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At least 289 records · Page 16

Source term analysis of FeCrAl accident tolerant fuel using MELCOR

It has been established that incremental improvements in beyond design basis accident performance can be achieved through accident tolerant fuel (ATF). However, they have the potential to recover margin with respect to conventional fuel and therefore enhance plant economics through uprate or cycle length increase. To realize this potential, it is necessary to quantify the reduction in source term due to use of ATF, and correspondingly how this is affected by increasing the cycle length and/or burnup. This requires development of a risk informed analysis methodology for ATF under high burnup conditions, which is being developed within LWRS. To this end, a MELCOR simulation of FeCrAl ATF in a recovered Large Break LOCA (LBLOCA) scenario has been developed, using a model based on the Zion Pressurized Water Reactor (PWR). The new user defined material capability, along with the inclusion of detailed neutronics- and depletion-derived parameters such as core power distribution, decay heat behavior, and fission product inventories, allows a more detailed simulation of FeCrAl clad material properties and behavior than has previously been possible using MELCOR. These detailed FeCrAl results were compared with a zircaloy clad model to investigate the differences between the two clad types and quantify the benefits of FeCrAl ATF with an 18-month cycle. Next, the fuel cycle with ATF was extended to 24 months, to determine whether any additional safety margin provided by FeCrAl ATF could be leveraged to implement high burnup FeCrAl-clad fuel while retaining the same operating and safety limits as current zircaloy-clad fuel. For the particular scenario analyzed, the delay to fuel failure from using ATF was of the same order as the LOCA recovery time, and hence significant in reducing fission product release, with the 24-month FeCrAl core performing better than the 18-month zircaloy core. It is noted that for other transients, the reduction in release due to using FeCrAl may be less significant. Furthermore, the material model developed here can be used in such further studies in support of determining the overall source term.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

User Manual for the Thermal Hydraulic Code SE2RCT

SE2-ANL is a modified version of SUPERENERGY-2 which interfaces the power distribution in the ANL maintained physics codes for the user. SE2RCT is a special version of SE2-ANL developed for specific use on models of the Experimental Breeder Reactor-II (EBR-II). SE2RCT fulfills a specific role in the calculated results as part of the Fuels Irradiation and Physics Database (FIPD) and is built to connect with the Physics and Analysis DataBase (PADB) for metallic fuel research and development in advanced sodium-cooled fast reactors (SFRs) created for EBR-II. SE2RCT is primarily a thermal analysis code that interfaces with the RCT based pin power details instead of the built-in pin power dehomogenization strategy in SE2-ANL. Beyond the thermal hydraulic calculation, the SE2RCT code provides detailed axial distributions of the RCT calculated results. SE2RCT also calculates the the axial distribution of pin wise DPA for the cladding materials which is part of the FIPD calculated results. This report serves as the user manual for SE2RCT and thus eliminates the QA gap of missing documentation on the SE2RCT software. All of the features and limitations of SE2RCT are documented in this report. The input and output specifications of SE2RCT are discussed in detail, and some unique features of SE2RCT, e.g. accurate pin power and temperature results for problems with non-uniform composition within an assembly, are also demonstrated and tested.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Loss of Flow Conditions in a Modern Pool-type SFR and In-Pile Experiment Design

The metallic fuel safety performance under unprotected design-basis transients is a key consideration for the deployment of advanced sodium fast reactors (SFRs). Reliable data are needed to validate advanced safety codes, reduce uncertainty in cladding failure thresholds, and strengthen confidence in licensing approaches. To address this need, this report develops blueprints for a conceptual sodium loss-of-flow (LOF) experiment in the Mk-IIIR loop at the Transient Reactor Test Facility (TREAT), providing the technical foundation for future integral testing.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

ECAR-7932 Rev 0 Large Eddy Simulation of MARVEL Reactor Core Subchannel to Evaluate Model Uncertainty of Reynolds-Averaged Navier-Stokes Equation Based Computational Fluid Dynamics Analysis

In the previous work (ECAR-7210), the peak cladding temperature of the MARVEL microreactor has been evaluated by steady-state Reynolds-Averaged Navier-Stokes (RANS) based computational fluid dynamics (CFD) simulations. Although numerical uncertainties of RANS-based CFD simulations has been assessed in ECAR-7210, the model uncertainty of RANS turbulence models must be investigated to resolve the issues related to inaccurate prediction of turbulent heat flux and flow pulsation in a tight lattice rod bundle using the steady-state RANS simulations. Consequently, this ECAR conducted a high-fidelity CFD analysis utilizing Large Eddy Simulation (LES) to generate reference data and investigated the model uncertainty of RANS-based CFD simulations.

