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At least 289 records · Page 16
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Gas Stopper Developments for Improved Purity and Intensity of Low-Energy, Rare Isotope Ion Beams (Final Technical Report)

This final technical report summarizes the work of the Michigan State University (MSU) team supported by grant # DE-SC0021423 awarded by the Office of Nuclear Physics, Department of Energy. Objectives: The successful fulfillment of the FRIB science mission hinges on ensuring the availability of fast, stopped, and reaccelerated beams consisting of rare isotopes. This project's research and development focus was dedicated to supporting the advancement and creation of a cutting-edge linear gas stopper. The primary aim is to efficiently convert the high-intensity fast beams of rare isotopes provided by FRIB into high-quality, low-energy beams. These beams are essential for conducting stopped beam experiments or for subsequent reacceleration. The overarching goal is to advance technology, aiming to increase the beam rate capability of the linear gas stopper for medium-to-heavy-mass rare isotopes by more than tenfold compared to the currently most effective gas stopper in operation, and to improve the purity of the delivered beams. Project Description: The existing technology employed in gas stopping devices designed for low-energy, rare-isotope beams presents limitations in both the purity of extracted beams and the intensities of injected beams. These limitations are incompatible with the requirements of the recently commissioned rare isotope beam facility, FRIB. Our research and development efforts, aligned with the previously outlined objectives, focused on addressing the most critical aspects for enhancing beam-rate capability and purity. Specifically, advanced particle-in-cell simulations were developed and integrated into a simulation pipeline to explore the efficacy of multi-layer RF carpets on increasing ion transport efficiency with high incoming beam rates that generate space charge fields which can limit it. We also explored the possibility of using a collision-induced-dissociation (CID) gas cell to break up molecular contaminant ions that are generated during the stopping process. A prototype CID gas cell was constructed and tested with beams from an offline ion source, validating the concept with the successful demonstration of breaking of molecular ions. The outcome of this research enabled the formulation a conceptual design for a next-generation linear gas stopping device specifically tailored for FRIB. This device is envisioned to deliver rare-isotope-ion beams at a rate of 10 8 particles per second or higher, accompanied by advancements in purity. Methods employed: This project leverages advancements in technologies initially designed for the Advanced Cryogenic Gas Stopper (ACGS), the current state-of-the-art linear gas stopper, through the use of new simulations and beam purification via collision-induced-dissociation. The methods include: 1. Development of a prototype low-energy, low-pressure CID gas stopper. This prototype features a thin, approximately 20 nm, Si 3 N 4 entrance window designed for dissociating stable and rare-isotope molecular ions. The goal is to enhance beam purification and overall efficiency. 2. Creation of Particle-in-cell (PIC) simulations to assess the advantages of multi-layer RF carpets and multi-point extraction for ion transport efficiency. These simulations rely on the 3DCylPIC package, specifically designed for studying devices of this nature. The goal is to quantify and mitigate ion transport losses due to space charge generated in the stopping process of large numbers of ions. 3. Perform ion transport simulations across an RF carpet using an 8-phase travelling wave and evaluate its performance. Compared to the 4-phase RF carpets used in ACGS, the 8-phase carpets will double the wavelength of the generated traveling wave allowing for larger maximum RF amplitudes that could result in improved ion transport efficiency for high-intensity incoming beams when large space charge fields are present. Impact: Tackling the primary challenges associated with transforming high-energy projectile fragment beams into low-energy beams—specifically, addressing efficiency and purity—holds significant promise for advancing FRIB science. This advancement will particularly impact precision mass measurements, laser spectroscopy of short-lived nuclei, and studies in astrophysics and nuclear reactions using reaccelerated beams. These domains play a crucial role in addressing key questions outlined in the 2023 NSAC long-range plan, spanning nuclear structure, nuclear astrophysics, and fundamental symmetries. Additionally, they contribute to addressing 10 out of the 17 benchmarks identified by the NRC RISAC. The development of a next-generation gas stopping device capable of delivering low-energy, rare-isotope beams at a rate of 10 8 particles per second, or more, with high purity holds the potential to unlock experiments that would otherwise be unfeasible. Furthermore, it is expected to reduce the time required for experiments at FRIB, thereby maximizing scientific output. The research and development activities performed as part of this project bolstered essential competencies at FRIB in beam physics and ion source technologies, provided valuable training opportunities for junior scientists.

