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Cosmology with the Laser Interferometer Space Antenna

The Laser Interferometer Space Antenna (LISA) has two scientific objectives of cosmological focus: to probe the expansion rate of the universe, and to understand stochastic gravitational-wave backgrounds and their implications for early universe and particle physics, from the MeV to the Planck scale. However, the range of potential cosmological applications of gravitational-wave observations extends well beyond these two objectives. This publication presents a summary of the state of the art in LISA cosmology, theory and methods, and identifies new opportunities to use gravitational-wave observations by LISA to probe the universe.

79 ASTRONOMY AND ASTROPHYSICS↗

Experimental targets for dark photon dark matter

Ultralight dark photon dark matter features distinctive cosmological and astrophysical signatures and is also supported by a burgeoning direct-detection program searching for its kinetic mixing with the ordinary photon over a wide mass range. Dark photons, however, cannot necessarily constitute the dark matter in all of this parameter space. In minimal models where the dark photon mass arises from a dark Higgs mechanism, early-Universe dynamics can easily breach the regime of validity of the low-energy effective theory for a massive vector field. In the process, the dark sector can collapse into a cosmic string network, precluding dark photons as viable dark matter. We establish the general conditions under which dark photon production avoids significant backreaction on the dark Higgs and identify regions of parameter space that naturally circumvent these constraints. After surveying implications for known dark photon production mechanisms, we propose novel models that set well-motivated experimental targets across much of the accessible parameter space. We also discuss complementary cosmological and astrophysical signatures that can probe the dark sector physics responsible for dark photon production.

Dark matter↗

Reconstructing the spatial structure of quantum correlations in materials

Quantum correlations are a fundamental property of quantum many-body states. Yet they remain experimentally elusive, hindering certification of genuine quantum behavior, especially in quantum materials. Here we show that the momentum-dependent dynamical susceptibility measured via inelastic neutron scattering enables the systematic reconstruction of a general family of quantum correlation functions, which express the degree of quantum coherence in the fluctuations of two spins at an arbitrary mutual distance. Using neutron scattering data for the compound KCuF 3 —a system of weakly coupled S = 1 / 2 Heisenberg chains—and numerically exact quantum Monte Carlo data, we show that quantum correlations possess a radically different spatial structure with respect to conventional correlations. Indeed, they exhibit a different emergent length scale—the quantum coherence length—which is finite at any finite temperature (including when long-range magnetic order develops). Moreover, we show theoretically that coupled Heisenberg spin chains exhibit a form of quantum monogamy, with a trade-off between quantum correlations along and transverse to the spin chains. These results highlight real-space quantum correlators as an informative, model-independent means of probing the underlying quantum state of real quantum materials. Published by the American Physical Society 2024

36 MATERIALS SCIENCE↗

GADRAS Batch Inject Tool User Guide

Gamma Detector Response and Analysis Software (GADRAS) is used by the radiation detection and emergency response community to perform modeling and spectral analysis for gamma detector systems. Built into GADRAS is the ability to define a detector, geometry, background characteristics and source composition to generate synthetic spectra for drills and exercises (injects). Consequence Management is currently in development of a sample result data simulator tool in which a deposition model is probed for source conditions at moments in time and locations in space. These values are used to generate realistic sample results for use in drills and exercises. In addition to sample results, there is a need to simulate the actual spectra that would be observed in the field by downlooking HPGe instruments given a deposition activity. This way, the FRMAC Gamma Spectroscopist can practice their process of generating quantified results from spectra on realistic data as well. Recognizing the decades of work done in GADRAS to accurately generate synthetic spectra, this team decided to build a link between the new simulator and GADRAS to generate these spectra quickly and easily. The simulator tool will generate a file that specifies the name of the spectra, its location, date/time of measurement, duration of measurement, height off the ground, and the deposition activity and age for every radionuclide in the simulation. Then, a new tool within the Inject Tab of GADRAS was developed to read in this file given a detector selection and generate In-Situ spectra for each row in the file in any file format the user chooses. This way, simulation cell staff can take these files and then upload them to the appropriate data system (RAMS or RadResponder) for use during drills and exercises. An advanced feature of this tool allows for generating any spectra given an appropriate model and mapping of source to model layer in the batch inject tool. This way, spectra from field sample counts, mobile laboratories, or even fixed laboratories can be generated in bulk given an estimate of the radioactivity concentration or total radioactivity in an import file. This expands the capabilities of this tool a great deal and will make it a more useful tool for CM and others to help estimate detector response for nearly any situation. This user guide will explain the steps needed to perform a batch inject file generation.

