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DOE OSTI2022

Magnetized laser–plasma interactions in high-energy-density systems: Parallel propagation

In this study, we investigate parametric processes in magnetized plasmas, driven by a large-amplitude pump light wave. Our focus is on laser–plasma interactions relevant to high-energy-density (HED) systems, such as the National Ignition Facility and the Sandia MagLIF concept. We present a self-contained derivation of a “parametric” dispersion relation for magnetized three-wave interactions, meaning the pump wave is included in the equilibrium, similar to the unmagnetized work of Drake et al., Phys. Fluids 17, 778 (1974). For this, we use a multi-species plasma fluid model and Maxwell's equations. The application of an external B field causes right- and left-polarized light waves to propagate with differing phase velocities. This leads to Faraday rotation of the polarization, which can be significant in HED conditions. Phase-matching and linear wave dispersion relations show that Raman and Brillouin scattering have modified spectra due to the background B field, though this effect is usually small in systems of current practical interest. We study a scattering process we call stimulated whistler scattering, where a light wave decays to an electromagnetic whistler wave (ω≲ω ce ) and a Langmuir wave. This only occurs in the presence of an external B field, which is required for the whistler wave to exist.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

NASA NTRS1993

Development of a large field-of-view KD potassium di-deuterium phosphate modulator: Center Director's Discretionary Fund

Magnetographs, which measure polarized light, allow solar astronomers to infer the magnetic field intensity on the Sun. The Marshall Space Flight Center (MSFC) Vector Magnetograph is such an imaging instrument. The instrument requires rapid modulation between polarization states to minimize seeing effects. The accuracy of those polarization measurements is dependent on stable modulators with small field-of-view errors. Although these devices are very important in ground-based telescopes, extending the field of view of electro-optical crystals such as KD*Ps (potassium di-deuterium phosphate) could encourage the development of these devices for other imaging applications. The work that was done at MSFC as part of the Center Director's Discretionary Fund (CDDF) to reduce the field-of-view errors of instruments that use KD*P modulators in their polarimeters is described.

West, E. A.↗

NASA NTRS2017

Measurements of the Magnetic Field of the Upper Chromosphere with Polarimetry

A major remaining challenge for heliophysics is to decipher the magnetic structure of the chromosphere. The chromosphere is the critical interface between the Sun's photosphere and corona: it contains more mass than the entire interplanetary heliosphere, requires a heating rate that is larger than that of the corona, and mediates all the energy driving the solar wind, solar atmospheric heating and solar eruptions. While measurements of the magnetic field in the photosphere are routine, the chromosphere poses several extra challenges. The magnetically sensitive lines formed in the upper chromosphere are in the ultraviolet, so space-based observations are required. The lines are often formed over a range of heights, sampling different plasma which complicates the inversion process. These lines are sensitive to the magnetic field via polarized light that is created or modified through the Hanle and Zeeman effects. There are a few observations of these lines, and a significant challenge remains in extracting the magnetic field from the polarization measurements, as detailed model atmospheres with advanced radiative transfer physics are needed. Real progress is obtained by a simultaneous improvement in both the observational side and the modeling side. We present information on the CLASP (Chromospheric LAyer Spectro-Polarimeter) sounding rocket program, and future prospects for these types of measurements.

