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NASA NTRS1982

A dehydration mechanism for the stratosphere

Although mean circulations are generally credited with dehydration of the earth's stratosphere, convective instability in the tropics converts mean circulations to small residuals of local convective circulations. The effects of large cumulonimbus which penetrate the stratosphere and form huge anvils in the lower stratosphere are discussed with respect to hydration and dehydration of the stratosphere. Radiative heating at anvil base combined with cooling at anvil top drives a dehydration engine considered essential to explain the dry stratosphere. Seasonal and longitudinal variations in dehydration potentials are examined with maximum potential attributed to Micronesian area during winter and early spring.

Danielsen, E. F.↗
NASA NTRS1982

Measurements of stratospheric aerosols over Mauna Loa, Hawaii and Boulder, Colorado

The direct solar radiation transmission record at Mauna Loa, dating from 1958 to the present, revealed with remarkable precision the presence of stratospheric aerosol from volcanic activity. This record can be used to quantify the intensity of the stratospheric volcanic aerosol perturbation following a significant eruption in reference to the Agung event in 1963. The Mount St. Helens' stratospheric cloud was first detected by lidar at 18 km over Mauna Loa on 17 July. The atmospheric transmission was seen to decrease slightly after that time, but only a few tenths of 1 percent. Although it is still fairly early to draw a definite conclusion on the ultimate magnitude of the Mount St. Helens stratospheric aerosol from the Mauna Loa results, it can be stated that the stratospheric aerosol optical depth presently observed is comparable with that observed from Fuego which erupted in 1974. At Boulder, Colorado, the atmospheric debris from Mount St. Helens was observed by lidar on a number of occasions. Also, observations of the diffuse, total and direct transmission of solar radiation were made on June 3 and 4. The latter set of observations is useful for deriving information on the scattering properties of the volcanic cloud. The lidar and solar radiation data are presented and some of their special features are discussed.

Deluisi, J. J.↗
NASA NTRS1983

SAM 2 measurements of the polar stratospheric aerosol. Volume 3: October 1979 to April 1980

The Stratospheric Aerosol Measurement (SAM) II sensor is aboard the Earth-orbiting Nimbus 7 spacecraft providing extinction measurements of the Antarctic and Arctic stratospheric aerosol with a vertical resolution of 1 km. Representative examples and weekly averages of aerosol data and corresponding temperature profiles for the time and place of each SAM II measurement (Oct. 1979 through Apr. 1980) are presented. Contours of aerosol extinction as a function of altitude and longitude or time are plotted and weekly aerosol optical depths are calculated. Seasonal variations and variations in space (altitude and longitude) for both polar regions are easily seen. Typical values of aerosol extinction at the SAM II wavelength of 1.0 microns for this time period are 2 to 4 times .0001/km in the main stratospheric aerosol layer. Optical depths for the stratosphere are about 0.002 to 0.003, up slightly over normal background levels (due to the eruption of Sierra Negra, Nov. 1979). Polar stratospheric clouds at altitudes of about 22 km were observed during the Arctic winter. A ready-to-use format containing a representative sample of the third 6 months of data to be used in atmospheric and climatic studies is presented.

Mccormick, M. P.↗
NASA NTRS1982

Photochemistry of the stratosphere of Venus - Implications for atmospheric evolution

The photochemistry of the Venus stratosphere is modeled using an updated and expanded chemical scheme along with the results of recent observations and laboratory studies. Three models, with H2 mixing ratio equal to 2 x 10 to the -5th, 5 x 10 to the -7th, and 1 x 10 to the -13th, respectively, are examined. All three models are found to satisfactorily account for the observations of CO, O2, O2(1Delta), and SO2 in the stratosphere, but only the last one may be able to account for the diurnal behavior of mesospheric CO and the UV albedo. Oxygen, derived from CO2 photolysis, is mainly consumed by CO2 recombination and oxidation of SO2 to H2SO4. The photolysis of HCl in the upper stratosphere provides a major source of odd hydrogen and free chlorine radicals, essential for the catalytic oxidation of CO. Oxidation of SO2 by O occurs in the lower stratosphere. The modeling reveals a number of interesting similarities, previously unsuspected between the chemistry of the stratosphere of Venus and that of the earth; photochemistry may have played a major role in the evolution of the atmosphere.

