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DOE OSTI2020

Quantifying long-term seasonal and regional impacts of North American fire activity on continental boundary layer aerosols and cloud condensation nuclei

An intimate knowledge of aerosol transport is essential in reducing the uncertainty of the impacts of aerosols on cloud development. Datasets from the U. S. Department of Energy (DOE) Atmospheric Radiation Measurement platform in the Southern Great Plains region (ARM-SGP) and the NASA Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2) showed seasonal increases in aerosol loading and total carbon concentration during the spring and summer months (2008-2016) which was attributed to fire activity and smoke transport within North America. The monthly mean MERRA-2 surface carbonaceous aerosol mass concentration and ARM-SGP total carbon products were strongly correlated (R=0.82, p<0.01) along with a moderate correlation with the ARM-SGP cloud condensation nuclei (N CCN ) product (0.5, p~0.1). The monthly mean ARM-SGP total carbon and N CCN products were strongly correlated (0.7, p~0.01). An additional product denoting fire number and coverage taken from the National Interagency Fire Center (NIFC) showed a moderate correlation with the MERRA-2 carbonaceous product (0.45, p<0.01) during the 1981-2016 warm season months (March-September). With respect to meteorological conditions, the correlation between the NIFC fire product and MERRA-2 850 hPa isobaric height anomalies was lower (0.26, p~0.13) due to the variability in the frequency, intensity, and number of fires in North America. An observed increase in the isobaric height anomaly during the past decade may lead to frequent synoptic ridging and drier conditions with more fires, thereby potentially impacting cloud/precipitation processes and decreasing air quality.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2020

Probing Axial Symmetry Breaking in the Galaxy with Gaia Data Release 2

We study a set of solar neighborhood ($d < 3$ kpc) stars from Gaia Data Release 2 to determine azimuthal star count differences, i.e., left and right of the line from the Galactic center through the sun - and compare these differences north and south. In this companion paper to Gardner et al. (2020), we delineate our procedures to remove false asymmetries from sampling effects, incompleteness, and/or interloper populations, as this is crucial to tests of axisymmetry. Particularly, we have taken care to make appropriate selections of magnitude, color, in-plane Galactocentric radius and Galactic $|b|$ and $|z|$. We find that requiring parallax determinations of high precision induces sampling biases, so that we eschew such requirements and exclude, e.g., regions around the lines of sight to the Magellanic clouds, along with their mirror-image lines of sight, to ensure well-matched data sets. After making conservative cuts, we demonstrate the existence of azimuthal asymmetries, and find differences in those, north and south. These asymmetries give key insights into the nature and origins of the perturbations on Galactic matter, allowing us to assess the relative influence of the Magellanic Clouds (LMC & SMC), the Galactic bar, and other masses on the Galactic mass distribution, as described in Gardner et al. (2020). The asymmetry's radial dependence reveals variations that we attribute to the Galactic bar, and it changes sign at a radius of $(0.95 \pm 0.03) R_0$, with $R_0$ the Sun-Galactic-Center (GC) distance, to give us the first direct assessment of the outer Lindblad resonant radius.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2025

Measurement report: A comparative analysis of an intensive incursion of fluorescing African dust particles over Puerto Rico and another over Spain

Measurements during episodes of African dust, made with two wideband integrated bioaerosol spectrometers (WIBSs), one on the northeastern coast of Puerto Rico and the other in the city of León, Spain, show unmistakable, bioaerosol-like fluorescing aerosol particles (FAPs) that can be associated with these dust episodes. The Puerto Rico event occurred during a major incursion of African dust during June 2020. The León event occurred in the late winter and spring of 2022, when widespread, elevated layers of dust inundated the Iberian Peninsula. Satellite and back-trajectory analyses confirm that dust from northern Africa was the source of the particles during both events. The WIBSs measure the size of individual particles in the range from 0.5 to 30 µm, derive a shape factor, and classify seven types of fluorescence from the FAPs. In general, it is not possible to directly determine the specific biological identity from fluorescence signatures; however, measurements of these types of bioaerosols in laboratory studies allow us to compare ambient fluorescence patterns with whole microbial cells measured under controlled conditions. Here we introduce some new metrics that offer a more quantitative approach for comparing FAP characteristics derived from particles measured under different environmental conditions. The analysis highlights the similarities and differences at the two locations and reveals differences that can be attributed to the age and history of the dust plumes, e.g., the amount of time that the air masses were in the mixed layer and the frequency of precipitation along the air mass trajectory.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2003

Numerical Simulations of the Steady and Unsteady Aerodynamic Characteristics of a Circulation Control Wing Airfoil

