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At least 289 records · Page 16

Large Volume Airborne Contamination Monitoring To Support Nuclear Processes' Deactivation and Decommissioning

Current D and D operations at Hanford have demonstrated a flaw in the current state of the art capability of defining airborne contamination boundaries - Airborne particulate emissions of Pu-239 from CM2H operations on the Hanford Pu Finishing Plant were detected well beyond areas controlled for airborne Pu, putting numerous workers at risk for radiological assimilations - Current air samplers and CAM systems were surveying insufficient volumes of air to accurately predict where respiratory protection was required - Hanford is located in a high radon environment, making air monitoring for alpha emitting actinides challenging in high alpha radon induced backgrounds. - Inexpensive HEPA based home and industrial air purifiers filter significantly higher volumes of air than commercially available continuous-air monitoring (CAM) systems. - Inexpensive models capable of filtered air volumes exceeding 1000 times that of a CAM. - Detector system can be built to detect x-rays generated from actinide decay. - Branching ratios of x-rays are 4 orders of magnitude more intense from Plutonium decay than its gamma emissions. - Detector system can be a low resolution systems, as x-ray region of interest is not terribly congested. - Detection systems evaluated will be designed based on slabs of NaI or pixelated NaI or CsI panels. - Simple graphical user interface software will be developed to operate the detection system. - Concept is to deploy some of these air-purifying systems in nonradiological areas around SRNL to confirm radon can be rejected with confidence. - Generate some filters contaminated with plutonium via electroplated Pu or lab generated simulated particles. - then deploy units in known airborne radiological environments to establish systems ability to accurately measure actinide based hot particles Lab analyses will follow up the system analyses to ensure hot particles were correctly identified. Analysis by Scintillation: - Application of scintillation media to the surface of the filters is being explored. - Evaluating slabs of ZnS(Ag), application of powdered ZnS(Cu) and spray on Perkin Elmer Enhance. - Scintillation events would then be digitized with a digital camera and quantified. - Comparing against sensitivity of a PMT or SiPD readout. - Currently evaluating a Thorlabs 8 Megapixel Monochrome Scientific CCD Camera, hermetically sealed cooled package with a wide angle lens. - Wide angle lens allows complete view of HEPA filter from 7 inches away. - Images taken of glow in the dark paint, as well as plutonium-induced fluorescence. - Plutonium was flamed mounted on a 1 inch diameter stainless steel planchet, covered with a layer of mylar and a section of scintillating ZnS obtained from Eljon. - Currently working on reducing signal-to-noise levels to boost sensitivity. - Dark box to hold contaminated or electroplated source covered filters under fabrication. Analysis by x-ray Spectroscopy: - Branching ratios for x-ray emissions from Plutonium isotopes are orders of magnitude more intense than gamma-ray emissions. - The nuclear databases are incomplete on the branching ratios of some of the isotopes. - Evaluating some custom built SrI2 x-ray spectrometers vs a conventional windowed NaI detector. - SrI2 detectors are carbon-composite-windowed 51 mm x 51 mm. - MCNP calculations to establish self absorbance of filter media on 17 keV x-ray. Radon Rejection: - Activated charcoal pre-filter acts as a Radon trap. - Adding a time lapse feature to camera to aid in radon rejection. SRS Plutonium Fuel Form D and D Operations: Currently deploying air sampler to D and D operation of Pu-238 facility at SRS to generate some field samples to analyze.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

An impulsive solar burst observed in H-alpha, microwaves, and hard X-rays

H-alpha, microwave, and hard X-ray observations of an unusually short duration impulsive spike burst are presented. The observations are analyzed, and it is found that the single spike is in fact composed of two separate acceleration episodes. The differences found in the time profiles for the two components stress the role of the decay rate and lead to a simple explanation for the often observed delay of the microwave peak. The approximate numbers of electrons responsible for the two types of emission are derived and compared.

