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DOE OSTI2025

Improving vertical detail in simulated temperature and humidity data using machine learning

Atmospheric models used for weather forecasting and climate predictions discretise the atmosphere onto a vertical grid. There are however atmospheric phenomena that occur on scales smaller than the thickness of those model layers. The formation of low-level clouds due to temperature inversions is an example. This leads to atmospheric models underestimating, or even missing, these clouds and their radiative effects. Using radiosonde observations as training data, a machine learning model is used to improve the vertical detail of modelled profiles of temperature and specific humidity. In addition, a physics-informed machine learning model is developed and compared to the traditional approach; showing improvements in the cloud fraction profiles calculated from its predictions. The vertically enhanced profiles also improve the representation of layers of convective inhibition and anomalous refractivity gradients. This work facilitates targeted improvements to the representation of certain atmospheric processes without the burden of increased memory and computational cost from increasing vertical resolution throughout the whole model.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2007

Comparison of Water Vapor Measurements by Airborne Sun Photometer and Near-Coincident in Situ and Satellite Sensors during INTEX/ITCT 2004

We have retrieved columnar water vapor (CWV) from measurements acquired by the 14-channel NASA Ames Airborne Tracking Sun photometer (AATS-14) during 19 Jetstream 31 (J31) flights over the Gulf of Maine in summer 2004 in support of the Intercontinental Chemical Transport Experiment (INTEX)/Intercontinental Transport and Chemical Transformation (ITCT) experiments. In this paper we compare AATS-14 water vapor retrievals during aircraft vertical profiles with measurements by an onboard Vaisala HMP243 humidity sensor and by ship radiosondes and with water vapor profiles retrieved from AIRS measurements during eight Aqua overpasses. We also compare AATS CWV and MODIS infrared CWV retrievals during five Aqua and five Terra overpasses. For 35 J31 vertical profiles, mean (bias) and RMS AATS-minus-Vaisala layer-integrated water vapor (LWV) differences are -7.1 percent and 8.8 percent, respectively. For 22 aircraft profiles within 1 hour and 130 km of radiosonde soundings, AATS-minus-sonde bias and RMS LWV differences are -5.4 percent and 10.7 percent, respectively, and corresponding J31 Vaisala-minus-sonde differences are 2.3 percent and 8.4 percent, respectively. AIRS LWV retrievals within 80 lan of J31 profiles yield lower bias and RMS differences compared to AATS or Vaisala retrievals than do AIRS retrievals within 150 km of the J31. In particular, for AIRS-minus-AATS LWV differences, the bias decreases from 8.8 percent to 5.8 percent, and the RMS difference decreases from 2 1.5 percent to 16.4 percent. Comparison of vertically resolved AIRS water vapor retrievals (LWVA) to AATS values in fixed pressure layers yields biases of -2 percent to +6 percent and RMS differences of -20 percent below 700 hPa. Variability and magnitude of these differences increase significantly above 700 hPa. MODIS IR retrievals of CWV in 205 grid cells (5 x 5 km at nadir) are biased wet by 10.4 percent compared to AATS over-ocean near-surface retrievals. The MODIS-Aqua subset (79 grid cells) exhibits a wet bias of 5.1 percent, and the MODIS-Terra subset (126 grid cells) yields a wet bias of 13.2 percent.

Livingston, J.↗

NASA NTRS2019

The Effects of a 1998 Observing System Change on MERRA-2-Based Ozone Profile Simulations

