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At least 289 records · Page 16
All sourcesNASA NTRSDOE OSTI
DOE OSTI2026

Light monitoring system for the lead tungstate calorimeter in Hall D at Jefferson Lab

A new electromagnetic calorimeter composed of 1596 lead tungstate (PbWO 4 ) scintillating crystals has been constructed for the GlueX detector in Hall D at Jefferson Lab. The calorimeter is equipped with a light monitoring system that uses light-emitting diodes. The light monitoring system was fabricated, installed, and integrated into the GlueX trigger system. It was successfully operated during detector commissioning and data collection, providing monitoring of the detector response and verification of the calibration with a precision better than 1%. In conclusion, the paper describes the design, installation, and performance of the light monitoring system.

Lead tungstate calorimeter↗
DOE OSTI2026

Dual particle imaging using time-of-flight neutron classification

Fast-neutron imaging technology is well-suited for passive nuclear material monitoring, secondary inspection of flagged cargo, and wide-area search for lost neutron sources. However, imaging systems that use pulse shape discrimination for event classification require complex pulse waveform analysis. In this work, we evaluate time-of-flight (TOF) based particle classification as an alternative solution for fast-neutron imaging by classifying all events with a TOF above a maximum threshold as neutrons. We measured a Cf-252 source next to Cs-137 using a 12-bar organic-glass scintillator array. By varying the TOF thresholds for neutron identification, we demonstrate a clear trade-off between event yield and backprojection image fidelity, with stricter thresholds improving precision at the cost of statistics, TOF thresholded data generated an image that predicted the neutron source direction with 20% reduced mean central angle prediction error compared to a traditional pulse shape discrimination (PSD) method with comparable event count. Time-of-flight particle classification shows promise as an alternative to pulse shape discrimination systems for fast neutron imaging systems looking to minimize costs and size of electronics with comparable imaging quality. The sources used demonstrate that the method is effective in classifying measured neutrons in a measurement environment with 150 μCi Cs-137 and 1.6 × 10 6 n/s Cf-252 sources positioned at distances of 66 cm and 81 cm from the detector. Additionally, the method classifies low-energy neutron events that pulse shape discrimination removes, so a combination of both methods would result in a higher overall neutron event efficiency.

Heriot, William [Univ. of Michigan, Ann Arbor, MI ↗
DOE OSTI2025

Characterization of dynamics and decay in the St. Benedict Paul trap

The St. Benedict experiment includes a linear Paul trap designed to measure the beta-neutrino angular correlation coefficient 𝑎 𝛽ν of mixed superallowed 𝛽-decay transitions between mirror nuclei via coincidence detection of 𝛽-particles and recoiling ions. The emitted 𝛽 particle and daughter ion are detected with plastic scintillators and micro-channel plate detectors, respectively, allowing for accurate measurements of their time-of-flights. From the shape of the coincidence time-of-flight distribution, a value of 𝑎 𝛽ν can be determined. This manuscript presents detailed simulations of the St. Benedict Paul trap, with a focus on ion cloud dynamics and recoiling daughter trajectories.

Linear Paul trap↗
DOE OSTI2025

Simulations of neutron unbound physics for Geant4

The study of neutron unbound systems via the invariant mass technique is the primary focus of the MoNA Collaboration, which built and operates the Modular Neutron Array (MoNA) and the Large multi-Institutional Scintillator Array (LISA) at FRIB. Advancements in nuclear structure from theory and experiment along the neutron dripline have presented opportunities to understand the nature of unbound systems in higher mass nuclei. The GEometry ANd Tracking (Geant4) platform has been used in high-energy and nuclear physics to simulate particle interactions with as much detail as the user desires. Geant4 currently does not have a physics class to simulate neutron unbound systems. Given the advancement of accelerator facilities and active searches along the neutron dripline, detailed simulations to study the breakup of neutron unbound systems, are necessary. Furthermore, the implementation of the breakup of neutron unbound systems in Geant4 will be presented.

