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At least 289 records · Page 16
All sourcesNASA NTRSDOE OSTI
NASA NTRS1990

Extraterrestrial halogen and sulfur contents of the stratosphere

Interplanetary dust represents a potential source of environmentally important chemical species in the earth's atmosphere. Previous studies have used computational models of atmospheric evolution of meteor debris to conclude that the steady-state stratospheric component of extraterrestrial matter is a small fraction of the total aerosol load. Observational data suggest such calculations may underestimate stratospheric residence times and, thus, concentrations. Two computational methods were employed here to obtain reasonable limits for the stratospheric contents of halogens and sulfur from extraterrestrial sources. The lower limit was based on the total stratospheric aerosol load and the relative influxes from interplanetary dust and tropospheric sources. The upper limit was obtained using a viscous settling method. These results suggest that the steady-state extraterrestrial influxes of halogens are minor compared to tropospheric sources but the sulfur input may be comparable to the present observed stratospheric content. Temporal enhancements in the meteoroid flux, such as passage through comet debris lanes or impact by large bodies, may produce significant chemical perturbations in the atmosphere.

Sutton, S. R.↗
NASA NTRS1991

Two-dimensional model calculation of fluorine-containing reservoir species in the stratosphere

Two-dimensional model calculations have been carried out of the distributions of the fluorine-containing reservoir species HF, CF2O, and CFClO. HF constitutes the largest fluorine reservoir in the stratosphere, but CF2O also makes an important contribution to the inorganic fluorine budget. CFClO amounts are most important in the tropical lower stratosphere. HF amounts increase with altitude throughout the stratosphere, while those of CF2O and CFClO fall off above their mixing ratio peaks due to photolysis. The model is in good qualitative agreement with observed vertical profiles of HF and CF2O but tends to underestimate the total column of HF. The calculated CFClO distribution is in good agreement with the very limited data. The disagreement in the HF columns is likely due to small inaccuracies in the model's treatment of lower stratospheric photolysis of chlorofluorocarbons. The model results support the suggestion that CF2O may be heterogeneously converted to HF on the surface of polar stratospheric cloud particles. The model results also suggest that the quantum yield for photolysis of CF2O is near unity.

Kaye, Jack A.↗
NASA NTRS1991

Homogeneous freezing nucleation of stratospheric solution droplets

The classical theory of homogeneous nucleation was used to calculate the freezing rate of sulfuric acid solution aerosols under stratospheric conditions. The freezing of stratospheric aerosols would be important for the nucleation of nitric acid trihydrate particles in the Arctic and Antarctic stratospheres. In addition, the rate of heterogeneous chemical reactions on stratospheric aerosols may be very sensitive to their state. The calculations indicate that homogeneous freezing nucleation of pure water ice in the stratospheric solution droplets would occur at temperatures below about 192 K. However, the physical properties of H2SO4 solution at such low temperatures are not well known, and it is possible that sulfuric acid aerosols will freeze out at temperatures ranging from about 180 to 195 K. It is also shown that the temperature at which the aerosols freeze is nearly independent of their size.

Jensen, Eric J.↗
NASA NTRS1990

Millimeter-wave ozone measurements for the network for the detection of stratospheric change

The primary research objective is to initiate long-term monitoring of stratospheric ozone with a ground-based millimeter-wave spectrometer, the first of several such instruments projected to be part of the Network for the Detection of Stratospheric Change. The ultimate goal of this monitoring is twofold. First, to detect any secular trend in stratospheric ozone abundance, whether of natural or anthropogenic origin and, second, to provide ground-truth validation for existing and future satellite measurements of ozone. With this goal in mind, a more immediate objective is to validate the millimeter-wave measurements by tests of the instrument, internal consistency tests on the data, and most importantly, by intercomparison with all other available ozone measurements. The validation process is expected to lead to refinements in the instrument and its operating procedures and in the data analysis. The final objective is to perform short-term scientific studies with the data, including studies of the ozone diurnal and seasonal variations, and comparison of ozone variations with changes in other geophysical parameters, notably temperature and water vapor. Routine observations are now ongoing; these will allow continuing intercomparisons with the Stratospheric Aerosol and Gas Experiment (SAGE II) and one of the lidars, which is permanently on site. The experience gained during the Stratospheric Ozone Intercomparison (STOIC) caused us to refine our calibration procedures and identify the need for internal shielding of the millimeter receiver from radio frequency interference. Installation of this shielding is planned for the near future and should allow improvements in the instrument calibration and a higher signal-to-noise ratio, both of which will result in improved measurement precision.

