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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 289 records · Page 16
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Realistic operation of two residential cordwood-fired outdoor hydronic heater appliances—Part 3: Optical properties of black and brown carbon emissions

Residential biomass combustion is a source of carbonaceous aerosol. Inefficient combustion, particularly of solid fuels produces large quantities of black and brown carbon (BC and BrC). These particle types are important as they have noted effects on climate forcing and human health. One method of measuring these quantities is by measurement of aerosol light-absorption and scattering, which can be performed using an aethalometer and nephelometer, respectively. These instruments are widely deployed in the study of ambient air and are frequently used in air quality modeling and source apportionment studies. In this study, we will describe (1) a method for measuring primary BC and BrC emissions from two residential log-fired wood hydronic heaters and (2) the BC and BrC emission from these devices over a wide range of operating conditions, such as cold-starts, warm-starts, four different levels of output ranging from 15% to 100% maximum rated output, and periods of repeated cycling. The range in flue-gas BC concentrations, measured using an aethalometer at the 880 nanometer (nm) wavelength, were between 5.09 × 10 2 and 2.24 × 10 4 micrograms per cubic meter (µg/m 3 ) while the scattering coefficient of the flue-gas, measured by a nephelometer at 880 nm, ranged between 2.20 × 10 3 and 8.56 × 10 5 inverse megameters (Mm –1 ). The BrC concentrations, measured using the 370 nm wavelength of an aethalometer, were between 9.10 × 10 1 and 3.56 × 10 4 µg/m 3 . The calculated Angstrom Absorption Exponent (AAE) of the flue-gas aerosol ranged between 1.54 and 3.63. Performing a comparison between the measured BC concentration and an external particulate matter (PM) concentration showed that overall BC makes up roughly a quarter of the PM emitted by either of the two appliances. Further for both appliances, the cold-start and the test phase immediately following it had the highest BC and BrC concentrations, the highest measured scattering coefficient, as well as a low AAE.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗
DOE OSTI2024

Seasonal variability and predictability of monsoon precipitation in Southern Africa

Rainfed agriculture is the mainstay of economies across Southern Africa (SA), where most precipitation is received during the austral summer monsoon. This study aims to further our understanding of monsoon precipitation predictability over SA. We use three natural climate forcings, El Niño–Southern Oscillation, Indian Ocean Dipole (IOD), and the Indian Ocean Precipitation Dipole (IOPD)—the dominant precipitation variability mode—to construct an empirical model that exhibits significant skill over SA during monsoon in explaining precipitation variability and in forecasting it with a five-month lead. While most explained precipitation variance (50%–75%) comes from contemporaneous IOD and IOPD, preconditioning all three forcings is key in predicting monsoon precipitation with a zero to five-month lead. Seasonal forecasting systems accurately represent the interplay of the three forcings but show varying skills in representing their teleconnection over SA. This makes them less effective at predicting monsoon precipitation than the empirical model.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Rapid retreat of the southwestern Laurentide Ice Sheet during the Bølling-Allerød interval

The timing of Laurentide Ice Sheet deglaciation along its southwestern margin controlled the evolution of large glacial lakes and has implications for human migration into the Americas. Accurate reconstruction of the ice sheet’s retreat also constrains glacial isostatic adjustment models and is important for understanding ice-sheet sensitivity to climate forcing. Despite its significance, retreat of the southwestern Laurentide Ice Sheet (SWLIS) is poorly constrained by minimum-limiting 14 C data. We present 26 new cosmogenic 10 Be exposure ages spanning the western Interior Plains, Canada. Using a Bayesian framework, we combine these data with geomorphic mapping, 10 Be, and high-quality minimum-limiting 14 C ages to provide an updated chronology. This dataset presents an internally consistent retreat record and indicates that the initial detachment of the SWLIS from its convergence with the Cordilleran Ice Sheet began by ca. 15.0 ka, concurrent with or slightly prior to the onset of the Bølling-Allerød interval (14.7–12.9 ka) and retreated >1200 km to its Younger Dryas (YD) position in ~2500 yr. Ice-sheet stabilization at the Cree Lake Moraine facilitated a meltwater drainage route to the Arctic from glacial Lake Agassiz within the YD, but not necessarily at the beginning. Our record of deglaciation and new YD constraints demonstrate deglaciation of the Interior Plains was ~60% faster than suggested by minimum 14 C constraints alone. In conclusion, numerical modeling of this rapid retreat estimates a loss of ~3.7 m of sea-level equivalent from the SWLIS during the Bølling-Allerød interval.