43 PARTICLE ACCELERATORS↗
DOE OSTI2024

Electron beam emittance at operational intensity in fourth-generation synchrotron light sources

For synchrotron light sources, the brightness of user X-ray beams is primarily determined by the electron beam emittance and energy spread at operational intensity. A common feature of fourth-generation synchrotrons is the short length of electron bunches combined with a very small transverse beam size. Consequently, the particle density is much higher than in machines of previous generations, leading to strong collective effects that significantly increase the emittance and limit the achievable brightness at operational beam intensity. In this article, we summarize our studies of the emittance scaled with the beam energy and intensity, taking into account the effects of intrabeam scattering, beam-impedance interaction, and bunch lengthening provided by higher-harmonic RF systems, to identify optimal combinations of machine and beam parameters.

43 PARTICLE ACCELERATORS↗
DOE OSTI2024

Large reductions in Permian Basin methane intensity shown in multi-year comparison of aerially-visible methane emissions

Spanning the US states of Texas and New Mexico, the Permian Basin has been a hotspot of methane emissions from oil and natural gas activity 1–4, although studies disagree over the magnitude of these emissions. The most comprehensive measurement campaigns published were conducted in 2019 1–5 .There have been large changes in the energy industry since then, including in the prices of oil and gas, both state and federal regulatory environments, investor and activist pressure over methane emissions, and the adoption of new technologies and policies by energy operators. Understanding how any or all of these might influence methane emissions is important for policy makers, oil and gas operators, and other stakeholders. We characterize the time evolution of Permian Basin methane emissions using a series of comprehensive aerial surveys conducted every year from 2020-2023 and compare them to the 2019 results cited above. To maintain comparability, all the data sets are from surveys using Insight M point source methane sensing technology. The scope of these surveys expanded over time: from 33-46% of wells, oil production, and gas production in 2020 to 60-65% in 2021, to 84% of wells and over 90% of both oil and gas production in 2023. These surveys by Insight M also include hundreds of gas processing plants and compressor stations as well as 1000s of km of gathering and transmission pipelines. Considering only the aerially detected portion of emissions (typically the majority of the total in such surveys 4), we find reductions of more than 70% in methane emissions intensity compared to the 2019 New Mexico-only Insight M survey, with variation depending on the year 3,4. Notably, although sources below 100 kg/hr contributed less than 10% of aerially measured emissions the 2019 New Mexico survey 3, these smaller sources constitute a larger proportion of total aerially measured emissions (although not the majority) in 2020-2023. Production facilities and gathering pipelines are responsible for the larges shares of total emissions, followed by compressor stations and gas processing plants. Permian methane emissions were also measured in a comprehensive 2019 Permian-wide survey by the Carbon Mapper team 2. That analysis led to a lower total emissions estimate at the time 4. These new Insight M-based emission rates are still roughly 30-70% lower than the aerially measured portion of the 2019 Carbon Mapper-based estimates 4. Further work is needed to harmonize these surveys in space and time to create the most intercomparable numbers possible 5. Additional analysis is needed to compare our findings to the more spatially constrained 2020, 2021, and 2023 Carbon Mapper surveys in the Permian 4,6. The evidence is strong from these two survey teams that emissions intensity has declined significantly since 2019. Reasons for this trend are currently unclear but point to possible success of emissions control programs. Future work investigating frequency, source, and operator-specific intensities could provide insights into the causes of this promising trend.

methane, oil and gas, data science, remote sensing↗
DOE OSTI2025

Development of a High-Intensity Heat Flux Gauge and Characterization Facility (Final Report)

