, axisymmetric 2-dimensional reactive flow situations.

Marchese, Anthony J.↗

Weber Number Tests in the NASA Icing Research Tunnel

A study of the Weber Number effects on droplets in the NASA Icing Research Tunnel is described. The work focuses on examining the droplet Weber Number effects observed for droplets accelerated by air flow in the contraction section of the Icing Research Tunnel to the test section. These results will aid in Supercooled Large Drop facility design studies. Measurements acquired with the Phase Doppler Interferometer and High Speed Imaging Dual Range Flight Probes at a series of locations through the contraction are presented alongside a 1D numerical model developed during this study to aid interpretation of the experimental results. An estimate of the maximum Weber Number observed in the Icing Research Tunnel for varying drop sizes up to 1000 m is presented and provided for incorporation into future design studies. Finally, experimental results coupled with a numerical model indicate that breakup of drops up to 1000 m is not occurring in the NASA Icing Research Tunnel up to 129 m/s.

Icing Wind Tunnel↗

Weber Number Tests in the NASA Icing Research Tunnel

A study of the Weber Number effects on droplets in the NASA Icing Research Tunnel is described. The work focuses on examining the droplet Weber Number effects observed for droplets accelerated by air flow in the contraction section of the Icing Research Tunnel to the test section. These results will aid in Supercooled Large Drop facility design studies. Measurements acquired with the Phase Doppler Interferometer and High Speed Imaging Dual Range Flight Probes at a series of locations through the contraction are presented alongside a 1D numerical model developed during this study to aid interpretation of the experimental results. An estimate of the maximum Weber Number observed in the Icing Research Tunnel for varying drop sizes up to 1000 μm is presented and provided for incorporation into future design studies. Finally, experimental results coupled with a numerical model indicate that breakup of drops up to 1000 μm is not occurring in the NASA Icing Research Tunnel up to 129 m/s.

Icing Wind Tunnel↗

Isokinetic Probe Total Water Content Measurements in the NASA Icing Research Tunnel with Supercooled Large Drop Conditions

An Isokinetic Total Water Content Evaporator (IKP2) was used to measure liquid water content (LWC) in the NASA Icing Research Tunnel (IRT) with spray conditions that ranged in LWC and cloud drop size spectra as characterized by the median volumetric diameter (MVD). The IKP2 measurements were made as part of an international collaborative effort to investigate the measurement of supercooled large drop (SLD) conditions in several icing wind tunnels. This report focuses on the IKP2 and background water vapor (BWV) measurements made within the NASA IRT during the October 2017 test entry. The IKP2 TWC results are compared to the IRT LWC calibration values for a range of LWC and MVD values. The IRT LWC calibration is based on measurements from a multi-element hot-wire probe. In general, the IKP2 TWC values were approximately 9% greater than the IRT LWC calibration values over a range of LWC from 0.4 g/m3 to 3.0 g/m3. The ratio of IKP2 TWC to IRT LWC calibration ranged from approximately 0.9 to 1.27 over a range of MVD from 15µm to 460 µm. Comparisons of this data set to IKP2 data from a 2014 IRT test entry show similar results in the regions where overlaps occurred. The results support the theory and observations of water mass loss from hot-wire TWC sensors when subjected to large MVD conditions.

Icing cloud instruments↗

Isokinetic Probe Total Water Content Measurements in the NASA Icing Research Tunnel with Supercooled Large Drop Conditions