58 GEOSCIENCES↗
DOE OSTI2023

Laurentide Ice Sheet persistence during Pleistocene interglacials

While there are no ice sheets in the Northern Hemisphere outside of Greenland today, it is uncertain whether this was also the case during most other Quaternary interglacials. We show, using in situ cosmogenic nuclides in ice-rafted debris, that the Laurentide Ice Sheet was likely more persistent during Quaternary interglacials than often thought. Low 26 Al/ 10 Be ratios (indicative of burial of the source area) in marine core sediment suggest sediment source areas experienced only brief (on the order of thousands of years) and/or infrequent ice-free interglacials over the past million years. Here these results imply that complete Laurentide deglaciation may have only occurred when climate forcings reached levels comparable to those of the early Holocene, making our current interglacial unusual relative to others of the mid-to-late Pleistocene.

58 GEOSCIENCES↗
DOE OSTI2020

A fast particle-based approach for calibrating a 3-D model of the Antarctic ice sheet

We consider the scientifically challenging and policy-relevant task of understanding the past and projecting the future dynamics of the Antarctic ice sheet. The Antarctic ice sheet has shown a highly nonlinear threshold response to past climate forcings. Triggering such a threshold response through anthropogenic greenhouse gas emissions would drive drastic and potentially fast sea level rise with important implications for coastal flood risks. Previous studies have combined information from ice sheet models and observations to calibrate model parameters. These studies have broken important new ground but have either adopted simple ice sheet models or have limited the number of parameters to allow for the use of more complex models. These limitations are largely due to the computational challenges posed by calibration as models become more computationally intensive or when the number of parameters increases. Here, we propose a method to alleviate this problem: a fast sequential Monte Carlo method that takes advantage of the massive parallelization afforded by modern high-performance computing systems. We use simulated examples to demonstrate how our sample-based approach provides accurate approximations to the posterior distributions of the calibrated parameters. The drastic reduction in computational times enables us to provide new insights into important scientific questions, for example, the impact of Pliocene era data and prior parameter information on sea level projections. These studies would be computationally prohibitive with other computational approaches for calibration such as Markov chain Monte Carlo or emulation-based methods. We also find considerable differences in the distributions of sea level projections when we account for a larger number of uncertain parameters. For example, based on the same ice sheet model and data set, the 99th percentile of the Antarctic ice sheet contribution to sea level rise in 2300 increases from 6.5 m to 13.1 m when we increase the number of calibrated parameters from three to 11. With previous calibration methods, it would be challenging to go beyond five parameters. Here, this work provides an important next step toward improving the uncertainty quantification of complex, computationally intensive and decision-relevant models.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Hydrologic Model Files (PRMS) for Historical Conditions in the East River Watershed, Colorado between 1987-2019

The data package contains model input and output file for the East River watershed (85 km2) located in the headwaters of the Colorado River. The model is the U.S. Geological Survey (USGS) Precipitation-Modeling Runoff System (PRMS) for the historical, or baseline, condition (1987-2019) to assess the efficiency of summer monsoon rains to generate streamflow. The finite difference grid resolution is 100 m with elevations resampled from the USGS National Elevation Dataset. LANDFIRE raster data is used to derive parameters of dominant cover type, summer and winter cover density, canopy interception characteristics for snow and rain and transmission coefficient for shortwave radiation. Climate forcing uses minimum and maximum daily temperature lapse rates defined by the two Snow Telemetry (SNOTEL) stations located in the vicinity of the East River adjusted for aspect. Schofield SNOTEL snowfall is spatially distributed using LiDAR derived snow depth observations from the Airborne Snow Observatory (ASO) flown 4 April 2016. Snow depths are converted to snow water equivalent based on ground surveys and density modeling. Rainfall is spatially distributed using the monthly Parameter-elevation Relationships on Independent Slopes Model 30-year monthly averages. Simulated solar radiation is calibrated to match weather station observations. Model verification of snow water equivalent (SWE) accumulation and ablation relies on the 2018 and 2019 ASO maps and weather station snow depth. The data package contains model input files in text format, model documentation in pfd and a readme.txt file to help users understand the file structure to run the program.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