Neutron dripline↗
DOE OSTI2025

A simulation pipeline for fast neutron imaging and spectroscopy using quantified detector attributes

Radiation imaging capabilities, essential in the nuclear nonproliferation regime, facilitate source localization and, in certain cases, spectroscopy. Scatter-based neutron cameras, which can measure the neutron signatures from special nuclear material, hold particular interest. Systems incorporating organic scintillators can extract neutron energy spectra, potentially distinguishing fission neutron sources from others, such as alpha-neutron sources. The development and testing of a scatter-based neutron imager, however, can be challenging without having an accurate simulation model or first constructing a prototype. This work describes a simulation pipeline that takes output from MCNPX-PoliMi simulations and creates the expected back-projection neutron images and neutron energy spectra. This pipeline was developed to improve the modeling of fast neutron imagers and bridge the current gap in literature, which predominantly focuses on gamma-ray Compton imager models. This work also reports on the significance of various real-world system considerations and their effects on the simulated detector responses. The pipeline was verified and validated with experimental data collected using a 252 Cf spontaneous fission source using a fast neutron scattering imager developed at the University of Michigan.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2025

Mild Hydrothermal Crystal Growth of Two Luminescing Uranyl Phosphates Exhibiting an Autunite-Type Sheet Structure

Two new layered uranyl phosphate compounds, K(UO 2 )PO 4 (H 2 O) 3 and Na(UO 2 )PO 4 (H 2 O) 1.52 , crystallizing in an autunite-type sheet structure, were successfully synthesized as both single-crystals and polycrystalline powders under mild hydrothermal conditions. The compound K(UO 2 )PO 4 (H 2 O) 3 crystallizes in the tetragonal crystal system with the space group P4/ncc, exhibiting lattice parameters of a = b = 6.99320(7) Å and c = 17.8389(3) Å. Similarly, Na(UO 2 )PO 4 (H 2 O) 1.52 also crystallizes in the tetragonal crystal system, however, in the space group P4/nmm and exhibits lattice parameters of a = b = 6.9787 Å and c = 8.6303(17) Å. Both compounds adopt layered structures, a characteristic feature of uranyl phosphates, and exhibit intense green fluorescence typical for uranyl-containing materials. As a result, the infrared spectroscopy, photoluminescence, and scintillation properties of these compounds were investigated.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2026

Ion-Specific Effects on PuO 2 Nanoparticle Aggregation and Dissolution in Concentrated Electrolytes

Hydrolytic PuO 2 nanoparticles (NPs) are a dominant aqueous Pu-bearing phase in high ionic strength nuclear wastes, yet their reactivity in nonideal brines remains poorly constrained. We quantify how electrolyte identity and concentration control PuO 2 NP aggregation and ligand-assisted dissolution in acidic, high salinity solutions (NaCl, NaNO 3 , NaClO 4 , Na 2 SO 4 , Na 2 C 2 O 4 up to 5 M). A multitechnique workflow combining liquid scintillation counting (operationally defined aqueous [Pu]), scattering/electrokinetic measurements (aggregate size and zeta potential), and spectroscopy (UV–vis, XPS, Raman) resolves electrolyte-dependent partitioning between colloidal and molecular Pu species. Weakly coordinating anions (ClO 4 – , Cl – , NO 3 – ) largely preserve the (aggregated) nanoparticulate fraction but generate distinct dissolved species at high concentration, i.e., Pu(IV)–nitrato complexes in NaNO 3 and Pu(VI)–chloro complexes in NaCl. In contrast, stronger ligands substantially perturb PuO 2 NP stability: sulfate promotes partial dissolution to Pu(IV)–sulfate complexes at low concentration but reduces aqueous [Pu] at higher sulfate levels via secondary Pu(IV) sulfate formation, whereas oxalate drives strong dissolution to aqueous Pu–oxalate complexes. Aged NPs show similar trends with reduced aqueous fractions and more dominant aggregation mechanisms. In conclusion, these spectroscopically constrained speciation data provide a foundation for incorporating PuO 2 NP reactivity into thermodynamic and reactive transport models for high salinity waste and brine environments.