Gary, D. E.↗

Investigation of Deuterium Loaded Materials Subject to X-Ray Exposure

Results are presented from an exploratory study involving x-ray irradiation of select deuterated materials. Titanium deuteride plus deuterated polyethylene, deuterated polyethylene alone, and for control, hydrogen-based polyethylene samples and nondeuterated titanium samples were exposed to x-ray irradiation. These samples were exposed to various energy levels from 65 to 280 kV with prescribed electron flux from 500 to 9000 μA impinging on a tungsten braking target, with total exposure times ranging from 55 to 280 min. Gamma activity was measured using a high-purity germanium (HPGe) detector, and for all samples no gamma activity above background was detected. Alpha and beta activities were measured using a gas proportional counter, and for select samples beta activity was measured with a liquid scintillator spectrometer. The majority of the deuterated materials subjected to the microfocus x-ray irradiation exhibited postexposure beta activity above background and several showed short-lived alpha activity. The HPE and nondeuterated titanium control samples exposed to the x-ray irradiation showed no postexposure alpha or beta activities above background. Several of the samples (SL10A, SL16, SL17A) showed beta activity above background with a greater than 4σ confidence level, months after exposure. Portions of SL10A, SL16, and SL17A samples were also scanned using a beta scintillator and found to have beta activity in the tritium energy band, continuing without noticeable decay for over 12 months. Beta scintillation investigation of as-received materials (before x-ray exposure) showed no beta activity in the tritium energy band, indicating the beta emitters were not in the starting materials.

x-ray irradiation↗

Flare asymmetry as seen in offband H-alpha filtergrams

Narrow-band H-alpha filtergrams at + or - 1 A and + or - 2 A from the line center were used to study the asymmetry of flares. Of the 60 flares studied, 92% show red asymmetry while 5% show blue asymmetry. Typically, the filtergrams show a striking dominance of the red wing over the blue wing from onset until late in the decay phase. The difference in intensity of the flare emissions is further augmented by the extensiveness of the emission area in the brighter wing. New kernel-like emissions were often found many minutes after the flare maximum. Spatially, they are displaced from the previous kernels. The late emissions show the same asymmetry as that of the earlier part of the flare.

Tang, F.↗

Calculations of neutron flux spectra induced in the earth's atmosphere by galactic cosmic rays

Calculations have been carried out to determine the neutron flux induced in the earth's atmosphere by galactic protons and alpha particles at solar minimum for a geomagnetic latitude of 42 N. Neutron flux spectra were calculated using Monte Carlo and discrete ordinates methods, and various comparisons with experimental data are presented. The magnitude and shape of the calculated neutron-leakage spectrum at the particular latitude considered support the theory that the cosmic-ray-albedo-neutron-decay mechanism is the source of the protons and electrons trapped in the Van Allen belts.

Armstrong, T. W.↗

The spatial, spectral, and temporal character of the hard X-ray flare of 1982 February 3

This paper presents spatially resolved, hard and soft X-ray, 17 GHz microwave and H-alpha observations of an X1.1 flare which occurred on February 3, 1982. The bulk of the 25-50 keV hard X-ray emission during impulsive peaks is produced by two sources of differing brightness which are separated by about 50 arcsec. Soft X-ray images reveal a single component that resides between the two hard sources. On the decay of the event, X-ray spectra provide direct evidence for a hot component that dominates the less than 50 keV flux. Hard X-ray images obtained at these times show a single source that is nearly coincident with the soft X-ray source. Interferometric microwave observations obtained during impulsive peaks support the idea that microwave emission is produced in the vicinity of high magnetic fields near the sunspot. The influence of an asymmetric loop or system of asymmetric loops is essential to interpreting the observations.

Nitta, Nariaki↗

Measurement of the anomalous spin precession frequency $\omega_\alpha$ in the Muon g-2 experiment at Fermilab

The Muon $g-2$ Experiment at Fermilab aims to measure the muon magnetic moment anomaly, $a_{\mu} = (g-2)/2$, with a final accuracy of 0.14 parts per million (ppm). A $3.1$-GeV muon beam is injected into a storage ring of $14\,$m diameter, in the presence of a $1.45\,$T magnetic field. The anomaly $a_\mu$ can be extracted by accurately measuring the anomalous muon spin precession frequency $\omega_a$, based on the arrival time distribution of decay positrons observed by $24$ calorimeters, and the magnetic field. In 2023, the experiment published its second result based on the two datasets Run-2 and Run-3, reaching the unprecedented sensitivity of $0.21\,$ppm --- a factor $\sim2.2$ improvement since its first result published in 2021, based on the first dataset (Run-1). In this paper, we will focus on the measurement of the $\omega_a$ frequency, describing the techniques and major sources of systematic uncertainty in the 2023 publication, and outlining the improvements since the 2021 result. We will also cover the status of the ongoing $\omega_a$ analysis for the last three datasets, collected from 2020 to 2023, along with the projected uncertainties on the final Muon $g-2$ measurement at Fermilab.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