The aerodynamic characteristics of a Circulation Control Wing (CCW) airfoil have been numerically investigated, and comparisons with experimental data have been made. The configuration chosen was a supercritical airfoil with a 30 degree dual-radius CCW flap. Steady and pulsed jet calculations were performed. It was found that the use of steady jets, even at very small mass flow rates, yielded a lift coefficient that is comparable or superior to conventional high-lift systems. The attached flow over the flap also gave rise to lower drag coefficients, and high L/D ratios. Pulsed jets with a 50% duty cycle were also studied. It was found that they were effective in generating lift at lower reduced mass flow rates compared to a steady jet, provided the pulse frequency was sufficiently high. This benefit was attributable to the fact that the momentum coefficient of the pulsed jet, during the portions of the cycle when the jet was on, was typically twice as much as that of a steady jet.

Liu, Yi↗

NASA NTRS2004

On the Cause of Eastern Equatorial Pacific Ocean T-S Variations Associated with El Nino

The nature of observed variations in temperature-salinity (T-S) relationship between El Nino and non-El Nino years in the pycnocline of the eastern equatorial Pacific Ocean (NINO3 region, 5(deg)S-5(deg)N, 150(deg)W-90(deg)W) is investigated using an ocean general circulation model. The origin of the subject water mass is identified using the adjoint of a simulated passive tracer. The higher salinity during El Nino is attributed to larger convergence of saltier water from the Southern Hemisphere and smaller convergence of fresher water from the Northern Hemisphere.

interannual variability↗

NASA NTRS2022

Thermospheric Neutral Density Variation During the “SpaceX” Storm: Implications From Physics-Based Whole Geospace Modeling

The Starlink satellites launched on 3 February 2022 were lost before they fully arrived in their designated orbits. The loss was attributed to two moderate geomagnetic storms that occurred consecutively on February 3-4. We investigate the thermospheric neutral mass density variation during these storms with the Multiscale Atmosphere-Geospace Environment (MAGE) model, a first-principles, fully coupled geospace model. Simulated neutral density enhancements are validated by Swarm satellite measurements at the altitude of 400-500 km. Comparison with standalone TIEGCM and empirical NRLMSIS 2.0 and DTM-2012 models suggests better performance by MAGE in predicting the maximum density enhancement and resolving the gradual recovery process. Along the Starlink satellite orbit in the middle thermosphere (∼ 200 km altitude), MAGE predicts up to 150% density enhancement near the second storm peak while standalone TIEGCM, NRLMSIS 2.0 and DTM-2012 suggest only ∼ 50% increase. MAGE also suggests altitudinal, longitudinal, and latitudinal variability of storm-time percentage density enhancement due to height dependent Joule heating deposition per unit mass, thermospheric circulation changes, and travelling atmospheric disturbances. This study demonstrates that a moderate storm can cause substantial density enhancement in the middle thermosphere. Thermospheric mass density strongly depends on the strength, timing, and location of high-latitude energy input, which cannot be fully reproduced with empirical models. A physics-based, fully coupled geospace model that can accurately resolve the high-latitude energy input and its variability is critical to modeling the dynamic response of thermospheric neutral density during storm time.

Starlink↗

NASA NTRS1983

Do all barium stars have a white dwarf companion?

International Ultraviolet Explorer short-wavelength, low-dispersion spectra were analyzed for four barium, two mild barium, and one R-type carbon star in order to test the hypothesis that the barium and related giants are produced by mass transfer from a companion now present as a white dwarf. An earlier tentative identification of a white dwarf companion to the mild barium star Zeta Cyg is confirmed. For the other stars, no ultraviolet excess attributable to a white dwarf is seen. Limits are set on the bolometric magnitude and age of a possible white dwarf companion. Since the barium stars do not have obvious progenitors among main-sequence and subgiant stars, mass transfer must be presumed to occur when the mass-gaining star is already on the giant branch. This restriction, and the white dwarf's minimum age, which is greater than 8 x 10 to the 8th yr, determined for several stars, effectively eliminates the hypothesis that mass transfer from an asymptotic giant branch star creates a barium star. Speculations are presented on alternative methods of producing a barium star in a binary system.

