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At least 307 records · Page 17

Hyperspectral modeling for extracting aerosols from aircraft/satellite data

Sensitivity studies using the Airborne Visible/Infrared Imaging Spectrometer (AVIRIS) bands are currently under investigation. The objective of this research is to develop improved algorithms for the determination of aerosol type (e.g., presently described by S(sub 12). Preliminary computer calculations were made using LOWTRAN 7, which is the most advanced atmospheric code of the Air Force Geophysics Laboratory. LOWTRAN 7 permits the calculation of atmospheric transmission and absorption caused by aerosols and molecules along a non-homogeneous path for a variety of aerosol models. The calculations used the Navy Aerosol Model (NAM), which was constructed for the marine environment using a three component size distribution model. Calculations of the total transmittance (L(sub T)), the path radiance (L(sub P)), and the reflected radiance (L(sub r)) were made as a function of wavelength (lambda) from 0.4 to 2.4 microns for each of the 224 10 nm wide AVIRIS bands. These calculations were made for various types of atmospheres for the troposphere (0-2 km).

Hickman, G. Daniel↗

Signal Processing and Calibration of Continuous-Wave Focused CO2 Doppler Lidars for Atmospheric Backscatter Measurement

Two continuous-wave(CW)focused C02 Doppler lidars (9.1 and 10.6 micrometers) were developed for airborne in situ aerosol backscatter measurements. The complex path of reliably calibrating these systems, with different signal processors, for accurate derivation of atmospheric backscatter coefficients is documented. Lidar calibration for absolute backscatter measurement for both lidars is based on range response over the lidar sample volume, not solely at focus. Both lidars were calibrated with a new technique using well-characterized aerosols as radiometric standard targets and related to conventional hard-target calibration. A digital signal processor (DSP), a surface acoustic and spectrum analyzer and manually tuned spectrum analyzer signal analyzers were used. The DSP signals were analyzed with an innovative method of correcting for systematic noise fluctuation; the noise statistics exhibit the chi-square distribution predicted by theory. System parametric studies and detailed calibration improved the accuracy of conversion from the measured signal-to-noise ratio to absolute backscatter. The minimum backscatter sensitivity is approximately 3 x 10(exp -12)/m/sr at 9.1 micrometers and approximately 9 x 10(exp -12)/m/sr at 10.6 micrometers. Sample measurements are shown for a flight over the remote Pacific Ocean in 1990 as part of the NASA Global Backscatter Experiment (GLOBE) survey missions, the first time to our knowledge that 9.1-10.6 micrometer lidar intercomparisons were made. Measurements at 9.1 micrometers, a potential wavelength for space-based lidar remote-sensing applications, are to our knowledge the first based on the rare isotope C-12 O(2)-18 gas.

Rothermel, Jeffry↗

Role of the Quasi-Biennial Oscillation in the Transport of Aerosols from the Tropical Stratospheric Reservoir to Midlatitudes

The temporal evolution of the stratospheric aerosol distribution in the tropical stratospheric reservoir after the eruption of Mount Pinatubo was observed from 1992 to 1995 by the HALOE instrument on the UARS satellite. Since the spatial gradient of aerosol loading is large at the boundaries of the tropical stratospheric reservoir due to the volcanic aerosols, the effect of the meridional circulation on the distribution is seen clearly. The mechanism for dispersal of aerosol in the lower stratosphere from the tropics into midlatitudes strongly depends on the phase of the equatorial zonal wind. The time-latitude cross sections of the normalized distribution of aerosol on isentropic surfaces are used to observe the equatorial variation as well as change in meridional dispersal during the quasi-biennial period. Observed tropical stratospheric winds are used with a simple analytical dynamical model to examine transport processes of tracers from the tropics during several phases of the quasi-biennial oscillation (QBO) from 1992 to 1995. The Lagrangian meridional circulation in the tropics is consistent with the vertical and meridional velocities correlated with the QBO in the zonal wind. We find that vertical motion plays a crucial role in vertical and subsequent meridional transport. The pattern of meridional divergence derived from the vertical velocity is closely related to the observed HALOE aerosol distributions and their temporal development in the equatorial region. The westerly (easterly) shear phase of the QBO is associated with sinking (rising) motions at the equator and subsequent poleward (equatorward) transport in the lower stratosphere.