First data from the CUPID-Mo neutrinoless double beta decay experiment

The CUPID-Mo experiment is searching for neutrinoless double beta decay in $^{100}$Mo, evaluating the technology of cryogenic scintillating Li$_{2}^{100}$MoO$_4$ detectors for CUPID (CUORE Upgrade with Particle ID). CUPID-Mo detectors feature background suppression using a dual-readout scheme with Li$_{2}$MoO$_4$ crystals complemented by Ge bolometers for light detection. The detection of both heat and scintillation light signals allows the efficient discrimination of $\alpha$ from $\gamma$&$\beta$ events. In this proceedings, we discuss results from the first 2 months of data taking in spring 2019. In addition to an excellent bolometric performance of 6.7$\,$keV (FWHM) at 2615$\,$keV and an $\alpha$ separation of better than 99.9% for all detectors, we report on bulk radiopurity for Th and U. Finally, we interpret the accumulated physics data in terms of a limit of $T_{1/2}^{0\nu}\,> 3\times10^{23}\,$yr for $^{100}$Mo and discuss the sensitivity of CUPID-Mo until the expected end of physics data taking in early 2020.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Excitation of solar p-modes

We investigate the rates at which energy is supplied to individual p-modes as a function of their frequencies nu and angular degrees l. The observationally determined rates are compared with those calculated on the hypothesis that the modes are stochastically excited by turbulent convection. The observationally determined excitation rate is assumed to be equal to the product of the mode's energy E and its (radian) line width Gamma. We obtain E from the mode's mean square surface velocity with the aid of its velocity eigenfuction. We assume that Gamma measures the mode's energy decay rate, even though quasi-elastic scattering may dominate true absorption. At fixed l, E(Gamma) arises as nu(exp 7) at low nu, reaches a peak at nu approximately equal 3.5 mHz, and then declines as nu(exp 4.4) at higher nu . At fixed nu, E(Gamma) exhibits a slow decline with increasing l. To calculate energy input rates, P(sub alpha), we rely on the mixing-length model of turbulent convection. We find entropy fluctuations to be about an order of magnitude more effective than the Reynolds stress in exciting p-modes . The calculated P(sub alpha) mimic the nu(exp 7) dependence of E(Gamma) at low nu and the nu(exp -4.4) dependence at high nu. The break of 11.4 powers in the nu-dependence of E(Gamma) across its peak is attributed to a combination of (1) the reflection of high-frequency acoustic waves just below the photosphere where the scale height drops precipitously and (2) the absence of energy-bearing eddies with short enough correlation times to excite high-frequency modes. Two parameters associated with the eddy correlation time are required to match the location and shape of the break. The appropriate values of these parameters, while not unnatural, are poorly constrained by theory. The calculated P(sub alpha) can also be made to fit the magnitude of E(Gamma) with a reasonable value for the eddy aspect ratio. Our resutls suggest a possible explanation for the decline of mode energy with increasing l at fixed nu. Entropy fluctuations couple to changes in volume associated with the oscillation mode. These decrease with decreasing n at fixed nu, becoming almost zero for the f-mode.

Goldreich, Peter↗

coh3

CoH3 (CoH ver.3) is an optical model, exciton pre-equilibrium, and Hauser-Feshbach statistical model code, which calculates nuclear reaction cross sections for medium to heavy targets in the keV to MeV energy region. This program is written in standard C++, divided into approximately 200 source and header files. CoH solves the Schroedinger equation for optical potentials defined in the code, and calculates differential elastic scattering, reaction, and total cross sections, for neutron, proton, deuteron, triton, 3He, and alpha-particle. Deformed optical potentials are solved with the coupled-channels method, in which the ground state rotational band members, or vibrational phonon states are coupled. The optical model gives particle transmission coefficients that are fed into the statistical model calculations. CoH includes the pre-equilibrium model (exciton model), the direct/semidirect capture model, and the multi-stage Hauser-Feshbach statistical decay with width fluctuation correction based on the Gaussian orthogonal ensemble. For weakly coupled levels, the DWBA (distorted wave Born approximation) method is used to calculate the direct inelastic scattering process to the excited states.

Kawano, Toshihiko↗

Spectrophotometry of prominences in the phase preceding decay

The results are presented of spectrophotometric processing of prominence spectra in both the quiet and the decay phases. A catalog was compiled of equivalent widths, central intensities, Doppler half-widths, and half-widths of emission lines. The reduced Doppler half-widths of D3 and of the H, K Ca(+) lines obtained in a prominence active phase are much larger than those obtained during a quiet phase. Comparison of the equivalent widths and central intensities of H sub alpha, H sub beta hydrogen and D3 helium lines shows that the values increase in the active phase for the D3 lines and decrease for the H sub alpha, H sub beta lines.

