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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 289 records · Page 16
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Two-proton decay from α-cluster states in 10 C and 11 N

Two-proton decay from excited states in 10 C and 11 N has been characterized from an analysis of the 2p + 2α and 3p + 2α exit channels. Data from four previously published invariant-mass studies associated with inelastic excitation, multinucleon knockout, and neutron pickup reactions have been considered. A rotational band in 10 C was identified built on the second 0 + state which has strong α-cluster molecular structure. The members of this band were tentatively identified up to J π = 4 + and all identified states have a prompt 2p decay branch. The spins of the 0 + and 2 + members were deduced from comparisons of the momentum correlations in their 2p branches to those from known 2p emitters. The 2 + and the tentative 4 + members are both above the α threshold and exhibit large reduced decay widths for α emission. This band exhibits a similar moment of inertia to its analog in the mirror nucleus 10 Be. Evidence is also presented for a molecular band in 11 N built on the second 3/2 – state which 2p decays. Furthermore, tentative members of this band have been assigned up to J π = 9/2 – and their excitation energies also match their likely analogs in the mirror nucleus 11 Be.

6 ≤ A ≤ 19↗
DOE OSTI2022

Search for neutrinoless β-plus-EC decay of 120 Te with CUORE

The Cryogenic Underground Observatory for Rare Events (CUORE) is a large-scale cryogenic experiment searching for neutrinoless double-beta decay (0νββ) in 130 Te. The CUORE detector is made of natural tellurium, providing the possibility of rare event searches on isotopes other than 130 Te. In this work we describe a search for neutrinoless positron-emitting electron capture (β + EC ) decay in 120 Te with a total TeO 2 exposure of 355.7 kg yr, corresponding to 0.2405 kg yr of 120 Te. Albeit 0νββ with two final-state electrons represents the most promising channel, the emission of a positron and two 511-keV γ 's make 0νβ + EC decay signature extremely clear. To fully exploit the potential offered by the detector modularity we include events with different topology and perform a simultaneous fit of five selected signal signatures. Using blinded data we extract a median exclusion sensitivity of 3.4 × 10 22 yr at 90% credibility interval (C.I.). After unblinding we find no evidence of 0νβ + EC signal and set a 90% C.I. Bayesian lower limit of 2.9 × 10 22 yr on 120 Te half-life. This result improves by an order of magnitude the existing limit from the combined analysis of CUORE-0 and Cuoricino.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2022

SS-HORSE extension of the no-core shell model: Application to resonances in He 7

Theoretical ab initio studies of resonances in the unbound 7 He nucleus are presented. We perform no-core shell-model calculations with NN interactions Daejeon16 and JISP16 and utilize the SS-HORSE method to calculate the S matrix for two-body channels n + 6 He and n + 6 He* with 6He respectively in the ground and excited 2 + states as well as for the four-body democratic decay channel 4 He + n + n + n. The resonant energies and widths are obtained by numerical location of the S-matrix poles. Here, we describe all experimentally known 7 He resonances and suggest an interpretation of an observed wide resonance of unknown spin-parity.

6 ≤ A ≤ 19↗
DOE OSTI2023

Measurement of the $\textit{B}(\textit{E}2 ↑)$ strengths of 36 Ca and 38 Ca

In this work, the $B(E2, 0^+_1 → 2^+_1)$ strengths of 36 Ca and 38 Ca are measured to be 131(20) $e^2\text{fm}^4$ and 101(11) $e^2\text{fm}^4$, respectively. The $\textit{B}(\textit{E}2)$ value for 36 Ca required a measurement of the p/γ branching ratio because the 2 + state is proton unbound. This branching ratio is $B_p$=0.087(8). These $\textit{B}(\textit{E}2)$ and branching-ratio values can be reproduced in the shell-model with the ZMB2 interaction, an interaction that predicts the $\textit{Z} = 20 \textit{sd}$-shell closure is incomplete with large proton pf-shell occupancies in the ground state. These occupancies are at odds with other shell-model and energy-density-functional calculations of 36 Ca. New data are used to provide an update on constraints of the density dependence of the symmetry energy through mirror charge-radii differences as well as to help reduce uncertainties of the astrophysical important 35 K(p,γ) reaction.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Structure studies of 13 Be from the 12 Be ⁢(𝑑,𝑝) reaction in inverse kinematics on a solid deuteron target