Choi, Wookap↗

Monte Carlo Simulation of Nanoparticle Encapsulation in Flames

Two critical challenges facing the application of flames for synthesis of nanopowder materials are: (1) overcoming formation of agglomerates and (2) ensuring that the highly reactive nanopowders that are synthesized in flames can be produced in such a manner that their purity is maintained during subsequent processing. Agglomerates are produced in flames because particle formation occurs in a high temperature and high number density environment. They are undesirable in most advanced applications of powders. For example, agglomerates have a deleterious effect on compaction density, leading to voids when nanopowders are consolidated. Efforts to avoid agglomeration in flames without substantially reducing particle number density and, consequently, production rate, have had limited success. Powder purity must also be maintained during subsequent handling of nanopowders and this poses a significant challenge for any synthesis route because nanopowders, particularly metals and non-oxide ceramic powders, are inherently reactive. Impurities acquired during handling of nanopowders have slowed the advancement of the nanostructured materials industry. One promising approach that has been proposed to address these problems is nano-encapsulation. In this approach, the core particles are encapsulated in a removable material while they are within the flame but before excessive agglomeration has occurred. Condensation can be very rapid so that core particles are trapped within the condensed material and agglomeration is limited. Nano-encapsulation also addresses the handling concerns for post-synthesis processing. Results have shown that when nano-encapsulated powders are exposed to atmosphere the core particles are protected from oxidation and/or hydrolysis. Thus, handling of the powders does not require extreme care. If, for example, at the time of consolidation the encapsulation material is removed by vacuum annealing, the resulting powder remains unagglomerated and free of impurities. In this work, we described a novel aerosol model that has been developed to simulate particle encapsulation in flames. The model will ultimately be coupled to a one-dimensional spherical flame code and compared to results from microgravity flame experiments.

Sun, Z.↗

Remote Sensing of Non-Aerosol (anomalous) Absorption in Cloud Free Atmosphere

The interaction of sunlight with atmospheric gases, aerosols and clouds is fundamental to the understanding of climate and its variation. Several studies questioned our understanding of atmospheric absorption of sunlight in cloudy or in cloud free atmospheres. Uncertainty in instruments' accuracy and in the analysis methods makes this problem difficult to resolve. Here we use several years of measurements of sky and sun spectral brightness by selected instruments of the Aerosol Robotic Network (AERONET), that have known and high measurement accuracy. The measurements taken in several locations around the world show that in the atmospheric windows 0.44, 0.06, 0.86 and 1.02 microns the only significant absorbers in cloud free atmosphere is aerosol and ozone. This conclusions is reached using a method developed to distinguish between absorption associated with the presence of aerosol and absorption that is not related to the presence of aerosol. Non-aerosol absorption, defined as spectrally independent or smoothly variable, was found to have an optical thickness smaller than 0.002 corresponding to absorption of sunlight less than 1W/sq m, or essentially zero.

Kaufman, Yoram J.↗

The NASA Micro-Pulse Lidar Network (MPLNET): Co-location of Lidars with AERONET

We present the formation of a global-ground based eye-safe lidar network, the NASA Micro-Pulse Lidar Network (MPLNET). The aim of MPLNET is to acquire long-term observations of aerosol and cloud vertical profiles at unique geographic sites within the NASA Aerosol Robotic Network (AERONET). Network growth follows a federated approach, pioneered by AERONET, wherein independent research groups may join MPLNET with their own instrument and site. MPLNET utilizes standard instrumentation and data processing algorithms for efficient network operations and direct comparison of data between each site. The micro-pulse lidar is eye-safe, compact, and commercially available, and most easily allows growth of the network without sacrificing standardized instrumentation gods. Red-time data products (next-day) are available, and include Level 1 daily lidar signal images from the surface to -2Okm, and Level 1.5 aerosol extinction provides at times co-incident with AERONET observations. Testing of our quality assured aerosol extinction products, Level 2, is near completion and data will soon be available. Level 3 products, continuous daylight aerosol extinction profiles, are under development and testing has begun. An overview of h4PL" will be presented. Successful methods of merging standardized lidar operations with AERONET will also be discussed, with the first 4 years of MPLNET results serving as an example.