Yung, Y. L.↗
NASA NTRS1985

Development of algorithms for using satellite meteorological data sets to study global transport of stratospheric aerosols and ozone

The utilization of stratospheric aerosol and ozone measurements obtained from the NASA developed SAM II and SAGE satellite instruments were investigated for their global scale transports. The stratospheric aerosols showed that during the stratospheric warming of the winter 1978 to 1979, the distribution of the zonal mean aerosol extinction ratio in the northern high latitude exhibited distinct changes. Dynamic processes might have played an important role in maintenance role in maintenance of this zonal mean distribution. As to the stratospheric ozone, large poleward ozone transports are shown to occur in the altitude region from 24 km to 38 km near 55N during this warming. This altitude region is shown to be a transition region of the phase relationship between ozone and temperature waves from an in-phase one above 38 km. It is shown that the ozone solar heating in the upper stratosphere might lead to enhancement of the damping rate of the planetary waves due to infrared radiation alone in agreement with theoretical analyses and an earlier observational study.

Want, P. H.↗
NASA NTRS1985

Aspects of the stratospheric circulation as derived from SSU data

Five years of global data are available for the stratosphere up to 1 mb from Stratospheric Sounding Units (SSUs) on board NOAA satellites. These data form the basis for a climatological study which concentrates on the seasonal and inter-annual variability of the stratosphere and the connection between the stratospheric circulation and that of the troposphere. Particular emphasis is on the structure of the Southern Hemisphere and how it compares with that of the Northern Hemisphere. The characteristic difference in the vertical structure and propagation of disturbances in the two hemispheres is related to differences in the tropospheric flow and the long-term variation of the basic state of the stratosphere. Disturbances in both hemispheres occur in preferred geographical locations. The final warming, marking the transition from westerly to easterly winds, is an example. These occur asymmetrically with respect to the pole as warm air moves over the pole, usually from the same region.

Michaelis, V.↗
NASA NTRS1985

A new model of resonance in the winter stratosphere

It is generally accepted that the planetary waves observed in the winter stratosphere are primarily a response to dynamical forcing from the troposphere. Nevertheless, the mechanism by which wave amplitudes sometimes become larger remains uncertain. It is possible that anomalously large waves in the stratosphere might simply be the result of anomalously large tropospheric forcing. However, it has also been suggested that they are a response to a stratospheric-tropospheric cavity being in a near-resonant configuration. It has been suggested that nonlinear self-tuning effects could play an important role in the behavior of such a cavity. Self-tuning may occur when a system starts to one side of resonance, such that the mean-state change induced by growing waves brings the system closer to resonance. A new model of the stratospheric cavity is introduced and is then used to re-examine the possibility of wave growth in the real atmosphere and in atmospheric models due to self-tuning effects. The new model is based on the picture of the winter-time stratosphere which has been revealed by the observations of Ertel's potential vorticity, Q. Isentropic maps of Q show two rather distinct regions, the first containing the circumpolar vortex, where gradients of Q are large and Rossby waves may propagate easily. Surrounding this is a second, low-latitude region where the gradients are generally weak and where, because the Eulerian-mean flow is comparable with their phase speed, Rossby waves must be continually breaking. As the waves are observed to grow the relative sizes of these two regions change in time. This leads to the interesting possibility that self-tuning, mainly due to irreversible changes in the size of the polar vortex, is taking place.

Haynes, P. H.↗
NASA NTRS1985

Rossby wavetrains in the stratosphere forced by localised disturbances in the troposphere

Studies have linked elements of the stratospheric circulation with particular localized features in the tropospheric circulation. This suggests a study of the response of the stratosphere to forcing by localized disturbances in the troposphere. A multilevel, primitive equation model is used of the stratosphere and mesosphere the height of whose lower boundary at 300 mb can be prescribed. Localized height disturbances which grow to steady amplitude are applied at this lower boundary, and the response of the initially axially symmetric stratosphere is studied. The perturbation, centered at 45 deg N, has a Gaussian distribution with a half width of 15 deg., corresponding roughly to the size of persistent troughs and blocking ridges in the troposphere. The forcing is nearly at fully amplitude 10 days after being switched on, and thereafter remains steady. Two types of experiments are conducted: in one the forcing is of small amplitude (100 gpm) and in the other it is of large amplitude (600 gpm). These pairs of experiments are compared to determine how nonlinear processes affect the perturbation fields. This is done locally by defining the perturbation response to the forcing as an anomaly, i.e., as a departure from the response in a controlled experiment in which no asymmetric forcing was applied at the lower boundary of the model. Experiments have been conducted for a number of atmospheric states obtained as zonal means of observations made by a stratospheric sounding unit (SSU). In this summary, results for the zonal mean flow on January 19, 1982 are outlined.