61 RADIATION PROTECTION AND DOSIMETRY↗

High Energy Physics Network Requirements Review (Final Report, July-October 2020)

Throughout 2020, ESnet and the Office of High Energy Physics (HEP) of the DOE SC organized an ESnet requirements review of HEP-supported activities. Preparation for this event included identification of key stakeholders: program and facility management, research groups, technology providers, and a number of external observers. These individuals were asked to prepare formal case study documents about their relationship to the HEP program to build a complete understanding of the current, near-term, and long-term status, expectations, and processes that will support the science going forward. A series of pre-planning meetings better prepared case study authors for this task, along with guidance on how the review would proceed in a virtual fashion.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Search for Q ~0 Order near a Forbidden Bragg Position in Bi 2.1 Sr 1.9 CaCu 2 O 8+x with Resonant Soft X-ray Scattering

Identifying what broken symmetries are present in the cuprates has become a major area of research. Many authors have reported evidence for so-called “Q ~ 0” order that involves broken inversion, mirror, chiral, or time-reversal symmetry that is uniform in space. Not all these observations are well understood and new experimental probes are needed. Here we use resonant soft x-ray scattering (RSXS) to search for Q ~ 0 order in Bi 2.1 Sr 1.9 CaCu 2 O 8+x (Bi-2212) by measuring the region of a forbidden Bragg peak, (0,0,3), which is normally extinguished by symmetry but may become allowed on resonance if valence band order is present. Using circularly polarized light, we found that this reflection becomes allowed on the CuL 3 resonance for temperatures T c < T < T*, though remains absent in linear polarization and at other temperatures. This observation suggests the existence of spatially uniform valence band order near the pseudogap temperature. In addition, we observed periodic oscillations in the specular reflectivity from the sample surface that resemble thin film interference fringes, though no known film is present. These fringes are highly resonant, appear in all polarizations, and exhibit a period that depends on the location where the beam strikes the sample surface. We speculate that these fringes arise from interaction between some intrinsic valence band instability and extrinsic structural surface morphologies of the material. Our study supports the existence of some kind of Q ~ 0 broken symmetry state in Bi-2212 at intermediate temperatures. Further studies using a microfocused beam, which could disentangle microscopic effects from macroscopic heterogeneities, are needed to ascertain the universality of the effect.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

