Detection of local-scale changes in greenhouse gas emissions in urban environments using micrometeorological methods and comparison to a high-resolution inventory
We used the Monin–Obukhov similarity theory (MOST) flux-variance relationship to estimate greenhouse gas (GHG) fluxes from high-precision mole fraction measurements at 3 instrumented urban communication towers over several years, demonstrating the ability of this method to detect and quantify changes in emissions. Depending on data availability, we used carbon dioxide (CO 2 ) and carbon monoxide (CO) measurements and/or tracer ratios to estimate fluxes at 1 urban site (Site 3) and 1 suburban site (Site 7) in Indianapolis, IN, USA, and 1 urban site (COM) in Los Angeles, CA, USA. We also compared the estimated fluxes of CO 2 from fossil fuel sources (CO 2 ff) at Sites 3 and 7 and the total CO 2 fluxes at Site 3 to 20 m, hourly resolution subdomains of the high-resolution CO 2 emissions inventory, Hestia, for the year 2020, introducing a new way to evaluate emissions inventories at small spatial and temporal scales. Using the flux-variance relationship, we detected and quantified abrupt decreases in CO and CO 2 fluxes at Site 3 and COM in April 2020, coinciding with the stay-at-home order due to COVID-19 pandemic, as well as abrupt decreases in CO and CO 2 fluxes at Site 3 in July 2018 coinciding with a highway closure next to the site. The Hestia emissions inventory detected a decrease in emissions in April 2020 at Sites 3 and 7, but this decrease differed in magnitude from those detected in the atmospheric estimates. Seasonal trends in emissions are similar between Hestia and the atmospheric estimates at Site 7. We use differences in seasonal and spatial trends between the flux estimation methods to identify potential sources of uncertainty in both the atmospheric and inventory methods. The results from this study show that the flux-variance estimation method is a useful tool to monitor local-scale emissions and evaluate high-resolution emissions inventories.