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At least 271 records · Page 15

Comparison of the CALIPSO Level 3 Ice Cloud Product with the DARDAR and 2C-ICE products

Understanding the vertical distribution of ice clouds is crucial for climate modeling and weather forecasting. Since its launch to space in 2006, the Cloud-Aerosol Lidar with Orthogonal Polarization instrument (CALIOP) onboard the CALIPSO spacecraft has been providing unprecedented high-quality profiles of ice clouds, especially optically thin cirrus clouds, during both day and night, on a global scale. Recently the lidar science working group at the NASA Langley Research Center delivered a level 3 (L3) ice cloud product which reports monthly statistics of ice cloud extinction coefficient and ice water content on a uniform 3-dimensional spatial grid. This presentation compares the ice cloud climatology derived from this product with two other ice cloud products, namely the raDAR/liDAR(DARDAR) ice cloud product and the CloudSat-CALIPSO Ice Cloud Property Product (2C-ICE). Using processing similar to the CALIPSO L3 product, granules of DARDAR and 2C-ICE data have been processed into monthly statistics for a better comparison. Similarities and differences will be presented and discussed. The findings illustrate the strengths of the different products and help to identify which product might be most appropriate for a given research topic.

Xia Cai↗

A Comparison of Stratospheric Smoke Events Seen by SAGE II (1984-2005) and SAGE III (2017-2021)

The Stratospheric Aerosol and Gas Experiment (SAGE II) operated for over 20 years (1984-2005) and collected near global observations of aerosol extinction coefficient from the upper troposphere to about40 km. SAGE III has flown aboard the International Space Station (ISS) since 2017 and has collected comparable aerosol measurements during this period. The SAGE II record is dominated by recovery from El Chichón (1982) and the Pinatubo eruption of 1991 with a few smaller volcanic events that are detectable in the data set. In addition, a number of pyrocumulus events injected smoke into the lower stratosphere with magnitudes that are comparable to the smaller volcanic events. The shorter SAGE III/ISS record is qualitatively different than SAGE II’s with a number of small to moderate volcanic eruptions in both low and high latitudes (e.g., Ambae in 2018 and Raikoke in 2020) as well several smokeevents including the two largest events seen by SAGE-like instruments: the BC pyrocumulus event in 2017 and the Australian brush fires of 2020/2021. In this paper, I will review the detection and quantification of the magnitude of these smoke events with a particular focus on the differences between the two data periods.

SAGE↗

Satellite-Based Evaluation of AeroCom Model Bias in Biomass Burning Regions

Global models are widely used to simulate biomass burning aerosol (BBA). Exhaustive evaluations on model representation of aerosol distributions and properties are fundamental to assess health and climate impacts of BBA. Here we conducted a comprehensive comparison of Aerosol Comparisons between Observations and Models (AeroCom) project model simulations with satellite observations. A total of 59 runs by 18 models from three AeroCom Phase-III experiments (i.e., biomass burning emissions, CTRL16, and CTRL19) and 14 satellite products of aerosols were used in the study. Aerosol optical depth (AOD) at 550 nm was investigated during the fire season over three key fire regions reflecting different fire dynamics (i.e., deforestation-dominated Amazon, Southern Hemisphere Africa where savannas are the key source of emissions, and boreal forest burning in boreal North America). The 14 satellite products were first evaluated against AErosol RObotic NETwork (AERONET) observations, with large uncertainties found. But these uncertainties had small impacts on the model evaluation that was dominated by modeling bias. Through a comparison with Polarization and Directionality of the Earth’s Reflectances measurements with the Generalized Retrieval of Aerosol and Surface Properties algorithm (POLDER-GRASP), we found that the modeled AOD values were biased by −93 % to 152 %, with most models showing significant underestimations even for the state-of-the-art aerosol modeling techniques (i.e., CTRL19). By scaling up BBA emissions, the negative biases in modeled AOD were significantly mitigated, although it yielded only negligible improvements in the correlation between models and observations, and the spatial and temporal variations in AOD biases did not change much. For models in CTRL16 and CTRL19, the large diversity in modeled AOD was in almost equal measures caused by diversity in emissions, lifetime, and the mass extinction coefficient (MEC). We found that in the AeroCom ensemble, BBA lifetime correlated significantly with particle deposition (as expected) and in turn correlated strongly with precipitation. Additional analysis based on Cloud-Aerosol LIdar with Orthogonal Polarization (CALIOP) aerosol profiles suggested that the altitude of the aerosol layer in the current models was generally too low, which also contributed to the bias in modeled lifetime. Modeled MECs exhibited significant correlations with the Ångström exponent (AE, an indicator of particle size). Comparisons with the POLDER-GRASP-observed AE suggested that the models tended to overestimate the AE (underestimated particle size), indicating a possible underestimation of MECs in models. The hygroscopic growth in most models generally agreed with observations and might not explain the overall underestimation of modeled AOD. Our results imply that current global models contain biases in important aerosol processes for BBA (e.g., emissions, removal, and optical properties) that remain to be addressed in future research.