Sandia National Laboratories (SNL) and Hukseflux Thermal Sensors (HTS) collaborated to advance the design and calibration of high-intensity heat flux gauges capable of measuring 2500 kW/m². An industry trade study was first conducted and highlighted the need for enhanced gauge designs and calibration methodology & services suited for high-intensities and broadband flux. We then developed, tested, and evaluated three prototype gauge designs along with four distinct coating types, each designed to extend the measurable flux range of existing HTS products to higher intensity levels. Following a down selection process, the project team refined the focus to a final product design, incorporating updated features to enhance its robustness during high flux exposure.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

Positron Emission Intensity in the Decay of 86 gY for Use in Dosimetry Studies

The β + -emitting radionuclide 86 gY (t 1/2 = 14.7 h) forms a matched-pair with the β – -emitting therapeutic radionuclide 90Y (t 1/2 = 2.7 d) for theranostic application in medicine. This approach demands a precise knowledge of the positron emission probability of the PET nuclide which was until recently rather uncertain for 86 gY. In this work, an 86 gY source of high radionuclidic purity was prepared and a direct measurement of the positron emission intensity per 100 decay of the parent (hereafter “positron emission intensity”) was performed using high-resolution HPGe detector γ-ray spectroscopy. The electron capture intensity was also determined as an additional check by measuring the K α and K β X-rays of energies 14.1 and 15.8 keV, respectively, using a low energy HPGe detector. From those measurements, normalized values of 27.2 ± 2.0% for β + -emission and 72.8 ± 2.0% for EC were obtained. These results are in excellent agreement with values recently reported in the literature based on a detailed decay scheme study.

61 RADIATION PROTECTION AND DOSIMETRY↗
DOE OSTI2020

Remote Detection of Uranium Using Self-Focusing Intense Femtosecond Laser Pulses

Optical measurement techniques can address certain important challenges associated with nuclear safety and security. Detection of uranium over long distances presents one such challenge that is difficult to realize with traditional ionizing radiation detection, but may benefit from the use of techniques based on intense femtosecond laser pulses. When a high-power laser pulse propagates in air, it experiences collapse and confinement into filaments over an extended distance even without external focusing. In our experiments, we varied the initial pulse chirp to optimize the emission signal from the laser-produced uranium plasma at an extended distance. While the ablation efficiency of filaments formed by self-focusing is known to be significantly lower when compared to filaments produced by external focusing, we show that filaments formed by self-focusing can still generate luminous spectroscopic signatures of uranium detectable within seconds over a 10-m range. The intensity of uranium emission varies periodically with laser chirp, which is attributed to the interplay among self-focusing, defocusing, and multi-filament fragmentation along the beam propagation axis. Grouping of multi-filaments incident on target is found to be correlated with the uranium emission intensity. The results show promise towards long-range detection, advancing the diagnostics and analytical capabilities in ultrafast laser-based spectroscopy of high-Z elements.

42 ENGINEERING↗
DOE OSTI2023

Detection of Cosmological 21 cm Emission with the Canadian Hydrogen Intensity Mapping Experiment