Connor, Brian J.↗
NASA NTRS1990

Aircraft deployment, and airborne arctic stratospheric expedition

The Airborne Arctic Stratospheric Expedition had two primary objectives: to study the production and loss mechanisms of ozone in the north polar stratosphere and to study the effect on ozone distribution of the Arctic Polar Vortex and of the cold temperatures associated with the formation of Polar Stratospheric Clouds. Two specially instrumented NASA aircraft were flown over the Arctic region. Each aircraft flew to acquire data on the meteorological, chemical and cloud physical phenomena that occur in the polar stratosphere during winter. The chemical processes which occur in the polar stratosphere during winter were also observed and studied. The data acquired are being analyzed.

Condon, Estelle↗
NASA NTRS1990

Airborne lidar stratospheric ozone and aerosol investigations

The objectives are to study the distribution of ozone (O3) and aerosols across the polar regions during the winter and spring periods and to relate these observations to chemical and dynamical processes that can contribute to the chemical perturbation of the polar stratosphere and the possible destruction of O3. The distribution and characteristics of stratospheric aerosols and polar stratospheric clouds (PSCs) are required to understand heterogeneous chemical processes that can lead to O3 depletion, and observation of O3 variations are important in the direct detection of O3 depletion and in tracing atmospheric dynamics. An airborne Differential Absorption Lidar (DIAL) system is operated in a zenith mode from the NASA DC-8 aircraft to obtain data on the large scale spatial variability of O3, and aerosol/PSC's in the lower stratosphere from about 11 to 23 km for O3, and 11 to 28 km for aerosols. The variability of O3 and aerosols/PSCs is studied in relation to chemical processes that can produce O3 depletion and to dynamics in the lower stratosphere that transport gases and aerosols inside the vortex and in some cases, across the edge of the vortex.

Browell, Edward V.↗
NASA NTRS1990

Stratospheric dynamics

A global circulation model is being used to study the dynamical behavior of stratospheric planetary waves (waves having horizontal wavelengths of tens of thousands of kilometers) forced by growing cyclonic disturbances of intermediate scale, typically with wavelengths of a few thousand kilometers, which occur in the troposphere. Planetary scale waves are the dominant waves in the stratosphere, and are important for understanding the distribution of atmospheric trace constituents. Planetary wave forcing by intermediate scale tropospheric cyclonic disturbances is important for producing eastward travelling planetary waves of the sort which are prominent in the Southern Hemisphere during winter. The same global circulation model is also being used to simulate and understand the rate of dispersion and possible stratospheric climatic feedbacks of the El Chichon volcanic aerosol cloud. By comparing the results of the model calculation with an established data set now in existence for the volcanic cloud spatial and temporal distribution, stratospheric transport processes will be better understood, and the extent to which the cloud modified stratospheric wind and temperature fields can be assessed.

Young, Richard E.↗
NASA NTRS1989

Trends in stratospheric temperature

Stratospheric temperatures for long-term and recent trends and the determination of whether observed changes in upper stratospheric temperatures are consistent with observed ozone changes are discussed. The long-term temperature trends were determined up to 30mb from radiosonde analysis (since 1970) and rocketsondes (since 1969 and 1973) up to the lower mesosphere, principally in the Northern Hemisphere. The more recent trends (since 1979) incorporate satellite observations. The mechanisms that can produce recent temperature trends in the stratosphere are discussed. The following general effects are discussed: changes in ozone, changes in other radiatively active trace gases, changes in aerosols, changes in solar flux, and dynamical changes. Computations were made to estimate the temperature changes associated with the upper stratospheric ozone changes reported by the Solar Backscatter Ultraviolet (SBUV) instrument aboard Nimbus-7 and the Stratospheric Aerosol and Gas Experiment (SAGE) instruments.

Schoeberl, M. R.↗
NASA NTRS1992

Aerosols and polar stratospheric clouds measurements during the EASOE campaign

Preliminary results of observations performed using two different lidar systems during the EASOE (European Arctic Stratospheric Ozone Experiment), which has taken place in the winter of 1991-1992 in the northern hemisphere lattitude regions, are presented. The first system is a ground based multiwavelength lidar intended to perform measurements of the ozone vertical distribution in the 5 km to 40 km altitude range. It was located in Sodankyla (67 degrees N, 27 degrees E) as part of the ELSA experiment. The objectives of the ELSA cooperative project is to study the relation between polar stratospheric cloud events and ozone depletion with high vertical resolution and temporal continuity, and the evolution of the ozone distribution in relation to the position of the polar vortex. The second system is an airborne backscatter lidar (Leandre) which allows for the study of the 3-D structure and the optical properties of polar stratospheric clouds. The Leandre instrument is a dual-polarization lidar system, emitting at 532 nm, which allows for the determination of the type of clouds observed, according to the usual classification of polar stratospheric clouds. More than 60 hours of flight were performed in Dec. 1991, and Jan. and Feb. 1992 in Kiruna, Sweden. The operation of the Leandre instrument has led to the observation of the short scale variability of the Pinatubo volcanic cloud in the high latitude regions and to several episodes of polar stratospheric clouds. Preliminary analysis of the data is presented.