An Isokinetic Total Water Content Evaporator (IKP2) was used to measure liquid water content (LWC) in the NASA Icing Research Tunnel (IRT) with spray conditions that ranged in LWC and cloud drop size spectra as characterized by the median volumetric diameter (MVD). The IKP2 measurements were made as part of an international collaborative effort to investigate the measurement of supercooled large drop (SLD) conditions in several icing wind tunnels. This report focuses on the IKP2 and background water vapor (BWV) measurements made within the NASA IRT during the October 2017 test entry. The IKP2 TWC results are compared to the IRT LWC calibration values for a range of LWC and MVD values. The IRT LWC calibration is based on measurements from a multi-element hot-wire probe. In general, the IKP2 TWC values were approximately 9% greater than the IRT LWC calibration values over a range of LWC from 0.4 g/m3 to 3.0 g/m3. The ratio of IKP2 TWC to IRT LWC calibration ranged from approximately 0.9 to 1.27 over a range of MVD from 15m to 460 m. Comparisons of this data set to IKP2 data from a 2014 IRT test entry show similar results in the regions where overlaps occurred. The results support the theory and observations of water mass loss from hot-wire TWC sensors when subjected to large MVD conditions.

o Aircraft Icing↗

Isokinetic Probe Total Water Content Measurements in the NASA Icing Research Tunnel with Supercooled Large Drop Conditions

An Isokinetic Total Water Content Evaporator (IKP2) was used to measure liquid water content (LWC) in the NASA Icing Research Tunnel (IRT) with spray conditions that ranged in LWC and cloud drop size spectra as characterized by the median volumetric diameter (MVD). The IKP2 measurements were made as part of an international collaborative effort to investigate the measurement of supercooled large drop (SLD) conditions in several icing wind tunnels. This report focuses on the IKP2 and background water vapor (BWV) measurements made within the NASA IRT during the October 2017 test entry. The IKP2 TWC results are compared to the IRT LWC calibration values for a range of LWC and MVD values. The IRT LWC calibration is based on measurements from a multi-element hot-wire probe. In general, the IKP2 TWC values were approximately 9% greater than the IRT LWC calibration values over a range of LWC from 0.4 g/m3 to 3.0 g/m3. The ratio of IKP2 TWC to IRT LWC calibration ranged from approximately 0.9 to 1.27 over a range of MVD from 15um to 460 um. Comparisons of this data set to IKP2 data from a 2014 IRT test entry show similar results in the regions where overlaps occurred. The results support the theory and observations of water mass loss from hot-wire TWC sensors when subjected to large MVD conditions.

o Aircraft Icing↗

Experimental study of the spray characteristics of a research airblast atomizer

Airblast atomization was studied using a especially designed atomizer in which the liquid first impinges on a splash plate, then is directed radially outward and is atomized by the air passing through two concentric, vaned swirlers that swirl the air in opposite directions. The effect of flow conditions, air mass velocity (mass flow rate per unit area) and liquid to air ratio on the mean drop size was studied. Seven different ethanol solutions were used to simulate changes in fuel physical properties. The range of atomizing air velocities was from 30 to 80 m/s. The mean drop diameter was measured at ambient temperature (295 K) and atmospheric pressure.

Acosta, W. A.↗

Experimental study of the spray characteristics of a research airblast atomizer

Airblast atomization was studied using a especially designed atomizer in which the liquid first impinges on a splash plate, then is directed radically outward and is atomized by the air passing through two concentric, vaned swirlers that swirl the air in opposite directions. The effect of flow conditions, air mass velocity (mass flow rate per unit area) and liquid to air ratio on the mean drop size was studied. Seven different ethanol solutions were used to simulate changes in fuel physical properties. The range of atomizing air velocities was from 30 to 80 m/s. The mean drop diameter was measured at ambient temperature (295 K) and atmospheric pressure.