Aggregation↗
DOE OSTI2026

Eutectic Processing of Semiconductor Colloidal Nanocrystals for Energy Applications

Colloidal semiconductor nanocrystals (NCs) offer a costeffective platform for light-energy conversion in X-ray scintillators, photovoltaics, lasers, and display technologies. Yet, device-relevant NCs often require complex heterostructured compositions, where lattice imperfections compromise the efficiency and stability of photoconversion processes. Here, we show that a simple synthetic detour through a eutectic state of II−VI semiconductor NCs (e.g., CdSe, ZnSe) with halide salts (e.g., CdCl 2 , ZnCl 2 ) overcomes this limitation by melting and reconstructing NC lattices into defect-free alloyed and core/shell architectures. Applied to ternary CdSeTe NCs, this process produces downconverters with record brightness and minimal line widths, delivering a 3-fold increase in film-side external quantum efficiency of commercial CdTe photovoltaic modules (First Solar Inc.). Meanwhile, eutectic processing of CdSe-based core/shell emitters yields an 8-fold enhancement in their photoluminescence stability under backlight operation, addressing the reliability bottleneck for display technologies. Together, these findings establish eutectic NC processing as a scalable route to efficient, durable photoconversion materials for energy applications.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2026

Optimized Photoemission from Organic Molecules in 2D Layered Halide Perovskites

In recent years, hybrid organic−inorganic metal halides have been at the forefront of materials research. Typically, the functional (e.g., optoelectronic) properties of hybrid halides are derived from the inorganic structural part, whereas the organic structural units can add extra advantages in terms of stability, rigidity, and processability. Here, we report the design, synthesis, and characterization of two new hybrid materials in which the outstanding photophysical properties originate from the organic structural part. The new compounds, (C 15 H 16 N) 2 CdCl 4 and ((Br)C 15 H 15 N) 2 CdCl 4 , have 2D layered Ruddlesden−Poppertype perovskite structures. These hybrids are blue-white light emitters just like their corresponding pure organic salts, but with much improved emission efficiencies. Optical spectroscopy and density functional theory (DFT) studies confirm that photoemission comes from the trans-stilbene organic cations. The photoluminescence quantum yield (PLQY) values of these new materials are among the highest known, 50.83% and 26.60% for (C 15 H 16 N) 2 CdCl 4 and ((Br)C 15 H 15 N) 2 CdCl 4 , respectively. This is up to a 5-fold increase as compared to the light emission efficiency of the precursor salt C 15 H 16 NCl (PLQY of 10.33%). Alongside their outstanding optical properties, their environmental and thermal stability allow their consideration for potential practical applications such as radiation detection. This work shows that hybrid metal halides can be compositionally and structurally engineered to have highly efficient photoemission originating from the organic components for fast scintillation applications.

Halogens↗
DOE OSTI2026

Terrestrial Gamma‐Ray Flash Following Intense Negative Return Stroke Observed With BIMAP‐3D

We report ground-based observations of a terrestrial gamma-ray flash (TGF) associated with a strong negative cloud-to-ground lightning strike (-CG) which occurred near Los Alamos National Laboratory (LANL) in New Mexico, USA. Gamma photons were detected by the Terrestrial High-energy Observations of Radiation (THOR) instrument, developed at the University of California, Santa Cruz, which has been hosted at LANL since 2022. Simultaneous measurements were also made with the 3-Dimensional Broadband Interferometric Mapping and Polarization (BIMAP-3D) system, which includes 3D lightning mapping, two fast antennas, and an additional plastic scintillator. Additional field change waveforms were obtained from the Earth Networks Total Lightning Network (ENTLN). The lightning initiated about 1 km above the ground, leading to a powerful -CG with an ENTLN peak current of −237 kA and bipolar field change matching the recently described “energetic compact stroke” (ECS) shape. The TGF was then observed ∼35 µs after the start of the return stroke. We also observe an electric field pulse likely produced by the TGF either in isolation or by coupling to the lightning channel. Based on modeling of the radiated electric field and photon propagation through the atmosphere we infer that the TGF source was on the order of 1⁢0 17 photons. This TGF and associated lightning are extremely similar to some recently reported ECS TGFs in coastal Japan in winter, but we report the first observation of this phenomenon outside of Japan in a different climate, terrain, and season.

58 GEOSCIENCES↗
DOE OSTI2024

Sensitive proton-radiation detectors

In this study, halide perovskite nanocrystal scintillators detect high-energy protons with sensitivity suitable for clinical applications.