Haner, D.↗
NASA NTRS1991

Polar stratospheric clouds and the ozone hole

An account is given of physical processes governing the formation of stratospheric particles, in order to dramatize the interactions between polar stratospheric clouds and the Antarctic ozone-destruction mechanism. Attention is given to the successive stages of particle nucleation, condensation/evaporation and sedimentation/coagulation phenomena, and the ways in which polar stratospheric clouds are observed. Considerable evidence exists that polar stratospheric cloud particles are composed of nitric acid. The relatively small Arctic ozone hole depletion is due to the much smaller duration of Arctic stratospheric clouds.

Hamill, Patrick↗
NASA NTRS1992

Planetary-scale disturbances in the southern stratosphere during early winter

The stratospheric circulation and planetary-scale dusturbances during early-winter (mid-April to mid-July) in the Southern Hemisphere are investigated using observational data collected for the 1979-1990 period, and a 3D primitive equation model of the stratosphere and mesosphere. It was found that there were six extended periods in the data set when wave 1 (which is usually quasi-stationary) traveled steadily eastward and had large amplitude. Results of simulations suggest that the development of the South Pacific warmings is connected with the amplification of wave 1 at 100 mb. The results also indicate that the development of stratospheric disturbances in the southern stratosphere during early winter depends more on the intensity of wave 1 at 100 mb than on the structure of the zonal-mean flow in the stratosphere.

Farrara, John D.↗
NASA NTRS1992

Statistical analysis of stratospheric temperature and ozone profile data for trends and model comparison

Work performed during the project period July 1, 1990 to June 30, 1992 on the statistical analysis of stratospheric temperature data, rawinsonde temperature data, and ozone profile data for the detection of trends is described. Our principal topics of research are trend analysis of NOAA stratospheric temperature data over the period 1978-1989; trend analysis of rawinsonde temperature data for the period 1964-1988; trend analysis of Umkehr ozone profile data for the period 1977-1991; and comparison of observed ozone and temperature trends in the lower stratosphere. Analysis of NOAA stratospheric temperature data indicates the existence of large negative trends at 0.4 mb level, with magnitudes increasing with latitudes away from the equator. Trend analysis of rawinsonde temperature data over 184 stations shows significant positive trends about 0.2 C per decade at surface to 500 mb range, decreasing to negative trends about -0.3 C at 100 to 50 mb range, and increasing slightly at 30 mb level. There is little evidence of seasonal variation in trends. Analysis of Umkehr ozone data for 12 northern hemispheric stations shows significant negative trends about -.5 percent per year in Umkehr layers 7-9 and layer 3, but somewhat less negative trends in layers 4-6. There is no pronounced seasonal variation in trends, especially in layers 4-9. A comparison was made of empirical temperature trends from rawinsonde data in the lower stratosphere with temperature changes determined from a one-dimensional radiative transfer calculation that prescribed a given ozone change over the altitude region, surface to 50 km, obtained from trend analysis of ozonsonde and Umkehr profile data. The empirical and calculated temperature trends are found in substantive agreement in profile shape and magnitude.

Tiao, G. C.↗
NASA NTRS1993

The atmospheric effects of stratospheric aircraft

This document presents a second report from the Atmospheric Effects of Stratospheric Aircraft (AESA) component of NASA's High-Speed Research Program (HSRP). This document presents a second report from the Atmospheric Effects of Stratospheric Aircraft (AESA) component of NASA's High Speed Research Program (HSRP). Market and technology considerations continue to provide an impetus for high-speed civil transport research. A recent United Nations Environment Program scientific assessment has shown that considerable uncertainty still exists about the possible impact of aircraft on the atmosphere. The AESA was designed to develop the body of scientific knowledge necessary for the evaluation of the impact of stratospheric aircraft on the atmosphere. The first Program report presented the basic objectives and plans for AESA. This second report presents the status of the ongoing research as reported by the principal investigators at the second annual AESA Program meeting in May 1992: Laboratory studies are probing the mechanism responsible for many of the heterogeneous reactions that occur on stratospheric particles. Understanding how the atmosphere redistributes aircraft exhaust is critical to our knowing where the perturbed air will go and for how long it will remain in the stratosphere. The assessment of fleet effects is dependent on the ability to develop scenarios which correctly simulate fleet operations.

Stolarski, Richard S.↗
NASA NTRS1992

Buffering of stratospheric circulation by changing amounts of tropical ozone - A Pinatubo case study

Stratospheric aerosol from Mount Pinatubo heated the tropical lower stratosphere by about 0.3 K/day mainly due to absorption of terrestrial infrared radiation. This heating was dissipated by: (1) an observed increase in stratospheric temperatures, which enhanced the radiation cooling; (2) additional mean upward motion, observed for the aerosol cloud, which led to adiabatic cooling; and (3) reductions in ozone concentrations resulting from enhanced upward motions. Each of these processes operated on a different time scale: maximum temperatures were observed after about 90 days; maximum ozone losses of about -1.5 ppm occurred after 140 days when the enhanced vertical velocities effectively lifted the ozone profile by about 2 km. We believe this shows that ozone plays an important role in buffering vertical motion in the tropical lower stratosphere, and hence the residual Brewer Dobson circulation of the whole stratosphere.

