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At least 289 records · Page 16

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DOE OSTI2024

Comparing the interactions between particulate matter and cloud properties over two populated cities in Texas using WRF-Chem fine-resolution modeling

Accurate modeling of aerosol-cloud interactions is essential for reliable weather and air quality simulations, given their significant impact on precipitation patterns, cloud dynamics, and aerosol distributions. This study employed the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) to examine the impact of enhanced meteorological simulations, achieved through advanced microphysics parameterization supported by data assimilation techniques, on air quality across Texas on August 19 and 20, 2022. We tested four distinct configurations: (1) the Morrison two-moment bulk microphysics scheme, (2) Morrison's with observation nudging, (3) the Spectral Bin Microphysics (SBM), and (4) SBM with observation nudging. While the SBM scheme is known for its detailed representation of aerosol-cloud interactions, our focus was on how improvements in meteorological accuracy translate to more precise air quality simulations. Our findings demonstrated a progressive improvement in simulation accuracy, starting with the Morrison's scheme and further enhanced by adopting the SBM scheme, complemented by incorporating observation nudging. Specifically, the combination of the SBM scheme and the nudging substantially enhanced the model's ability to capture convective precipitation events, as shown by better alignment with NEXRAD radar reflectivity, with R increasing from –0.21 to 0.82, IOA from 0.10 to 0.87, and NMB decreasing from 99% to 34% in Houston. The enhanced meteorology translated into more accurate PM 2.5 concentration simulations, particularly through the more accurate representation of aerosol washout during precipitation events. In Houston, the SBM scheme with nudging improved the model's PM 2.5 simulations significantly, with NMB decreasing from –20% to 5% and IOA improving from 0.43 to 0.61. In San Antonio, improvements were also notable, with NMB improved from –27% to –22%, R increased from 0.48 to 0.82, and IOA increased from 0.66 to 0.86. Furthermore, our results underscore the crucial role of accurate meteorological simulations in refining our understanding of aerosol behaviors in relation to precipitation patterns, directly enhancing the reliability and effectiveness of air quality modeling.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2025

Predicting runtime and resource utilization of jobs on integrated cloud and HPC systems

Recent advances in virtualization technologies used in cloud computing offer performance that closely approaches bare-metal levels. Combined with specialized instance types and high-speed networking services for cluster computing, cloud platforms have become a compelling option for high-performance computing (HPC). However, most current batch job schedulers in HPC systems are designed for homogeneous clusters and make decisions based on limited information about jobs and system status. Scientists typically submit computational jobs to these schedulers with a requested runtime that is often over- or under-estimated. More accurate runtime predictions can help schedulers make better decisions and reduce job turnaround times. Here, they can also support decisions about migrating jobs to the cloud to avoid long queue wait times in HPC systems.

97 MATHEMATICS AND COMPUTING↗

DOE OSTI2025

Microphysics Dominates Sub‐Cloud Rain Evaporation in Trade Cumuli Over Barbados

This study investigates the microphysical and thermodynamic influences on North Atlantic trade-cumulus rain evaporation in the sub-cloud layer over Barbados from January to November 2020. Using radar observations and a 1-D model, the results reveal that microphysical properties, namely geometric mean diameter (D g ) and raindrop concentration, primarily control evaporation processes under conditions of limited thermodynamic variability. Thermodynamic factors like cloud base height and relative humidity exert a smaller influence due to their narrow observed ranges. Small D g leads to rapid increases in rain evaporation fraction (REF), as small drops evaporate completely, while larger D g yields slower, more gradual REF changes. Frequent weak-rain cases reduce the mean evaporation flux, whereas infrequent intense-rain events substantially enhance it. These findings highlight the pivotal role of microphysical variability in shaping sub-cloud evaporation in this trade cumulus regime, while thermodynamic effects may be more important in other environments.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2025