21 - SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLAN↗

Software Verification of VARPOW

The VARPOW program is a post-processing utility program for DIF3D, specifically DIF3DVARIANT, and it was developed to provide interface files for the thermal analysis program DASSH. The basic methodology of VARPOW is to take the neutron and gamma flux (moments) calculated by DIF3D (or GAMSOR) and combine them with the heating (coefficient) cross sections to calculate the spatial power distributions using the DIF3DVARIANT spatial basis. VARPOW can use the output from GAMSOR (both steady state neutron and gamma flux calculations) or standard DIF3D/REBUS calculations (neutron flux only). The correct approach for defining the power distribution is to use GAMSOR as its purpose was to properly compute the gamma heating throughout the modeled domain. The power desnities calculated by VARPOW are broken into fuel, cladding and coolant terms for which isotope-wise categorization is needed. VARPOW has built in options the user can select for the isotope categorization or VARPOW can import a file that details the isotope categorization. VARPOW can export the solution in the polynomial basis of DIF3D-VARIANT or the monomial basis of DIF3D-VARIANT. The purpose of this work is to verify the power distribution results calculated by VARPOW from both the GAMSOR and DIF3D input options and verify that the input and output options are consistent with the manual. Hand calculation and independent numerical calculation are used for this verification work.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Applying U.S. metal fuel experience to new fuel designs for fast reactors

With the increasing interest in small modular reactors or microreactors, developers are working to design and submit licensing approval requests of U–10Zr-fueled fast reactors. The developers and their proponents cite prior metal fuel experience (worldwide, but U.S. experience in particular for many developers) as the motivation and justification for their reactor concepts. The experience with metal fuel deployment in sodium-cooled fast reactors as well as the underlying irradiation testing database, provide a suitable basis for analytically justifying the use of metal fuel in new reactors. The evolution of metal fuel design and capability illustrates the importance of key fuel design parameters to consider in new applications of the prior experience: fuel smeared density, plenum-to-fuel volume ratio, the ratio of cladding radius to thickness, fuel composition, and cladding and duct materials. In-service operating and deployment conditions to be considered include fuel linear heat generation rate, fuel temperature, cladding temperature, peak burnup and peak fast fluence. Fuel designs and in-service conditions that are bounded by the database and experience are most easily addressed, but deviations from those previous parameters and conditions can be addressed by considering impacts on previously established behavior and applying other mitigating conservatisms, as appropriate. Here, the authors recommend any new deployment proceed with fuel surveillance and monitoring to mitigate risk, application of conservative measures to address uncertainties, and a fuel qualification program that addresses a range of in-service operating conditions with production fuel. The work reported should be of interest to students and regulators unfamiliar with metal fuel in fast reactors.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Large Eddy Simulation of Low-Reynolds-Number Turbulent Flow of Low-Prandtl-Number Fluid in a Tight Lattice Bundle for Assessment of Reynolds-Averaged Navier-Stokes Turbulence Model

The MARVEL (Microreactor Applications Research Validation and Evaluation) microreactor utilizes natural circulation as core cooling mechanism and liquid metal as a primary coolant. Moreover, the reactor core has a pitch-to-diameter ratio of 1.056, which is considered a tight lattice configuration. Numerous studies have widely reported that Reynolds-Averaged Navier-Stokes (RANS) turbulence models inaccurately predict heat transfer in liquid metals and fail to capture flow pulsations that can occur within tight lattices, leading to further inaccuracies in simulation results. Therefore, evaluating the accuracy of RANS turbulence models in the thermal-hydraulic analysis of the MARVEL microreactor core is crucial for assessing reactor safety. In this study, a Large Eddy Simulation (LES) of the MARVEL microreactor core subchannel was conducted and compared with a RANS simulation to evaluate the accuracies and conservatism of the RANS model. The flow pulsation in a tight lattice predicted by LES enhanced the heat transfer, whereas the RANS model underpredicted it. Consequently, the RANS model predicted the peak cladding temperature higher than the LES model, but the discrepancy between the two approaches was not significant due to the good thermal characteristics of the liquid metal. It can be concluded that the steady-state RANS model is effective for the thermal analysis of liquid-metal-cooled MARVEL microreactor core and can provide conservative predictions from a safety analysis perspective.