Welton, Ellsworth J.↗

Characterization of Custom-Designed Charge-Coupled Devices for Applications to Gas and Aerosol Monitoring Sensorcraft Instrument

Custom-designed charge-coupled devices (CCD) for Gas and Aerosols Monitoring Sensorcraft instrument were developed. These custom-designed CCD devices are linear arrays with pixel format of 512x1 elements and pixel size of 10x200 sq m. These devices were characterized at NASA Langley Research Center to achieve a full well capacity as high as 6,000,000 e-. This met the aircraft flight mission requirements in terms of signal-to-noise performance and maximum dynamic range. Characterization and analysis of the electrical and optical properties of the CCDs were carried out at room temperature. This includes measurements of photon transfer curves, gain coefficient histograms, read noise, and spectral response. Test results obtained on these devices successfully demonstrated the objectives of the aircraft flight mission. In this paper, we describe the characterization results and also discuss their applications to future mission.

Refaat, Tamer F.↗

Estimating Random Errors Due to Shot Noise in Backscatter Lidar Observations

In this paper, we discuss the estimation of random errors due to shot noise in backscatter lidar observations that use either photomultiplier tube (PMT) or avalanche photodiode (APD) detectors. The statistical characteristics of photodetection are reviewed, and photon count distributions of solar background signals and laser backscatter signals are examined using airborne lidar observations at 532 nm using a photon-counting mode APD. Both distributions appear to be Poisson, indicating that the arrival at the photodetector of photons for these signals is a Poisson stochastic process. For Poisson-distributed signals, a proportional, one-to-one relationship is known to exist between the mean of a distribution and its variance. Although the multiplied photocurrent no longer follows a strict Poisson distribution in analog-mode APD and PMT detectors, the proportionality still exists between the mean and the variance of the multiplied photocurrent. We make use of this relationship by introducing the noise scale factor (NSF), which quantifies the constant of proportionality that exists between the root-mean-square of the random noise in a measurement and the square root of the mean signal. Using the NSF to estimate random errors in lidar measurements due to shot noise provides a significant advantage over the conventional error estimation techniques, in that with the NSF uncertainties can be reliably calculated from/for a single data sample. Methods for evaluating the NSF are presented. Algorithms to compute the NSF are developed for the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) lidar and tested using data from the Lidar In-space Technology Experiment (LITE). OCIS Codes:

Liu, Zhaoyan↗

Satellite Perspective of Aerosol Intercontinental Transport: From Qualitative Tracking to Quantitative Characterization

Evidence of aerosol intercontinental transport (ICT) is both widespread and compelling. Model simulations suggest that ICT could significantly affect regional air quality and climate, but the broad inter-model spread of results underscores a need of constraining model simulations with measurements. Satellites have inherent advantages over in situ measurements to characterize aerosol ICT, because of their spatial and temporal coverage. Significant progress in satellite remote sensing of aerosol properties during the Earth Observing System (EOS) era offers opportunity to increase quantitative characterization and estimates of aerosol ICT, beyond the capability of pre-EOS era satellites that could only qualitatively track aerosol plumes. EOS satellites also observe emission strengths and injection heights of some aerosols, aerosol precursors, and aerosol-related gases, which can help characterize aerosol ICT. After an overview of these advances, we review how the current generation of satellite measurements have been used to (1) characterize the evolution of aerosol plumes (e.g., both horizontal and vertical transport, and properties) on an episodic basis, (2) understand the seasonal and inter-annual variations of aerosol ICT and their control factors, (3) estimate the export and import fluxes of aerosols, and (4) evaluate and constrain model simulations. Substantial effort is needed to further explore an integrated approach using measurements from on-orbit satellites (e.g., A-Train synergy) for observational characterization and model constraint of aerosol intercontinental transport and to develop advanced sensors for future missions.