biomass burning aerosols↗

A Comparison of Stratospheric Smoke Events Seen by SAGE II (1984-2005) and SAGE III (2017-2021)

The ongoing Stratospheric Aerosol and Gas Experiment aboard the International Space Station (SAGE III/ISS) has mostly occurred during a period of relatively low aerosol loading. At the same time, it has almost observed a number of small to moderate injections of volcanic material in the stratosphere from the Aoba/Ambae eruption of 2018 to that of Karymsky in 2022. In addition, two of the largest known smoke intrusions into the stratosphere have occurred during the SAGE III/ISS mission (the British Columbia fire of August 2017 and the Australian Wildfire Event of 2019/2020). At least two other much smaller smoke events have also been observed in the SAGE III data (California Creek in September 2020 and McKay Creek in June 2021). Particularly with the two large events, it is tempting to speculate that these events are increasing in intensity and frequency possibly due to ongoing climate change. Realistically, change is difficult to assess since instrument data sets that can be used for quantifying historical events can be quite different in what and where they provide measurements. This complicates comparing one event to another potentially separated by many years. An exception to this issues are the measurements by SAGE III/ISS and those of its predecessor SAGE II (1984-2005). Both use the same measurement strategy, measure aerosol extinction coefficient at 1020 nm, and have similar spatial/temporal coverage. Both instruments are known to observe smoke events in the stratosphere. However, both have the same low observation density characteristic of solar occultation such that near-global coverage takes almost a month and characterizing effectively instant events like smoke and volcanic events take a matter of weeks depending on the vagaries of where the observations are being made at a critical juncture unlike instruments with high temporal/spatial resolution like limb-scatter instruments such as OMPS and OSIRIS. The goal of this work will be to use the same analysis approach to both the SAGE II and SAGE III data and compare both the frequency and intensity of smoke events observed by these instruments. While we do not expect to be able to make conclusions about change between the periods, the analysis is a first step in interpreting changes in the contribution of smoke to the stratospheric aerosol budget between the time frames encompassed by these instruments.

L. W. Thomason↗

Polarimeter + Lidar Derived Aerosol Particle Number Concentration

In this study, we propose a simple method to derive vertically resolved aerosol particle number concentration (Na) using combined polarimetric and lidar remote sensing observations. This method relies on accurate polarimeter retrievals of the fine-mode column-averaged aerosol particle extinction cross section and accurate lidar measurements of vertically resolved aerosol particle extinction coefficient such as those provided by multiwavelength high spectral resolution lidar. We compare the resulting lidar + polarimeter vertically resolved Na product to in situ Na data collected by airborne instruments during the NASA aerosol cloud meteorology interactions over the western Atlantic experiment (ACTIVATE). Based on all 35 joint ACTIVATE flights in 2020, we find a total of 32 collocated in situ and remote sensing profiles that occur on 11 separate days, which contain a total of 322 cloud-free vertically resolved altitude bins of 150 m resolution. We demonstrate that the lidar + polarimeter Na agrees to within 106% for 90% of the 322 vertically resolved points. We also demonstrate similar agreement to within 121% for the polarimeter-derived column-averaged Na. We find that the range-normalized mean absolute deviation (NMAD) for the polarimeter-derived column-averaged Na is 21%, and the NMAD for the lidar + polarimeter-derived vertically resolved Na is 16%. Taken together, these findings suggest that the error in the polarimeter-only column-averaged Na and the lidar + polarimeter vertically resolved Na are of similar magnitude and represent a significant improvement upon current remote sensing estimates of Na.