Marks, C. J.↗
NASA NTRS1986

SAM 2 measurements of the polar stratospheric aerosol, volume 2

The Stratospheric Aerosol Measurement (SAM) 2 sensor aboard Nimbus 7 is providing extinction measurements of Antarctic and Arctic stratospheric aerosols with a vertical resolution of 1 km. Representative examples and weekly averages including corresponding temperature profiles provided by NOAA for the time and place of each SAM 2 measurement (Oct. 1981 - Apr. 1982) are presented. Contours of aerosol extinction as a function of altitude and longitude or time are plotted, and aerosol optical depths are calculated for each week. Typical values of aerosol extinction at 1.0 micron in the main lower stratospheric aerosol layer for this time period are 2 to 4 times 10 to the -4 power/km. for the Antarctic region and 0.5 to 1 times 10 to the -3 power/km. for the Arctic region. Stratospheric optical depths are about 0.001 to 0.004 for the Antarctic region and 0.003 to 0.004 at the beginning to about 0.006 at the end of the time period for the Arctic region. Polar stratospheric clouds (PSC's) were observed during the Arctic winter, as expected. This report provides, in a ready-to-use format, a representative sample of the seventh semester of data to be used in atmospheric and climatic studies.

Mccormick, M. P.↗
NASA NTRS1986

SAM 2 measurements of the polar stratospheric aerosol, volume 8

The Stratospheric Aerosol Measurement (SAM) 2 sensor aboard Nimbus 7 is providing extinction measurements of Antarctic and Arctic stratospheric aerosols with a vertical resolution of 1 km. Representative examples and weekly averages including corresponding temperature profiles provided by NOAA for the time and place of each SAM 2 measurement (Apr. 1982 - Oct. 1982) are presented. Contours of aerosol extinction as a function of altitude and longitude or time are plotted, and aerosol optical depths are calculated for each week. Typical values of aerosol extinction at 1.0 microns in the main stratospheric aerosol layer are approximately 4 to 6 times .0001/km at the beginning to 1 to 2 times .001/km at the end of the time period for the Antarctic region and approximately 1 to 3 times .001/km for the Arctic region throughout the time period. Stratospheric optical depths are about 0.002 to 0.009 for the Antarctic region and about 0.007 at the beginning to 0.024 at the end of the time period for the Arctic region. Polar stratospheric clouds were observed during the Antarctic winter, as expected. This report provides, in a ready-to-use format, a representative sample of the eighth 6 months of data to be used in atmospheric and climatic studies.

Mccormick, M. P.↗
NASA NTRS1985

Some aspects of stratospheric dynamics

Observations of the stratosphere are analyzed. The behavior of the wind and temperature in the stratosphere is compared to that of the troposphere. Techniques for observing the circulation and temperatures of the stratosphere and the basic circulation and temperature characteristics are described. The propagation of tropospheric planetary waves to the stratosphere and their interaction with the mean flow are studied. The stability of the zonal-mean state in the stratosphere is investigated by calculating the meridional gradient of zonal-mean quasi-geostrophic potential vorticity.

Hartmann, D. L.↗
NASA NTRS1986

The water vapour budget of the stratosphere studied using LIMS and SAMS satellite data

Monthly zonal mean observations of H2O and CH4 made by the limb infrared monitor of the stratosphere and the stratospheric and mesospheric sounder instruments on Nimbus 7 have been used to investigate whether the H2O mixing ratios in the stratosphere are consistent with a source via the oxidation of CH4. While both sets of data show considerable seasonally varying structure, total hydrogen (neglecting molecular hydrogen) is relatively featureless with a mean value over the stratosphere of 6.0 + or - 0.35 ppmm(1sigma) for the five-month period studied. The uniformity of the total hydrogen fields points to the validity of the CH4 oxidation hypothesis. The derived fields of total hydrogen are used to deduce a mean H2O mixing ratio for air as it enters the stratosphere of 2.7 + or - 0.35 ppmv (1sigma) from which a desiccation temperature may be deduced.

Jones, R. L.↗
NASA NTRS1986

Planetary wave activity in the troposphere and stratosphere during the Northern Hemisphere winter

The relation between planetary wave activity in the troposphere and stratosphere during the Northern Hemisphere winter from December 1981-March 1982 is studied. The Eliassen-Palm (E-P) flux diagnostics was applied to global tropospheric data for 1000 to 100 mb and global stratospheric data for 70 to 0.4 mb. The vertical component of the E-P flux, which is a measure of the vertical propagation of wave activity, and wave driving are examined. It is observed that the magnitude of the vertical component of the E-P flux varies with a period of 10-15 days in both the troposphere and the stratosphere; however, the correlation between the wave activity in the troposphere and stratosphere is different during the pre- and postwarming periods. The two types of correspondence between the wave activity are: (1) an out-of-plane relationship and (2) an upward propagation of wave activity from the troposphere to the stratosphere. The dynamical features of these two periods are described.