A Novel Technique for Distributed Measuring of Strain in the Vadose Zone

Characterizing water content and pressure changes in the vadose zone is important to understanding a variety of geologic processes, ranging from permeability, to evapotranspiration, and aquifer recharge. Changes in water content, or pressure, cause strain in the solid porous medium of the vadose zone, and it is possible that measuring those strains could be used a characterization tool. The Coherence-length-gated Microwave Photonics Interferometry (CMPI) technique measures strain at high resolution along many intervals defined by pairs of reflectors distributed along an optical fiber. This technique has recently been developed at Clemson University, and it has the spatial, and temporal resolution to characterize the strains that are expected to occur with hydrologic changes in the vadose zone. However, the technique has never been used to measure strain in porous media, so its capabilities remain uncertain. The objective of this thesis is to evaluate the ability of using CMPI to measure strain changes in the vadose zone. The research approach consists of conducting laboratory tests using a column filled with sand that was subjected to changes in water content and pressure. An optical fiber with CMPI reflectors was deployed in a high surface area ribbon and used to measure strain along the axis of the column. The column was made from 8-inch, Schedule 40 PVC pipe (75 cm tall, 20 cm inner diameter) and filled with medium-grained sand (K = 2.5x10-6 m/s, porosity = 0.28, Coefficient of Uniformity = 2, van Genuchten (n = 4.34 and  = 0.00039 m-1), Young’s Modulus = 18 – 47 MPa). Five pressure and four temperature sensors attached to probes inserted into the wall. The optical fiber includes five reflectors spaced 10 cm apart on the inside and outside of the column along the vertical axis. Strain measurements are made between pairs of reflectors. The reflectors are created in 250-micron-diameter acrylate-coated single mode Corning SMF28e+ optical fiber using a femtosecond laser. The optical fiber was laminated between two pieces of polyester film creating a large surface area to transfer strain from the porous media to the optical fiber. The experiments were conducted by filling the column from the bottom or infiltrating water from the top. The water was allowed to equilibrate to room temperature prior to each test in order to limit thermoelastic strain. Five injection tests with a rate of 250 ml/min and three infiltration tests at varying rates were conducted, and the results show patterns of strain and pressure are generally similar. Hydrologic conditions define three zones based on the pressure magnitude and distribution. 1.) Ambient Zone where the pressure heads are quasi-static and the pressure gradient is roughly unity (head gradient of zero). This is the uppermost zone and is characterized by negative pressures. 2.) Transition Zone where the pressures increase from ambient to zero, are changing relatively rapidly and the pressure gradient is relatively steep (pressure head gradients of 2). The Transition zone is 10 to 15 cm thick. 3.) Positive Pressure Zone where the pressure is positive, the rate of change is slower than in the transition zone and the gradient is flatter (pressure head gradient 1.1 to 1.2). This is the lowest zone in the column. Injection of water causes the pressure to increase and the three zones to move upward. The Transition zone moves at a rate of approximately 0.0002 m/s +/- .00005, according to analyses of pressure profiles. This is the same as the average velocity of the water calculated as volumetric flux/effective porosity =5.4x10-5 m/s/0.28. Strain signals in the range of 10s  were observed with a noise level of generally less than 0.1  (signal to noise ratio of greater than 100) during injection and drainage. The spatial and temporal distributions of strain caused by injection depend on the location of the moving pressure zones. The locations of the different pressure zones were determined from pressure profiles at different times and these data were transferred to strain time series. This showed that strain in the Ambient pressure zone is either unchanged or slightly compressive, whereas strain in Transition zone is tensile and roughly proportional to the pressure change, and strain ranges from tensile to compressive in the Positive Pressure zone. In general, the strain is variable at the top of the Positive Pressure zone, but it appears to be consistently tensile lower in the zone. The spatial distribution of strain causes three distinct stages in the strain times series measured between pairs of CMPI reflectors. The strain is unchanged or slightly compressive during Stage 1, it increases (positive strain is tensile) approximately linearly at a rate of 0.02 to 0.03 μ/s during the Stage 2, and then flattens out in Stage 3. The strain increases again during Stage 4 of the time series. The pressure also changes in stages. It is unchanged during Stage 1 and then increases relatively rapidly at a rate of between 4 and 10 Pa/s during Stage 2 and continues to increase during Stages 3 and 4, but at a rate slightly slower than during Stage 2 (from 2.5 to 3.5 Pa/s). The rates of pressure and strain change are consistent with basic analyses. The rate of pressurization is similar to the calculated velocity of flow in the saturated zone, and this is similar to the measured velocity of the strain increase. The ratio of the pressurization rate and strain rate during Stage 2 (2.5 (Pa/s) /0.03 (μ/s)) is 80 MPa, which is approximately equal to the upper range expected considering the uniaxial compression and the Young’s Modulus of the sand. An interesting effect occurs when the upper surface of the sand becomes saturated. Significant compression (several 10s of ) occurs as the pressure and saturation increase at the upper surface. Compression occurs throughout the column, but the effect is greatest at the top of the column. The rate of compression is fastest slightly before ponding occurs, but it slows markedly and nearly stops when water starts to accumulate at the surface (ponding). This effect reverses when the surface of the sand is drained, resulting in tension throughout the column. The compression caused by this effect can be as large or larger than the tensile strain that accumulated during filling. This effect was unexpected because increasing pressure is normally associated with tensile strain. Nevertheless, this effect was observed consistently in all tests where the pressure changes at the upper surface, including tests where water was injected from below or infiltrated from above. This effect behaves as if the pore pressure at the upper surface of the sand exerts a normal force on the boundary (increasing pore pressure exerts a downward compression on the boundary). The results of these laboratory experiments indicate that CMPI can measure strain caused by fluid pressure changes in the vadose zone with a signal to noise ratio of 100 or more. Injection and drainage cause a strain signal that is complex, but repeatable. The magnitudes of the strain signal are consistent with magnitudes that are expected based on poroelastic calculations using independently measured properties of the sand. These results indicate that the CMPI technique with an optical fiber laminated in a polyester ribbon generates data that represent the strain distribution during hydrologic processes of imbibition and drainage in variably saturated sand. This suggests that distributed strain measurements using CMPI could be a viable approach for evaluating processes in the vadose zone, laying the groundwork for future field implementation.