Model simulations of ozone (O3) driven by meteorological reanalyses are useful for filling observational gaps and interpreting observed O3 variability and trends. However, the transport circulation of reanalysis products is impacted by changes to the observing system (the data assimilated into the reanalyses). We examine the impacts of these changes on simulated O3 from two models, Global Modeling Initiative (GMI) Chemistry Transport Model (GMI CTM) and Modern‐Era Retrospective Analysis for Research Applications version 2 (MERRA‐2) GMI Replay (M2 GMI Replay) simulation, using observations from global ozonesondes (>50,000 profiles) and satellites from 1980 to 2016. Both models are constrained by meteorology from the NASA MERRA‐2 reanalysis, and both use versions of NASA's GMI chemical mechanism. We focus on an observing system change affecting simulated O3 after 1998, associated with the assimilation of temperature and humidity data from new microwave profiling satellites. A large post‐1998 O3 increase, mainly confined to 15–20‐km altitude, of ~10 Dobson units (DU) in midlatitudes occurs in the GMI CTM, worsening the bias compared to observations. In contrast, an increase in M2 GMI Replay simulation O3 of ~10 DU is observed only near −60° latitude, reducing the bias compared to observations. The GMI CTM O3 high biases display a Quasi‐Biennial Oscillation (QBO)‐like periodicity that result from excessive transport from the tropical stratosphere to the midlatitude lower stratosphere during the QBO westerly phase. We quantify O3 discontinuities caused by MERRA‐2 observing system changes and demonstrate how the MERRA‐2 Global Modeling Initiative Replay simulation dampens the effects of these changes and QBO‐driven artifacts on simulated lower stratospheric and total O3. We caution against using simulations driven by a reanalysis to derive multidecadal O3 trends, especially prior to 1998.

Replay↗

NASA NTRS2002

Moisture Advection and Fresh Water Flux over Oceans

Moisture transport in the atmosphere is one of the most significant components in the hydrological cycle. Under stationary condition, ocean surface fresh water flux, which is the difference between precipitation (P) and evaporation (E), is balanced by the divergence of column-integrated moisture transport (IMT) in the atmosphere. Characterizing accurately a global picture of IMT from observation is a difficult task. It requires measurements of vertical profiles for wind vector and humidity. More specifically, IMT can be defined as the integration in pressure coordinates the product of specific humidity q and wind vector u, where g is the gravitational acceleration, and p, is the atmospheric pressure at ocean surface.In this study, a statistical relationship is derived between u, and u(sub)s using data from numerical weather prediction model. The relationship is then validated using surface and vertical profile from radiosonde data, before applied to spacebased measurements.

scatterometers↗

NASA NTRS2002

SHADOZ (Southern Hemisphere ADditional Ozonesondes): What Have We Learned About Tropical Tropospheric Ozone from the First Three Years' (1998-2000) Data?

The first climatological overview of total, stratospheric and tropospheric ozone in the southern hemisphere tropical and subtropics is based on ozone sounding data from 10 sites comprising the Southern Hemisphere Additional OZonesondes (SHADOZ) network. The period covered is 1998-2000. Observations were made over: Ascension Island; Nairobi, Kenya; Irene, South Africa; RCunion Island; Watukosek, Java; Fiji; Tahiti; American Samoa; San Cristobal, Galapagos; Natal, Brazil. Campaign data were collected on a trans-Atlantic oceanographic cruise and during SAFARI-2000 in Zambia. The ozone data, with simultaneous temperature profiles to approx. 7 hPa and relative humidity to approx. 200 hPa, reside at: . SHADOZ ozone time-series and profiles give a perspective on tropical total, stratospheric and tropospheric ozone in 1998-2000. Prominent features are highly variable tropospheric ozone, a zonal wave-one pattern in total (and tropospheric) column ozone, and signatures of the Quasi-Biennial Oscillation (QBO) in stratospheric ozone. Total, stratospheric and tropospheric column ozone amounts peak between August and November and are lowest between March and May. Tropospheric ozone variability over the Indian and Pacific Ocean displays influences of the Indian Ocean Dipole, and convective mixing. Pollution transport from Africa, South American and the Maritime Continent is a seasonal feature. Tropospheric ozone seasonality over the Atlantic Basin shows effects of regional subsidence and recirculation as well as biomass burning. Dynamical and chemical influences appear to be of comparable magnitude though model studies are needed to quantify this.