Solar; Chromosphere; Polarization↗

NASA NTRS2016

Polarimetry and Flux Distribution in the Debris Disk Around HD 32297

We present high-contrast angular differential imaging (ADI) observations of the debris disk around HD32297 in H-band, as well as the first polarimetric images for this system in polarized differential imaging (PDI) mode with Subaru/HICIAO. In ADI, we detect the nearly edge-on disk at > or = 5(sigma) levels from approx. 0.45" to approx.1.7" (50-192AU) from the star and recover the spine deviation from the midplane already found in previous works. We also find for the first time imaging and surface brightness (SB) indications for the presence of a gapped structure on both sides of the disk at distances of approx. 0.75" (NE side) and approx. 0.65" (SW side). Global forward-modeling work delivers a best-fit model disk and well-fitting parameter intervals that essentially match previous results, with high-forward scattering grains and a ring located at 110AU. However, this single ring model cannot account for the gapped structure seen in our SB profiles. We create simple double ring models and achieve a satisfactory fit with two rings located at 60 and 95AU, respectively, low-forward scattering grains and very sharp inner slopes. In polarized light we retrieve the disk extending from approx. 0.25-1.6", although the central region is quite noisy and high S/N are only found in the range approx. 0.75-1.2". The disk is polarized in the azimuthal direction, as expected, and the departure from the midplane is also clearly observed. Evidence for a gapped scenario is not found in the PDI data. We obtain a linear polarization degree of the grains that increases from approx. 10% at 0.55" to approx. 25% at 1.6". The maximum is found at scattering angles of 90, either from the main components of the disk or from dust grains blown out to larger radii.

high-contrast angular differential imaging (ADI)↗

DOE OSTI2025

Attosecond Optical Orientation

Circularly polarized light offers opportunities to probe symmetry-dependent properties of matter such as chirality and spin. Circular-dichroic measurements typically require further intrinsic or extrinsic breaking of symmetry by, e.g., enantiomeric excess, orientation, magnetic fields, or direction-sensitive detectors. Here we introduce circular-dichroic attosecond transient absorption spectroscopy by leveraging the angular momentum of two circularly polarized pulses, both pump and probe, in an isotropic medium, optically orienting the angular momentum of excited states on an attosecond timescale. We investigate a circular-dichroic measurement of the attosecond transient absorption of He Rydberg states. By limiting the allowed pathways via dipole selection rules for co- and counterrotating circularly polarized near-infrared and extreme ultraviolet (XUV) pulses, different spectral reshapings of the XUV transient absorption due to the AC Stark effect are observed. Furthermore, paired with time-dependent Schrödinger equation calculations, the results show the role of selection and propensity rules and open up new opportunities to study coupling pathways of excited states as well as spin-dependent dynamics in atoms and beyond via attosecond optical orientation.

Angular momentum of light↗

DOE OSTI2026

Synergistic Alignment of Low Aspect‐Ratio π‐Conjugated Molecules Enables Exceptional UV–vis–NIR Polarization Detection

Abstract Polarization detection enhances signal contrast and is widely utilized in diverse advanced applications. An ongoing challenge is the development of high‐performance polarization‐sensitive photodetectors based on optically anisotropic organic semiconductors, particularly in the near‐infrared (NIR) region. While uniaxially aligned π‐conjugated polymers with high aspect ratios exhibit strong linear dichroism and have shown promise, their limited NIR performance and heavy reliance on polymer material now represent critical limitations. Here, a breakthrough is reported in achieving giant linear dichroism and exceptional polarization detection with low aspect‐ratios (AR) non‐fullerene small‐molecule (NFSM) acceptors, extending polarization sensitivity from the UV–vis to the NIR range. An impressive dichroic ratio of 27.1 at 605 nm and 12.0 at 780 nm is demonstrated. The maximum polarization photocurrent ratio is 11.2 at 780 nm under parallel versus perpendicular polarized light. This unprecedented performance originates from synergistic molecular alignment, wherein NFSMs significantly enhance the uniaxial orientation of both the polymer matrix and the NFSMs themselves during self‐assembly and thermal annealing. Besides, such a linear‐polarization‐sensitive photodetectors (LPS‐PDs) are showcased in generating degree‐of‐linear‐polarization imaging. The work establishes NFSMs as a viable material system for next‐generation of organic LPS‐PDs and provides fundamental insights into structural origins of polarization sensitivity in low AR organic semiconductors.