21 - SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLAN↗

Characterization of Large Batch 14YWT Heat (NFA-2) for JOYO Irradiations (Rev.1)

The development and deployment of advanced cladding materials in advanced reactors requires the collection of relevant performance data for each cladding concept. Novel cladding concepts typically undergo significant innovation and iteration over the course of their development, and intention should be given to providing a snapshot of present performance. Thus, a modern heat of the nanostructured ferritic alloy (NFA) 14YWT is produced using state-of-the-art procedures for impurity minimization combined with thermomechanical processing methods designed to optimize fracture toughness, tensile strength, and ductility. This new heat of 14YWT, NFA-2, will provide the Advanced Fuels Campaign with adequate material for upcoming irradiation and mechanical testing campaigns. This report outlines procurement of new gas atomized 14YWT powder, production of four new bars of 14YWT, and subsequent mechanical and microstructural property characterization.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

DISCOVARY PROJECT: Material Background Report

UC/UO 2 composites have been proposed as a next generation fuel for light water reactors (LWRs). Accident tolerant fuels (ATF) have been a focus in the Advanced Fuels Campaign (AFC) to improve the safety and performance of LWRs and includes research and development efforts on the cladding and fuel. The 10 wt.% UC/UO 2 composite fuel was selected as a result of an extensive literature review and was selected due to the improvement of the fuel cycle cost. The inclusion of a UC phase in the composite material improves on the properties of standard UO 2 by increasing the uranium density of the fuel and increasing the thermal conductivity. Significant development has been carried out to refine the processing and sintering parameters and has led to a dense composite without ternary phases present. Characterization of the chemistry and microstructure has been carried out to send ahead of neutron irradiations in the Belgium Research Reactor (BR2) at SCK-CEN.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Full-core high-burnup BWR LOCA fuel performance analysis and FFRD susceptibility

The susceptibility of the boiling water reactor (BWR) Limerick Unit 1 to fuel fragmentation, relocation, and dispersal during a postulated large-break loss-of-coolant accident (LBLOCA) was calculated using a multiphysics framework. The simulations include full-core, rod-resolved neutronic, thermal hydraulic, and fuel performance models using the VERA, TRACE, and BISON codes. This work focused on the transient BISON simulations, which include both the normal operation and LBLOCA periods in the same simulations. Cladding integrity was assessed using two correlations that are included with BISON. make page break Several new BWR-specific features were recently added to BISON. This work represents the first time these features have been included in a core-scale set of simulations. This study hence evaluates the performance of these new models for an operating reactor with realistic operating conditions. Simulation results showed that cladding integrity was maintained (i.e., no rods burst). Finally, future work to improve BWR and PWR predictions using this framework is suggested.

BISON↗

Literature Review Investigating Adsorbents for Mercury Removal from Salt Batch Feed Material

The Savannah River Site (SRS) Liquid Waste System (LWS) contains mercury that originated from decades of canyon processing where it was used as a catalyst for dissolving aluminum cladding of reactor fuel. Since the start of radioactive operations, the Salt Waste Processing Facility (SWPF) has experienced processing difficulties due to the presence of mercury-laden solids. In response to these challenges, Savannah River National Laboratory (SRNL) has been requested by Savannah River Mission Completion (SRMC)/Salt Waste Processing Facility (SWPF) personnel to perform a literature review to assess the feasibility of chemical strikes to salt waste-containing tanks at the SRS as an option to reduce mercury introduction into SWPF. The literature review should evaluate known technologies and chemistries for decreasing mercury concentration and the anticipated efficacy of each technology on various mercury species known to exist in SRS waste.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Mechanical Property Assessment of Unirradiated Cladding After Exposure to Time at Temperature