We present a detection of 21 cm emission from large-scale structure (LSS) between redshift 0.78 and 1.43 made with the Canadian Hydrogen Intensity Mapping Experiment. Radio observations acquired over 102 nights are used to construct maps that are foreground filtered and stacked on the angular and spectral locations of luminous red galaxies (LRGs), emission-line galaxies (ELGs), and quasars (QSOs) from the eBOSS clustering catalogs. We find decisive evidence for a detection when stacking on all three tracers of LSS, with the logarithm of the Bayes factor equal to 18.9 (LRG), 10.8 (ELG), and 56.3 (QSO). An alternative frequentist interpretation, based on the likelihood ratio test, yields a detection significance of 7.1σ (LRG), 5.7σ (ELG), and 11.1σ (QSO). These are the first 21 cm intensity mapping measurements made with an interferometer. We constrain the effective clustering amplitude of neutral hydrogen (H I ), defined as ${{ \mathcal A }}_{{\rm{H}}\,{\rm\small{I}}}\equiv {10}^{3}\,{{\rm{\Omega }}}_{{\rm{H}}\,{\rm\small{I}}}\left({b}_{{\rm{H}}\,{\rm\small{I}}}+\langle \,f{\mu }^{2}\rangle \right)$, where Ω H I is the cosmic abundance of H I , b H I is the linear bias of H I , and $\langle$fμ 2 $\rangle$ = 0.552 encodes the effect of redshift-space distortions at linear order. We find ${{ \mathcal A }}_{{\rm{H}}\,{\rm\small{I}}}={1.51}_{-0.97}^{+3.60}$ for LRGs (z = 0.84), ${{ \mathcal A }}_{{\rm{H}}\,{\rm\small{I}}}={6.76}_{-3.79}^{+9.04}$ for ELGs (z = 0.96), and ${{ \mathcal A }}_{{\rm{H}}\,{\rm\small{I}}}={1.68}_{-0.67}^{+1.10}$ for QSOs (z = 1.20), with constraints limited by modeling uncertainties at nonlinear scales. We are also sensitive to bias in the spectroscopic redshifts of each tracer, and we find a nonzero bias Δ v = - 66 ± 20 km s -1 for the QSOs. We split the QSO catalog into three redshift bins and have a decisive detection in each, with the upper bin at z = 1.30 producing the highest-redshift 21 cm intensity mapping measurement thus far.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

Seasonal controls on isolated convective storm drafts, precipitation intensity, and life cycle as observed during GoAmazon2014/5

Abstract. Isolated deep convective cloud life cycle and seasonal changes in storm properties are observed for daytime events during the US Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Green Ocean Amazon Experiment (GoAmazon2014/5) campaign to understand controls on storm behavior. Storm life cycles are documented using surveillance radar from initiation through maturity and dissipation. Vertical air velocity estimates are obtained from radar wind profiler overpasses, with the storm environment informed by radiosondes. Dry-season storm conditions favored reduced morning shallow cloud coverage and larger low-level convective available potential energy (CAPE) than wet-season counterparts. The typical dry-season storm reached its peak intensity and size earlier in its life cycle compared with wet-season cells. These cells exhibited updrafts in core precipitation regions (Z>35 dBZ) to above the melting level as well as persistent downdrafts aloft within precipitation adjacent to their cores. Moreover, dry-season cells recorded more intense updrafts to earlier life cycle stages as well as a higher incidence of strong updrafts (i.e., >5 m s−1) at low levels. In contrast, wet-season storms were longer-lived and featured a higher incidence of moderate (i.e., 2–5 m s−1) updrafts aloft. These storms also favored a shift in their most intense properties to later life cycle stages. Strong downdrafts were less frequent within wet-season cells aloft, indicating a potential systematic difference in draft behaviors, as linked to graupel loading and other factors between the seasons. Results from a stochastic parcel model suggest that dry-season cells may expect stronger updrafts at low levels because of larger low-level CAPE in the dry season. Wet-season cells anticipate strong updrafts aloft because of larger free-tropospheric relative humidity and reduced entrainment-driven dilution. Enhanced dry-season downdrafts are partially attributed to increased evaporation, dry-air entrainment mixing, and negative buoyancy in regions adjacent to sampled dry-season cores.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Flux Sensor Measurement and Calibration Requirements for High-Intensity Heat Flux Applications: A Trade Study