Aerosol number concentration↗

The Tables of Aerosol Optics (TAO) Project

The Table of Aerosol Optics (TAO) project is a community repository of optics computations (extinction, absorption, single-scatter albedo, lidar ratio, etc) that are useful for global models and remote sensing applications. TAO expands upon historical efforts (e.g., Hess et al., 1998) by building an open database that uses recent measurements and new computational techniques for non-spherical particles. The ‘open’ aspect of TAO is important, since the size distributions, hygroscopicities, refractive indices, and morphological recommendations of today will undoubtedly yield to different values in the future; the open framework of TAO allows scientists to keep adding new computations to the database as the science evolves. TAO is meant to be a community repository where specialists can put their computations for other scientists to use. So for instance, some groups are advancing new techniques that can accommodate complex fractal aggregates of black carbon, other groups are working on realistic irregular shapes for mineral dust, and different groups are updating the hygroscopicity of various aerosol types using new techniques. The TAO database gives these scientists a place to distribute their products. As TAO grows, modelers and remote sensing specialists will look to TAO as a place to find a wide variety of choices for testing. Meanwhile, global modelers can also use TAO to lobby for new tables that accommodate their needs. Eventually, TAO will provide mass extinction coefficients, mass absorption coefficients, lidar ratios, etc., at popular remote sensing and global modeling wavelengths (0.25-40 µm) for all pertinent species (sulfate, sea salt, BC, OC, BrC, dust, etc.). TAO will also accept computations for aerosol ‘type’ (e.g., biomass burning, urban, background, etc.) that may include regional and seasonal variability. Multiple tables may be created for each species or type to account for the multiple valid size distributions, hygroscopicities, complex refractive indices, and shapes that can be found in the literature.

Greg Schuster↗

The PCM is Dead! Long Live O-PCM!

The ability to reconfigure the optical behavior of a device enables free-space applications ranging from imaging to sensing and signal control. Such optical devices can be compacted via meta-surfaces, patterned structures with feature sizes below the incident wavelength. Leveraging geometry in addition to material properties and CMOS fabrication techniques has allowed meta-surfaces for lenses, holograms, beam steerers and more. To incorporate multiple optical functions into one device, various methods of device control have been implemented, such as stretching of flexible substrates, tuning the refractive index of the comprising meta-atoms via the electro-optic or the thermo-optic effects, phase transition materials such as VO2 and more. Chalcogenide glasses used as optical phase change materials, such as Ge¬2Sb2Te5 (GST), have gained increased traction in the optics community for potential use in the near infrared (NIR) and mid infrared (MIR) bands, including the telecom bands. Various chalcogenides such as Sb2Se3, Sb2S3, Ge2Sb¬2Se5 and Ge2Sb2Se4Te (GSST) have been investigated due to their broad NIR or MIR transparency window and large changes in refractive index. In their amorphous phase, these materials usually display a lower refractive index and low absorption when compared to their crystalline state which display a higher refractive index and typically larger extinction coefficients. The amorphous-crystalline reversible switching can be done via fast melt-quenching thermal processes triggered by laser or electrical impulses, relying on a substrate as a heat sink. The potential of PCMs in photonic devices can be limited by intrinsic material limitations as well as by device fabrication issues. To explore the cyclability of GSST, a PCM with large refractive index contrast and on-chip electrothermal switching on a silicon-on-insulator platform has been done to analyze potential failure mechanisms from both a material and device perspective. A brief outline of the instrumentation and phase change contrast analysis is provided. Dewetting of the PCM, delamination of and damage in the PECVD SiNx protective layer, elemental migration in the PCM and optical contrast decay have been observed in cycled GSST devices. Guidelines for device performance improvement are proposed, and an improved design with larger endurance is shown in progress.