High Performance, High Fidelity: A GPU‐Accelerated Doubly‐Periodic Configuration of the Simple Cloud‐Resolving E3SM Atmosphere Model Version 1 (DP‐SCREAMv1)

The development of the Simplified Cloud Resolving Energy Exascale Earth System Atmosphere Model (SCREAMv1) enables global storm-resolving simulations on modern GPU-based supercomputers. However, the high computational cost of SCREAMv1 limits its routine use for process-level studies, creating a need for efficient proxy configurations. This study addresses this gap by introducing DP-SCREAMv1, a doubly periodic cloud-resolving model designed to be fully consistent with SCREAMv1 while enabling high-resolution, long-duration simulations at significantly reduced computational expense by simulating a limited doubly periodic domain rather than the entire globe. Built on a C++/Kokkos architecture, DP-SCREAMv1 achieves exceptional performance scalability on GPU systems and includes a rich library of cases for validation and scientific exploration. In this work, we demonstrate short wall-clock times at SCREAMv1's default resolution and show that DP-SCREAMv1 supports routine execution of large-domain, high-resolution experiments that were previously challenging in practice. Furthermore, we show that DP-SCREAMv1 enables routine execution of “Giga-LES” style simulations and facilitates large-domain, high-resolution simulations that were recently considered burdensome to perform. These results document an efficient, fully consistent process-level configuration for SCREAMv1 (DP-SCREAMv1) and illustrate its use for long-duration and large-domain experiments at cloud-resolving to eddy-permitting resolution.

Environmental sciences↗

DOE OSTI2024

Training the next generation of researchers in exploring cloud dynamics and microphysics using millimeter-wavelength radars

Millimeter-wavelength radars, with their ability to collect observations and high spatiotemporal resolution, have become cornerstone instruments for investigating cloud and precipitation microphysics and dynamics in the last two decades. Since the1990s the US Department of Energy Atmospheric Radiation Measurement (ARM) program has invested in mm-wavelength radar technology progressively adding scanning capability, additional frequencies and polarimetric capability. In addition, atmospheric observatories including those technologies have been operated overseas. Those technologies have enhanced our understanding of cloud and precipitation processes. Only a few universities operate those instruments and use them for educational purposes. The central role of mm- wavelength radars and their role will be further highlighted in the next decade. NASA and other international space agencies are planning to launch millimeter-wavelength (i.e., Ku, Ka, W, G- bands) Doppler radar in space to improve our understanding of cloud and precipitation formation, evolution and their impacts on global climate.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2024

LAACI – Light Absorbing Aerosol-Cloud Interactions Experiment

The “Light Absorbing Aerosol-Cloud Interactions Experiment” project aimed at studying the interactions of light-absorbing aerosols from biomass burning (e.g., wildfires or prescribed fires) with clouds. The core of the project was carried out at the Michigan Technological University turbulent cloud chamber facility (hereafter referred to as the Pi-Chamber). Light-absorbing aerosols from biomass burning include black carbon (BC) and brown carbon (BrC) organic material.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2026

Warped and Hooked: Mapping the Magellanic Clouds in Three Dimensions Using Red Clump Stars