Yu, Hongbin↗

Multiangle Implementation of Atmospheric Correction (MAIAC):: Radiative Transfer Basis and Look-up Tables - 1

This paper describes a radiative transfer basis of the algorithm MAIAC which performs simultaneous retrievals of atmospheric aerosol and bidirectional surface reflectance from the Moderate Resolution Imaging Spectroradiometer (MODIS). The retrievals are based on an accurate semianalytical solution for the top-of-atmosphere reflectance expressed as an explicit function of three parameters of the Ross-Thick Li-Sparse model of surface bidirectional reflectance. This solution depends on certain functions of atmospheric properties and geometry which are precomputed in the look-up table (LUT). This paper further considers correction of the LUT functions for variations of surface pressure/height and of atmospheric water vapor, which is a common task in the operational remote sensing. It introduces a new analytical method for the water vapor correction of the multiple ]scattering path radiance. It also summarizes the few basic principles that provide a high efficiency and accuracy of the LUT ]based radiative transfer for the aerosol/surface retrievals and optimize the size of LUT. For example, the single-scattering path radiance is calculated analytically for a given surface pressure and atmospheric water vapor. The same is true for the direct surface-reflected radiance, which along with the single-scattering path radiance largely defines the angular dependence of measurements. For these calculations, the aerosol phase functions and kernels of the surface bidirectional reflectance model are precalculated at a high angular resolution. The other radiative transfer functions depend rather smoothly on angles because of multiple scattering and can be calculated at coarser angular resolution to reduce the LUT size. At the same time, this resolution should be high enough to use the nearest neighbor geometry angles to avoid costly three ]dimensional interpolation. The pressure correction is implemented via linear interpolation between two LUTs computed for the standard and reduced pressure levels. A linear mixture and a modified linear mixture methods are used to represent different aerosol types in the aerosol/surface retrievals from several base models of the fine and coarse aerosol fractions. In summary, the developed LUT algorithm allows fast high-accuracy simulations of the outgoing radiance with full variability of the atmospheric and surface bidirectional reflectance properties for the aerosol/surface remote sensing.

Lyapustin, Alexei↗

The GOddard SnoW Impurity Module (GOSWIM) for the NASA GEOS-5 Earth System Model: Preliminary Comparisons with Observations in Sapporo, Japan

The snow darkening module evaluating dust, black carbon, and organic carbon depositions on mass and albedo has been developed for the NASA Goddard Earth Observing System, Version 5 (GEOS-5) Earth System Model, as the GOddard SnoW Impurity Module (GOSWIM). GOSWIM consists of the snow albedo scheme from a previous study (Yasunari et al. 2011) with updates and a newly developed mass concentration scheme, using aerosol depositions from the chemical transport model (GOCART) in GEOS-5. Compared to observations at Sapporo, the numerical experiments, forced by observation-based meteorology and aerosol depositions from GOES-5, better simulated the seasonal migration of snow depth, albedos, and impurities of dust, BC, and OC in the snow surface. However, the magnitude of the impurities is underestimated, compared to the sporadic snow impurity measurements. Increasing the deposition rates of dust and BC could explain the differences on the snow darkening effect between observation and simulation. Ignoring BC deposition can possibly lead to an extension of snow cover duration in Sapporo for four days. Comparing the off-line GOSWIM and the GEOS-5 global simulations, we found that determining better local precipitation and deposition rates of the aerosols are key factors in generating better GOSWIM snow darkening simulation in NASA GEOS-5.

land surface processes↗

Improving Decision-Making Activities for Meningitis and Malaria

Public health professionals are increasingly concerned about the potential impact that climate variability and change can have on infectious disease. The International Research Institute for Climate and Society (IRI) is developing new products to increase the public health community's capacity to understand, use and demand the appropriate climate data and climate information to mitigate the public health impacts of climate on infectious disease, in particular meningitis and malaria. In this paper, we present the new and improved products that have been developed for: (i) estimating dust aerosol for forecasting risks of meningitis and (ii) for monitoring temperature and rainfall and integrating them into a vectorial capacity model for forecasting risks of malaria epidemics. We also present how the products have been integrated into a knowledge system (IRI Data Library Map Room, SERVIR) to support the use of climate and environmental information in climate-sensitive health decision-making.