Light water reactors in the United States are operated within inherent safety limits designed to account for anticipated operational occurrences (AOOs). Unlike more severe reactor transients, these events permit the potential reuse of reactor cladding, highlighting the nuanced role of thresholds in influencing reactor efficiency compared to design-basis or beyond-design-basis transient conditions. The threshold designated for AOO peak cladding and fuel temperatures are currently grounded around thermal hydraulic limits such as surpassing the critical heat flux (CHF), rather than in fuel-cladding material performance. This CHF criterion therefore represents a conservative approach to AOO transients during the reactor lifetime. Extending this threshold to higher temperatures than CHF can result in additional operation efficiency gains. Here, a material performance-based approach is assessed to better understand the physical material limits of short time scale exposures to elevated temperatures. This approach, termed time at temperature (t@T), references fuel cladding microstructural and mechanical response to rapid temperature transients in absence of radiation damage. The results of this work are expected to help identify margin for the United States reactor fleet, which could be utilized to increase operational efficiencies through decreased reactor outages.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Development of Large Bore Rabbit Capsules in Support of BWR Cladding Irradiations in HFIR

The High Flux Isotope Reactor (HFIR) is an ideal tool for materials irradiation testing because of its intense steady-state neutron flux. Many programs take advantage of HFIR’s central flux trap for irradiation experiments using capsules, also known as rabbits, to support advanced materials development and reactor design. The facility that makes up the HFIR flux trap has recently undergone a design change that increases the HFIR primary coolant volumetric flow rate by removing restrictions in the system. As a result, the usable cross-sectional area within the facility increased, opening the door to increase the cross-sectional area of the rabbit capsules that fill the facility. This report documents a new large-diameter rabbit housing that increases the usable volume within the rabbit capsule by 22.6%. However, challenges arise with increasing the capsule size, such as establishing a new maximum capsule operating pressure and determining the thermal-hydraulic characteristics. This report addresses those challenges with previously adopted HFIR safety methods. The rupture pressure of the rabbit housings is demonstrated while verifying that capsule swelling during and after rupture will not block coolant flow. Then, a safety factor is applied to ascertain an administrative operating pressure. Additionally, the thermal-hydraulic performance of the HFIR facility filled with large-diameter rabbit capsules is shown to not violate previously determined safety criteria. Next, heat transfer coefficients are determined for use in design calculations. Furthermore, this report gives an example of internal configurations for the new, larger rabbit capsules that use relevant boiling water reactor (BWR) cladding geometry. Finally, this report documents an example thermal design performance for a rabbit capsule containing six gauge-curved tensile tube specimens. The thermal performance gives predicted temperature distributions within the capsule and shows the expected temperature of the passive thermometers for post-irradiation temperature comparisons.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Material Characterization Report of EBR II Mark IV Fuel Element

The focus of this report is the characterization of an unirradiated as-built fuel element from the Experimental Breeder Reactor II (EBR-II) Mark IV driver fuel design. The fuel in this element is a metallic uranium-zirconium alloy, and the cladding material is HT9 stainless steel. Both the metallic fuel and cladding materials are characterized, including chemical composition, grain size, morphology, phase composition, precipitate composition, crystallography, density, and hardness.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

STAT7 v1.2 User Guide: The STAT7 Code for Statistical Propagation of Uncertainties in Steady-State Thermal Hydraulics Analysis of Plate-Fueled Reactors

The STAT7 software was developed to perform steady-state, single-phase thermal hydraulics analysis of plate-fueled reactors based on statistical propagation of uncertainties. Application of the software is for non-power research and test reactors, including conversion to low-enriched uranium fuel of U.S. High-Performance Research Reactors such as Massachusetts Institute of Technology Research Reactor. Since it can be necessary to repeat analysis during fuel reloading, STAT7 accommodates flexibility in analyzing many realistic aspects of reactor fuel management. STAT7 uses a Monte Carlo approach to model uncertainty in common fuel fabrication parameters and other key reactor operating parameters required for thermal hydraulics analyses of research and test reactors. These safety calculations are ultimately intended to protect against high fuel plate temperatures due to critical heat flux, or onset of flow instability. STAT7 supports water properties based on the IAPWS-IF97 functions (The International Association for the Properties of Water and Steam Industrial Formulation 1997 for the Thermodynamic Properties of Water and Steam) in addition to the fit functions. STAT7 predicts axial profiles of fuel, cladding, and coolant temperature along a lateral stripe that runs the full length of the fuel plate from the bottom to the top. STAT7 can simultaneously analyze all of the axial nodes of all of the fuel plates and all of the coolant channels for one latera stripe of a fuel element. Power splits are calculated for each axial node of each plate to determine how much of the power goes out each face of the plate. By running STAT7 multiple times, full core analysis can be performed by analyzing the margin to onset of nucleate boiling and onset of flow instability for each axial node of each stripe of each plate of each fuel element in the core.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Computational Investigation of Fuel Dispersal Phenomena during Large-Break Loss of Coolant Accident in Light-Water Reactors