The Large Magellanic Cloud (LMC) and Small Magellanic Cloud (SMC) are the Milky Way’s nearest interacting galaxy pair, offering a unique laboratory for studying tidal effects on galactic disks. Despite extensive survey efforts, the 3D geometry of the Magellanic Clouds, particularly the putative warp of the LMC, remains poorly constrained due to incompleteness in their crowded centers and the low stellar density of their peripheries, which demand wide-field coverage. Using red clump (RC) stars as standard candles, corrected for age- and metallicity-dependent population effects with empirically calibrated color–magnitude relations and spatially resolved star formation histories, we construct the most detailed distance map of the Magellanic system to date. Based on ∼2.3 million RC stars from Gaia Data Release 3 combined with modern reddening maps, we measure median heliocentric distances of 50.62 ± 2.32 kpc for the LMC (to ∼23°) and 60.75 ± 2.85 kpc for the SMC (to ∼12°). The maps reveal substructures including the LMC Northern Arm, southern hooks, the Magellanic Bridge, and SMC peripheral overdensities, with refreshed distance estimates. Fitting the LMC disk within 7° yields a global inclination of $i=25\mathop{.}\limits^{^\circ }32\pm 0\mathop{.}\limits^{^\circ }10$ and a line-of-nodes position angle of $\theta = 142\mathop{.}\limits^{^\circ }34\pm 0\mathop{.}\limits^{^\circ }21$. Most strikingly, we find the LMC periphery is warped azimuthally into a U-shaped structure reaching a vertical amplitude of ∼7 kpc at a radius of ∼15 kpc. In future work, we will perform detailed comparisons with live N-body simulations to assess possible formation scenarios for the LMC warp.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2025

Prescribing the aerosol effective radiative forcing in the Simple Cloud-Resolving E3SM Atmosphere Model v1

Aerosol effective radiative forcing critically influences climate projections but remains poorly constrained. Using the Simple Cloud-Resolving E3SM Atmosphere Model (SCREAM) v1 configuration, we assess the sensitivity of the radiative forcing due to anthropogenic aerosol changes using a simplified prescribed aerosol scheme (SPA) derived from E3SM v3. Nudged simulations at 3 and 12 km horizontal grid spacings reveal a more negative aerosol forcing than the reference 100 km E3SM v3 whence the SPA properties are derived. The resulting globally averaged aerosol forcing signal is largely due to aerosol–cloud interactions and exhibits little overall resolution sensitivity, while hints of resolution sensitivity appear regionally between the 3 and 12 km runs. While the default SPA scheme overestimates cloud droplet dependence on aerosols, parameterization adjustments in the activation process reconcile forcing estimates with the reference model. Our results demonstrate the ability to use a prescribed aerosol scheme to hold aerosol forcing to a desired strength across resolutions.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2026

W-Band ARM Scanning Cloud Radar (WSACR) 2nd Generation CF-Radial Spectral Data, Vertically-Pointing Scan, Co-Polarization Mode (a1)

ARM's scanning cloud radars are fully coherent dual-frequency, dual-polarization Doppler radars mounted on a common scanning pedestal. Each pedestal includes a Ka-band radar (2kW peak power) and the deployment location determines whether the second radar is a W-band (WSACR; 1.7 kW peak power) or X-band (XSACR; 20 kW peak power). Beamwidths at Ka and W bands are roughly matched at 0.3 degrees. Due to the narrow antenna beamwidth, ARM’s scanning cloud radars use scanning strategies that are unlike typical weather radars. Rather than focusing on plan position indicator, or PPI, scans, the Ka-SACR uses range height indicator, or RHI, scans at numerous azimuths to obtain cloud volume data. Measurements collected with the W-SACR are copolar and cross-polar radar reflectivity, Doppler velocity, spectra width and spectra when not scanning, and linear depolarization ration.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2026

W-Band ARM Scanning Cloud Radar (WSACR) 2nd Generation CF-Radial Spectral Data, Vertically-Pointing Scan, Cross Mode (a1)

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2026

W-Band ARM Scanning Cloud Radar (WSACR) 2nd Generation CF-Radial Spectral Data, Vertically-Pointing Scan, Cross-Polarization Model (a1)

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2025

The Two Arctic Wintertime Boundary Layer States: Disentangling the Role of Cloud and Wind Regimes in Reanalysis and Observations During MOSAiC