Rakhubovskiy, A. S.↗

The development of X-ray flare onsets near active region filaments

Skylab X-ray images of the early phases of six active region transient brightenings were compared with simultaneous H-alpha images to study the spatial relationships between filaments and the X-ray brightenings. When the X-ray loops were roughly perpendicular to the axes of the H-alpha filaments, the filaments did not disappear. X-ray loops which appeared nearly parallel to the filaments were generally associated with the disappearances of those filaments. It is suggested that the perpendicular loops correspond to the class I X-ray flares of Pallavicinic et al. (1977) while the parallel loops are the early phases of their class II flares characterized in the decay phases by arcades of large loops with low energy densities. Both kinds of X-ray flares can be associated with impulsive phases.

Kahler, S. W.↗

The stability properties of cylindrical force-free fields - Effect of an external potential field

A large-scale potential field with an embedded smaller-scale force-free structure gradient x B equals alpha B is studied in cylindrical geometry. Cases in which alpha goes continuously from a constant value alpha 0 on the axis to zero at large r are considered. Such a choice of alpha (r) produces fields which are realistic (few field reversals) but not completely stable. The MHD-unstable wavenumber regime is found. Since the considered equilibrium field exhibits a certain amount of magnetic shear, resistive instabilities can arise. The growth rates of the tearing mode in the limited MHD-stable region of k space are calculated, showing time-scales much shorter than the resistive decay time.

Chiuderi, C.↗

Solar gradual hard X-ray bursts and associated phenomena

White-light coronagraph, H-alpha and radio data are presented as well as hard X-ray data for a sample of 10 gradual hard X-ray bursts (GHBs) in an attempt to better understand the nature of these events. It is found that: (1) the hard X-ray photon energy spectrum began to harden near the onset of the GHBs and continued in this fashion during the decay phase; (2) a coronal mass ejection (CME) occurred in association with at least nine of the GHBs; (3) the GHBs occurred in the late phase of major flares; (4) the centimeter wavelength bursts associated with the GHBs had relatively low frequency spectral maxima, and in relation to the observed hard X-ray emission, they were microwave-rich; (5) the associated decimetric bursts showed significant intensity variations on time scales ranging from 0.1 to approximately greater than 1 minute; and (6) the GHBs were most strongly associated with type IV events. It is concluded that the acceleration and trapping of radiating electrons occurs in the postflare loop systems following CMEs.

Cliver, E. W.↗

Properties of an impulsive compact solar flare determined from Solar Maximum Mission X-ray measurements

Soft X-ray, hard X-ray magnetogram, and H-alpha data have been analyzed for an impulsive compact solar flare which occurred on May 21, 1985. The derived flare loop dimensions are about 20,000 km length and about 150 km diameter. Measurements of line ratios from the Mg XI ion indicate that the plasma density varied from about 4 x 10 to the 12th/cu cm early in the flare to about 10 to the 12th/cu cm during the flare decay. The initial temperature of this plasma was about 8 x 10 to the 6th K and dropped to about 5 x 10 to the 6th K during the decay phase. The simplest interpretation of the event is one in which the source of the soft X-ray flare emission is confined to a thin loop of very high density.

Linford, G. A.↗

Time-Resolved Radioluminescence of the Polynuclear Copper(I) Phosphor Cu4I6²–. Different Temporal responses to Photo, X-Ray, β-Ray and α-Particle Excitation

Described for the first time are the time-resolved radioluminescence (TRRL) properties of the highly luminescent copper(I) cluster Cu4I62– using X-ray, b-ray and a-particle excitation. The copper(I) phosphors are two crystalline salts of this anion, [Na2(18-crown-6)2(H2O)3][Cu4I6] (I) and [Li(benzo-15-crown-5)2(H2O)]2[Cu4I6] (II), that had been shown to display strong photoluminescence (PL) when excited with ultraviolet light. The integrated radioluminescence (RL) spectra observed when pulsed X-rays were used as the excitation source are virtually the same as the PL spectra under comparable conditions. These temporal RL spectra are invariant at all observation times indicating that the observed scintillation occurs from a common excited state (or set of excited states). When the TRRL is collected from excitation with a pulsed X-ray source, b-ray decay from 90Sr or a-decay from 244Cm, the longer components (>2 μs) of the TRRL displayed (in each case) lifetimes comparable to those of the strictly exponential PL decays recorded under pulsed laser UV excitation. However, at shorter observation times (< 500 ns), the RL decay deviated from the exponential model, indicating a markedly different temporal luminescence behavior when these materials were excited with pulsed high energy radiation. Furthermore, this effect was the most pronounced for the a-particle excitation. These results suggest that the absorption of a very high energy X-ray photon, b-ray or a-particle at a site within the crystalline solid leads to a high local density of electronic excited states and that coupling between these states provides an alternative channel for excited state decay. Given that the patterns observed