36 MATERIALS SCIENCE↗
DOE OSTI2025

Search for light sterile neutrinos with two neutrino beams at MicroBooNE

The existence of three distinct neutrino flavours, ν e , ν μ and ν τ , is a central tenet of the Standard Model of particle physics. Quantum-mechanical interference can allow a neutrino of one initial flavour to be detected sometime later as a different flavour, a process called neutrino oscillation. Several anomalous observations inconsistent with this three-flavour picture have motivated the hypothesis that an additional neutrino state exists, which does not interact directly with matter, termed as ‘sterile’ neutrino, ν s . This includes anomalous observations from the Liquid Scintillator Neutrino Detector (LSND)3 experiment and Mini-Booster Neutrino Experiment (MiniBooNE), consistent with ν μ → ν e transitions at a distance inconsistent with the three-neutrino picture. Here we use data obtained from the MicroBooNE liquid-argon time projection chamber in two accelerator neutrino beams to exclude the single light sterile neutrino interpretation of the LSND and MiniBooNE anomalies at the 95% confidence level (CL). Moreover, we rule out a notable portion of the parameter space that could explain the gallium anomaly. This is one of the first measurements to use two accelerator neutrino beams to break a degeneracy between ν e appearance and disappearance, which would otherwise weaken the sensitivity to the sterile neutrino hypothesis. We find no evidence for either ν μ → ν e flavour transitions or ν e disappearance that would indicate non-standard flavour oscillations. Our results indicate that previous anomalous observations consistent with ν μ → ν e transitions cannot be explained by introducing a single sterile neutrino state.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Advances in detection for neutron reflectometry with time-resolved imaging detectors

Thermal neutron detection in neutron scattering science is a challenging endeavour due to a limited number of technologies which are sensitive to these weakly interacting particles. While many improvements to conventional detectors are underway at various facilities, there is a great opportunity to make a leap in performance by combining the spatial resolution benefits of imaging and the temporal resolution and background discrimination of event-driven radiation detectors. This idea has been realized by using a neutron sensitive scintillator read out by a single-photon sensitive camera based on a Timepix3 ASIC. We demonstrate how such data-driven imaging sensors can enable unprecedented performance in neutron reflectometry using the ASTERIX instrument at the Los Alamos Neutron Scattering Center. Several samples were measured with both the new and a conventional 3 He detector systems. The results from this work demonstrate that these imaging based systems can satisfy performance parameters for the future QIKR reflectometer to be built at the Second Target Station at Oak Ridge National Laboratory. Further improvements to the detector are already underway which will allow streamlined and expedited experiments. We demonstrate at least a two order of magnitude increase in detection rate at an acceptable dead time and introduce a new way of tuning the detector efficiency using light collecting optics to accommodate highly intense direct beams which cannot be measured with any current detectors without severe attenuation. This will allow measurements of complete reflectometry profiles and using a single sample measurement combined with fewer direct beam calibration measurements on QIKR and potentially other reflectometers.

36 MATERIALS SCIENCE↗
DOE OSTI2025

Detection and quantification of trace technetium in the presence of molybdenum using laser-induced breakdown spectroscopy

Technetium (Tc) is a very important element that is encountered in many aspects, from its presence in radioactive waste and its potential environmental impact to its use as a medical radioisotope. Its detection and quantification in liquid samples is traditionally cumbersome, involving detailed sample preparation and analysis by mass spectrometry or scintillation. This article demonstrates the first comprehensive emission spectral analysis of Tc from a liquid sample by immobilization in a polymer and analysis by laser-induced breakdown spectroscopy (LIBS). A survey of LIBS spectra was completed to identify the strongest analytical lines for quantification of trace Tc in the presence of Mo. The quantification of Tc in a Mo-containing matrix was selected because Tc radioisotopes are the daughter products of Mo isotope decay. The first reported calibration curves by LIBS are provided with limits of detection and quantification down to 0.710 µg mL −1 and 1.39 µg mL −1 , respectively. Ultimately, this study demonstrated the feasibility of trace Tc quantification using LIBS and will serve as a reference for future research related to monitoring this radioactive species.