reconfigurable photonics↗

Polarimeter + Lidar–Derived Aerosol Particle Number Concentration

In this study, we propose a simple method to derive vertically resolved aerosol particle number concentration (Na) using combined polarimetric and lidar remote sensing observations. This method relies on accurate polarimeter retrievals of the fine-mode column-averaged aerosol particle extinction cross section and accurate lidar measurements of vertically resolved aerosol particle extinction coefficient such as those provided by multiwavelength high spectral resolution lidar. We compare the resulting lidar + polarimeter vertically resolved N(a) product to in situ N(a) data collected by airborne instruments during the NASA aerosol cloud meteorology interactions over the western Atlantic experiment (ACTIVATE). Based on all 35 joint ACTIVATE flights in 2020, we find a total of 32 collocated in situ and remote sensing profiles that occur on 11separate days, which contain a total of 322 cloud-free vertically resolved altitude bins of 150 m resolution. We demonstrate that the lidar + polarimeter N(a) agrees to within 106% for 90% of the 322 vertically resolved points. We also demonstrate similar agreement to within 121% for the polarimeter-derived column-averaged N(a). We find that the range-normalized mean absolute deviation (NMAD) for the polarimeter-derived column-averaged Na is 21%, and the NMAD for the lidar + polarimeter-derived vertically resolved Na is 16%. Taken together, these findings suggest that the error in the polarimeter-only column-averaged N(a) and the lidar + polarimeter vertically resolved N(a) are of similar magnitude and represent a significant improvement upon current remote sensing estimates of N(a).

RSP↗

Great Salt Lake Health and Air Quality: Monitoring Lakebed Exposure and its Impact on Air Quality and Environmental Hazards in the Great Salt Lake Watershed

Water flow into the Great Salt Lake has declined rapidly over the last forty years due to human withdrawals and climate change. As a result of declining lake levels, over 50% of the lakebed is now exposed. Dust storms may grow in frequency and intensity across Northern Utah as lakebed dust becomes airborne under specific meteorological conditions. In our research project, we utilized satellite imagery from Terra and Aqua, Sentinel-5P, CALIPSO, Landsat 5 TM, Landsat 7 ETM+, Landsat 8 OLI-2, Suomi NPP, ground sensor environmental data, and demographic data to understand the relationship between lake desiccation and dust, and the impact of pollution upon the communities surrounding the Great Salt Lake. By plotting changes in Lake Surface Area against Aerosol Optical Depth (AOD) over our study period (2010-2022), we found an inverse relationship (R2=0.3423) between lake surface area and dust levels within our study area. We conducted a Vertical Feature Mask (VFM) and Extinction Coefficient Plot, from which we identified that during dust events, the aerosol type is mainly polluted dust and the aerosol height is 200 meters from the surface. Lastly, we created bivariate choropleth maps, which demonstrate which census tracts within our study area are most vulnerable to AOD (a proxy for PM2.5 from dust), NO2 and HCHO (precursors to ozone). In summary, our findings revealed that declining lake levels are associated with an increase in intensity of dust events, and these dust events will particularly impact residents of Tooele County and the west side of Salt Lake City. Project resources support partner needs by informing targeted air monitoring efforts, lakebed management practices, and advocacy efforts for GSL stewardship.