Xue, Yingying↗

DOE OSTI2025

Enantioselective Se lattices for stable chiroptoelectronic processing media

Chiroptoelectronic devices are crucial for applications in quantum computing, spin optical communications, and magnetic recording. However, the limited efficiency and low stability of conventional circularly polarized light (CPL)-sensing materials have restricted their broader use. Here, we introduce atomic chiral Se nanorod (NRs) films as broadband CPL detectors, leveraging the intrinsic chirality and stability of Se nanocrystals. We also perform incident circular polarization (ICP)-Raman optical activity (ROA) to explore the chiroptical activity of the large-area films. The Se NRs thin films detected CPL across a broad range from ultraviolet (UV) to short-wavelength infrared (SWIR), with a responsivity dissymmetry factor of up to 0.4, maintaining high stability under ambient conditions for longer than 13 months. CPL-sensitive Se NRs with intrinsic chirality have potential applications in chiral photonic synapses, chiral spin devices, and CPL-sensitive photocatalysts. ICP-ROA mapping also advances the analysis of 2D chiral materials.

Nanophotonics and plasmonics↗

DOE OSTI2022

Multiparameter laser performance characterization of liquid crystals for polarization control devices in the nanosecond regime

Abstract Interactions of liquid crystals (LC’s) with polarized light have been studied widely and have spawned numerous device applications, including the fabrication of optical elements for high-power and large-aperture laser systems. Currently, little is known about both the effect of incident polarization state on laser-induced–damage threshold (LIDT) and laser-induced functional threshold (LIFT) behavior at sub-LIDT fluences under multipulse irradiation conditions. This work reports on the first study of the nanosecond-pulsed LIDT’s dependence on incident polarization for several optical devices employing oriented nematic and chiral-nematic LC’s oriented by surface alignment layers. Accelerated lifetime testing was also performed to characterize the ability of these devices to maintain their functional performance under multipulse irradiation as a function of the laser fluence at both 1053 nm and 351 nm. Results show that the LIDT varies as a function of input polarization by 30–80% within the same device, while the multipulse LIFT (which can differ from the nominal LIDT) depends on irradiation conditions such as laser fluence and wavelength.

47 OTHER INSTRUMENTATION↗

NASA NTRS1990

Real-time image difference detection using a polarization rotation spacial light modulator

An image difference detection system is described, of the type wherein two created image representations such as transparencies representing the images to be compared lie coplanar, while light passes through the two transparencies and is formed into coincident images at the image plane for comparison. The two transparencies are formed by portions of a polarization rotation spacial light modulator display such as a multi-pixel liquid crystal display or a magneto optical rotation type. In a system where light passing through the two transparencies is polarized in transverse directions to enable the use of a Wollaston prism to bring the images into coincidence, a liquid crystal display can be used which is devoid of polarizing sheets that would interfere with transverse polarizing of the light passing through the two transparencies.

Chao, Tien-Hsin↗

DOE OSTI2021

Shape- and Orientation-Dependent Scattering of Isolated Gold Nanostructures Using Polarized Dark-Field Microscopy

In this work, we demonstrate a simple and robust method for measuring the shape- and orientation-dependent optical scattering of various plasmonic nanostructures adsorbed onto a solid surface using polarized dark-field microscopy. By analyzing the dark-field scattering images of gold nanostructures using grazing incidence polarized light with a bench-top microscope, we are able to correlate optical scattering from the individual nanostructures with their shape and orientation. Depending on the size, shape, and orientation of the plasmonic nanostructures, they exhibit characteristic angle- and polarization-dependent scattering signals. Extracting the red, green, and blue channels of the scattering signals from a color-imaging detector as a function of azimuthal angle provides a polar plot of color intensity values that is characteristic of the underlying nanostructure. Examples are presented for various nanostructures, including spherical nanoparticles, nanotriangles, and nanorods. Experimental results are complemented by numerical calculations of the scattering spectra of representative model nanostructures. We demonstrate that the polarization- and orientation-dependent scattering behavior is a consequence of various localized surface plasmon modes existing in the nanostructures and can be used to verify the shape of individual objects as well as quickly identify the orientation of numerous objects on a densely populated substrate. We anticipate that this method will provide a rapid and efficient complement to the typical structural analysis of nanoparticles that is achieved by electron microscopy as well as providing a simple method for generating detailed information of the optical scattering of various types of individual plasmonic nanostructures.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

NASA NTRS1993

Optical and Hubble Space Telescope ultraviolet spectropolarimetry of 3C 273 and PG 1114+445