Thompson, Anne M.↗

NASA NTRS2002

SHADOZ (Southern Hemisphere ADditional Ozonesondes}: What Have We Learned About Tropical Tropospheric Ozone from the First Three Years (1998-2000) Data

The first climatological overview of total, stratospheric and tropospheric ozone in the southern hemisphere tropical and subtropics is based on ozone sounding data from 10 sites comprising the Southern Hemisphere Additional OZonesondes (SHADOZ) network. The period covered is 1998-2000. Observations were made over: Ascension Island; Nairobi, Kenya; Irene, South Africa; Reunion Island; Watukosek, Java; Fiji; Tahiti; American Samoa; San Cristobal, Galapagos; Natal, Brazil. Campaign data were collected on an Trans-Atlantic oceanographic cruise and during SAFARI-2000 in Zambia. The ozone data, with simultaneous temperature profiles to approximately 7 hPa and relative humidity to approximately 200 hPa, reside at: . SHADOZ ozone time-series and profiles give a perspective on tropical total, stratospheric and tropospheric ozone in 1998-2000. Prominent features are highly variable tropospheric ozone, a zonal wave-one pattern in total (and tropospheric) column ozone, and signatures of the Quasi-Biennial Oscillation (QBO) in stratospheric ozone. Total, stratospheric and tropospheric column ozone amounts peak between August and November and are lowest between March and May. Tropospheric ozone variability over the Indian and Pacific Ocean displays influences of the Indian Ocean Dipole, and convective mixing. Pollution transport from Africa, South American and the Maritime Continent is a seasonal feature. Tropospheric ozone seasonality over the Atlantic Basin shows effects of regional subsidence and recirculation as well as biomass burning. Dynamical and chemical influences appear to be of comparable magnitude though model studies are needed to quantify this.

Thompson, Anne M.↗

NASA NTRS2002

Tropical Tropospheric Ozone from SHADOZ (Southern Hemisphere ADditional Ozonesondes) Network: A Project for Satellite Research, Process Studies, Education

The first climatological overview of total, stratospheric and tropospheric ozone in the southern hemisphere tropical and subtropics is based on ozone sounding data from 10 sites comprising the Southern Hemisphere Additional OZonesondes (SHADOZ) network. The period covered is 1998-2000. Observations were made over: Ascension Island; Nairobi, Kenya; Irene, South Africa; Reunion Island; Watukosek, Java; Fiji; Tahiti; American Samoa; San Cristobal, Galapagos; Natal, Brazil. Campaign data were collected on a trans-Atlantic oceanographic cruise and during SAFARI-2000 in Zambia. The ozone data, with simultaneous temperature profiles to approx. 7 hPa and relative humidity to approx. 200 hPa, reside at: . SHADOZ ozone time-series and profiles give a perspective on tropical total, stratospheric and tropospheric ozone. Prominent features are highly variable tropospheric ozone and a zonal wave-one pattern in total (and tropospheric) column ozone. Total, stratospheric and tropospheric column ozone amounts peak between August and November and are lowest between March and May. Tropospheric ozone variability over the Indian and Pacific Ocean displays influences of the Indian Ocean Dipole and convective mixing. Pollution transport from Africa and South America is a seasonal feature. Tropospheric ozone seasonality over the Atlantic Basin shows effects of regional subsidence and recirculation as well as biomass burning. Dynamical and chemical influences appear to be of comparable magnitude though model studies are needed to quantify this.

Thompson, Anne M.↗

NASA NTRS1984

Radiosonde pressure sensor performance - Evaluation using tracking radars

The standard balloon-borne radiosonde employed for synoptic meteorology provides vertical profiles of temperature, pressure, and humidity as a function of elapsed time. These parameters are used in the hypsometric equation to calculate the geopotential altitude at each sampling point during the balloon's flight. It is important that the vertical location information be accurate. The present investigation was conducted with the objective to evaluate the altitude determination accuracy of the standard radiosonde throughout the entire balloon profile. The tests included two other commercially available pressure sensors to see if they could provide improved accuracy in the stratosphere. The pressure-measuring performance of standard baroswitches, premium baroswitches, and hypsometers in balloon-borne sondes was correlated with tracking radars. It was found that the standard and premium baroswitches perform well up to about 25 km altitude, while hypsometers provide more reliable data above 25 km.