Terminal Saline Lake↗

Quantifying SAGE II (1984-2005) and SAGE III/ISS (2017-2022) Observations of Smoke in the Stratosphere

The Stratospheric Aerosol and Gas Experiment (SAGE II) operated for over 20 years (1984-2005) and collected near global observations of aerosol extinction coefficient from the upper troposphere to about 40 km. SAGE III has flown aboard the International Space Station (ISS) since 2017 and has collected comparable aerosol measurements during this period. The SAGE II record is dominated by recovery from El Chichón (1982) and the Pinatubo eruption of 1991 with a few smaller volcanic events that are detectable in the data set. In addition, a number of pyrocumulus events injected smoke into the lower stratosphere with magnitudes that are comparable to the smaller volcanic events. The shorter SAGE III/ISS record is qualitatively different than SAGE II’s with a number of small to moderate volcanic eruptions in both low and high latitudes (e.g., Ambae in 2018 and Raikoke in 2020) as well several smoke events including the two largest events seen by SAGE-like instruments: the BC pyrocumulus event in 2017 and the Australian brush fires of 2020/2021. In this paper, I will review the detection and quantification of the magnitude of these smoke events with a particular focus on the differences between the two data periods.

Smoke↗

The Tables of Aerosol Optics (TAO) Project

The Table of Aerosol Optics (TAO) project is a community repository of optics computations (extinction, absorption, single-scatter albedo, lidar ratio, etc) that are useful for global models and remote sensing applications. TAO expands upon historical efforts (e.g., Hess et al., 1998) by building an open database that uses recent measurements and new computational techniques for non-spherical particles. The ‘open’ aspect of TAO is important, since the size distributions, hygroscopicities, refractive indices, and morphological recommendations of today will undoubtedly yield to different values in the future; the open framework of TAO allows scientists to keep adding new computations to the database as the science evolves. TAO is meant to be a community repository where specialists can put their computations for other scientists to use. So for instance, some groups are advancing new techniques that can accommodate complex fractal aggregates of black carbon, other groups are working on realistic irregular shapes for mineral dust, and different groups are updating the hygroscopicity of various aerosol types using new techniques. The TAO database gives these scientists a place to distribute their products. As TAO grows, modelers and remote sensing specialists will look to TAO as a place to find a wide variety of choices for testing. Meanwhile, global modelers can also use TAO to lobby for new tables that accommodate their needs. Eventually, TAO will provide mass extinction coefficients, mass absorption coefficients, lidar ratios, etc., at popular remote sensing and global modeling wavelengths (0.25-40 µm) for all pertinent species (sulfate, sea salt, BC, OC, BrC, dust, etc.). TAO will also accept computations for aerosol ‘type’ (e.g., biomass burning, urban, background, etc.) that may include regional and seasonal variability. Multiple tables may be created for each species or type to account for the multiple valid size distributions, hygroscopicities, complex refractive indices, and shapes that can be found in the literature.

Elisabeth Andrews↗

Quantifying SAGE II (1984-2005) and SAGE III/ISS (2017-2022) Observations of Smoke in the Stratosphere

The Stratospheric Aerosol and Gas Experiment (SAGE II) operated for over 20 years (1984-2005) and collected near global observations of aerosol extinction coefficient from the upper troposphere to about 40 km. SAGE III has flown aboard the International Space Station (ISS) since 2017 and has collected comparable aerosol measurements during this period. The SAGE II record is dominated by recovery from El Chichón (1982) and the Pinatubo eruption of 1991 with a few smaller volcanic events that are detectable in the data set. In addition, a number of pyrocumulus events injected smoke into the lower stratosphere with magnitudes that are comparable to the smaller volcanic events. The shorter SAGE III/ISS record is qualitatively different than SAGE II’s with a number of small to moderate volcanic eruptions in both low and high latitudes (e.g., Ambae in 2018 and Raikoke in 2020) as well several smoke events including the two largest events seen by SAGE-like instruments: the BC pyrocumulus event in 2017 and the Australian brush fires of 2020/2021. In this talk, I will review the detection and quantification of the magnitude of these smoke events with a particular focus on the differences between the two data periods.