The low-lying structure of 13 Be has remained an enigma for decades. Despite numerous experimental and theoretical studies, large inconsistencies remain. Being both unbound and one neutron away from 14 Be, the heaviest bound beryllium nucleus, 13 Be is difficult to study through simple reactions with weak radioactive-ion beams or more complex reactions with stable-ion beams. Here, we present the results of a study using the 12 Be (𝑑,𝑝)⁢ 13 Be reaction in inverse kinematics using a 9.5 MeV per nucleon 12 Be beam from the ISAC-II facility. The solid deuteron target of IRIS was used to achieve an increased areal thickness compared to conventional deuterated polyethylene targets. The 𝑄-value spectrum below −4.4 MeV was analyzed using a Bayesian method with geant4 simulations. A three-point angular distribution with the same 𝑄-value gate was fit with a mixture of 𝑠- and 𝑝-wave, 𝑠- and 𝑑-wave, or pure 𝑝-wave transfer. The 𝑄-value spectrum was also compared with geant simulations obtained using the energies and widths of states reported in four previous works. As a result, it was found that our results are incompatible with works that revealed a wide 5/2 + resonance but shows better agreement with ones that reported a narrower width.

6 ≤ A ≤ 19↗
DOE OSTI2024

Formation of transfermium elements in reactions with Pb 208

Within the Langevin framework, we investigate the dynamics of the fusion process for production of transfermium elements in reactions of Ca 48 , Ti 50 , Cr 54 , and Fe 58 with Pb 208 . After the reacting nuclei have made contact, the early dynamical stage is dominated by the dissipation of the initial radial kinetic energy, while the subsequent shape evolution is diffusive. The probability for surmounting the inner barrier and forming a compound system is obtained by simulating the evolution as a Metropolis random walk in a five-dimensional potential-energy landscape. Good agreement with the available data is obtained, especially for the maximal formation probability. Published by the American Physical Society 2024

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Extending the Southern Shore of the Island of Inversion to F 28

Detailed spectroscopy of the neutron-unbound nucleus 28 F has been performed for the first time following proton/neutron removal from 29 Ne/ 29 F beams at energies around 230 MeV / nucleon . The invariant-mass spectra were reconstructed for both the 27 F(*) + n and 26 F(*) + 2n coincidences and revealed a series of well-defined resonances. A near-threshold state was observed in both reactions and is identified as the 28 F ground state, with S n ( 28 F) = -199(6) keV, while analysis of the 2n decay channel allowed a considerably improved S n ( 27 F) = 162(60) keV to be deduced. Comparison with shell-model predictions and eikonal-model reaction calculations have allowed spin-parity assignments to be proposed for some of the lower-lying levels of 28 F. Importantly, in the case of the ground state, the reconstructed 27 F + n momentum distribution following neutron removal from 29 F indicates that it arises mainly from the 1p 3/2 neutron intruder configuration. Finally, this demonstrates that the island of inversion around N = 20 includes 28 F, and most probably 29 F, and suggests that 28 O is not doubly magic.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

First Observation of the Four-Proton Unbound Nucleus 18 Mg

18 Mg was observed, for the first time, by the invariant-mass reconstruction of 14 O + 4p events. The ground-state decay energy and width are E T = 4.865(34) MeV and Γ = 115(100) keV, respectively. The observed momentum correlations between the five particles are consistent with two sequential steps of prompt 2p decay passing through the ground state of 16 Ne. The invariant-mass spectrum also provides evidence for an excited state at an excitation energy of 1.84(14) MeV, which is likely the first excited 2 + state. As this energy exceeds that for the 2 + state in 20 Mg, this observation provides an argument for the demise of the N = 8 shell closure in nuclei far from stability. Furthermore, in open systems this classical argument for shell strength is compromised by Thomas-Ehrman shifts.