Parsons, C. L.↗

NASA NTRS2016

MISTiC Winds, a Micro-Satellite Constellation Approach to High Resolution Observations of the Atmosphere Using Infrared Sounding and 3D Winds Measurements

MISTiC(TM) Winds is an approach to improve short-term weather forecasting based on a miniature high resolution, wide field, thermal emission spectrometry instrument that will provide global tropospheric vertical profiles of atmospheric temperature and humidity at high (3-4 km) horizontal and vertical ( 1 km) spatial resolution. MISTiCs extraordinarily small size, payload mass of less than 15 kg, and minimal cooling requirements can be accommodated aboard a 27U-class CubeSat or an ESPA-Class micro-satellite. Low fabrication and launch costs enable a LEO sunsynchronous sounding constellation that would collectively provide frequent IR vertical profiles and vertically resolved atmospheric motion vector wind observations in the troposphere. These observations are highly complementary to present and emerging environmental observing systems, and would provide a combination of high vertical and horizontal resolution not provided by any other environmental observing system currently in operation. The spectral measurements that would be provided by MISTiC Winds are similar to those of NASA's AIRS that was built by BAE Systems and operates aboard the AQUA satellite. These new observations, when assimilated into high resolution numerical weather models, would revolutionize short-term and severe weather forecasting, save lives, and support key economic decisions in the energy, air transport, and agriculture arenasat much lower cost than providing these observations from geostationary orbit. In addition, this observation capability would be a critical tool for the study of transport processes for water vapor, clouds, pollution, and aerosols. Key remaining technical risks are being reduced through laboratory and airborne testing under NASA's Instrument Incubator Program.

Maschhoff, K. R.↗

NASA NTRS2006

Moisture correspondence between lower and upper troposphere over oceans using AIRS observations

The Atmospheric Infrared Sounder (AIRS) mounted on Aqua space craft measures vertical profiles of air temperature and humidity using both microwaves and infrared irradiance. The AIRS' level III data that provide gridded values of 1(sup o) latitude by 1(sup o) longitude for the highest temporal resolution of twice per day became available recently (Granger et al. 2005). This level III data were derived from the level II Version 4.0 AIRS retrieval algorithm. This study uses this level III AIRS moisture profile data to reveal geographical correspondences of atmospheric moisture content between the lower and upper troposphere.

Ye, Hengchun↗

NASA NTRS2023

Influence of Lower Tropospheric Moisture on Local Soil Moisture-Precipitation Feedback Over the U.S. Southern Great Plains

Land-atmosphere coupling (LAC) has long been studied focusing on land surface and atmospheric boundary layer processes. However, the influence of lower tropospheric (LT) humidity on LAC remains largely unexplored. In this study, we use radiosonde observations from the U.S. Southern Great Plains (SGP) site and an entrained parcel buoyancy model to investigate the impact of LT humidity on LAC there during the warm season (May–September). We quantify the effect of LT humidity on convective buoyancy by measuring the difference between the 2–4 km vertically integrated buoyancy with and without the influence of background LT humidity. Our results show that, under dry soil conditions, anomalously high LT humidity is necessary to produce the buoyancy profiles required for afternoon precipitation events (APEs). These APEs under dry soil moisture cannot be explained by commonly used local land-atmosphere coupling indices such as the convective triggering potential/low-level humidity index (CTP/HI Low ), which do not account for the influence of the LT humidity. On the other hand, consideration of LT humidity is unnecessary to explain APEs under wet soil moisture conditions, suggesting the boundary layer moisture alone could be sufficient to generate the required buoyancy profiles. These findings highlight the need to consider the impact of LT humidity, which is often decoupled from the humidity near the surface and largely controlled by moisture transport, in understanding land-atmospheric feedbacks over dry soil conditions, especially during droughts or dry spells over the SGP.