47 OTHER INSTRUMENTATION↗

Experimental and Computational Analysis of NEAMS Pebble Bed Reactors

The Advanced High-Temperature Pebble Bed Reactor concept leverages a particle-based fuel format consisting of discrete spherical graphite pebbles arrayed in a packed bed architecture. Thermal regulation achieved via flow of gas (e.g., helium) or liquid (e.g., molten salt) coolants through the void spaces between pebbles in the bed (characteristic pebble diameters: ~ 6 cm, gas cooled; ~ 3 cm, liquid cooled). This design is of interest owing to inherent advantages including passive safety features and highly efficient heat transfer characteristics that enable high power densities to be achieved. Fully leveraging these advantages requires a fundamental understanding of the complex coolant flow structure within the pebble-shaped fuel bed. Unfortunately, complexities associated with non-invasively probing the micro-scale flow phenomena within the complex network of void spaces between pebbles have hindered efforts to characterize the underlying transport phenomena. Without this fundamental foundation, it becomes challenging to rationally construct macroscopic transport models based upon volume averages of micro-scale parameters that accurately capture the observed flow behavior. Consequently, this lack of fundamental knowledge has limited previous work to coarse comparisons between theory and extremely limited experimental data. Moreover, these comparisons have been made only in terms of integral or macroscopic results. Therefore, multipoint measurements with a high level of spatial and temporal resolution are critically needed to fully map the complex flow patterns and to provide data at high spatial density to permit accurate volume averaging in the pebble bed. For this project, we performed a coordinated experimental and computational effort to quantitatively map the full-field velocity and temperature fields in the interstitial spaces within the pebble bed. The major accomplishments of this project included the important knowledge acquired for the flow mixing and heat transfer in the interstitial pore scales, the effects of flow mixing in the near-wall and far-wall regions, and the by-pass flows of pebble bed systems. The produced high-resolution experimental data (not broadly available in existing literature) were then used for the numerical studies enabling the refinement and validation of standard simulation tools (Nek5000).

42 ENGINEERING↗

The Milky Way, coming into focus: Precision astrometry probes its evolution and its dark matter

The growing trove of precision astrometric observations from the Gaia space telescope and other surveys is revealing the structure and dynamics of the Milky Way in ever more exquisite detail. We summarize the current status of our understanding of the structure and the characteristics of the Milky Way, and we review the emerging picture: the Milky Way is evolving through interactions with the massive satellite galaxies that stud its volume, with evidence pointing to a cataclysmic past. It is also woven with stellar streams, and observations of streams, satellites, and field stars offer new constraints on its dark matter, both on its spatial distribution and its fundamental nature. The recent years have brought much focus to the study of dwarf galaxies found within our Galaxy’s halo and their internal matter distributions. In this review, we focus on the predictions of the cold dark matter paradigm at small mass scales through precision astrometric measurements, and we summarize the modern consensus on the extent to which small-scale probes are consistent with this paradigm. We note the discovery prospects of these studies, and also how they intertwine with probes of the dynamics and evolution of the Milky Way in various and distinct ways.