WHONDRS Surface Water Dissolved Organic Carbon and FTICR-MS across Glacial Features in Svalbard 2022

This dataset supports a broader study examining climatic forcing of terrestrial greenhouse gas emission through permafrost and glaciers in Svalbard. The dataset provides geochemistry and organic matter characterization data generated from surface water collected from 11 sites across central Svalbard. Data were also collected in 2021 and can be found at https://data.ess-dive.lbl.gov/view/doi:10.15485/1888571. Additional related data were collected and will be published separately in collaboration with Yde and Kleber.This dataset is comprised of one main data folder containing (1) file-level metadata; (2) data dictionary; (3) field metadata; (4) dissolved organic carbon (DOC; measured as non-purgeable organic carbon; NPOC); (5) surface water sampling protocol; (6) readme; (7) methods codes; (8) international geo-sample number (IGSN) mapping file; (9) a folder of field photos; and (10) folder of high resolution characterization of organic matter via 7 Tesla Fourier transform ion cyclotron resonance mass spectrometry (FTICR-MS) generated through the Environmental Molecular Sciences Laboratory (EMSL; https://www.pnnl.gov/environmental-molecular-sciences-laboratory). The FTICR folder contains two subfolders, one containing the .xml data files and the other containing instructions for using Formularity (https://omics.pnl.gov/software/formularity) and an R script to process the data based on the user's specific needs. All files are .csv, .pdf, .R, .ref, or .xml.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2026

A bespoke model of Arctic river basins based on hillslope delineation: Model Archive

This dataset is a model archive of the paper A bespoke model of Arctic river basins based on hillslope delineation (in prep), which introduces a watershed decomposition and parameterization method for large scale permafrost hydrology simulation. With this dataset, this study aims to address the research question: whether a computationally efficient hillslope-based modeling framework can reliably simulate discharge at Arctic river-basin scales. This dataset contains model input and output data for five modeling scenarios at a study site located in the Sagavanirktok River basin. The five modeling scenarios include three modeling cases under temperate conditions using full 3D, decomposed 3D, and decomposed 2D modeling strategies; and two modeling cases under actual Arctic conditions with permafrost using full 3D and decomposed 2D modeling strategies. Simulations were performed using the Advanced Terrestrial Simulator (ATS, v1.6 for three temperate scenarios and v1.5 for two Arctic scenarios), a physics-rich integrated surface–subsurface hydrologic model with cryo-hydrology features. For the three temperate models, simulations were conducted for the period of 10/01/1993 - 09/30/2002; and for the two Arctic models, simulations were conducted for the period of 01/01/1994 - 12/31/2002. To facilitate reproducibility of simulations, all datasets are organized hierarchically. The dataset contains: (1) Mesh files (.exo) for full 3D model, decomposed 3D models, and decomposed 2D models, located in huc/190604020802_gauge15906000/mesh/. Mesh files can be visualized through Paraview or read by Python. (2) Climate forcings (.h5) for full 3D model and decomposed 3D/2D models are located in huc/190604020802_gauge15906000/daymet_onePiece/, and huc/190604020802_gauge15906000/vp_pr_revised_daymet_1980_2006_with_wind/ separately. Accessible by Python. (3) Raw measured gage discharge (.csv) from USGS, located in huc/190604020802_gauge15906000/gaged_basin15906000_discharge_usgs/. Accessible by Python. (4) Delineated subdomain raster (.tif) and shape files (.shp), and the final parameterized results (.npy) for decomposed models, located in huc/190604020802_gauge15906000/data_preprocessed-meshing. Accessible by Python. (5) Temperate models are located in nonpermaf_huc190604020802_gauge15906000/, which includes three cases: decomposed 2D models (inside model_0*-hillslope_*), decomposed 3D models (inside model_1*-subcatchment_*), and full 3D model (inside model_2*-onepiece_*). Two step spin-up results (checkpoint_final.h5) are located in model_*1-*_spinup_steadystate and model_*2-*_spinup_cycle, separately, which are used to initialize real transient models. The input files (.xml) and output results (.dat) of the real transient models are located in model_*3-*_transient/. Especially, for two example hillslope models (ID=-11 and 11), additional h5py files are included in model_03-hillslope_transient/hillslope-11/, model_03-hillslope_transient/hillslope11, model_13-subcatchment_transient/subcatchment-11/, model_13-subcatchment_transient/subcatchment/11, respectively, which are used to plot the saturation figure (Figure 5) in the manuscript. Accessible by Python. (6) Arctic models are located in huc190604020802_gauge15906000/, which includes two cases: decomposed 2D models (inside model_04-hillslope_transient), and full 3D model (inside model_05-onepiece_transient_mannp1_ra). Three step spin-up results (checkpoint_final.h5) are located in model_01-column_freezeup/, model_02-column_spinup/, model_03-hillslope_spinup/, respectively, which are used to initialize real 2D transient hillslope models. The input files (.xml) and output results (.dat) of transient 2D hillslope models are located in model_04-hillslope_transient/. The input files (.xml) and output results (.dat) of the full 3D transient model is located in model_05-onepiece_transient_mannp1_ra/. The full 3D transient model is initialized by model_02-column_spinup/. Accessible by Python. (7) The MOSART routed discharge results (.csv) under Arctic conditions is located in huc190604020802_gauge15906000/MOSART/. Accessible by Python. (8) All Python codes (.py) used to parameterize full 3D model to decomposed 2D models are located in script/. These codes fit with watershed workflow (a watershed delineation tool) v1.4 under the branch gaob/v1.4 from https://github.com/gaobhub/watershed-workflow.git.