parasitic diseases↗

Air Pollution Over the Ganges Basin and Northwest Bay of Bengal in the Early Postmonsoon Season Based on NASA MERRAero Data

The MERRA Aerosol Reanalysis (MERRAero) has been recently developed at NASA's Global Modeling Assimilation Office. This reanalysis is based on a version of the Goddard Earth Observing System-5 (GEOS-5) model radiatively coupled with Goddard Chemistry, Aerosol, Radiation, and Transport aerosols, and it includes assimilation of bias-corrected aerosol optical thickness (AOT) from the Moderate Resolution Imaging Spectroradiometer (MODIS) sensor on both Terra and Aqua satellites. In October over the period 2002-2009, MERRAero showed that AOT was lower over the east of the Ganges basin than over the northwest of the Ganges basin: this was despite the fact that the east of the Ganges basin should have produced higher anthropogenic aerosol emissions because of higher population density, increased industrial output, and transportation. This is evidence that higher aerosol emissions do not always correspond to higher AOT over the areas where the effects of meteorological factors on AOT dominate those of aerosol emissions. MODIS AOT assimilation was essential for correcting modeled AOT mainly over the northwest of the Ganges basin, where AOT increments were maximal. Over the east of the Ganges basin and northwest Bay of Bengal (BoB), AOT increments were low and MODIS AOT assimilation did not contribute significantly to modeled AOT. Our analysis showed that increasing AOT trends over northwest BoB (exceeding those over the east of the Ganges basin) were reproduced by GEOS-5, not because of MODIS AOT assimilation butmainly because of the model capability of reproducing meteorological factors contributing to AOT trends. Moreover, vertically integrated aerosol mass flux was sensitive to wind convergence causing aerosol accumulation over northwest BoB.

AOT↗

TPSAS-NF1676L-18834-DND

This presentation will give an overview of the 20-plus years of pulsed transmit laser development at NASA Langley Research Center (LaRC) to enable a coherent Doppler wind lidar to measure global winds from earth orbit. Our group at LaRC has been developing the pulsed laser and other coherent lidar technologies for the global wind mission since the late 1980s. The causal path followed has been from space mission requirements to coherent lidar requirements to component requirements to technology development and finally to ground and aircraft validation. We will describe the development and deployment of Doppler Aerosols Wind Lidar (DAWN) for airborne measurement of wind velocity and direction. The will also present the status of ongoing fully conductively-cooled 2-micron wind lidar transmitter for NASA 3-D winds mission.

Upendra N Singh↗

Remote sensing of tropospheric gases and aerosols with airborne DIAL system

The multipurpose airborne DIAL system developed at NASA Langley Research Center is characterized, and the published results of tropospheric O3, H2O, and aerosol-backscatter remote-sensing experiments performed in 1980 and 1981 are summarized. The system comprises two tunable dye lasers pumped by frequency-doubled Nd:YAG lasers, dielectric-coated steering optics, a 36-cm-diameter Cassegrain receiver telescope, gateable photomultiplier tubes, and a minicomputer data-processing unit for real-time calculation of gas concentrations and backscattering profiles. The transmitted energy of the 100-microsec-separated dye-laser pulses is 40, 80, or 50 mJ/pulse at around 300, 600, or 720-nm wavelength, respectively. Good agreement was found between DIAL-remote-sensed and in-situ H2O and O3 profiles of the lower troposphere and O3 profiles of the tropopause region, and the usefulness of DIAL backscattering measurements in the study of boundary-layer and tropospheric dynamics is demonstrated. The feasibility of DIAL sensing of power-plant or urban plume SO2, of urban-area (or rural-area column-content) NO2, and of temperature and H2O (simultaneously using a third laser) has been suggested by simulation studies.