6 ≤ A ≤ 19↗
DOE OSTI2022

Universal Properties of Weakly Bound Two-Neutron Halo Nuclei

We construct an effective field theory of a two-neutron halo nucleus in the limit where the two-neutron separation energy B and the neutron-neutron two-body virtual energy ε n are smaller than any other energy scale in the problem, but the scattering between the core and a single neutron is not fine-tuned, and the Efimov effect does not operate. The theory has one dimensionless coupling which formally runs to a Landau pole in the ultraviolet. We show that many properties of the system are universal in the double fine-tuning limit. The ratio of the mean-square matter radius and charge radius is found to be < r$^{2}_{m}$ > / < r$^{2}_{c}$ > = Af(ε n /B), where A is the mass number of the core and f is a function of the ratio ε n / B which we find explicitly. In particular, when B >> ε n , < r$^{2}_{m}$ > / < r$^{2}_{c}$ > = 2/3 A . Here, the shape of the E1 dipole strength function also depends only on the ratio ε n /B and is derived in explicit analytic form. We estimate that for the 22 C nucleus higher-order corrections to our theory are of the order of 20% or less if the two-neutron separation energy is less than 100 keV and the s-wave scattering length between a neutron and a 20 C nucleus is less than 2.8 fm.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Strontium-84 Enrichments in Presolar Grains Provide First Evidence of p -process Nucleosynthesis in Core-collapse Supernovae

This study reports detection of rare p-process isotopes within presolar grains. Presolar grains are relic dust grains from dying stars. These microscopic dust particles are found in primitive solar system materials. Their distinct isotopic compositions record the nucleosynthetic processes in their parent stars and the Galactic chemical environment in which these stars formed. We studied presolar graphite grains of high-density type from the Murchison meteorite and found five grains with subgrains that show enrichments in 84 Sr compared to the solar abundance. 84 Sr is the neutron-deficient isotope of strontium that can be produced in the deep oxygen-rich interior of high-mass stars that end their lives as core-collapse supernovae. The observed 84 Sr excesses cannot be produced in low-mass asymptotic giant branch stars, the source of most high-density presolar graphites found in meteorites. High-density graphites with embedded 84 Sr excesses are, instead, compatible with a core-collapse supernovae origin. The graphite subgrains condensed from carbon-rich materials in the outer layers of core-collapse supernovae, where 84 Sr was destroyed by neutron captures during hydrostatic evolution of the stars and their final explosion. Based on current theoretical stellar models, a few percent of contribution from the inner regions of core-collapse supernovae, which are enriched in p-process nuclides, to the outer carbon-rich regions is the most likely explanation for the observed enrichment of 84 Sr in the subgrains of the high-density graphites. In this study, we present the first observational evidence that core-collapse supernovae produce and eject isotopes made by the p-process.

Astronomy and AstroPhysics↗
DOE OSTI2020

Chemical Fractionation is not a Constant: Revisiting Bomb Vapor Chemistry

The debris produced by a nuclear explosion forms a hazard to response, can serve as a record used to interpret the event, and may persist in the environment necessitating long term management. Hence, understanding the radiochemical inventory of nuclear debris remains an important area of study, particularly the behavior and resulting distribution of actinides and fission products. Despite formation in a high energy environment, it has been recognized for decades that the chemical and isotopic composition of debris rarely, if ever, captures a homogenized blend of the bomb products. Instead, during cooling and debris formation, a variety of chemical processes cause separation of the different constituents. This process of chemical fractionation creates debris with a variety of different radionuclide inventories. Here we provide an overdue re-examination of our historic basis for understanding chemical fractionation in nuclear explosions through the context of new characterization of a large set of historical nuclear test data. Finally, we then discuss the implications of our findings for advancing models of radionuclide distribution and postdetonation chemical fractionation.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗
DOE OSTI2023

Rare K 40 Decay with Implications for Fundamental Physics and Geochronology

Potassium-40 is a widespread, naturally occurring isotope whose radioactivity impacts subatomic rare-event searches, nuclear structure theory, and estimated geological ages. A predicted electron-capture decay directly to the ground state of argon-40 has never been observed. Here, the KDK (potassium decay) collaboration reports strong evidence of this rare decay mode. A blinded analysis reveals a nonzero ratio of intensities of ground-state electron-captures (I EC 0 ) over excited-state ones (I EC $\star$ ) of I EC 0 /I EC $\star$ = 0.0095 $^{stat}_{±}$ 0.0022 $^{sys}_{±}$ 0.0010 (68% C.L.), with the null hypothesis rejected at 4σ. In terms of branching ratio, this signal yields I EC 0 = 0.098 % $^{stat}_{±}$ 0.023 % $^{sys}_{±}$ 0.010 % , roughly half of the commonly used prediction, with consequences for various fields [L. Hariasz et al., companion paper, Phys. Rev. C 108, 014327 (2023)].