EARTH SCIENCE > CRYOSPHERE↗
DOE OSTI2020

Paleo-Megadroughts and Abrupt Climate Changes in the Speleothem Records. Final report

This project is motivated by the speleothem isotope records in Asia, which show regional responses in the hydrologic cycle to different climate forcings. Speleothem isotopic records are typically interpreted in terms of local precipitation variations or monsoon intensity. Our study demonstrates that non-local processes also play an important role. We started this project to understand the regional difference in speleothem isotopic composition between the Last Glacial Maximum (LGM) and the present-day. The record in Southwest China showed greater depletion during the LGM compared to those in East China. Our modeling and analysis showed that speleothems record, in addition, large scale changes in atmospheric circulation and moisture transport and their subsequent impact on precipitation. We developed an algorithm to partition total precipitation according to their formation dynamics, namely into frontal and non-frontal precipitation, and showed that the two have different trends and hence different causal mechanism. We then focused our subsequent attention on circulation impacts on precipitation changes. We applied a machine learning algorithm to detect rainbands in the ERA-Interim reanalysis product, and showed that the seasonal migrations of the rainbands are tied to the seasonal migrations of the jet stream, in particular the northerlies of the jet meanders. These northerlies, in turn, are partly topographic Rossby waves excited as the upstream westerlies impinge on the Tibetan Plateau. The seasonal variations of these upstream westerlies thus contribute to the seasonal movements of the rainbands and regional precipitation changes. Our analysis of the modern precipitation isotope record further confirms the importance of jet stream changes in the isotopic variations and shows that isotope-enriched years have reduced summer seasonality, with less pronounced northward migration of the jet.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Toward Hybrid Physics-Machine Learning to improve Land Surface Model predictions

A critical challenge for Land Surface Models (LSMs) is to simulate processes at the surface and the subsurface and their feedbacks to the atmosphere. Even using the same climate forcings, different LSMs predict different surface fluxes and soil moisture conditions due to differences in the formulations of individual processes, parameterizations, and representation of spatial heterogeneity. Ultimately, these differences contribute to the LSM prediction errors and uncertainty. This research seeks to address this challenge by coupling physics-based modeling with state-of-the-art machine learning (ML) techniques to describe complex physical and biogeochemical processes and narrow the gap between model predictions and observations.