Dominy, J. F.↗

NASA NTRS1989

Parametric Cost Analysis: A Design Function

Parametric cost analysis uses equations to map measurable system attributes into cost. The measures of the system attributes are called metrics. The equations are called cost estimating relationships (CER's), and are obtained by the analysis of cost and technical metric data of products analogous to those to be estimated. Examples of system metrics include mass, power, failure_rate, mean_time_to_repair, energy _consumed, payload_to_orbit, pointing_accuracy, manufacturing_complexity, number_of_fasteners, and percent_of_electronics_weight. The basic assumption is that a measurable relationship exists between system attributes and the cost of the system. If a function exists, the attributes are cost drivers. Candidates for metrics include system requirement metrics and engineering process metrics. Requirements are constraints on the engineering process. From optimization theory we know that any active constraint generates cost by not permitting full optimization of the objective. Thus, requirements are cost drivers. Engineering processes reflect a projection of the requirements onto the corporate culture, engineering technology, and system technology. Engineering processes are an indirect measure of the requirements and, hence, are cost drivers.

Dean, Edwin B.↗

NASA NTRSDate not supplied

Low-Temperature Formation of Carbonaceous Grains from PAHs

Astronomical observations have detected interstellar carbon in the form of polycyclic aromatic hydrocarbons(PAHs) as well as carbonaceous dust, confirming its presence in both gaseous and solid phases. The goal of this study is to experimentally investigate low-temperature chemical pathways between these two phases in order to better understand the evolution of cosmic carbon. Cosmic dust analogs are produced in the supersonic expansion of an argon jet seeded with aromatic molecules: benzene, naphthalene, anthracene, phenanthrene, and pyrene. These are prototype aromatic molecules of compact and non compact structure, and are used to evaluate the effect of precursor structure on the molecular complexity of the resulting grains. The seeded jet is exposed to an electrical discharge and the carbonaceous grains are collected and probed ex situ via laser desorption mass spectrometry. Mass spectra reveal a rich molecular diversity within the grains, including fragments of the parent molecule but also growth into larger complex organic molecules (COMs). In all experiments, the largest number of products is found in the m/z range 200-250, and C16H10 (attributed to pyrene and/or its isomers) is found to be a dominant product, pointing at the formation of this stable PAH as a preferential route in the growth to larger PAHs. Comparison to mass spectra from the Murchison meteorite reveals a similar dominance of compounds related toC16H10 at m/z = 202. Evidence of the methyl addition-cyclization mechanism in the anthracene experiment is reported. PAH structure is found to impact the dust production yield, as seen by the greater yield for the anthracene compared to the phenanthrene experiment. PAH growth at low temperatures via barrierless routes involving the addition of alkyl- and phenyl-type radicals is suggested as a viable pathway to COMs. These results suggest that PAH growth and dust formation from PAHs are feasible at low temperatures in photon-dominated regions and circumstellar envelopes.

L Gavilan↗

DOE OSTI2020

The Significance of Environmental Attributes as Indicators of the Life Cycle Environmental Impacts of Packaging and Food Service Ware

The environmental impacts of packaging and food service ware (FSW) are increasingly the subject of government policy, public discourse, and industry commitments. While some consideration is given to reducing the impacts of packaging across its entire life cycle, most of the focus is on packaging waste or feedstock substitution. Efforts typically focus on specific packaging characteristics, or material attributes, commonly perceived to be environmentally preferable. This article summarizes an extensive meta-review of existing published literature that was performed to determine whether the material attributes recyclability, recycled content, compostability, and biobased, commonly considered to be environmentally beneficial, correlate with lower net environmental impacts across the full life cycle of the packaging and FSW. Seventy-one unique life cycle assessment (LCA) studies that quantify the environmental impacts throughout the entire life cycle of packaging and FSW were analyzed. These studies included over 5000 comparisons for 13 impact categories commonly analyzed in LCA studies. The results from the meta-review identified a number of instances where material attributes do not correlate with environmental benefits for packaging and FSW. Rather, other characteristics such as material choice or mass of the packaging/FSW products can have higher influence in determining life cycle impacts.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2020

Probing unintentional Fe impurity incorporation in MOCVD homoepitaxy GaN: Toward GaN vertical power devices

Unintentional impurity incorporation in GaN drift layers represents a challenging issue that can limit their potential performance in vertical power devices. In this paper, we focus on studying the origins of Fe impurity incorporation in metal-organic chemical vapor deposition (MOCVD) grown GaN materials. Acting as a compensator in n-type GaN drift layers, Fe impurities can reduce the electron mobility in GaN and limit the lowest controllable doping level. Two sources, the sample cleaning process and growth susceptor, were identified as the main mechanisms of Fe incorporation in the MOCVD GaN growth process. It was found that solvent cleaning of the wafer can introduce significant Fe contamination at the growth interface, which would slowly be incorporated into the GaN epilayer, thus causing background Fe impurity as high as 10 17 cm -3 level. Moreover, the Fe impurity in the coating material on the susceptor can introduce additional Fe impurity during the growth process. Our studies revealed that the Fe impurity level could be significantly suppressed by more than two orders when an alternative cleaning process was used and the susceptor surface was fully covered by substrates. Characterization of the Fe impurity concentrations was performed via secondary ion mass spectrometry. The trap level (E C - 0.57) eV from deep-level transient spectroscopy that had previously been attributed to Fe confirmed the carrier compensation effect from Fe. Room temperature Hall mobility as high as 1007 cm 2 /V s was achieved on the MOCVD grown low-Fe GaN. Results from this work will provide guidance for achieving high purity GaN toward high performance GaN vertical power devices.