Stakeholders of CSP and non-CSP high-intensity broadband flux measurements were surveyed and interviewed to obtain flux sensor design and calibration requirements. Existing sensor technologies and existing calibration facilities were then compared against this standard. Stakeholders require a flux sensor designed for >5,000 kW/m2 flux measurements, >1,000 life cycles, <500 ms response time, >60-minute exposure at maximum flux, and <5% measurement uncertainty. Stakeholders also require a sensor with minimal cost, short procurement lead time, and a high-intensity broadband flux calibration. Commercial CSP stakeholders primarily rely on infrared (IR) temperature measurements of receiver equipment to control CSP plant process operation, whereas CSP research and development (R&D) and non-CSP stakeholders rely on accurate flux gauge measurements for a variety of applications. It was determined that existing flux sensor technologies and calibration facilities do not comprehensively meet stakeholder needs. This study suggests a more robust circular foil gauge with a high-intensity solar flux calibration comprehensively meets stakeholder flux measurement needs. Improved circular foil gauge designs and an improved flux sensor calibration facility are discussed.

McLaughlin, Luke (ORCID:0000000303711310)↗
DOE OSTI2023

High-resolution (30-m) urban land cover projections for Los Angeles California Urban Area: 2010 to 2100 under SSP3 and SSP5 [Updated simulations based on population-driven urban intensity transitions]

These data (v3) are updated from previous versions (1 and 2) in that they include consider the effects of population on transitions in urban land intensity. This leads to more reasonable differences in urban land projections under variant SSPs. For the present dataset, both SSP3 and SSP5 are provided. These data represent simulations of future land use and land cover (LULCC) for Los Angeles urban area (U.S. Census Bureau defined area) as raster tiff images at a 30-m pixel resolution and at decadal time steps from 2010 to 2100. LULCC classes in this product follow the National Land Cover Dataset (NLCD) classification. NLCD 21-24 correspond to open developed, low developed, medium developed, and high developed urban land classes, respectively. Only urban land cover classes (NLCD class 21, 22, 23, and 24) are dynamic over time; however, all NLCD classes are included in the final product. Therefore, NLCD classes that do not convert to an urban class will be similar to year 2000. The products were developed using a hybridized statistical and cellular automata approach. Linear mixed models (LMMs) were used to estimate future urban land budgets based on 1-km urban land fraction projections from Gao and Pesaresi (2021), whereas separate generalized linear mixed models (GLMMs) were used to estimate shifts in urban land intensities based on retrospective shifts in NLCD urban class intensities over a 20- year period. Based on urban land allocations from the statistical models, a cellular-automata and downscaling routine was used to simulate dynamic urban land expansion at a 30-m resolution based on suitability criteria. Scenarios of future urban landcover change projections include variant solutions for the Shared Socioeconomic Pathway 5 (SSP5) and SSP 3 based on different population assumptions, different land use intensification assumptions, variable land zoning constraints, and iterative adjustments to correct for over allocation of urban expansion across decadal time periods from 2010 to 2100. This results in 320 raster products.

Land↗
NASA NTRS1972

Anisotropies in the interplanetary intensity of solar protons E sub p 0.3 MeV

From the data on solar protons with energy 0.3 MeV obtained by Explorer 35 since July 1967, ten events were selected for the study of intensity vs time and of angular distributions of intensity in interplanetary space near the earth. The bases of selection were that the events be of adequate intensity for statistically satisfactory study and that they be attributable to a single solar flare so that their time histories were not complicated by overlapping emissions of particles. The principal findings for these events are presented.

Innanen, W. G.↗
NASA NTRS1972

Relative intensity calculations for nitrous oxide.

A tabulation of calculated rotational line intensities, relative to the integrated intensity of a vibration-rotation band, is given for Sigma-Sigma, Pi-Sigma, Sigma-Pi, Pi-Pi, and Delta-Pi transitions of nitrous oxide. These calculations were made for temperatures of 250 K and 300 K. A summary of band-intensity measurements is also presented.

Young, L. D. G.↗
NASA NTRS1970

Hazards from High Intensity Lamps and Arcs

The principal occupational health problem generally associated with high intensity arc lamps results from exposure of the eye and skin to ultraviolet radiation. Occasionally, the chorioretinal burns are of concern. The eye is generally more susceptible than the skin to injury from high intensity optical radiation sources whether ultraviolet, visible or infrared. Recent developments in technology have shown that some high intensity optical radiation sources which have output parameters greatly different from those encountered in the natural environment present a serious chorioretinal burn hazard.