58 GEOSCIENCES↗
DOE OSTI2022

NGEE Arctic LANL Overview [Slides]

The Next-Generation Ecosystem Experiments (NGEE Arctic) project has a goal to "deliver a process-rich ecosystem model, extending from bedrock to the top of the vegetative canopy/atmospheric interface, in which the evolution of Arctic ecosystems in a changing climate can be modeled at the scale of a high resolution Earth System Model (ESM) grid cell." LANL works across multiple NGEE Arctic science questions, such as: Q1. How does the structure and organization of the landscape control permafrost evolution and associated carbon and nutrient fluxes in a changing climate? Q5. Where, when, and why will the Arctic become wetter or drier, and what are the implications for climate forcing? and Q6. What controls the vulnerability of Arctic ecosystems to disturbance, and how do disturbances alter the structure and function of these ecosystems? This report features LANL's research summaries.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Cleaner Cooking: Exploring Tools to Measure and Understand the Long-term Adoption and Environmental Significance of Cookstoves in India

About 40% of the world’s population, or roughly 3 billion people, rely on solid biomass fuels like coal, wood, dung, and crop residues to cook and meet their household energy needs. This outdated energy system has severe social, health, and environmental implications. Women are disproportionately affected as they predominantly bear the burden of cooking and collecting fuelwood, which exacerbates the “time poverty” trap that restricts them from participating in economic and educational activities. Exposure to indoor solid fuel combustion, also known as household air pollution, is responsible for 3-4 million premature deaths per year and is a leading risk factor for chronic obstructive pulmonary disease, childhood pneumonia, stroke, ischemic heart disease, and lung cancer. Solid-fuel cooking contributes to 16% of global ambient air pollution, emitting CO 2 and other climate-forcing pollutants like carbon monoxide, black carbon, and methane.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗
DOE OSTI2025

PNNL-ANL Hydrometeorological Super Ensemble

The current dataset contains data upload links to the following **hydrologic (water balance), river routing (water management), and hydropower simulation** data over CONUS: * Climate Forcing: **Livneh** (https://www.nature.com/articles/sdata201542) * Simulation Scenario: **Historical** * Simulation Period: **1971-2013 (1972-2013 for Hydropower)** * Simulation Models: **VIC (Variable Infiltration Capacity)**, **mosartwmpy (Model for Scale Adaptive River Transport-Water Management in Python)**, and **PNNL B1Hydro** * Output Format: **NetCDF** and **CSV**

Tidwell, Vincent C [Pacific Northwest National Lab↗
DOE OSTI2025

PNNL-ANL Hydrometeorological Super Ensemble

The current dataset contains data upload links to the following hydrologic (water balance), river routing (water management), and hydropower simulation data over CONUS: Climate Forcing: ClimRR (https://climrr.anl.gov/climrrdata) Simulation Scenario: Historical, Mid-Century, End-Century Simulation Period: 1995-2004, 2045-2054, 2085-2094 Simulation Models: VIC (Variable Infiltration Capacity), mosartwmpy (Model for Scale Adaptive River Transport-Water Management in Python), and PNNL B1Hydro Output Format: NetCDF and CSV

Tidwell, Vincent C [Pacific Northwest National Lab↗
DOE OSTI2025

TGW Hydrology, River Routing, and Hydropower Simulation Datasets

he current dataset contains data upload links to the following hydrologic (water balance), river routing (water management), and hydropower simulation data over CONUS: Climate Forcing: TGW (https://tgw-data.msdlive.org/) Simulation Scenario: Historical, Mid-Century, End-Century Simulation Period: 1980-2024, 2020-2059, 2060-2099 Simulation Models: VIC (Variable Infiltration Capacity), mosartwmpy (Model for Scale Adaptive River Transport-Water Management in Python), and PNNL B1Hydro Output Format: NetCDF and CSV

Tidwell, Vincent C [Pacific Northwest National Lab↗
DOE OSTI2023

Source apportionment of soot particles and aqueous-phase processing of black carbon coatings in an urban environment

