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Phonon states effective density in neodymium trichloride from vibronic spectra accompanying electronic transitions in trivalent Pr and Nd ions
Computer program to predict spectra from electronic transitions of diatomic molecules and atoms, noting line intensity distribution by Voigt profile
Electron energy spectra construction from Al, Sn and Au target layers transmission angular distribution measurements, using computer calculated spectra for comparison
Electron scattering spectra of CO2 are reported in the 7 to 10 eV energy-loss range, at energies of 0.2, 0.35, 0.6, 0.7, and 7.0 eV above threshold, and at a scattering angle of 90 deg. Several new distinct overlapping continua with weak, diffuse bands superimposed are observed to lie in this energy-loss range. The experimental spectra are discussed in the light of recent ab initio configuration-interaction calculations of the vertical transition energies of CO2. The experimental spectra are shown to be consistent with the excitation states of CO2.
Electron scattering spectra of nitrous oxide are reported in the 5- to 10-eV energy-loss range at scattering angles of 20, 30, 90, and 130 deg at a residual energy of 7.0 eV; and at residual energies of 10.0, 2.0, 1.0, 0.6, and 0.2 eV at a scattering angle of 90 deg. Several new distinct and overlapping continua are observed to lie in this energy-loss range. The experimental spectra are discussed in the light of semiempirical INDO calculations of Chutjian and Segal (1972) of the vertical transition energies of N2O. An assignment of the symmetries of the observed excitations consistent with the experimental and theoretical data is suggested.
The penetration, diffusion and slowing down of electrons in a semiinfinite air medium has been studied by the Monte Carlo method. The results are applicable in the atmosphere at altitudes up to 300 km. Most of the results pertain to monoenergetic electron beams, with energies between 2 keV and 2 MeV, injected into the atmosphere at a height of 300 km, either vertically downwards or with a pitch-angle distribution isotropic over the downward hemisphere. Some results were also obtained for various initial pitch angles between 0 and 90 deg. Information has been generated concerning the backscattering of electrons from the atmosphere, the altitude dependence of energy deposition by electrons and by secondary bremsstrahlung, and the evolution of electron flux spectra as function of the atmospheric depth.
A high time resolution electron detector has been developed for use in sounding rocket studies of the aurora. The detector is used to look for particle bunching in the range 50 kHz-10 MHz. The design uses an electron multiplier and an onboard frequency spectrum analyzer. By using the onboard analyzer, the data can be transmitted back to ground on a single 93-kHz voltage-controlled oscillator. The detector covers the 50 kHz-10 MHz range six times per second and detects modulation on the order of a new percent of the total electron flux. Spectra are presented for a flight over an auroral arc.
The report discusses completed and proposed research in atomic and molecular physics conducted at the Columbia Radiation Laboratory from July 1972 to June 1973. Central topics described include the atomic spectra and electronic structure of alkali metals and helium, molecular microwave spectroscopy, the resonance physics of photon echoes in some solid state systems (including Raman echoes, superradiance, and two photon absorption), and liquid helium superfluidity.
Flux profiles which were derived from data returned by Pioneer 10 during Jupiter encounter, form the basis for a new set of numerical models for the energy spectra of electrons and protons in Jupiter's inner magnetosphere.
A large data base obtained from NASA Convair auroral expeditions is used to illustrate the variability in 6300A/4278A and 5577A/4278A ratios in auroras. The variation is well bounded by theoretical curves for characteristic spectral energies between 0.3 and 10 keV, which are typical for auroral precipitation. Coordinated measurements with the OV1-18 satellite show good agreement between the parameters of the precipitating-proton and electron-energy spectra derived from photometric measurements and those measured directly.