39 ≤ A ≤ 58↗
DOE OSTI2023

Little vertical and circumferential variations in stem xylem water Δ 2 H and Δ 18 O in three tree species

Vertical and circumferential patterns of xylem water isotope signatures in large trees are rarely characterized but may influence interpretation of water source investigations and soil/xylem water isotope offsets. Furthermore, to examine vertical and circumferential variation in xylem water δ 2 H and δ 18 O, we collected xylem tissue at 5 heights (0, 1, 4, 7 and 10 m) from three replicate trees of three species with contrasting xylem anatomy, two angiosperms (Liquidambar styraciflua and Quercus nigra) and one gymnosperm (Pinus taeda). Concurrently, we also determined δ 2 H and δ 18 O of groundwater, soil water, and recent precipitation. On a different day, we collected circumferential samples at 1 m from the same trees to test for sectorality effects. Water from stem and soil samples were cryogenically extracted and analyzed for δ 2 H and δ 18 O. Mean xylem water δ 2 H and δ 18 O were significantly different between species, both vertically and circumferentially. We did not find significant (p = 0.05) systematic variation in δ 2 H or δ 18 O with height. We found no significant evidence for sectorality effects on δ 2 H, δ 18 O. Variances of vertical synoptic xylem water δ 2 H or δ 18 O were similar between species, 7.2–10.4‰ for δ 2 H and 0.58–0.81‰ for δ 18 O. Circumferential variances were also similar between species, 4.0–6.0 for δ 2 H and 0.37–0.44 for δ 18 O. A mixing model showed that sweetgum, water oak and loblolly pine, were drawing most of their water from deep soil from 45 to 190 cm (84.7, 68.4 and 53.2%, respectively) however, soil water-excess values indicate δ 2 H fractionation effects on these estimates. Dual isotope mixing model evaluation with single and multiple sample configurations showed that source water estimates were not affected by within tree variability of xylem water signatures. Xylem water δ 2 H and δ 18 O variability with height or circumference, was 3.2 and 2.7 times less than between tree variation because of transient temporal and spatial processes and is, therefore, not likely to affect interpretations of water sourcing in these three species.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2023

Spherical powders: Control over the size and morphology of powders for additive manufacturing and enriched stable isotope nuclear targets

Metal powders are a fundamental starting point for fabricating many types of nuclear targets. Elemental powder properties can differ drastically between batches, even when using the same method. Therefore, the variation in morphology and the size of metal powders can cause variable quality and produce inconsistent results with what are otherwise proven target manufacturing techniques. Additive manufacturing has additional requirements for higher quality and more uniform feedstock. The production of spheroidized powders with uniform, reproducible properties and a narrow size distribution represents unexplored opportunities for experiments. These opportunities include experimenting with solid metals that can now flow like liquids, new options for powder handling and dispensing, and new target fabrication methods using additive manufacturing. The Stable Isotope Materials and Chemistry Group at Oak Ridge National Laboratory obtained an AMAZEMET rePowder ultrasonic metal atomization tool for creating limited batches of fully dense, free flowing, spherical powders with a narrow size distribution of extremely rare materials. Early results are presented with materials that were produced. The team explores the anticipated limits of this instrument with extremely rare materials (e.g., enriched stable isotopes) and highlights research into new fabrication techniques that provide additional options benefitting the international nuclear target community.

Zach, Mike↗
DOE OSTI2025

Berkelium–carbon bonding in a tetravalent berkelocene

Interest in actinide–carbon bonds has persisted since actinide organometallics were first investigated for applications in isotope separation during the Manhattan Project. Transplutonium organometallics are rarely isolated and structurally characterized, likely owing to limited isotope inventories, a scarcity of suitable laboratory infrastructure, and intrinsic difficulties with the anaerobic conditions required. In this paper, we report the discovery of an organometallic “berkelocene” complex prepared from 0.3 milligrams of berkelium-249. Single-crystal x-ray diffraction shows a tetravalent berkelium ion between two substituted cyclooctatetraene ligands, resulting in the formation of berkelium–carbon bonds. The coordination in berkelocene resembles that of uranocene, and calculations show that the berkelium 5f orbitals engage in covalent overlap with the δ-symmetry orbitals of the cyclooctatetraenide ligand π system. Charge transfer from the ligands is diminished relative to uranocene and other actinocenes, which maximizes contributions from the stable, half-filled 5f 7 configuration of tetravalent berkelium.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