Andrews, Hunter B. [Oak Ridge National Laboratory ↗
DOE OSTI2024

Alternatives to NIST Cf-252 Iirradiations for Transfer Calibration of S-32 Neutron Monitors

Gas-flow proportional counting systems are used by the Radiation Metrology Laboratory (RML) at Sandia National Laboratories for reactor fluence monitoring with the 32 S(n,p) 32 P reaction. Calibration of these systems has traditionally been accomplished by fluence-transfer irradiations at the NIST 252 Cf facility. Such calibrations have become increasingly difficult as the NIST 252 Cf source decayed to unusable levels. To minimize the risk to the testing programs from an inability to properly calibrate these systems, the RML has developed two alternative calibration techniques: 1) development and implementation of certified 32 P sources for activity calibrations and subsequent calculation of neutron fluence, and 2) direct counting of non-certified reactor-irradiated sulfur pellets by liquid scintillation counting to determine 32 P activity for the subsequent calibration of gas-flow proportional counters. Preliminary comparisons show that the several calibration methods are capable of overall uncertainties within about 5 percent.

Vehar, David W.↗
DOE OSTI2025

Lead tungstate calorimeter of the Jefferson Lab Eta Factory experiment

A new electromagnetic calorimeter (ECAL) consisting of 1596 lead tungstate PbWO 4 scintillating crystals has been fabricated and installed in the experimental Hall D at Jefferson Lab (JLab). The highgranularity, high-resolution calorimeter is required by the JLab Eta Factory experiment, whose main physics goal is to study rare decays of eta mesons. The ECAL replaced the inner part of the forward lead glass calorimeter of the GlueX detector. Signals from the detector will be digitized using twelve-bit flash analog-to-digital converters operated at a sampling rate of 250 MHz. The ECAL is integrated into the trigger system of the GlueX detector using electronics modules designed at JLab. The ECAL is currently at the commissioning stage and should be ready for the physics run in January 2025. We will give an overview of the JEF experiment, the design and construction of the ECAL, and the integration of the detector and its infrastructure into the Hall D experimental setup.

Somov, Alexander [Thomas Jefferson National Accele↗
DOE OSTI2025

Development of High-Granularity Dual-Readout Calorimetry with psec Timing

Dual-readout and particle flow algorithm (PFA) are technologies proposed for precise jet energy measurement in future colliders. While PFA requires highly granular calorimeters, dual-readout has mainly been used with fiber-based calorimeters that do not have highly segmented capabilities. It is still non-trivial to combine these two technologies in one calorimeter system because of the use of fibers in most of the dualreadout calorimeters, which is not compatible with the high granularity requirement of PFA technologies. The aim of this study is to develop a novel calorimetry that combines dual-readout and PFA by adopting a highly segmented tile-based configuration. This paper compares the improvement of energy resolution using dual-readout approach across several configurations of highly granular hadron calorimeters through simulation. Results indicate that setups with fine sampling and close placement of scintillators and Cherenkov detectors improve dual-readout performance.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2025

Overview of the front-end electronics of CMS HGCal - including readout and powering

The end-cap calorimeters of CMS will be upgraded to a single High Granularity Calorimeter (HG-Cal) for the HL-LHC, including both silicon sensors and scintillator tiles with on-tile SiPMs as active elements. The readout of the active elements is performed by an ASIC (HGCROC in 130 nm CMOS technology) that measures the amplitude and arrival time of the signals. The amplitude is measured over a large dynamic range to allow calibration with single particles and the measurement of TeV showers. The time of arrival of high-energy showers will be measured with a precision of around 30 ps. A second pair of “concentrator” ASICs - ECON-T and ECON-D - takes the data from the HGCROC channels and packages them for transmission via optical links to the off-detector electronics. The ECON-T transmits trigger data at 40 MHz, to form part of the level-1 trigger. The ECON-D transmits concentrated data packets at up to 1 MHz, upon reception of a level-1 trigger signal. In addition to these ASICs, HGCal will use modified versions of common HL-LHC electronics developments, for the power chain and the optical control and readout. The dense nature of the HGCal provides additional challenges for the electronic boards and cabling. In this proceedings the overall HGCal front electronics scheme, including the latest performance of the HGCROC and ECON ASICs is presented.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