New optical spectropolarimetry and broad-band measurements, made during periods when the linear polarization of the quasar 3C 273 was no greater than 1 pct, are combined with ultraviolet polarization measurements made with the Faint Object Spectrograph of the Hubble Space Telescope. Very weak UV polarization during the time of observation is seen in the HST measurements, which is consistent with the completely unpolarized UV continuum and emission lines. Optical spectropolarimetry, however, reveals polarized light, the source of which is consistent with a nonthermal component, diluted by other unpolarized emission sources, such as the 'big blue bump'. Optical spectropolarimetry of the radio-quiet quasar PG 1114+445 is also presented. The polarization of this QSO is thought to result from scattering by dust external to the narrow-line region. 3C 273 and PG 1114+445 are useful in illustrating the range of polarizing mechanisms which can operate in low-polarization QSOs.

Smith, Paul S.↗

NASA NTRS1988

Real-time image difference detection using a polarization rotation spacial light modulator

An image difference detection system is described, of the type wherein two created image representations such as transparencies representing the images to be compared lie coplanar, while light passes through the two transparencies and is formed into coincident images at the image plane for comparison. The two transparencies are formed by portions of a polarization-rotation spatial light modulator display such as a multi-pixel liquid crystal display or a magnetooptical rotation type display. In a system where light passing through the two transparencies is polarized in transverse directions to enable the use of a Wollaston prism to bring the images into coincidence, a liquid crystal display can be used which is devoid of polarizing sheets that would interfere with transverse polarizing of the light passing through the two transparencies.

Chao, Tien-Hsin↗

NASA NTRSDate not supplied

A New Linear Polarizer Design for Application in the Far-Ultraviolet Spectral Range

New mission concepts that are under consideration by NASA (such as the Polstar MIDEX mission concept) call for the design and implementation of Far Ultraviolet (FUV) polarizer technologies that have not been developed yet. A team that includes members from the NASA Goddard Space Flight Center (GSFC), Arizona State University (ASU), and Woodruff Consulting, worked on the design and development of a polarizer design that may produce extinction ratios higher than have ever been reported before in the FUV spectral range (100-200 nm). This polarizer consists of transmitting linearly polarized light through a series of reflections from a combination of two silicon carbide (SiC) and two lithium fluoride (LiF) crystals positioned at angles of incidence (relative to surface normal) close to the LiF Brewster’s angle. The performance of this polarizer concept was fabricated and tested with an existing McPherson 225 Vacuum Ultraviolet (VUV) spectrometer located in the Optics Branch at NASA-GSFC. Initial testing has shown that in the FUV spectral range, this design can produce state-of-the-art extinction ratios at the Hydrogen Lyman-Alpha (Ly-α) wavelength of 121.6 nm. A polarizer with such a performance has never been reported and it signifies a breakthrough in FUV polarization technology. The levels of effectiveness paired with the design’s compact design allows for a new polarizer capability that would one day be implemented in a future spectropolarimetry space mission. In addition, this polarizer concept could potentially be used to characterize the optical properties of new mirror coatings that will be used in a future Habitable World Observatory (HWO) mission concept as proposed by the 2020 Decadal Survey.2

Far Ultraviolet (FUV), polarimetry, instrumentatio↗

NASA NTRSDate not supplied

Linear Polarizer Design for Application in the Far-Ultraviolet Spectral Range

Far Ultraviolet (FUV), polarimetry, instrumentatio↗

DOE OSTI2020

First Resolved Scattered-light Images of Four Debris Disks in Scorpius-Centaurus with the Gemini Planet Imager