Smoke Stratosphere SAGE↗

Sage III/ISS Stratospheric Aerosols and Gas Experiment An Earth Science Mission on the International Space Station

Stratospheric aerosols play key roles in the chemistry and radiation balance of the atmosphere and are a key input parameter for global chemistry and climate models. The degree to which aerosols impact chemistry and radiation balance depends primarily on the relative abundance of different sized particles within the sample volume, often referred to as the particle size distribution (PSD). If the PSD is accurately known then other key modeling parameters (e.g., surface area density and effective radius) can be derived. Historically, occultation observations from orbital instruments such as SAGE III/ISS have been used to infer these PSD parameters by inverting the extinction coefficient spectra. However, past efforts routinely failed to account for measurement uncertainty and lacked a rigorous estimate of the inferred PSD uncertainty. We developed a PSD solution algorithm that infers single mode and bimodal distribution parameters and applied this algorithm to the SAGE II and SAGE III/ISS data record. Herein we describe the algorithm, evaluate its performance, and show results from the 2022 Hunga Tonga eruption.

Travis N. Knepp↗

Quantifying SAGE II (1984-2005) and SAGE III/ISS (2017-2022) Observations of Smoke in the Stratosphere

The Stratospheric Aerosol and Gas Experiment (SAGE II) operated for over 20 years (1984-2005) and collected near global observations of aerosol extinction coefficient from the upper troposphere to about 40 km. SAGE III has flown aboard the International Space Station (ISS) since 2017 and has collected comparable aerosol measurements during this period. The SAGE II record is dominated by recovery from El Chichón (1982) and the Pinatubo eruption of 1991 with a few smaller volcanic events that are detectable in the data set. In addition, a number of pyrocumulus events injected smoke into the lower stratosphere with magnitudes that are comparable to the smaller volcanic events. The shorter SAGE III/ISS record is qualitatively different than SAGE II’s with a number of small to moderate volcanic eruptions in both low and high latitudes (e.g., Ambae in 2018 and Raikoke in 2020) as well several smoke events including the two largest events seen by SAGE-like instruments: the BC pyrocumulus event in 2017 and the Australian brush fires of 2020/2021. In this talk, I will review the detection and quantification of the magnitude of these smoke events with a particular focus on the differences between the two data periods.

SAGE↗

The Tables of Aerosol Optics (TAO) Project

The Table of Aerosol Optics (TAO) project is a community repository of optics computations (extinction, absorption, single-scatter albedo, lidar ratio, etc) that are useful for global models and remote sensing applications. TAO expands upon historical efforts (e.g., Hess et al., 1998) by building an open database that uses recent measurements and new computational techniques for non-spherical particles. The ‘open’ aspect of TAO is important, since the size distributions, hygroscopicities, refractive indices, and morphological recommendations of today will undoubtedly yield to different values in the future; the open framework of TAO allows scientists to keep adding new computations to the database as the science evolves. TAO is meant to be a community repository where specialists can put their computations for other scientists to use. So for instance, some groups are advancing new techniques that can accommodate complex fractal aggregates of black carbon, other groups are working on realistic irregular shapes for mineral dust, and different groups are updating the hygroscopicity of various aerosol types using new techniques. The TAO database gives these scientists a place to distribute their products. As TAO grows, modelers and remote sensing specialists will look to TAO as a place to find a wide variety of choices for testing. Meanwhile, global modelers can also use TAO to lobby for new tables that accommodate their needs. Eventually, TAO will provide mass extinction coefficients, mass absorption coefficients, lidar ratios, etc., at popular remote sensing and global modeling wavelengths (0.25-40 µm) for all pertinent species (sulfate, sea salt, BC, OC, BrC, dust, etc.). TAO will also accept computations for aerosol ‘type’ (e.g., biomass burning, urban, background, etc.) that may include regional and seasonal variability. Multiple tables may be created for each species or type to account for the multiple valid size distributions, hygroscopicities, complex refractive indices, and shapes that can be found in the literature.