A procedure has been developed whereby nitrogen can be incorporated into an organic film from an ethylene-nitrogen gas mixture using an internal electrode capacitively coupled radio frequency reactor. The presence of nitrogen has been shown directly by infrared transmittance spectra and electron spectroscopic chemical analysis data, and further indirect evidence was provided by dielectric measurements and by the reverse osmosis properties of the film. Preparation of a nitrogen containing film did not require vapor from an organic nitrogen containing liquid monomer. Some control over the bonding and stoichiometry of the polymer film was provided by the added degree of freedom of the nitrogen partial pressure in the gas mixture. This new parameter strongly affected the dielectric properties of the plasma polymerized film and could affect the reverse osmosis behavior.
A structure, quite different from inelastic tunneling peaks, has been observed in electron-tunneling spectra of MOM junctions. A capacitance peak is associated with this structure, which is attributed to traps in the oxide at energies smaller than those previously reported. The C-V characteristics calculated using a single-energy trap model agree with experimental results; however, no satisfactory explanation has yet been found to account for the strong temperature dependence of the trap energy levels.
Plasma electron observations made onboard Mariner 10 are reported. Three encounters with the planet Mercury show that the planet interacts with the solar wind to form a bow shock and a permanent magnetosphere. The observations provide a determination of the dimensions and properties of the magnetosphere, independently of and in general agreement with magnetometer observations. The magnetosphere of Mercury appears to be similar in shape to that of the Earth but much smaller in relation to the size of the planet. Electron populations similar to those found in the Earth's magnetotail, within the plasma sheet and adjacent regions, were observed at Mercury; both their spatial location and the electron energy spectra within them bear qualitative and quantitative resemblance to corresponding observations at the Earth. The magnetosphere of Mercury resembles to a marked degree a reduced version of that of the Earth, with no significant differences of structure.
The following transitions are observed in the electronic absorption spectra of lunar titanaugites: Fe(2+) spin-allowed and spin-forbidden crystal field; Ti(3+) spin allowed and Jahn-Teller split crystal field; Ti(3+)-Ti(4+) CT; Fe(2+)-Ti(4+) CT; and O(2-)-Fe(2+), Ti(3+), Ti(4+) CT. Of these, the transitions involving Ti(3+) are unique to lunar or nonferric-bearing titanaugites. All titanaugites have the Fe(2+) crystal field and Fe(2+)-Ti(4+) CT transitions in common. These features in the diffuse reflectance spectra of lunar materials give rise to the '1.0 band' and to the observed absorption around 0.5-0.6 micron, respectively. Since regolith contains a variety of phases with coexisting Fe(2+), Ti(3+), and Ti(4+) ions, several metal-metal charge transfer processes are possible.
The paper demonstrates that information about Saturn's Ring E particle size is potentially obtainable from observations of Saturnian trapped radiation. It is shown that observations of the radial dependence of the intensities, energy spectra, electron-to-proton intensity ratio, and pitch angle distributions of energetic charged particles trapped outside of Ring A can potentially provide information (1) on the existence of Ring E, (2) on the effective size of the particulate matter therein, and (3) on the magnitude of the radial diffusion coefficient for energetic particles. A parametric study of these possibilities is specialized to the characteristics of the University of Iowa detectors on Pioneer 11 which was scheduled to make a close encounter with Saturn in 1979.
The various manifestations of energetic particles in solar flares are examined, and possible mechanisms for the acceleration of these particles are considered. Hard X-ray observations and possible mechanisms for the production of the dominant form of solar energetic particles, electrons with energies between 10 and 100 keV, are discussed, with consideration of thin-target models, thick-target models and thick-target models with reverse currents, and first-phase acceleration mechanisms for energetic electrons emitting impulsive microwave and fast-drift Type III radio bursts as well as impulsive hard X rays, which are detected themselves 20 min after the flare at 1 AU are considered. Radio evidence on the number, energy and pitch-angle distributions of energetic particles produced during solar flares is summarized, and observations at 1 AU of proton and electron energy spectra, the proton/electron ratio and energetic particle events rich in He-3 from solar flares are discussed. Finally, consideration is given to gamma-ray evidence of nuclear reactions in flares and white-light flares
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