In this work, we present the first spatially resolved scattered-light images of four debris disks around members of the Scorpius-Centaurus (Sco-Cen) OB association with high-contrast imaging and polarimetry using the Gemini Planet Imager (GPI). All four disks are resolved for the first time in polarized light, and one disk is also detected in total intensity. The three disks imaged around HD 111161, HD 143675, and HD 145560 are symmetric in both morphology and brightness distribution. The three systems span a range of inclinations and radial extents. The disk imaged around HD 98363 shows indications of asymmetries in morphology and brightness distribution, with some structural similarities to the HD 106906 planet–disk system. Uniquely, HD 98363 has a wide comoving stellar companion, Wray 15-788, with a recently resolved disk with very different morphological properties. HD 98363 A/B is the first binary debris disk system with two spatially resolved disks. All four targets have been observed with ALMA, and their continuum fluxes range from one nondetection to one of the brightest disks in the region. With the new results, a total of 15 A/F stars in Sco-Cen have resolved scattered-light debris disks, and approximately half of these systems exhibit some form of asymmetry. Combining the GPI disk structure results with information from the literature on millimeter fluxes and imaged planets reveals a diversity of disk properties in this young population. Overall, the four newly resolved disks contribute to the census of disk structures measured around A/F stars at this important stage in the development of planetary systems.

79 ASTRONOMY AND ASTROPHYSICS↗

NASA NTRS1988

Tunable superlattice p-i-n photodetectors: Characteristics, theory, and applications

Extended measurements and theory on the recently developed monolithic wavelength demultiplexer consisting of voltage-tunable superlattice p-i-n photodetectors in a waveguide configuration are discussed. It is shown that the device is able to demultiplex and detect two optical signals with a wavelength separation of 20 nm directly into different electrical channels at a data rate of 1 Gb/s and with a crosstalk attenuation varying between 20 and 28 dB, depending on the polarization. The minimum acceptable crosstalk attenuation at a data rate of 100 Mb/s is determined to be 10 dB. The feasibility of using the device as a polarization angle sensor for linearly polarized light is also demonstrated. A theory for the emission of photogenerated carriers out of the quantum wells is included, since this is potentially a speed limiting mechanism in these detectors. It is shown that a theory of thermally assisted tunneling by polar optical phonon interaction is able to predict emission times consistent with the observed temporal response.

Larsson, Anders↗

DOE OSTI2025

Light-induced anomalous Hall conductivity in the massive three-dimensional Dirac semimetal Co 3 ⁢Sn 2 ⁢S 2

Weyl semimetals can emerge from Dirac semimetals when the time-reversal or spatial-inversion symmetries are broken. Recently, it has been proposed based on Floquet theory that Dirac semimetals can be converted into Weyl semimetals even by shining circularly polarized light (CPL). Here we have investigated the possibility of such a Dirac-Weyl conversion by measuring the CPL-induced anomalous Hall conductivity (AHC) in a massive 3D Dirac semimetal Co 3 ⁢Sn 2 ⁢S 2 in the paramagnetic phase using ultrafast midinfrared pump-terahertz Faraday rotation probe spectroscopy. We find that the field-strength and driving frequency dependence of the observed AHC is well accounted for by CPL-induced nonzero Berry curvature associated with the splitting of the Dirac bands as predicted by the Floquet theory. As a result, the estimated splitting of the Dirac bands reaches about 60% of the mass gap and the calculated CPL-induced AHC quantitatively reproduces the experimental observation, demonstrating a promising route toward the realization of Floquet-Weyl states from massive Dirac semimetals.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2024

Floquet-driven indirect exchange interaction mediated by topological insulator surface states

Light drives offer a potential tool for the dynamical control of magnetic interactions in matter. We theoretically investigate the indirect exchange coupling between two parallel chains of magnetic impurities on the surface of a topological insulator, driven by a time-periodic circularly polarized light field in the high-frequency, off-resonant regime. We derive a closed-form analytic expression for the spin susceptibility of the photon-dressed topological insulator surface states and obtain the irradiation dependence of the Ising, Heisenberg, and Dzyaloshinskii-Moriya exchange couplings between the impurity chains. Our results show a two-pronged modification of these exchange couplings by periodic drives. First, the Ruderman-Kittel-Kasuya-Yosida (RKKY) oscillation period of the exchange couplings can be extended by enhancing the driving strength. Second, increasing driving strength enhances the envelope of RKKY oscillations of the Ising type while suppressing those of the Heisenberg type and Dzyaloshinskii-Moriya type. Furthermore, our work provides useful insights for realizing Floquet engineering of collinear and noncollinear indirect exchange interactions in topological insulating systems.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