Acosta, W. A.↗

Some Recent Observations on the Burning of Isolated N-Heptane and Alcohol Droplets

In a joint program involving Prof. F.A. Williams of the University of California, San Diego and Dr. V. Nayagam of the National Center for Microgravity Research on Combustion and Fluid Dynamics, the combustion of liquid fuel droplets of n-heptane, n-decane, methanol, methanol-water, ethanol and ethanol-water having initial diameters between about 1 mm and 6 mm continues to be studied. The objectives of the work are to improve fundamental knowledge of droplet combustion dynamics for pure fuels and fuel-water mixtures through microgravity experiments and theoretical analyses. The Princeton contributions to the collaborative program supports the engineering design, data analysis, and data interpretation requirements for the study of initially single component, spherically symmetric, isolated droplet combustion studies through experiments and numerical modeling. The complementary UCSD contributions apply asymptotic theoretical analyses and are described in the published literature and in a companion communication in this conference. The combined program continues to focus on analyses of results obtained from Fiber Supported Droplet Combustion (FSDC) experiments (FSDC-2, STS- 94) conducted with the above fuels in shuttle cabin air and Droplet Combustion Experiment (DCE) data obtained for unsupported and fiber supported droplets of n-heptane in Helium-Oxygen mixtures and cabin air (STS-83, STS-94). The program is preparing for a second DCE experimental mission using methanol/methanol-water as fuels and helium-oxygen-nitrogen environments. DCE-2 is to be conducted aboard the International Space Station. Emphases of recent Princeton work are on the study of simple alcohols (methanol, ethanol) and alcohol/water mixtures as fuels, with time-dependent measurements of drop size, flame-standoff, liquid-phase composition, and finally, extinction. Ground based experiments have included bench-scale studies at Princeton and collaborative experimental studies in the 2.2 second drop tower at NASA-Glenn Research Center.

Dryer, F. L.↗

Calculation of Water Drop Trajectories to and About Arbitrary Three-Dimensional Bodies in Potential Airflow

Calculations can be performed for any atmospheric conditions and for all water drop sizes, from the smallest cloud droplet to large raindrops. Any subsonic, external, non-lifting flow can be accommodated; flow into, but not through, inlets also can be simulated. Experimental water drop drag relations are used in the water drop equations of motion and effects of gravity settling are included. Seven codes are described: (1) a code used to debug and plot body surface description data; (2) a code that processes the body surface data to yield the potential flow field; (3) a code that computes flow velocities at arrays of points in space; (4) a code that computes water drop trajectories from an array of points in space; (5) a code that computes water drop trajectories and fluxes to arbitrary target points; (6) a code that computes water drop trajectories tangent to the body; and (7) a code that produces stereo pair plots which include both the body and trajectories. Code descriptions include operating instructions, card inputs and printouts for example problems, and listing of the FORTRAN codes. Accuracy of the calculations is discussed, and trajectory calculation results are compared with prior calculations and with experimental data.

Norment, H. G.↗

Production of polydisperse sprays.

A device which produces a spray with a controllable drop size distribution is described. This system is especially well suited for generating nonsmooth (e.g., bimodal) distributions, although smooth distributions can also be produced. Droplets of uniform size result from the rapid growth of an oscillatory disturbance in a free liquid jet. Simultaneous generation of droplets of various diameters by this method produces the polydisperse spray. The range of drop diameters is approximately 300-3000 microns.

Pierce, T. H.↗

Some Recent Observations on the Burning of Isolated N-Heptane and Alcohol Droplets

In a joint program involving Prof F.A. Williams of the University of California, San Diego and Dr. Vedha Nayagam of the National Center for Microgravity Research on Fluid and Combustion, the combustion of liquid fuel droplets having initial diameters between about 1 mm and 6 mm is being studied. The objectives of the work are to improve fundamental knowledge of droplet combustion dynamics through microgravity experiments and theoretical analyses. The Princeton contributions to the collaborative program supports the engineering design, data analysis, and data interpretation requirements for the study of initially single component, spherically symmetric, isolated droplet combustion studies through experiments and numerical modeling. The complementary UCSD contributions apply asymptotic theoretical analyses and are described in the published literature and in a companion communication in this volume. Emphases of the Princeton work are on the study of simple alcohols (methanol, ethanol), alcohol/water mixtures, and pure alkanes (n-heptane, n-decane) as fuels, with time dependent measurements of drop size, flame-stand-off, liquid-phase composition, and finally, extinction. Ground based experiments have included bench-scale studies at Princeton and collaborative experimental studies in the 2.2 and 5.18 second drop towers at NASA-Glenn Research Center. Spacelab studies have included fiber-supported droplet combustion (FSDC) experiments in the Glovebox facility with accompanying numerical analyses. Experiments include FSDC-1, performed on the USML-2 mission in October, 1995 (STS-73) and FSDC-2, on the second flight of the MSL-1 mission in July, 1997 (STS-94).