In the event of cladding rupture, which could occur in light water reactor fuel assemblies during a loss-of-coolant accident (LOCA), fuel particles, along with fission gases, can be expelled into the reactor core from the fractured fuel rod. This expulsion of fragmented fuel particles, referred as fuel dispersal, is the subject of investigation to evaluate the safety implications of increasing fuel burnup in light water reactors, with a specific focus on fuel fragmentation, relocation, and dispersal. Particle trajectories and the resulting mass distribution of the settled particles within the reactor pressure vessel can pose a long-term cooling challenge for the reactor core. The fuel dispersal phenomenon is significantly influenced by the ejection characteristics of the fuel fragments, as well as the size and shape of the cladding rupture and fuel rod depressurization history during LOCA transients. In this study, the transport of fuel particles within a scaled 5 × 5 lattice of a pressurized water reactor rod bundle geometry is modeled through a two-fluid Eulerian framework that treats the gas and solid phases as interpenetrating continua. The required boundary conditions are evaluated from the fuel performance code BISON in a postulated large-break LOCA scenario. The modeling framework considers solid fuel particles as granular matter, interacting with the gaseous dry steam phase and fission gases through the governing interfacial momentum and energy exchange between the gas and solid phases. The simulation results provide the volume fraction of the solids settled on the bottom surface of the fuel bundle, quantifying the deposition within the bundle geometry.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

The Impact of the Halden Reactor Project on the Development of the Bison Fuel Performance Code

The Bison fuel performance code has been under development at Idaho National Laboratory by various programs within the U.S. Department of Energy since 2009. As part of any fuel performance code development, validation is necessary. To this end, several Halden experiments have been used. Early on, the focus was on validating the thermal mechanical behaviour, including pellet cladding mechanical interaction and fission gas release models implemented in Bison. Support for design-basis accident capabilities began in approximately 2014. Also in 2014, the development of models for accident tolerant fuel (ATF) concepts also began. This includes dopedUO2 fuel for which Halden has some experiments with temperature and fission gas release measurements. The Bison team has been fortunate to have two senior developers be secondees to Halden for a year: the late Dr. Giovanni Pastore from May 2015 to April 2016 and the now retired Dr. Richard Williamson in 2018. The paper will provide examples of Bison validation using Halden data for standard UO2 fuel under normal operation and loss-of-coolant accident condition, and ATF concepts. A tribute to the legacy that both the late Giovanni and retired Richard left on the Bison code is provided.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Nanostructured Alumina Forming Austenitic Alloy (NAFA) Production using Advanced Manufacturing

Alumina-forming austenitic (AFA) alloys are well known for their exceptional corrosion-resistant properties due to the formation of a dense oxide scale beneficial in their application as a nuclear material. However, use of the alloys in core material applications is limited due to the high nickel-transmutation and helium generation rate in service, leading to swelling and reduced lifetimes. Enhancing the sink strength to pin gas bubbles and increasing gas management of the material may mitigate many of the degradation phenomena expected during alloy deployment (such as high-temperature helium embrittlement and cavity swelling for lead-cooled fast-reactor applications). Nanostructured materials are usually produced using a time-consuming and expensive batch process like mechanical alloying to achieve the fine homogenous distribution of nanoprecipitates throughout the matrix material. Integrating the nanoprecipitates in modern additive manufacturing processes has proven difficult, as the required nano-sizes or number densities cannot be achieved simultaneously. Efforts to increase the number density of precipitates by adding more precipitate-forming rare-earth elements led to agglomeration of such elements, while the nano-sized precipitates did not form in sufficient quantity when not enough rare-earth element was use. In this work a novel approach to advanced manufacturing and the fabrication of Nanostructured AFA (NAFA) materials was chosen. A dual precipitate-forming NAFA steel with a chemistry more suitable for advanced reactor applications was produced to create an environmentally resistant, high-sink-strength austenitic alloy for advanced reactor cladding applications.

36 MATERIALS SCIENCE↗