Kinne, S.↗
NASA NTRS1992

Modeling the quasi-biennial oscillation's effect on the winter stratospheric circulation

The influence of the equatorial quasi-biennial oscillation (QBO) on the winter middle atmosphere is modeled with a mechanistic global primitive equation model. The model's polar vortex evolution is sensitive to the lower stratosphere's tropical winds, with the polar vortex becoming more (less) disturbed as the lower stratospheric winds are more easterly (westerly). This agrees with the observed relationship between wintertime polar circulation strength and the phase of the QBO in the lower stratosphere. In these experiments it is the extratropical planetary Rossby waves that provide the tropical-extratropical coupling mechanism. More easterly tropical winds in the lower stratosphere act to confine the extratropical Rossby waves farther north and closer to the vortex at the QBO altitudes, weakening the vortex relative to the case of westerly QBO phase. While the QBO winds occur in the lower stratosphere, the anomaly in the polar vortex strength is strongest at higher levels.

O'Sullivan, Donal↗
NASA NTRS1993

Global normal-mode Rossby waves observed in stratospheric ozone data

Westward-propagating Rossby normal-mode planetary waves are documented in stratospheric ozone data using Solar Backscatter Ultraviolet (SBUV) satellite measurements. These modes are evidenced by enhanced spectral power and near-global coherence for westward-traveling zonal wave 1 oscillations with periods of 5-10 days. The ozone waves have maxima in high latitudes of the middle stratosphere (due to transport) and over midlatitudes in the upper stratosphere (due to photochemistry). These modes are nearly continuous throughout the eight years of SBUV observations, with maximum global coherence during the equinoxes. The upper-stratospheric waves are symmetric (in phase) between hemispheres, even for modes previously identified as antisymmetric in geopotential height. This behavior is due to differing wave vertical structure in each hemisphere; the planetary temperature waves are nearly in phase in the upper stratosphere, even though the height waves are out of phase. The observed ozone waves are furthermore compared to calculations based on linear wave transport and photochemistry, incorporating derived wind and temperature fields. Good agreement is found, showing that normal modes provide an idealized context to study the linear wave behavior of trace constituents in the real atmosphere.

Randel, William J.↗
NASA NTRS1993

Radon measurements in the lower tropical stratosphere - Evidence for rapid vertical transport and dehydration of tropospheric air

During the tropical experiment of NASA's Stratosphere-Troposphere Exchange Program (STEP), in situ radon and other trace constituent measurements were made aboard a NASA ER-2 high-altitude research aircraft to investigate the mechanisms of irreversible transfers from the troposphere into the tropical stratosphere. Observations made in and downwind of the cirrus shields of three large tropical cyclones and downwind of the cirrus anvil of a large cumulonimbus cloud cluster showed several clear instances of elevated radon activity occurring simultaneously with low total water mixing ratios. These observations are unambiguous evidence of an effective dehydration process, capable of reducing total water vapor mixing ratios to less than 2.5 ppmv, occurring in conjunction with troposphere-to-stratosphere transport and indicate that rapid localized convection, rather than slow regional mean motions, was responsible for the observed transports and associated with the accompanying dehydration. Radon activities measured in regions of active or recent troposphere-to-stratosphere transport were consistent with the 17 pCi/scm mean value needed to support the observed abundance of stratospheric 210 Pb.

Kritz, Mark A.↗
NASA NTRS1992

The coupling of the troposphere and stratosphere

A linear, time-dependent, primitive-equation, 3D numerical model is used to investigate the dynamical coupling between the troposphere and stratosphere through the vertical propagation of planetry waves. Attention is given to the roles of the tropopause in affecting the propagation of planetary waves and to the extent to which the stratosphere can determine its own wave driving, i.e., the sensitivity of the generation of the wave activity in the troposphere to the change of zonal wind in the stratosphere. Two maxima in Eliassen-Palm (EP) flux convergence are found for wave 1 in high latitudes, one in the upper stratosphere and the other in the upper troposphere. For wave 2 there is a third maximum north of the zero wind line in the tropical stratosphere. The formation of the maximum in EP-flux convergence in the upper troposphere is related to the dissipation of non-WKBJ waves near a local maximum of the refractive index. The existence of the local maximum in refractive index at the tropopause is a result of the great gradient of the buoyancy frequency as well as the vertical shear of the zonal flow there.

Chen, Ping↗