Dryer, F. L.↗

Comparison of Lagrangian Superdroplet and Eulerian Double-Moment Spectral Microphysics Schemes in Large-Eddy Simulations of an Isolated Cumulus Congestus Cloud

Abstract Advanced microphysics schemes (such as Eulerian bin and Lagrangian superdroplet) are becoming standard tools for cloud physics research and parameterization development. This study compares a double-moment bin scheme and a Lagrangian superdroplet scheme via large-eddy simulations of nonprecipitating and precipitating cumulus congestus clouds. Cloud water mixing ratio in the bin simulations is reduced compared to the Lagrangian simulations in the upper part of the cloud, likely from numerical diffusion, which is absent in the Lagrangian approach. Greater diffusion in the bin simulations is compensated by more secondary droplet activation (activation above cloud base), leading to similar or somewhat higher droplet number concentrations and smaller mean droplet radius than the Lagrangian simulations for the nonprecipitating case. The bin scheme also produces a significantly larger standard deviation of droplet radius than the superdroplet method, likely due to diffusion associated with the vertical advection of bin variables. However, the spectral width in the bin simulations is insensitive to the grid spacing between 50 and 100 m, suggesting other mechanisms may be compensating for diffusion as the grid spacing is modified. For the precipitating case, larger spectral width in the bin simulations initiates rain earlier and enhances rain development in a positive feedback loop. However, with time, rain formation in the superdroplet simulations catches up to the bin simulations. Offline calculations using the same drop size distributions in both schemes show that the different numerical methods for treating collision–coalescence also contribute to differences in rain formation. The stochastic collision–coalescence in the superdroplet method introduces more variability in drop growth for a given rain mixing ratio.

54 ENVIRONMENTAL SCIENCES↗

A wind tunnel investigation of the shape of uncharged raindrops in the presence of an external, electric field

Results of a wind tunnel experiment in which electrically uncharged water drops of 500 to 3000 microns equivalent radius are freely suspended in the vertical air stream of the UCLA cloud tunnel are presented. During this suspension the drops were exposed to external vertical electric fields of 500 to 8,000 volts/cm. The change in drop shape with drop size and electric field strength was noted and is discussed in the light of theoretical work cited in the literature which unfortunately does not take into account the effects of air flow past the drop. The wind tunnel study is documented by stills from a 16 mm film record that demonstrates the shape of water drops in response to both hydrodynamic and electric forces.

Pruppacher, H. R.↗

Particle diagnostics and turbulence measurements in a confined isothermal liquid spray

An experimental study of the behavior and structure of a liquid spray immersed in a strong swirling field is reported. In order to simulate some of the aerodynamic conditions experienced by a spray in a model combustor, an experimental setup using an acrylic chamber, a vane-type swirler, and separate air supplies for both the secondary air and swirl air were integrated to perform the experiments in the wind tunnel. The effect of the swirling flow on the original spray cone is to widen it substantially, and to provide a vortex core where intense mixing results in large changes in particle size distribution and in particle number density. Outside the recirculation region, both the D32 and N sub d attain more uniform values. Inside the recirculation region, the mean axial velocity averaged over all the drop sizes has larger values than the mean air velocity. Outside the recirculation region, both the particles and the air exhibit virtually the same velocities. The turbulence measurements showed regions of high turbulence intensity in the boundaries of the recirculation region.

Brena De La Rosa, A.↗