Greg Schuster↗

An Empirical Characterization of the Aerosol Angstrom Exponent Interpolation Bias using SAGE III/ISS Data

This work uses multispectral measurements of vertically resolved aerosol extinction coefficients from the Stratospheric Aerosol and Gas Experiment (SAGE) III on the International Space Station (ISS) to demonstrate how the use of the Ångström exponent for interpolation of aerosol data between two different wavelengths creates a bias. An empirical relationship is derived between the magnitude of this bias and the Ångström exponent at several different SAGE wavelengths. This relationship can thus be used as a correction factor for other studies, such as multi-instrument intercomparisons or merging, that wish to convert aerosol data from one wavelength to another using the Ångström exponent and is applicable to all stratospheric non-cloud aerosol except highly aged particles that are evaporating at altitudes above the Junge layer.

Aerosol↗

Radiative transfer theory for inhomogeneous media with random extinction and scattering coefficients

The small-angle scattering approximation of the scalar radiative transfer equation (RTE) is examined for the case where the extinction and scattering coefficients have a component that is a deterministic function of position along the propagation path and a component that is a random function of position transverse to the propagation direction. It is found that the resulting stochastic RTE can be reduced to a system of two stochastic integrodifferential equations for the average and fluctuating components of the radiant intensity. Two transfer equations are obtained describing the average radiant intensity and the spatial correlation function of the intensity fluctuations. The average intensity equation is then solved and applied to a simple propagation scenario. An approximate solution is also derived for the equation giving the correlation function. The developed equations can be applied to problems involving short wavelength electromagnetic wave propagation through media possessing the variable characteristics of turbulence and turbidity, such as plasmas, the atmosphere, and the ocean.

Manning, Robert M.↗

A model predicting the evolution of ice particle size spectra and radiative properties of cirrus clouds. Part 2: Dependence of absorption and extinction on ice crystal morphology

This study builds upon the microphysical modeling described in Part 1 by deriving formulations for the extinction and absorption coefficients in terms of the size distribution parameters predicted from the micro-physical model. The optical depth and single scatter albedo of a cirrus cloud can then be determined, which, along with the asymmetry parameter, are the input parameters needed by cloud radiation models. Through the use of anomalous diffraction theory, analytical expressions were developed describing the absorption and extinction coefficients and the single scatter albedo as functions of size distribution parameters, ice crystal shapes (or habits), wavelength, and refractive index. The extinction coefficient was formulated in terms of the projected area of the size distribution, while the absorption coefficient was formulated in terms of both the projected area and mass of the size distribution. These properties were formulated as explicit functions of ice crystal geometry and were not based on an 'effective radius.' Based on simulations of the second cirrus case study described in Part 1, absorption coefficients predicted in the near infrared for hexagonal columns and rosettes were up to 47% and 71% lower, respectively, than absorption coefficients predicted by using equivalent area spheres. This resulted in single scatter albedos in the near-infrared that were considerably greater than those predicted by the equivalent area sphere method. Reflectances in this region should therefore be underestimated using the equivalent area sphere approach. Cloud optical depth was found to depend on ice crystal habit. When the simulated cirrus cloud contained only bullet rosettes, the optical depth was 142% greater than when the cloud contained only hexagonal columns. This increase produced a doubling in cloud albedo. In the near-infrared (IR), the single scatter albedo also exhibited a significant dependence on ice crystal habit. More research is needed on the geometrical properties of ice crystals before the influence of ice crystal shape on cirrus radiative properties can be adequately understood. This study provides a way of coupling the radiative properties of absorption, extinction, and single scatter albedo to the microphysical properties of cirrus clouds. The dependence of extinction and absorption on ice crystal shape was not just due to geometrical differences between crystal types, but was also due to the effect these differences had on the evolution of ice particle size spectra. The ice particle growth model in Part 1 and the radiative properties treated here are based on analytical formulations, and thus represent a computationally efficient means of modeling the microphysical and radiative properties of cirrus clouds.

Mitchell, David L.↗