The wintertime central Arctic atmosphere comprises a radiatively clear and a radiatively opaque state, which are linked to synoptic forcing and mixed-phase clouds. Weather and climate models often lack process representations surrounding these states, but prior work mostly treated the problem as an aggregate of synoptic conditions, resulting in partially overlapping biases. Here, we disaggregate the Arctic states and confront ERA5 reanalysis with observations from the MOSAiC campaign over the central Arctic sea ice during winter 2019/2020. Low-level winds and liquid water path (LWP) are combined to derive different synoptic classes. Results show that the clear state is primarily formed by weak/moderate winds and the absence of liquid-bearing clouds, while strong winds and enhanced LWP primarily form the radiatively opaque state. ERA5 struggles to reproduce these basic statistics, shows too weak sensitivity of thermal radiation to synoptic forcing, and overestimates thermal radiation for similar LWP amounts. The latter is caused by a warm bias, which has a pronounced inversion structure and is largest in clear and calm conditions. Under strong synoptic forcing, the warm bias is constant with height and discrepancies in mixed-phase cloud altitude appear. Separating synoptic conditions is regarded as useful for process-oriented evaluation of the Arctic troposphere in models.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2024

Accelerating Computational Materials Discovery with Machine Learning and Cloud High-Performance Computing: from Large-Scale Screening to Experimental Validation

High-throughput computational materials discovery has promised significant acceleration of the design and discovery of new materials for many years. Despite a surge in interest and activity, the constraints imposed by large-scale computational resources present a significant bottleneck. Furthermore, examples of large-scale computational discovery carried through experimental validation remain scarce, especially for materials with product applicability. In this paper, we demonstrate how this vision became reality by first combining state-of-the-art artificial intelligence (AI) models and traditional physics-based models on cloud high performance computing (HPC) resources to quickly navigate through more than 32 million candidates and predict around half a million potentially stable materials. Focusing on solid-state electrolytes for battery applications, our discovery pipeline further identified 18 promising candidates with new compositions and rediscovered a decade’s worth of collective knowledge in the field as a byproduct. By employing around one thousand virtual machines in the cloud, this process took less than 80 hours. We then synthesized and experimentally characterized the structures and conductivities of our top candidates, the Na x Li 3-x YCl 6 (0.5 ≤ x ≤ 2.5) series, demonstrating the potential of these compounds to serve as solid electrolytes. Additional candidate materials are currently under experimental investigation that could offer more examples of the computational discovery of new phases of Li- and Na-conducting solid electrolytes. We believe this unprecedented approach of synergistically integrating AI models and cloud HPC not only accelerates materials discovery but also showcases the potency of AI-guided experimentation in unlocking transformative scientific breakthroughs with real-world applications.

36 MATERIALS SCIENCE↗

DOE OSTI2024

How Well Does the DOE Global Storm Resolving Model Simulate Clouds and Precipitation Over the Amazon?

This study assesses a 40-day 3.25-km global simulation of the Simple Cloud-Resolving E3SM Model (SCREAMv0) using high-resolution ground-based observations from the Atmospheric Radiation Measurement (ARM) Green Ocean Amazon (GoAmazon) field campaign. SCREAMv0 reasonably captures the diurnal timing of boundary layer clouds yet underestimates the boundary layer cloud fraction and mid-level congestus. SCREAMv0 well replicates the precipitation diurnal cycle, however it exhibits biases in the precipitation cluster size distribution compared to scanning radar observations. Specifically, SCREAMv0 overproduces clusters smaller than 128 km, and does not form enough large clusters. Such biases suggest an inhibition of convective upscale growth, preventing isolated deep convective clusters from evolving into larger mesoscale systems. This model bias is partially attributed to the misrepresentation of land-atmosphere coupling. This study highlights the potential use of high-resolution ground-based observations to diagnose convective processes in global storm resolving model simulations, identify key model deficiencies, and guide future process-oriented model sensitivity tests and detailed analyses.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2024

Source Levels of In‐Cloud Air in Shallow Cumulus: Consistency Between Paluch Diagram and Lagrangian Particle Tracking