Abstract. The impacts of soot particles on climate and human health depend on the concentration of black carbon (BC) as well as the thickness and composition of the coating material, i.e., organic and inorganic compounds internally mixed with BC. In this study, the size-resolved chemical composition of BC-containing aerosol was measured using a high-resolution soot particle aerosol mass spectrometer (SP-AMS) during wintertime in Fresno, California, a location influenced by abundant combustion emissions and frequent fog events. Concurrently, particle optical properties were measured to investigate the BC absorption enhancement. Positive matrix factorization (PMF) analysis was performed on the SP-AMS mass spectral measurements to explore the sources of soot particles and the atmospheric processes affecting the properties of BC coatings. The analysis revealed that residential woodburning and traffic are the dominant sources of soot particles. Alongside primary soot particles originating from biomass burning (BBOABC) and vehicles (HOABC) two distinct types of processed BC-containing aerosol were identified: fog-related oxidized organic aerosol (FOOABC) and winter-background OOABC (WOOABC). Both types of OOABC showed evidence of having undergone aqueous processing, albeit with differences. The concentration of FOOABC was substantially elevated during fog events, indicating the formation of aqueous secondary organic aerosol (aqSOA) within fog droplets. On the other hand, WOOABC was present at a relatively consistent concentration throughout the winter and was likely related to the formation of secondary organic aerosol (SOA) in both the gas phase and aerosol liquid water. By comparing the chemical properties and temporal variations in FOOABC and WOOABC, we gain insights into the key aging processes of BC aerosol. It was found that aqueous-phase reactions facilitated by fog droplets had a significant impact on the thickness and chemical composition of BC coatings, thereby affecting the light absorption and hygroscopic properties of soot particles. These findings underscore the important role of chemical reactions occurring within clouds and fogs and influencing the climate forcing of BC aerosol in the atmosphere.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

A remote sensing algorithm for vertically resolved cloud condensation nuclei number concentrations from airborne and spaceborne lidar observations

Cloud condensation nuclei (CCN) are mediators of aerosol–cloud interactions (ACIs), contributing to the largest uncertainties in the understandings of global climate change. We present a novel remote-sensing-based algorithm that quantifies the vertically resolved CCN number concentrations (N CCN ) using aerosol optical properties measured by a multiwavelength lidar. The algorithm considers five distinct aerosol subtypes with bimodal size distributions. The inversion used the lookup tables developed in this study, based on the observations from the Aerosol Robotic Network, to efficiently retrieve optimal particle size distributions from lidar measurements. The method derives dry aerosol optical properties by implementing hygroscopic enhancement factors in lidar measurements. The retrieved optically equivalent particle size distributions and aerosol-type-dependent particle composition are utilized to calculate critical diameters using κ-Köhler theory and N CCN at six supersaturations ranging from 0.07 % to 1.0 %. Sensitivity analyses indicate that uncertainties in extinction coefficients and relative humidity greatly influence the retrieval error in N CCN . The potential of this algorithm is further evaluated by retrieving N CCN using airborne lidar from the NASA ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES) campaign and is validated against simultaneous measurements from the CCN counter. The independent validation with robust correlation demonstrates promising results. Furthermore, the N CCN has been retrieved for the first time using a proposed algorithm from spaceborne lidar – Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) – measurements. The application of this new capability demonstrates the potential for constructing a 3D CCN climatology at a global scale, which helps to better quantify ACI effects and thus reduce the uncertainty in aerosol climate forcing.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Atmospheric processing and aerosol aging responsible for observed increase in absorptivity of long-range-transported smoke over the southeast Atlantic

Biomass burning aerosol (BBA) from agricultural fires in southern Africa contributes about one-third of the global carbonaceous aerosol load. These particles have strong radiative effects in the southeast Atlantic (SEA), which depend in part on the radiative contrast between the aerosol layer in the free troposphere (FT) and the underlying cloud layer. However, there is large disagreement in model estimates of aerosol-driven climate forcing due to uncertainties in the vertical distribution, optical properties, and life cycle of these particles. This study applies a novel method combining remote sensing observations with regional model outputs to investigate the aging of the BBA and its impact on the optical properties during transatlantic transport from emission sources in Africa to the SEA. Results show distinct variations in extinction Ångström exponent (EAE) and single-scattering albedo (SSA) as aerosols age. Near the source, fresh aerosols are characterized by low mean SSA (0.84) and high EAE (1.85), indicating smaller, highly absorbing particles. By isolating marine contributions from the total column during BBA transport across the SEA, our analysis reveals an initial decrease in BBA absorptivity, with mean FT SSA of 0.87 after 6–7 d, followed by increased absorptivity with mean FT SSA of 0.84 after 10 d, suggesting enhanced absorption due to chemical aging. These findings indicate that BBA becomes more absorbing during extended transport across the SEA, with implications for reducing model uncertainties. Our remote-sensing-based results agree well with previous in situ studies and offer new insights into aerosol–radiation interactions and the energy balance over the SEA.

54 ENVIRONMENTAL SCIENCES↗