42 ENGINEERING↗

DOE OSTI2025

Aerosol hygroscopicity over the South-East Atlantic Ocean during the biomass burning season – Part 2: Influence of sea salt and burning conditions on CCN hygroscopicity

Biomass burning (BB) significantly influences cloud condensation nuclei (CCN) concentrations over the southeastern Atlantic; however, aerosol hygroscopicity (κ) – a key factor for CCN activation – remains poorly constrained during the BB season. This study investigates κ variability using in situ measurements from Ascension Island during the 2016 and 2017 BB seasons. Results show substantial monthly variability, with κ values lowest in August and increasing through October. On average, κ was significantly higher in 2017 (∼ 0.55) than in 2016 (∼ 0.33), suggesting that the aerosols in 2017 were more hygroscopic and more easily activated as CCN. Sulfate and sea salt were the two dominant contributors to κ and the primary drivers of its interannual variability. During the 2017 BB season, sulfate – the major inorganic component – accounted for ∼ 34 % of the submicron aerosol mass, while sea salt, estimated via κ-closure analysis, contributed ∼ 17 %. The higher κ in 2017 was largely attributed to increased sea salt, likely driven by stronger marine winds. Approximately 67 % of sulfate was linked to BB emissions. Variations in BB combustion efficiency, modulated by regional meteorology, influenced sulfate fraction and thus κ values. Specifically, higher relative humidity and lower wind speeds over BB source regions in 2017 favored smoldering combustion, explaining the higher sulfate fraction. Overall, the observed interannual differences in aerosol hygroscopicity reflect the combined impacts of BB combustion characteristics and sea salt emissions, underscoring the critical roles of both BB and marine aerosol sources in regulating aerosol-cloud interactions over the southeastern Atlantic.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1983

Discovery of 9.3 s X-ray pulsations from 2S 1553-542 and a determination of the orbit

X-ray pulsations with a period of 9.3 s from the transient galactic X-ray source 2S 1553-542 were detected. The data were obtained with SAS 3 during the only known outburst of the source in 1975 June. Pulse-timing analyses of the data, which span an interval of 20 days, show that there were large changes in the pulse period that are readily attributable to binary orbital motion. The inferred orbital period is 30.6 + or - 2.2 days and the X-ray mass function is 5.0 + or - 2.1 solar masses. These orbital parameters, the transient nature of the source, and the probable lack of an early-type giant companion star, lead to the tentative conclusion that 2S 1553-542 is a Be/X-ray binary system.

Kelley, R. L.↗

NASA NTRS1985

Discovery of fast-moving oxygen filaments in Puppis A

A number of faint filaments in the Puppis A supernova remnant have been found to have spectra with strong oxygen lines, extremely weak Balmer lines, and radial velocities greater than 1500 km/s. These are very different from the bright filaments, which are nitrogen-rich and have velocities less than 300 km/s. The newly discovered filaments are spectroscopically similar to those found in young, oxygen-rich remnants, as typified by the fast-moving knots in Cas A. These Puppis A filaments are interpreted as knots of oxygen-rich supernova ejecta which remain relatively uncontaminated by interstellar material, despite the probable age of Puppis A of several thousand years. Spectra of the newly discovered filaments show, in addition to strong forbidden lines of O I, O II, and O III, permitted lines of O I: 7774, 8446 A. The permitted lines are attributed to recombination of O(+), and their strength relative to H is used to estimate that the O:H mass ratio is about 30.