Shiotani, Masato↗
NASA NTRS1988

The ozone hole - The role of polar stratospheric cloud particles

The role of polar stratospheric clouds in the formation of the Antarctic ozone hole is considered. Several researchers have suggested that the decrease in ozone over Antarctica is related to the polar stratospheric clouds (PSCs) which had been observed in the antarctic winter stratosphere. Some of the pertinent characteristics of polar stratospheric clouds are discussed, and it is shown how these clouds may participate in the ozone destruction process. The satellite data for PSCs is analyzed, and statistical information regarding the number and maximum extinctions of these clouds is presented. Evidence that the polar stratospheric clouds are composed of frozen nitric acid is considered. It is suggested that the evaporation of the clouds, in late August and September, will release HOCl and HNO3 to the environment. This could be followed by the photodissociation of HOCl to OH and Cl, which would very effectively destroy ozone. However, the ozone destruction mechanism could be halted when enough of the evaporated nitric acid is photolized.

Hamill, Patrick↗
NASA NTRS1989

Water vapor and methane in the upper stratosphere - An examination of some of the Nimbus 7 measurements

The zonal mean volume mixing ratios of water vapor and methane from January to May, 1979, derived from the Nimbus-7 limb IR monitor of the stratosphere and from stratosphere and mesosphere sounder experiments are investigated. The water vapor mixing ratio of air that enters the stratosphere from the troposphere and the yield of water vapor from photochemical oxidation of methane in the stratosphere are examined. The water vapor yield averaged between 1.5 and 2.0, although variability with time and level was relatively large. It is suggested that water vapor yield increases with height in the 16- to 3-mbar range. The average water vapor mixing ratio fo air entering the stratosphere during the study period was about 3.25 X 10 to the -6th.

Hansen, Anthony R.↗
NASA NTRS1990

The Airborne Arctic Stratospheric Expedition - Prologue

This paper presents an introduction to the initial scientific results of the Airborne Arctic Stratospheric Expedition (AASE), as well as data from other atmospheric experiments and analyses carried out during the Arctic polar winter of 1989. Mission objectives of the AASE were to study the mechanisms of ozone depletion and redistribution in the northern polar stratosphere, including the influences of Arctic meteorology, and polar stratospheric clouds formed at low temperatures. Some major aspects of the AASE are described including: logistics and operations, meteorology, polar stratospheric clouds, trace composition and chemistry, and ozone depletion. It is concluded that the Arctic-89 experiments have provided the scientific community with a wealth of new information that will contribute to a better understanding of the polar winter stratosphere and the critical problem of global ozone depletion.

Turco, Richard↗
NASA NTRS1990

Stratospheric temperatures during the 88-89 Northern Hemisphere winter

The Airborne Arctic Stratospheric Expedition (AASE) was conducted during January and February 1989. The polar stratosphere during this period was characterized by cold conditions from January to mid-February. A mid-February wave 2 major warming considerably warmed the polar stratosphere, but did not immediately lead to a lower stratospheric vortex breakup. As inferred from temperature data, January temperatures were sufficient for polar stratospheric cloud (PSC) formation. PSC regional extent was greater than the long-term average, but not significantly larger than in previous years.

Newman, Paul A.↗
NASA NTRS1990

In situ measurements of NO(x) in the Airborne Arctic Stratospheric Expedition

In situ measurements of NO and NO2 were made simultaneously from the NASA DC-8 aircraft as part of the Airborne Arctic Stratospheric Expedition. Mixing ratios of NO(x) (NO + NO2) were typically higher in the arctic troposphere than in the stratosphere, with median values of 59 and 40 pptv, respectively. In the stratosphere, there tended to be a positive correlation between NO(x) and water vapor and negative correlations between NO(x) and ozone and between NO(x) and total reactive odd-nitrogen, NO(y). The ratio of NO(x) to NO(y), in conjunction with NO(y), appears to be an excellent tracer of tropospheric or stratospheric air at northern latitudes during winter. Tropospheric NO(x) was typically 10 to 50 percent of gas-phase NO(y), while in the stratosphere, NO(x) was typically less than 10 percent, and frequently less than 5 percent of gas-phase NO(y).

Carroll, Mary Anne↗