79 ASTRONOMY AND ASTROPHYSICS↗

Searching for Strongly-Interacting Dark Matter with the Heavy Photon Search Experiment

The Heavy Photon Search Experiment (HPS) is a fixed-target experiment at Jefferson Lab’s Hall B, designed to explore a hidden sector (HS) of particles containing dark matter and a new force mediator known as the “heavy photon” (A'). The A' is a massive spin-1 gauge boson associated with a new U (1)D symmetry in the HS that kinetically mixes with the Standard Model () photon with a weak coupling strength parameterized by ¿, with ¿2 ~ 10-2 -10-10. HPS utilizes a high-intensity electron beam on a thin tungsten target to produce heavy photons in the MeV-GeV mass range via “dark bremsstrahlung,” a process analogous to SM bremsstrahlung but suppressed by ¿2. The A' can decay resonantly to SM leptons, allowing HPS to conduct both mass resonance searches for prompt decays (large ¿) and displaced vertex searches for long-lived particles (small ¿). In addition to the minimal A' model, HPS probes more complex extensions such as the QCD-like strongly-interacting massive particles (SIMPs) HS containing “dark” pions (pD) and vector mesons (VD), with pD as dark matter candidates. These particles introduce new thermal dark matter freeze- out scenarios and visible signals through long-lived VD decays to SM leptons, which are accessible to HPS. This analysis conducted a displaced vertex search for VD ¿ e-e+ in the mass range 30 MeV to 124 MeV and ¿ between 10-6 < ¿ < 10-2 using data from the 2016 Engineering Run (10.753 nb-1) at 2.3 GeV. Unlike the minimal A' search, SIMP signal kinematics required new approaches to signal normalization and SM background rejection. The strongest signal evidence was a local p-value of 0.01317 for mVD = 119 MeV, corresponding to a global significance of 0.9s. Although no signal was found, this search excluded a region of the SIMP parameter space at 90 % confidence. This work demonstrates HPS’s competitive capability to probe SIMP sectors within cosmologically significant parameters and introduces a new method for HPS displaced vertex searches using track vertical impact parameter cuts

Spellman, Alic [Univ. of California, Santa Cruz, C↗

Effective bias expansion for 21-cm cosmology in redshift space

A near-future detection of the 21-cm signal from the epoch of reionization will provide unique opportunities to probe the underlying cosmology, provided that such cosmological information can be extracted with precision. To this end, we further develop effective field theory (EFT) inspired techniques for the 21-cm brightness temperature field during the epoch of reionization, incorporating renormalized bias and a treatment of redshift space distortions. Notably, we confirm that in redshift space, measures of the 21-cm brightness, e.g., the power spectrum, should have irreducible contributions that lack a bias coefficient and therefore contain direct, astrophysics-free information about the cosmological density field; in this work, we study this effect beyond linear order. To validate our theoretical treatment, we fit the predicted EFT Fourier-space shapes to the thesan suite of hydrodynamical simulations of reionization at the field level, where the considerable number of modes prevents overfitting. We find agreement at the level of a few percent between the 21-cm power spectrum from the EFT fits and simulations over the wave number range k ≲ 0.8 h/Mpc and neutral fraction x HI ≳ 0.4, which is imminently measurable by the Hydrogen Epoch of Reionization Array and future experiments. Furthermore, the ability of the EFT to describe the 21-cm signal extends to simulations that have different astrophysical prescriptions for reionization as well as simulations with interacting dark matter.

79 ASTRONOMY AND ASTROPHYSICS↗

Chromatic effects on the PSF and shear measurement for the Roman Space Telescope High-Latitude Wide Area Survey

Weak gravitational lensing (WL) is a key cosmological probe that requires precise measurement of galaxy images to infer shape distortions, or shear, and constrain cosmology. Accurate estimation of the point spread function (PSF) is crucial for shear measurement, but the wavelength dependence of the PSF introduces chromatic biases that can systematically impact shear inference. We focus on biases arising from spectral energy distribution (SED) differences between stars, used for PSF modelling, and galaxies, used for shear measurement. We investigate these effects in Roman’s four design reference mission WL bands (Y106, J129, H158, F184) and wide filter (W146). Using Roman-like image simulations, we quantify the induced shear biases and compare them to requirements on those biases. Multiplicative biases over all galaxies hover around ~0.2 per cent in the WL bands and 2 per cent in the wide filter, exceeding the mission requirement of |m| < 0.032 per cent and relaxed requirement of |m| < 0.1 per cent⁠. In individual redshift bins, biases can reach 0.4–0.9 per cent for the WL bands and 3–6 per cent for the wide filter. Additive biases remain acceptable in the WL bands but exceed systematic limits in the wide filter. We develop and test PSF-level corrections, showing that a first-order correction reduces biases within survey requirements for the WL bands; however, higher-order terms are necessary for the wide filter. Our results highlight the necessity of chromatic corrections for precision WL with Roman and provide a framework for mitigating these biases. Finally, we compare analytical colour-based corrections to self-organizing maps and find that both methods effectively reduce biases.