Browell, E. V.↗

TPSAS-NF1676L-28149-DND

An Optimal Estimation (OE) inversion method has been developed to retrieve vertical profiles of aerosol size distributions, volume/surface concentrations, complex refractive indices, and single scattering albedos using the High Spectral Resolution Lidar (HSRL) and polarimeter measurements. By combining the active and passive remote sensing data, we can take advantages of the high vertical resolution of the lidar measurements and the high information content of the combined observations. There are three components to the new retrieval system: 1) simultaneous aerosol vertical profile retrieval using HSRL data, 2) standalone aerosol retrieval using Research Scanning Polarimeter (RSP), and 3) combined HSRL and RSP optimal estimation retrieval. For the LIDAR retrieval, we solve for number concentrations, mode fractions, aerosol size distributions, and real and imaginary part of refractive indices simultaneously. Based on this information, other parameters such as effective particle radius, surface and volume concentration, single scattering albedo can be derived. The combined HSRL-polarimeter algorithm will provide improved single scattering albedo and refractive index retrievals. The newly developed retrieval algorithm is very fast, and it provides an optimal estimation solution with associated error estimates. By solving for the aerosol vertical profiles using HSRL extinctions and backscattering coefficients from different layers, the new OE method can effectively reduce the impact of measurement noise on the retrieved aerosol microphysical properties. It also enables us to effectively combing HSRL and RSP data in the single OE retrieval system since the passive polarimeter instruments measure path-integrated intensity and polarizations. We have performed sensitivity studies using simulated data and applied the OE algorithms to NASA airborne field data measured by the HSRL-2 and the RSP instruments.

Xu Liu↗

Reducing Aerosol Forcing Uncertainty by Combining Models With Satellite and Within-The-Atmosphere Observations: A Three-Way Street

Aerosol forcing uncertainty represents the largest climate forcing uncertainty overall. Its magnitude has remained virtually undiminished over the past 20 years despite considerable advances in understanding most of the key contributing elements. Recent work has produced modest increases only in the confidence of the uncertainty estimate itself. This review summarizes the contributions toward reducing the uncertainty in the aerosol forcing of climate made by satellite observations, measurements taken within the atmosphere, as well as modeling and data assimilation. We adopt a more measurement-oriented perspective than most reviews of the subject in assessing the strengths and limitations of each; gaps and possible ways to fill them are considered. Currently planned programs supporting advanced, global-scale satellite and surface-based aerosol, cloud, and precursor gas observations, climate modeling, and intensive field campaigns aimed at characterizing the underlying physical and chemical processes involved, are all essential. But in addition, new efforts are needed: (a) to obtain systematic aircraft in situ measurements capturing the multi-variate probability distribution functions of particle optical, microphysical, and chemical properties (and associated uncertainty estimates), as well as co-variability with meteorology, for the major aerosol airmass types; (b) to conceive, develop, and implement a suborbital (aircraft plus surface-based) program aimed at systematically quantifying the cloud-scale microphysics, cloud optical properties, and cloud-related vertical velocities associated with aerosol-cloud interactions; and (c) to focus much more research on integrating the unique contributions of satellite observations, suborbital measurements, and modeling, to reduce the persistent uncertainty in aerosol climate forcing.

aerosol climate forcing↗

Progress Toward a Global, EOS-Era Aerosol Air Mass Type Climatology

The MISR and MODIS instruments aboard the NASA Earth Observing System's Terra Satellite have been collecting data containing information about the state of Earth's atmosphere and surface for over eleven years. Data from these instruments have been used to develop a global, monthly climatology of aerosol amount that is widely used as a constraint on climate models, including those used for the 2007 IPCC assessment report. The next frontier in assessing aerosol radiative forcing of climate is aerosol type, and in particular, the absorption properties of major aerosol air masses. This presentation will focus on the prospects for constraining aerosol type globally, and the steps we are taking to apply a combination of satellite and suborbital data to this challenge.

Kahn, Ralph A.↗