Sliney, D. H.↗
NASA NTRS1973

Odor intensity and characterization studies of exhaust from a turbojet engine combustor

Sensory odor tests of the exhaust from a turbojet combustor operating at simulated idle conditions were made by a human panel sniffing diluted exhaust gas. Simultaneously, samples of undiluted exhaust gas were collected on adsorbent substrates, subsequently removed by solvent flushing, and analyzed chemically by liquid chromatographic methods. The concentrations of the principal malodorous species, the aromatic (unburned fuel-related) and the oxygenated (partially burned fuel) fractions, as determined chromatographically, correlated well with the intensity of the odor as determined by sniffing. Odor intensity increased as combustion efficiency decreased. Combustor modifications which increased combustion efficiency decreased odor intensity.

Butze, H. F.↗
NASA NTRS1974

Shear-stress intensity factors for elastic sheets with cover plates

Shear stress intensity factors are calculated for three problems concerning inextensible cover plates either bonded to or embedded in an elastic sheet which is under uniaxial tension. The stress intensity factors are small when the ratio of sheet thickness to cover plate length is small and, as the ratio increase, rapidly approach their asymptotic values for infinite sheet thickness. In the problem of the embedded cover plate, the stress intensity factor also depends on the Poisson's ratio of the sheet material. The dependence on Poisson's ratio, however, is significant only when the ratio of sheet thickness to cover plate length is small. Some possible implications of the present results for debonding of reinforced sheets under cyclic loading are briefly discussed.

Fichter, W. B.↗
NASA NTRS1973

Odor intensity and characterization studies of exhaust from a turbojet engine combustor

Sensory odor tests of the exhaust from a turbojet combustor operating at simulated idle conditions were made by a human panel sniffing diluted exhaust gas. Simultaneously, samples of undiluted exhaust gas were collected on adsorbent substrates, subsequently removed by solvent flushing, and analyzed chemically by liquid chromatographic methods. The concentrations of the principal malodorous species, the aromatic (unburned fuel-related) and the oxygenated (partially burned fuel) fractions, as determined chromatographically, correlated well with the intensity of the odor as determined by sniffing. Odor intensity increased as combustion efficiency decreased. Combustor modifications which increased combustion efficiency decreased odor intensity.

Butze, H. F.↗
NASA NTRS1974

Predicted intensities of cosmic-ray-produced gamma-ray lines

The relative intensities of nuclear gamma-ray lines produced by inelastic collisions of low-energy cosmic ray nuclei with interstellar hydrogen have been calculated using assumed interstellar spectra which are power laws in kinetic energy. The intensity of the line at 511 keV produced by the annihilation of positrons emitted by radioactive nuclei resulting from similar collisions was also calculated. The 478 keV gamma-ray due to inelastic scattering of Li-7 is more intense than the positron line for spectral indicies Li-7 assuming that presently accepted cosmic ray abundances apply at low energies.

Rygg, T. A.↗
NASA NTRS1975

Stress analysis and stress intensity factors for finite geometry solids containing rectangular surface cracks

The line method of analysis is applied to the Navier-Cauchy equations of elastic equilibrium to calculate the displacement field in a finite geometry bar containing a variable depth rectangular surface crack under extensionally applied uniform loading. The application of this method to these equations leads to coupled sets of simultaneous ordinary differential equations whose solutions are obtained along sets of lines in a discretized region. Using the obtained displacement field, normal stresses and the stress intensity factor variation along the crack periphery are calculated for different crack depth to bar thickness ratios. Crack opening displacements and stress intensity factors are also obtained for a through-thickness, center cracked bar with variable thickness. The reported results show a considerable potential for using this method in calculating stress intensity factors for commonly encountered surface crack geometries in finite solids.

Gyekenyesi, J. P.↗