79 ASTRONOMY AND ASTROPHYSICS↗

The solenoidal large intensity device (SoLID) for JLab 12 GeV

The solenoidal large intensity device (SoLID) is a new experimental apparatus planned for Hall A at the Thomas Jefferson National Accelerator Facility (JLab). SoLID will combine large angular and momentum acceptance with the capability to handle very high data rates at high luminosity. With a slate of approved high-impact physics experiments, SoLID will push JLab to a new limit at the QCD intensity frontier that will exploit the full potential of its 12 GeV electron beam. In this paper, we present an overview of the rich physics program that can be realized with SoLID, which encompasses the tomography of the nucleon in 3D momentum space from semi-inclusive deep inelastic scattering, expanding the phase space in the search for new physics and novel hadronic effects in parity-violating DIS, a precision measurement of J/ψ production at threshold that probes the gluon field and its contribution to the proton mass, tomography of the nucleon in combined coordinate and momentum space with deep exclusive reactions, and more. To meet the challenging requirements, the design of SoLID described here takes full advantage of recent progress in detector, data acquisition and computing technologies. In addition, we outline potential experiments beyond the currently approved program and discuss the physics that could be explored should upgrades of CEBAF become a reality in the future.

3D imaging↗

Variability and origins of grain boundary electric potential detected by electron holography and atom-probe tomography

A number of grain boundary phenomena in ionic materials, in particular, anomalous (either depressed or enhanced) charge transport, have been attributed to space charge effects. Developing effective strategies to manipulate transport behaviour requires deep knowledge of the origins of the interfacial charge, as well as its variability within a polycrystalline sample with millions of unique grain boundaries. Electron holography is a powerful technique uniquely suited for studying the electric potential profile at individual grain boundaries, whereas atom-probe tomography provides access to the chemical identify of essentially every atom at individual grain boundaries. Using these two techniques, we show in this paper that the space charge potential at grain boundaries in lightly doped, high-purity ceria can vary by almost an order of magnitude. We further find that trace impurities (<25 ppm), rather than inherent thermodynamic factors, may be the ultimate source of grain boundary charge. These insights suggest chemical tunability of grain boundary transport properties. A number of grain boundary phenomena in ionic materials, such as anomalous charge transport, have been attributed to space charge effects. Space charge potential at grain boundaries in lightly doped, high-purity ceria is now shown to vary by almost an order of magnitude.

36 MATERIALS SCIENCE↗

Constraints on Metastable Helium in the Atmospheres of WASP-69b and WASP-52b with Ultranarrowband Photometry

Infrared observations of metastable 2{sup 3}S helium absorption with ground- and space-based spectroscopy are rapidly maturing, as this species is a unique probe of exoplanet atmospheres. Specifically, the transit depth in the triplet feature (with vacuum wavelengths near 1083.3 nm) can be used to constrain the temperature and mass-loss rate of an exoplanet’s upper atmosphere. Here, we present a new photometric technique to measure metastable 2{sup 3}S helium absorption using an ultranarrowband filter (FWHM 0.635 nm) coupled to a beam-shaping diffuser installed in the Wide-field Infrared Camera on the 200 inch Hale Telescope at Palomar Observatory. We use telluric OH lines and a helium arc lamp to characterize refractive effects through the filter and to confirm our understanding of the filter transmission profile. We benchmark our new technique by observing a transit of WASP-69b and detect an excess absorption of 0.498% ± 0.045% (11.1σ), consistent with previous measurements after considering our bandpass. We then use this method to study the inflated gas giant WASP-52b and place a 95th percentile upper limit on excess absorption in our helium bandpass of 0.47%. Using an atmospheric escape model, we constrain the mass-loss rate for WASP-69b to be 5.25{sub −0.46}{sup +0.65}×10{sup −4} M{sub J} Gyr{sup −1} (3.32{sub −0.56}{sup +0.67}×10{sup −3} M{sub J} Gyr{sup −1}) at 7000 K (12,000 K). Additionally, we set an upper limit on the mass-loss rate of WASP-52b at these temperatures of 2.1×10{sup −4} M{sub J} Gyr{sup −1} (2.1×10{sup −3} M{sub J} Gyr{sup −1}). These results show that ultranarrowband photometry can reliably quantify absorption in the metastable helium feature.