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Low Level Calibration of Liquid Scintillation Counting

Liquid Scintillation Counting (LSC) is an analytical laboratory method that quantifies the concentrations of alpha and beta emitting isotopes. The LSC method can be utilized for the detection of tritium, both environmentally and at nuclear facilities. Most LSC samples are aqueous-based and prepared as a radioactive sample dissolved or suspended in a high efficiency scintillation cocktail that converts radioactive energy into light pulses. When placed in counting vials, the liquid scintillation cocktail allows for optical coupling in which energy is released from the samples radioactive decay, and transferred to the scintillator. That energy is then absorbed to produce excited electrons that fall back to their ground-state and emit a pulse of light that is detected by the liquid scintillation analyzers photomultiplier tubes. Quench is a signal attenuation due to physical, chemical, or color interferences. To compensate for quench, quench standards of a known concentration are implemented at increasing increments of quench per vial to create a quench curve. Quench standards can be purchased pre-made or customized from the manufacturer, however, there are several issues that arise from purchasing the pre-made quench standards. The main issues with ordering pre-made quench standards is that they use higher count values, between 30,000 and 250,000 disintegrations per minute (dpm) of tritium per vial and only come in glass vials. Using higher counting standards in glass vials makes it hard to see lower concentrations in plastic vials. Additionally, when using higher energy standards the accuracy of the calibration readings tend to be lower. On the other hand, making a set of quench standards in-house allows for the customization of the dpm concentration to roughly 1,500-3,000 and preparation in plastic vials. This allows for lower activity readings that results in closer precision of the samples' true concentration. Technical Objectives: Create a quench curve and calibrate the LSA for tritium. Verify the calibration of the quench curve prior to cross sample runs. Check calibration against Quality Control (QC) reference value. Conclusion: a tritium quench curve calibration was performed using a scintillation cocktail with ultima gold (AB and AB/F), acetone (only with AB), and water (only with AB/F). By performing the tritium quench curve calibration, the counting efficiency was correlated to various levels of quench. Calibration checks with quality control standards were also performed to verify that the calibration was correct. The observed results provided acceptable values that matched the quality control standard reference values with an acceptable uncertainty. The next step will be fine tuning and cross comparison checks with legacy instrumentation.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

X-Ray Flare Characteristics in the B2e Star Lambda Eridani (ROSAT)

We document the results of a simultaneous wavelength monitoring on the B2e star (lambda) Eri. This campaign was carried out from ground stations and with the ROSAT, ASCA, IUE, and Voyager 2 space platforms during a week in February-March 1995; a smaller follow-up was conducted in September 1995. During the first of these intervals (lambda) Eri exhibited extraordinary wind and disk-ejection activity. The ROSAT/HRI X-ray light curves showed no large flares such as the one the ROSAT/PSCA observed in 1991. However, possible low level fluctuations in the February-March ROSAT data occurred at the same time as unusual activity in H(alpha) He I (lambda)6678, He II (lambda)1640, and the C IV doublet. For example, the hydrogen and helium lines exhibited an emission in the blue half of their profiles, probably lasting several hours. The C IV lines showed a strong high-velocity Discrete Absorption Component (DAC) accompanied by unusually strong absorption at lower velocities. The helium line activity suggests that a mass ejection occurred at the base of the wind while the strong C III (Voyager) and C IV (IUE) lines implies that shock interactions occurred in the wind flow. It is not clear that the X-ray elevations are directly related to the strong C IV absorptions because the former changed on a much more rapid timescale than absorptions in the C IV lines. Within hours of the mild X-ray flux variations found by ROSAT on February 28, the Voyager UVS observed a "ringing" that decayed over three 3-hr. cycles. The amplitude of these fluctuations was strong (50%) at (lambda)(lambda)950-1100, decreased rapidly with wavelength, and faded to nondetection longward of (lambda)1300. Various considerations indicate that these continuum variations were not due to an instrumental pathology in the UVS. Rather, they appear to be due to a time-dependent flux deficit in the (lambda)(lambda)950-1250 region. We outline a scenario in which a dense plasma structure over the star's surface is heated and cooled quasi-periodically to produce such flux changes. Observations of new examples of this phenomenon are badly needed. Amateur astronomers can make a significant contribution to its understanding by searching for ringing in light curves of Be stars during their outburst phases. Finally we draw attention to an increase in the emission of the H(alpha) line that occurred at about the time the FUV ringing started. This increased emission hints that approximately 50,000K plasma near the star's surface can influence the circumstellar disc at approximately 12R. by its increased Lyman continuum flux.

Smith, Myron A.↗