Abstract The Paluch diagram is a widely used tool for interpreting aircraft measurements of shallow cumulus clouds. A prior study conducted by Heus et al. (2008,https://doi.org/10.1175/2008jas2572.1) concluded that the source levels of in‐cloud air inferred from the Paluch diagram exhibit biases, sometimes of several hundred meters, in comparison to those derived from Lagrangian particle tracking. In this short study we revisit this comparison. The results indicate that the upper source levels of in‐cloud air determined from the Lagrangian Particle Tracking and the Paluch diagram are consistent, and the choice of statistical methods is crucial. The significance of this research lies in confirming the reliability of the Paluch analysis, enabling its confident application to aircraft data.

Meteorology & Atmospheric Sciences↗

DOE OSTI2024

Improving Low‐Cloud Fraction Prediction Through Machine Learning

Abstract In this study, we evaluated the performance of machine learning (ML) models (XGBoost) in predicting low‐cloud fraction (LCF), compared to two generations of the community atmospheric model (CAM5 and CAM6) and ERA5 reanalysis data, each having a different cloud scheme. ML models show a substantial enhancement in predicting LCF regarding root mean squared errors and correlation coefficients. The good performance is consistent across the full spectrums of atmospheric stability and large‐scale vertical velocity. Employing an explainable ML approach, we revealed the importance of including the amount of available moisture in ML models for representing spatiotemporal variations in LCF in the midlatitudes. Also, ML models demonstrated marked improvement in capturing the LCF variations during the stratocumulus‐to‐cumulus transition (SCT). This study suggests ML models' great potential to address the longstanding issues of “too few” low clouds and “too rapid” SCT in global climate models.

Geology↗

DOE OSTI2025

Studying Aerosol, Clouds, and Air Quality in the Coastal Urban Environment of Southeastern Texas

A multi-agency succession of field campaigns was conducted in southeastern Texas during July 2021 through October 2022 to study the complex interactions of aerosols, clouds and air pollution in the coastal urban environment. As part of the Tracking Aerosol Convection interactions Experiment (TRACER), the TRACER- Air Quality (TAQ) campaign the Experiment of Sea Breeze Convection, Aerosols, Precipitation and Environment (ESCAPE) and the Convective Cloud Urban Boundary Layer Experiment (CUBE), a combination of ground-based supersites and mobile laboratories, shipborne measurements and aircraft-based instrumentation were deployed. These diverse platforms collected high-resolution data to characterize the aerosol microphysics and chemistry, cloud and precipitation micro- and macro-physical properties, environmental thermodynamics and air quality-relevant constituents that are being used in follow-on analysis and modeling activities. We present the overall deployment setups, a summary of the campaign conditions and a sampling of early research results related to: (a) aerosol precursors in the urban environment, (b) influences of local meteorology on air pollution, (c) detailed observations of the sea breeze circulation, (d) retrieved supersaturation in convective updrafts, (e) characterizing the convective updraft lifecycle, (f) variability in lightning characteristics of convective storms and (g) urban influences on surface energy fluxes. The work concludes with discussion of future research activities highlighted by the TRACER model-intercomparison project to explore the representation of aerosol-convective interactions in high-resolution simulations.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2024

Coastal Cloud Chemistry during EPCAPE Field Campaign Report

For this campaign, Principal Investigator Markus Petters deployed a suite of instruments inside Lynn Russell’s container that was sited at Mt. Soledad during the Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE) campaign. Funding for this activity was provided by National Science Foundation Award 2410536. The instrument rack (Figure 1) included a differential mobility analyzer, a condensation particle counter, a portable optical particle spectrometer, and a continuous flow diffusion cloud condensation nuclei counter (CCN). The instruments sampled from a counterflow virtual impactor (CVI) inlet and an isokinetic inlet. The measurements provided aerosol size distribution, size-resolved CCN activity, and denuded versus undenuded CCN activity of aerosols and cloud drop residuals.

54 ENVIRONMENTAL SCIENCES↗