Gaoyun Wang↗

NASA NTRS2001

SHADOZ (Southern Hemisphere ADditional Ozonesondes): A Look at the First Three Years' (1998-2000) Tropospheric Ozone Data

The first climatological overview of total, stratospheric and tropospheric ozone in the southern hemisphere tropical and subtropics is based on ozone sounding data from 10 sites comprising the Southern Hemisphere ADditional OZonesondes (SHADOZ) network. The period covered is 1998-2000. Observations were made over: Ascension Island; Nairobi, Kenya; Irene, South Africa; RCunion Island; Watukosek, Java; Fiji; Tahiti; American Samoa; San Cristobal, Galapagos; Natai, Brazil. Campaign data were collected on a trans-Atlantic oceanographic cruise and during SAFARI-2000 in Zambia. The ozone data, with simultaneous temperature profiles to approx. 7 hPa and relative humidity to approx. 200 hPa, reside at an open archive: . SHADOZ ozone time-series and profiles give a perspective on tropical total, stratospheric and tropospheric ozone in 1998-2000. Prominent features are highly variable tropospheric ozone, a zonal wave-one pattern in total (and tropospheric) column ozone, and signatures of the Quasi-Biennial Oscillation (QBO) in stratospheric ozone. Total, stratospheric and tropospheric column ozone amounts peak between August and November and are lowest between March and May. Tropospheric ozone variability over the Indian and Pacific Ocean displays influences of the Indian Ocean Dipole, ENSO, and Madden-Julian circulation on convective mixing. Pollution transport from Africa, South American and the Maritime Continent is a seasonal feature. Tropospheric ozone seasonality over the Atlantic Basin shows effects of regional subsidence and recirculation as well as biomass burning. Dynamical and chemical influences appear to be of comparable magnitude.

Thompson, Anne M.↗

DOE OSTI2025

Operando Neutron Imaging of Reaction Extent and Particle Swelling Informs Limiting Factors for Salt Hydrate Thermochemical Energy Storage

Salt hydrates are a promising thermochemical energy storage medium that stores heat through the reversible uptake (hydration) and release (dehydration) of water vapor. Our study deploys operando neutron imaging to investigate salt hydrate performance with high spatial resolution (42 μm pixels). For flow over a packed bed with diffusion-driven transport, measurements reveal the formation of a solid diffusion layer due to particle swelling for the pure SrBr2 salt. In contrast, the SrBr2–vermiculite composite exhibits significantly less swelling and more than a 2-fold increase in the apparent water vapor diffusivity. For axial flow through a packed bed, neutron imaging confirms theoretically predicted transitions from a moving reaction front to a homogeneous profile with an increase in humid air flow rate. Our study establishes neutron imaging as a powerful technique to advance fundamental understanding of thermochemical systems and help guide composite material design.

Kinzer, Bryan [ORNL] (ORCID:0000000337804910)↗

NASA NTRS1976

Advanced atmospheric sounder and imaging radiometer /AASIR/ for STORMSAT

The principal mission of the three-axis stabilized STORMSAT spacecraft is to provide the necessary meteorological data for tracking, studying the detailed structure, and modeling mesoscale weather phenomena. In the area of mesoscale events, the following meteorological objectives are indicated: high-quality imagery, visible and infrared; wind velocity from cloud tracers (1 m/sec), atmospheric temperature profiles (1 K), and atmospheric humidity sounding. These objectives are reflected in the functional characteristics of the AASIR, which is a second generation meteorological sensor based on the Visible Infrared Spin-Scan Radiometer (VISSR) and the Atmospheric Sounder (VAS). The AASIR design and interface constraints with the STORMSAT spacecraft is discussed.