79 ASTRONOMY AND ASTROPHYSICS↗

A high-temperature sample changer for parallelized in situ X-ray studies to efficiently explore reaction space

A sample environment for high-throughput X-ray scattering studies in transmission geometry to probe the mechanism and kinetics of moderate-temperature reactions in solution, molten fluxes and solids is described. This high-temperature sample changer enables efficient studies of reactions that are slow relative to the timescale of the X-ray scattering measurements by allowing up to 18 samples to be probed at the same temperature in parallel. This significantly enhances the throughput ofin situX-ray scattering studies as the sample changer effectively facilitates systematic studies that compare different reaction parameters (e.g.concentration, precursor, composition, additives), reference samples (e.g.background, pure precursors) and replicates (to demonstrate reproducibility) with enhanced consistency afforded by the quasi-simultaneous nature of the measurements. The large sample volumes, compared with those typically used for X-ray scattering measurements, are on a similar scale to those in the laboratory, making the results more directly comparable.

Chemistry↗

GENESIS: Gamma Energy Neutron Energy Spectrometer for Inelastic Scattering

Improved neutron inelastic scattering cross section data are needed to inform integral benchmark studies and advance applications in a wide variety of areas including nuclear energy, stockpile stewardship, nonproliferation, and space exploration. Neutron inelastic scattering also serves as a non-selective probe of low-lying nuclear structure. To help meet these needs, the Gamma Energy Neutron Energy Spectrometer for Inelastic Scattering (GENESIS) was constructed at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. This array couples high-resolution γ-ray detectors and fast neutron detectors to achieve single and coincident n/γ detection over a broad energy range. The current configuration of the array includes 26 organic liquid scintillators and four high-purity germanium detectors (two single-crystal and two four-crystal CLOVER detectors with two-fold segmentation). The array was constructed with minimal supporting material and designed to cover a wide range of secondary particle angles and energies with limited inter-element scattering. Data acquisition is accomplished using Mesytec MDPP-16 multi-channel high-resolution digital pulse processing modules. The array characteristics, including γ-ray and neutron energy resolution, timing resolution, and detection efficiency were measured and used to validate a Geant4 model of the array. Furthermore, the primary sources of neutron background and the uncertainties in the determination of incident and secondary neutron energy were assessed. GENESIS provides a new capability to address nuclear data needs and facilitates the advancement of a wide range of nuclear applications.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Flux and estimated spectra from a low-intensity laser-driven X-ray source

Laser-driven X-rays as probes for high-energy-density physics spans an extremely large parameter space with laser intensities varying by 8 orders of magnitude. We have built and characterized a soft X-ray source driven by a modest intensity laser of 4 × 10 13 W/cm 2 . Emitted X-rays were measured by diamond radiation detectors and a filtered soft X-ray camera. A material-dependence study on Al, Ti, stainless steel alloy 304, Fe, Cu and Sn targets indicated 5-μm-thick Cu foils produced the highest X-ray yield. X-ray emission in the laser direction and emission in the reverse direction depend strongly on the foil material and the thickness due to the opacity and hydrodynamic disassembly time. The time-varying X-ray signals are used to measure the material thinning rate and is found to be ~1.5 μm/ns for the materials tested implying thermal temperature around 0.6 eV. The X-ray spectra from Cu targets peaks at ~2 keV with no emission >4 keV and was estimated using images with eight different foil filters. One-dimensional hydrodynamic and spectral calculations using HELIOS-CR provide qualitative agreement with experimental results. Modest intensity lasers can be an excellent source for nanosecond bursts of soft X-rays.

47 OTHER INSTRUMENTATION↗