Winkler, P. F.↗

NASA NTRS2016

Coordinated Isotopic and Mineral Characterization of Highly Fractionated 18O-Rich Silicates in the Queen Alexandra Range 99177 CR3 Chondrite

Carbonaceous chondrites contain a mixture of solar system condensates, pre-solar grains, and primitive organic matter. Each of these materials record conditions and processes in different regions of the solar nebula, on the meteorite parent body, and beyond the solar system. Oxygen isotopic studies of meteorite components can trace interactions of distinct oxygen isotopic reservoirs in the early solar system and secondary alteration processes. The O isotopic compositions of the earliest solar system condensates fall along a carbonaceous chondrite anhydrous mineral (CCAM) line of slope approximately 1 in a plot of delta 17O against delta 18O. This trend is attributed to mixing of material from 16O-poor and 16O-rich reservoirs. Secondary processing can induce mass-dependent fractionation of the O isotopes, shifting these compositions along a line of slope approximately 0.52. Substantial mass-dependent fractionation of O isotopes has been observed in secondary minerals in CAIs, calcite, and FUN inclusions. These fractionations were caused by significant thermal or aqueous alteration. We recently reported the identification of four silicate grains with extremely fractionated O isotopic ratios (delta 18O equals 37 - 55 per mille) in the minimally altered CR3 chondrite QUE 99177. TEM analysis of one grain indicates it is a nebular condensate that did not experience substantial alteration. The history of these grains is thus distinct from those of the aforementioned fractionated materials. To constrain the origin of the silicate grains, we conducted further Mg and Fe isotopic studies and TEM analyses of two grains.

Nguyen, A. N.↗

NASA NTRS2004

Phobos Ephemeris Improvement from Recent Spacecraft Observations

Despite 127 years of observations, there is still room for improvement in the ephemeris of the Martian satellite Phobos. Early in this history, Earth-based astrometric observations of Phobos and Deimos were used to estimate the mass and oblateness of Mars. As more data accumulated, it became clear that a secular acceleration in the longitude of Phobos was occurring, and this was attributed to tidal dissipation within Mars, yielding rough estimates of the tidal quality factor, or Q. At the epoch of the earliest spacecraft observations of Phobos, from Mariner 9 and the Viking Orbiters and Landers, the gravitational field of Mars, and resulting forces on Phobos, were still not particularly well known. Thus observations of natural and artificial satellite motions continued to contribute, each in their own way, to knowledge of the mass distribution within Mars. Improvements in tracking system accuracy, and the placement of satellites, like the 1996 Mars Global Surveyor and 2001 Mars Odyssey, in circular polar orbits has lead to dramatic improvements to knowledge of the Mars gravity field. The direct gravitational influence on Phobos is no longer expected to be a limiting factor in predicting its orbital motion. Despite that progress, a variety of observations of Phobos from recent orbiters and landers suggest that the best satellite ephemeris still has along-track orbit errors which are accumulating at a rate of 1.75 kilometers per year, with Phobos gaining on the predicted positions. These recent observations alone do not span sufficient time to separately resolve the positional error into changes in mean motion and changes in secular acceleration. However, combining them with earlier observations will allow improvements in both the mean motion and its first derivative. This latter parameter is particularly interesting, as it relates to tidal dissipation, and thus uniquely constrains the internal structure of Mars. The current best estimate of the secular acceleration rate of Mars implies a surprisingly low value for the tidal dissipation factor Q = (94 plus or minus 1). For the Earth, most tidal dissipation occurs within the oceans. The terrestrial mantle tidal Q is 280. An issue of interest is then: why, where, and how does Mars dissipate tidal energy so effectively.

Bills, B. G.↗

NASA NTRS2016

Center of Mass Estimation for a Spinning Spacecraft Using Doppler Shift of the GPS Carrier Frequency

A sequential filter is presented for estimating the center of mass (CM) of a spinning spacecraft using Doppler shift data from a set of onboard Global Positioning System (GPS) receivers. The advantage of the proposed method is that it is passive and can be run continuously in the background without using commanded thruster firings to excite spacecraft dynamical motion for observability. The NASA Magnetospheric Multiscale (MMS) mission is used as a test case for the CM estimator. The four MMS spacecraft carry star cameras for accurate attitude and spin rate estimation. The angle between the spacecraft nominal spin axis (for MMS this is the geometric body Z-axis) and the major principal axis of inertia is called the coning angle. The transverse components of the estimated rate provide a direct measure of the coning angle. The coning angle has been seen to shift slightly after every orbit and attitude maneuver. This change is attributed to a small asymmetry in the fuel distribution that changes with each burn. This paper shows a correlation between the apparent mass asymmetry deduced from the variations in the coning angle and the CM estimates made using the GPS Doppler data. The consistency between the changes in the coning angle and the CM provides validation of the proposed GPS Doppler method for estimation of the CM on spinning spacecraft.

Spacecraft↗

NASA NTRS2016

Center of Mass Estimation for a Spinning Spacecraft Using Doppler Shift of the GPS Carrier Frequency

Estimation↗