Chase, S. C.↗

NASA NTRS1980

Weather and climate needs for Lidar observations from space and concepts for their realization

The spectrum of weather and climate needs for Lidar observations from space is discussed with emphasis on the requirements for wind, temperature, moisture, and pressure data. It is shown that winds are required to realistically depict all atmospheric scales in the tropics and the smaller scales at higher latitudes, where both temperature and wind profiles are necessary. The need for means to estimate air-sea exchanges of sensible and latent heat also is noted. A concept for achieving this through a combination of Lidar cloud top heights and IR cloud top temperatures of cloud streets formed during cold air outbreaks over the warmer ocean is outlined. Recent theoretical feasibility studies concerning the profiling of temperatures, pressure, and humidity by differential absorption Lidar (DIAL) from space and expected accuracies are reviewed. An alternative approach to Doppler Lidar wind measurements also is presented. The concept involves the measurement of the displacement of the aerosol backscatter pattern, at constant heights, between two successive scans of the same area, one ahead of the spacecraft and the other behind it a few minutes later. Finally, an integrated space Lidar system capable of measuring temperature, pressure, humidity, and winds which combines the DIAL methods with the aerosol pattern displacement concept is described.

Atlas, D.↗

NASA NTRS1981

Weather and climate needs for lidar observations from space and concepts for their realization

The spectrum of weather and climate needs for lidar observations from space is discussed. This paper focuses mainly on the requirements for winds, temperature, moisture, and pressure. Special emphasis is given to the need for wind observations, and it is shown that winds are required to depict realistically all atmospheric scales in the tropics and the smaller scales at higher latitudes, where both temperature and wind profiles are necessary. The need for means to estimate air-sea exchanges of sensible and latent heat also is noted. Lidar can aid here by measurement of the slope of the boundary layer. Recent theoretical feasibility studies concerning the profiling of temperature, pressure, and humidity by differential absorption lidar (DIAL) from space and expected accuracies are reviewed. Initial ground-based trials provide support for these approaches and also indicate their direct applicability to path-average temperature measurements near the surface. An alternative approach to Doppler lidar wind measurements also is presented. The concept involves the measurement of the displacement of the aerosol backscatter pattern, at constant height, between two successive scans of the same area, one ahead of the spacecraft and the other behind it, a few minutes later. Finally, an integrated space lidar system capable of measuring temperature, pressure, humidity, and winds which combines the DIAL methods with the aerosol pattern displacement concept is described briefly.

Atlas, D.↗

NASA NTRS1987

A multifrequency microwave radiometer of the future

The design of the High-Resolution Multifrequency Microwave Radiometer (HMMR), which is to be installed on EOS, is described. The HMMR is to consist of the Advanced Microwave Sounding Unit (AMSU), the Advanced Mechanically Scanned Radiometer (AMSR), and the Electronically Scanned Thinned Array Radiometer (ESTAR). The AMSU is a 20-channel microwave radiometer system designed to measure profiles of atmospheric temperature and humidity and the AMSR is a microwave imager with channels at 6, 10, 18, 21, 37, and 90 GHz for measuring snow cover over land, the age and areal extent of sea ice, the intensity of precipitation over oceans and land, and the amount of water in the atmosphere. ESTAR is an imaging radiometer operating near 1.4 GHz capable of obtaining global maps of surface soil moisture with a spatial resolution of about 10 km. The antenna and signal processing utilized in the ESTAR to achieve the real aperture resolution are examined.

Le Vine, D.↗

NASA NTRS1988

Aerosol measurements in the winter/spring Antarctic stratosphere. I - Correlative measurements with ozone. II - Impact on polar stratospheric cloud theories

Aerosol measurements collected from August 25-November 3, 1986 at McMurdo Station using balloon-borne optical particle counters are examined in order to study the relationship between aerosol and ozone distribution and the formation of polar stratospheric clouds (PSCs). Ozone, aerosol, and condensation nuclei profiles, and pressure, temperature, and humidity measurements are analyzed. It is observed that the height of the stratospheric sulfate layer decreases over the period of measurement suggesting that upwelling in the votex is not important in the zone depletion process. Three theories on PSC formation are described, and the effects of the aerosol measurements on the theories are considered. The three theories are: (1) the original theory of water vapor pressure over a solution of H2SO4 of Steele et al. (1983) and Hamill and Mc Master (1984); (2) the nitric acid theory of PSCs of Toon et al. (1986) and Hamill et al. (1986); and (3) the quasi-cirrus cloud theory of Heymsfield (1986).

Hofmann, D. J.↗